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1.
Transport and retention of Escherichia coli through the mixture of quartz, Al‐coated and Fe‐coated sands was examined using column experiments to investigate the effect of geochemical heterogeneity on bacteria transport. The first set of the experiments was performed in quartz, Al‐coated and Fe‐coated sand mixtures (coated sand: 0, 5, 10, 25, 50, 100%) to examine the influence of positively‐charged sand grains on bacteria transport. The second experiments were carried out to observe the impact of pH (range 6·74–8·21) on bacteria transport in the mixture of quartz 50% and Fe‐coated sand 50%. The third experiments were conducted to analyse the effect of ionic strength (0, 50, 100, 200 mM) on bacteria transport in the mixture of quartz 50% and Al‐coated sand 50%. The first experiments show that bacterial mass recoveries were in the range of 3·6–43·4%, decreasing nonlinearly as the content of Al‐ and Fe‐coated sands increased. In the second experiments, the bacterial mass recoveries were in the range of 35·5–79·2%, increasing linearly as the solution pH increased. In the third experiments, the mass recovery was 3·4% at 0 mM. As the ionic strength increased to 50mM, the mass recovery decreased to 0%. When the ionic strength increased further to 100 and 200 mM, no bacterial mass was recovered as in the case of 50 mM. It indicates that in the mixed medium of quartz 50% and Al‐coated sand 50% both positive (increment of bacterial adhesion) and negative (decrement) effects of ionic strength may be counterbalanced, minimizing the impact of ionic strength on the bacterial adhesion. This study helps to understand the role of metal oxides and solution chemistry in the transport of bacteria in geochemically heterogeneous media Copyright © 2008 John Wiley & Sons, Ltd. 相似文献
2.
By means of the analysis of sediments cored in the small river Gurk (Carinthia/Austria), the input of Ag, Cd, Ce, Cr, Hg, La, Mo, Ni, V, and W from a chemical industrial plant could be detected. To estimate the actual load, and to obtain data for comparison with other sites, both unsieved fine sediments and sediments sieved to 20 μm were investigated from the same cores. Environmental mobilities of toxic heavy metals (Co, Cr, Cu, Ni, Zn) have been shown by sequential leaching following Tessier/Förstner. In the last step, HNO3 leaches a purely geogenic fraction, which is fairly constant along the investigated river. Whereas the additional Cr from the input of the chemical plant is mainly found in the oxalate-leachable fraction, short-time-load to unpolluted sediments in the laboratory is found mainly in hydroxylamine/acetic acid. Both is due to the high affinity of Cr to Fe- and Mn-oxides. Adsorption/desorption experiments reveal that the low carbonate content of the Gurk sediments increases the importance of Fe/Mn-oxides for the sorption of Cr compared to other samples containing carbonate. The Ni-load was primarily found in weak-acid-leachable and oxalate-leachable fractions. Similarly, the oxalate-leachable fraction is dominant for adsorption of other metals and phosphorus. Other interelement relationships among the amounts leached, which are attributable partly to carbonate-, silicate-, organic or coating phases, have been found by means of factor analyses together with marker fractions for each type. 相似文献
3.
Abstract The adsorption of lead and zinc ions on bed sediments of the River Kali in western Uttar Pradesh, India, has been studied. The role of the coarser sediment fraction (210–250 μm) in controlling metal pollution has been elucidated and compared to those of the clay and silt fractions. The parameters controlling metal uptake, viz., solution pH, sediment dose, contact time, and particle size have been evaluated. The optimum contact time needed to reach equilibrium is of the order of 45 min for both the metal ions. The extent of adsorption increases with an increase of pH. Furthermore, the adsorption of the metal ions increases with increasing adsorbent doses and decreases with adsorbent particle size. The two geochemical phases of iron and manganese oxide act as the active support material for the adsorption of the metal ions. 相似文献
4.
Craig Amerigian 《Earth and Planetary Science Letters》1977,36(3):434-442
Deposition experiments have been carried out to measure the effect of particle size variation on the relationship between detrital remanent magnetization (DRM), anhysteretic remanent magnetization (ARM), and geomagnetic field intensity in sediments.Foraminiferal ooze from a box core taken in the Columbian Basin south of Jamaica was separated into several particle size ranges and redeposited in the laboratory in known magnetic fields. The intensity and alternating field (AF) demagnetization characteristics of the DRM and a subsequently applied ARM were compared for the various particle size ranges.The results show a variation of DRM/ARM ratios with particle size. The DRM intensities and directions indicate that particle sizes greater than 38 μm do not contribute significantly to the DRM of the total sediment. ARM intensities for larger particle sizes and particle size analysis of the whole sediment indicate that the fraction greater than 38 μm does make a significant contribution to the total ARM of a sample. Use of the DRM/ARM ratio in experimental measurements of magnetic paleointensity indicates that the method is unsatisfactory for sediments having a significant fraction of magnetic particles larger than 38 μm. It is also shown that, for sediments having a significant fraction of high-coercivity magnetic grains, the relative orientation of the ARM and DRM will affect ARM intensities, making necessary the use of corrected ARM and DRM intensities for ratio calculations. 相似文献
5.
Petroleum hydrocarbons in the sediments of the Bothnian Bay, Baltic proper, Öresund, Kattegatt and Skagerrak were analysed in a survey of oil pollution along the Swedish coast in 1974 and 1975. Sixty-one of these sediment stations were revisited in 1982 and analysed with the methods used in the first survey. The mean content of petroleum hydrocarbons (paraffin-naphthene fraction) in the sediment surface showed a statistically significant increase from 199 to 252 μg g?1 dry wt. The main increase had taken place in the coastal areas. Within 0–20 km distance of urbanized areas (>20 000 inhabitants) petroleum hydrocarbons had increased from 371 to 447 μg g?1. Sediment levels increased from 76 to 117 μg g?1, 20–50 km from urbanized areas. The increase in these areas was equivalent to 0.119 g m?2 yr?1. 相似文献
6.
Plastic debris is a worldwide threat to marine environments and Portugal is not immune to it. Though never quantified, items of all sizes can be found in the Portuguese coastline; therefore the objective of this work is the identification of main size classes in stranded plastic debris. Beaches sediment was sampled and in the laboratory plastic items were sorted in 11 classes from <1 to >10 mm, counted and weighted. Plastic size ranged from 50 μm to 20 cm and microplastics (<5 mm) were the majority (72%). Most plastic fits in the smaller size classes, due to expected high residence time in the sea enhancing degradation processes, which increase surface exposure and potentially persistent organic pollutants (POP) adsorption. These results point out the important contribution of microplastics to marine debris pollution, its risks, and the need to set a higher focus on this size class. 相似文献
7.
《Limnologica》2019
Biologically configured ββ-hopanes, geologically configured αβ-hopanes and the biogenic hopenes were determined in dated sediment cores from Lake Fuxian in SW China and Lake Changdang in Eastern China in order to investigate anthropogenic influences on the abundance, composition and provenance of hopanoid hydrocarbons in lake sediments. Based on the results, hopenes were prevalent, with maximum values reaching 148.9 μg g−1 TOC in sediments of Lake Fuxian, an oligotrophic deep lake (average depth 89.6 m), where the long water column provided ample potential for the growth of hopene-producing bacteria especially the cyanobacteria. Sediment hopenes have diminished in abundance to values of 13.4–78.5 μg g−1 TOC in Lake Changdang, a eutrophic shallow (average 0.8–1.2 m) body, reflecting comparatively reduced importance of nutrient level on hopene production. Historical trends in hopenes input to the sediments of each lake are strongly dependent on nutrient status. During the last few decades, human-induced eutrophication has greatly boosted bacterial production, enhancing the accumulation of hopenes in sediments. Inputs of petroleum-derived αβ-hopanes were exceptionally high (average 71.2 μg g−1 TOC) in post-1968 sediments from Lake Changdang, their increase coinciding with the advent and acceleration of petroleum product use around the lake, in particular by fishing boats. Lake Fuxian on the other hand, has undergone slower economic development and the appearance of petroleum-derived αβ-hopanes in sediments was delayed to 1990 since when the average value has been 27.1 μg g−1 TOC. The abundance of αβ-hopanes in Lake Changdang has created a marked decrease in the relative contribution of hopenes to total hopanoids since 1968. Conversely, the amounts of αβ-hopanes introduced to Lake Fuxian since 1990 has yet to yield a clear change in the overall proportion of hopenes, but the abundance of ββ-hopanes has declined relative to total hopanoid levels for the period. 相似文献
8.
为研究滇池内源污染特征,2013年利用GIS软件针对滇池全湖布设36个采样点,采集表层沉积物,研究滇池表层沉积物铵态氮(NH_4+-N)吸附特征,同时分析沉积物的理化性质对NH_4+-N吸附特性的影响.结果表明:滇池表层沉积物对NH_4+-N的吸附量在前2 h之内呈增长趋势,吸附速率较大,之后沉积物对NH_4+-N的吸附量不随时间变化而变化,基本达到平衡,最大吸附速率均发生在0~5 min内;不同区域表层沉积物NH_4+-N最大吸附速率平均值表现为:外海南部湖心区外海北部草海,最大吸附量平均值表现为:湖心区外海南部外海北部草海,吸附效率平均值表现为:外海北部草海湖心区外海南部;沉积物对NH4+-N的吸附量与NH_4+-N的初始浓度大致呈线性关系,并且低浓度下表现出很好的吸附/解吸特征;滇池表层沉积物NH_4+-N的吸附解吸平衡浓度(ENC0)高于上覆水中NH_4+-N浓度,表明沉积物中NH_4+-N有向上覆水中释放的风险,沉积物在很长一段时间内起到水体污染"源"的作用;ENC0与沉积物中总氮、NH_4+-N含量呈显著正相关,本底吸附量和有机质总量呈显著负相关,沉积物吸附NH_4+-N主要受有机质的影响. 相似文献
9.
Aziz Ghaderpour Khairul Nazrin Mohd Nasori Li Lee Chew Ving Ching Chong Kwai Lin Thong Lay Ching Chai 《Marine pollution bulletin》2014
The deltaic estuarine system of the Matang Mangrove Forest Reserve of Malaysia is a site where several human settlements and brackish water aquaculture have been established. Here, we evaluated the level of fecal indicator bacteria (FIB) and the presence of potentially pathogenic bacteria in the surface water and sediments. Higher levels of FIB were detected at downstream sampling sites from the fishing village, indicating it as a possible source of anthropogenic pollution to the estuary. Enterococci levels in the estuarine sediments were higher than in the surface water, while total coliforms and E. coli in the estuarine sediments were not detected in all samples. Also, various types of potentially pathogenic bacteria, including Klebsiella pneumoniae, Serratia marcescens and Enterobacter cloacae were isolated. The results indicate that the Matang estuarine system is contaminated with various types of potential human bacterial pathogens which might pose a health risk to the public. 相似文献
10.
湖泊沉积物的重金属污染防治一直是环境领域的热点问题.本研究采用氨基生物炭作为覆盖材料,利用梯度扩散薄膜技术(DGT),研究了上覆水不同pH及水流扰动条件下Cu(Ⅱ)、Pb(Ⅱ)在沉积物水界面间的原位释放特征,以及氨基生物炭对湖泊沉积物重金属污染的原位修复效果.研究结果表明,在0 r/min或100 r/min水动力条件下,可移动态重金属离子有不断由沉积物向其他介质扩散的趋势,1.81 kg/m 2的氨基生物炭覆盖强度可降低Cu(Ⅱ)、Pb(Ⅱ)释放通量达89%以上,有效减小了水环境中重金属的潜在生态风险.在pH=5的酸性及pH=9的碱性水环境中原位修复效果较差,水体中大量的H+或络合物均会削弱氨基生物炭对重金属离子的吸附,当上覆水在pH=7的中性条件时原位修复效果最佳.100 r/min水流扰动下的上覆水Cu(Ⅱ)、Pb(Ⅱ)含量在释放平衡时较0 r/min条件下高出0.036~0.096μg/mL,说明高强度的水流扰动易造成覆盖材料的扬起和浮动,导致覆盖材料与重金属发生解吸. 相似文献
11.
Paraskevi N. Polymenakou Glykeria Fragkioudaki Anastasios Tselepides 《Continental Shelf Research》2007
Recently, black carbon has been introduced as the form of carbon that may be separated from the biologically mediated carbon cycle thereby representing the non-bioavailable fraction of the estimated organic carbon. It has been speculated that the bioavailability of organic matter may be a limiting factor for the presence of active bacteria within the sediments. In order to address this question, marine sediments were collected from the Thracian Sea (Eastern Mediterranean), a complex system impacted by riverine inputs and Black Sea water masses. In addition to counts of total bacteria, we estimated the fraction of active bacteria by using a destaining step to the DAPI staining method. Black carbon was also estimated following the thermal oxidation method in order to determine the fraction of the refractory organic matter. The fraction of black carbon to total organic carbon varied from 16% to 53% indicating that black carbon constitutes a significant pool of sedimentary organic carbon in the Thracian sea. A fraction ranging from 18% to 97% was scored as nucleoid containing cells. We did not record any significant differences in the fraction of nucleoid-containing bacteria among sediment depths (P<0.05) indicating that there was no accumulation of dead bacterial cells with depth. The same was observed for the fraction of black carbon and bioavailable organic carbon with sediment depth (P<0.05) indicating that benthic consumers are not the key regulators of the organic matter pool in these sediments but have a minor effect. A possible reason for these observations and for the uncoupling between the active bacterial fraction and the bioavailability of organic matter could be (i) the presence of refractory components in the estimated bioavailable organic matter and (ii) the hydrological and geological complexity of the study area. The North Aegean marginal slopes are highly unstable experiencing frequent seismic events. These events are capable of inducing sediment transport from the upper slopes thus altering the entire sediment profile. On the other hand, the significant correlations that were recorded between nucleoid-containing cells and phytopigments (chlorophyll a, phaeopigments, chloroplastic pigment equivalents) at all sediment depths indicate that bacterial communities respond immediately to the deposited phytodetritus, using it as a primary source of carbon and energy. Our data suggests that the Thracian Sea sediments are by no means homogeneous and can best be described as a mosaic controlled by numerous local and regional environmental factors. 相似文献
12.
N. M. Kalinkina N. A. Berezina A. I. Sidorova N. A. Belkina A. K. Morozov 《Water Resources》2013,40(6):657-666
The results of bioassay and physicochemical analysis of bottom sediments from large water bodies in Northwestern Russia are presented. The water bodies under consideration include Lake Onega, Vygozerskoe Reservoir, and freshwater part of the Neva Estuary (the Eastern Gulf of Finland), which are locally subject to eutrophication and toxic pollution. The potential toxicity of bottom sediments, evaluated by the survival rate of two crustacean species (Gmelinoides fasciatus and Ceriodaphnia affinis) in 7-day tests, varied from high to low values, characterizing 5 quality classes: high, good, moderate, poor, and heavy, with appropriate degrees of toxic pollution from no to very high pollution. Bad zones were identified in the Kondopoga and Petrozavodsk bays of Onega Lake, the northern and southern parts of the Vygozerskoe Reservoir, and the southern part of the Neva Bay near the dam. Bottom sediments were found to have high quality in the open central areas of Lake Onega and the Vygozerskoe Reservoir and in the western part of Neva Estuary. 相似文献
13.
Lin Liu Zhongwu Li Haibing Xiao Bing Wang Xiaodong Nie Chun Liu Lingshan Ni Danyang Wang 《地球表面变化过程与地形》2019,44(10):1895-1909
Organic carbon (OC) is easily enriched in sediment particles of different sizes due to aggregate breakdown and selective transport for sheet erosion. However, the transport of aggregate-associated OC has not been thoroughly investigated. To address this issue, 27 simulated rainfall experiments were conducted in a 1 m × 0.35 m box on slope gradients of 15°, 10°, and 15°and under three rainfall intensities of 45 mm h−1, 90 mm h−1 and 120 mm h−1. The results showed that OC was obviously enriched in sediment particles of different sizes under sheet erosion. The soil organic carbon (SOC) concentrations of each aggregate size class in sediments were different from those in the original soil, especially when the rainfall intensity or slope was sufficiently low, such as 45 mm h–1 or 5°, respectively. Under a slope of 5°, the SOC enrichment ratios (ERocs) of small macroaggregates and microaggregates were high but decreased over time. As rainfall intensity increased, OC became enriched in increasingly fine sediment particles. Under a rainfall intensity of 45 mm h–1, the ERocs of the different aggregate size classes were always high throughout the entire erosion process. Under a rainfall intensity of > 45 mm h–1 and slope of > 5°, the ERocs of the different aggregate size classes were close to 1.0, especially those of clay and silt. Therefore, the high ERocs in sediments resulted from the first transport of effective clay. Among total SOC loss, the proportion of OC loss caused by the transport of microaggregates and silt plus clay-sized particles was greater than 50%. We also found that low stream power and low water depth were two requirements for the high ERocs in aggregates. Stream power was closely related to sediment particle distribution. Flow velocity was significantly and positively related to the percentage of OC-enriched macroaggregates in the sediments (P > 0.01). Our study will provide important information for understanding the fate of SOC and building physical-based SOC transport models. © 2019 John Wiley & Sons, Ltd. 相似文献
14.
Zhao Wei Youze Xu Yanyan Zhao Yuanyuan Zhao Leilei Bai Helong Jiang Changhui Wang 《国际泥沙研究》2021,36(4):542-554
Sediment resuspension is an important way for shallow lake internal pollution to interact with the overlying water column,and the pollution risks are reasonably related to the retention of resuspended sediment particles in overlying water.In the current study,the settling of resuspended sediment particles was comprehensively investigated under different disturbances using five urban lake sediments.The results show that the particle size distributions of resuspended sediment from different lakes exhibited similar variations during settling with disturbance,although varied settling times were observed under static conditions.During settling with and without disturbance,sediment particle sizes were mainly within 8-63μm at the initial stage,and were<8μm in the later stages of settling.Based on these settling characteristics,the sediment particle size was divided into sand(>63μm),silt(8-63μm),and very fine silt and clay(<8μm)fractions.Kinetic analysis suggested that sediment settling for different particle sizes could be well described by the first-and second-order kinetic equations,especially when settling was disturbed(r2=0.727-0.999).The retention of resuspended sediment could be enhanced as particle sizes decreased and disturbance intensities increased.Furthermore,a water elutriation method was successfully optimized,with separation efficiencies of 56.1%-83%,to separate sediment particles into the defined three particle size fractions.The chemical compositions of sediment were found to change with different particle sizes.Typically,calcium tended to form large-size sediment,while the total contents of aluminum,iron,magnesium,and manganese showed significantly negative correlations with sediment particle sizes(p<0.01)and tended to distribute in small-size particles(e.g.,<8μm).Overall,the sediment particle size related settling dynamics and physicochemical properties suggested the necessity on determining the pollution of resuspended sediment at different particle sizes for restoration of shallow lakes. 相似文献
15.
悬浮物在自然水体（池塘、河流、湖泊等）中普遍存在，相较于上覆水，是微生物更为倾向的附着载体。相较于沉积物，更易获取硝酸盐，是水体反硝化发生的热点微区。悬浮物在水体中经历一系列碰撞、絮凝、溶解、离子交换、吸附解吸等物理化学过程，从而会引起颗粒物粒径、营养盐浓度等发生变化；悬浮物的沉降和再悬浮过程也会引起上覆水和沉积物之间的物质交换，并在好氧缺氧过渡过程中对氮转化造成影响，从而直接或者间接影响水体反硝化速率。本文概括了国内外关于悬浮物影响水体反硝化的研究进展和热点，总结了不同浓度、粒径、组成和种类的悬浮物对反硝化作用的影响，从溶解氧、功能微生物、无机氮、有机碳等环境因素重点归纳了悬浮物影响反硝化的过程，比较和分析了悬浮物反硝化的测定方法。结合当前悬浮物反硝化研究现状，建议未来可以从新兴污染物悬浮物、机理模型、测定方法等方面展开深入研究。 相似文献
16.
17.
Hargrave BT Doucette LI Haya K Friars FS Armstrong SM 《Marine pollution bulletin》2008,56(8):1439-1445
A micro-dilution technique with changes in optical density (OD) used to measure bacterial growth over 72 h in culture media containing 0, 5, 10, 20, 40, 80 and 160 microg OTC (oxytetracycline)ml(-1) was applied to determine growth inhibition (GI) in mixed bacterial strains cultured from samples of marine sediments and salmon feed pellets. Growth of control cultures (Aeromonas salmonicida) was inhibited at all OTC concentrations. Some feed pellet samples and under-cage sediments from salmon aquaculture sites in the Bay of Fundy showed GI up to > or = 160 microg OTCml(-1). Lower values (40 to 80 microg OTC ml(-1)) occurred in subsurface (5-18 cm) sediments, > 100 m from salmon pens and adjacent to sewage outfalls in Halifax Harbour. GI values < 20 microg OTC ml(-1) in sediment from reference locations in Halifax Harbour and mussel aquaculture sites are considered to reflect natural background levels for OTC resistance. 相似文献
18.
Bacterial abundances and activity, estimated by 4′,6-diamidino-2-phenylindole staining (DAPI) and the reduction of 2-(p-iodophenyl)-3-(p-nitrophenyl)-5-phenyl tetrazolium chloride (INT), were investigated in two oligotrophic artificial groundwater lakes and the surrounding aquifers. To evaluate the effect of lake water on groundwater downstream, samples were taken from wells at different distances from the lakes, and the total number of bacteria and the number of active bacteria in these samples were compared with samples collected upstream. In addition, sterilized sandy sediments were exposed in groundwater wells to measure the number and activity of bacteria attached to particles. At one of the study sites, where the lake sediments were disturbed by dredging, total bacterial abundance and the number of respiring bacteria in the groundwater aquifer was clearly influenced by the lake water. The average bacterial abundances decreased from 2.6 ± 1.9 × 105 cells ml−1 in the well closest to the lake (S2) to 2.9 ± 3.8 × 104 cells ml−1 in the most distant one (S4), which was equivalent to cell numbers in the upstream well. The number of respiring bacteria showed a similar tendency with 1.3 ± 2.7 × 104 active cells ml−1 in S2 and 1.9 ± 1.5 × 103 active cells ml−1 in S4. At the second study site, which was not influenced by dredging, bacteria in the downstream wells seemed not to be affected by the lake water. The number and activity of bacteria, which colonized exposed sediments, were not significantly different in the upstream and downstream wells, indicating a minor influence of lake water on this habitat. Our results suggest that gravel-pit lakes may influence the free living bacterial assemblages in nearshore groundwater systems, but do not visibly affect numbers and activity of bacteria attached to the surface of aquifer sediments. 相似文献
19.
Sulfate reduction is an important oxidation process involving transformation of organic matter and its components and taking place in the aquatic environment and bottom sediments of water bodies (both fresh and marine) under anaerobic conditions. The intensification of sulfate reduction in water bodies is a sign of a stronger anthropogenic impact on the environment and natural water bodies. The development of sulfate reduction under natural conditions reflects the influence of many environmental factors. The effect of the most important factors (the concentration of organic matter and its components and sulfates, the temperature of aquatic environment, and the abundance and activity of sulfate-reducing bacteria) on the process of sulfate reduction in the aquatic environment and bottom sediments in water bodies is considered. 相似文献
20.
Spatial and temporal dynamics of bacterial contamination in South France coastal rivers: focus on in‐stream processes during low flows and floods 
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下载免费PDF全文 Y. Chu M. G. Tournoud C. Salles P. Got J. L. Perrin C. Rodier A. Caro M. Troussellier 《水文研究》2014,28(8):3300-3313
Faecal indicator bacteria (thermotolerant coliform and faecal streptococci) were enumerated in a Mediterranean coastal river to evaluate bacterial contamination levels in relation to hydrological conditions, to estimate delivery of bacterial loads to transitional and coastal waters (Thau lagoon) and to identify bacterial sources of pollution and their contribution to the bacterial flow. Results showed that (1) in low flow conditions, mean bacterial concentrations were higher than EU guidelines for bathing waters; (2) floods had higher concentrations of indicator bacteria than low flows; (3) low flow conditions represented a negligible proportion of bacterial loads compared with high flow and flood periods; (4) during medium and low flow conditions, bacteria were stored in riverbed fine sediments forming in‐stream stores that may be flushed during floods; (5) the first flush effect was highlighted during an early autumn flood as was the role of in‐stream stores during the course of the flood; and (6) point sources that continuously feed the river are contributing to the pool of bacteria accumulated in the riverbed sediment. Copyright © 2013 John Wiley & Sons, Ltd. 相似文献