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1.
The Tonle Sap is an invaluable resource for the people of Cambodia, and is a globally significant ecological site. Much of the literature published on the environmental health and management of the lake suggests that its sustainability is threatened by accelerated rates of infilling related to unfettered land-use in the catchment. However, the evidence for supposedly increased sedimentation rates is confused and contradictory, and there have been very few studies that have attempted to actually measure the rate at which sediment is accumulating on the bed of the lake. This research measures long-term sedimentation rates in the Tonle Sap in an attempt to provide an empirically derived baseline against which more recent and allegedly accelerated sedimentation rates can be compared. Radiometric dating techniques (14C, 210Pb, 137Cs) reveal that sediment has been accumulating in the lake at an average long-term rate of less than 1 mm per year. There is a clear and consistent decline in the rate of sediment accumulation in the lake basin over time, with the highest rates recorded in the middle to early Holocene epoch. It is recommended that research be directed toward measuring changes in the morphology of the lake margin over time, rather than focus on changes in the bathymetry of the lake basins themselves, which are here shown to be effectively stable in terms of sediment accumulation.  相似文献   

2.
In 2008, three short sedimentary cores were collected from Nanyihu Lake in the lower Yangtze River Basin using a gravity corer. Heavy metals, including Pb, Cu, Zn, Cr, Ni, Mn, and major elements, including Al, Fe, K, Na, Mg and Ti, were measured. Radionuclides, including 210Pb and 137Cs, were analyzed to date the sediments. The significant Mn enrichment in the uppermost sediments of the three cores did not influence the distribution of Pb, Cu, Zn, Cr and Ni. The Pb, Cu, Zn, Cr and Ni contents have increased over the past 30–40 years. The decline of 206Pb/207Pb ratios toward the surface indicated increasing anthropogenic Pb loading to the lake sediments. However, the heavy metal enrichment was low overall because of the high sediment accumulation rates and the low anthropogenic heavy metal flux into the Nanyihu Lake.  相似文献   

3.
Frozen sediment cores from Lake Pupuke in Auckland City, New Zealand, contain a high resolution decadal to annual scale record of changing lake paleoenvironments and geochemistry that reflects changing landuse and hydrology in the catchment over the past c. 190 years. A reliable chronology is available from AMS 14C and 210Pb dating of the sediments, with the timing of the older part of the record supported by the first appearance of pollen of introduced Pinus and Plantago lanceolata associated with European settlement of Auckland in the early 1840s. Diatom stratigraphy, sediment elemental and carbon isotope geochemistry reflect changes in sediment sources and lake conditions commensurate with European development of the Lake Pupuke catchment, in particular enhanced algal productivity controlled by the influx of nutrients after c. 1920 AD. Attempts to prevent nuisance algal blooms in 1933, 1934 and 1939 using CuSO4 addition produced Cu spikes in the sediment that allowed confirmation of the accuracy of the 210Pb chronology. Hence, the elemental and isotopic composition of the Lake Pupuke sediments reflect the timing of significant anthropogenic activities, rather than climatic variations, that have occurred within the watershed over the past c. 190 years. The comparison of records of land use change in the catchment with the multi-proxy record of changes in the sediments usually allowed unambiguous identification of the signatures of change and their causes.  相似文献   

4.
A simple binary mixing model is used to determine the isotopic ratios of lead (Pb) pollution sources to a lake located near a smelter closed because of excessive Pb aerosols (Horseshoe Lake Madison County, Illinois, USA). As a control, we also examine a relatively unpolluted lake in a rural area of Southern Illinois (Horseshoe Lake Alexander County). Sediment cores were taken from both lakes and analyzed for Pb and Pb isotopes by ICP-MS. The mixing model shows that Madison County Horseshoe Lake had 3 different sources of Pb in its history. The first source is sediment from the Mississippi River with an intermediate 206Pb/207Pb ratio (1.223 ± 0.009) which dominates inputs in pre-settlement times. From 1750 to 1933, the source of pollution Pb has the high 206Pb/207Pb ratio (1.256 ± 0.005) characteristic of ore from the southeast Missouri Pb mines. The most recently deposited pollution Pb comes from a source with a low 206Pb/207Pb ratio (1.202 ± 0.005). This source is similar in isotopic composition to pollution Pb found by several other investigators in the Eastern US and probably represents the mixture of ores used in modern industrial processes. It is unclear from the isotopic composition whether this source at Horseshoe Lake is the local Pb smelter or vehicle exhaust. The sediment core from Horseshoe Lake, Alexander County, shows a less variable isotopic composition. The binary mixing model showed a source composition of 1.225 ± 0.003 before 1850 and 1.231 ± 0.003 after this date. The change does not indicate a pollution source, but may be a shift in the sources of natural sediment with slightly different isotopic ratios to the lake. Our results show the value of simple binary mixing models to reconstruct the isotopic composition of Pb sources to lakes.  相似文献   

5.
Past atmospheric Pb deposition in Lake Qinghai,northeastern Tibetan Plateau   总被引：2，自引：0，他引：2  
Two short sediment cores were recovered from sub-basins of Lake Qinghai, China and were analyzed for concentrations of Pb and 16 other elements to determine historic, regional atmospheric Pb deposition on the Tibetan Plateau. Core chronologies, dating back to the eighteenth century, were established using activities of 210Pb and 137Cs. The 17 elements were divided into three principal components. Variations in concentrations of PC1 elements (Al, Cr, Cu, Fe, K, Mn, Ni, and Ti) demonstrate different patterns between the two cores, and are attributed to different sediment sources in the two sub-basins. PC2 elements (Ba, Ca, Na, and Sr) may be associated with the degree of catchment weathering and/or water chemistry. Four elements (Pb, Zn, P, and Co) are related to both PC1 and PC2, and reflect a mixture of natural and anthropogenic sources. The PC3 element is Mg in the north sub-basin, and is perhaps related to aragonite precipitation and/or increased farming. Elevated Pb concentrations in uppermost sediments of both cores signify a recent regional/global increase in anthropogenic Pb release into the environment. After subtracting lithogenic Pb, derived from rock weathering and/or dust and normalized to the background immobile element Ti, results suggest that excess, anthropogenic Pb is transferred to the lake and its sediments predominantly via the atmosphere. This anthropogenic atmospheric Pb is comparable in magnitude and displays similar variation patterns in the two cores, reflecting regional atmospheric deposition and local erosion. The average anthropogenic Pb deposition rate in Lake Qinghai since the 1960s has been ~12.2 ± 3.5 mg/m2/a, comparable with atmospheric Pb fluxes reported for sites elsewhere in the northern hemisphere.  相似文献   

6.
The global cycling of anthropogenic trace metals intensified during the twentieth century, impacting aquatic systems throughout the world. There are, however, few quantitative records showing the history of this contamination in large rivers. Here we present a well-dated sedimentary record of trace metal accumulation in Lake St. Croix, a natural riverine lake on the St. Croix River (Minnesota and Wisconsin, USA), revealing the history of heavy metal inputs to the river over the past 200 years. Concentrations of Hg, Pb, Ag, Cd, Cr and Zn and stable Pb isotopes were measured in eight 210Pb-dated sediment cores collected from profundal depositional areas throughout the lake. Time trends of trace metal concentrations and accumulation rates differed greatly between the upper lake (above Valley Creek) and the lower lake, reflecting contrasting sediment sources along the flow axis of the lake. For most of the study period (1800–2000 AD), sediment deposited throughout the lake derived almost exclusively from the suspended sediment load carried by the main-stem river into the lake. From 1910 through 1970, however, large inputs of eroded soils and stream channel sediments from side-valley tributaries resulted in greatly increased sediment and trace metal accumulation in the lower lake. Anthropogenic accumulation rates of Hg, Pb, Cd, Zn, and Ag in the upper lake correlate well with those from Square Lake, a small, relatively undisturbed nearby lake that has received trace metal inputs almost exclusively via atmospheric deposition. The similarity of these records suggests that atmospheric deposition was primarily responsible for trace metal accumulation trends in upper Lake St. Croix. Trace metal accumulation in the lower lake was also strongly influenced by atmospherically derived inputs, but metal contributions from native soils were important, as well, during the period of elevated sediment inputs from side-valley tributaries. Concentrations and accumulation rates of trace metals in both upper and lower lake sediments have decreased substantially since the 1970s due to decreased atmospheric inputs and sediment loadings, but accumulation rates remain well above pre-settlement values. Metal inputs to Lake St. Croix have been far lower than those to nearby Lake Pepin, located on the Mississippi River downstream of the Minneapolis-St. Paul metropolitan area, but there nevertheless remains a clear record of anthropogenic impact on the relatively pristine St. Croix River.  相似文献   

7.
Devils Lake is a closed, saline lake in North Dakota; it is typical of lake basins in the Great Plains Region, where windy conditions and fluctuating water-levels disturb sediment and confound chronostratigraphy. Pollen analysis and 210Pb dating of two cores collected from bathymetrically contrasting embayments demonstrate (1) how certain agriculture-related pollen types differ in their value as chronostratigraphic markers, (2) how pollen and 210Pb stratigraphies can be reconciled to determine the approximate depth of sediment mixing, and (3) the importance of coring-site selection, especially in lakes with unstable sedimentary conditions.  相似文献   

8.
Lake Duluti is a small, topographically closed crater lake located on the flanks of Mt Meru, northern Tanzania. Analyses of diatoms in three short sediment cores and four modern samples from Lake Duluti were used to infer past environmental changes. 210Pb and 137Cs activity profiles combined with AMS 14C dates provide the chronological framework. Weak agreement between the 210Pb and 14C records, together with dating uncertainty, precludes construction of precise age models. The modern diatom flora, from plankton and three periphytic habitats, is dominated by Aulacoseira ambigua (Grunow) Simonsen, Gomphonema parvulum (Kützing) Grunow and Nitzschia amphibia Grunow. All three cores display similar stratigraphic succession, but the relative ratio of habitats represented by the diatoms varies substantially between cores. Diatoms indicate that the oldest part of the record is characterized by relatively low lake level and swampy vegetation. In the late nineteenth or early twentieth century there was a rapid lake level rise and the swamp turned into an open-water lake. High lake levels have prevailed since that time.  相似文献   

9.
A high-resolution sedimentological study of Lake Bourget was conducted to reconstruct the flood frequency and intensity (or magnitude) in the area over the last 350 years. Particular emphasis was placed on investigating the spatio-temporal distribution of flood deposits in this large lake basin. The thicknesses of deposits resulting from 30 flood events of the Rhône River were collected over a set of 24 short sediment cores. Deposit thicknesses were compared with instrumental data for the Rhône River discharge for the period from 1853 to 2010. The results show that flood frequency and intensity cannot be reliably reconstructed from a single core because of the inhomogeneous flood-deposit geometry in such a large lake. From all documented flood-deposit thicknesses, volumes of sediment brought into the lake during each flood event were computed through a Kriging procedure and compared with the historical instrumental data. The results show, in this study, that reconstructed sediment volumes are well correlated to maximal flood discharges. This significant correlation suggests that the increase of embankment and dam settlements on the Rhône River during the last 150 years has not significantly affected the transport of the smallest sediment fraction during major flood events. Hence, assessment of the flood-sediment volumes deposited in the large Lake Bourget is the only way to reliably reconstruct the flood frequency and intensity.  相似文献   

10.
澜沧江──湄公河是中国和东南亚地区最为重要的国际河流，目前成为国际上众多国家、国际组织关注和投资的热点地区［１，３］。按亚洲开发银行（ＡＤＢ）组织的“大湄公河次区域合作计划”［４］直接影响地域２３２×１０４ｋｍ２，人口超过２．２亿，大范围内的自然环境、社会和经济状况都将发生巨大变化。１９９５年４月５日下湄公河四国签署的《湄公河流域持续发展合作协定》［５］，为该流域区的持续发展注入了新机。据初步分析，如果以水资源多目标综合利用为目的进行整体规划和管理，将能源开发集中在澜沧江干流和下湄公河支流，在洞里萨湖修建拦河闸堰，在湄公河三角洲修建泄洪道，在大城市与人口和耕地集中而易遭受洪水危害的干流两侧兴建防洪堤，并加强水文、气象预测和预报，则下湄公河流域的电力需求及灌溉、洪水、咸水入侵以及土壤酸性水危害等问题，在很大程度上均可得到解决，无需兴建庞大的下湄公河干流梯级电站（水库），这不仅可以避免大量的资金投入、大规模的移民和土地淹没，而且可以阻止大坝对湄公河水生生物的危害，促进流域持续发展。  相似文献   

11.
Sediment cores from Lake Pepin, a natural lake on the Upper Mississippi River, reveal the historical trends in trace metal use and discharge in the watershed. Lead-210 dated concentration profiles of trace metals (Ag, Cd, Cr, Cu, Hg, Pb, V, Zn) in sediment cores from throughout the lake generally showed low and stable concentrations prior to settlement (circa 1830), peak concentrations between 1940 and 1975, and substantial decreases thereafter. Whole-lake sediment accumulation rates increased greatly over the period of record, from 79,000 metric tons year−1 prior to 1830, to 876,000 metric tons year−1 during the 1990s. Whole-lake accumulation rates of most trace metals peaked in the 1960s but decreased sharply after that. Sediment and trace metal accumulation rates decreased in the downstream direction, and approximately two-thirds of the sediment and trace metal mass accumulated in Lake Pepin since 1800 was deposited in the upper 30% (by area) of the lake. The dramatic declines in trace metal concentrations and accumulation rates in Lake Pepin sediments since 1970 coincide with increased pollution control and prevention efforts throughout the watershed, including the implementation of secondary treatment at a large municipal wastewater treatment plant upstream. This is one of eight papers dedicated to the “Recent Environmental History of the Upper Mississippi River” published in this special issue of the Journal of Paleolimnology. D.R. Engstrom served as guest editor of the special issue.  相似文献   

12.
We studied sediment cores from four Florida (USA) lakes that have received groundwater hydrologic supplements (augmentation) for >30 years to maintain lake stage. Top samples (0–4 cm) from sediment cores taken in Lakes Charles, Saddleback, Little Hobbs, and Crystal had 226Ra activities of 44.9, 17.5, 7.6, and 8.5 dpm g−1, respectively, about an order of magnitude greater than values in deeper, older deposits. The surface sample from Lake Charles yielded the highest 226Ra activity yet reported from a Florida lake core. Several lines of evidence suggest that groundwater augmentation is responsible for the high 226Ra activities in recent sediments: (1) 226Ra activity in cores increased recently, (2) the Charles, Crystal, and Saddleback cores display 226Ra/210Pb disequilibrium at several shallow depths, suggesting 226Ra entered the lakes in dissolved form, (3) cores show recent increases in Ca, which, like 226Ra, is abundant in augmentation groundwater, and (4) greater Sr concentrations are associated with higher 226Ra activities in recent Charles and Saddleback sediments. Sr concentrations in Eocene limestones of the deep Floridan Aquifer are high relative to Sr concentrations in surficial quartz sands around the lakes. Historical water quality inferences for the lakes were based on diatom assemblages in sediments. Recent alkalization in Lakes Charles, Saddleback, Little Hobbs, and Crystal was inferred from weighted-averaging calibration (WACALIB). The lakes also show recent trophic state increases based on WACALIB-derived estimates for limnetic total P. Although residential and agricultural sources might contribute to increased P loading, P in augmentation waters probably has had significant influence on eutrophication. Dystrophic diatoms were abundant in the early history of Lakes Saddleback, Little Hobbs, and Crystal, which suggests that these lakes contained more tannic waters during the past than at present, perhaps as a consequence of greater inflows from surrounding wetlands. Ionic content of lake waters increased, as indicated by diatom autecological analysis. Recent geochemical and biological changes detected in cores from these lakes probably are a result of deliberate groundwater augmentation, although inputs of groundwater pumped for agricultural and residential development in the watersheds also might have contributed to limnological changes.  相似文献   

13.
The level of Kluane Lake in southwest Yukon Territory, Canada, has fluctuated tens of metres during the late Holocene. Contributions of sediment from different watersheds in the basin over the past 5,000 years were inferred from the elemental geochemistry of Kluane Lake sediment cores. Elements associated with organic material and oxyhydroxides were used to reconstruct redox fluctuations in the hypolimnion of the lake. The data reveal complex relationships between climate and river discharge during the late Holocene. A period of influx of Duke River sediment coincides with a relatively warm climate around 1,300 years BP. Discharge of Slims River into Kluane Lake occurred when Kaskawulsh Glacier advanced to the present drainage divide separating flow to the Pacific Ocean via Kaskawulsh and Alsek rivers from flow to Bering Sea via tributaries of Yukon River. During periods when neither Duke nor Slims river discharged into Kluane Lake, the level of the lake was low and stable thermal stratification developed, with anoxic and eventually euxinic conditions in the hypolimnion.  相似文献   

14.
Southeastern Missouri has been a major Pb mining region since 1720 AD. Missouri mines produce a Pb ore that has a distinctive elevated 206Pb/207Pb isotopic ratio (>1.30) that is easily recognized in Pb-contaminated sediments. Five 210Pb dated sediment cores from Horseshoe Lake, Madison County, Illinois were examined to reconstruct Pb-contamination of the site from southeastern Missouri mines and from a local Pb smelter located adjacent to the lake. Pb concentrations increased in the cores from 5 ppm in the early 1800s to approximately 350 ppm in the late 1940s and 1950s. Pb concentrations in recently deposited sediment range from 100 to 300 ppm depending on the location within the lake. Throughout the 1800s and early 1900s the 206Pb/207Pb ratios in the sediment cores increased indicating contamination from southeastern Missouri (mean = 1.243). After the local smelter began recycling lead-acid storage batteries in the 1950s, the 206Pb/207Pb ratio declined (mean = 1.224) suggesting contamination of Horseshoe Lake with Pb from sources elsewhere around the world. The results of this study demonstrate how isotopic ratios of Pb can be used to reconstruct historical anthropogenic contamination.  相似文献   

15.
There is an important volume of published information on Lac Dufault (Québec) which describes the history of metal inputs over 70 years and the changes that occurred in the lake as a result of this contamination. We used this abundant source of chronological markers to test the hypothesis that lake sediments can provide true historical records of trace metal loading from metal mining. Sediment cores were obtained from the deepest zone of the lake (19 m). The sediments were dated using 210Pb and 137Cs and they were analyzed for total elemental concentrations (Ca, Cd, Cu, Fe, P, Pb, S, Zn). Metal profiles in the sediment core preserved the distinct signatures of different mine exploitations documented in the lake watershed. In particular, the core recorded: the beginning of industrialization in 1926; increasing sedimentation rates associated with perturbations in the lake watershed; the maximum of sediment [Cu] and the contemporary exploitation of ore bodies rich in Cu; the maximum of sediment [Fe] and the contemporary production of pyrite by a mining operation; the low sediment [Cu] and [Zn] in the 1950s and the low contemporary production of these metals by mining operations; the maximum of sediment [Cd] and the contemporary production of Cd by a subsequent mining operation. Anomalies in the distribution of 214Pb activities in sediments reflected the intensity of acid mine drainage (AMD). There is good evidence that the lake resisted acidification from this AMD for the last thirty years. Overall, our results support the thesis that profiles of sedimentary Cd, Cu, Zn, Pb and Fe levels reflect the past history of metal input to Lac Dufault.  相似文献   

16.
This paper reports results and analysis of210Pb-activity measurements in 51 lake-sediment cores from 32 lakes in the four PIRLA (Paleoecological Investigations of Recent Lake Acidification) project regions (Adirondack Mountains [New York], Northern New England, Northern Florida, and the Northern Great Lakes States). General application of the Constant Rate of Supply (Constant Flux) model for210Pb dating is valid for lakes in the PIRLA study, although application of the model is equivocal in a few lakes.210Pb inventories and profiles are replicable among closely spaced cores within a lake. Specific210Pb activity in surface sediments is negatively correlated with bulk sediment accumulation rate in seepage lakes, but not in drainage lakes. Drainage lakes with lower pH have lower unsupported210Pb inventories in sediments, but the relationship does not occur in seepage lakes.210Pb profiles in only seven of the cores, all from either the Adirondacks or the northern Great Lakes states, exhibit exponential decay curves. Deviations from an exponential profile include a flattening of the profile in the top few cm or excursions of one or a few measurements away from an exponential curve.210Pb dates typically agree with other chronostratigraphic markers, most of which are subject to greater uncertainty. Several hypotheses, including sediment mixing, hydrologic regime, sediment focusing, and acidification, are proposed to explain variation of210Pb distribution among lakes and regions. Hydrologic factors exert control on unsupported210Pb inventories in PIRLA lakes, and there is a strong focusing effect in drainage lakes but a weak focusing effect in seepage lakes.This is the third of a series of papers to be published by this journal following the 20th anniversary of the first application of210Pb dating of lake sediments. Dr P. G. Appleby is guest editing this series.  相似文献   

17.
Long-term changes in sediment and phosphorus loading to the upper Mississippi River were quantified from an array of 25 sediment cores from Lake Pepin, a large natural impoundment downstream of the Minneapolis-St Paul metropolitan area. Cores were dated and stratigraphically correlated using 210Pb, 137Cs, 14C, magnetic susceptibility, pollen analysis, and loss-on-ignition. All cores show a dramatic increase in sediment accumulation beginning with European settlement in 1830. Accumulation rates are highest and show the greatest post-settlement increases in the upper end of the lake. Present-day sediment-phosphorus concentrations are roughly twice those of pre-settlement times, and the Fe/Al-bound fraction makes up a greater portion of the total. Diatom assemblages record a marked increase in nutrient availability over the last 200 years, changing from clear-water benthic forms and mesotrophic planktonic taxa in pre-settlement times to exclusively planktonic assemblages characteristic of highly eutrophic conditions today. Lake-water total-phosphorus concentrations, estimated by weighted averaging regression and calibration, increased from 50 to 200 μg l−1 during this period. Sediment loading to Lake Pepin from the Mississippi River has increased by an order of magnitude since 1830. Modern fluxes are about 900,000 metric tons annually, and are more than 80% detrital mineral matter. About 17% of the lake’s volume in 1830 has been replaced by sediment, and at current accumulation rates the remainder will be filled in another 340 years. Phosphorus accumulation in Lake Pepin sediments has increased 15-fold since 1830, rising from 60 to 900 metric tons annually. This rise represents a sevenfold increase in phosphorus loading from the Mississippi River coupled with more efficient retention of phosphorus inflows by bottom sediments. More efficient trapping of phosphorus in Lake Pepin over the last century resulted from higher rates of sediment burial. The most dramatic changes in nutrient and sediment inputs to Lake Pepin have occurred since 1940, although gradual increases began shortly following European settlement. Sediment accumulation rates rose sharply between 1940 and 1970 and then leveled off, while phosphorus inflows record their largest increases after 1970. This is one of eight papers dedicated to the “Recent Environmental History of the Upper Mississippi River” published in this special issue of the Journal of Paleolimnology. D. R. Engstrom served as guest editor of the special issue.  相似文献   

18.
Lake St. Croix is a natural impoundment of the lowermost 37 km of the St. Croix River in Minnesota and Wisconsin, making this one of a few large river systems in the world possessing a long-term depositional basin at its terminus. The river’s relatively pristine condition led to its designation as a National Scenic Riverway in 1968, but increasing urbanization in its lower reaches has raised concerns about impacts on water quality. This study was initiated to reconstruct historical loadings of suspended sediment and phosphorus (P) from the sediment record in Lake St. Croix. Twenty-four piston cores, with an average length of 2 m, were collected along eight transects of the lake. Dated chronologies from 210Pb, 137Cs and 14C were used to calculate the rate of sediment accumulation in the lake over the past 100+ years. Diatom microfossil analysis was used to reconstruct historical lakewater P concentrations over the same time period, and sediment P analysis quantified the amount of P trapped in lake sediments. Using a whole-lake mass balance approach, the loading of sediment and P to Lake St. Croix over the last 100+ years was calculated. Beginning in 1850, sediment accumulation increased dramatically to a peak in 1950–1960 of eight times background rates prior to European settlement. The peak is driven largely by sediment contributions from small side-valley catchment tributaries to the downstream half of the lake. The total P load to the lake increased sharply after 1940 and remains high, at around four times the level of pre-European settlement conditions. The timing of peak sediment and P loading to the lake shows that early settlement activities, such as logging and the conversion of forest and prairie to agricultural land between 1850 and 1890, had only modest impacts on the lake. By contrast, the mid-1900s brought major increases in sediment and P loading to the lake, suggesting that relatively recent activities on the landscape and changes to nutrient balances in the watershed have caused the current eutrophic condition of this important recreational and natural resource. This is one of eight papers dedicated to the “Recent Environmental History of the Upper Mississippi River” published in this special issue of the Journal of Paleolimnology. D. R. Engstrom served as guest editor of the special issue.  相似文献   

19.
Reconstructing recent limnological history often relies on lead-210 dating to accurately ascribe a chronology to a sediment profile. In Lake Okeechobee, Florida, a large, shallow subtropical lake that may experience severe mixing, multiple dating methods are required to confirm that conformable sedimentation has been preserved and that the assumptions of the 210Pb method are satisfied. This study uses stratigraphic profiles of heavy metals, 137Cs, PCBs and pollen as independent dating markers to validate the sediment chronology as determined by 210Pb for three cores from the central mud zone of the lake. Unsupported 210Pb and most dating markers show distinct concentration/depth profiles, suggesting that the sediments have not been severely mixed for at least the last 75 years. Onset and maximum activity of the radioisotope 137Cs in the cores coincides with the 210Pb-dated interval of 1945–1970. This agrees well with the known timing of atmospheric deposition of 137Cs that resulted from above-ground nuclear testing during late 1940s until 1963. Sediment core profiles of atmospherically deposited metals such as Zn and Pb, which reflect regional increases during industrialization and decreases after regulation in the 1970s, exhibit expected concentration increases and peaks coinciding within 5–15 years of the predicted 210Pb dates. Uranium, a contaminant in some phosphate fertilizers, shows large concentration increases at core depths dated to be about 1950 by 210Pb, matching the intensification of agriculture after WWII. PCBs, which are expected to peak in the early 1970s, were measured in one core, and the observed peak corresponds to a 210Pb date of about 1960. Pollen makers were unable to verify specific events, but increases in disturbance taxa and declines in native types correspond generally with the expected dates assigned by 210Pb dating. Conformity between the 210Pb defined dates and independent markers of < ±15 years confirm that Lake Okeechobee sediments do preserve a sequential and reliable stratigraphic history of the lake, useful for reconstructing past limnological conditions.  相似文献   

20.
A combination of water and sediment chemistry was used to investigate carbonate production and preservation in Lake Pumayum Co (altitude 5,030 m a.s.l.), south Tibet, China. We compared the chemical composition of lake water in various parts of the lake with that of input rivers and found that the loss of Ca2+ results from calcite sedimentation induced by evaporation and biogenic precipitation. This is supported by evaporation data from the catchment and δ18O measurements on water. Results suggest that CaCO3 is the predominant carbonate in this lake. There is a positive correlation in the sediments among concentrations of total inorganic carbon (TIC), Ca, total organic carbon (TOC), and total nitrogen, confirming that most carbonates in sediment are endogenic. The Jiaqu River is the largest inflow to Lake Pumayum Co and has a strong influence on both lake water chemistry and sediment composition. The river and lake bathymetry influence carbonate sedimentation by affecting water flow velocity and growing conditions for macrophytes. Different carbon contents and relationships between TIC and TOC in the two long cores from different depths in the lake reveal that hypolimnetic conditions also influence carbonate precipitation and preservation.  相似文献   

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