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1.
The source and hydrochemical makeup of a stream reflects the connectivity between rainfall, groundwater, the stream, and is reflected to water quantity and quality of the catchment. However, in a semi-arid, thick, loess covered catchment, temporal variation of stream source and event associated behaviours are lesser known. Thus, the isotopic and chemical hydrographs in a widely distributed, deep loess, semi-arid catchment of the northern Chinese Loess Plateau were characterized to determine the source and hydrochemical behaviours of the stream during intra-rainfall events. Rainfall and streamflow were sampled during six hydrologic events coupled with measurements of stream baseflow and groundwater. The deuterium isotope (2H), major ions (Cl−, SO42−, NO3−, Ca2+, K+, Mg2+, and Na+) were evaluated in water samples obtained during rainfall events. Temporal variation of 2H and Cl− measured in the groundwater and stream baseflow prior to rainfall was similar; however, the isotope compositions of the streamflow fluctuated significantly and responded quickly to rainfall events, likely due to an infiltration excess, overland dominated surface runoff during torrential rainfall events. Time source separation using 2H demonstrated greater than 72% on average, the stream composition was event water during torrential rainfall events, with the proportion increasing with rainfall intensity. Solutes concentrations in the stream had loglinear relationships with stream discharge, with an outling anomaly with an example of an intra-rainfall event on Oct. 24, 2015. Stream Cl− behaved nonconservative during rainfall events, temporal variation of Cl− indicated a flush and washout at the onset of small rainfall events, a dilution but still high concentration pattern in high discharge and old water dominated in regression flow period. This study indicates rainfall intensity affects runoff responses in a semi-arid catchment, and the stored water in the thick, loess covered areas was less connected with stream runoff. Solute transport may threaten water quality in the area, requiring further analysis of the performance of the eco-restoration project.  相似文献   

2.
Stable isotope variations are extremely useful for flow partitioning within the hydrologic cycle but remain poorly understood throughout the tropics, particularly in watersheds with rapidly infiltrating soils, such as Andisols in Central America. This study examines the fluctuations of stable isotope ratios (δ18O and δ2H) in the hydrologic components of a tropical coffee agroforestry watershed (~1 km2) with Andisol soils in Costa Rica. Samples were collected in precipitation, groundwater, springs, and stream water over 2 years. The local meteoric water line for the study site was δ2H = 8.5 δ18O + 18.02 (r2 = 0.97, n = 198). The isotope ratios in precipitation exhibited an enriched trend during the dry season and a notable depletion at the beginning of the wet season. The δ18O compositions in groundwater (average = ?6.4‰, σ = 0.7) and stream water (average = ?6.7‰, σ = 0.6) were relatively stable over time, and both components exhibited more enriched values in 2013, which was the drier year. No strong correlation was observed between the isotope ratios and the precipitation amount at the event or daily time‐step, but a correlation was observed on a monthly scale. Stream water and base flow hydrograph separations based on isotope end‐member estimations showed that pre‐event water originating from base flow was prevalent. However, isotope data indicate that event water originating from springs appears to have been the primary driver of initial rises in stream flow and peak flows. These results indicate that isotope sampling improves the understanding of water balance components, even in a tropical humid location, where significant variations in rainfall challenge current modelling efforts. Further research using fine‐scale hydrometric and isotopic data would enhance understanding the processes driving spring flow generation in watersheds.  相似文献   

3.
Deuterium and oxygen‐18 are common environmental tracers in water used to investigate hydrological processes such as evaporation and groundwater recharge, and to trace moisture source. In this study, we collected event precipitation from 01 January 2010 to 28 February 2011 at a site in Changsha, Yangtze River Basin to estimate the influence of moisture source and atmospheric conditions on stable isotope compositions. The local meteoric water line, established as δD = (8.45 ± 0.13) δ18O + (17.7 ± 0.9) (r2 = 0.97, n = 189), had a higher slope and intercept than global meteoric water line. Temperature–δ18O exhibited complex correlations, with positive correlations during Nov.–Apr. superior to during Jun.–Sep., which was attributed to distinctive moisture sources, but vague the overall period; amount effect examined throughout the year. Linear regressions between δ18O and δD value in different precipitation event size classes revealed progressively decreasing slope and intercept values with decreasing precipitation amount and increasing vapour pressure deficit, indicating that small rainfall events (0–5 mm) were subject to secondary evaporation effects during rainwater descent. In contrast, snowfall and heavy precipitation events exhibited high slope and intercepts for the regression equation between δ18O and δD. High concentrations of heavy isotopes were associated with precipitation events sourced from remote westerly air masses, degenerated tropical marine air masses from the Bay of Bengal (BoB), and inland moisture in the pre‐monsoon period, as determined from backward trajectories assessed in the HYSPLIT model. Meanwhile, low concentrations of heavy isotopes were found to correspond with remote maritime moisture from BoB, the South China Sea, and the west Pacific at three different air pressures in summer monsoon and post‐monsoon using HYSPLIT and records of typhoon paths. These findings suggest that stable isotope compositions in precipitation events are closely associated with the meteorological conditions and respond sensitively to moisture source in subtropical monsoon climates. Copyright © 2013 John Wiley & Sons, Ltd.  相似文献   

4.
In snowmelt-driven mountain watersheds, the hydrologic connectivity between meteoric waters and stream flow generation varies strongly with the season, reflecting variable connection to soil and groundwater storage within the watershed. This variable connectivity regulates how streamflow generation mechanisms transform the seasonal and elevational variation in oxygen and hydrogen isotopic composition (δ18O and δD) of meteoric precipitation. Thus, water isotopes in stream flow can signal immediate connectivity or more prolonged mixing, especially in high-relief mountainous catchments. We characterized δ18O and δD values in stream water along an elevational gradient in a mountain headwater catchment in southwestern Montana. Stream water isotopic compositions related most strongly to elevation between February and March, exhibiting higher δ18O and δD values with decreasing elevation. These elevational isotopic lapse rates likely reflect increased connection between stream flow and proximal snow-derived water sources heavily subject to elevational isotopic effects. These patterns disappeared during summer sampling, when consistently lower δ18O and δD values of stream water reflected contributions from snowmelt or colder rainfall, despite much higher δ18O and δD values expected in warmer seasonal rainfall. The consistently low isotopic values and absence of a trend with elevation during summer suggest lower connectivity between summer precipitation and stream flow generation as a consequence of drier soils and greater transpiration. As further evidence of intermittent seasonal connectivity between the stream and adjacent groundwaters, we observed a late-winter flush of nitrate into the stream at higher elevations, consistent with increased connection to accumulating mineralized nitrogen in riparian wetlands. This pattern was distinct from mid-summer patterns of nitrate loading at lower elevations that suggested heightened human recreational activity along the stream corridor. These observations provide insights linking stream flow generation and seasonal water storage in high elevation mountainous watersheds. Greater understanding of the connections between surface water, soil water and groundwater in these environments will help predict how the quality and quantity of mountain runoff will respond to changing climate and allow better informed water management decisions.  相似文献   

5.
Water samples were collected from cold and warm karst springs for stable isotopes (δ18O and δD) and 3H from SE of Kashmir valley (western Himalayas) to distinguish the sources of recharge and infer their recharge areas. The spring water samples were most depleted in heavier isotopes in May (average δ18O: ?8.87‰ and δD: ?50.3‰) and enriched in September (average δ18O: ?7.58‰ and δD: ?48.1‰). The depleted 18O and 2H of spring waters bear the signatures of winter precipitation while as the enriched 18O and 2H of spring waters bear the signature of summer rainfall. D‐excess and 3H corroborate with the stable isotope results that the spring flow in spring season (May) and autumn (September) is dominantly controlled by the melting of winter snowmelt and summer rainfall, respectively. The results showed that unlike δD, the δ18O value in the karst spring waters decreases in January suggesting δ18O shift. The spring water samples also fall above the Local Meteoric Water Line and Global Meteoric Water Line indicating the δ18O shift due to interaction of groundwater with the host carbonate rocks during its traverse. The mean elevation of the recharge areas of the springs using δ18O and δD tracers was also estimated. Copyright © 2014 John Wiley & Sons, Ltd.  相似文献   

6.
Rapidly transforming headwater catchments in the humid tropics provide important resources for drinking water, irrigation, hydropower, and ecosystem connectivity. However, such resources for downstream use remain unstudied. To improve understanding of the behaviour and influence of pristine rainforests on water and tracer fluxes, we adapted the relatively parsimonious, spatially distributed tracer‐aided rainfall–runoff (STARR) model using event‐based stable isotope data for the 3.2‐km2 San Lorencito catchment in Costa Rica. STARR was used to simulate rainforest interception of water and stable isotopes, which showed a significant isotopic enrichment in throughfall compared with gross rainfall. Acceptable concurrent simulations of discharge (Kling–Gupta efficiency [KGE] ~0.8) and stable isotopes in stream water (KGE ~0.6) at high spatial (10 m) and temporal (hourly) resolution indicated a rapidly responding system. Around 90% of average annual streamflow (2,099 mm) was composed of quick, near‐surface runoff components, whereas only ~10% originated from groundwater in deeper layers. Simulated actual evapotranspiration (ET) from interception and soil storage were low (~420 mm/year) due to high relative humidity (average 96%) and cloud cover limiting radiation inputs. Modelling suggested a highly variable groundwater storage (~10 to 500 mm) in this steep, fractured volcanic catchment that sustains dry season baseflows. This groundwater is concentrated in riparian areas as an alluvial–colluvial aquifer connected to the stream. This was supported by rainfall–runoff isotope simulations, showing a “flashy” stream response to rainfall with only a moderate damping effect and a constant isotope signature from deeper groundwater (~400‐mm additional mixing volume) during baseflow. The work serves as a first attempt to apply a spatially distributed tracer‐aided model to a tropical rainforest environment exploring the hydrological functioning of a steep, fractured‐volcanic catchment. We also highlight limitations and propose a roadmap for future data collection and spatially distributed tracer‐aided model development in tropical headwater catchments.  相似文献   

7.
Stable isotopes of water have been widely used in understanding the hydrological functions of alpine inland catchments. This study identifies dominant runoff generation mechanisms based on isotopic data (δ18O and δ2H) of 487 rainwater and river-water samples from three tributaries in the Tarim River Basin in China for the period May–September 2013. The isotope hydrograph separation results provide a comprehensive overview of the rainfall influence on hydrological processes. Stream water and groundwater have varied responses to different intensities of rainfall events. Only a small proportion of rainfall is directly transported to the stream during such events. An inconsistent temporal trend of event water contribution is observed in the three catchments. The average fractional contributions of rainfall for the Tizinafu, Kumalak and Huangshuigou rivers are 10.3% (±1.1%), 9.7% (±2.9%) and 8.7% (±2.4%), respectively.  相似文献   

8.
Models simulating stream flow and conservative tracers can provide a representation of flow paths, storage distributions and mixing processes that is advantageous for many predictive purposes. Compared with models that only simulate stream flow, tracer data can be used to investigate the internal consistency of model behaviour and to gain insight into model performance. Here, we examine the strengths and weaknesses of a data‐driven, spatially distributed tracer‐aided rainfall‐runoff model. The model structure allowed us to assess the influence of landscape characteristics on the routing and mixing of water and tracers. The model was applied to a site in the Scottish Highlands with a unique tracer data set; ~4 years of daily isotope ratios in stream water and precipitation were available, as well as 2 years of weekly soil and ground water isotopes. The model structure was based on an empirically based, lumped tracer‐aided model previously developed for the catchment. The best model runs were selected from Monte Carlo simulations based on dual calibration criteria using objective functions for both stream isotopes and discharge at the outlet. Model performance for these criteria was reasonable (Nash–Sutcliffe efficiencies for discharge and isotope ratios were ~0.4–0.6). The model could generally reproduce the variable isotope signals in the soils of the steeper hill slopes where storage was low, and damped isotope responses in valley bottom cells with high storage. The model also allowed us to estimate the age distributions of internal stores, water fluxes and stream flow. Average stream water age was ~1.6 years, integrating older groundwater in the valley bottom and dynamic younger soil waters. By tracking water ages and simulating isotopes, the model captured the changes in connectivity driven by distributed storage dynamics. This has substantially improved the representation of spatio‐temporal process dynamics and gives a more robust framework for projecting environmental change impacts. Copyright © 2016 The Authors Hydrological Processes Published by John Wiley & Sons Ltd.  相似文献   

9.
We characterize the precipitation and groundwater in a mountainous (peaks slightly above 3000 m a.s.l.), semi‐arid river basin in SE Spain in terms of the isotopes 18O and 2H. This basin, with an extension of about 7000 km2, is an ideal site for such a study because fronts from the Atlantic and the Mediterranean converge here. Much of the land is farmed and irrigated both by groundwater and runoff water collected in reservoirs. A total of approximately 100 water samples from precipitation and 300 from groundwater have been analysed. To sample precipitation we set up a network of 39 stations at different altitudes (800–1700 m a.s.l.), with which we were able to collect the rain and snowfall from 29 separate events between July 2005 and April 2007 and take monthly samples during the periods of maximum recharge of the aquifers. To characterize the groundwater we set up a control network of 43 points (23 springs and 20 wells) to sample every 3 months the main aquifers and both the thermal and non‐thermal groundwater. We also sampled two shallow‐water sites (a reservoir and a river). The isotope composition of the precipitation forms a local meteoric water line (LMWL) characterized by the equation δD = 7·72δ18O + 9·90, with mean values for δ18O and δD of − 10·28‰ and − 69·33‰, respectively, and 12·9‰ for the d‐excess value. To correlate the isotope composition of the rainfall water with groundwater we calculated the weighted local meteoric water line (WLMWL), characterized by the equation δD = 7·40δ18O + 7·24, which takes into account the quantity of water precipitated during each event. These values of (dδD/dδ18O)< 8 and d‐excess (δD–8δ18O)< 10 in each curve bear witness to the ‘amount effect’, an effect which is more manifest between May and September, when the ground temperature is higher. Other effects noted in the basin were those of altitude and the continental influence. The isotopic compositions of the groundwater are represented by the equation δD = 4·79δ18O − 18·64. The groundwater is richer in heavy isotopes than the rainfall, with mean values of − 8·48‰ for δ18O and − 59·27‰ for δD. The isotope enrichment processes detected include a higher rate of evaporation from detrital aquifers than from carbonate ones, the effects of recharging aquifers from irrigation return flow and/or from reservoirs' leakage and enrichment in δ18O from thermal water. Copyright © 2010 John Wiley & Sons, Ltd.  相似文献   

10.
Understanding the isotopic composition of precipitation in a forested catchment is critical for ecohydrological studies. Changes in the water isotopes of rainfall were assessed during its passage through the canopy in throughfall, and the effect of different forest stands on the isotope composition of throughfall. In a cool temperate forest in Korea, rainfall and throughfall samples collected under Pinus densiflora (red pine), Castanea crenata (chestnut), Robinia pseudoacacia (black locust) and mixed stands (mix of these three species) were analysed for oxygen and hydrogen isotopes. Throughfall δ18O and δD were enriched compared to rainfall. A difference of δ18O and δD among throughfall may be related to the difference in interception–storage capacity of different species due to dissimilar canopy characteristics. Since isotopic composition of throughfall and rainfall are different due to canopy isotopic effects, use of rainfall isotopic signatures for ecohydrological studies in forested ecosystem can lead to biases.  相似文献   

11.
Three main reservoirs were identified that contribute to the shallow subsurface flow regime of a valley drained by a fourth‐order stream in Brittany (western France). (i) An upland flow that supplied a wetland area, mainly during the high‐water period. It has high N‐NO3? and average Cl? concentrations. (ii) A deep confined aquifer characterized by low nitrate and low chloride concentrations that supplied the floodplain via flow upwelling. (iii) An unconfined aquifer under the riparian zone with high Cl? and low N‐NO3? concentrations where biological processes removed groundwater nitrate. This aquifer collected the upland flow and supplied a relict channel that controlled drainage from the whole riparian zone. Patterns of N‐NO3? and Cl? concentrations along riparian transects, together with calculated high nitrate removal, indicate that removal occurred mainly at the hillslope–riparian zone interface (i.e. first few metres of wetland), whereas dilution occurred in lower parts of the transects, especially during low‐water periods and at the beginning of recharge periods. Stream flow was modelled as a mixture of water from the three reservoirs. An estimation of these contributions revealed that the deep aquifer contribution to stream flow averaged 37% throughout the study period, while the contribution of the unconfined reservoir below the riparian zone and hillslope flow was more variable (from ca 6 to 85%) relative to rainfall events and the level of the riparian water table. At the entire riparian zone scale, NO3? removal (probably from denitrification) appeared most effective in winter, despite higher estimated upland NO3? fluxes entering the riparian zone during this period. Copyright © 2003 John Wiley & Sons, Ltd.  相似文献   

12.
It is often assumed that stable water isotopes (δD and δ18O) provide redundant information for a given sample of water. In this note we illustrate that the choice of isotope used may influence the resultant hydrograph separation. This is especially true in light of the spatial and temporal variability in the isotopic composition of rainfall water at the catchment scale. We present several possible hydrograph separations based on both δD and δ18O observed in rainfall for a single runoff event occurring in the southwest USA. This study demonstrates the potential of using both stable water isotopes by showing that δD and δ18O may provide unique information for catchment hydrologists. We also report on the utility of new technology capable of simultaneous measurements of both δD and δ18O using off‐axis integrated cavity output spectroscopy (OA‐ICOS) methods. This may be of interest to catchment hydrologists seeking to incorporate this type of equipment into their laboratory. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

13.
Characterization of spatial and temporal variability of stable isotopes (δ18O and δ2H) of surface waters is essential to interpret hydrological processes and establish modern isotope–elevation gradients across mountainous terrains. Here, we present stable isotope data for river waters across Kyrgyzstan. River water isotopes exhibit substantial spatial heterogeneity among different watersheds in Kyrgyzstan. Higher river water isotope values were found mainly in the Issyk‐Kul Lake watershed, whereas waters in the Son‐Kul Lake watershed display lower values. Results show a close δ18O–δ2H relation between river water and the local meteoric water line, implying that river water experiences little evaporative enrichment. River water from the high‐elevation regions (e.g., Naryn and Son‐Kul Lake watershed) had the most negative isotope values, implying that river water is dominated by snowmelt. Higher deuterium excess (average d = 13.9‰) in river water probably represents the isotopic signature of combined contributions from direct precipitation and glacier melt in stream discharge across Kyrgyzstan. A significant relationship between river water δ18O and elevation was observed with a vertical lapse rate of 0.13‰/100 m. These findings provide crucial information about hydrological processes across Kyrgyzstan and contribute to a better understanding of the paleoclimate/elevation reconstruction of this region.  相似文献   

14.
In the McMurdo Dry Valleys of Antarctica, glaciers are the source of meltwater during the austral summer, and the streams and adjacent hyporheic zones constitute the entire physical watershed; there are no hillslope processes in these systems. Hyporheic zones can extend several metres from each side of the stream, and are up to 70 cm deep, corresponding to a lateral cross‐section as large as 12 m2, and water resides in the subsurface year around. In this study, we differentiate between the near‐stream hyporheic zone, which can be characterized with stream tracer experiments, and the extended hyporheic zone, which has a longer time‐scale of exchange. We sampled stream water from Green Creek and from the adjacent saturated alluvium for stable isotopes of D and 18O to assess the significance and extent of stream‐water exchange between the streams and extended hyporheic zones over long time‐scales (days to weeks). Our results show that water residing in the extended hyporheic zone is much more isotopically enriched (up to 11‰ D and 2·2‰ 18O) than stream water. This result suggests a long residence time within the extended hyporheic zone, during which fractionation has occurred owing to summer evaporation and winter sublimation of hyporheic water. We found less enriched water in the extended hyporheic zone later in the flow season, suggesting that stream water may be exchanged into and out of this zone, on the time‐scale of weeks to months. The transient storage model OTIS was used to characterize the exchange of stream water with the extended hyporheic zone. Model results yield exchange rates (α) generally an order magnitude lower (10?5 s?1) than those determined using stream‐tracer techniques on the same stream. In light of previous studies in these streams, these results suggest that the hyporheic zones in Antarctic streams have near‐stream zones of rapid stream‐water exchange, where ‘fast’ biogeochemical reactions may influence water chemistry, and extended hyporheic zones, in which slower biogeochemical reaction rates may affect stream‐water chemistry at longer time‐scales. Copyright © 2003 John Wiley & Sons, Ltd.  相似文献   

15.
To understand the moisture regime at the southern slopes of Mt. Kilimanjaro, we analysed the isotopic variability of oxygen (δ18O) and hydrogen (δD) of rainfall, throughfall, and fog from a total of 2,140 samples collected weekly over 2 years at 9 study sites along an elevation transect ranging from 950 to 3,880 m above sea level. Precipitation in the Kilimanjaro tropical rainforests consists of a combination of rainfall, throughfall, and fog. We defined local meteoric water lines for all 3 precipitation types individually and the overall precipitation, δDprec = 7.45 (±0.05) × δ18Oprec + 13.61 (±0.20), n  = 2,140, R 2 = .91, p  < .001. We investigated the precipitation‐type‐specific stable isotope composition and analysed the effects of amount, altitude, and temperature. Aggregated annual mean values revealed isotope composition of rainfall as most depleted and fog water as most enriched in heavy isotopes at the highest elevation research site. We found an altitude effect of δ18Orain = ?0.11‰ × 100 m?1, which varied according to precipitation type and season. The relatively weak isotope or altitude gradient may reveal 2 different moisture sources in the research area: (a) local moisture recycling and (b) regional moisture sources. Generally, the seasonality of δ18Orain values follows the bimodal rainfall distribution under the influences of south‐ and north‐easterly trade winds. These seasonal patterns of isotopic composition were linked to different regional moisture sources by analysing Hybrid Single Particle Lagrangian Integrated Trajectory backward trajectories. Seasonality of d excess values revealed evidence of enhanced moisture recycling after the onset of the rainy seasons. This comprehensive dataset is essential for further research using stable isotopes as a hydrological tracer of sources of precipitation that contribute to water resources of the Kilimanjaro region.  相似文献   

16.
Two‐component hydrograph separation was performed on 19 low‐to‐moderate intensity rainfall events in a 4·1‐km2 urban watershed to infer the relative and absolute contribution of surface runoff (e.g. new water) to stormflow generation between 2001 and 2003. The electrical conductivity (EC) of water was used as a continuous and inexpensive tracer, with order of magnitude differences in precipitation (12–46 µS/cm) and pre‐event streamwater EC values (520–1297 µS/cm). While new water accounted for most of the increased discharge during storms (61–117%), the contribution of new water to total discharge during events was typically lower (18–78%) and negatively correlated with antecedent stream discharge (r2 = 0·55, p < 0·01). The amount of new water was positively correlated with total rainfall (r2 = 0·77), but hydrograph separation results suggest that less than half (9–46%) of the total rainfall on impervious surfaces is rapidly routed to the stream channel as new water. Comparison of hydrograph separation results using non‐conservative tracers (EC and Si) and a conservative isotopic tracer (δD) for two events showed similar results and highlighted the potential application of EC as an inexpensive, high frequency tracer for hydrograph separation studies in urban catchments. The use of a simple tracer‐based approach may help hydrologists and watershed managers to better understand impervious surface runoff, stormflow generation and non‐point‐source pollutant loading to urban streams. Copyright © 2007 John Wiley & Sons, Ltd.  相似文献   

17.
Riparian vegetation is important for stream functioning and as a major landscape feature. For many riparian plants, shallow groundwater is an important source of water, particularly in areas where rainfall is low, either annually or seasonally, and when extended dry conditions prevail for all or part of the year. The nature of tree water relationships is highly complex. Therefore, we used multiple lines of evidence to determine the water sources used by the dominant tree species Eucalyptus camaldulensis (river red gum), growing in riparian and floodplain areas with varying depth to groundwater and stream perenniality. Dendrometer bands were used to measure diel, seasonal, and annual patterns of tree water use and growth. Water stable isotopes (δ2H and δ18O) in plant xylem, soil water, and groundwater were measured to determine spatial and temporal patterns in plant water source use. Our results indicated riparian trees located on relatively shallow groundwater had greater growth rates, larger diel responses in stem diameter, and were less reactive to extended dry periods, than trees in areas of deep groundwater. These results were supported by isotope analysis that suggested all trees used groundwater when soil water stores were depleted at the end of the dry season, and this was most pronounced for trees with shallow groundwater. Trees may experience more frequent periods of water deficit stress and undergo reduced productivity in scenarios where water table accessibility is reduced, such as drawdown from groundwater pumping activities or periods of reduced rainfall recharge. The ability of trees to adapt to changing groundwater conditions may depend on the speed of change, the local hydrologic and soil conditions as well as the species involved. Our results suggest that E. camaldulesis growing at our study site is capable of utilizing groundwater even to depths >10 m, and stream perenniality is likely to be a useful indicator of riparian tree use of groundwater.  相似文献   

18.
This work provides a comprehensive physically based framework for the interpretation of the north Australian rainfall stable isotope record (δ18O and δ2H). Until now, interpretations mainly relied on statistical relationships between rainfall amount and isotopic values on monthly timescales. Here, we use multiseason daily rainfall stable isotope and high resolution (10 min) ground‐based C‐band polarimetric radar data and show that the five weather types (monsoon regimes) that constitute the Australian wet season each have a characteristic isotope ratio. The data suggest that this is not only due to changes in regional rainfall amount during these regimes but, more importantly, is due to different rain and cloud types that are associated with the large scale circulation regimes. Negative (positive) isotope anomalies occurred when stratiform rainfall fractions were large (small) and the horizontal extent of raining areas were largest (smallest). Intense, yet isolated, convective conditions were associated with enriched isotope values whereas more depleted isotope values were observed when convection was widespread but less intense. This means that isotopic proxy records may record the frequency of which these typical wet season regimes occur. Positive anomalies in paleoclimatic records are most likely associated with periods where continental convection dominates and convection is sea‐breeze forced. Negative anomalies may be interpreted as periods when the monsoon trough is active, convection is of the oceanic type, less electric, and stratiform areas are wide spread. This connection between variability of rainfall isotope anomalies and the intrinsic properties of convection and its large‐scale environment has important implications for all fields of research that use rainfall stable isotopes.  相似文献   

19.
Understanding the influence of storm events on nitrate (NO3?) dynamics is important for efficiently managing NO3? pollution. In this study, five sites representing a downstream progression of forested uplands underlain by resistant sandstone to karst lowlands with agricultural, urban and mixed land‐use were established in Spring Creek, a 201 km2 mixed land‐use watershed in central Pennsylvania, USA. At each site, stream water was monitored during six storm events in 2005 to assess changes in stable isotopes of NO3? (δ15N‐NO3? and δ18O‐NO3?) and water (δ18O‐H2O) from baseflow to peakflow. Peakflow fractions of event NO3? and event water were then computed using two‐component mixing models to elucidate NO3? flow pathway differences among the five sites. For the forested upland site, storm size appeared to affect NO3? sources and flow pathways. During small storms (<35 mm rainfall), greater event NO3? fractions than event water fractions indicated the prevalence of atmospheric NO3? source contributions at peakflow. During larger storms (>35 mm rainfall), event NO3? fractions were less than event water fractions at peakflow suggesting that NO3? was flushed from stored sources via shallow subsurface flow pathways. For the urbanized site, wash‐off of atmospheric NO3? was an important NO3? source at peakflow, especially during short‐duration storms where event water contributions indicated the prevalence of overland flow. In the karst lowlands, very low fractions of event water and even lower fractions of event NO3? at peakflow suggested the dominance of ground water flow pathways during storms. These ground water flow pathways likely flushed stored NO3? sources into the stream, while deep soils in the karst lowlands also may have promoted NO3? assimilation. The results of this study illustrated how NO3? isotopes and δ18O‐H2O could be combined to show key differences in water and NO3? delivery between forested uplands, karst valleys and fully urbanized watersheds. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

20.
High‐frequency sampling of stable water isotopes in precipitation and stream water during winter and summer storm events was carried out in a 2·3 km2 lowland agricultural catchment. During peak flows of monitored events, the responses of δ2H and δ18O were comparable and inferred the dominance (ca 70%) of ‘old’ pre‐event water. Transit Time Distribution (TTD) inferred by a gamma function were fitted (Nash–Sutcliffe = 0·8) and were also similar for δ2H and δ18O. However, the shape (α) and scaling (β) parameters were markedly different for summer and winter events. Consequently, when antecedent wetness was high, mean transit times were in the order of days; when drier, they increased to months. Moreover, while the responses of δ2H and δ18O exhibited similar gradual recovery to pre‐event conditions during winter hydrograph recessions, they differed dramatically on summer recessions. Time series analysis showed that δ2H isotope content was correlated with the diurnal cycle of air temperature, suggesting an evaporative fractionation pattern which could be reproduced by a temperature‐based first‐order autoregressive model. The heavier δ18O isotope showed no evidence for such diurnal variability. The study highlights the utility of high‐frequency stable isotope sampling to explore the time‐variant nature of TTDs. Furthermore, it shows that the time of sampling in a diurnal cycle may have crucial significance for interpreting stream isotope signatures, particularly δ2H. Copyright © 2011 John Wiley & Sons, Ltd.  相似文献   

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