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1.
Abstract— Analyses of the isotopic compositions of multiple elements (Mo, Zr, and Ba) in individual mainstream presolar SiC grains were done by resonant ionization mass spectrometry (RIMS). While most heavy element compositions were consistent with model predictions for the slow neutron capture process (s‐process) in low‐mass (1.5–3 M⊙) asymptotic giant branch stars of solar metallicity when viewed on single‐element three‐isotope plots, grains with compositions deviating from model predictions were identified on multi‐element plots. These grains have compositions that cannot result from any neutron capture process but can be explained by contamination in some elements with solar system material. Previous work in which only one heavy element per grain was examined has been unable to identify contaminated grains. The multi‐element analyses of this study detected contaminated grains which were subsequently eliminated from consideration. The uncontaminated grains form a data set with a greatly reduced spread on the three‐isotope plots of each element measured, corresponding to a smaller range of 13C pocket efficiencies in parent AGB stars. Furthermore, due to this reduced spread, the nature of the stellar starting material, previously interpreted as having solar isotopic composition, is uncertain. The constraint on 13C pocket efficiencies in parent stars of these grains may help uncover the mechanism responsible for formation of 13C, the primary neutron source for s‐process nucleosynthesis in low‐mass stars.  相似文献   

2.
Abstract— We have measured the titanium isotopic compositions of 23 silicon carbide grains from the Orgueil (CI) carbonaceous chondrites for which isotopic compositions of silicon, carbon, and nitrogen and aluminum‐magnesium systematics had been measured previously. Using the 16 most‐precise measurements, we estimate the relative contributions of stellar nucleosynthesis during the asymptotic giant branch (AGB) phase and the initial compositions of the parent stars to the compositions of the grains. To do this, we compare our data to the results of several published stellar models that employ different values for some important parameters. Our analysis confirms that s‐process synthesis during the AGB phase only slightly modified the titanium compositions in the envelopes of the stars where mainstream silicon carbide grains formed, as it did for silicon. Our analysis suggests that the parent stars of the >1 μm silicon carbide grains that we measured were generally somewhat more massive than the Sun (2–3 M⊙) and had metallicities similar to or slightly higher than solar. Here we differ slightly from results of previous studies, which indicated masses at the lower end of the range 1.5–3 M⊙ and metallicities near solar. We also conclude that models using a standard 13C pocket, which produces a good match for the main component of s‐process elements in the solar system, overestimate the contribution of the 13C pocket to s‐process nucleosynthesis of titanium found in silicon carbide grains. Although previous studies have suggested that the solar system has a significantly different titanium isotopic composition than the parent stars of silicon carbide grains, we find no compelling evidence that the Sun falls off of the array defined by those stars. We also conclude that the Sun does lie on the low‐metallicity end of the silicon and titanium arrays defined by mainstream silicon carbide grains.  相似文献   

3.
We studied 14 presolar SiC mainstream grains for C‐, Si‐, and S‐isotopic compositions and S elemental abundances. Ten grains have low levels of S contamination and CI chondrite‐normalized S/Si ratios between 2 × 10?5 and 2 × 10?4. All grains have S‐isotopic compositions compatible within 2σ of solar values. Their mean S isotope composition deviates from solar by at most a few percent, and is consistent with values observed for the carbon star IRC+10216, believed to be a representative source star of the grains, and the interstellar medium. The isotopic data are also consistent with stellar model predictions of low‐mass asymptotic giant branch (AGB) stars. In a δ33S versus δ34S plot the data fit along a line with a slope of 1.8 ± 0.7, suggesting imprints from galactic chemical evolution. The observed S abundances are lower than expected from equilibrium condensation of CaS in solid solution with SiC under pressure and temperature conditions inferred from the abundances of more refractory elements in SiC. Calcium to S abundance ratios are generally above unity, contrary to expectations for stoichiometric CaS solution in the grains, possibly due to condensation of CaC2 into SiC. We observed a correlation between Mg and S abundances suggesting solid solution of MgS in SiC. The low abundances of S in mainstream grains support the view that the significantly higher abundances of excess 32S found in some Type AB SiC grains are the result of in situ decay of radioactive 32Si from born‐again AGB stars that condensed into AB grains.  相似文献   

4.
Abstract— Primitive meteorites contain a few parts per million (ppm) of pristine interstellar grains that provide information on nuclear and chemical processes in stars. Their interstellar origin is proven by highly anomalous isotopic ratios, varying more than 1000-fold for elements such as C and N. Most grains isolated thus far are stable only under highly reducing conditions (C/O > 1), and apparently are “stardust” formed in stellar atmospheres. Microdiamonds, of median size ～ 10 Å, are most abundant (～ 400–1800 ppm) but least understood. They contain anomalous noble gases including Xe-HL, which shows the signature of the r- and p-processes and thus apparently is derived from supernovae. Silicon carbide, of grain size 0.2–10 μm and abundance ～ 6 ppm, shows the signature of the s-process and apparently comes mainly from red giant carbon (AGB) stars of 1–3 solar masses. Some grains appear to be ≥109 a older than the Solar System. Graphite spherules, of grain size 0.8–7 μm and abundance <2 ppm, contain highly anomalous C and noble gases, as well as large amounts of fossil 26Mg from the decay of extinct 26Al. They seem to come from at least three sources, probably AGB stars, novae, and Wolf-Rayet stars.  相似文献   

5.
Abstract— The classical model of s-process nucleosynthesis, based on the concept of a steady neutron flux under astrophysical conditions pertaining to the He-burning phase of red giant stars, has successfully described observed isotopic abundances and provided information on the physical conditions of the s-process environment. Because most of the isotopes on the s-process path are stable, their relevant nuclear parameters can be measured in the laboratory so that as more accurate elemental abundance and neutron capture cross-section data have become available, the classical model has been tested under increasingly stringent conditions. Accurate determinations of the neutron capture cross sections at appropriate astrophysical conditions for the Ba isotopes have shown that the abundance of the s-only isotope 136Ba is under-produced by ～20% according to the classical model. This paper describes the accurate assessment of the meteoritic abundance of Ba by the stable isotope dilution mass spectrometric technique, based on the Cl carbonaceous chondrites Orgueil and Ivuna. Repeated analyses of these two Cl chondrites give an abundance that is identical to the presently accepted solar system value for Ba within experimental errors, which indicates a deficiency in the classical model. When combined with similar data for the s-only nuclides 116Sn and 142Nd, it is apparent that the classical model, having served a valuable function for many years, must be replaced by stellar models that more accurately reflect the dynamic nature of the He-burning phase in red giant stars, in particular, during the thermal pulses of low-mass asymptotic giant branch (AGB) stars.  相似文献   

6.
Abstract— We have determined the recoil losses from silicon carbide (SiC) grain‐size fractions of spallation Ne produced by irradiation with 1.6 GeV protons. During the irradiation, the SiC grains were dispersed in paraffin wax in order to avoid reimplantation into neighboring grains. Analysis for spallogenic 21Ne of grain‐size separates in the size range 0.3 to 6 μm and comparison with the 22Na activity of the SiC + paraffin mixture indicates an effective recoil range of 2–3 μm with no apparent effect from acid treatments, which are routinely used in the isolation of meteoritic SiC grains. Our results indicate that the majority of presolar SiC grains in primitive meteorites, which are micrometer‐sized, will have lost essentially all spallogenic Ne produced by cosmic‐ray interaction in the interstellar medium. This argues against the validity of previously published presolar ages of Murchison SiC (～10 to ～130 Ma, increasing with grain size; Lewis et al., 1994), where recoil losses had been based on calculated recoil energies. It is argued that the observed variations in meteoritic SiC grain‐size fractions of 21Ne/22Ne ratios are more likely due to the effects of nucleosynthesis in the He‐burning shell of the parent AGB stars which imposes new boundary conditions on nuclear parameters and stellar models. It is suggested that spallation‐Xe produced on the abundant Ba and REE in presolar SiC, rather than spallogenic Ne, may be a promising approach to the presolar age problem. There is a hint in the currently available Xe data (Lewis et al., 1994) that the large (>1 μm) grains may be younger than the smaller (<1 μm) grains. The retention of spallogenic 21Ne produced by the bombardment of SiC grains of different grain sizes with 1.6 GeV protons, avoiding reimplantation into neighboring grains by dispersing the SiC grains in paraffin wax, has been derived from a comparison of mass spectrometrically determined 21Ne, retained in the grains, with the 22Na activity of the grains‐plus‐paraffin mixture. Compared to estimates of retention used in previous attempts to determine presolar ages for SiC (Tang and Anders, 1988b; Lewis et al., 1990, 1994), the results indicate significantly lower values. They do, however, agree with retention as expected from previous measurements of recoil ranges in similar systems (Nyquist et al., 1973; Steinberg and Winsberg, 1974). The prime reason for the discrepancy must lie in the energy of the recoiling nuclei entering in the calculation of retention by Tang and Anders (1988b), which is based on considerations by Ray and Völk (1983). Based on the results, it appears questionable that spallation contributes significantly to the observed variations of 21Ne/22Ne ratios among various SiC grain‐size separates (Lewis et al., 1994). We rather suggest that the variations, just as it has been observed for Kr and Ba already (Lewis et al., 1994; Prombo et al., 1993), have a nucleosynthetic origin. Confirmation needs input of improved nuclear data and stellar models into new network calculations of the nucleosynthesis in AGB stars of elements in the Ne region. Finally we argue that, to determine presolar system irradiation effects, spallation Xe is more favorable than is Ne, primarily because of smaller recoil losses for Xe. Although preliminary estimates hint at the possibility that the larger (>1 μm) grains are younger than the smaller (<1 μm) ones, the major uncertainty for a quantitative evaluation lies in the exact composition of the Xe‐N component thought to originate from the envelope of the SiC grains' parent stars.  相似文献   

7.
Abstract— Carbon stars are an important source of presolar TiC, SiC, and graphite grains found in meteorites. The elemental abundances in the stellar sources of the SiC grains are inferred by using condensation calculations. These elemental abundances, together with C isotopic compositions, are used to identify possible groups of carbon stars that may have contributed SiC grains to the presolar dust cloud. The most likely parent stars of meteoritic SiC mainstream grains are N-type carbon stars and evolved subgiant CH stars. Both have s-process element abundances higher than solar and 10 < 12C/13C < 100 ratios. The J stars and giant CH stars, with solar and greater than solar abundances of s-process elements, respectively, are good candidate parents for the ‘A’ and ‘B’ SiC grains with low 12C/13C ratios. A special subgroup of CH giant stars with very large 12C/13C ratios could have parented the ‘Y’ SiC grains with 12C/13C ratios > 100. The carbon star population (e.g., N, R, J, CH groups) needed to provide the observed SiC grains is compared to the current population of carbon stars. This comparison suggests that low-metallicity CH stars may have been more abundant in the past (>4.5 Ga ago) than at present. This suggestion is also supported by condensation-chemistry modeling of the trace element patterns in the SiC grains that shows that subsolar Fe abundances may be required in the stellar sources for many SiC grains. The results of this study suggest that presolar SiC grains in meteorites can provide information about carbon stars during galactic evolution.  相似文献   

8.
Abstract— We report measurements of isotopic ratios of C, N, Mg, Si, Ca, Ti, Cr, and Fe in bulk samples (aggregates of many grains) of up to seven different fractions of silicon carbide (SiC), ranging from 0.38 to 3.0μm in diameter, from the Murchison CM2 carbonaceous chondrite. Ratios of 12C/13C range from 37 to 42 and 14N/15N ratios from 370 to 520, within the range of single‐grain measurements on coarser samples and in agreement with an asymptotic giant branch (AGB) star origin of most of the grains. Variations among size fractions do not show any simple trend and can be explained by varying contamination with isotopically normal material. Silicon isotopic ratios vary only little and, with one exception, lie to the right of the singlegrain mainstream correlation line. This might indicate a higher percentage of the minor populations Y and Z among finer grain‐size fractions. All bulk samples have large 26Mg excesses attributed to the presence of short‐lived 26Al at the time of grain formation. Inferred 26Al/27Al ratios are much larger than those measured in single larger mainstream grains. This is probably because of the presence of SiC grains of type X; we obtain an estimate of 0.4 for their 26Al/27Al ratio. Our Ca‐isotopic measurements, the first made on presolar SiC grains, show excesses in 42Ca and 43Ca, which is in general agreement with theoretical expectations for AGB stars. Calcium‐44 excesses are much larger than expected and are probably because of X grains, which have high44Ca excesses because of the decay of short‐lived 44Ti produced in supernova explosions. We arrive at an estimate of 0.014 for the initial 44Ti/48Ti ratio of the X grains, within the range obtained from previous single X grain measurements. The Ti‐isotopic ratios of the bulk samples show a V‐shaped pattern with excesses of all isotopes relative to 48Ti. Isotopes 46Ti, 47Ti, and 50Ti show excesses relative to the correlation between Ti and Si ratios for single grains and are in general agreement with theoretical models of s‐process nucleosynthesis in AGB stars. In contrast, 49Ti does not show any excess relative to the singlegrain data; it also fails to agree with theory, which predicts much larger excesses than observed. Measured 53Cr/52Cr and 57Fe/56Fe ratios are normal within errors. The first result is expected even for Cr in AGB star envelopes, but the second result suggests that most of the Fe analyzed originates from contamination. We have found no simple trends in isotopic composition with respect to grain size that can be interpreted in terms of nucleosynthetic origin, unlike the results for Kr, Xe, Ba, and Sr.  相似文献   

9.
Abstract– The composition of the most primitive solar system condensates, such as calcium‐aluminum‐rich inclusions (CAIs) and micron‐sized corundum grains, show that short‐lived radionuclides (SLR), e.g., 26Al, were present in the early solar system. Their abundances require a local or stellar origin, which, however, is far from being understood. We present for the first time the abundances of several SLR up to 60Fe predicted from stars with initial mass in the range approximately 7–11 M⊙. These stars evolve through core H, He, and C burning. After core C burning they go through a “Super”‐asymptotic giant branch (Super‐AGB) phase, with the H and He shells activated alternately, episodic thermal pulses in the He shell, a very hot temperature at the base of the convective envelope (approximately 108 K), and strong stellar winds driving the H‐rich envelope into the surrounding interstellar medium. The final remnants of the evolution of Super‐AGB stars are mostly O–Ne white dwarfs. Our Super‐AGB models produce 26Al/27Al yield ratios approximately 0.02–0.26. These models can account for the canonical value of the 26Al/27Al ratio using dilutions with the solar nebula of the order of 1 part of Super‐AGB mass per several 102 to several 103 of solar nebula mass, resulting in associated changes in the O‐isotope composition in the range Δ17O from 3 to 20‰. This is in agreement with observations of the O isotopic ratios in primitive solar system condensates, which do not carry the signature of a stellar polluter. The radionuclides 41Ca and 60Fe are produced by neutron captures in Super‐AGB stars and their meteoritic abundances are also matched by some of our models, depending on the nuclear and stellar physics uncertainties as well as the meteoritic experimental data. We also expect and are currently investigating Super‐AGB production of SLR heavier than iron, such as 107Pd.  相似文献   

10.
Abstract— We report the first measurements of lithium and boron isotope ratios and abundances measured in “gently separated” presolar SiC grains. Almost all analyses of presolar SiC grains since their first isolation in 1987 have been obtained from grains that were separated from their host meteorite by harsh acid dissolution. We recently reported a new method of “gently” separating the grains from meteorites by using freeze‐thaw disaggregation, size, and density separation to retain any nonrefractory coatings or alteration to the surfaces of the grains that have been acquired in interstellar space. Nonrefractory coats or amorphized surfaces will almost certainly be removed or altered by the traditional acid separation procedure. High Li/Si and B/Si ratios of up to ～10?2 were found implanted in the outer 0.5 μm of the grains dropping to ～10?5 in the core of the grains. 7Li/6Li and 11B/10B ratios indistinguishable from solar system average values were found. Analyses obtained from SiC grains from the acid dissolution technique showed isotope ratios that were the same as those of gently separated grains, but depth profiles that were different. These results are interpreted as evidence of implantation of high velocity (1200–1800 km s?1) Li and B ions into the grains by shock waves as the grains traveled through star‐forming regions some time after their condensation in the outflow of an AGB star that was their progenitor. The results are in line with spectroscopic measurements of Li and B isotope ratios in star‐forming regions and may be used to infer abundances and isotopic sources in these regions.  相似文献   

11.
Abstract— Concentrations of the trace elements Mg, Al, Ca, Ti, V, Fe, Sr, Y, Zr, Ba and Ce were determined by ion microprobe mass spectrometry in 60 individual silicon carbide (SiC) grains (in addition, Nb and Nd were determined in 20 of them), from separate KJH (size range 3.4–5.9 μm) of the Murchison carbonaceous meteorite, whose C-, N- and Si-isotopic compositions have been measured before (Hoppe et al., 1994) and provide evidence that these grains are of stellar origin. The selected SiC grains represent all previously recognized subgroups: mainstream (20 < 12C/13C < 120; 200 < 14N/15N; Si isotopes on slope 1.34 line), grains A (12C/13C < 3.5), grains B (3.5 < 12C/13C < 10), grains X (15N excesses, large 28Si excesses) and grains Y (150 < 12C/13C < 260; Si isotopes on slope 0.35 line). Data on these grains are compared with measurements on fine-grained SiC fractions. Trace-element patterns reflect both the condensation behavior of individual elements and the source composition of the stellar atmospheres. A detailed discussion of the condensation of trace elements in SiC from C-rich stellar atmospheres is given in a companion paper by Lodders and Fegley (1995). Elements such as Mg, Al, Ca, Fe and Sr are depleted because their compounds are more volatile than SiC. Elements whose compounds are believed to be more refractory than SiC can also be depleted due to condensation and removal prior to SiC condensation. Among the refractory elements, however, the heavy elements from Y to Ce (and Nd) are systematically enriched relative to Ti and V, indicating enrichments by up to a factor of 14 of the s-process elements relative to elements lighter than Fe. Such enrichments are expected if N-type carbon stars (thermally pulsing AGB stars) are the main source of circumstellar SiC grains. Large grains are less enriched than small grains, possibly because they are from different AGB stars. The trace-element patterns of subgroups such as groups A and B and grains X can at least qualitatively be understood if grains A and B come from J-type carbon stars (known to be lacking in s-process enhancements shown by N-type carbon stars) or carbon stars that had not experienced much dredge-up of He-shell material and if grains X come from supernovae. However, a remaining puzzle is how stars become carbon stars without much accompanying dredge-up of s-process elements.  相似文献   

12.
Abstract— A wide range of stellar nucleosynthetic sources has been analyzed to derive their contributions of short‐lived and stable nuclei to the presolar cloud. This detailed study is required to infer the most plausible source(s) of short‐lived nuclei through a critical comparison among the various stellar sources that include AGB stars, novae, supernovae II, Ia, and Wolf‐Rayet stars that evolved to supernovae Ib/c. In order to produce the canonical value of 26Al/27Al in the early solar system, almost all stellar sources except low‐mass AGB stars imply large isotopic anomalies in Ca‐Al‐rich inclusions (CAIs). This is contrary to the observed isotopic compositions of CAIs. The discrepancy could impose stringent constraints on the formation and thermal evolution of CAIs from different chondrites. Among the various stellar scenarios, the injection of short‐lived nuclei into the previously formed solar protoplanetary disc by a massive star of an ad hoc chosen high‐injection mass cut is a possible scenario. There is a possibility of the contribution of short‐lived nuclides by a 1.5–3 M⊙ AGB star as it implies the smallest shift in stable isotopes. A low‐mass AGB star of relatively low metallicity would be even a better source of short‐lived nuclei. However, this scenario would require independent gravitational collapse of the presolar cloud coupled with ambipolar diffusion of magnetic flux. Alternatively, numerous scenarios can be postulated that involve distant (≥10 pc) massive stars can contribute 60Fe to the presolar cloud and can trigger its gravitational collapse. These scenarios would require production of 26Al and 41Ca by irradiation in the early solar system. Significant production of 26Al and 60Fe can be explained if massive, rotating Wolf‐Rayet stars that evolved to supernovae Ib/c were involved.  相似文献   

13.
We carried out Fe isotopic analyses on 21 O‐rich presolar grains from the Acfer 094 ungrouped carbonaceous chondrite. Presolar grains were identified on the basis of oxygen isotopic ratios, and elemental compositions were measured by Auger spectroscopy. The Fe isotopic measurements were carried out by analyzing the Fe isotopes as negative secondary oxides with the NanoSIMS to take advantage of the higher spatial resolution of the Cs+ primary ion beam. Our results demonstrate the effectiveness of this approach for measuring both 54Fe/56Fe and 57Fe/56Fe. The ion yield for FeO– is significantly lower than for Fe+, but this is not a serious limitation for presolar silicate grains with Fe as a major element. Most of the grains analyzed are ferromagnesian silicates, but we also measured four oxide grains. Iron contents are high in all of the grains, ranging from 10 to 40 atom%. Three of the grains belong to oxygen isotope Group 4. All of them have 54Fe/56Fe and 57Fe/56Fe ratios that are solar within errors, consistent with an origin in the outer zones of a Type II supernova, as indicated by their oxygen isotopic compositions. The remaining grains belong to oxygen isotope Group 1, with origins in low‐mass AGB stars. The majority of these also have solar 54Fe/56Fe and 57Fe/56Fe ratios. However, four grains are depleted in 57Fe; one is also slightly depleted in 54Fe. Current AGB models predict excesses in 57Fe with 54Fe/56Fe ratios that largely reflect the metallicity of the parent star. While the solar 57Fe/56Fe ratios are consistent with formation of the grains in early third dredge‐up episodes, these models cannot account for the grains with 57Fe depletions. Comparison with galactic evolution models suggests formation of these grains from stars with significantly subsolar metallicity; however, these models also predict large depletions in 54Fe, which are not observed in the grains. Thus, the isotopic compositions of these grains remain unexplained.  相似文献   

14.
太阳系原始同位素组成是研究太阳系起源和演化的基础。评述了太阳星云的原始放射性核素丰度特征及解释此丰度特征的分子云自增丰模型、AGB星污染模型和散裂反应模型。陨石包体中前太阳矿物颗粒的同位素组成异常表明,前太阳颗粒中低密度石墨、X型碳硅石可能来源于超新星爆发,而AGB星或红巨星被认为是尖晶石和碳硅石的最可能的恒星来源。太阳系中比较特殊的氖和氙的同位素组成异常也与超新星爆发密切相关。  相似文献   

15.
Abstract— We report isotopic abundances for C, N, Mg‐Al, Si, Ca‐Ti, and Fe in 99 presolar silicon carbide (SiC) grains of type X (84 grains from this work and 15 grains from previous studies) from the Murchison CM2 meteorite, ranging in size from 0.5 to 1.5 μm. Carbon was measured in 41 X grains, n in 37 grains, Mg‐Al in 18 grains, Si in 87 grains, Ca‐Ti in 25 grains, and Fe in 8 grains. These X grains have 12C/13C ratios between 18 and 6800, 14N/15n ratios from 13 to 200, δ29Si/28Si between ?750 and +60%0, δ30Si/28Si from ?770 to ?10%0, and 54Fe/56Fe ratios that are compatible with solar within the analytical uncertainties of several tens of percent. Many X grains carry large amounts of radiogenic 26Mg (from the radioactive decay of 26Al, half‐life ? 7 times 105 years) and radiogenic 44Ca (from the radioactive decay of 44Ti, half‐life = 60 years). While all X grains but one have radiogenic 26Mg, only ～20% of them have detectable amounts of radiogenic 44Ca. Initial 26Al/27Al ratios of up to 0.36 and initial 44Ti/48Ti ratios of up to 0.56 can be inferred. The isotopic data are compared with those expected from the potential stellar sources of SiC dust. Carbon stars, Wolf‐Rayet stars, and novae are ruled out as stellar sources of the X grains. The isotopic compositions of C and Fe and abundances of extinct 44Ti are well explained both by type Ia and type II supernova (SN) models. The same holds for 26Al/27Al ratios, except for the highest 26Al/27Al ratios of >0.2 in some X grains. Silicon agrees qualitatively with SN model predictions, but the observed 29Si/30Si ratios in the X grains are in most cases too high, pointing to deficiencies in the current understanding of the production of Si in SN environments. The measured 14n/15n ratios are lower than those expected from SN mixing models. This problem can be overcome in a 15 Modot; type II SN if rotational mixing, preferential trapping of N, or both from 15n‐rich regions in the ejecta are considered. The isotopic characteristics of C, N, Si, and initial 26Al/27Al ratios in small X grains are remarkably similar to those of large X grains (2–10 μm). Titanium‐44 concentrations are generally much higher in smaller grains, indicative of the presence of Ti‐bearing subgrains that might have served as condensation nuclei for SiC. The fraction of X grains among presolar SiC is largely independent of grain size. This implies similar grain‐size distributions for SiC from carbon stars (mainstream grains) and supernovae (X grains), a surprising conclusion in view of the different conditions for dust formation in these two types of stellar sources.  相似文献   

16.
Abstract— We have determined the recoil range of spallation xenon produced by irradiation of Ba glass targets with ?1190 and ?268 MeV protons, using a catcher technique, where spallation products are measured in target and catcher foils. The inferred range for 126Xe produced in silicon carbide is ?0.19 μm, which implies retention of ?70% for 126Xe produced in “typical” presolar silicon carbide grains of 1 μm size. Recoil loss of spallation xenon poses a significantly smaller problem than loss of the spallation neon from SiC grains. Ranges differ for the various Xe isotopes and scale approximately linearly as function of the mass difference between the target element, Ba, and the product. As a consequence, SiC grains of various sizes will have differences in spallation Xe composition. In an additional experiment at ?66 MeV, where the recoil ranges of 22Na and 127Xe produced on Ba glass were determined using γ‐spectrometry, we found no evidence for recoil ranges being systematically different at this lower energy. We have used the new data to put constraints on the possible presolar age of the SiC grains analyzed for Xe by Lewis et al. (1994). Uncertainties in the composition of the approximately normal Xe component in SiC (Xe‐N) constitute the most serious problem in determining an age, surpassing remaining uncertainties in Xe retention and production rate. A possible interpretation is that spallation contributions are negligible and that trapped 124Xe/126Xe is ?5% lower in Xe‐N than in Q‐Xe. But also for other reasonable assumptions for the 124Xe/126Xe ratio in Xe‐N (e.g., as in Q‐Xe), inferred exposure ages are considerably shorter than theoretically expected lifetimes for interstellar grains. A short presolar age is in line with observations by others (appearance, grain size distribution) that indicate little processing in the interstellar medium (ISM) of surviving (crystalline) SiC. This may be due to amorphization of SiC in the ISM on a much shorter time scale than destruction, with amorphous SiC not surviving processing in the early solar system. A large supply of relatively young grains may be connected to the proposed starburst origin (Clayton 2003) for the parent stars of the mainstream SiC grains.  相似文献   

17.
Abstract— –We present data from TEM and NanoSIMS investigations of Murchison (CM2) KFC1 presolar graphites. TEM examinations of graphite ultramicrotome sections reveal varying degrees of graphite disorder, leading to distinctions between well‐graphitized onions, more turbostratic platy graphites, and the most disordered cauliflower graphites. Aside from their larger size, platy graphites are roughly similar in isotopic composition and in internal grain properties to the well‐graphitized onions. Most carbide‐containing platy graphites exhibit large s‐process element enrichments (∼200× solar Mo/Ti ratios), suggesting origins predominantly in AGB carbon stars. The C isotopic distribution of platy graphites is similar to onions, with representatives in both 12C‐depleted (5 < 12C/13C < 40) and 12C‐enriched groups (100 < 12C/13C < 350) and a pronounced gap in the 40 < 12C/13C < 75 region that contains 75% of mainstream SiCs. The large 12C enrichments combined with the extreme s‐process element enrichments suggest formation in an environment inhomogeneously enriched in the nucleosynthetic products of thermal pulses in AGB stars. In contrast, numerous scaly cauliflower graphites show 18O enrichments and lack s‐process‐enriched carbides, suggesting a SN origin, as was the case for many Murchison KE3 SN graphites. The more turbostratic graphites (platy and scaly) are on average larger than onions, likely resulting from formation in a gas with higher C number density. Oxygen content increases progressively with increasing degree of graphite disorder, which can stabilize these grains against further graphitization and may be a reflection of higher O/C ratios in their formation environments.  相似文献   

18.
Abstract— We demonstrate that a massive asymptotic giant branch (AGB) star is a good candidate as the main source of short‐lived radionuclides in the early solar system. Recent identification of massive (4–8 M⊙) AGB stars in the galaxy, which are both lithium‐ and rubidium‐rich, demonstrates that these stars experience proton captures at the base of the convective envelope (hot bottom burning), together with high‐neutron density nucleosynthesis with 22Ne as a neutron source in the He shell and efficient dredge‐up of the processed material. A model of a 6.5 M⊙ star of solar metallicity can simultaneously match the abundances of 26Al, 41Ca, 60Fe, and 107Pd inferred to have been present in the solar nebula by using a dilution factor of 1 part of AGB material per 300 parts of original solar nebula material, and taking into account a time interval between injection of the short‐lived nuclides and consolidation of the first meteorites equal to 0.53 Myr. Such a polluting source does not overproduce 53Mn, as supernova models do, and only marginally affects isotopic ratios of stable elements. It is usually argued that it is unlikely that the short‐lived radionuclides in the early solar system came from an AGB star because these stars are rarely found in star forming regions, however, we think that further interdisciplinary studies are needed to address the fundamental problem of the birth of our solar system.  相似文献   

19.
Abstract— We investigate heterogeneous nucleation and growth of graphite on precondensed TiC grains in the gas outflows from carbon‐rich asymptotic giant branch (AGB) stars employing a newly‐derived heterogeneous nucleation rate taking into account of the chemical reactions at condensation. Competition between heterogeneous and homogeneous nucleations and growths of graphite is investigated to reveal the formation conditions of the TiC core‐graphite mantle spherules found in the Murchison meteorite. It is shown that no homogeneous graphite grain condenses whenever TiC condenses prior to graphite in the plausible ranges of the stellar parameters. Heterogeneous condensation of graphite occurs on the surfaces of growing TiC grains, and prevents the TiC cores from reaching the sizes realized if all available Ti atoms were incorporated into TiC grains. The physical conditions at the formation sites of the TiC core‐graphite mantle spherules observed in the Murchison meteorite are expressed by the relation 0.2 < n?0.1 (M5/ζ)?1/2L41/4 < 0.7, where v0.1 is the gas outflow velocity at the formation site in units of 0.1 km s?1, M5 the mass loss rate in 10?5 M⊙ year?1, L4 the stellar luminosity in 104 L⊙, and M/ζ is the effective mass loss rate taking account of non‐spherical symmetry of the gas outflows. The total gas pressures Pc at the formation sites for the effective mass loss rates M/ζ = 10?5‐10?3 M⊙ year?1 correspond to 0.01 < Pc < 0.9 dyn cm?2, implying that the observed TiC core‐graphite mantle spherules are formed not only at the superwind stage but also at the earlier stage of low mass loss rates. The constraint on the C/O abundance ratio, 1 < ? ? 1.03, is imposed to reproduce the observed sizes of the TiC cores. The derived upper limit of the C/O ratio is lower than the values estimated from the calculations without taking into account of heterogeneous condensation of graphite, and is close to the lower end of the C/O ratios inferred from the astronomical observations of carbon‐rich AGB stars. Brief discussion is given on other types of graphite spherules.  相似文献   

20.
The abundances of 22 heavy elements from Sr to Pb have been determined for the halo star HD 29907 (T eff = 5500 K, log g = 4.64) with [Fe/H] = −1.55 using high-quality VLT/UVES spectra (ESO, Chile). The star has a moderate enhancement of r-process elements (Eu-Tm) with [r/Fe] = 0.63. In the range from Ba to Yb, the derived abundance pattern agrees well with those for strongly r-process enhanced stars (r-II stars with [Eu/Fe] > 1 and [Ba/Eu] < 0), such as CS 22892-052 and CS 31082-001, as well as with the scaled solar r-process curve and the r-process model HEW. Thus, Ba-Yb in HD 29907 originate in the r-process. Just as other moderately r-process enhanced stars studied in the literature, HD 29907 exhibits higher Sr, Y, and Zr abundances than those for r-II stars. These results confirm the assumption by other authors about the existence of an additional Sr-Zr synthesis mechanism in the early Galaxy before the onset of nucleosynthesis in asymptotic giant branch (AGB) stars. The same mechanism can be responsible for the enhancement of Mo-Ag in the star being investigated compared to r-II stars. There are no grounds to suggest the presence of s-nuclei of lead in the material of the star being investigated, because its measured abundance ratio log ɛ(Pb/Eu) = 1.20 lies within the range for the comparison stars: from log ɛ(Pb/Eu) = 0.17 (CS 31082-001) to < 1.55 (HE 1219-0312). Thus, even if there was a contribution of AGB stars to the heavy-element enrichment of the interstellar medium at the epoch with [Fe/H] = −1.55, it was small, at the level of the abundance error.  相似文献   

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