Residence times in river basins as determined by analysis of long-term tritium records     

Robert L. Michel 《Journal of Hydrology》1992,130(1-4):367-378

The US Geological Survey has maintained a network of stations to collect samples for the measurement of tritium concentrations in precipitation and streamflow since the early 1960s. Tritium data from outflow waters of river basins draining 4500–75000 km² are used to determine average residence times of water within the basins. The basins studied are the Colorado River above Cisco, Utah; the Kissimmee River above Lake Okeechobee, Florida; the Mississippi River above Anoka, Minnesota; the Neuse River above Streets Ferry Bridge near Vanceboro, North Carolina; the Potomac River above Point of Rocks, Maryland; the Sacramento River above Sacramento, California; the Susquehanna River above Harrisburg, Pennsylvania. The basins are modeled with the assumption that the outflow in the river comes from two sources—prompt (within-year) runoff from precipitation, and flow from the long-term reservoirs of the basin. Tritium concentration in the outflow water of the basin is dependent on three factors: (1) tritium concentration in runoff from the long-term reservoir, which depends on the residence time for the reservoir and historical tritium concentrations in precipitation; (2) tritium concentrations in precipitation (the within-year runoff component); (3) relative contributions of flow from the long-term and within-year components. Predicted tritium concentrations for the outflow water in the river basins were calculated for different residence times and for different relative contributions from the two reservoirs. A box model was used to calculate tritium concentrations in the long-term reservoir. Calculated values of outflow tritium concentrations for the basin were regressed against the measured data to obtain a slope as close as possible to 1. These regressions assumed an intercept of zero and were carried out for different values of residence time and reservoir contribution to maximize the fit of modeled versus actual data for all the above rivers. The final slopes of the fitted regression lines ranged from 0.95 to 1.01 (correlation coefficient > 0.96) for the basins studied. Values for the residence time of waters within the basins and average relative contributions of the within-year and long-term reservoirs to outflow were obtained. Values for river basin residence times ranged from 2 years for the Kissimmee River basin to 20 years for the Potomac River basin. The residence times indicate the time scale in which the basin responds to anthropogenic inputs. The modeled tritium concentrations for the basins also furnish input data for urban and agricultural settings where these river waters are used.  相似文献   

The rates of tritium input to the world oceans     

Wolfgang Weiss  Wolfgang Roether 《Earth and Planetary Science Letters》1980,49(2):435-446

Mean annual rates of tritium input into the ocean averaged over 5° latitude bands are presented for the major oceans, for the period 1952–1975. The rates are obtained by converting tritium concentrations in marine precipitation into net oceanic tritium input, by means of a hydrological model. The tropospheric tritium pattern is specified on the basis of available observations, and climatological means from the literature are used for the rates of evaporation and precipitation and for the relative humidity in ship's height, that enter the model. Tritium input by water vapor exchange exceeds that by precipitation about three-fold. Tritium input by river runoff and by net tropospheric tritium outflow from the continents is also accounted for. This contribution is small except for the northern Indian Ocean and the North Atlantic.The inputs have hemispheric maxima near 50° latitude. The northern hemisphere inputs were strongly peaked in 1963–1964, whereas temporal changes in the southern hemisphere were much more gradual. By 1972, about 75% of the total oceanic input had been received by the northern ocean. For the Pacific, the computed total input agrees with the actual tritium inventory within the limits of uncertainty (about ±20%). The global tritium inventory is estimated at 1.9 GCi in 1972, which corresponds to an average tritium yield of 0.9 kg tritium per megaton TNT equivalent of nuclear fusion.  相似文献   

Spatial and temporal variation of precipitation in Sudan and their possible causes during 1948–2005     

Zengxin Zhang  Chong-Yu Xu  Majduline El-Haj El-Tahir  Jianrong Cao  V. P. Singh 《Stochastic Environmental Research and Risk Assessment (SERRA)》2012,26(3):429-441

Temporal and spatial patterns of precipitation are essential to the understanding of soil moisture status which is vital for vegetation regeneration in the arid ecosystems. The purposes of this study are (1) to understand the temporal and spatial variations of precipitation in Sudan during 1948–2005 by using high quality global precipitation data known as Precipitation REConstruction (PREC), which has been constructed at the National Oceanic and Atmospheric Administration (NOAA) Climate Prediction Center, and (2) to discuss the relationship between precipitation variability and moisture flux based on the NCEP/NCAR reanalysis data in order to ascertain the potential causes of the spatial and temporal variations of precipitation in the region. Results showed that (1) annual and monthly precipitation in Sudan had great spatial variability, and mean annual precipitation varied from almost nil in the North to about 1500 mm in the extreme Southwest; (2) precipitation of the main rain season, i.e., July, August and September, and annual total precipitation in the central part of Sudan decreased significantly during 1948–2005; (3) abrupt change points were found in the annual, July, August and September in the late 1960s, when precipitation decreased more rapidly than in other periods; and (4) the decreasing precipitation was associated with the weakening African summer monsoon. The summer moisture flux over Sudan tended to be decreasing after the late 1960s which decreased the northward propagation of moisture flux in North Africa. This study provides a complementary view to the previous studies that attempted to explain the Sahel persistent drought and possible causes.  相似文献   

Tritium hydrology of the Mississippi River basin     

Robert L. Michel 《水文研究》2004,18(7):1255-1269

In the early 1960s, the US Geological Survey began routinely analysing river water samples for tritium concentrations at locations within the Mississippi River basin. The sites included the main stem of the Mississippi River (at Luling Ferry, Louisiana), and three of its major tributaries, the Ohio River (at Markland Dam, Kentucky), the upper Missouri River (at Nebraska City, Nebraska) and the Arkansas River (near Van Buren, Arkansas). The measurements cover the period during the peak of the bomb‐produced tritium transient when tritium concentrations in precipitation rose above natural levels by two to three orders of magnitude. Using measurements of tritium concentrations in precipitation, a tritium input function was established for the river basins above the Ohio River, Missouri River and Arkansas River sampling locations. Owing to the extent of the basin above the Luling Ferry site, no input function was developed for that location. The input functions for the Ohio and Missouri Rivers were then used in a two‐component mixing model to estimate residence times of water within these two basins. (The Arkansas River was not modelled because of extremely large yearly variations in flow during the peak of the tritium transient.) The two components used were: (i) recent precipitation (prompt outflow) and (ii) waters derived from the long‐term groundwater reservoir of the basin. The tritium concentration of the second component is a function of the atmospheric input and the residence times of the groundwaters within the basin. Using yearly time periods, the parameters of the model were varied until a best fit was obtained between modelled and measured tritium data. The results from the model indicate that about 40% of the flow in the Ohio River was from prompt outflow, as compared with 10% for the Missouri River. Mean residence times of 10 years were calculated for the groundwater component of the Ohio River versus 4 years for the Missouri River. The mass flux of tritium through the Mississippi Basin and its tributaries was calculated during the years that tritium measurements were made. The cumulative fluxes, calculated in grams of ³H were: (i) 160 g for the Ohio (1961–1986), (ii) 98 g for the upper Missouri (1963–1997), (iii) 30 g for the Arkansas (1961–1997) and (iv) 780 g for the Mississippi (1961–1997). Copyright © 2004 John Wiley & Sons, Ltd.  相似文献   

A continuous record of artificial tritium fallout at the South Pole (1954–1978)     

J. Jouzel  L. Merlivat  M. Pourchet  C. Lorius 《Earth and Planetary Science Letters》1979,45(1):188-200

Snow samples were taken from a 5-m-deep pit located near the South Pole station in January 1975 and continuous deuterium, tritium and β activity profiles have been obtained from them. These three measurements and the stratigraphic observations allow us to deduce a precise chronology of the pit from 1950 to 1975, providing a continuous record of artificial tritium fallout in the southern hemisphere; this record has been extended to 1978 using samples from a second pit taken this last year. Taking advantage of the unusual 1957–1958 stable isotope content in the snow, we have demonstrated that an important part of the isotopic signal in the precipitation is retained in the snow in spite of the low accumulation rate (8.2 g cm^?2 yr^?1).The first artificial tritium, due to the 1952 Ivy experiments was detected during 1954. A two-year delay between explosions and fallout is well established and allows us to relate the tritium fallout to the main nuclear tests from 1952 to 1960. This delay appears longer for the large 1961–1962 devices. A stratospheric half residence time equal to 20 months is deduced from the fallout decrease occurring after the 1966 peak. For the French southern hemisphere experiments, it is about one year. A sharp tritium decrease is observed after a high 1973 peak, providing a new tritium reference level for future glaciological studies in Antarctica.The β and tritium peaks occur respectively during the Antarctic summer and the Antarctic winter, showing different injection mechanisms. This winter input and the high tritium values registered at the South Pole indicate a preferential tritium transfer over the pole area. Two mechanisms, stratospheric-tropospheric exchange and direct stratospheric cloud precipitation could account for this injection.  相似文献   

Tritium in the Arctic Ocean and East Greenland Current   总被引：1，自引：0，他引：1  

H.G. Dorsey  W.H. Peterson 《Earth and Planetary Science Letters》1976,32(2):342-350

High concentrations of tritium are found in the surface water of the Arctic Ocean (up to 50 TU) and in the East Greenland Current (up to 70 TU). These high tritium values are a direct result of atmospheric testing of nuclear weapons in the early 1960's. A box model with a time-dependent input of highly tritiated precipitation predicts that high tritium concentrations are to be expected in the surface layer of the Arctic Ocean and its various outflows. We suggest that a few tritium stations in the Arctic Ocean would provide a powerful analytical tool for assigning time scales to exchange processes.  相似文献   

A simplified approach to analysing historical and recent tritium data in surface waters          下载免费PDF全文

Robert L. Michel  Pradeep Aggarwal  Luis Araguas‐Araguas  Brent D. Newman  Tomas Vitvar 《水文研究》2015,29(4):572-578

Tritium concentrations in river and stream waters from different locations can be compared by normalizing them using the ratio of tritium concentrations in precipitation and surface water (C_p/C_s) in the study area. This study uses these ratios in a hydrological residence time context to make regional‐ and global‐scale comparisons about river basin dynamics. Prior to the advent of nuclear weapons testing, the C_p/C_s ratio was greater than or equal to 1 everywhere because of the decay of tritium in the watershed after it was deposited by precipitation. After an initial increase in the ratios during the bomb peak, the ratio dropped to less than 1 for most surface waters in the following years. This post‐bomb change in the ratio is due to the retention of the bomb‐pulse water in watersheds on timescales that are long relative to the residence time of tritium in the atmosphere. Ratios were calculated for over 6500 measurements of tritium in river and stream waters compiled by the International Atomic Energy Agency. These measurements span the post‐nuclear era (1940s to present) and include many long‐term datasets, which make it possible to examine residence times of waters in watersheds on a global basis. Plotting C_p/C_s versus time shows that ratios tended to reach a minimum in approximately one to two decades after the bomb peak for most locations. This result suggests that changes affecting quantity and quality of river flows need to be assessed on a multi‐decadal timescale. These long lag times have significant implications for assessing climate or land‐use change impacts on a large number of river systems around the world. The continuing value of tritium in studying surface water systems for both the Southern and Northern Hemisphere is also demonstrated. Published 2014. This article is a U.S. Government work and is in the public domain in the USA.  相似文献   

Overview of tritium records from precipitation and surface waters in Germany     

Axel Schmidt  Gabriele Frank  Willibald Stichler  Lars Duester  Thomas Steinkopff  Christine Stumpp 《水文研究》2020,34(6):1489-1493

Tritium is one of the most important environmental tracers in isotope hydrology for understanding the dynamics of groundwater and connected surface water and has been used in a wide range of applications at different scales. A key requirement for using tritium as a tracer is the knowledge of its spatial and temporal distribution in different water types. As a fundamental input, quantity long-term time series of tritium in precipitation are of particular importance. In this paper, the authors present an overview of tritium data sets of the Federal Institute of Hydrology (BfG), the Helmholtz Zentrum München (HMGU) and the German Weather Service (DWD). Since the 1970s, all three institutions have monitored the tritium concentration at 53 surface water and 37 precipitation stations on a monthly basis. The primary purpose of the data set was to provide baseline information for different water types all over Germany as an integral part of the German radiation protection monitoring system. Additionally, as geochemically inert tracer, tritium provides a unique tool to different user groups in a wide range of research questions and applications.  相似文献   

Higher tritium concentrations measured in permafrost thaw lakes in northern Alberta          下载免费PDF全文

J. J. Gibson  S. J. Birks  Y. Yi 《水文研究》2016,30(2):245-249

Tritium concentrations were measured in a survey of 24 lakes, 15 wetlands, and 133 groundwaters in the oil sands region of northeastern Alberta and compared with both recent precipitation and precipitation sampled during the 1960s tritium peak caused by atmospheric thermonuclear weapons testing. Water samples from lakes included a group of 14 thaw lakes that had higher runoff attributed to melting of permafrost in peat plateaus within their watersheds. While tritium in all lakes was found to be intermediate between recent and 1960s concentrations, the thaw lakes were found to be significantly enriched in tritium compared with other lakes, as were unfrozen wetlands characterized by a thick sequence of low‐hydraulic conductivity peat. The results provide further evidence of different water sources to the thaw lakes and may indicate that melting of modern permafrost in part formed since the 1950s is occurring in these systems. Copyright © 2015 John Wiley & Sons, Ltd.  相似文献   

Estimating mean residence time of karst groundwater in mountainous catchments of Western Himalaya,India     

Rouf A. Shah  Noble Jacob 《水文科学杂志》2017,62(8):1230-1242

The mean residence time (MRT) of karst groundwater in three mountainous catchments of the Western Himalaya was estimated using multiple approaches: the tritium method, the sine wave model and tracer tests. Water samples were collected from precipitation, glacier melt, streams and karst springs for δ²H and tritium analysis during 2012 and 2013. High tritium values were observed in winter precipitation and low values in summer precipitation. The variation of tritium in karst springs was similar to that of the streams, whereas glacier melt showed lower tritium values. The MRT of cold karst springs was shorter than that of warm karst springs. The tracer breakthrough curves (TBC) retrieved for different springs suggested a short travel time for groundwater and possibly conduit flow. Deterioration of water quality and variation in flux magnitude are the two main practical consequences of the short travel time of karst groundwater in the region.