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1.
ZHANG Jinqiang XUAN Yuejian YAN Xiaolu LIU Mingyuan XIA Xiang ao PANG Li HENG Xiangdong TIAN Hongmin 《大气科学进展》2014,31(4):938-947
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R. D. Bojkov E. Kosmidis J. J. DeLuisi I. Petropavlovskikh V. E. Fioletov S. Godin C. Zerefos 《Meteorology and Atmospheric Physics》2002,79(3-4):127-158
Summary Umkehr observations taken during the 1957–2000 period at 15 stations located between 19 and 52° N have been reanalyzed using
a significantly improved algorithm-99, developed by DeLuisi and Petropavlovskikh et al. (2000a,b). The alg-99 utilizes new
latitudinal and seasonally dependent first guess ozone and temperature profiles, new vector radiative transfer code, complete
aerosol corrections, gravimetric corrections, and others. Before reprocessing, all total ozone values as well as the N-values
(radiance) readings were thoroughly re-evaluated. For the first time, shifts in the N-values were detected and provisionally
corrected. The re-evaluated Umkehr data set was validated against satellite and ground based measurements. The retrievals
with alg-99 show much closer agreement with the lidar and SAGE than with the alg-92. Although the latitudinal coverage is
limited, this Umkehr data set contains ∼ 44,000 profiles and represent the longest (∼ 40 years) coherent information on the
ozone behavior in the stratosphere of the Northern Hemisphere. The 14-months periods following the El-Chichon and the Mt.
Pinatubo eruptions were excluded from the analysis. Then the basic climatological characteristics of the vertical ozone distribution
in the 44–52° N and more southern locations are described. Some of these characteristics are not well known or impossible
to be determined from satellites or single stations. The absolute and relative variability reach their maximum during winter–spring
at altitudes below 24 km; the lower stratospheric layers in the middle latitudes contain ∼ 62% of the total ozone and contribute
∼ 57% to its total variability. The layer-5 (between ∼ 24 and 29 km) although containing 20% of the total ozone shows the
least fluctuations, no trend and contributes only ∼ 11% to the total ozone variability. Meridional cross-sections from 19
to 52° N of the vertical ozone distribution and its variability illustrate the changes, and show poleward-decreasing altitude
of the ozone maximum. The deduced trends above 33 km confirm a strong ozone decline since the mid-1970s of over 5% per decade
without significant seasonal differences. In the mid-latitude stations, the decline in the 15–24 km layer is nearly twice
as strong in the winter-spring season but much smaller in the summer and fall. The effect of including 1998 and 1999 years
with relatively high total ozone data reduces the overall-declining trend. The trends estimated from alg-99 retrievals are
statistically not significantly different from those in WMO 1998a; however, they are stronger by about 1% per decade in the lower stratosphere and thus closer to the estimates by sondes.
Comparisons of the integrated ozone loss from the Umkehr measurements with the total ozone changes for the same periods at
stations with good records show complete concurrence. The altitude and latitude appearances of the long-term geophysical signals
like solar (1–2%) and QBO (2–7%) are investigated.
Received April 12, 2001 Revised September 19, 2001 相似文献
4.
Om P. Tripathi S. G. Jennings C. D. O’Dowd K. P. Lambkin E. Moran 《Journal of Atmospheric Chemistry》2013,70(4):297-316
Sixteen years (1994 – 2009) of ozone profiling by ozonesondes at Valentia Meteorological and Geophysical Observatory, Ireland (51.94° N, 10.23° W) along with a co-located MkIV Brewer spectrophotometer for the period 1993–2009 are analyzed. Simple and multiple linear regression methods are used to infer the recent trend, if any, in stratospheric column ozone over the station. The decadal trend from 1994 to 2010 is also calculated from the monthly mean data of Brewer and column ozone data derived from satellite observations. Both of these show a 1.5 % increase per decade during this period with an uncertainty of about ±0.25 %. Monthly mean data for March show a much stronger trend of?~?4.8 % increase per decade for both ozonesonde and Brewer data. The ozone profile is divided between three vertical slots of 0–15 km, 15–26 km, and 26 km to the top of the atmosphere and a 11-year running average is calculated. Ozone values for the month of March only are observed to increase at each level with a maximum change of +9.2?±?3.2 % per decade (between years 1994 and 2009) being observed in the vertical region from 15 to 26 km. In the tropospheric region from 0 to 15 km, the trend is positive but with a poor statistical significance. However, for the top level of above 26 km the trend is significantly positive at about 4 % per decade. The March integrated ozonesonde column ozone during this period is found to increase at a rate of ~6.6 % per decade compared with the Brewer and satellite positive trends of ~5 % per decade. 相似文献
5.
该文介绍了中国科学院大气物理研究所（简称IAP）研制的电化学浓度电池（ECC）型臭氧（O3）探空仪基本性能测试和2013年上半年室外比对观测结果。结果表明:ECC的背景电流（Ibg）在0.1 μA以下或更低;测量O3的响应时间为21~26 s;NO2（SO2）使O3测值偏高（低）;抽气泵低压泵效系数（Cef）在100 hPa高度以下为1.0左右,在该高度以上上升,10 hPa达到1.17±0.10,5 hPa达到1.28±0.16,性能略低于同类进口产品（1.055以下）。国产和进口仪器在气象探空或抽气泵等部件上具有良好兼容性;两者所测O3垂直分布廓线总体一致。IAP O3探空仪O3总量与Brewer光谱仪测值比值为0.9~1.1;Cef和Ibg订正有效降低了IAP O3探空仪在平流层低层与进口仪器测值的差别,这一订正对O3柱浓度在平流层和对流层的贡献分别为约15 DU和4~6 DU;在对流层,IAP O3探空仪测值与进口仪器间的绝对差别稳定且低于0.5 mPa;而平流层受泵效影响较明显。因此,建议IAP O3探空仪提高其Cef的稳定性,参与国际比对测试,国产气象探空平台数据接收处理增加必要的滤波技术以降低平流层探测数据（包括O3）的振荡。 相似文献
6.
Based on the Stratospheric Aerosol and Gas Experiment (SAGE) II and the Halogen Occultation Experiment (HALOE) ozone profiles and the Total Ozone Mapping Spectrometer (TOMS) total ozone data sets, an empirical model for estimating the vertical distribution of stratospheric ozone over China is proposed. By using this model, the vertical distribution of stratospheric (16–50 km) ozone can be estimated according to latitude, month and total ozone. Comparisons are made between the modeled ozone profiles and the ... 相似文献
7.
Abstract An intercomparison of ozonesondes was held at Vanscoy, Saskatchewan, from 13 to 24 May 1991. The intercomparison, which was sponsored by the WMO and hosted by the Atmospheric Environment Service (AES) of Canada, was attended by scientists from six countries: Canada, Finland Germany, India, Japan and the United States. Four different makes of ozonesondes were used: the ECC sonde, the Brewer‐Mast sonde, the Indian ozonesonde and the Japanese RSH‐KC79 ozonesonde. These represent most of the sonde types that are in routine operation in the Global Ozone Observing System. A balloon payload and telemetry system was developed to accommodate up to eight ozonesondes that could operate independently and transmit data simultaneously to a ground receiver. Ten flights were launched, each carrying 7 or 8 sondes, and a total of 65 successful profile measurements were made. The payloads were carried to altitudes between 35 and 40 km. The measured profiles are used to determine statistically meaningful evaluations of the different sonde types. The results compared with those from previous intercomparisons indicate that there has been a general improvement in performance for most of the types. In addition there appears to have been changes with time in the relative sensitivity to tropospheric ozone for different sonde types. This result should be considered when drawing conclusions regarding trends in tropospheric ozone. 相似文献
8.
S. Yonemura S. Kawashima H. Matsueda Y. Sawa S. Inoue H. Tanimoto 《Theoretical and Applied Climatology》2008,92(1-2):47-58
Summary The application of principal components and cluster analysis to vertical ozone concentration profiles in Tsukuba, Japan, has
been explored. Average monthly profiles and profiles of the ratio between standard deviation and the absolute ozone concentration
(SDPR) of 1 km data were calculated from the original ozone concentration data. Mean (first) and gradient (second) components
explained more than 80% of the variation in both the 0–6 km tropospheric and 11–20 km troposphere–stratosphere (interspheric)
layers. The principal components analysis not only reproduced the expected inverse relationship between mean ozone concentration
and tropopause height (r
2 = 0.41) and that in the tropospheric layer this is larger in spring and summer, but also yielded new information as follows.
The larger gradient component score in summer for the interspheric layer points to the seasonal variation of the troposphere–stratosphere
exchange. The minimum SDPR was at about 3 km in the tropospheric layer and the maximum was at about 17 km in the interspheric
layer. The tropospheric SDPR mean component score was larger in summer, possibly reflecting the mixing of Pacific maritime
air masses with urban air masses. The cluster analysis of the monthly ozone profiles for the 1970s and 2000s revealed different
patterns for winter and summer. The month of May was part of the winter pattern in the 1970s but part of the summer pattern
during the 2000s. This statistically detected change likely reflects the influence of global warming. Thus, these two statistical
analysis techniques can be powerful tools for identifying features of ozone concentration profiles.
Authors’ addresses: S. Yonemura, S. Kawashima, S. Inoue, National Institute for Agro-Environmental Sciences, 3-1-3 Kannondai,
Tsukuba, Ibaraki 305-0031, Japan; H. Matsueda, Y. Sawa, Meteorological Research Institute, 1-1 Nagamine, Tsukuba, Ibaraki
305-0052, Japan; H. Tanimoto, National Institute for Environmental Studies, 16-2 Onogawa, Tsukuba, Ibaraki 305-8506, Japan. 相似文献
9.
AbstractRegular ground-based measurements of total ozone are available over the full Russian territory using M-124 filter ozonometers, Brewer spectrophotometers, and Système d'Analyse par Observation Zénithale (SAOZ) spectrometers in the Arctic region where these observations are essential for evaluating ozone loss in winter. Daily measurements are performed by three Brewer spectrophotometers; these are located in Kislovodsk (43.7°N, 42.7°E), Obninsk (55.1°N, 36.6°E), and Tomsk (56.5°N, 85.1°E). Two SAOZ spectrometers are deployed at the Arctic Circle in Salekhard (66.5°N, 66.7°E) and Zhigansk (66.8°N, 123.4°E). In addition, regular winter–spring ozonesonde soundings are carried out in Salekhard. Altogether, they have provided the unique measurements over the eastern Arctic required for characterizing ozone loss during each winter and will also monitor the anticipated ozone recovery following the reduction of chlorine and bromine ozone-depleting substances in the atmosphere. 相似文献
10.
Abstract Ground‐based measurements of total ozone were made during the polar night from Arctic stations in the winters of 1987–88 and 1988–89. The measurements were made with automated Brewer ozone spectrophotometers using the moon as a light source. Data were obtained from Alert and Resolute in Canada for both winters and from Heiss Island, USSR, for the second winter. The method of measurement is briefly reviewed and data from the three stations are presented. The ground‐based total ozone measurements are compared with the integrated values derived from ozonesonde profiles. 相似文献
11.
全球大气位温的两个不等价约束及其服从Gamma分布的证明 总被引：4，自引：0，他引：4
本文对全球大气位温积分守恒和热力学总熵守恒的物理含义及其不等价性进行了讨论。认为，作为对大气热力学状态较完整的描述，应将大气热力学总熵守恒这一约束条件补入数值预报模式中去。利用最大熵原理和上述两个约束条件，在理论上对大气位温服从Gamma分布这一从实际资料中揭示出来的事实进行了证明，得到了理论与实际完全吻合的结果。 相似文献
12.
北半球中纬度地区上层臭氧变化的合成分析研究 总被引：1，自引：1，他引：0
应用逆转方法（C）,对北半球中纬度地区8个观测质量较好的O3地面站的近30年地面遥感逆转资料进行标准处理。采用合成分析方法,对中纬度带上层O3进行了分析研究,发现上层O3总的长期演变趋势较为平坦,仅80年代初及90年代初在36km以上层O3含量有突降现象。这可能与EL Chichon大火山焊发和Pinatubo大火山爆发有较大关系。此外。在上层O3含量的长期演变过程中,还可看到准11年周期,并证实28～36km层及36km以上层O3含量季节变化位相相反。本研究结果可能对南极O3洞的形成机制及近年来O3层变浅薄的机制的认识提供依据并产生影响。
相似文献
13.
利用建立的球面分层大气散射模式，研究了Ｂｒｅｗｅｒ仪器工作波长进行Ｕｍｋｅｈｒ短法反演所包含的信息量，给出Ｂｒｅｗｅｒ仪器探测大气臭氧垂直廓线的方法。同时，用气溶胶光学厚度计算得到气溶胶订正系数，建立了Ｕｍｋｅｈｒ反演的程序，用此程序对ＴａｂｌｅＭｏｕｎｔａｉｎ资料进行气溶胶修正，得到了较好的结果。对北京测站１９９１年１─３月资料进行由气溶胶造成的臭氧反演廓线的误差计算，结果表明，用常规反演方法得到的各层臭氧含量的误差与平流层气溶胶光学厚度有一近似线性的关系；进行气溶胶修正后，与国外的臭氧反演廓线的误差修正工作￣［１］比较，结果较一致。研究提出的气溶胶订正反演方法为更好地对平流层臭氧变化趋势进行研究提供了可能性和可靠的基础。 相似文献
14.
Karanam Kishore Kumar Debadatta Swain Sherine Rachel John Geetha Ramkumar 《Climate Dynamics》2011,37(9-10):1961-1973
Owing to the importance of middle atmosphere, recently, a Middle Atmospheric Dynamics (MIDAS) program was carried out during the period 2002?C2007 at Thumba (8.5°N, 77°E). The measurements under this program, involving regular radiosonde/rocket flights as well as atmospheric radars, provided long period observations of winds and temperature in the middle atmospheric region from which waves and oscillations as well as their forcing mechanisms particularly in the low-latitude middle atmosphere could be analyzed. However, a detailed analysis of the forcing mechanisms remains incomplete due to the lack of important measurements like ozone which is a significant contributor to atmospheric dynamics. Presently, profiles of ozone are available from TIMED/SABER (Thermosphere, Ionosphere, Mesosphere Energetics and Dynamics/Sounding of the Atmosphere using Broad Emission Radiometry) satellite globally from about 15 to 100?km, over multiple years since 2002. In this regard, a comprehensive study has been carried out on ozone and its variability at Quasi Biennial Oscillation (QBO) and Semiannual Oscillation (SAO) scales using TIMED/SABER ozone observations during the MIDAS campaign period. Before using the TIMED/SABER ozone measurements, an inter-comparison has been carried out with in situ measurements of ozone obtained under the Southern Hemisphere Additional Ozonesondes (SHADOZ) campaign for the year 2007 at few stations. The inter-comparison showed very good agreement between SABER and ozonesonde derived ozone profiles. After validating the SABER observations, ozone profiles are used extensively to study the QBO and SAO along with temperature and winds in the 20?C100?km height region. It is known that the SAO in mesosphere and stratosphere are in opposite phases, but the present study for the first time reports the aspect of opposite phases in the mesosphere itself. Thus, the present work attempts to study the long-period oscillations in stratosphere and mesosphere in ozone, temperature and winds simultaneously for the first time over this latitude. These observations provided a unique opportunity to explore long-period oscillations in chemistry, dynamics and thermal structure of the middle atmosphere simultaneously. 相似文献
15.
Gill-Ran Jeong Beatriz M. Monge-Sanz Eun-Hee Lee Jerald R. Ziemke 《Asia-Pacific Journal of Atmospheric Sciences》2016,52(5):479-494
The two types of ozone, the simulation with interactive (prognostic) ozone using linear photochemistry parameterization (LPP) (INTR) and the simulation with non-interactive ozone using ozone climatology (CLIM), were used in the global forecast model. These two types of ozone were compared with ozone observations from the Aura Microwave Lim Sounder (MLS) and ozonesondes from 16-30 September 2008. The INTR is sensitive to LPP schemes while less sensitive to the time average of initial ozone data. Among three LPP schemes, CARIOLLE, COPCAT, and LINOZ, the COPCAT produces ozone profiles with least differences from MLS and ozonesondes. CLIM overestimates MLS at 200-20 hPa while INTR with COPCAT scheme underestimates MLS ozone above 5 hPa. Over the Antarctic in the lower stratosphere CLIM overestimates MLS and ozonesondes whereas INTR underestimates MLS but overestimates the ozonesonde data. Thus, COPCAT agrees better with ozonesonde data than any other LPP schemes and CLIM. Changing the ozone distribution from CLIM to INTR affects temperature profiles mainly through the modification of differential radiative fluxes. The correlations between ozone, differential radiative fluxes, and temperature are distinguished by altitude (or pressure levels). The correlations are strong or moderate between 3-1000 hPa (lower atmosphere) and weak above 3 hPa (upper atmosphere). This study demonstrates that the simulation of ozone using an appropriate LPP scheme is excellent in overcoming the drawbacks of using climatological ozone profiles that poorly agree with observations in extreme ozone hole events. 相似文献
16.
AbstractThe influence of variations in atmospheric temperature and ozone profiles on the total ozone column (TOC) derived from a Brewer MKII spectrophotometer operating in Thessaloniki, Greece, is investigated using three different sets of ozone absorption cross-sections. The standard Brewer total ozone retrieval algorithm uses the Bass and Paur (1985) cross-sections without accounting for the temperature dependence of the ozone cross-sections which produces a seasonally dependent bias in the measured TOC. The magnitude of this temperature effect depends on the altitude where the bulk of the ozone absorption occurs. Radiosonde measurements for the period 2000 to 2010 combined with climatological ozone profiles were used to calculate the effective temperature of ozone absorption and investigate its effect on the retrieved ozone column. Three different ozone absorption cross-section spectra convolved with the instrument's slit function were used: those of Bass and Paur (hereafter BP), currently used in the standard Brewer retrieval algorithm; those of Brion, Daumont, and Malicet (Malicet et al., 1985; hereafter BDM); and the recently published set by Serdyuchenko et al. (2013 hereafter S13). The temperature dependence of the differential ozone absorption coefficient ranges between 0.09 and 0.13% per degree Celsius for BP, between ?0.11 and ?0.06% per degree Celsius for BDM, and between 0.018 to 0.022% per degree Celsius for S13, resulting in a seasonal bias in the derived TOC of up to 2%, 1.8%, and 0.4%, respectively. The temperature sensitivity of the differential ozone absorption coefficient for the Brewer spectrophotometer at Thessaloniki for the BP and BDM cross-sections is found to be within the range reported for other Brewer instruments in earlier studies, whereas the seasonal bias in TOC is minimized when using the new S13 cross-sections because of their small temperature dependence. 相似文献
17.
Data of stratospheric ozone measurements with the AK-3 lidar over Obninsk in 2012–2015 are compared with Aura/MLS and Aura/OMI satellite data and parallel surface observations of total ozone (TO) with the Brewer spectrophotometer. The maximum difference in mean ozone concentration between the lidar and Aura/MLS data in the altitude range of 13 to 32 km does not exceed 0.2 x 1012 mol./cm3 (or the maximum of 9% at the altitude of 13 km). At the same time, Aura/OMI data have a positive bias of about 20% relative to lidar data in the range of 13 to 20 km that is associated with OMI measurement errors according to literature data. Total ozone values calculated from lidar measurements jointly with the known climatology data are compared with those measured with the Brewer spectrophotometer. It is demonstrated that the correlation between the results of measurements obtained by two methods is close to linear, and the mean relative difference in the overall measurement range does not exceed 5%. 相似文献
18.
胡顺星 naol.hfcas.ac.cn 胡欢陵 naol.hfcas.ac.cn 周军 naol.hfcas.ac.cn 吴永华 naol.hfcas.ac.cn 《Acta Meteorologica Sinica》2002,(2)
In this paper the effects of aerosol on tropospheric ozone measurements by three-wavelength(266-289-308nm) dual differential absorption lidar (DIAL) and two-wavelength (266-289 nmand 266-308 nm) DIAL are simulated.By using the two kinds of DIAL.vertical profiles of ozonedensity from 2 to 3.6 km altitude range are measured.Both simulation and observation resultsshow that the three-wavelength dual-DIAL method is more effective to reduce the effects of aerosolthan the two-wavelength DIAL method.Therefore,accurate ozone density distributions can beretrieved by the three wavelength dual DIAL method. 相似文献
19.
国产GPSO3与芬兰Vaisala臭氧探空仪的比对试验 总被引：10，自引：0，他引：10
臭氧探空仪是一种主要而又直接的探测大气臭氧垂直分布的技术手段。为了了解国产GPSO3臭氧探空仪的测量精度、灵敏度和可靠性．我们开展了与芬兰Vaisala ECC臭氧探空仪的系列平行比对试验,包括实验室臭氧传感器比对测试．室外地面臭氧传感器比对测试,低压环境下进气柱塞泵(效)比对测试和臭氧探空施放比对试验。测试结果分析表明,国产GPSO3臭氧探空仪的主要指标性能与国际通用的Vaisala臭氧探空仪的相当。 相似文献
20.
In this paper the effects of aerosol on tropospheric ozone measurements by three-wavelength (266-289-308nm) dual differential absorption lidar (DIAL) and two-wavelength (266-289 nm and 266-308 nm) DIAL are simulated.By using the two kinds of DIAL.vertical profiles of ozone density from 2 to 3.6 km altitude range are measured.Both simulation and observation results show that the three-wavelength dual-DIAL method is more effective to reduce the effects of aerosol than the two-wavelength DIAL method.Therefore,accurate ozone density distributions can be retrieved by the three wavelength dual DIAL method. 相似文献