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1.
In organic soils, hydraulic conductivity is related to the degree of decomposition and soil compression, which reduce the effective pore diameter and consequently restrict water flow. This study investigates how the size distribution and geometry of air‐filled pores control the unsaturated hydraulic conductivity of peat soils using high‐resolution (45 µm) three‐dimensional (3D) X‐ray computed tomography (CT) and digital image processing of four peat sub‐samples from varying depths under a constant soil water pressure head. Pore structure and configuration in peat were found to be irregular, with volume and cross‐sectional area showing fractal behaviour that suggests pores having smaller values of the fractal dimension in deeper, more decomposed peat, have higher tortuosity and lower connectivity, which influences hydraulic conductivity. The image analysis showed that the large reduction of unsaturated hydraulic conductivity with depth is essentially controlled by air‐filled pore hydraulic radius, tortuosity, air‐filled pore density and the fractal dimension due to degree of decomposition and compression of the organic matter. The comparisons between unsaturated hydraulic conductivity computed from the air‐filled pore size and geometric distribution showed satisfactory agreement with direct measurements using the permeameter method. This understanding is important in characterizing peat properties and its heterogeneity for monitoring the progress of complex flow processes at the field scale in peatlands. Copyright © 2010 John Wiley & Sons, Ltd.  相似文献   

2.
Reclamation of peat bogs for agriculture changes the physical and chemical characteristics of the peat matrix, for example, drainage and tillage accelerate decomposition, altering peat porosity, pore size distribution, and hydraulic properties. This study investigated changes in near-saturated hydraulic conductivity over time after drainage of peat soil for agricultural use by conducting tension infiltrometer measurements in a mire that has been gradually drained and reclaimed for agriculture during the past 80 years (with fields drained 2, 12, 40, and 80 years before the measurements). At pore water pressure closest to saturation (pressure head −1 cm), hydraulic conductivity in the newest field was approximately nine times larger than that in the oldest field, and a decreasing trend with field age was observed. A similar (but weaker) trend was observed with −3 cm pressure head (approximately four times larger in the newest field in comparison to the oldest), but at −6 cm head, there were no significant differences. These results indicate that peat degradation reduces the amount of millimetre-sized pores in particular. They also indicate that changes in peat macroporosity continue for several decades before a new steady state is reached.  相似文献   

3.
Coastal peatlands represent an interface between marine and terrestrial ecosystems; their hydrology is affected by salt and fresh water inflow alike. Previous studies on bog peat have shown that pore water salinity can have an impact on the saturated hydraulic conductivity (Ks) of peat because of chemical pore dilation effects. In this study, we aimed at quantifying the impact of higher salinities (up to 3.5% NaCl) on Ks of fen peat. Two experiments employing a constant‐head upward‐flow permeameter and differing in measurement and salinity change duration were conducted. Additionally, a third experiment to determine the impact of water salinity on the release of dissolved organic carbon (DOC) of the studied peat type was carried out. The results show a decrease of Ks with time, which does not depend on the water salinity but is differently shaped for different peat types. We assume pore clogging due to a conglomerate of physical, chemical, and biological processes, which rather depend on water movement rate and time than on water salinity. However, an increased water salinity did increase the DOC release. We conclude that salinity‐dependent behaviour of Ks is a function of peat chemistry and that for some peat types, salinity may only affect the DOC release without having a pronounced impact on water flow.  相似文献   

4.
Geophysical surveys and chemical analyses on cores were carried out in three Ontario peatlands, from which we have gained a better understanding of the peat properties that control the geophysical responses. The electrical conductivity depends linearly on the concentration of total dissolved solids in the peat pore waters and the pore waters in turn bear the ionic signatures of the underlying mineral sediments. The ionic concentration, and thus the electrical conductivity, increase linearly from the surface to basement. The average bulk electrical conductivity of peatlands at Ellice Marsh, near Stratford, and at Wally Creek Area Forest Drainage Project, near Cochrane, are of the order of 25 mS/m. The Mer Bleue peatland, near Ottawa, has extremely high electrical conductivity, reaching levels of up to 380 mS/m near the base of the peat. The Mer Bleue peatland water has correspondingly high values of total dissolved solids, which originate from the underlying Champlain Sea glaciomarine clays. The dielectric permittivity in peats is largely controlled by the bulk water content. Ground penetrating radar can detect changes in water content greater than 3%, occurring within a depth interval less than 15 cm. The principal peatland interfaces detected are the near-surface aerobic to anaerobic transition and the peat to mineral basement contact. The potential for the successful detection of the basement contact using the radar can be predicted using the radar instrument specifications, estimates of the peatland depth, and either the bulk peat or the peat pore water electrical conductivities. Predicted depths of penetration of up to 10 m for Ellice Marsh and Wally Creek exceed the observed depths of 1 to 2 m. At Mer Bleue, on the other hand, we observe that, as predicted, a 100 MHz signal will penetrate to the base of a 2 m thick peat but a 200 MHz signal will not.  相似文献   

5.
The relationship between aquifer hydraulic conductivity and aquifer resistivity, either measured on the ground surface by vertical electrical sounding (VES) or from resistivity logs, or measured in core samples have been published for different types of aquifers in different locations. Generally, these relationships are empirical and semi-empirical, and confined in few locations. This relation has a positive correlation in some studies and negative in others. So far, there is no potentially physical law controlling this relation, which is not completely understood. Electric current follows the path of least resistance, as does water. Within and around pores, the model of conduction of electricity is ionic and thus the resistivity of the medium is controlled more by porosity and water conductivity than by the resistivity of the rock matrix. Thus, at the pore level, the electrical path is similar to the hydraulic path and the resistivity should reflect hydraulic conductivity. We tried in this paper to study the effect of degree of groundwater saturation in the relation between hydraulic conductivity and bulk resistivity via a simple numerical analysis of Archie’s second law and a simplified Kozeny-Carmen equation. The study reached three characteristic non-linear relations between hydraulic conductivity and resistivity depending on the degree of saturation. These relations are: (1) An inverse power relation in fully saturated aquifers and when porosity equals water saturation, (2) An inverse polynomial relation in unsaturated aquifers, when water saturation is higher than 50%, higher than porosity, and (3) A direct polynomial relation in poorly saturated aquifers, when water saturation is lower than 50%, lower than porosity. These results are supported by some field scale relationships.  相似文献   

6.
Part of the relationship between positive pore water pressures and hydraulic conductivity in peat soils may be explained by accumulations of methane bubbles. We show how compression and expansion of gas bubbles with changes in pore water pressure could cause changes in hydraulic conductivity and thus help to explain some observations of dependency of hydraulic conductivity in peats on pore water pressure. Consideration is also given to the effect on hydraulic conductivities of methane gas going into solution with increase in pore water pressure.  相似文献   

7.
Major challenges exist in delineating bedrock fracture zones because these cause abrupt changes in geological and hydrogeological properties over small distances. Borehole observations cannot sufficiently capture heterogeneity in these systems. Geophysical techniques offer the potential to image properties and processes in between boreholes. We used three‐dimensional cross borehole electrical resistivity tomography (ERT) in a 9 m (diameter) × 15 m well field to capture high‐resolution flow and transport processes in a fractured mudstone contaminated by chlorinated solvents, primarily trichloroethylene. Conductive (sodium bromide) and resistive (deionized water) injections were monitored in seven boreholes. Electrode arrays with isolation packers and fluid sampling ports were designed to enable acquisition of ERT measurements during pulsed tracer injections. Fracture zone locations and hydraulic pathways inferred from hydraulic head drawdown data were compared with electrical conductivity distributions from ERT measurements. Static ERT imaging has limited resolution to decipher individual fractures; however, these images showed alternating conductive and resistive zones, consistent with alternating laminated and massive mudstone units at the site. Tracer evolution and migration was clearly revealed in time‐lapse ERT images and supported by in situ borehole vertical apparent conductivity profiles collected during the pulsed tracer test. While water samples provided important local information at the extraction borehole, ERT delineated tracer migration over spatial scales capturing the primary hydrogeological heterogeneity controlling flow and transport. The fate of these tracer injections at this scale could not have been quantified using borehole logging and/or borehole sampling methods alone.  相似文献   

8.
Transient high pore‐water pressures, up to 50 cm higher than ambient pressure, developed over the summer season at various depths in a shallow (1 m) fen peat. The excess pressures had a pattern of gradual increases and sharp drops, and their initiation and release typically corresponded to abrupt changes in atmospheric pressure. We conclude that these phenomena depend on gas bubbles (probably methane) generated by biological activity, both by clogging pores and by building up pressure as they grow. These transient and spatially discontinuous high‐pressure zones were found using pressure transducers in sealed (backfilled) pits, but not in piezometers open to the atmosphere. Piezometers may provide a conduit for the release of gas and pressure, thus rendering them unsuitable for measuring this phenomenon. Although the development of localized zones of high pressure causes erratic and unpredictable hydraulic gradients, we suggest that their effect on the flow of water or solutes is offset by the reduced permeability caused by the bubbles, which allows them to be sustained. These zones, however, probably deflect flows driven by the dominant hydraulic gradients. Furthermore, they may cause the peat volume to adjust (swell). The use and interpretation of traditional methods for estimating hydraulic head and conductivity in peat soils thus require great caution. Copyright © 2004 John Wiley & Sons, Ltd.  相似文献   

9.
— Pressure-induced variations in pore geometry were studied on dry- and fluid- saturated samples by means of electrical impedance spectroscopy and permeability measurements. Hydrostatic pressures (up to 120 MPa) and uniaxial pressures (up to failure) were applied. Hydrostatic pressures reduce the aspect ratio of cracks and thus cause a decrease of permeability and electrical bulk conductivity. The opposite was observed in uniaxial pressure experiments where new cracks were formed and consequently permeability and electrical conductivity were increased. More specific informations of these generated observations were derived from the interpretation of the frequency dispersion of the complex electrical conductivity. This least-squares-refinement considers electrochemical interactions between the fluid pore electrolyte and the inner surface of the sample, thus providing informations on the pore geometry and pressure-induced variations. Consequently changes in aspect ratio, size and geometry of the pore system can be detected by means of impedance spectroscopy.  相似文献   

10.
The hydraulic conductivity (K) of peat beneath the water table varies over short (annual) periods. Biogenic gas bubbles block pores and reduce K, and seasonal changes in the water table position cause peat deformation, altering peat pore size distribution. Although it has been hypothesized that both processes reduce K during warm dry summer conditions, temporal variations in K under field conditions have been explained previously by peat volume changes (strain) alone. We determine the effect of both controls on K by monitoring changes in gas content (Δγ), strain and K within a poor fen. Over the growing season, K decreased by an order of magnitude. In the near‐surface peat (0.3–0.7 m), this reduction is more strongly correlated with Δγ, providing the first field‐based evidence that biogenic gas bubbles reduce K. In the deeper peat (0.7–1.3 m), K is correlated principally with strain. However, causality is uncertain because of multicollinearity between strain and Δγ. To mitigate for multicollinearity, we took advantage of a peatland drainage experiment where the water table was artificially dropped at the beginning of the growing season, reducing correlations between strain and Δγ. Δγ remained the primary cause of K variations just beneath the water table at a depth of 0.5–0.7 m, although further down through the peat profile (0.7–1.2 m) changes in K were controlled by strain. We suggest that the larger pore structure of the poorly decomposed peat just below the water table is impacted less by volume changes than that of the more decomposed peat at depth. However, within this poorly decomposed peat, K is reduced by the high gas contents that result from higher rates of methane production. Copyright © 2012 John Wiley & Sons, Ltd.  相似文献   

11.
J. Holden  T. P. Burt 《水文研究》2003,17(6):1227-1237
A key parameter used in wetland hydrological and landform development models is hydraulic conductivity. Head recovery tests are often used to measure hydraulic conductivity, but the calculation techniques are usually confined to rigid soil theory. This is despite reports demonstrating the misapplication of rigid soil theory to non‐rigid soils such as peats. Although values of hydraulic conductivity calculated using compressible techniques have been presented for fenland peats, these data have never, to the authors' knowledge, been compared with such calculations in other peat types. Head recovery tests (slug withdrawal) were performed on piezometers at depths ranging from 10 to 80 cm from the surface on north Pennines blanket peats. Results were obtained using both rigid and compressible soil theories, thus allowing comparison of the two techniques. Compressible soil theory gives values for hydraulic conductivity that are typically a factor of five times less than rigid soil calculations. Hydraulic conductivity is often assumed to decrease with depth in upland peats, but at the study site in the northern Pennines it was not found to vary significantly with depth within the range of peat depths sampled. The variance within depth categories was not significantly different to the variance between depth categories showing that individual peat layers did not have characteristic hydraulic conductivity values. Thus, large lateral and vertical differences in hydraulic conductivity over short distances create problems for modelling but may help account for the high frequency of preferential flow pathways within what is otherwise a low matrix hydraulic conductivity peat. Hydraulic conductivity was found to vary significantly between sampling sites, demonstrating that hillslope‐ or catchment‐scale variability may be more important than plot‐scale variability. Values for compressibility of the peats are also reported. These generally decline with depth, and they also vary significantly between sampling sites. There are implications for the way in which measurements of hydraulic conductivity and other properties of blanket peat are interpreted, as the effects of environmental change in one part of a peat catchment may be very different to those in another. Copyright © 2002 John Wiley & Sons, Ltd.  相似文献   

12.
Entrapped gas bubbles in peat can alter the buoyancy, storativity, void ratio and expansion/contraction properties of the peat. Moreover, when gas bubbles block water‐conducting pores they can significantly reduce saturated hydraulic conductivity and create zones of over‐pressuring, perhaps leading to an alteration in the magnitude and direction of groundwater flow and solute transport. Some previous researches have demonstrated that these zones of over‐pressuring are not observed by the measurements of pore‐water pressures using open‐pipe piezometers in peat; rather, they are only observed with pressure transducers sealed in the peat. In has been hypothesized that open‐pipe piezometers vent entrapped CH4 to the atmosphere and thereby do not permit the natural development of zones of entrapped gas. Here we present findings of the study to investigate whether piezometers vent subsurface CH4 to the atmosphere and whether the presence of piezometers alters the subsurface concentration of dissolved CH4. We measured the flux of methane venting from the piezometers and also determined changes in pore‐water CH4 concentration at a rich fen in southern Ontario and a poor fen in southern Quebec, in the summer of 2004. Seasonally averaged CH4 flux from piezometers was 1450 and 37·8‐mg CH4 m?2 d?1 at the southern Ontario site and Quebec site, respectively. The flux at the Ontario site was two orders of magnitude greater than the diffusive flux at the site. CH4 pore‐water concentrations were significantly lower in open piezometers than in water taken from sealed samplers at both the Ontario and Quebec sites. The flux of CH4 from piezometers decreased throughout the season suggesting that CH4 venting through the piezometer exceeded the rate of methanogenesis in the peat. Consequently we conclude that piezometers may alter the gas dynamics of some peatlands. We suggest that less‐invasive techniques (e.g. buried pressure transducers, tracer experiments) are needed for the accurate measurement of pore‐water pressures and hydraulic conductivity in peatlands with a large entrapped gas component. Furthermore, we argue that caution must be made in interpreting results from previous peatland hydrology studies that use these traditional methods. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

13.
A new probe was designed to quantify groundwater-surface water exchange in the hyporheic zone under dynamic stage condition. Current methods focus on either vertical pore water velocity or Darcy flux measurements. Both parameters must be understood to evaluate residence time and mass flux of constituents. Furthermore, most instruments are not well suited for monitoring instantaneous velocity or flux under dynamic exchange conditions. For this reason, the flux detection probe (FDP) was designed that employs electrogeophysical measurements to estimate in situ sediment porosity, which can be used to convert pore water velocity to Darcy flux. Dynamic pore water velocity is obtained by monitoring fluid conductivity and temperature along the FDP probe. Pressure sensors deployed at the top and bottom of the probe provide the additional information necessary to estimate vertical permeability. This study focuses on the use of a geophysical method to estimate pore water velocity, porosity, and permeability within a controlled soil column where simulated river water displaces simulated groundwater. The difference between probe derived and theoretical pore water velocity using natural tracers such as electrical conductivity and temperature was −4.9 and 3.9% for downward flow and 1.1 and 12.8% for upward flow, respectively. The difference in porosity calculated from mass and volume packed in the soil column and probe measure porosity ranged between −3.2% and 1.5%. Also, the calculated hydraulic conductivity differed from probe derived values by −8.9%.  相似文献   

14.
The selective radius shift model was used to relate changes in mineral volume due to precipitation/dissolution reactions to changes in hydraulic properties affecting flow in porous media. The model accounts for (i) precipitation/dissolution taking place only in the water-filled part of the pore space and further that (ii) the amount of mineral precipitation/dissolution within a pore depends on the local pore volume. The pore bundle concept was used to connect pore-scale changes to macroscopic soil hydraulic properties. Precipitation/dissolution induces changes in the pore radii of water-filled pores and, consequently, in the effective porosity. In a time step of the numerical model, mineral reactions lead to a discontinuous pore-size distribution because only the water-filled pores are affected. The pore-size distribution is converted back to a soil moisture characteristic function to which a new water retention curve is fitted under physically plausible constraints. The model equations were derived for the commonly used van Genuchten/Mualem hydraulic properties. Together with a mixed-form solution of Richards’ equation for aqueous phase flow, the model was implemented into the geochemical modelling framework PHREEQC, thereby making available PHREEQC’s comprehensive geochemical reactions. Example applications include kinetic halite dissolution and calcite precipitation as a consequence of cation exchange. These applications showed marked changes in the soil’s hydraulic properties due to mineral precipitation/dissolution and the dependency of these changes on water contents. The simulations also revealed the strong influence of the degree of saturation on the development of the saturated hydraulic conductivity through its quadratic dependency on the van Genuchten parameter α. Furthermore, it was shown that the unsaturated hydraulic conductivity at fixed reduced water content can even increase during precipitation due to changes in the pore-size distribution.  相似文献   

15.
A pore‐scale model based on measured particle size distributions has been used to quantify the changes in pore space geometry of packed soil columns resulting from a dilution in electrolyte concentration from 500 to 1 mmol l?1 NaCl during leaching. This was applied to examine the effects of particle release and re‐deposition on pore structure and hydraulic properties. Two different soils, an agricultural soil and a mining residue, were investigated with respect to the change in hydraulic properties. The mining residue was much more affected by this process with the water saturated hydraulic conductivity decreasing to 0·4% of the initial value and the air‐entry value changing from 20 to 50 cm. For agricultural soil, there was little detectable shift in the water retention curve but the saturated hydraulic conductivity decreased to 8·5% of the initial value. This was attributed to localized pore clogging (similar to a surface seal) affecting hydraulic conductivity, but not the microscopically measured pore‐size distribution or water retention. We modelled the soil structure at the pore scale to explain the different responses of the two soils to the experimental conditions. The size of the pores was determined as a function of deposited clay particles. The modal pore size of the agricultural soil as indicated by the constant water retention curve was 45 µm and was not affected by the leaching process. In the case of the mining residue, the mode changed from 75 to 45 µm. This reduction of pore size corresponds to an increase of capillary forces that is related to the measured shift of the water retention curve. Copyright © 2007 John Wiley & Sons, Ltd.  相似文献   

16.
Abstract

The theoretical spatial distribution of hydraulic head during infiltration is used to interpret the results of infiltration experiments made in the field on a single, isolated, column of herbaceous peat in a flood-plain wetland in central England. Crusts of different hydraulic resistance were applied to the column surface. These regulated the water influx enabling the hydraulic conductivity of the peat to be estimated at between 1 and 19.5 m day-1. It is inferred that, when the hydraulic gradient changes, water may follow different pathways through the peat. Water moves rapidly through macropores in proportion to the applied hydraulic gradient, and infiltrates the peat matrix from the macropore walls. The results indicate the significance of hydraulic conductivity variations with depth, and the importance of precipitation intensity.  相似文献   

17.
In coastal zones globally, salinization is rapidly taking place due to the combined effects of sea level rise, land subsidence, altered hydrology, and climate change. Although increased salinity levels are known to have a great impact on both biogeochemical and hydrological processes in aquatic sediments, only few studies have included both types of processes and their potential interactions. In the present paper, we used a controlled 3‐year experimental mesocosm approach to test salinity induced interactions and discuss mechanisms explaining the observed hydrological changes. Surface water salinity was experimentally increased from 14 to 140 mmol Cl per L (0.9 and 9 PSU) by adding sea salt which increased pore water salinity but also increased sulfate reduction rates, leading to higher sulfide, and lower methane concentrations. By analyzing slug test data with different slug test analysis methods, we were able to show that hydraulic conductivity of the hyporheic zone increased 2.8 times by salinization. Based on our hydrological and biogeochemical measurements, we conclude that the combination of pore dilation and decreased methane production rates were major controls on the observed increase in hydraulic conductivity. The slug test analysis method comparison allowed to conclude that the adjusted Bouwer and Rice method results in the most reliable estimate of the hydraulic conductivity for hyporheic zones. Our work shows that both physical and biogeochemical processes are vital to explain and predict hydrological changes related to the salinization of hyporheic zones in coastal wetlands and provides a robust methodological approach for doing so.  相似文献   

18.
E. Rosa  M. Larocque 《水文研究》2008,22(12):1866-1875
Flow dynamics within a peatland are governed by hydraulic parameters such as hydraulic conductivity, dispersivity and specific yield, as well as by anisotropy and heterogeneity. The aim of this study is to investigate hydraulic parameters variability in peat through the use of different field and laboratory methods. An experimental site located in the Lanoraie peatland complex (southern Quebec, Canada) was used to test the different approaches. Slug and bail tests were performed in piezometer standpipes to investigate catotelm hydraulic conductivity. Combined Darcy tests and tracer experiments were conducted on cubic samples using the modified cube method (MCM) to assess catotelm hydraulic conductivity, anisotropy and dispersivity. A new laboratory method is proposed for assessing acrotelm hydraulic conductivity and gravity drainage using a laboratory experimental tank. Most of slug tests' recovery curves were characteristic of compressible media, and important variability was observed depending on the initial head difference. The Darcy experiments on cubic samples provided reproducible results, and anisotropy (Kh > Kv) was observed for most of samples. All tracer experiments displayed asymmetrical breakthrough curves, suggesting the presence of retardation and/or dual porosity. Hydraulic conductivity estimates performed using the experimental tank showed K variations over a factor of 44 within the upper 40 cm of the acrotelm. The results demonstrate that the intrinsic variability associated with the different field and laboratory methods is small compared with the spatial variability of hydraulic parameters. It is suggested that a comprehensive assessment of peat hydrological properties can be obtained through the combined use of complementary field and laboratory investigations. Copyright © 2007 John Wiley & Sons, Ltd.  相似文献   

19.
Measurement of complex electrical conductivity as a function of frequency is an extremely sensitive probe for changes in pore and crack volume, crack connectivity, and crack surface topography. Such measurements have been made as a function of pore fluid chemistry, hydrostatic confining pressure, as well as uniaxial and triaxial deformation. This paper will; (1) describe the effects of triaxial deformation on the complex electrical conductivity of saturated porous rocks, (2) use the electrical data to model the mechanical stress-strain behaviour, and (3) compare the modelled behaviour with the stress-strain behaviour measured during the deformation. Experimental conductivity data tracks how the rock undergoes compaction with progressive loss of crack volume, followed by dilatation due to new crack formation, growth of existing cracks, crack interlinkage, and finally failure, as axial strain is increased. We have used the complex electrical data to produce a direction-sensitive (anisotropic) crack damage parameter, and used it to calculate the effective Young's modulus by employing the models of Walsh and Bruner. Comparison of the synthetic stress-strain curves so produced, with the experimentally derived stress-strain curves shows good agreement, particularly for undrained tests. This modelling is an improvement on similar curves produced using isotropic crack damage parameters derived from acoustic emission data. The improvement is likely to be due to the directional sensitivity of the electrical conductivity measurement, and its ability to discriminate between the formation of isolated cracks, and those cracks that contribute to the inter-connected crack space i.e. those cracks upon which transport properties of the rock such as electrical conductivity, and mechanical properties depend most critically during triaxial deformation.  相似文献   

20.
Considering heterogeneity in porous media pore size and connectivity is essential to predicting reactive solute transport across interfaces. However, exchange with less‐mobile porosity is rarely considered in surface water/groundwater recharge studies. Previous research indicates that a combination of pore‐fluid sampling and geoelectrical measurements can be used to quantify less‐mobile porosity exchange dynamics using the time‐varying relation between fluid and bulk electrical conductivity. For this study, we use macro‐scale (10 s of cm) advection–dispersion solute transport models linked with electrical conduction in COMSOL Multiphysics to explore less‐mobile porosity dynamics in two different types of observed sediment water interface porous media. Modeled sediment textures contrast from strongly layered streambed deposits to poorly sorted lakebed sands and cobbles. During simulated ionic tracer perturbations, a lag between fluid and bulk electrical conductivity, and the resultant hysteresis, is observed for all simulations indicating differential loading of pore spaces with tracer. Less‐mobile exchange parameters are determined graphically from these tracer time series data without the need for inverse numerical model simulation. In both sediment types, effective less‐mobile porosity exchange parameters are variable in response to changes in flow direction and fluid flux. These observed flow‐dependent effects directly impact local less‐mobile residence times and associated contact time for biogeochemical reaction. The simulations indicate that for the sediment textures explored here, less‐mobile porosity exchange is dominated by variable rates of advection through the domain, rather than diffusion of solute, for typical low‐to‐moderate rate (approximately 3–40 cm/day) hyporheic fluid fluxes. Overall, our model‐based results show that less‐mobile porosity may be expected in a range of natural hyporheic sediments and that changes in flowpath orientation and magnitude will impact less‐mobile exchange parameters. These temporal dynamics can be assessed with the geoelectrical experimental tracer method applied at laboratory and field scales.  相似文献   

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