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乌鲁木齐地区水汞空白值较高原因分析 总被引：2，自引：0，他引：2
从蒸馏水的制备过程及乌鲁木齐10号泉的化学成份等方面入手，通过分析认为乌鲁木齐水汞空白值较高的原因是：①在蒸馏水的制备过程中自来水中汞富集到蒸馏水中；②乌鲁木齐10号泉水中含有较高的S^2-，使10号泉水汞测值偏低。另外，还探讨了如何利用水汞空白值来处理水汞资料，从而提高水汞观测资料的质量及其在地震分析预报中的作用。 相似文献
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对2000年1月15日姚安6．5级地震前后云南水汞异常进行分析研究，结果表明：在9个观测台站中，地震前有1个观测台站的水汞出现中期趋势异常，1个台站的水汞出现远震异常，4个台站的水汞出现短期异常，1个台站的水汞出现临震异常。地震前3个月内，水汞短期异常有活跃，平静的过程，在平静中(仅1个台站出现临震异常)发生姚安6．5级地震。姚安地震发生在距出现远震异常的水汞观测台站70km的地方。出现远震异常的水汞观测台站附近，可能是未来强震的发震地区。 相似文献
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山西奇村水汞相关性分析与与区域分布特征的研究—剖析山西奇村水汞与空白样同步的原因 总被引：1，自引：2，他引：1
为揭示山西奇村水汞与空白样测值同步的原因，对水化热水井与空白样、水化热水井与制作空白样的冷水井、制作空白样的冷水井与空白样的特征进行了分析，并对忻定盆地南部近1 000km^2不同深度、不同水温的21眼井进行了水汞测量。研究表明，测区各井具有水汞含量一致、动态变化同步的基本特征，提出水汞动态可能反映了来自大构造及深层的变化信息的看法。 相似文献
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怀来4井水汞前兆异常特征分析 总被引：2，自引：0，他引：2
本文介绍了１９９８年张北６．２级地震前水汞的异常变化;多点突跳、变化幅度大和持续时间长是震前水汞异常的特点。同时还根据以往水汞的多次震例,归纳出怀来４井水汞具有形态的多样性,对应距离为９０～２８０ｋｍ,异常出现后１５～４７天内发震等特点。从而加深了对该井水汞异常与地震关系的认识,有助于今后水汞预测地震水平的提高 相似文献
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通过对山西忻州奇村水化站水汞观测水样与空白样测值曲线所含信息的研究,论述了两者产生同步现象的原因及其动态特征,进而提出排除水汞干扰、识别水汞异常的方法。 相似文献
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Mercury (Hg) concentration was investigated during 2010 based on road runoff from Nanjing Ring Highway, China. The emphasis was placed on impact of rainfall characteristics on Hg speciation concentration, and on variation characteristics of Hg speciation during road runoff for different rainfall patterns. Results indicated that average concentration of total mercury (THg) was in the range from 0.472 to 1.304 µg/L, and steady Hg (SHg) was the dominant form of Hg. Rainfall and average rainfall intensity were two important factors of determining Hg speciation concentrations during road runoff for different rainfall patterns. Rainfall pattern had significantly influence on variation of available Hg and dissolved Hg during road runoff, and on their proportions in THg. However, the proportion of SHg in THg was not obviously affected by rainfall pattern. On the other hand, toxic degree of Hg to soil environment is various for different rainfall patterns, based on Hg speciation variation. 相似文献
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Joseph T. Bushey Charles T. Driscoll Myron J. Mitchell Pranesh Selvendiran Mario R. Montesdeoca 《水文研究》2008,22(25):4813-4826
Concentrations and fluxes of mercury (Hg) species in surface waters of forested watersheds are affected by hydrological events. The mechanisms of Hg transport during these events are poorly understood and yet may influence Hg bioavailability and exposure to aquatic biota. Three storm events with varying magnitude and intensity were investigated (June, September and November 2005) at a forested watershed in the Adirondack region of New York State, USA. Concentrations of Hg species increased during these events, both above and downstream of wetlands in the watershed. While Hg flux was higher from wetland drainage, the Hg flux from the upland site exhibited a greater relative increase to elevated runoff. Hg flux was controlled by discharge; however, Hg species concentrations were not well correlated with discharge, dissolved organic carbon (DOC), or total suspended solids (TSS) through the duration of events. A counter‐clockwise hysteresis response of DOC with increasing runoff contrasted with the clockwise response for total Hg, suggesting different contributions from source areas for these solutes. Correspondence with elevated total K and NO3? (α < 0·05) during the rising limb of the hydrograph suggests rapid delivery of throughfall Hg, potentially enhanced by hillslope hollows, to the stream channel. As the watershed saturated, stream Hg appears to be derived from the soil Hg pool. Results suggest that particulate Hg did not contribute substantially to total Hg flux during events (<25%). These results emphasize the role of watershed attributes and storm characteristics in Hg transport and bioavailability. Copyright © 2008 John Wiley & Sons, Ltd. 相似文献
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Distribution and speciation of mercury in surficial sediments from main mangrove wetlands in China 总被引：4，自引：0，他引：4
The purpose of this study was to establish the distribution, speciation and bioavailability of mercury in mangrove sediments. A systemic survey of surficial sediments from 13 mangrove wetlands of China was carried out. Hg concentrations ranged from 2.3–903.6 ng g−1, with an average value of 189.4 ng g−1. Of the 13 areas surveyed, the Hg content in sediments was similar to background levels in 6 areas but was much higher in the other seven areas. Hg levels were affected by natural and anthropogenic factors, including terrestrial pollutants, geomorphic properties, and indirectly by economic status. Hg levels were positively correlated with organic matter, pH, and silt and clay fractions, but Hg was negatively correlated with sand fraction. In most mangrove wetlands, Hg existed primarily in the form of volatile Hg. Hg is easily bioaccumulated in mangrove wetlands and may be the natural source of Hg emissions to the atmosphere. 相似文献
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本文通过对红河断裂北段相态汞的构造地球化学特征研究,认为表生条件下土壤汞主要以氯化汞和硫化汞存在。可用土壤相态汞进行活动断层勘查,其中反映较好的有气态汞、总汞、氯化汞和硫化汞。红河断裂上部较高的气态汞含量反映其强烈活动性。本文最后讨论了表生条件下土壤相态汞的可能转化模式。 相似文献
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汞观测中干扰因素的研究 总被引：2，自引：0，他引：2
本文通过实验及机理的分析研究表明：１．测汞仪气路中硅胶管对汞的的吸附水平受其本身温度的影响。温度升高，吸附汞的能力下降，释放其吸附汞的速度加快。在一定的温度下，硅胶管存在一个管内吸附汞与通过其中的气体中汞的释放和吸附的平衡；２．观测室温度的变化，除通过影响仪器气路（如硅胶管等）的温度百而影响观测结果外，主要是影响观测测室内壁汞进入空气的量，而影响空气汞本底，严重时可引起本底值值发生数十位的变化；３ 相似文献
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Jian Pang Jialiang Han Xuelu Fan Chan Li Xian Dong Longchao Liang Zhuo Chen 《Acta Geochimica》2019,(3):391-403
Mercury(Hg) is a global pollutant and can be accumulated in the food chain, posing exposure risks to humans. In this study, rice plants and corresponding rhizosphere soil samples were collected from a watershed of the Wawu River Basin that is heavily impacted by historic Hg mining and retorting activities. Total mercury(THg)and methylmercury(MeHg) in rice grains, as well as other tissues and soil samples, were measured. Five soil Hg fractions, as well as soil parameters, were also determined.The results show that the average concentrations of THg and MeHg in rice grains were 14 ± 7.0 lg kg-1 and7.2 ± 4.0 lg kg-1. Soil organic-bound(Hg-o) and strong complex-bound(Hg-s) were the main Hg fractions,accounting for 44% of the total. To estimate the Hg–ligand interaction in the soils, soil-N/Hg(R = 0.451, p \ 0.05),-S/Hg(R = 0.372, p \ 0.1), and-OM/Hg ratio(R = 0.320,p \ 0.5) with MeHgsoil were observed with significant positive correlations, indicating that the formation of Hg–OM, Hg–N–OM or Hg–S–OM complexes could prevent Hg(II) from methylation in soils. The significant positive correlations of the-N/Hg ratio,-S/Hg ratio and-OM/Hg ratio with MeHg in rice tissues suggested that Hg methylation and MeHg demethylation occurred throughout the rice paddy ecosystem. The estimated MeHg daily intake(EDI) was 0.075 ± 0.041 lg kg-1 bw d-1 and was lower than the RfD level of 0.1 lg kg-1 bw d-1 recommended by the US EPA. However, approximately 29% of the hazardous index(HI) of MeHg in grain exceeded 1, posing a potential threat to local populations, particularly pregnant women and children. 相似文献
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Total mercury (Hg) was measured in coastal fishes from Southern New England (RI, USA), and Hg exposure was estimated for anglers and family members that consumed these resources. Fish Hg was positively related to total length (n = 2028 across 7 fish species), and interspecies differences were evident among legally harvestable fish. Many recreational anglers and their families experienced excessively high Hg exposure rates, which was attributed to the enriched Hg content of frequently consumed fishes. Specifically, 51.5% of participants in this study had Hg exposures exceeding the US EPA reference dose, including 50.0% of women of childbearing years. These results are noteworthy given that Hg neurotoxicity occurs in adults and children from direct and prenatal low-dose exposure. Moreover, this study underscores the need for geographic-specific research that accounts for small-scale spatial variations in fish Hg and dietary habits of at-risk human populations. 相似文献
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Tomáš Navrátil James B. Shanley Jan Rohovec Irena Dobešová Šárka Matoušková Michal Roll Tereza Nováková Filip Oulehle 《水文研究》2021,35(6):e14255
From 2011 to 2019, mercury (Hg) stores and fluxes were studied in the small forested catchment Lesní potok (LES) in the central Czech Republic using the watershed mass balance approach together with internal measurements. Mean input fluxes of Hg via open bulk deposition, beech throughfall and spruce throughfall during the periodwere 2.9, 3.9 and 7.6 μg m−2 year−1, respectively. These values were considerably lower than corresponding deposition Hg fluxes reported in the early years of the 21st century from catchments in Germany. Current bulk precipitation inputs at unimpacted Czech mountainous sites were lower than those in Germany. The largest Hg inputs to the catchment were via litterfall, averaging 22.6 and 17.8 μg m−2 year−1 for beech and spruce stands. The average Hg input, based on the sum of mean litterfall and throughfall deposition, was 23.0 μg m−2 year−1, compared to the estimated Hg output in runoff of 0.5 μg m−2 year−1, which is low compared to other reported values. Thus, only ~2% of Hg input is exported in stream runoff. Stream water Hg was only weakly related to dissolved organic carbon (DOC) but both concentrations were positively correlated with water temperature. The estimated total soil Hg pool averaged 47.5 mg m−2, only 4% of which was in the O-horizon. Thus Hg in the O-horizon pool represents 72 years of deposition at the current input flux and 3800 years of export at the current runoff flux. Age-dating by 14C suggested that organic soil contains Hg from recent deposition, while mineral soil at 40–80 cm depth contained 4400-year old carbon, suggesting the soil had accumulated atmospheric Hg inputs through millennia to reach the highest soil Hg pool of the soil profile. These findings suggest that industrial era intensification of the Hg cycle is superimposed on a slower-paced Hg cycle during most of the Holocene. 相似文献
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Surface sediments and sediment cores collected from the Pearl River Estuary (PRE) were analyzed for total mercury (THg) concentrations and speciation using a sequential extraction method. The mobility of Hg in sediments was also assessed using a series of single extraction methods. The surface sediments from the PRE showed slightly elevated levels of Hg, with concentrations ranging from 109 to 453 ng/g. The vertical profile of THg in sediment cores indicated an accelerated input of Hg over the past decades. The organo-chelated and strong-complexed Hg species were the dominant Hg species in the sediments, while the more mobile phases of Hg made up less than 0.5% of THg. Less than 10% of the Hg in the sediments was extracted by single extraction, depending on the extractant employed. Significant relationships were found between the total organic carbon and THg, geochemical speciation, and extractability, indicating the important role of organic matter in controlling the distribution, mobility, and bioavailability of Hg in sediments. 相似文献
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Hg input into the ecosystem elements of the Sheksna Reservoir is studied. The accumulation and distribution of Hg in water, bottom sediment, fish, and snow falling onto the reservoir surfaces are considered. The distribution of Hg in water, bottom sediment, and snow is found to be specially nonuniform. The main sources of Hg are shown to be atmospheric precipitation and surface runoff from the watershed. The regularities of Hg accumulation in fish in different parts of the reservoir are studied. 相似文献