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1.
人为和生物排放量对春季东亚地面臭氧的协同贡献   总被引：2，自引：0，他引：2  
屈玉  安俊岭  周慧 《大气科学》2009,33(4):670-680
臭氧O3的生成是多因子影响的复杂非线性过程, 一个因子在其他因子起作用时的贡献可以分为纯贡献与协同贡献。本文采用因子分离方法和改进后的区域空气质量模式 (RAQM) 计算了人为氮氧化物 (NOx＝NO+NO2)、人为可挥发性有机化合物(AVOCs)以及生物可挥发性有机化合物(BVOCs)对春季东亚地区地面臭氧浓度的协同贡献及总贡献(＝纯贡献+协同贡献)。结果表明, AVOCs、BVOCs与NOx对O3生成量的贡献依赖于AVOCs、BVOCs排放量的相对大小。AVOCs或BVOCs排放量显著偏高的地区, 其总贡献主要来源于其与NOx的协同贡献。从区域角度 (1°×1°) 来看, BVOCs对东亚春季地面O3浓度的贡献较小, BVOCs排放量明显偏高的个别地区除外。BVOCs总贡献有很强的日变化特征, BVOCs总贡献有可能小于其协同贡献。个例研究的成果应用于O3调控对策的制定和实施很可能达不到预期的效果。我国北方 (30°N以北) 应控制人为源; 我国南方BVOCs排放量显著偏高的地区, 生物源和人为源的贡献都必须考虑。  相似文献   

2.
In this study, an improved and complete secondary organic aerosols (SOA) chemistry scheme was implemented in the CHIMERE model. The implementation of isoprene chemistry for SOA significantly improves agreement between long series of simulated and observed particulate matter concentrations. While simulated organic carbon concentrations are clearly improved at elevated sites by adding the SOA scheme, time correlation are impaired at low level sites in Portugal, Italy and Slovakia. At several sites a clear underestimation by the CHIMERE model is noticed in wintertime possibly due to missing wood burning emissions as shown in previous modeling studies. In Europe, the CHIMERE model gives yearly average SOA concentrations ranging from 0.5 μg m  − 3 in the Northern Europe to 4 μg m  − 3 over forested regions in Spain, France, Germany and Italy. In addition, our work suggests that during the highest fire emission periods, fires can be the dominant source of primary organic carbon over the Mediterranean Basin, but the SOA contribution from fire emissions is low. Isoprene chemistry has a strong impact on SOA formation when using current available kinetic schemes.  相似文献   

3.
Emissions of oxygenated volatile organic compounds (OVOC) from several plant species were measured in continuously stirred tank reactors (CSTR). High emission pulses of OVOCs were observed when plants were exposed to stress. Absolute emission rates were highly variable ranging up to 10–13 mol · cm–2 · s–1. The temporal shape of these emissions was described by a formalism similar to that of a consecutive reaction of pseudo first order kinetics. The main emitted OVOC was (Z)-3-hexenol together with other C6-aldehydes and alcohols, suggesting that lipoxygenase activity on linolenic acid was mainly responsible for OVOC production. Various stress factors induced lipoxygenase activity and subsequent emissions of OVOCs. These factors were exposure to high ozone concentrations, pathogen attack, and wounding. The pattern of OVOC emissions from tobacco was similar for different stress applications and the same products of lipoxygenase activity were emitted from all investigated plant species. Our results imply that these emissions occur as general response of the plants to stress. Since plants experience various abiotic or biotic stress factors in the environment, OVOC emissions as a response to stress are likely to be of significant importance for atmospheric chemistry.Now at  相似文献   

4.
Summary ?A major limitation in predicting the ultraviolet-B irradiance on humans, plant leaves and flowers and aquatic organisms is the difficulty in estimating exposure. This study analyzes the spatial variability in the daily exposure of narrow band 300 nm and 368 nm and broadband 290–315 nm (UVB) solar radiation between twelve paired locations in the United States Department of Agriculture (USDA) UVB Climate Network over two summer growing seasons (May through August of 2000 and 2001). The spatial correlation of the UVB, 300 nm and 368 nm daily exposures between locations was approximately 0.7 to 0.8 for spacing distances of 100 km. The 300 nm daily exposure was typically more highly correlated between locations than the 368 nm daily exposure. Both the diffuse and direct beam components to the 300 nm daily exposure were similarly correlated with distance between locations. The 368 nm diffuse component of the daily exposures was less correlated with distance than the direct beam component, limiting the ability to interpolate daily exposures from measurement locations. In general the variability in daily exposures of UVB in the USDA UVB Climate Network is too large to interpolate daily exposures of solar radiation, with estimated 300 nm, 368 nm and broadband UVB errors at one-half the mean station spacing of the USDA Network of 22%, 21% and 16% respectively. More accurate interpolations of UVB exposure from this network will require either the incorporation of cloud cover variability from satellite imagery for daily exposure or the use of longer periods of accumulated exposure. Received May 14, 2002; revised October 25, 2002; accepted November 16, 2002  相似文献   

5.
Summary  Transpiration of an adult corn crop was measured with the sap flow method using the stem heat balance technique. The 1 ha-field was located in the Parisian region and the measurements were taken over two consecutive years (1993 and 1994). The experiments were carried out during the active growing season, leaf area index being ≈4.0. In order to individuate the “mean plant” a preliminary analysis was carried out to determine the frequency distribution of plant stem diameters as measured on 34 randomly chosen samples. According to this analysis, the mean corn plant diameter was around 20 mm for both years. As a consequence, the sap flow gauges were installed on plants having this diameter. The sap flow transpiration data was compared with the actual evapotranspiration measured by the Bowen ratio method on the same experimental field at the hourly and daily scales. The comparison between sap flow transpiration and actual evapotranspiration showed that the values are more widely spread at the hourly scale than at the daily scale due to the kinetics of plant water content during the day. Sap flow transpiration was 88–90% of actual evapotranspiration: this lack of about 10–12% is of the same order as soil water evaporation. In conclusion, the sap flow transpiration method could be considered a valuable method to use for measuring transpiration of certain crop plants in the field, especially for small plots. This method is substantially improved if sap flow measurement is carried out on plants screened by the analysis of plant diameter distribution in the field. Received October 6, 1999 Revised June 21, 2000  相似文献   

6.
Ammonia emissions from stored farm manures form a small but significant proportion (∼10%) of the total emitted annually from UK sources. These emissions are regulated by factors including: the surface area of the store; the storage method; the physical form of the stored manure and the source of manure. A method was developed to estimate in situ emissions from a range of store types (weeping wall and earth-banked lagoon) that are currently under-represented in UK emissions estimates. Passive diffusion samplers (Willems Badges) were used to determine vertical concentration profiles to a height of 4.5 m at a number of locations around each slurry store. An atmospheric dispersion model was applied to estimate the contribution from emissions from other on-farm ammonia sources to the measured data and also to determine the emission rates from the stored manure. A procedure was applied whereby the emission rates from each source were allowed to vary and a numerical equation solver was applied to backfit the modelled data set to the field measurements. Measurements were collected at four farms on a monthly basis throughout the year, with each dataset being collected over 24 h. The uncertainties in the estimates of emissions from the slurry stores during individual measurement periods typically ranged between 20–40% though higher uncertainties occurred when emission fluxes from the stores were below 0.25 g NH3–N m−2 day−1 and were entrained in the wakes, and mixed with the emissions, of adjacent buildings. The average emission from the farms was 0.6 g NH3–N m−2 day−1 which agrees with other recent data on ammonia emissions from crusted slurry stores and, though it is within the range of data considered in the UK emissions inventory, suggests that emissions from weeping wall stores and earth-banked lagoons may be currently overestimated in national predictions.  相似文献   

7.
The carbon kinetic isotope effects (KIEs) in the reactions of several unsaturated hydrocarbons with chlorine atoms were measured at room temperature and ambient pressure using gas chromatography combustion isotope ratio mass spectrometry (GCC-IRMS). All measured KIEs, defined as the ratio of the rate constants for the unlabeled and labeled hydrocarbon reaction k 12/k 13, are greater than unity or normal KIEs. The KIEs, reported in per mil according to Cl ɛ = (k 12/k 13−1) × 1000‰ with the number of experimental determinations in parenthesis, are as follows: ethene, 5.65 ± 0.34 (1); propene, 5.56 ± 0.18 (2); 1-butene, 5.93 ± 1.16 (1); 1-pentene, 4.86 ± 0.63 (1); cyclopentene, 3.75 ± 0.14 (1); toluene, 2.89 ± 0.31 (2); ethylbenzene, 2.17 ± 0.17 (2); o-xylene, 1.85 ± 0.54 (2). To our knowledge, these are the first reported KIE measurements for reactions of unsaturated NMHC with Cl atoms. Relative rate constants were determined concurrently to the KIE measurements. For the reactions of cyclopentene and ethylbenzene with Cl atoms, no rate constant has been reported in refereed literature. Our measured rate constants are: cyclopentene (7.32 ± 0.88) relative to propene (2.68 ± 0.32); ethylbenzene (1.15 ± 0.04) relative to o-xylene (1.35 ± 0.21), all × 10−10 cm3 molecule−1 s−1. The KIEs in reactions of aromatic hydrocarbons with Cl atoms are similar to previously reported KIEs in Cl-reactions of alkanes with the same numbers of carbon atoms. Unlike the KIEs for previously studied gas-phase hydrocarbon reactions, the KIEs for alkene–Cl reactions do not exhibit a simple inverse dependence on carbon number. This can be explained by competing contributions of normal and inverse isotope effects of individual steps in the reaction mechanism. Implications for the symmetries of the transition state structures in these reactions and the potential relevance of Cl-atom reactions on stable carbon isotope ratios of atmospheric NMHC are discussed.  相似文献   

8.
Long-living wood products contribute to the mitigation of climate change in many ways. They act as a carbon pool during their service life, as they withdraw CO2 from its natural cycle. After their service life, they can stitute for fossil fuels if they are incinerated in adequate furnaces. Furthermore, wood products can stitute for more energy-intense products made of ‘conventional’ materials. This paper quantifies the stitution and pool effects of an increased use of wood in the building sector in Switzerland for the years 2000–2130. Life cycle data on greenhouse gas (GHG) emissions of 12 wood products and their stitutes are used as proxies for relevant building products; this data is linked to the forecasted wood flows for each group of building products in a cohort-model. For the political assessment, GHG effects occurring abroad and in Switzerland are distinguished. The results show that the pool effect of an increased use of long-living wood products is of minor importance, whereas the energetic and material stitution effects are much more relevant, especially on a long-term. For construction products, the Swiss share of the GHG effect related to the material stitution is relatively high, as mainly nationally produced materials are stituted for. For interior products, the Swiss share of the GHG effect related to the material stitution is rather small because mainly imports are stituted for. The results must be considered as rough estimates. Nonetheless, these calculations show that an increased use of wood in the building sector is a valid and valuable option for the mitigation of greenhouse gas emissions and for reaching GHG emission targets in a mid- to long-term. Still, the pool and stitution capacity of an increased use of wood is relatively small compared to the overall GHG emissions of Switzerland.  相似文献   

9.
Sergio Pacca 《Climatic change》2007,84(3-4):281-294
Greenhouse gas (GHG) emissions from hydroelectric dams are often portrayed as nonexistent by the hydropower industry and have been largely ignored in global comparisons of different sources of electricity. However, the life cycle assessment (LCA) of any hydroelectric plant shows that GHG emissions occur at different phases of the power plant’s life. This work examines the role of decommissioning hydroelectric dams in greenhouse gas emissions. Accumulated sediments in reservoirs contain noticeable levels of carbon, which may be released to the atmosphere upon decommissioning of the dam. The rate of sediment accumulation and the sediment volume for six of the ten largest United States hydroelectric power plants is surveyed. The amount of sediments and the respective carbon content at the moment of dam decommissioning (100 years after construction) was estimated. The released carbon is partitioned into CO2 and CH4 emissions and converted to CO2 equivalent emissions using the global warming potential (GWP) method. The global warming effect (GWE) due to dam decommissioning is normalized to the total electricity produced over the lifetime of each power plant. The estimated GWE of the power plants range from 128–380 g of CO2eq./kWh when 11% of the total available sediment organic carbon (SOC) is mineralized and between 35 and 104 g of CO2eq./kWh when 3% of the total SOC is mineralized. Though these values are below emission factors for coal power plants (890 g of CO2eq./kWh), the amount of greenhouse gases emitted by the sediments upon dam decommissioning is a notable amount that should not be ignored and must be taken into account when considering construction and relicensing of hydroelectric dams.  相似文献   

10.
Aerosol and rain samples were collected between 48°N and 55°S during the KH-08-2 and MR08-06 cruises conducted over the North and South Pacific Ocean in 2008 and 2009, to estimate dry and wet deposition fluxes of atmospheric inorganic nitrogen (N). Inorganic N in aerosols was composed of ~68% NH4+ and ~32% NO3– (median values for all data), with ~81% and ~45% of each species being present on fine mode aerosol, respectively. Concentrations of NH4+ and NO3− in rainwater ranged from 1.7–55 μmol L−1 and 0.16–18 μmol L−1, respectively, accounting for ~87% by NH4+ and ~13% by NO3− of total inorganic N (median values for all data). A significant correlation (r = 0.74, p < 0.05, n = 10) between NH4+ and methanesulfonic acid (MSA) was found in rainwater samples collected over the South Pacific, whereas no significant correlations were found between NH4+ and MSA in rainwater collected over the subarctic (r = 0.42, p > 0.1, n = 6) and subtropical (r = 0.33, p > 0.5, n = 6) western North Pacific, suggesting that emissions of ammonia (NH3) by marine biological activity from the ocean could become a significant source of NH4+ over the South Pacific. While NO3− was the dominant inorganic N species in dry deposition, inorganic N supplied to surface waters by wet deposition was predominantly by NH4+ (42–99% of the wet deposition fluxes for total inorganic N). We estimated mean total (dry + wet) deposition fluxes of atmospheric total inorganic N in the Pacific Ocean to be 32–64 μmol m−2 d−1, with 66–99% of this by wet deposition, indicating that wet deposition plays a more important role in the supply of atmospheric inorganic N than dry deposition.  相似文献   

11.
Samples of airborne PM2.5 particles in Guangzhou urban area were collected during the autumn of 2006 and the spring of 2007. The morphologies and elemental compositions of individual particles were determined by Scanning Electron Microscopy coupled with Energy Dispersive X-ray Spectrometer (SEM-EDX). The obtained images were further analyzed for size distribution by an image analysis system. Based on the morphology, particles in PM2.5 were classified into four groups: soot aggregates, minerals, fly ash and others. The amount of soot aggregates and minerals were higher than that of fly ashes. The distributions of particles by number and size in two seasons were bimodal with 90% less than 1.0 μm in diameter. The primary peak from the autumn samples was in the size range of 0.4 ~ 0.5 μm, and 0.3 ~ 0.4 μm for the spring samples. More soot aggregates (36.1%) and minerals (61.5%) were found than fly ash (2.4%) in autumn, but soot aggregates (89.9%) was the dominant particle type in spring. The size distribution of particles according to the volume was generally opposite to that according to the number. Particles less than 1.0 μm were as high as 89.5% in number but contributed only 18.9% in volume, indicating that fine particles contributed relatively little in volume although existing in large numbers.  相似文献   

12.
中国地区臭氧前体物对地面臭氧的影响   总被引：5，自引：1，他引：4  
利用GEOS-Chem模式的数值试验结果,研究中国地区NOx和两类VOCs对O3质量浓度分布及其化学机理的影响。研究表明,NOx的减少会使得中国西部O3质量浓度显著降低,但在冬季NOx的减少会使得东北、华北地区O3质量浓度上升。而京津唐地区由于VOCs/NOx比值偏低,不能通过单一减少NOx来控制O3质量浓度。VOCs排放的减少会使得我国东部地区O3质量浓度大幅减少,其中人为VOCs的减少能降低我国东部地面O3质量浓度,而生物VOCs的减少只能在夏秋季有效减少我国东部地区35°N以南区域的地面O3质量浓度。控制地面O3质量浓度时,中国西部主要考虑NOx的减排,东部35°N以北主要考虑AVOCs的减排,而30~35°N应同时考虑AVOCs和BVOCs的减排,在30°N以南的地区,则需要全面考虑NOx和VOCs的减排。  相似文献   

13.
Summary  Net ecosystem CO2 exchange was measured over a mountain birch forest in northern Finland throughout the growing season. The maximal net CO2 uptake rate of about − 0.5 mg(CO2) m−2 s−1 was observed at the end of July. The highest nocturnal respiration rates in early August were 0.2 mg(CO2) m−2 s−1. The daily CO2 balances during the time of maximal photosynthesis were about −15 g(CO2) m−2 d−1. The mountain birch forest acted as a net sink of CO2 from 30 June to 28 August. During that period the net CO2 balance was −448 g(CO2)m−2. The interannual representativeness of the observed balances was studied using a simplified daily balance model, with daily mean global radiation and air temperature as the input parameters. The year-to-year variation in the phenological development was parameterised as a function of the cumulative effective temperature sum. The daily balance model was used for estimating the variability in the seasonal CO2 balances due to the timing of spring and meteorological factors. The sink term of CO2 in 1996 was lower than the 15-year mean, mainly due to the relatively late emergence of the leaves. Received October 11, 1999 Revised April 25, 2000  相似文献   

14.
There is a gap between the increased scientific understanding of carbon pools and fluxes at individual trees/stand and that of forested landscape with complex structures (i.e. variety of species, age classes, site characteristic and management practices). The question about how results generated from a simulated physiologically distinct individual(s)/stands grown at a particular location (scale) can be extrapolated (scaling) across a diverse population in time and space with diverse environments, has been troubling scientists for many years. Scale and scaling present three problems in common: (a) spatial heterogeneity, (b) non-linearity in response and (c) disturbance regimes. Scale, in particular, presents other three problems: (d) threshold scale for processes, (e) dominant processes with scales and (f) emerging properties of the system. Scaling presents problems with (g) feedbacks between plants and environment and (h) plant interactions. The present study proposes a modeling framework linking a process-based model SECRETS – to overcome some of the scale and scaling problems (a, b, c, d and g) – to a C accounting model GORCAM – to integrate the effects of C stock in wood products and from fossil fuel substitution. The capabilities of the modeling framework are tested against three theoretical complex forested landscapes that combine some of the five following scenarios: existing multifunctional forest under (1) actual and (2) changing environmental conditions, and afforestation of an agricultural area with (3) a new multifunctional forest or with (4) a short rotation coppice (poplar) or with (5) an agricultural crop (miscanthus) for bioenergy production. Forest reserves calculations are included for completeness of the landscape C balance and as reference. Results, on the one hand, suggest that the framework is able to simulate C sequestration and stock in ecosystem pools, wood products and fossil fuel substitution of the scenarios under actual environmental conditions. However, comparison of results under changing environmental conditions, against specific plant literature suggest SECRETS formulation must be improved with recent development in photosynthesis, stomatal conductance and N balances. On the other hand, results also suggest that under actual environmental conditions, the optimum landscape scenario to sequester C and avoid fossil emissions to the atmosphere is composed by existing multifunctional forest, reserves and afforestation with short rotation coppice for bioenergy production.  相似文献   

15.
The kinetics of heterogeneous reactions of NO2 with 17 polycyclic aromatic hydrocarbons (PAHs) adsorbed on laboratory generated kerosene soot surface was studied over the temperature range (255–330) K in a low pressure flow reactor combined with an electron-impact mass spectrometer. The kinetics of soot-bound PAH consumption due to their desorption and reaction with NO2 were monitored using off-line HPLC measurements of their concentrations in soot samples as a function of reaction time, NO2 concentrations in the gas phase being analyzed by mass spectrometer. No measurable decay of PAHs due to the reaction with NO2 was observed under experimental conditions of the study (maximum NO2 concentration of 5.5 × 1014 molecule cm−3 and reaction time of 45 min), which allowed to determine the upper limits of the first-order rate constants for the heterogeneous reactions of 17 soot-bound PAHs with NO2: k < 5.0 × 10−5 s−1 (for most PAHs studied). Comparison of these results to previous studies carried on different carbonaceous substrates, showed that heterogeneous reactivity of PAHs towards NO2 is, probably, dependent on the substrate nature even for resembling, although different carbonaceous materials. Results show that particulate PAHs degradation by NO2 alone is of minor importance in the atmosphere  相似文献   

16.
 An improved concept of the best analogues method was used to reconstruct the Last Glacial Maximum (LGM) climate from a set of botanical records from the former Soviet Union and Mongolia. Terrestrial pollen and macrofossil taxa were grouped into broad classes – plant functional types (PFTs), defined by the ecological and climatic parameters used in the BIOME1 model. PFT scores were then calibrated in terms of modern climate using 1245 surface pollen spectra from Eurasia and North America. In contrast to individual taxa, which exhibit great variability and may not be present in the palaeoassemblages, even in suitable climates, PFTs are more characteristic of the vegetation types. The modified method thus allows climate reconstruction at time intervals with partial direct analogues of modern vegetation (e.g. the LGM). At 18 kBP, mean temperatures were 20–29 °C colder than today in winter and 5–11 °C colder in summer in European Russia and Ukraine. Sites from western Georgia show negative, but moderate temperature anomalies compared to today: 8–11 °C in January and 5–7 °C in July. LGM winters were 7–15 °C colder and summers were 1–7 °C colder in Siberia and Mongolia. Annual precipitation sums were 50–750 mm lower than today across northern Eurasia, suggesting a weakening of the Atlantic and Pacific influences. Reconstructed drought index shows much drier LGM conditions in northern and mid-latitude Russia, but similar to or slightly wetter than today around the Black Sea and in Mongolia, suggesting compensation of precipitation losses by lower-than-present evaporation. Received: 11 May 1998 / Accepted: 25 September 1998  相似文献   

17.
 The atmospheric general circulation model ECHAM-4 is coupled to a chemistry model to calculate sulfate mass distribution and the radiative forcing due to sulfate aerosol particles. The model simulates the main components of the hydrological cycle and, hence, it allows an explicit treatment of cloud transformation processes and precipitation scavenging. Two experiments are performed, one with pre-industrial and one with present-day sulfur emissions. In the pre-industrial emission scenario SO2 is oxidized faster to sulfate and the in-cloud oxidation via the reaction with ozone is more important than in the present-day scenario. The atmospheric sulfate mass due to anthropogenic emissions is estimated as 0.38 Tg sulfur. The radiative forcing due to anthropogenic sulfate aerosols is calculated diagnostically. The backscattering of shortwave radiation (direct effect) as well as the impact of sulfate aerosols on the cloud albedo (indirect effect) is estimated. The model predicts a direct forcing of −0.35 W m-2 and an indirect forcing of −0.76 W m-2. Over the continents of the Northern Hemisphere the direct forcing amounts to −0.64 W m-2. The geographical distribution of the direct and indirect effect is very different. Whereas the direct forcing is strongest over highly polluted continental regions, the indirect forcing over sea exceeds that over land. It is shown that forcing estimates based on monthly averages rather than on instantaneous sulfate pattern overestimate the indirect effect but have little effect on the direct forcing. Received: 16 October 1996/Accepted: 24 October 1996  相似文献   

18.
Summary The similarities in time series recorded at sites which are distant from each other are called teleconnections. In this paper, the loss of such correlations with inter-site distance was investigated for both climatic and dendrochronological data sets, with 70 tree-ring chronologies. A dense network of weather stations was studied in the southeastern French Alps, covering complex climatic gradients over three departments. 78 sites with precipitation data (with a total of 48 756 monthly values), and 48 stations that recorded temperature (with 20 722 monthly mean values) were analysed. In the same area, four coniferous species (mountain pine and stone pine, European larch and Norway spruce) provided 37 ring-width chronologies for high elevation sites near the timberline. Both silver fir and Norway spruce provided a second tree-ring chronology network for 33 different sites at lower elevations. The teleconnections between precipitation series were found to be higher than those observed for temperature over short distances, but the maximum threshold distance was lower (193 km) compared to a positive correlation distance that exceeds 500 km for temperature. The maximum temperatures had stronger teleconnections than minimum values (522 km versus 476 km), since the latter are linked more with other site factors, such as slope, exposure and local topography. As expected, the tree-ring chronologies showed weaker teleconnections than the climatic series, with a threshold distance of 374 km obtained for all high elevation forests. The coniferous species with high intra-specific teleconnections over large distances were, in decreasing importance, Pinus uncinata (> 500 km), Picea abies (477 km), Pinus cembra (over 254 km) and Larix decidua (over 189 km only). The two former species showed the highest intra-specific correlations (with mean correlation R=0.625 and 0.666). The dendrochronological teleconnections were found to have a extent lesser for trees species that depend on rainfall (such as larch, and stone pine). They are enhanced, however, for temperature sensitive species such as spruce and mountain pine (a drought resistant tree). Therefore, these two latter conifers appear to be especially suitable for climatic reconstruction over large distances in mountainous areas. However, teleconnections within silver fir (Abies alba) and spruce chronologies were sharply reduced (over 131 km and 135 km) in lower elevation forests, underlining the interest of timberline forests for dendroclimatology. A better knowledge of the spatial correlations in climatic series and ring-width data may enable the optimisation of weather station networks. It may also permit a better choice of weather stations used for dendroclimatology, either for tree-ring and climate relationship calibration or for climate reconstructions. In dendrochronology, wood dating also requires the knowledge of to what extent remote ring-width chronologies can be used. Received September 11, 2000 Revised March 26, 2001  相似文献   

19.
Summary ?Microclimatological data obtained during a field experiment in the nongrowing winter period were used to study the microclimatologically stable night conditions of a 200 × 150 m miscanthus (Miscanthus cv. giganteus) stand and compared to open field conditions. The microclimatological pattern within the miscanthus canopy was characterized by long-wave radiative cooling of the plant stand and by an established temperature inversion within the canopy at calm nights. The results show that there are significant differences in air temperature and energy balance components between the open field and the miscanthus field during calm and clear nights. In general, net radiation difference during the cold and calm nights was relatively constant and about 20 W m−2 less negative in miscanthus (because of lower surface temperatures) than at the open field. Air temperature differences also remained fairly constant and were up to 3 °C lower than at the open field (at the height of 1 m). Through thermal inversion cold air accumulated in the lower parts of the canopy as shown by the vertical air temperature profiles. They showed a greater amplitude within the diurnal cycle in the miscanthus stand than in the open field. Through the onset of wind, temperature profiles changed rapidly and differences diminished. Vertical katabatic air drainage into the canopy layers was estimated indirectly by using the energy balance approach. It was calculated from the significant energy balance closure gap and showed a mean air exchange rate of up to 22 m3 m−2 h−1, related to a stand volume of 1 m2 area and 4 m height, during the mostly calm and clear nights, depending on the canopy net radiation and turbulent heat exchange forced by slight wind spells. Quantitative uncertainties in calculated cold air drainage which are introduced by the measurement method and certain assumptions in the calculations, were considered in a sensitivity analysis. In spite of these uncertainties evidence of katabatic cold air flow is given. Received July 29, 1999; revised June 11, 2001; accepted March 14, 2002  相似文献   

20.
The Mediterranean has been identified as particularly vulnerable to climate change, yet a high-resolution temperature reconstruction extending back into the Medieval Warm Period is still lacking. Here we present such a record from a high-elevation site on Mt. Smolikas in northern Greece, where some of Europe’s oldest trees provide evidence of warm season temperature variability back to 730 CE. The reconstruction is derived from 192 annually resolved, latewood density series from ancient living and relict Pinus heldreichii trees calibrating at r1911–2015 = 0.73 against regional July–September (JAS) temperatures. Although the recent 1985–2014 period was the warmest 30-year interval (JAS Twrt.1961–1990 = + 0.71 °C) since the eleventh century, temperatures during the ninth to tenth centuries were even warmer, including the warmest reconstructed 30-year period from 876–905 (+ 0.78 °C). These differences between warm periods are statistically insignificant though. Several distinct cold episodes punctuate the Little Ice Age, albeit the coldest 30-year period is centered during high medieval times from 997–1026 (− 1.63 °C). Comparison with reconstructions from the Alps and Scandinavia shows that a similar cold episode occurred in central Europe but was absent at northern latitudes. The reconstructions also reveal different millennial-scale temperature trends (NEur = − 0.73 °C/1000 years, CEur = − 0.13 °C, SEur = + 0.23 °C) potentially triggered by latitudinal changes in summer insolation due to orbital forcing. These features, the opposing millennial-scale temperature trends and the medieval multi-decadal cooling recorded in Central Europe and the Mediterranean, are not well captured in state-of-the-art climate model simulations.  相似文献   

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