The²³⁸U spontaneous fission decay constant re-determined by fission tracks     

K. Thiel  W. Herr 《Earth and Planetary Science Letters》1976,30(1):50-56

The decay constant(λ_f²³⁸) for the spontaneous fission of²³⁸U was re-determined by means of a man-made uranium glass of known age (126 yr). The spontaneous U fission tracks that had accumulated since the date of manufacture were counted on internal faces of the glass with an error of less than 1.7%. No thermal annealing of the spontaneous tracks was observed. The U content was determined by induced fission tracks. The value obtained forλ_f²³⁸ is(8.57 ± 0.42) × 10^?17yr^?1. Main sources of error are the date of glass melting and the determination of the thermal neutron dose.  相似文献   

Investigations on cosmic-ray-produced nuclides in iron meteorites, 3. Exposure ages,meteoroid sizes and sample depths determined by mass spectrometric analyses of potassium and rare gases     

H. Voshage  H. Feldmann 《Earth and Planetary Science Letters》1979,45(2):293-308

Three physical quantities define the essentials of the cosmic ray exposure history of a sample of an iron meteorite: (1) the cosmic ray exposure age T, (2) the pre-atmospheric “size” S of the irradiated body, and (3) the location, i.e. the “depth” D, of the samples within the body. To establish these quantities for a given sample three independent quantities must be determined experimentally. In the present work T is ascertained by the ⁴¹K/⁴⁰K method and the ⁴He and ²¹Ne concentrations (C₄ and C₂₁) are measured by the isotope dilution method. Signer and Nier's evaluation of the rare gas distribution in the meteorite Grant and the measured exposure age for this meteorite provide the relationships allowing to ascertain for any meteorite the quantities S and D from the ²¹Ne production rate (P₂₁ = C₂₁/T) and the ⁴He/²¹Ne ratio.Earlier measurements have provided data on the isotopic composition of potassium in 74 different iron meteorites. New rare gas measurements are reported for some 40 samples. Results on the age, size and depth are obtained for almost 60 samples. These data suggest that Signer and Nier's model is well suited for describing not only the rare gas distribution in a single selected meteorite (Grant) but also the exposure histories of the great majority of all irons. For a few samples, however, secondary breakups of the meteoroid and a two- or multiple-stage irradiation must be invoked. Further measurements are proposed for testing and, possibly, refining the still somewhat uncertain relationships between the abundances of cosmogenic nuclides and the quantities T, S, and D in very large meteorites.Histograms are presented showing the age distributions for irons of different chemical groups and of different size ranges.The feasibility and the relative merits of other methods for the determination of T, S, and D are discussed.  相似文献   

Variations of characteristics of fission tracks in muscovites by thermal effects     

M.S.M. Mantovani 《Earth and Planetary Science Letters》1974,24(2):311-316

The applicability of the method of uranium fission tracks was studied in a number of sheets from a muscovite of about 600 m.y. Diagrams for fission track density (ρ) versus the chemical etching time (t_A), as well as the larger diameter of the transversal section (D) versus t_A curves were constructed, and the uranium concentration and uniformity of distribution were calculated. Some samples were heated at different constant temperatures for various time intervals, and the features presented by the heated and unheated tracks were analysed. The conclusions can be applied to corrections in age determination of muscovites that suffered natural annealing effects.  相似文献   

Evidence for²⁴⁴Pu fission tracks in hibonites from Murchison carbonaceous chondrite     

R.S. Rajan  A.S. Tamhane 《Earth and Planetary Science Letters》1982,58(1):129-135

We have developed a technique for revealing nuclear tracks in the mineral hibonite (CaAl₁₂O₁₉), found in the refractory inclusions from carbonaceous chondrites. The tracks in hibonitesfrom Murchison carbonaous chondrite are dominated by fission tracks from²⁴⁴Pu (constituting more than 90% of the total). The measured uranium contents in these crystals range from 1.2 to 62 ppb. We deduce that the average value for the²⁴⁴Pu/²³⁸U ratio in most of the Murchison hibonites at the time of track retention is0.022 ± 0.011.  相似文献   

Approximation of terrestrial lead isotope evolution by a two-stage model   总被引：13，自引：0，他引：13  

J.S. Stacey  J.D. Kramers 《Earth and Planetary Science Letters》1975,26(2):207-221

Parameters on which models for terrestrial lead isotope evolution are based have recently been revised. These parameters are the isotopic composition of troilite lead, the age of the meteorite system and the decay constants of uranium and thorium. As a result, the normal single-stage model in which the age of the earth is taken to be that of the meteorite system is now untenable.A two-stage model has been constructed which permits the age of the earth to be that of the meteorite system and which also yields good model ages for samples of all ages. The new model postulates that lead developed initially from a primordial composition assumed to be that of troilite lead beginning at 4.57 b.y. ago. The average values of ²³⁸U/²⁰⁴Pb and ²³²Th/²⁰⁴Pb for this first stage were 7.19 and 32.21 respectively. At approximately 3.7 b.y. ago differentiation processes brought about the conditions of a second stage, in which ²³⁸U/²⁰⁴Pb ≈ 9.74 and ²³²Th/²⁰⁴Pb ≈ 37.19 in those portions of the earth which took part in mixing events, giving rise to average lead.  相似文献   

⁸⁷Rb–⁸⁷Sr history of the Norton County enstatite achondrite     

J.F. Minster  C.J. Allegre 《Earth and Planetary Science Letters》1976,32(2):191-198

⁸⁷Rb⁸⁷Sr analysis of the Norton County achondrite has been achieved with special attention to the rubidium analysis. Enstatite crystals and polycrystalline material give an “age” of 4.48 ± 0.04 × 10⁹ years and an initial ratio ⁸⁷Sr/⁸⁶Sr_I= 0.7005 ± 0.0004 (λ = 1.39 × 10^?11yr^?1, maximum errors). The feldspar component of the meteorite contains about 70% of the strontium and 30% of the rubidium of the whole sample, and does not lie on the isochron. Its model age relative to the strontium initial ratio of Allende is 4.6 × 10⁹ years. The data are consistent with a complex history dealing with an incomplete isotopic reequilibration of the meteorite, 120 m.y. after its formation at 4.6 × 10⁹ years, with an initial ratio similar to that of Allende.  相似文献   

The records of solar wind and solar flares in aubrites     

G. Poupeau  T. Kirsten  F. Steinbrunn  D. Storzer 《Earth and Planetary Science Letters》1974,24(2):229-241

A large number of individual enstatite crystals of the gas-rich aubrites Khor Temiki, Staroe Pesyanoe and Bustee was analyzed for implanted helium and for steep gradient ion tracks in order to investigate the relation between solar flare irradiation and solar wind implantation with extreme local resolution. Irradiated and non-irradiated crystals coexist within the gas-rich phases of the aubrites investigated. Statistically in a given meteorite the proportion of crystals with implanted solar wind is similar to the proportion of solar flare irradiated crystals. It varies from aubrite to aubrite in the sequence of their bulk contents of trapped rare gases.For nine enstatites, tracks and rare gases were subsequently measured within the same crystal. The results support the intimate association of solar flare tracks and implanted He. The⁴He-surface concentrations of irradiated crystals vary between <5 × 10^?7 and 10^?4 cm³ STP/cm².The absence of saturation effects together with the low degree of elemental gas fractionation indicates very short solar wind exposure times (< 100 yr) rather than strong diffusion losses. The evidence from tracks and rare gases can be understood in terms of an early simultaneous irradiation of aubritic crystals by solar wind and solar flare particles on top of a regolith-covered parent body.  相似文献   

⁴⁰Ar/³⁹Ar age and thermal history of the Kirin chondrite     

Sungshan Wang  Ian McDougall  Neil Tetley  T. Mark Harrison 《Earth and Planetary Science Letters》1980,49(1):117-131

The Kirin meteorite, a large (2800kg) H5 chondrite, fell in Kirin Province, China in 1976. A sample from each of the two largest fragments (K-1, K-2) yield⁴⁰Ar/³⁹Ar total fusion ages of 3.63 ± 0.02b.y. and 2.78 ± 0.02b.y. respectively.⁴⁰Ar/³⁹Ar age spectra show typical diffusional argon loss profiles. Maximum apparent ages of 4.36 b.y. (K-1) and ～4.0 b.y. (K-2) are interpreted as possible minimum estimates for the age of crystallization of the parent body.The⁴⁰Ar/³⁹Ar ages found for gas released at low temperature are about 2.2 b.y. for K-1 and about 0.5 b.y. for K-2, suggesting that this meteorite may have suffered two discrete collisional events that caused degassing of radiogenic argon. Modelling of possible thermal events in the parent body indicates that samples K-1 and K-2 were at a depth of less than 3 m from the base of an impact melt of a thickness less than 7 m and separated by no more than ～2 m from one another at the time of the heating event about 0.5 b.y. ago. Further, the duration of heating was probably less than a few years.Calculations from³⁸Ar data yield exposure ages for samples K-1 and K-2 of about 5 m.y., similar to that found for many other H chondrites.  相似文献   

Nuclear track records in the Abee enstatite chondrite     

J.N. Goswami 《Earth and Planetary Science Letters》1983,62(1):159-164

Nuclear track records in fourteen samples taken from different locations of a cut-slab of the Abee enstatite chondrite were studied to determine its pre-atmospheric mass and to delineate its cosmic ray exposure history. The measured track densities in different samples range from 10⁴ to 10⁶ cm^?2. No significant variations in track densities for individual grains from a given location was found. Excess tracks of fissionogenic origin were found near the grain edges, and across cleavage planes in eight enstatite grains out of ～ 300 grains analysed in the present work. The compaction age of the meteorite could not be obtained due to the absence of suitable oldhamite-enstatite contacts in thick sections. The track data rule out pre-irradiation of any of the analysed samples with shielding less than a few tens of centimeter. The iso-track-density contours on the plane of the slab imply an asymmetric ablation of the Abee chondrite during its atmospheric transit. A spherical body having a radius of ～ 30 cm closely approximates the pre-atmospheric shape and size of the Abee meteorite. The mass loss during ablation was ～ 70% of the original mass.  相似文献   

Spalogenic rare gases in iron meteorites with anomalous silver     

I.M. Villa  J.C. Huneke  G.J. Wasserburg 《Earth and Planetary Science Letters》1981

He, Ne, and Ar have been measured in seven iron meteorites for which anomalous Ag isotopic compositions were reported, in order to determine if¹⁰⁷Ag excesses could be related to galactic cosmic-ray bombardment of these meteorites. Our results show that no correlation exists between¹⁰⁷Ag excess and either the fluence or the energy spectrum of the particles producing spallogenic rare gases. Cosmic-ray-produced¹⁰⁷Ag estimated from³⁸Ar concentrations can account for only about 1% of the observed excess. Elimination of cosmic-ray bombardment as a production mechanism for¹⁰⁷Ag excess strengthens the conclusion that the excess¹⁰⁷Ag is the decay product of short-lived¹⁰⁷Pd (τ_1/2=6.5Myr). The iron meteorite Pin?on is shown to contain trapped rare gases with⁴He/²⁰Ne～600.  相似文献   

Sm-Nd isotopic evolution of chondrites   总被引：8，自引：0，他引：8  

Stein B. Jacobsen  G.J. Wasserburg 《Earth and Planetary Science Letters》1980,50(1):139-155

The¹⁴³Nd/¹⁴⁴Nd and¹⁴⁷Sm/¹⁴⁴Nd ratios have been measured in five chondrites and the Juvinas achondrite. The range in¹⁴³Nd/¹⁴⁴Nd for the analyzed meteorite samples is 5.3 ε-units (0.511673–0.511944) normalized to¹⁵⁰Nd/¹⁴²Nd= 0.2096. This is correlated with the variation of 4.2% in¹⁴⁷Sm/¹⁴⁴Nd (0.1920–0.2000). Much of this spread is due to small-scale heterogeneities in the chondrites and does not appear to reflect the large-scale volumetric averages. It is shown that none of the samples deviate more than 0.5 ε-units from a 4.6-AE reference isochron and define an initial¹⁴³Nd/¹⁴⁴Nd ratio at 4.6 AE of0.505828 ± 9. Insofar as there is a range of values of¹⁴⁷Sm/¹⁴⁴Nd there is no unique way of picking solar or average chondritic values. From these data we have selected a new set of self-consistent present-day reference values for CHUR (“chondritic uniform reservoir”) of (¹⁴³Nd/¹⁴⁴Nd)_CHUR⁰ = 0.511836and(¹⁴⁷Sm/¹⁴⁴Nd)_CHUR⁰ = 0.1967. The new¹⁴⁷Sm/¹⁴⁴Nd value is 1.6% higher than the previous value assigned to CHUR using the Juvinas data of Lugmair. This will cause a small but significant change in the CHUR evolution curve. Some terrestrial samples of Archean age show clear deviations from the new CHUR curve. If the CHUR curve is representative of undifferentiated mantle then it demonstrates that depleted sources were also tapped early in the Archean. Such a depleted layer may represent the early evolution of the source of present-day mid-ocean ridge basalts. There exists a variety of discrepancies with most earlier meteorite data which includes determination of all Nd isotopes and Sm/Nd ratios. These discrepancies require clarification in order to permit reliable interlaboratory comparisons. The new CHUR curve implies substantial changes in model ages for lunar rocks and thus also in the interpretation of early lunar chronology.  相似文献   

Nickel isotopic studies in meteorites     

Philippe Morand  Claude J. Allègre 《Earth and Planetary Science Letters》1983,63(2):167-176

We have analyzed the nickel isotopic composition of meteoritic materials by high-precision mass spectrometry. The samples analyzed include almost all meteorite types for which large isotopic anomalies have been reported for oxygen, silver, magnesium and titanium. These samples are C₁, C₃, L, LL, H and E chondrites, IVB irons, Eagle Station pallasite and inclusion, matrix and “whole rock” samples of the Allende meteorite. The result is that we have not found any anomaly for nickel isotopic compositions within our accuracy of 0.7‰ for⁶¹Ni/⁶⁰Ni, 0.4-0.08‰ for⁶²Ni/⁶⁰Ni and 1–1.5‰ for⁶⁴Ni/⁶⁰Ni.  相似文献   

The registration-temperature dependence of heavy-ion track-etch rates and annealing sensitivity in crystals: implications for cosmic ray identification and fission track dating of meteorites     

K. James  S.A. Durrani 《Earth and Planetary Science Letters》1988,87(1-2)

Etch rates and etchable lengths of cosmic ray tracks in meteoritic crystals have been used by several workers to derive the charge spectrum of ancient cosmic rays. This is done by comparing the fossil cosmic ray track record with fresh accelerator-produced calibration tracks. These calibration tracks are generally produced at room temperature, while meteorites spend a high proportion of their lifetimes orbiting at large distances from the Sun ( 3–5 AU) and are, consequently, at much lower temperatures (typically 100–150 K) during most of their cosmic ray exposure ages. We have irradiated crystals of apatite, olivine, enstatite and diopside held at 77, 293, 473 and 573 K, with 2 MeV/nucleon⁸¹Br ions, and then etched them. We find that their track etching properties are dependent upon the temperature of the mineral during registration. The track etch velocity generally increases with registration temperature up to 300 or 500 K (the upper limit depending upon the type of crystal). Our results also indicate that the annealing sensitivity of fission tracks in fluorapatite may be influenced by the registration temperature. This temperature dependence has important implications not only for cosmic ray particle identification but also for fission track dating of meteorites in view of the fact that the meteorite parent bodies were at elevated temperatures at the beginning af their life when²⁴⁴Pu fission tracks were being generated abundantly.  相似文献   

SmNd isotopic systematics of Enderby Land granulites and evidence for the redistribution of Sm and Nd during metamorphism     

M.T. McCulloch  L.P. Black 《Earth and Planetary Science Letters》1984,71(1):46-58

Measurements of¹⁴³Nd/¹⁴⁴Nd and¹⁴⁷Sm/¹⁴⁴Nd are reported for whole rocks and mineral separates from granulites of the Napier Complex at Fyfe Hills. Charnockites, leuconorites and gabbros yield a whole rock SmNd isochron age of3060 ± 160m.y. and an initial¹⁴³Nd/¹⁴⁴Nd ratio of0.50776 ± 10 (?_Nd(3060m.y.) = ?2.0 ± 1.8). The negative ?_Nd value and the presence of geologically induced dispersion in the data suggest that the isochron age does not represent the time of primary crystallization of the complex but instead indicates a time of later redistribution of Sm and Nd and partial re-equilibration of¹⁴³Nd/¹⁴⁴Nd ratios. This probably occurred during the upper granulite facies metamorphism which has also been dated at～ 3100m.y. by RbSr and UPb zircon studies [1]. Coexisting clinopyroxene, apatite and total rock fractions in two adjacent samples define an approximately linear array corresponding to an age of 2300 ± 300 m.y. This array indicates that redistribution of Sm and Nd and re-equilibration of¹⁴³Nd/¹⁴⁴Nd ratios occurred on an intermineral scale during the upper amphibolite to lower granulite facies metamorphism at～ 2450m.y.Due to the resetting of the SmNd system on both whole rock and mineral scales, the primary crystallization age of the igneous protolith is not well constrained by the present data, although it is clearly3100m.y. If it is assumed that the complex was derived initially from a depleted mantle reservoir(?_Nd(T) ? 2), evolution of the negative ?_Nd value of ?2.0 with the observed Sm/Nd ratios requires a prehistory of～ 380m.y. This implies a primary age of～ 3480m.y. However, substantially older primary ages can be inferred if the source reservoirs had?_Nd(T) > 2 and/or substantial reductions in the Sm/Nd ratio occurred in whole rocks during the granulite facies metamorphism at 3100 m.y. Such an inferred reduction in the Sm/Nd ratio may have been the result of preferential loss of Sm relative to Nd, or introduction of a low Sm/Nd fluid with?_Nd ≥ 0 during granulite facies metamorphism.  相似文献   

Space weathering processes on airless bodies: Fe isotope fractionation in the lunar regolith     

René A. Wiesli  Brian L. Beard  Clark M. Johnson 《Earth and Planetary Science Letters》2003,216(4):457-465

Nanophase Fe metal grains (np-Fe°) are a product of space weathering, formed by processes related to meteorite impacts, and solar-wind sputtering on airless planetary bodies, such as the Moon. Iron isotopes of lunar soils are fractionated during these processes, and the np-Fe° in the finest (<10 μm), mature, size fractions of the soil become enriched in heavier isotopes by ∼0.3‰ in ⁵⁶Fe/⁵⁴Fe in comparison to the bulk rocks (0.03±0.05‰), from which the soil was formed. A positive correlation of δ⁵⁶Fe values with the soil maturity index, I_S/FeO, suggests that the high δ⁵⁶Fe values reflect production of nanophase Fe metal that is produced by space weathering that occurs on airless planetary bodies. Furthermore, the enrichment of δ⁵⁶Fe in the smallest size fraction of lunar soils supports a model for creation of np-Fe° through vapor deposition induced by micrometeorites, as well as that by solar-wind sputtering.  相似文献   

Chondrule mass distribution and the Rosin and Weibull statistical functions     

David W. Hughes 《Earth and Planetary Science Letters》1978,39(3):371-376

Near-spherical chondrules disaggregated from the meteorite Bjurböle are not found to give a good fit to Rosin's size distribution law but do obey with considerable precision a Weibull distribution law in which Y, the mass percentage of the chondrules which passes through a sieve of mesh size d mm, is given by: Y = 100{1?exp[?0.471 (d ?0.32)^1.84]}  相似文献   

Cosmogenic neon produced from sodium in meteoritic minerals     

S.P. Smith  J.C. Huneke 《Earth and Planetary Science Letters》1975,27(2):191-199

Cosmogenic neon in sodium-rich oligoclase feldspar from the ordinary chondrites St. Severin and Guaren?a is characterized by an unusually high²²Ne/²¹Ne = 1.50 ± 0.02. This high ratio is due to the cosmogenic²²Ne/²¹Ne production ratio in sodium which is 2.9 ± 0.3, two to three times the production ratio in any other target element. The relative production rate of²¹Ne per gram sodium is one quarter the production rate per gram magnesium. The striking enrichment of²²Ne relative to²¹Ne in sodium arises from enhanced indirect production from²³Na via²²Na.The unusual composition of cosmogenic neon in sodium and sodium-rich minerals explains the high²²Ne/²¹Ne ratios observed in inclusions of the Allende carbonaceous chondrite, and observed during low-temperature extraction of neon from ordinary chondrites. The isotopic composition of cosmogenic neon released during the stepwise heating of a trapped gas-rich meteorite containing sodium-rich phases can be expected to vary, and use of a constant cosmogenic neon composition to derive the composition of the trapped gas may not be justified. Preferential loss of this²²Ne-enriched cosmogenic neon from meteoritic feldspar can result in a 2–3% drop in the measured cosmogenic²²Ne/²¹Ne ratio in a bulk meteorite sample. This apparent change in composition can lead to overestimation of the minimum pre-atmospheric mass of the meteorite by a factor of two.  相似文献   

Rb-Sr whole-rock age of the contact aureole of the Stillwater Igneous Complex,Montana     

Paul A. Mueller  Joseph L. Wooden 《Earth and Planetary Science Letters》1976,29(2):384-388

Fourteen whole-rock samples from three traverses through the contact aureole of the Stillwater Complex were analyzed for Rb, Sr and⁸⁷Sr/⁸⁶Sr. Twelve of these samples yielded an age of 2750 ± 45m.y.; (⁸⁷Sr/⁸⁶Sr)₀ = 0.705 ± 0.003 (2σ). In addition one whole rock and a biotite separate derived from it gave an age of 2544 m.y.; (⁸⁷Sr/⁸⁶Sr)₀ = 0.714. These data support a minimum age of 2750 m.y. for the intrusion of the complex.  相似文献   

Comment on “The July 9 and 23, 1905, Mongolian earthquakes,a surface-wave investigation” by Emile Okal     

A.V. Ilyin 《Earth and Planetary Science Letters》1978,41(1):107-109

K-Ar ages have been determined for sulfide minerals for the first time. The occurrence of adequate amounts of potassium-bearing sulfides with ideal compositions K₃Fe₁₀S₁₄ (～10 wt.% K) and KFe₂S₃ (～16 wt.% K) in samples from a mafic alkalic diatreme at Coyote Peak, California, prompted an attempt to date these materials. K₃Fe₁₀S₁₄, a massive mineral with conchoidal fracture, gives an age of 29.4 ± 0.5m.y.(⁴⁰Ar/³⁹Ar), indistinguishable from the 28.3 ± 0.4m.y.(⁴⁰Ar/³⁹Ar) and 30.2 ± 1.0m.y.8 (conventional K-Ar) ages obtained for associated phlogopite (8.7 wt.% K). KFe₂S₃, a bladed, fibrous sulfide, gives a younger age, 26.5 ± 0.5m.y.(⁴⁰Ar/³⁹Ar), presumably owing to Ar loss.  相似文献   

Extra-terrestrial ⁵³Mn in Antarctic ice     

R. Bibron  R. Chesselet  G. Crozaz  G. Leger  J.P. Mennessier  E. Picciotto 《Earth and Planetary Science Letters》1974,21(2):109-116

The reasons why⁵³Mn (a cosmogenic radionuclide with a half-life of 3.7 × 10⁶ y) appears as one of the best indicators of the presence of interplanetary dust are summarized. This paper reports the detection of⁵³Mn in pre-1952 snow samples collected on the Eastern Antarctic Plateau in the vicinity of Plateau Station. The measurements were carried out by neutron activation and X-ray spectrometry on three samples weighing a few hundred kg and covering each the time interval 1935–1950. The specific activity of⁵³Mn was found to be (0.82 ± 0.17) disint.min^?1/10³ tons of snow, corresponding to a deposition rate at Plateau Station of (2.2 ± 0.5) × 10^?5 disint. min^?1 m^?2 y^?1. The mean global deposition rate would be three times higher if⁵³Mn were assumed to behave in the same way as stratospheric⁹⁰Sr. By comparing this figure with existing data on the meteorite flux reaching the earth and with the galactic and solar production rates of⁵³Mn, it is concluded that the bulk of the⁵³Mn found at Plateau Station is associated with interplanetary dust in which it had been produced by the action of solar protons on iron. The deposition rate of extra-terrestrial dust-borne iron must be between 1.3 × 10^?5 and 1.3 × 10^?4 g m^?2 y^?1 at Plateau Station. These results support jointly with other studies the concept of an interplanetary zodiacal cloud of dust with a chemical composition and density not essentially different from chondritic meteorites, with a relatively ‘flat’ grain size distribution and a mass influx to the earth of the order of 10⁵ tons/y.  相似文献