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1.
The evolution of smoke plume over European Russia (ER) during the massive forest and peatbog fires of summer 2010 has been studied using observations of aerosol optical depth (AOD) from MODIS instruments (both Aqua and Terra platforms), objective analysis of meteorological fields performed at the Russian Hydrometeorological Research Center, NCEP/NCAR reanalysis, as well as upper air data. A relation between the structure inhomogeneities of the AOD field and regional atmospheric circulation has been found. It is shown that, on August 5–9, 2010, the maximum of smoke pollution did complete turn around Moscow, while remaining at a distance of 200 to 650 km from the megacity. Both regionally averaged shortwave aerosol radiative forcings (ARFs) at the top and the bottom of the atmosphere are estimated for the period of extreme smoke pollution over ER. The spatial distributions of ARF values over the territory of the region and the estimates of the local and spatially distributed thermal effects of smoke aerosol are given. It is shown that, on August 5–9, 2010, the spatial distribution of AOD and the calculated thermal effects of smoke aerosol were in agreement with the spatial distributions of air-temperature anomalies observed in the lower 1.5-km layer of the atmosphere. MODIS’s AOD data obtained during the wildfires were validated by AOD observations from the CIMEL sun photometer operated at the AERONET station Zvenigorod.  相似文献   

2.
We have investigated the variability of smoke aerosol absorbing ability with variations in the content of brown carbon (BrC) and black carbon (BC). Using monitoring data on radiative characteristics of smoke aerosol at AERONET stations and the spatial distribution of aerosol optical depth (AOD) obtained by the MODIS spectrometer (Terra satellite), we have detected large-scale smokes during boreal forest fires in Russia and Canada (1995–2012). The spatial distribution (50°–70° N, 95°–125° W) and temporal variability (at AERONET station Fort McMurray) of AOD during the smoking of a part of Canada in July 2012 have been analyzed. AOD probability distributions for July 14–18, 2012, and an estimate of aerosol radiative forcing of smoke aerosol at the upper boundary of the atmosphere have been obtained. We have proposed a technique for the diagnostics of BrC and BC in smoke aerosol particles from the spectral dependence of the imaginary part of the refractive index. At a wavelength of 440 nm, the contributions of BrC and BC to the smokeaerosol absorbing abitity can be comparable in magnitude. In many cases, the absorption spectra of smoke aerosol can be adequately approximated by either power or exponential functions. The presence of BrC in smoke-aerosol particles highly extends the variety of observed absorption spectra in a smoky atmosphere and spectral dependences of single scattering albedo. In the spectral range of 440–1020 nm, the radiative characteristics of smoke aerosol are largely contributed by its fine mode.  相似文献   

3.
气象条件对青岛地区气溶胶光学特性的影响   总被引：8，自引：0，他引：8  
利用 2 0 0 2年 4月至 2 0 0 3年 10月多波段太阳光度计资料和同期的气象观测资料 ,分析了不同气象条件下青岛气溶胶光学特性的变化。气象条件的转变与青岛地区气溶胶光学特性之间具有很好的响应关系 :南风盛行时会加大光学厚度 ,并增强气溶胶对 >5 0 0nm波段太阳辐射的散射能力 ;轻雾和霾在青岛气溶胶光学厚度中占有较大比重 ,而霾对 <5 0 0nm波段辐射的散射能力较强。  相似文献   

4.
dimethylsulphide (DMS)的海空通量是海洋生物气溶胶的主要来源之一,对气候（特别是北冰洋的气候）具有重要的辐射影响。利用卫星数据得到的气溶胶光学深度(AOD)作为气溶胶负荷的代表,在夏季和秋季表现的尤其明显。春季海冰的融化是北极气溶胶前体的重要来源。然而,早春的高浓度气溶胶可能与南方大陆污染的平流有关(北极霾)。更高的AOD通常在研究区域的南部出现。海冰浓度(SIC)和AOD呈正相关,而云盖(CLD)和AOD则呈负相关。SIC和CLD的季节性峰值均在AOD峰值的前一个月。AOD与SIC之间存在强烈的正相关关系。融冰与叶绿素（CHL)几乎在3月至9月呈正相关,但与春季和初夏的AOD呈负相关。春季和初夏较高的AOD有可能是由融冰和春季强风在该地区的结合影响。由于春季风的升高和冰的融化,在春季出现了DMS通量的峰值。从3月到五月,DMS浓度和AOD及融冰都呈正相关。早秋季升高的AOD可能与浮游植物合成的生物气溶胶的排放有关。到2100年,格陵兰海的DMS通量将增加3倍以上。生物气溶胶的显著增加可以部分抵消格陵兰海的增温现象。  相似文献   

5.
利用专门为太阳能资源评估应用的 WRF-Solar数值模式系统,结合 MODIS 气溶胶光学厚度（AOD550 nm）数据,设置了5种山东区域总辐射模拟方案,使用山东济南、福山、吉县3个太阳辐射站总辐射观测数据,对晴天、阴天、雨天以及四季代表月等逐时总辐射模拟结果进行了对比检验。 结果表明：WRF-Solar数值模式对总辐射模拟能力在晴天和少云天最好,阴雨天较差,四季代表月中,天气过程较少的秋季和冬季模拟效果较好,春季次之,夏季相对较差;晴天和少云天、阴天和雨天以及不考虑天气过程的四季代表月所有日条件下,长、短波辐射方案分别采用RRTMG方案、new Goddard 方案,积云对流参数化方案均采用Grell 3D集合方案,同时使用AOD550 nm的气溶胶数据的总辐射模拟能力最强;WRF-Solar模式中加入 MODIS 气溶胶光学厚度资料后,山东区域晴天总辐射模拟结果明显改善,秋季、冬季代表月亦明显改善,但阴天和雨天总辐射模拟结果改善不明显,低能见度日总辐射模拟结果有所改善。  相似文献   

6.
由多波段天空辐射计观测的太阳直接辐射和散射辐射计算得到2006年春季22个晴天的大气气溶胶光学厚度(AOD),利用OMI(臭氧监测仪)的气溶胶指数(AI)线性插值得到相应22 d的气溶胶指数,说明AOD与AI具有较好的相关关系,并拟合出两者的线性关系式.分析AOD与实测水平能见度的关系,说明春季在少云或无云天气,大气中气溶胶含量高是导致能见度水平下降的主要原因.根据2个不同的能见度公式,分别由浑浊度系数和消光系数来计算22 d的水平能见度,并与实际观测值做相关,得到相关系数分别为0.764,0.760.当气溶胶标高取1.3 km时,由消光系数计算得到的水平能见度整体小于实测水平能见度;由浑浊度系数计算得到的能见度有11 d大于实测水平能见度,另外11 d小于s实测水平能见度.  相似文献   

7.
Peculiarities of the formation of carbon gas and fine aerosol emissions into the atmosphere during wildfires are analyzed. A prompt satellite monitoring system and technique for the assessment of burnt areas and volumes of CO2, CO, and PM2.5 emissions from wildfires are described. The results of satellite monitoring of the Russian Federation and some Russian regions for different months over 2010–2014 are given; burnt areas and volumes of carbon gas and aerosol emissions throughout the entire territory are assessed. The peculiarities of seasonal frequencies of wildfires and volumes of hazardous gas and fine aerosol emissions in the regions under study are identified.  相似文献   

8.
Methods and algorithms for the retrieval of optical characteristics of the aerosol atmosphere and underlying surface by data from a multispectral satellite sensor (MSSS) are described. A procedure for the joint processing of MSSS and multizonal imaging system (MZIS) data is proposed and described with the aim of retrieving the albedo of the Earth’s surface with a high spatial resolution. In this case the spectral optical characteristics of the aerosol atmosphere are retrieved by MSSS data in the visible range of 400–700 nm. According to these results, transmission functions of the atmosphere in MZIS spectral channels are calculated and an atmospheric correction of MZIS data is performed. The accuracy of determining the albedo of the underlying surface in spectral channels of MZIS with high-spatial-resolution is estimated.  相似文献   

9.
针对大气校正常使用的基于查找表的方法建表速度缓慢、查找精度低等问题,提出在6S大气校正模型的基础上,以气溶胶厚度为自变量对大气参数进行拟合的算法,使用该算法对GF-1多光谱影像进行大气校正研究。对半球反射率、路径辐射项等效反射率、大气透过率3个大气参数使用三次多项式进行拟合,拟合后的决定系数都达到了0. 999 8;根据拟合结果使用MODIS气溶胶产品作为输入,逐像元计算大气参数,并对影像进行大气校正,将校正结果与FLAASH模型校正结果进行对比。结果表明,该算法能有效校正大气对GF-1多光谱影像的影响,并与FLAASH校正结果具有很好的一致性。  相似文献   

10.
Estimates of some aerosol and radiation characteristics of the atmosphere in the summer of 2010 are obtained according to the results of the measurements made at the Meteorological Observatory (MO) at Moscow State University and are compared with the results of the measurements performed in 2002 and 1972 during the forest and peat fires. In contrast to 1972 and 2002, the period under study in 2010 is characterized by a greater frequency of the highest class of fire danger according to Nesterov, higher aerosol optical depths of the atmosphere up to 4.6, and a more significant weakening of solar radiation in different spectrum regions. In 2010 the smoke aerosol caused losses of the total shortwave radiation of 33%, visible radiation of 39%, ultraviolet radiation of 300–380 nm of 51%, and erythemal radiation of 63%. At the same time, an increase in the downward long-wave radiation to 40–50 W/m2 under extreme aerosol optical depths is recorded.  相似文献   

11.
The results of an analysis of variations in the optical depth of a vertical atmospheric column on the basis of a 30-year (1976–2006) series of observations obtained by the Russian actinometric network are generalized. This analysis is based on the Atmosphere Transparency special-purpose database created at the Voeikov Main Geophysical Observatory on the basis of observational data obtained at the actinometric stations of the Russian Hydrometeorological Research Center. The general regularities of spatial variations in the atmospheric optical depth (AOD) over Russia are revealed: there is a monotonic decrease from the southwest to the northeast, with localized areas having different aerosol loads due to the global and regional factors of their formation. A spatiotemporal structure of the anomalies of AOD annual values within the time interval under consideration, including the El Chichon (1982) and Pinatubo (1991) eruptions, is studied.  相似文献   

12.
A method for reconstructing the parameters of postvolcanic stratospheric aerosol from the results of joint measurements of the aerosol backscattering coefficient with lidar systems based on the Nd:YAG laser and the aerosol extinction coefficient with the SAGE III satellite instrumentation is developed. The most informative set of optical characteristics is determined for each of the microphysical parameters under consideration (concentration, surface area, volume, and effective size of particles of the fine and coarse aerosol fractions). Multiple polynomial regressions between optical and microphysical characteristics of aerosol are obtained. These regressions make it possible to determine the microphysical characteristics of aerosol within a wide range without solving incorrect inverse problems. The results are compared with independent experimental data. The errors of reconstructing microphysical parameters of aerosol are estimated for different situations in the stratosphere. The influence of the shape of particles of the dust fraction on the results of a reconstruction of the microphysical parameters of aerosol is considered.  相似文献   

13.
The aerosol longwave radiative forcing of the atmosphere and heating rate of the near-surface aerosol layer are estimated for the extreme smoke conditions in the Moscow region in summer 2010. Thermal radiation fluxes in the atmosphere are determined using the integral transmission function and semiempirical aerosol model developed on the basis of standard aerosol models and measurements at the Zvenigorod Scientific Station, Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences. The aerosol radiative forcing reached 33 W/m2 at the lower atmospheric boundary and ranged between–1.0 and 1.0 W/m2 at the upper atmospheric boundary. The heating rate of the 10-m atmospheric layer near surface was up to 0.2 K/h during the maximum smoke conditions on August 7–9. The sensitivity of the aerosol longwave radiative forcing to the changes in the aerosol absorption coefficient and aerosol optical thickness are estimated.  相似文献   

14.
The influence of the aerosol component on the total transmission of sounding IR radiation is analyzed. The emissions of both industrial and natural origins into the atmosphere were regarded as the medium. It is noted that, in studying the radiative transport through gas-aerosol mixtures, it is necessary to take into account both molecular absorption and scattering from aerosol particles. It is shown that there are certain boundary values of the microphysical parameters of aerosol where it is sufficient to take into account only one of the above-mentioned factors of radiation extinction. The quantitative values of the parameters of an aerosol medium, on the basis of which the solution of the transport equation can be significantly simplified, are given.  相似文献   

15.
气溶胶的光学厚度与反射率比的处理方法   总被引：2，自引：0，他引：2  
气溶胶光学厚度与气溶胶反射率比都是大气校正所需的重要大气参数，同时也是海洋水色卫星主要的数据产品，它们的测量精度将直接到卫星数据产品正演的精度和卫星数据产品的应用。文章在简述气溶胶光学厚度与气溶胶反射率比的基本测量原理和处理方法的基础上，结合多次试验数据结果进行简要的评价。  相似文献   

16.
A combined mathematical model has been developed to reproduce space and time variations in the concentrations of multicomponent gas constituents and aerosols in the atmosphere on both regional and urban scales. This model contains blocks of transport of gas constituents and aerosols in the atmosphere with consideration for homogeneous binary nucleation, the kinetic processes of condensation/evaporation and coagulation, chemical processes occurring in both gas and liquid phases, and the processes of mass exchange during the gas-droplet (particle) interaction. A nonhydrostatic model of atmospheric mesoscale processes is used to calculate the fields of meteorological elements and turbulent characteristics. The generation of new-phase particles from precursor gases by the mechanism of homogeneous binary nucleation and their interaction with background aerosol are considered. The results of numerical experiments are compared with the data obtained from field observations of both space and time variations in the concentrations of gas constituents and aerosols and in the ionic content of aerosol particles over the Baikal region under the influence of emissions from powerful industrial sources.  相似文献   

17.
The behavior of the vertical aerosol structure (profiles of the ratio of the coefficients of the backward total and molecular scattering) in the height interval 30–80 km is analyzed from the results of lidar observations in Kamchatka over the period from October 2007 through December 2009. The obtained data revealed a regular two-layer aerosol structure in this height range with the maxima of the ratio of the scattering coefficients in the upper stratosphere at heights 35–50 km and in the mesosphere at heights of 60–75 km, as well as a relation between seasonal variations in the aerosol stratification and the circumpolar vortex affecting dynamic processes in the atmosphere of midlatitudes. The procedure of including the aftereffect of the Hamamatsu-M8259-01 PEM, which influences the error in the calculation of the ratio of scattering coefficients, is described.  相似文献   

18.
气溶胶光学厚度的时空变化   总被引：2，自引：0，他引：2  
在大气中气溶胶微粒是一种重要的大气微量成分。气溶胶光学厚度也是大气校正所需的重要大气参数，同时也是海洋水色卫星主要的数据产品。由于气溶胶光学厚度的时空变化较大，所以如何准确获取大气校正和卫星数据产品真实性检验所需的气溶胶光学厚度则是至关重要的。在简述气溶胶光学性质的基础上，并结合2002年6月HY—1南海实验数据来阐述现场气溶胶光学厚度的准确获取。  相似文献   

19.
A thermodynamics-microphysics model of the formation and evolution of stratospheric clouds is developed. This model was integrated into the global chemistry-climate model of the lower and middle atmosphere. Model experiments on the study of the evolution of the gas and aerosol compositions of the Arctic and Antarctic atmosphere were performed. The results of an investigation into the observed differences of changes in the contents of gaseous impurities and aerosol in polar regions showed that the presence of nitrification in the Antarctic and its absence in the Arctic are the main factors controlling distinctions between the formation of a full-value ozone hole in the Antarctic and only occasional “mini-holes” in the Arctic.  相似文献   

20.
The microphysical characteristics of aerosol were measured in the atmospheric surface layer simultaneously over the center of Moscow and its vicinity (Zvenigorod Scientific Station, Obukhov Institute of Atmospheric Physics, Russian Academy of Sciences) from June 15 to June 30, 2009, in order to compare the mass concentrations, particle-size distribution functions, and elemental compositions of aerosol over the megapolis and the background zone. During the fire peak of 2010, on August 8, aerosol samples were taken in the center of Moscow and their chemical composition was determined. Comparing results obtained from the simultaneous measurements of the concentrations of aerosol and its elemental composition made it possible to determine their interdiurnal variability, which suggests that the features of time variations are of a regional character and they are determined mainly by the dynamics of the synoptical processes of air-mass exchange. The chemical composition of obtained samples was determined using the method of atomic absorption spectrometry. The measurement results obtained in June 2009 revealed an increase in the content of anthropogenic elements in the atmosphere over Moscow when compared to their content in the atmosphere over the background zone. In Moscow, during the summer fires of 2010, the concentration of sulfur exceeded its concentration in June 2009 by an order of magnitude, and the concentrations of Na, Mg, Al, Si, K, Ca, and Fe increased several times. The mean mass concentration of aerosol amounted to 917 μg/m3 in August 2010 and 50–70 μg/m3 in June 2009.  相似文献   

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