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1.
Present study has continued the investigation on distribution of mercury in estuarine sediments of Patos Lagoon which began whilst assessing the after-effect of enormous accidental discharge of sulfuric acid into the estuary. An attempt to evaluate the contribution of anthropogenic effluents on mercury pollution in sediments was undertaken. The effluents from Rio Grande City sewages were categorized into four groups based on their sources. Comparison of mercury concentrations from those, indicated that domestic effluent was prevalent. Apparent geographic controls of effluent locations enriched in mercury on zones of polluted estuarine sediments were also revealed. Insufficient control on waste collecting and absence of sewage treatment are considered the principal causes of mercury pollution in estuarine sediments.  相似文献   

2.
This paper proposes an explanation of the mud deposits on the inner Shelf of Cassino Beach, South Brazil, by using computational modeling. These mud deposits are mainly formed by sediments delivered from Patos Lagoon, a coastal lagoon connected to the Shelf, next to Cassino Beach. The deposits are characterized by (soft) mud layers of about 1 m thick and are found between the −5 and −20 isobaths.  相似文献   

3.
Riverine waters bring to seas a variety of suspended materials, which are ultimately deposited on the shelf or exported to the deep ocean. Investigation of the mineralogical contents of these continental-borne constituents on seafloors may reveal valuable information about the environmental conditions in the drainage basin. In this note we report results of X-ray diffraction and other analysis of sediments in bottom samples collected on the continental shelf under influence of the Plata River and the Patos Lagoon, in South America. The analysis reveals that non-clay materials are mostly concentrated south of 33°S, while clay sediments are relatively more abundant further north. We propose that such distributions are controlled by the circulation pattern and water mass distribution of the lower and upper layers, respectively.  相似文献   

4.
Concentrations of selected heavy metals (Cu, Pb, Zn, Cd, Cr, Ni and Fe) in surface sediments from nine sites in western Xiamen Bay and its vicinity were studied in order to understand current metal contamination due to urbanization and economic development in Xiamen, China. The sediment samples were collected in December 2004 and July 2005 respectively in order to examine temporal variations. In this study, we found that heavy metal concentrations in surface sediments sampled in the western Xiamen Bay and adjacent Maluan Bay and Yuandang Lagoon varied from 19 to 97mg kg(-1) for Cu, 45 to 60mg kg(-1) for Pb, 65 to 223mg kg(-1) for Zn, 0.11 to 1.01mg kg(-1) for Cd, 37 to 134mg kg(-1) for Cr, 25 to 65mg kg(-1) for Ni and 3.08 to 4.81% for Fe. Although all metal concentrations in sediments meets Chinese National Standard Criteria for Marine Sediment Quality, both metal enrichment factors (EF) and geoaccumulation index (I(geo)) show that Pb contamination exists in the entire study area and contamination of other metals are also present in some locations depending on the sources, of which sewage outlets and commercial ports are the main sources of contaminants to the area. This study shows that using the sediment quality standard criteria only to assess sediments cannot properly reflect sediment contamination. A multiple approaches should be applied for the sediment quality assessment.  相似文献   

5.
《Marine pollution bulletin》2014,78(1-2):209-212
This study reports results of analysis of sediment cores collected from the Patos Lagoon estuary. This estuary receives materials from land runoff into Patos and Mirim lagoons and from exchange with the adjacent South Atlantic Ocean through a narrow inlet. Sediment from these sources is mostly natural, but additional contributions associated with source/activities related to the port of Rio Grande. The aim of this study was to estimate rates of accumulation of the sediments and to assess the significance of metal inputs from these activities relative to natural inputs. Our results indicate an average sedimentation rate of 0.3 cm/yr and that the transport of suspended solids from offshore sources into the estuary was enhanced after the deepening of the channel and construction of the breakwaters (in the early 1900). Results for metal accumulation in these sediments suggest that there have been only minor enrichments which can be attributed to anthropogenic sources.  相似文献   

6.
This paper evaluates the concentration of Polyaromatic hydrocarbons - PAHs in the Estuarine area of the Patos Lagoon, more precisely in a local named "Saco do Laranjal" in Pelotas City (southern Brazil). The samples were collected in May 2008. The concentrations of 16 US-EPA priority polycyclic aromatic hydrocarbons (PAHs) were determined by gas chromatography with a mass spectrometry detector (GC/MS). The sum of PAHs concentration ranged from 7.3 to 92.8μgkg(-1) in dry weight. The positive correlation (Pearson test) between the total organic material (TOM) and the total PAH concentration (0.98) suggests that TOM plays an important role in controlling the PAHs levels in the sediments. According to the observed ratios of individual PAHs, the contamination in the studied area is originated, predominantly pyrolytic sources. The values found are considered under normal levels and indicates a not impacted area.  相似文献   

7.
The single, long and narrow channel that usually connects choked coastal lagoons to the ocean can serve as a natural hydraulic low-pass filter that reduces or eliminates tidal and subtidal effects inside the lagoon. This study proposes an alternative method of estimating the attenuation of the tidal and subtidal oscillations throughout the Patos Lagoon estuary. The attenuation is estimated for conditions of contrasting river runoff and weather (summer and winter). A high-pass/low-pass filter (fast fourier transformation technique – FFT) is applied to time series of sea-surface elevation (SSE) measured at the mouth of the Patos Lagoon. The resulting high-frequency (tidal) and low-frequency (subtidal) signals are used in independent simulations to force the TELEMAC-2D model. Attenuation of the tidal and subtidal signals throughout the estuary is estimated by applying cross-spectral analysis between the model-generated SSE time series at different locations throughout the estuary and the filtered SSE time series measured at the mouth. Results from the proposed method suggest that: (1) the low-frequency (subtidal) oscillations are less attenuated and propagate further than the high-frequency (tidal) oscillations in the Patos Lagoon estuary; (2) the filtering capability of the Patos Lagoon estuary is expected to follow a seasonal pattern, although further investigations on an interannual time scale are recommended in order to confirm this hypothesis; (3) the influence of the oceanic boundary processes on the SSE dynamics of the lagoon is restricted to the lower estuary. Further inland, the local forcing generated by the wind and freshwater input is likely to be the main forcing effect controlling the dynamics of the system. The proposed method proved to be an efficient and alternative way of estimating the attenuation of energy in the tidal and subtidal bands throughout the access channel of a choked coastal lagoon located in an area of reduced tidal influence.Responsible Editor: Iris Grabemann  相似文献   

8.
The heavy metal inventory and the ecological risk of the estuarine sediments in Hailing Bay, an important maricultural zone along the southern coast of China, were investigated. Results show that the surface sediments were mainly polluted by As (2.17-20.34 mg/kg), Ni (1.37-42.50mg/kg), Cu (1.21-58.84 mg/kg) and Zn (11.69-219.22 mg/kg). Furthermore, the aquafarming zone was significantly more polluted than the non-aquafarming zone, and cluster analysis suggested additional sources of heavy metal input in the aquafarming zone. As, Cr, Cu, Ni, Pb and Zn were mainly present in the non-bioavailable residual form in the surface sediments, whereas Cd was predominantly in the highly mobile acid soluble and reducible fractions. The ecological risk of the polluted sediments stemmed mainly from Cd, and from As, Cu and Pb to less degrees. The highest potential risks occurred near the aquaculture base, indicating the need to control heavy metal inputs from aquafarming activities.  相似文献   

9.
The Curonian Lagoon is the biggest fresh water basin in Lithuania influenced by the exchange of the fresh Nemunas and other smaller rivers’ water and saline water of the Baltic Sea. The lagoon ecosystem is influenced by fresh, brackish and brackish water masses. A long-term water balance of the Curonian Lagoon was calculated for the period of 1960–2009. The sum river inflow is 21.784 km3/year, precipitation—1.199 km3/year, evaporation—1.007 km3/year, inflow of brackish water from the Baltic Sea to the Curonian Lagoon—6.171 km3/year, and fresh water runoff from the Curonian Lagoon to the Baltic Sea—27.642 km3/year. The lagoon water balance elements have been influenced by climate change. The water balance forecasting has been performed for the period of 2011–2100. The climate change impact on the water balance of the Lagoon has been evaluated using Global Climate Models (ECHAM5 and HadCM3), greenhouse gas emission scenarios (A2, A1B and B1), and hydrological modelling by Hydrologiska Byrans Vattenbalansavdelning (HBV) software. One scenario was selected for the prediction of the Baltic Sea water level. Considerable changes of the Curonian Lagoon water balance are forecasted in the 21st century. Increase of weather temperature and changes in precipitation will influence the elements of water balance of the Curonian Lagoon. In the period of 2011–2100, the river inflow and outflow from the Baltic Sea into the Lagoon will decrease respectively by 20.4 and 16.6% in comparison with the baseline period (1961–1990). The amount of precipitation and evaporation will increase respectively by 3.8 and 25.1%, while inflow from the Baltic Sea into the Curonian Lagoon will increase up to 39.7% in comparison with the baseline period.  相似文献   

10.
The Southern Brazilian Shelf (SBS) is a freshwater-influenced region, but studies on the dynamics of coastal plumes are sparse and lack in space-time resolution. Studies on the dynamics of the Patos Lagoon plume are even more limited. The aim of this paper is to investigate the influence of the principal physical forcing for the formation and behavior of the Patos Lagoon coastal plume. The study is carried out through 3D numerical modeling experiments and empirical orthogonal function (EOF) analysis. Results showed that the amount of freshwater is the principal physical forcing controlling the plume formation. The Coriolis effect enhances the northward transport over the shelf, while the tidal effects contribute to intensify horizontal and vertical mixing, which are responsible for spreading the freshwater over the shelf. The wind effect, on the other hand, is the main mechanism controlling the behavior of the Patos Lagoon coastal plume over the inner SBS in synoptic time scales. Southeasterly and southwesterly winds contribute to the northeastward displacement of the plume, breaking the vertical stratification of the inner continental shelf. Northeasterly and northwesterly winds favor ebb conditions in the Patos Lagoon, contributing to the southwestward displacement of the plume enhancing the vertical stratification along and across-shore. The EOF analysis reveals two modes controlling the variability of the plume on the surface. The first mode (explaining 70% of the variability) is associated to the southwestward transportation of the plume due to the dominance of north quadrant winds, while the second mode (explaining 19% of the variability) is associated to the intermittent migration of the plume northeastward due to the passage of frontal systems over the area. Large scale plumes can be expected during winter and spring months, and are enhanced during El Niño events.  相似文献   

11.
Extensive mud deposits superimposed on the predominantly sandy inner continental shelf adjacent to the Patos Lagoon estuary, indicates that the Lagoon is a potential source of fine sediments to the coastal sedimentary system. The lagoon is large and shallow, and the water movement is mainly controlled by wind-driven set-up and set-down. The mean river inflow is around 2000 m3 s−1, although peak flow rates exceeding 20,000 m3 s−1 have been observed during El Niño periods. Though the tidal elevations are small, tidal velocities in the lagoon's inlet can be significant due to the large extension of the backwaters. Moreover, significant exchange flows can be generated between the estuary and coastal area due to barotropic pressure gradients established as a function of wind and freshwater discharge. The predominant net flow is seawards, but opposite near-bed flows due to pronounced vertical salinity stratification can also be observed. The coastal area is characterized by small tidal effects, large scale ocean circulation, wind-induced residual flows and wave-driven currents, where the waves originate from swell or are locally generated.  相似文献   

12.
The concentrations, compositional profiles, and potential ecological risk of polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs), polychlorinated biphenyls (PCBs) and polychlorinated naphthalenes (PCNs) in sediments of the Daliao River Estuary were investigated. Total concentrations of PCDD/Fs, PCBs, and PCNs were in the range of 11.3-133.2 ng/kg dry weight (dw), 1 971-37 632 ng/kg dw and 33.1-284.4 ng/kg dw, respectively. The total TEQ values varied from 0.37 to 4.08 ng/kg dw, with the dominant contributions by PCDD/Fs, then by PCBs and PCNs. The spatial distributions of PCDD/Fs, PCBs and PCNs in the river estuary were much related to hydrodynamic conditions. The risk of contamination to the deeper sea was increased in the flood seasons. Moreover, our data confirmed that both organic matter in sediments and molecular properties of dioxin-like compounds were the factors which strongly influenced the partition behavior of these dioxin-like compounds between sediments and water phase in the estuarine zone.  相似文献   

13.
The two-dimensional barotropic, hydrodynamic and transport model MOHID is applied to the Patos Lagoon system using a nested modelling approach to reproduce both the lagoon and estuary hydrodynamics. A new Lagrangian oil spill model is presented and used to simulate a hypothetical oil spill in the estuary. Hydrodynamic fields are validated and used to force the oil model. Results show that the hydrodynamics of this system is mainly controlled by the wind and freshwater discharge. The dispersion, concentration and thickness evolution of the oil in the first day after the spill is determined by the equilibrium between these two factors. The freshwater discharge is the major factor controlling the oil dispersion for discharges greater than 5000 m3 while the wind assumes control for lower discharge amounts. The results presented are a first step toward a coastal management tool for the Patos Lagoon.  相似文献   

14.
The focus of this work is to explore the use of the netted whelk, Nassarius reticulatus (L.), as an indicator of mercury (Hg) contamination, by assessing the concentration of Hg in the sediments and in the whelk along the entire Portuguese coast. Total Hg concentrations ranged from below the detection limit (0.01 ng absolute mercury) up to 0.87 mg kg(-1) dry weight (dwt) in sediments and between 0.06 and 1.02 mg kg(-1) (dwt) for organisms, with no significant differences between males and females. Although organic mercury was not detected in the sediments, it represented, on average, 52% of the total Hg in the whelk tissues, and as high as 88% in some cases, suggesting mercury accumulation from dietary intake. Significant negative correlations were found between the total Hg concentrations in the sediments and the log(10) of Hg concentrations in whelk tissues males (r=-0.64; P<0.01) and females (r=-0.52; P<0.01) indicating that the species is a poor indicator of Hg contamination. Nevertheless, since the highest concentrations of organic mercury in the whelk tissues were found in the least contaminated areas, this species must be highly relevant in the trophic web, namely on the possible biomagnification of mercury. The high dietary mercury accumulation from feeding on carrion and the low bioavailability of mercury to whelks in estuarine sediments may be the basis of the mercury accumulation pattern in N. reticulatus.  相似文献   

15.
Surface sediment samples in the Laptev Sea have average 137Cs content of 7.1 Bq kg(-1), a value intermediate between that of the western Kara Sea (23 Bq kg(-1) and the East Siberian Sea (4.2 Bq kg-'). Both surface sediment content and sediment inventory of 137Cs in the Laptev Sea sediments show significant variability, and the influence of a variety of environmental factors.137Cs concentrations in the Laptev Sea surface sediments range from 0.8 to 16 Bq kg(-1). There is a marked increase in 137Cs content of surface sediment samples collected near the Lena River delta, and a local enrichment in the 137Cs inventories at these sites is also evident. Fine-grained mixed-layer illite/ smectite rich sediments in the estuary provide effective adsorption sites to fix 137Cs, in spite of desorption processes associated with low salinities in estuarine mixing. The Lena River-Laptev Sea mixing zone is a major site of sea-ice production. River and shelf sediments are incorporated into sea-ice formed in this region (Holmes and Creager, 1974). The irregular 137Cs activity profiles of the Lena River estuary cores indicate disturbance or removal of 137Cs-laden sediments via sea-ice related processes. Lena River and Estuary sediments may have served as a secondary source (i.e. other than direct fallout) of 137Cs in sea-ice. North-east of the Lena River estuary, sediment contains a thin layer of 137Cs-bearing material over an erosion surface. The 137Cs-laden surface layer may be the result of transient deposition of estuarine sediments being delivered by sea-ice or spring floods.  相似文献   

16.
含铁盐的高砷沉积物中,上覆水p H值和总磷浓度的变化对砷迁移的影响尚不明确.以含铁盐的高砷沉积物为研究对象,通过实验观测其暴露在不同p H值的上覆水及经过不同初始p H值、不同初始总磷浓度的溶液淋洗后,沉积物中砷的迁移规律.结果表明:当沉积物暴露在p H=10和11的上覆水时,分别在第11 d和第6 d后,沉积物中的砷溶出速度突然增大,说明当沉积物处于强碱性上覆水环境中,碱性越强,砷的溶出速度越快、溶出量越大.从室内实验条件的角度来看,上覆水的碱化有可能会增加沉积物中砷溶出的风险.而上覆水p H值在4~8之间时,上覆水的酸碱度对沉积物砷的迁移影响较小.此外,当上覆水总磷浓度不高于0.5 mg/L时,磷的竞争吸附对砷的迁移影响较小.  相似文献   

17.
Water column profiles and near-bed time series of pressure, current velocity, suspended-particulate matter (SPM) concentration and seawater temperature and salinity were collected during three short cruises carried out in May 2005 in the shoreface and inner shelf area adjacent to Cassino Beach, southern Brazil. The measurements were part of the Cassino Experiment, a project conducted at an open, sandy coastal area known for the occurrence of patches of fairly large amounts of muddy sediments that are sporadically fluidized, transported onshore and eventually stranded on the beach. The study area is close to the Patos Lagoon mouth, being influenced by its water and suspended-sediment discharge. The presence of the Patos Lagoon outflow on the inner shelf was detected in one of the cruises (May 13) through measurements of near-surface salinity: while close to shore salinity was 29.4, a minimum value of 13.8 was measured at ∼10 km from the coast. Four days later, no trace of the plume was detected in the area. Regarding seawater temperature, no large temporal or spatial variability was documented with measured values ranging from 19.3 to 20 °C. Water column currents were prominently to N and NE, except at the outermost station, located ∼42 km from the coast, where NW-directed flows were observed at surface and mid-depth. Maximum near-bed current velocity oscillated between 18 and 42 cm s−1 in the east–west direction and between 14 and 42 cm s−1 in the north–south direction. Near-surface concentration of SPM oscillated between 11 and 99 mg L−1, in general one order of magnitude lower than near-bed values. However, near-bed concentration of SPM showed large spatial variability: the highest value (2200 mg L−1) was yielded by a water sample collected at ∼8 m water depth, at a station located ∼2 km away from the shoreline; two water samples collected 500 m, apart from this station, yielded SPM concentrations of 148 and 205 mg L−1, one order of magnitude lower. Spectral analyses of near-bed current speed and SPM concentration indicate the relevance of oscillations in the low-frequency (<0.05 Hz) range. Detailed sampling of bottom sediment indicated that in May 2005 the mud patch was centered at ∼8.5 m water depth.  相似文献   

18.
洞庭湖平原中小型湖群沉积物中砷污染特征与评价   总被引：1，自引：1，他引：0  
本文研究了洞庭湖平原10个中小型湖泊沉积物砷的空间分布特征,并采用地累积指数法对其污染进行了评价.结果表明:各湖表层沉积物中砷浓度在10.1 -33.7 mg/kg之间变化,平均值为15.8 mg/kg,砷含量水平较低;在空间上表层沉积物中砷含量次序为岳阳南湖＞芭蕉湖＞黄盖湖＞安乐湖＞毛里湖＞柳叶湖＞东湖＞珊珀湖＞大通...  相似文献   

19.
Beside damages of infrastructure in industrial regions, extreme floods can cause contamination with particle‐bound pollutants, e. g., due to erosion of soils and sediments. In order to predict contamination with inorganic pollutants, the transport and fate of arsenic, lead, and mercury during a fictive flood event of River Vereinigte Mulde in the region of Bitterfeld (Germany) with 200 years recurrence time was modeled. The finite element model system Telemac2D, which is subdivided into a hydrodynamic (Telemac‐2D), a transport (Subief‐2D), and a water quality module (wq2subief) was applied. The transport and water quality model models were calibrated using results of sediment trap exposures in the floodplain of River Vereinigte Mulde. Model results exhibited that the spatial patterns of particle‐associated arsenic and lead concentrations significantly changed. Extended, mostly agriculturally used areas showed arsenic and lead concentrations between 150 and 200 mg kg–1 and 250 and 300 mg kg–1, respectively, while urban areas were to a great extent spared from high contamination with arsenic and lead. Concentrations of particle‐associated mercury showed a pattern distinct from those of arsenic and lead. Outside of small patches with concentrations up to 63 mg kg–1, concentrations of particle‐associated mercury remained close to zero. Differences in the spatial patterns of the three pollutants regarded mainly arise from significantly different initial and boundary conditions. Sensitivity analyses of initial and boundary conditions revealed a high sensitivity of particle‐bound pollutant concentrations, whereas the sensitivities of concentrations of suspended sediments and soluble pollutants were mediocre to negligible.  相似文献   

20.
Concentrations of trace metals (Zn, Cr, Cu, V, Cd and Pb), total organic carbon (TOC), black carbon (BC) and their granulometry were examined in 25 surface sediment samples from the northern Bering Sea, Chukchi Sea and adjacent areas. Trace metal concentrations in the sediments varied from 21.06-168.21 mg kg(-1) for Zn, 8.91-46.94 mg kg(-1) for Cr, 2.69-49.39 mg kg(-1) for Cu, 32.46-185.54 mg kg(-1) for V, 0.09-0.92 mg kg(-1) for Cd, and 0.95-15.25 mg kg(-1) for Pb. The geoaccumulation index (Igeo) indicated that trace metal contamination (Zn and Cd) existed in some stations of the study area. The distribution of grain size plays an important role in influencing the distribution of trace metals (Zn, Cr, Cu, V, and Pb) in sediments from the Chukchi Sea and adjacent areas.  相似文献   

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