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1.
Influence of wave on sediment resuspension and nutrients release from sediments, collected from Lake Taihu and Lake Chaohu, was studied in flume experiments. Under strong-wave conditions, concentrations of suspended solids (SS), total phosphorus (TP) and dissolved total phosphorus (DTP) in overlying water were increased significantly following the sediments re-suspension. During the experiments on sediments of Lake Taihu and Lake Chaohu, TP concentrations increased 6 times and 3 times, and DTP concentration increased 100% and 70% more than it in presuspension, respectively. Concentration of soluble reactive phosphorus (SRP) of experiment on sediment of Lake Taihu increased 25%. During the massive sediment suspension, the dissolved phosphorus in pore water and much of the phosphorus adsorbed by the sediment particles were released into overlying water. The phenomena in this wave flume experiment are quite similar to the situation observed in situ of Lake Taihu. The critical wave stresses of sediment re-suspension are nearly equal. The change of concentrations of SS, TP, and SRP was the same as that in situ situation. This study showed that concentrations of TP and SRP in lake water could be increased significantly by wave disturbance. Phosphorus release was significantly enhanced by wave disturbance at the beginning of massive sediment re-suspension, but decreased later.  相似文献   

2.
This paper is a review of research works concerning the nutrient transportation, transformation and exchange between water, sediment and biota in the lakes from the middle and lower reaches of the Yangtze River conducted in the context of project entitled "The Processes and Mechanism of Lake Eutrophication in Middle and Lower Reaches of Yangtze River". All the lakes from this area are shallow lakes. According to the typical lake site research, the lakes from the middle and lower reaches of Yangtze River have a higher baseline of nutrition in the history. Normally the trophic status of these lakes can be categorized into medium-trophic or eutrophic. Human activities have been enhanced during the last decades, which speed up the lake eutrophic process. Lake eutrophication control needs to reduce not only the external nutrient inputs from watershed but also the internal loading from the sediments. Investigations revealed that the lake sediments in this area are considerablly high in nutrition in which at most about 30% of phosphorus exists in the form of bio-available in the sediment. The surface sediment will exert great effects on the nutrient exchange between water-sediment interface via adsorption and release of nutrient. The nutrient release from the sediment in these shallow lakes is mainly in two ways, i.e. in the undisturbed condition the nutrient is released through diffusion created by the nutrient gradient from sediment to overlying water; whereas in disturbed condition, the nutrient release is determined by the hydrodynamic forcing intensity and the sediment resuspension. Metallic elements such as the iron, manganese and aluminium and the aerobic-anaerobic ambience will affect the release of nutrients. The disturbed release will increase the total nutrients in the water column significantly in the short period. At the beginning of sediment resuspension, the dissolved nutrient concentration will increase. This increase will be damped if the ferric oxide and aluminium are rich in sediment because of the adsorption and flocculation. This means that the lakes have capability of eliminating the nutrient loadings. Investigations for the lakes from middle and down stream of Yangtze River have suggested that most lakes have the self-cleaning capability. Dredging the control of the internal loading, therefore, is only applicable to the small lakes or undisturbed bays which normally are situated nearby the city or town and rich in organic materials in the sediment. In addition, the strong reduction condition and weak aeration of these lakes and bays make these small lakes and bays release much more bio-available nutrient and without much self-eliminating capability. Moreover, eutrophication induced algal bloom in these lakes will change the pH of water, which further induces the increase in the nutrient release. In turn, the increase in nutrient release promotes the growth of phytoplankton and results in severe algal bloom. For the heavily polluted water, research suggests that the biomass of bacteria and alkaline phosphatase activity will be higher corresponding to the higher concentration of nutrients, which accelerates the nutrient recycling between water, sediment and biota. Quick recycling of nutrient, in turn, promotes the production and biomass growth of microorganism and leads to more severe eutrophication. Further research work should focus on the nutrient transformation mechanism and the effects of microbial loop on the eutrophication.  相似文献   

3.
Phosphatase may accelerate the process of lake eutrophication through improving phosphorus bioavailability. This mechanism was studied in three Chinese eutrophic shallow lakes (Lake Taihu, Lake Longyang and Lake Lianhua). Phosphatase activity was related to the concentration of soluble reactive phosphorus (SRP) and chlorophyll a. Stability of dissolved phosphatase in reverse micelles may be attributed to molecular size, conformation and active residues of the enzyme. At the site with Microcystis bloomed in Lake Taihu, dissolved phosphatase activity was higher and more stable in micelles, SRP concentrations were lower in interstitial water, the contents of different forms of phosphorus and the amounts of aerobic bacteria were lower while respiration efficiency was higher in sediments. Phosphobacteria, both inorganic and organic and other microorganisms were abundant in surface water but rare in sediments. Therefore, internal phosphorus may substantially flux into water column by enzymatic hydrolysis and anaerobic release, together with mobility of bacteria, thereby initiating the bloom. In short, biological mechanism may act in concert with physical and chemical factors to drive the internal phosphorus release and accelerate lake eutrophication.  相似文献   

4.
Spatiotemporal variations of P species and adsorption behavior in water column, interstitial water, and sediments were investigated in the large shallow eutrophic Lake Chaohu. Ortho-phosphate (Ortho-P) and total phosphorus (TP) concentrations were significantly higher in the western part than in the eastern part of the lake, due to different nutrient inputs from the surrounding rivers. Moreover, paniculate phosphorus (PP) concentration was in a similar spatial pattern to Ortho-P and TP concentrations, and also showed significantly positive correlation with the biomass of Microcystis, indicating more uptake and store of phosphorus by Microcystis than by other algae. Increase of pH and intensive utilization of P by phytoplankton were the main factors promoting P (especially Fe-P) release from the sediment to interstitial water during the cyanobacterial blooms in Lake Chaohu. Spatial dynamics in TP concentration, P species and adsorption behavior of the sediment, coupled with the statistical analyses, suggested that the spatial heterogeneity of P contents in the sediment was influenced by various factors, e.g. human activities, soil geochemistry and mineral composition. In spite of similar TP contents in the sediments, increase in proportion of Fe-P concentration in the sediment may result in a high risk of P release.  相似文献   

5.
It was indicated in this study that there were negative relations between the concentrations of suspended solid (SS) and transparency according to the analysis of measured data of Lake Taihu. Their relations in pervious studies were reviewed, which showed that the changes of transparency in Lake Taihu could be reflected by simulating suspended solid concentration (SSC). Measured data showed that the changes of SSC with wind speed were similar at different water depths. SSC increased with the increasing of wind speed. Both wave and lake current of Lake Taihu had positive relations with SSC. However, wave was the main factor affecting sediment suspension, while flow took the second place. In this study, a numerical model coupling lake current, wave and SSC of Lake Taihu was developed. In the SS model, the combined effects of wave and current were included. The amounts of suspended and deposited sediments near the lake bed surface layer were treated separately. The stochastic characteristics of turbulent flow pulsation near lake beds were also considered, and the start-up conditions of sediment suspension were introduced to the model. The model elucidated the mutual exchange processes between sediment particles in SS and active sediments within and on the bed surface layer. Simulated results showed that lake current had relatively significant effects on the SSC at littoral areas of Lake Taihu, while SSC at the central area of the lake was mainly influenced by wave. The changes of transparency with SSC were simulated for Lake Taihu using this model. Calculated results were validated by measured data with good fitness, which indicated that the model is basically suitable for the simulation and prediction of transparency of Lake Taihu.  相似文献   

6.
Forms of phosphorus in sediments from 25 lakes in the middle and lower reaches of Yangtze River were analyzed by the sequential extraction procedure. Contents and spatial distrubution of algal available phosphorus (AAP) in sediments of Lake Taihu, the third largest freshwater lake of China, were also studied. Relationships between phosphorus forms in sediment and macrophytes coverage in sample sites, as well as phosphorus forms in sediments and chlorophyal contents in lake water were discussed. Exchangeable form of phosphorus (Ex-P) in surface sediments was significantly positive correlative to total phosphorus (IP), dissolved total phosphorus (DTP) and soluble reactive phosphorus (SRP) contents in the lake water. Bioavailable phosphorus (Bio-P) contents in sediments from macrophytes dominant sites were significantly lower than that in no macrophyte sites. In Lake Taihu, Ex-P content in top 3 cm sediment was highest. However, content of ferric fraction phosphorus (Fe-P) was highest in 4 - 10 cm. Bioavalilble phosphorus (Bio-P) contents in surface sediments positively correlated to Chlorophyll a contents in water of Lake Taihu with significant difference. Therefore, contents of Bio-P and AAP could be acted as the indicators of risks of internal release of phosphorus in the shallow lakes. It was estimated that there were 268.6 ton AAP in top 1 cm sediments in Lake Taihu. Sediment suspension caused by strong wind-induced wave disturbance could carry plenty of AAP into water in large shallow lakes like Lake Taihu.  相似文献   

7.
《国际泥沙研究》2016,(4):330-340
The resuspension and transportation of sediments affect the nutrient or contaminants cycles in water column. Therefore, hurricane-induced sediment resuspension in coastal waters may cause environment impacts on coastal ecosystems. In this study, field observed data during a hurricane event from the Rookery Bay National Estuarine Research Reserve (Rookery Bay NERR), Florida, were studied. Based on the relationship between sediment and turbidity, variations of turbidity in the Rookery Bay NERR were discussed in this paper under the impact of the Hurricane Isaac in 2012. Time series analysis indicates that Hurricane Isaac causes the substantial increase of turbidity. Traditional direct regression analysis with raw data was found to result in poor correlation (R2 o 0.41) between wind speed and turbidity due to the impacts of multi-factors in coastal waters of study region during hurricane. Then Hanning Filter was used to remove tidal effect, which shows some improvement of correlations (R2 4 0.6) between wind speed and turbidity. Further improvement was made by introducing a phase factor to account for the lag time between the peak turbidity and peak wind speed, which lead to further improvement of the regression equation between wind speed and turbidity. By using Hanning Filter and phase factor, the regression equation between turbidity and wind speed fits well with observations (R2 4 0.96). Different lag time between wind speed and turbidity at different locations illustrated that wind had different effects on turbidity due to the locations and water depth. Based on the approximate empirical rela-tionship between turbidity and sediment concentration, a regression equation between wind speed and sediment concentration was derived approximately. The equation could be applied to approximately estimate the sediment concentration using wind speed during hurricane, especially with the strong wind speed above 4 m/s. It can be used to provide technical supports for sediment assessment and coastal zone research under extreme clime in the study region.  相似文献   

8.
Because of the obvious importance of P as a nutrient that often accelerates growth of phytoplankton (including toxic cyanobacteria) and therefore worsens water quality, much interest has been devoted to P exchange across the sediment-water interface. Generally, the release mode of P from the sediment differed greatly between shallow and deep lakes, and much of the effort has been focused on iron and oxygen, and also on the relevant environmental factors, for example, turbulence and decomposition, but a large part of the P variation in shallow lakes remains unexplained. This paper reviews experimental and field studies on the mechanisms of P release from the sediment in the shallow temperate (in Europe) and subtropical (in the middle and lower reaches of the Yangtze River in China) lakes, and it is suggested that pH rather than DO might be more important in driving the seasonal dynamics of internal P loading in these shallow lakes, i.e., intense photosynthesis of phytoplankton increases pH of the lake water and thus may increase pH of the surface sediment, leading to enhanced release of P (especially iron-bound P) from the sediment. Based on the selective pump of P (but not N) from the sediment by algal blooms, it is concluded that photosynthesis which is closely related to eutrophication level is the driving force for the seasonal variation of internal P loading in shallow lakes. This is a new finding. Additionally, the selective pump of P from the sediment by algal blooms not only explains satisfactorily why both TP and PO4-P in the hypereutrophic Lake Donghu declined significantly since the mid-1980s when heavy cyanobacterial blooms were eliminated by the nontraditional biomanipulation (massive stocking of the filter-feeding silver and bighead carps), but also explains why TP in European lakes decreased remarkably in the spring clear-water phase with less phytoplankton during the seasonal succession of aquatic communities or when phytoplankton biomass was decreased by traditional biomanipulation. Compared with deep lakes, wax and wane of phytoplankton due to alternations in the ecosystem structure is also able to exert significant influences on the P exchange at the sediment-water interface in shallow lakes. In other words, biological activities are also able to drive P release from sediments, and such a static P release process is especially more prominent in eutrophic shallow lakes with dense phytoplankton.  相似文献   

9.
The mechanisms which controls the fixation and/or release of P in sediment of an extremely acidic lake（pH = 2.0 to 3.0） and its response to the influence of eutrophic urban waste water were investigated.The results,in the chemical composition,in the mineralogy of the sediment and in the material as obtained from sediment traps,show that the lake sediments are mainly volcanic material reflecting volcanic features of the basin.The sedimentation rate calculated for the lake(2.5×10-2 mg m-2 day-1) was higher than that observed in other similar glacial lakes in both Andean Patagonia and also elsewhere in the world.The Total Phosphorus concentration in sediments was higher than figures reported by other authors for mining acid lakes,and the main fraction of P was found associated with organic matter.There was no control by Fe or Al on P,because both are in solution at pH < 3.0.It was concluded that changes in the natural input of nutrients（derivatives of Copahue volcano fluid,the discharge of sewage,or basin run-off） are responsible for a high concentration of SRP and N-NH4+ in the lake.Laboratory experiments showed that sediments have no ability to retain phosphorus and a continuous release of P from the sediments into the water column was observed.The assays where the pH was artificially increased showed that the P still remains in solution until at least pH 7.0.It was concluded that changes in the natural input of nutrients due to:1) the volcanic fluids,2) the increase in sewage charges,or 3) surface runoff upstream,maintain a high trophic state with high concentrations of dissolved P and N-NH4+,although the threshold of neutral pH in the lake is exceeded.This study will enable a better understanding about of the mechanism of release/fixation of phosphorus in acidic sediments in order to assist in making decisions regarding the conservation and management of this natural environment.  相似文献   

10.
Variation of wind speed and the physico-chemical parameters, such as dissolved phosphate, ferrous and manganese in lake water were observed on site. Together with the chemistry analysis and simulated experiment in lab, the change of phosphate concentration in lake water was analyzed. The variation of ferrous/phosphate ratio explained that along with the enhancement of wind-wave effect and the oxidation ability of lake water, the effects of co-precipitation and removal of dissolved phosphate and iron in the lake water were reinforced. The ferrous/phosphate ratio in pore water was less than 2.0, demonstrating that the dissolved phosphate can be released into the overlying water. But, in the lake water, the stability of phosphate was controlled by the water dynamics. The phosphate release experiment showed that molecular release was only part of the whole and the direct discharge of phosphate in the pore water was also a part. The mineralization and biological process of suspended particulates in the water may be another important reason for the whole phosphate loadings.  相似文献   

11.
Estimation of internal nutrient release in large shallow Lake Taihu,China   总被引：1，自引：0，他引：1  
Based on field investigation of wave, sediment suspension and the changes in nutrient concentration of the water column in Lake Taihu, China, we proposed two release models to quantify nutrient release under static and dynamic conditions, respectively. Under static conditions, nutrient release from sediments to the overlying water mainly depends on chemical diffusion induced by concentration gradient, in which the nutrient release is controlled by the temperature, dissolved oxygen concentration in the sediment-water interface, oxidation-reduction potential and the concentration difference between porewater and overlying water. Under dynamic condition (or disturbed condition), both dissolved and particulate nutrients in sediments are released into the water column because of wind-induced sediment suspension. The amount of nutrient release under dynamic conditions is larger than that under the static condition. The release of dissolved nutrients, however, does not increase because the wind induced turbulence made oxidation of metallic elements such as Fe (ferric iron), Mn which are capable of precipitating soluble reactive phosphate (SRP). Under dynamic conditions, therefore, the release of total phosphorus (TP) increases dramatically but the release of SRP is close to those under static conditions. In sediments of Lake Taihu, high Fe content leads to a high ratio of Fe to P contents in sediments (Fe:P ratio). Under dynamic conditions, therefore, nutrient release is controlled by the intensity of disturbance, sediment consolidation and nutrient content in sediments. As for dissolved nutrients, especially SRP, the release is also controlled by the intensity of dynamic re-oxidation, Fe content in sediments and nutrient concentration gradient between porewater and overlying water. Based on these two release modes, the release flux in Lake Taihu has been estimated. In the static condition (i.e. laboratory experimental condition), total release of NH4 +-N for whole lake is ca. 10,000 ton/a, and PO4 3?-P is ca. 900 ton/a. In the dynamic condition, nutrient release following sediment suspension was estimated according to three different intensities of wind forcing which were defined as “calm” (wind speed is less than 2 m/s), “gentle” (wind speed is greater than 2 m/s and less than 6 m/s) and “gust” (wind speed is greater than 6 m/s). The release rate in the condition of “calm” was estimated in terms of the nutrient release in the laboratory experimental static condition; whereas the release rate in conditions of “gentle” and “gust” was estimated in terms of measurement during sediment resuspension conducted in flume experiments. With the observation of wind velocity and frequency in 2001, each type of wind forcing took the frequency of 12%, 82% and 6% for “calm”, “gentle” and “gust”, respectively. The yearly release of nitrogen was 81,000 ton and phosphorus was 21,000 ton, which is about 2–6 folds of annual external loading, respectively.  相似文献   

12.

Based on field investigation of wave, sediment suspension and the changes in nutrient concentration of the water column in Lake Taihu, China, we proposed two release models to quantify nutrient release under static and dynamic conditions, respectively. Under static conditions, nutrient release from sediments to the overlying water mainly depends on chemical diffusion induced by concentration gradient, in which the nutrient release is controlled by the temperature, dissolved oxygen concentration in the sediment-water interface, oxidation-reduction potential and the concentration difference between porewater and overlying water. Under dynamic condition (or disturbed condition), both dissolved and particulate nutrients in sediments are released into the water column because of wind-induced sediment suspension. The amount of nutrient release under dynamic conditions is larger than that under the static condition. The release of dissolved nutrients, however, does not increase because the wind induced turbulence made oxidation of metallic elements such as Fe (ferric iron), Mn which are capable of precipitating soluble reactive phosphate (SRP). Under dynamic conditions, therefore, the release of total phosphorus (TP) increases dramatically but the release of SRP is close to those under static conditions. In sediments of Lake Taihu, high Fe content leads to a high ratio of Fe to P contents in sediments (Fe:P ratio). Under dynamic conditions, therefore, nutrient release is controlled by the intensity of disturbance, sediment consolidation and nutrient content in sediments. As for dissolved nutrients, especially SRP, the release is also controlled by the intensity of dynamic re-oxidation, Fe content in sediments and nutrient concentration gradient between porewater and overlying water. Based on these two release modes, the release flux in Lake Taihu has been estimated. In the static condition (i.e. laboratory experimental condition), total release of NH4 +-N for whole lake is ca. 10,000 ton/a, and PO4 3−-P is ca. 900 ton/a. In the dynamic condition, nutrient release following sediment suspension was estimated according to three different intensities of wind forcing which were defined as “calm” (wind speed is less than 2 m/s), “gentle” (wind speed is greater than 2 m/s and less than 6 m/s) and “gust” (wind speed is greater than 6 m/s). The release rate in the condition of “calm” was estimated in terms of the nutrient release in the laboratory experimental static condition; whereas the release rate in conditions of “gentle” and “gust” was estimated in terms of measurement during sediment resuspension conducted in flume experiments. With the observation of wind velocity and frequency in 2001, each type of wind forcing took the frequency of 12%, 82% and 6% for “calm”, “gentle” and “gust”, respectively. The yearly release of nitrogen was 81,000 ton and phosphorus was 21,000 ton, which is about 2–6 folds of annual external loading, respectively.

  相似文献   

13.
Influence of wave on sediment resuspension and nutrients release from sediments, collected from Lake Taihu and Lake Chaohu, was studied in flume experiments. Under strong-wave conditions, concentrations of suspended solids (SS), total phosphorus (TP) and dissolved total phosphorus (DTP) in overlying water were increased significantly following the sediments re-suspension. During the experiments on sediments of Lake Taihu and Lake Chaohu, TP concentrations increased 6 times and 3 times, and DTP concentration increased 100% and 70% more than it in presuspension, respectively. Concentration of soluble reactive phosphorus (SRP) of experiment on sediment of Lake Taihu increased 25%. During the massive sediment suspension, the dissolved phosphorus in pore water and much of the phosphorus adsorbed by the sediment particles were released into overlying water. The phenomena in this wave flume experiment are quite similar to the situation observed in situ of Lake Taihu. The critical wave stresses of sediment re-suspension are nearly equal. The change of concentrations of SS, TP, and SRP was the same as that in situ situation. This study showed that concentrations of TP and SRP in lake water could be increased significantly by wave disturbance. Phosphorus release was significantly enhanced by wave disturbance at the beginning of massive sediment re-suspension, but decreased later.  相似文献   

14.
Forms of phosphorus in sediments from 25 lakes in the middle and lower reaches of Yangtze River were analyzed by the sequential extraction procedure. Contents and spatial distrubution of algal available phosphorus (AAP) in sediments of Lake Taihu, the third largest freshwater lake of China, were also studied. Relationships between phosphorus forms in sediment and macrophytes coverage in sample sites, as well as phosphorus forms in sediments and chlorophyal contents in lake water were discussed. Exchangeable form of phosphorus (Ex-P) in surface sediments was significantly positive correlative to total phosphorus (TP), dissolved total phosphorus (DTP) and soluble reactive phosphorus (SRP) contents in the lake water. Bioavailable phosphorus (Bio-P) contents in sediments from macrophytes dominant sites were significantly lower than that in no macrophyte sites. In Lake Taihu, Ex-P content in top 3 cm sediment was highest. However, content of ferric fraction phosphorus (Fe-P) was highest in 4–10 cm. Bioavalilble phosphorus (Bio-P) contents in surface sediments positively correlated to Chlorophyll a contents in water of Lake Taihu with significant difference. Therefore, contents of Bio-P and AAP could be acted as the indicators of risks of internal release of phosphorus in the shallow lakes. It was estimated that there were 268.6 ton AAP in top 1 cm sediments in Lake Taihu. Sediment suspension caused by strong wind-induced wave disturbance could carry plenty of AAP into water in large shallow lakes like Lake Taihu.  相似文献   

15.
为探讨水丝蚓(Tubificid worms)扰动对磷在湖泊沉积物-水界面间迁移的影响,选取太湖梅梁湾与大浦口两富营养化湖区为研究对象,通过室内培养实验,利用Rhizon间隙水采样器等技术,研究了水丝蚓扰动对太湖沉积物-水界面理化性质及溶解活性磷(SRP)在界面通量的影响.结果表明水丝蚓扰动能够增大表层沉积物含水率、氧化还原电位,减小间隙水中Fe2+浓度.水丝蚓没有显著改变梅梁湾间隙水中SRP浓度,同时促进了梅梁湾沉积物中SRP向上覆水的释放;但水丝蚓显著减小了大浦口间隙水中SRP浓度,并抑制了大浦口沉积物中SRP向上覆水的释放.水丝蚓扰动对磷在沉积物-水界面间迁移的不同影响可能是由沉积物中Fe2+含量差异较大造成的.  相似文献   

16.
Phosphatase may accelerate the process of lake eutrophication through improving phosphorus bioavailability. This mechanism was studied in three Chinese eutrophic shallow lakes (Lake Taihu, Lake Longyang and Lake Lianhua). Phosphatase activity was related to the concentration of soluble reactive phosphorus (SRP) and chlorophyll a. Stability of dissolved phosphatase in reverse micelles may be attributed to molecular size, conformation and active residues of the enzyme. At the site with Microcystis bloomed in Lake Taihu, dissolved phosphatase activity was higher and more stable in micelles, SRP concentrations were lower in interstitial water, the contents of different forms of phosphorus and the amounts of aerobic bacteria were lower while respiration efficiency was higher in sediments. Phosphobacteria, both inorganic and organic and other microorganisms were abundant in surface water but rare in sediments. Therefore, internal phosphorus may substantially flux into water column by enzymatic hydrolysis and anaerobic release, together with mobility of bacteria, thereby initiating the bloom. In short, biological mechanism may act in concert with physical and chemical factors to drive the internal phosphorus release and accelerate lake eutrophication.  相似文献   

17.
模拟水体pH控制条件下太湖梅梁湾沉积物中磷的释放特征   总被引：9，自引：1，他引：8  
采用缓冲溶液控制水体pH值,模拟研究了太湖梅梁湾沉积物扰动悬浮状态下水体磷的释放规律(48h),分析了实验前后沉积物中磷的赋存形态组成及变化特征.结果表明,pH条件对沉积物磷释放具有显著影响,强酸性(pH=2.0)及碱性(pH=9.5,11.8)条件下皆利于磷的释放,但强酸性水体磷含量随时间逐渐降低,而碱性水体磷呈持续释放状态;中性条件(pH=7.2)磷的释放释放作用不明显,磷释放达到稳定状态(14b)后,碱性条件下(pH=9.5,11.8)磷释放量为酸性(pH=2.0,4.6)及中性(pH=7.2)条件下的4倍以上,通过对比释放前、后沉积物中磷的形态组成可知,酸性条件主要为钙结合态磷的释放;碱性条件主要是铁结合态磷释放,部分可发生再沉淀,转化为钙结合态磷,研究表明,梅梁湾沉积物中铁结合态磷的解析是沉积物磷的主要释放源,是水体内源磷增加的重要贡献者.  相似文献   

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