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1.
The production rate of cosmogenic 3He in apatite, zircon, kyanite and garnet was obtained by cross-calibration against 10Be in co-existing quartz in glacial moraine boulders from the Nepalese Himalaya. The boulders have 10Be ages between 6 and 16 kyr and span elevations from 3200 to 4800 m. In all of these minerals 3He correlates with 10Be and is dominantly cosmogenic in origin. After modest correction for non-cosmogenic components, 3He/10Be systematics imply apparent sea-level high-latitude (SLHL) apparent production rates for 3He of 226 atoms g? 1 yr? 1 in zircon, 254 atoms g? 1 yr? 1 in apatite, 177 atoms g? 1 yr? 1 in kyanite, and 153 atoms g? 1 yr? 1 in garnet. These production rates are unexpectedly high compared with rates measured elsewhere in the world, and also compared with proposed element-specific production rates. For apatite and zircon, the data are sufficient to conclude that the 3He/10Be ratio increases with elevation. If this reflects different altitudinal scaling between production rates for the two isotopes then the SLHL production rates estimated by our approach are overestimates. We consider several hypotheses to explain these observations, including production of 3He via thermal neutron capture on 6Li, altitudinal variations in the energy spectrum of cosmic-ray neutrons, and the effects of snow cover. Because all of these effects are small, we conclude that the altitudinal variations in production rates of cosmogenic 3He and 10Be are distinct from each other at least at this location over the last ～ 10 kyr. This conclusion calls into question commonly adopted geographic scaling laws for at least some cosmogenic nuclides. If confirmed, this distinction may provide a mechanism by which to obtain paleoelevation estimates.  相似文献   

2.
Over the last decades, cosmogenic exposure dating has permitted major advances in many fields of Earth surface sciences and particularly in paleoglaciology. Yet, exposure age calculation remains a complicated and dense procedure. It requires numerous choices of parameterization and the use of an accurate production rate.This study describes the CREp program (http://crep.crpg.cnrs-nancy.fr) and the ICE-D production rate online database (http://calibration.ice-d.org). This system is designed so that the CREp calculator will automatically reflect the current state of this global calibration database production rate, ICE-D. ICE-D will be regularly updated in order to incorporate new calibration data and reflect the current state of the available literature.CREp is a Octave/Matlab© online code that computes Cosmic Ray Exposure (CRE) ages for 3He and 10Be. A stand-alone version of the CREp code is also released with the present article. Note however that only the online version is connected to the online database ICE-D. The CREp program offers the possibility to calculate ages with two scaling models: i.e. the empirical Lal-Stone time-dependent model (Balco et al., 2008; Lal, 1991; Stone, 2000) with the muon parameters of Braucher et al. (2011), and the Lifton-Sato-Dunai (LSD) theoretical model (Lifton et al., 2014). The default atmosphere model is the ERA-40 database (Uppala et al., 2005), but one may also use the standard atmosphere for comparison (N.O.A.A, 1976). To perform the time-dependent correction, users may import their own geomagnetic database for paleomagnetic corrections or opt for one of the three proposed datasets (Lifton, 2016; Lifton et al., 2014; Muscheler et al., 2005).For the important choice of the production rate, CREp is linked to a database of production rate calibration data that is part of the ICE-D (Informal Cosmogenic-nuclide Exposure-age Database) project (http://calibration.ice-d.org). This database includes published empirical calibration rate studies that are publicly available at present, comprising those of the CRONUS-Earth and CRONUS-EU projects, as well as studies from other projects. In the present study, the efficacy of the different scaling models has also been evaluated looking at the statistical dispersion of the computed Sea Level High Latitude (SLHL) production rates. Lal/Stone and LSD models have comparable efficacies, and the impact of the tested atmospheric model and the geomagnetic database is also limited.Users however have several possibilities to select the production rate: 1) using a worldwide mean value, 2) a regionally averaged value (not available in regions with no data), 3) a local unique value, which can be chosen among the existing dataset or imported by the user, or 4) any combination of multiple calibration data.If a global mean is chosen, the 1σ uncertainty arising from the production rate is about 5% for 10Be and 10% for 3He. If a regional production rate is picked, these uncertainties are potentially lower.CREp is able to calculate a large number of ages in a reasonable time (typically < 30 s for 50 samples). The user may export a summary table of the computed ages and the density probability function associated with each age (in the form of a spreadsheet).  相似文献   

3.
Well-dated records of tropical glacier fluctuations are essential for developing hypotheses and testing proposed mechanisms for past climate changes. Since organic material for radiocarbon dating is typically scarce in low-latitude, high-altitude environments, surface exposure-age dating, based on the measurement of in situ produced cosmogenic nuclides, provides much of the chronologic information on tropical glacier moraines. Here, we present a locally calibrated 10Be production rate for a low-latitude, high-altitude site near Quelccaya Ice Cap (∼13.95°S, 70.89°W, 4857 m asl) in the southeastern Peruvian Andes. Using an independent age (12.35 +0.2, −0.02 ka) of the late glacial Huancané IIa moraines based on thirty-four bracketing radiocarbon ages and twelve 10Be concentrations of boulders on the moraines, we determine a local production rate of 43.28 ± 2.69 atoms gram−1 year−1 (at g−1 yr−1). Reference 10Be production rates (i.e., production rates by neutron spallation appropriate for sea-level, high-latitude sites) range from 3.97 ± 0.09 to 3.78 ± 0.09 at g−1 yr−1, determined using scaling after Lal (1991) and Stone (2000) and depending on our assumed boulder surface erosion rate. Since our boulder surface erosion rate estimate is a minimum value, these reference production rates are also minimum values. A secondary control site on the Huancané IIIb moraines suggests that the 10Be production rates are at least as low as, or possibly lower than, those derived from the Huancané IIa moraines. These sea-level, high-latitude production rates are at least 11–15% lower than values derived using the traditional global calibration dataset, and they are also lower than those derived from the late glacial Breque moraine in the Cordillera Blanca of Peru. However, our sea-level, high-latitude production rates agree well with recently published, locally calibrated production rates from the Arctic, New Zealand, and Patagonia. The production rates presented here should be used to calculate 10Be exposure ages in low-latitude, high-altitude locations, particularly in the tropical Andes, and should improve the ability to compare the results of studies using 10Be exposure-age dating with other chronological data.  相似文献   

4.
Well-dated bedrock surfaces associated with the highstand and subsequent catastrophic draining of Pleistocene Lake Bonneville, Utah, during the Bonneville flood are excellent locations for in situ cosmogenic nuclide production rate calibration. The CRONUS-Earth project sampled wave-polished bedrock and boulders on an extensive wave-cut bench formed during the Bonneville-level highstand that was abandoned almost instantaneously during the Bonneville flood. CRONUS-Earth also sampled the Tabernacle Hill basalt flow that erupted into Lake Bonneville soon after its stabilization at the Provo level, following the flood. New radiocarbon dating results from tufa at the margins of Tabernacle Hill as part of this study have solidified key aspects of the exposure history at both sites. Both sites have well-constrained exposure histories in which factors such as potential prior exposure, erosion, and shielding are either demonstrably negligible or quantifiable. Multi-nuclide analyses from multiple labs serve as an ad hoc inter-laboratory comparison that supplements and expands on the formalized CRONUS-Earth and CRONUS-EU inter-laboratory comparisons (Blard et al., 2015; Jull et al., 2015; Vermeesch et al., 2015). Results from 10Be, 26Al, and 14C all exhibit scatter comparable to that observed in the CRONUS-Earth effort. Although a 36Cl inter-laboratory comparison was not completed for Jull et al. (2015), 36Cl from plagioclase mineral separates exhibits comparable reproducibility. Site production rates derived from these measurements provide valuable input to the global production rate calibration described by Borchers et al. (2015). Whole-rock 36Cl concentrations, however, exhibit inter-laboratory variation exceeding analytical uncertainty and outside the ranges observed for the other nuclides (Jull et al., 2015). A rigorous inter-laboratory comparison studying the systematics of whole-rock 36Cl extraction techniques is currently underway with the goals of delineating the source(s) of this discrepancy and standardizing these procedures going forward.  相似文献   

5.
An important constraint on the reliability of cosmogenic nuclide exposure dating is the rigorous determination of production rates. We present a new dataset for 10Be production rate calibration from Mount Billingen, southern Sweden, the site of the final drainage of the Baltic Ice Lake, an event dated to 11,620 ± 100 cal yr BP. Five samples of flood-scoured bedrock surfaces (58.5°N, 13.7°E, 105–120 m a.s.l.) unambiguously connected to the drainage event yield a reference 10Be production rate of 4.19 ± 0.20 atoms g−1 yr−1 for the CRONUS-Earth online calculator Lm scaling and 4.02 ± 0.18 atoms g−1 yr−1 for the nuclide specific LSDn scaling. We also recalibrate the reference 10Be production rates for four sites in Norway and combine three of these with the Billingen results to derive a tightly clustered Scandinavian reference 10Be production rate of 4.13 ± 0.11 atoms g−1 yr−1 for the CRONUS Lm scaling and 3.95 ± 0.10 atoms g−1 yr−1 for the LSDn scaling scheme.  相似文献   

6.
A combination of numerical analysis and 10Be concentrations measured in sediment samples from the high‐relief Torrente catchment, southern Spain, allows us to investigate the sampling requirements for determining erosion rates using cosmogenic nuclides in high‐relief, landslide‐dominated terrain. We use simple modelling to quantify the effect of particle spalling and/or landsliding on erosion rates determined using a cosmogenic in‐situ produced isotope. Analytical results show that the cosmogenic nuclide concentration of a surface experiencing regular detachment of a grain or block may be considered to be in steady state, and ‘in‐situ’ erosion rates estimated, when an appropriate number of spatially independent samples are amalgamated. We present equations that enable calculation of the number of bedrock samples that must be amalgamated for the estimation of mean erosion rates on an outcrop experiencing regular detachment of a grain or chip of thickness L every T years. Our findings confirm that mean catchment erosion rates may be reliably estimated from 10Be concentrations in fluvial sediment in high‐relief rapidly eroding terrain. These catchment‐wide integrated erosion rates can be calculated where erosion is primarily accomplished through shallow (<3 m) spalling processes; where deep‐seated (>3 m) landslides are the dominant mode of erosion only minimum erosion rates can be determined. Lastly, we present erosion rate measurements from the Torrente catchment that reveal variation of two orders of magnitude (0·03–1·6 m ka?1) quantifying the high degree of spatial variation in erosion rates expected within rapidly uplifting catchments. Copyright © 2006 John Wiley & Sons, Ltd.  相似文献   

7.
In situ Terrestrial Cosmogenic Nuclides (hereafter TCNs) are increasingly important for absolutely dating terrestrial events and processes. This study aimed at improving our knowledge of the production rate of Terrestrial Cosmogenic 3He formed in situ in rock surfaces at low latitude and sea level as well as re-evaluation of the Canary Islands as a calibration site for TCNs. For this purpose, we sampled basaltic lava flows from some of the youngest and yet undated volcanic sites and used the 40Ar/39Ar incremental heating method on groundmass samples and in situ cosmogenic 3He on olivine and clinopyroxene phenocrysts. 40Ar/39Ar analysis was done on a Hiden HAL Series 1000 triple filter quadrupole mass spectrometer with extraction furnace. Incremental heating data shows ages in the Late Pleistocene from 52.7 ± 21.6 ka to 398.6 ± 27.6 ka.We measured cosmogenic 3He concentrations in olivine and clinopyroxene phenocrysts from flow top samples on a MAP 215-50 sector mass spectrometer with a crushing device and a diode laser extraction system. Exposure age calculations yielded ages in the range 38.9 ± 4.0 ka to 62.3 ± 6.7 ka for the youngest lava flow and the data series is in broad agreement with the argon data up to 250 ka and reveals a more continuous time line of volcanism during the late Pleistocene on the island. However, the dataset was not sufficient for calculation of production rates for in situ Terrestrial Cosmogenic 3He as many samples showed signs of erosion. Calculated erosion rates range from none to as high as 7.3 mm/kyr assuming a rock density of 2.9 g/cm2. This finding puts a constraint on the use of Fuerteventura as a calibration site for exposure histories older than 50–100 ka. A comparison with cosmogenic 36Cl data supports these findings and indicates substantial weathering.  相似文献   

8.
Stable cosmogenic isotopes such as 3He and 21Ne are useful for dating of diverse lithologies, quantifying erosion rates and ages of ancient surfaces and sediments, and for assessing complex burial histories. Although many minerals are potentially suitable targets for 3He and 21Ne dating, complex production systematics require calibration of each mineral–isotope pair. We present new results from a drill core in a high-elevation ignimbrite surface, which demonstrates that cosmogenic 3He and 21Ne can be readily measured in biotite and hornblende. 21Ne production rates in hornblende and biotite are similar, and are higher than that in quartz due to production from light elements such as Mg and Al. We measure 21Nehbl/21Neqtz = 1.35 ± 0.03 and 21Nebio/21Neqtz = 1.3 ± 0.02, which yield production rates of 25.6 ± 3.0 and 24.7 ± 2.9 at g? 1 yr? 1 relative to a 21Neqtz production rate of 19.0 ± 1.8 at g? 1 yr? 1. We show that nucleogenic 21Ne concentrations produced via the reaction 18O(α,n)21Ne are manageably small in this setting, and we present a new approach to deconvolve nucleogenic 21Ne by comparison to nucleogenic 22Ne produced from the reaction 19F(α,n)22Ne in F-rich phases such as biotite. Our results show that hornblende is a suitable target phase for cosmogenic 3He dating, but that 3He is lost from biotite at Earth surface temperatures. Comparison of 3He concentrations in hornblende with previously measured mineral phases such as apatite and zircon provides unambiguous evidence for 3He production via the reaction 6Li(n,α)3H → 3He. Due to the atypically high Li content in the hornblende (~ 160 ppm) we estimate that Li-produced 3He represents ~ 40% of total 3He production in our samples, and must be considered on a sample-specific basis if 3He dating in hornblende is to be widely implemented.  相似文献   

9.
Precise 40Ar/39Ar age determinations made on basalt groundmass collected from the SP and upper and lower Bar Ten lava flows in the San Francisco and Uinkaret volcanic fields of Arizona, USA, yield ages of 72 ± 4, 97 ± 10, and 123 ± 12 ka (2σ; relative to Renne et al., 2010, 2011, full external precision), respectively. Previous ages of the SP lava flow include a K–Ar age of 70 ± 8 ka and OSL ages of 5.5–6 ka. 40Ar/39Ar age constraints, relative to the optimization model of Renne et al. (2010, 2011), of 81 ± 50 and 118 ± 64 ka (2σ; full external precision) were previously reported for the upper and lower Bar Ten lava flows, respectively. The new 40Ar/39Ar ages are within uncertainty of previous age constraints, and are more robust, accurate, and precise. Preliminary cosmogenic 3He and 21Ne production rates from the Bar Ten flows reported by Fenton et al. (2009) are updated here, to account for the improved quality of the 40Ar/39Ar data. The new 40Ar/39Ar age for the SP flow yields cosmogenic 3He and 21Ne production rates for pyroxene (119 ± 8 and 26.8 ± 1.9 at/g/yr; error-weighted mean, 2σ uncertainty; Dunai (2000) scaling method) that are consistent with production rate values reported throughout the literature. The 40Ar/39Ar and cosmogenic 3He and 21Ne data support field observations indicating the SP flow has undergone negligible erosion. The SP flow contains co-existing phenocrysts of olivine and pyroxene, as well as xenocrysts of quartz in a fine-grained groundmass facilitating cross-calibration of cosmogenic production rates and production-rate (3He, 10Be, 14C, 21Ne, 26Al, and 36Cl). Thus, we propose the SP flow is an excellent location for a cosmogenic nuclide production-rate calibration site (SPICE: the SP Flow Production-Rate Inter-Calibration Site for Cosmogenic-Nuclide Evaluations).  相似文献   

10.
Models of the production of cosmogenic nuclides typically incorporate an adjustable production rate parameter that is scaled for variations in production with latitude and altitude. In practice, this production rate parameter is set by calibration of the model using cosmogenic nuclide data from sites with independent age constraints. In this paper, we describe a calibration procedure developed during the Cosmic-Ray Produced Nuclide Systematics on Earth (CRONUS-Earth) project and its application to an extensive data set that included both new CRONUS-Earth samples and samples from previously published studies. We considered seven frameworks for elevation and latitude scaling and five commonly used cosmogenic nuclides, 3He, 10Be, 14C, 26Al, and 36Cl. In general, the results show that the calibrated production rates fail statistical tests of goodness-of-fit. One conclusion from the calibration results is that two newly developed scaling frameworks and the widely used Lal scaling framework provide qualitatively similar fits to the data, while neutron-monitor based scaling frameworks have much poorer fit to the data. To further test the fitted models, we computed site ages for a number of secondary sites not included in the primary calibration data set. The root-mean-square percent differences between the median computed ages for these secondary sites and independent ages range from 7.1% to 27.1%, differences that are much larger than the typical uncertainties in the site ages. The results indicate that there are substantial unresolved difficulties in modeling cosmogenic nuclide production and the calibration of production rates.  相似文献   

11.
To constrain the depth-dependence of in situ 14C production we measured the cosmogenic 14C concentration of quartz separates along a quartzite core from the Leymon High site in northwest Spain. A total of 16 quartz samples were measured over a depth range of 1–1545 cm (3–4017 g cm−2). The obtained 14C profile was modeled using a neutron production rate, exponentially decreasing with depth, and a fast and negative muon production parameterized as a function of the local muon flux as derived by (Heisinger et al., 2002a, 2002b). This model yields a total negative muon capture probability of 1.72 (+0.22/−0.56) × 10−2 and a fast muon reaction cross section of 0 (+11.8/−0.00) μb. Rescaled to sea level high latitude using a Lal/Stone scaling scheme, these estimates yield a surface muon production rate of 3.31 (+0.43/−1.07) and 0 (+0.42/−0.00) at·g−1 yr−1 for negative muon capture and fast muons, respectively. This is the first muon production estimate for in situ 14C from a natural setting and is within uncertainty of the previous experimental estimates. The present contribution also provides new long-term blank and standard (PP-4, CRONUS-A & CRONUS-N) in situ 14C data from the ETH Zürich 14C extraction line.  相似文献   

12.
Because the intensity and energy spectrum of the cosmic ray flux are affected by atmospheric depth and geomagnetic-field strength, cosmogenic nuclide production rates increase considerably with altitude and to a lesser degree with latitude. The scaling methods used to account for spatial variability in production rates assume that all cosmogenic nuclides have the same altitude dependence. In this study we evaluate whether the production rates of cosmogenic 36Cl, 3He and 21Ne change differently with altitude, which is plausible due to the different threshold energies of their production reactions. If so, nuclide-specific scaling factors would be required.Concentrations of the three cosmogenic nuclides were determined in mafic phenocrysts over an altitude transect between 1000 and 4300 m at Kilimanjaro volcano (3°S). Altitude dependence of relative production rates was assessed in two ways: by determination of concentration ratios and by calculation of apparent exposure age ratios for all nuclide pairs. The latter accounts for characteristics of 36Cl that the stable nuclides 3He and 21Ne do not possess (radioactive decay, high sensitivity to mineral composition and significant contributions from production reactions other than spallation). All ratios overlap within error over the entire transect, and altitudinal variation in relative production rates is not therefore evident. This suggests that nuclide-specific scaling factors are not required for the studied nuclides at this low-latitude location. However, because previous studies have documented anomalous altitude-dependent variations in 3He production at mid-latitude sites, the effect of latitude on cross-calibrations should be further evaluated.We determined cosmogenic 21Ne/3He concentration ratios of 0.1864 ± 0.0085 in pyroxenes and 0.377 ± 0.018 in olivines, agreeing with those reported in previous studies.Despite the absence of independently determined ages for the studied lava surfaces, the consistency in the dataset should enable progress to be made in the determination of the production rates of all three nuclides as soon as the production rate of one of the nuclides has been accurately defined.To our knowledge this is the first time that 36Cl has been measured in pyroxene. The Cl extraction method was validated by measuring 36Cl in co-existing plagioclase phenocrysts in one of the samples.  相似文献   

13.
Many glacial deposits in the Quartermain Mountains, Antarctica present two apparent contradictions regarding the degradation of unconsolidated deposits. The glacial deposits are up to millions of years old, yet they have maintained their meter‐scale morphology despite the fact that bedrock and regolith erosion rates in the Quartermain Mountains have been measured at 0·1–4·0 m Ma?1. Additionally, ground ice persists in some Miocene‐aged soils in the Quartermain Mountains even though modeled and measured sublimation rates of ice in Antarctic soils suggest that without any recharge mechanisms ground ice should sublimate in the upper few meters of soil on the order of 103 to 105 years. This paper presents results from using the concentration of cosmogenic nuclides beryllium‐10 (10Be) and aluminum‐26 (26Al) in bulk sediment samples from depth profiles of three glacial deposits in the Quartermain Mountains. The measured nuclide concentrations are lower than expected for the known ages of the deposits, erosion alone does not always explain these concentrations, and deflation of the tills by the sublimation of ice coupled with erosion of the overlying till can explain some of the nuclide concentration profiles. The degradation rates that best match the data range 0·7–12 m Ma?1 for sublimation of ice with initial debris concentrations ranging 12–45% and erosion of the overlying till at rates of 0·4–1·2 m Ma?1. Overturning of the tills by cryoturbation, vertical mixing, or soil creep is not indicated by the cosmogenic nuclide profiles, and degradation appears to be limited to within a few centimeters of the surface. Erosion of these tills without vertical mixing may partially explain how some glacial deposits in the Quartermain Mountains maintain their morphology and contain ground ice close to the surface for millions of years. Copyright © 2010 John Wiley & Sons, Ltd.  相似文献   

14.
Terrestrial cosmogenic nuclide (TCN) concentrations measured in river sediments can be used to estimate catchment‐wide denudation rates. By investigating multiple TCN the steadiness of sediment generation, transport and depositional processes can be tested. Measurements of 10Be, 21Ne and 26Al from the hyper‐ to semi‐arid Rio Lluta catchment, northern Chile, yield average single denudation rates ranging from 12 to 75 m Myr–1 throughout the catchment. Paired nuclide analysis reveals complex exposure histories for most of the samples and thus the single nuclide estimates do not exclusively represent catchment‐wide denudation rates. The lower range of single nuclide denudation rates (12–17 m Myr–1), established with the noble gas 21Ne, is in accordance with palaeodenudation rates derived from 21Ne/10Be and 26Al/10Be ratio analysis. Since this denudation rate range is measured throughout the system, it is suggested that a headwater signal is transported downstream but modulated by a complex admixture of sediment that has been stored and buried at proximal hillslope or terrace deposits, which are released during high discharge events. That is best evidenced by the stable nuclide 21Ne, which preserves the nuclide concentration even during storage intervals. The catchment‐wide single 21Ne denudation rates and the palaeodenuation rates contrast with previous TCN‐derived erosion rates from bedrock exposures at hillslope interfluves by being at least one order of magnitude higher, especially in the lower river course. These results support earlier studies that identified a coupling of erosional processes in the Western Cordillera contrasting with decoupled processes in the Western Escarpment and in the Coastal Cordillera. Copyright © 2008 John Wiley & Sons, Ltd.  相似文献   

15.
Basin-wide erosion rates can be determined through the analysis of in situ-produced cosmogenic nuclides. In transient landscapes, and particularly in mountain catchments, erosion and transport processes are often highly variable and consequently the calculated erosion rates can be biased. This can be due to sediment pulses and poor mixing of sediment in the stream channels. The mixing of alluvial sediment is one of the principle conditions that need to be verified in order to have reliable results. In this paper we perform a field-based test of the extent of sediment mixing for a ∼42 km2 catchment in the Alps using concentrations of river-born 10Be. We use this technique to assess the mechanisms and the spatio-temporal scales for the mixing of sediment derived from hillslopes and tributary channels. The results show that sediment provenance and transport, and mixing processes have a substantial impact on the 10Be concentrations downstream of the confluence between streams and tributary channels. We also illustrate that the extent of mixing significantly depends on: the sizes of the catchments involved, the magnitude of the sediment delivery processes, the downstream distance of a sample site after a confluence, and the time since the event occurred. In particular, continuous soil creep and shallow landsliding supply high 10Be concentration material from the hillslope, congruently increasing the 10Be concentrations in the alluvial sediment. Contrariwise, a high frequency of mass-wasting processes or the occurrence of sporadic but large-magnitude events results in the supply of low-concentration sediment that lowers the cosmogenic nuclide concentration in the channels. The predominance of mass-wasting processes in a catchment can cause a strong bias in detrital cosmogenic nuclide concentrations, and therefore calculated erosion rates may be significantly over- or underestimated. Accordingly, it is important to sample as close as possible to the return-period of large-size sediment input events. This will lead to an erosion rate representative of the “mass-wasting signal” in case of generally high-frequency events, or the “background signal” when the event is sporadic. Our results suggest that a careful consideration of the extent of mixing of alluvial sediment is of primary importance for the correct estimation of 10Be-based erosion rates in mountain catchments, and likewise, that erosion rates have to be interpreted cautiously when the mixing conditions are unknown or mixing has not been achieved.  相似文献   

16.
Cosmogenic 21Ne was utilised to determine exposure ages of young subaerial basaltic lava flows from the Newer Volcanic Province, western Victoria, Australia. The ages (36–53 ka) determined from co-existing cosmogenic 21Ne and 3He in olivines separated from basalts are consistent within analytical uncertainties with ages previously determined by cosmogenic 36Cl exposure dating. This paper illustrates the potential of cosmogenic neon exposure ages in studying the eruption, surface morphology, and erosion history of young volcanic rocks, which are difficult to date using other conventional methods, such as K-Ar or 40Ar/39Ar dating. The present study demonstrates that combined cosmogenic 3He and 21Ne dating, specifically measured cosmogenic 3He/21Ne ratios, on the same samples, is powerful for evaluating the validity of calculated cosmogenic 3He and 21Ne surface exposure ages.  相似文献   

17.
Conventional methods for the determination of past soil erosion provide only average rates of erosion of the sediment's source areas and are unable to determine the rate of at-a-site soil loss. In this study, we report in-situ produced cosmogenic 10Be, and 14C measurements from erratic boulders and two depth-profiles from Younger Dryas moraines in Scotland, and assess the extent to which these data allow the quantification of the amount and timing of site-specific Holocene soil erosion at these sites. The study focuses on two sites located on end moraines of the Loch Lomond Readvance (LLR): Wester Cameron and Inchie Farm, both near Glasgow. The site near Wester Cameron does not show any visible signs of soil disturbance and was selected in order to test (i) whether a cosmogenic nuclide depth profile in a sediment body of Holocene age can be reconstructed, and (ii) whether in situ 10Be and 14C yield concordant results. Field evidence suggests that the site at Inchie Farm has undergone soil erosion and this site was selected to explore whether the technique can be applied to determine the broad timing of soil loss. The results of the cosmogenic 10Be and 14C analyses at Wester Cameron confirm that the cosmogenic nuclide depth-profile to be expected from a sediment body of Holocene age can be reconstructed. Moreover, the agreement between the total cosmogenic 10Be inventories in the erratics and the Wester Cameron soil/till samples indicate that there has been no erosion at the sample site since the deposition of the till/moraine. Further, the Wester Cameron depth profiles show minimal signs of homogenisation, as a result of bioturbation, and minimal cosmogenic nuclide inheritance from previous exposure periods. The results of the cosmogenic 10Be and 14C analyses at Inchie Farm show a clear departure from the zero-erosion cosmogenic nuclide depth profiles, suggesting that the soil/till at this site has undergone erosion since its stabilisation. The LLR moraine at the Inchie Farm site is characterised by the presence of a sharp break in slope, suggesting that the missing soil material was removed instantaneously by an erosion event rather than slowly by continuous erosion. The results of numerical simulations carried out to constrain the magnitude and timing of this erosion event suggest that the event was relatively recent and relatively shallow, resulting in the removal of circa 20–50 cm of soil at a maximum of ∼2000 years BP. Our analyses also show that the predicted magnitude and timing of the Inchie Farm erosion event are highly sensitive to the assumptions that are made about the background rate of continuous soil erosion at the site, the stabilisation age of the till, and the density of the sedimentary deposit. All three parameters can be independently determined a priori and so do not impede future applications to other localities. The results of the sensitivity analyses further show that the predicted erosion event magnitude and timing is very sensitive to the 14C production rate used and to assumptions about the contribution of muons to the total production rate of this nuclide. Thus, advances in this regard need to be made for the method presented in this study to be applicable with confidence to scenarios similar to the one presented here.  相似文献   

18.
The possibility of quantifying surface processes in mafic or volcanic environment using the potentialities offered by the in situ-produced cosmogenic nuclides, and more specifically by the in situ-produced 10Be, is often hampered by the rarity of quartz minerals in the available lithologies. As an alternative to overcome this difficulty, we explore in this work the possibility of relying on feldspar minerals rather that on quartz to perform in situ-produced 10Be measurements in such environments. Our strategy was to cross-calibrate the total production rate of 10Be in feldspar (P10fsp) against the total production rate of 3He in pyroxene (P3px) by measuring 3He and 10Be in cogenetic pyroxene (3Hepx) and feldspar (10Befsp). The samples were collected from eight ignimbritic boulders, exposed from ca 120 to 600 ka at elevations ranging from 800 to 2500 m, along the preserved rock-avalanche deposits of the giant Caquilluco landslide (18°S, 70°W), Southern Peru. Along with data recently published by Blard et al. (2013a) at a close latitude (22°S) but higher elevation (ca. 4000 m), the samples yield a remarkably tight cluster of 3Hepx - 10Befsp total production ratios whose weighted-mean is 35.6 ± 0.5 (1σ). The obtained weighted-mean 3Hepx - 10Befsp total production ratio combined with the local 3Hepy total production rate in the high tropical Andes published by Martin et al. (2017) allows to establish a total SLHL 10Be in situ-production rate in feldspar mineral (P10fsp) of 3.57 ± 0.21 at.g−1.yr−1 (scaled for the LSD scaling scheme, the ERA40 atm model and the VDM of Lifton, 2016).Despite the large elevation range covered by the whole dataset (800–4300 m), no significant variation of the 3Hepx - 10Befsp total production ratios in pyroxene and feldspar was evidenced. As an attempt to investigate the effect of the chemical composition of feldspar on the total 10Be production rate, major and trace element concentrations of the studied feldspar samples were analyzed. Unfortunately, giving the low compositional variability of our dataset, this issue is still pending.  相似文献   

19.
Landscapes evolve in response to external forces, such as tectonics and climate, that influence surface processes of erosion and weathering. Internal feedbacks between erosion and weathering also play an integral role in regulating the landscapes response. Our understanding of these internal and external feedbacks is limited to a handful of field‐based studies, only a few of which have explicitly examined saprolite weathering. Here, we report rates of erosion and weathering in saprolite and soil to quantify how climate influences denudation, by focusing on an elevation transect in the western Sierra Nevada Mountains, California. We use an adapted mass balance approach and couple soil‐production rates from the cosmogenic radionuclide (CRN) 10Be with zirconium concentrations in rock, saprolite and soil. Our approach includes deep saprolite weathering and suggests that previous studies may have underestimated denudation rates across similar landscapes. Along the studied climate gradient, chemical weathering rates peak at middle elevations (1200–2000 m), averaging 112·3 ± 9·7 t km–2 y–1 compared to high and low elevation sites (46·8 ± 5·2 t km?2 y?1). Measured weathering rates follow similar patterns with climate as those of predicted silica fluxes, modeled using an Arrhenius temperature relationship and a linear relationship between flux and precipitation. Furthermore, chemical weathering and erosion are tightly correlated across our sites, and physical erosion rates increase with both saprolite weathering rates and intensity. Unexpectedly, saprolite and soil weathering intensities are inversely related, such that more weathered saprolites are overlain by weakly weathered soils. These data quantify exciting links between climate, weathering and erosion, and together suggest that climate controls chemical weathering via temperature and moisture control on chemical reaction rates. Our results also suggest that saprolite weathering reduces bedrock coherence, leading to faster rates of soil transport that, in turn, decrease material residence times in the soil column and limit soil weathering. Copyright © 2009 John Wiley & Sons, Ltd.  相似文献   

20.
Combining cosmogenic 3He and 21Ne (3Hec and 21Nec) measurements on both pyroxene and olivine from the Pleistocene Bar Ten flows (85–107 ka) greatly increases our ability to evaluate the accuracy of 3Hec and 21Nec production rates and, therefore, 3Hec and 21Nec surface exposure ages. Comparison of 3Hec and 21Nec age-pairs yielded by experimentally determined production rates and composition-based model calculations indicates that the former give more accurate surface exposure ages than the latter in this study. However, experimental production rates should be adjusted to the composition of the minerals being analyzed to obtain the best agreement between 3Hec and 21Nec ages for any given sample. 21Nec/3Hec values are 0.400 ± 0.029 and 0.204 ± 0.014 for olivine and pyroxene, respectively, in Bar Ten lava flows, in agreement with previously published values, and indicate that 21Nec/3Hec in olivine and pyroxene is not affected by erosion and remains constant with latitude, elevation, and time (up to 10 Myr). Samples with 21Nec/3Hec that do not agree with these values may indicate the presence of non-cosmogenic helium and/or neon. The neon three-isotope diagram can also indicate whether or not all excess neon in mineral separates comes from cosmogenic sources. An error-weighted regression for olivine defines a spallation line [y = (1.033 ± 0.031)x + (0.09876 ± 0.00033)], which is indistinguishable from that for pyroxene (Schäfer et al., 1999). We have derived a production rate of 25 ± 8 at/g/yr for 21Nec in clinopyroxene (En43–44) based on the 40Ar/39Ar age of the upper Bar Ten flow. Our study indicates that the production rate of 21Nec in olivine may be slightly higher than previously determined. Cosmogenic 3He and 21Ne remain extremely useful, particularly when paired, in determining accurate eruption ages of young olivine- and pyroxene-rich basaltic lava flows.  相似文献   

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