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1.
Berlin relies on induced bank filtration from a broad‐scale, lake‐type surface water system. Because the surface water contains treated sewage, wastewater residues are present in surface water and groundwater. Multiple environmental tracers, including tritium and helium isotopes (3H, 3He, 4He), stable isotopes (δ18O and δ2H) and a number of persistent sewage indicators, such as chloride, boron and a selection of pharmaceutical residues (phenazone‐type analgesics and their metabolites, carbamazepine and anthropogenic gadolinium, Gdexcess), were used to estimate travel times from the surface water to individual production and observation wells at two sites. The study revealed a strong vertical age stratification throughout the upper aquifer, with travel times varying from a few months to several decades in greater depth. Whereas the shallow bank filtrate is characterized by the reflection of the time‐variant tracer input concentrations and young 3H/3He ages, the deeper, older bank filtrate displays no tracer seasonality, 3H/3He ages of a few years to decades and strongly deviating concentrations of several pharmaceutical residues, reflecting concentrations of the source surface water over time. The phenazone‐type pharmaceuticals persist in the aquatic environments for decades. Bank filtration in Berlin is only possible at the sandy lakeshores. In greater water depth, impermeable lacustrine sapropels inhibit infiltration. The young bank filtrate originates from the nearest shore, whereas the older bank filtrate infiltrates at more distant shores. This paper illustrates the importance of using multiple tracer methods, capable of resolving a broad range of residence times, to gain a comprehensive understanding of time‐scales and infiltration characteristics in a bank filtration system. Copyright © 2007 John Wiley & Sons, Ltd.  相似文献   

2.
The results of a series of investigations are presented, performed by the governmental chemical laboratory Karlsruhe (CLUA) in order to determine pesticides in drinking water for purposes of food monitoring. 231 samples of 8 municipal water supplies (groundwater wells/no bank filtrate) and 34 private water supplies close to the bank of the river Rhine (groundwater wells/partly bank filtrate) were analysed. The sampling sites were located between Mannheim and Greffern, Germany. In 1986 high amounts of atrazine and simazine were determined in the drinking water wells of several private water supplies, especially at the sampling sites in the south. The likewise high chloride content of the samples was taken as a proof of bank filtrate contributing to the water. The decrease of atrazine load in the river water of the Rhine since 1987 has its parallel in the analytical results for the concerned drinking water wells. Obviously the pesticide contamination of water from bank filtrate pumping wells is mainly depending on the pesticide load of the river water. The application of fertilizers and pesticides in the fields seems not to be a significant source of the pesticide contamination of dringing waters derived from bank filtrate water. For reasons of public health a monitoring of pesticide content in bank filtrate pumping wells of private water supplies is recommended.  相似文献   

3.
The large volume of groundwater stored in the Tedori River alluvial fan, Ishikawa Prefecture, Japan, is an important source of local drinking and industrial water. The Tedori River was observed to be highly turbid from the beginning of May 2015 to at least November 2017 due to a landslide in the upper reach of the river. After the landslide, the groundwater level was drawn down by several to 10 m near the middle river section during paddy irrigation periods in 2015 and 2016. This study addresses the impacts of the highly turbid water on groundwater recharge from the river and paddy fields. In 2016, we sampled groundwater, river water, paddy irrigation water, paddy ponding water, and precipitation five times at 2-month intervals. We analysed the H, O, and Sr stable isotopic compositions and major dissolved ion (and Sr) concentrations and compared our data to previous data obtained in June 2011. Ca, Sr, Cl, SO4, and TN concentrations and δ18O values were higher in June 2016 than in June 2011; these increases were more extreme along the left bank of the Tedori River than along the right bank. We explored the mixing of Tedori River water with groundwater using a two-endmember mixing model based on their Sr concentrations and isotopic compositions. Compared to June 2011, mixing ratios were decreased near the Tedori River in 2016, and larger decreases were observed along the left bank and in the middle stream area. These results confirm that the contribution to groundwater recharge from the river decreased during the turbidity event, particularly along the left bank.  相似文献   

4.
Few studies have investigated large reaches of rivers in which multiple sources of groundwater are responsible for maintaining baseflow. This paper builds upon previous work undertaken along the Fitzroy River, one of the largest perennial river systems in north‐western Australia. Synoptic regional‐scale sampling of both river water and groundwater for a suite of environmental tracers (4He, 87Sr/86Sr, 222Rn and major ions), and subsequent modeling of tracer behavior in the river, has enabled definition and quantification of groundwater input from at least three different sources. We show unambiguous evidence of both shallow “local” groundwater, possibly recharged to alluvial aquifers beneath the adjacent floodplain during recent high‐flow events, and old “regional” groundwater introduced via artesian flow from deep confined aquifers. We also invoke hyporheic exchange and either bank return flow or parafluvial flow to account for background 222Rn activities and anomalous chloride trends along river reaches where there is no evidence of the local or regional groundwater inputs. Vertical conductivity sections acquired through an airborne electromagnetic (AEM) survey provide insights to the architecture of the aquifers associated with these sources and general groundwater quality characteristics. These data indicate fresh groundwater from about 300 m below ground preferentially discharging to the river, at locations consistent with those inferred from tracer data. The results demonstrate how sampling rivers for multiple environmental tracers of different types—including stable and radioactive isotopes, dissolved gases and major ions—can significantly improve conceptualization of groundwater—surface water interaction processes, particularly when coupled with geophysical techniques in complex hydrogeological settings.  相似文献   

5.
The acidic discharge from Cement Creek, containing elevated concentrations of dissolved metals and sulphate, mixed with the circumneutral‐pH Animas River over a several hundred metre reach (mixing zone) near Silverton, CO, during this study. Differences in concentrations of Ca, Mg, Si, Sr, and SO42? between the creek and the river were sufficiently large for these analytes to be used as natural tracers in the mixing zone. In addition, a sodium chloride (NaCl) tracer was injected into Cement Creek, which provided a Cl? ‘reference’ tracer in the mixing zone. Conservative transport of the dissolved metals and sulphate through the mixing zone was verified by mass balances and by linear mixing plots relative to the injected reference tracer. At each of seven sites in the mixing zone, five samples were collected at evenly spaced increments of the observed across‐channel gradients, as determined by specific conductance. This created sets of samples that adequately covered the ranges of mixtures (mixing ratios, in terms of the fraction of Animas River water, %AR). Concentratis measured in each mixing zone sample and in the upstream Animas River and Cement Creek were used to compute %AR for the reference and natural tracers. Values of %AR from natural tracers generally showed good agreement with values from the reference tracer, but variability in discharge and end‐member concentrations and analytical errors contributed to unexpected outlier values for both injected and natural tracers. The median value (MV) %AR (calculated from all of the tracers) reduced scatter in the mixing plots for the dissolved metals, indicating that the MV estimate reduced the effects of various potential errors that could affect any tracer. Copyright © 2006 John Wiley & Sons, Ltd.  相似文献   

6.
Understanding groundwater–surface water (GW–SW) interactions is vital for water management in karstic catchments due to its impact on water quality. The objective of this study was to evaluate and compare the applicability of seven environmental tracers to quantify and localize groundwater exfiltration into a small, human-impacted karstic river system. Tracers were selected based on their emission source to the surface water either as (a) dissolved, predominantly geogenic compounds (radon-222, sulphate and electrical conductivity) or (b) anthropogenic compounds (predominantly) originating from wastewater treatment plant (WWTP) effluents (carbamazepine, tramadol, sodium, chloride). Two contrasting sampling approaches were compared (a) assuming steady-state flow conditions and (b) considering the travel time of the water parcels (Lagrangian sampling) through the catchment to account for diurnal changes in inflow from the WWTP. Spatial variability of the concentrations of all tracers indicated sections of preferential groundwater inflow. Lagrangian sampling techniques seem highly relevant for capturing dynamic concentration patterns of WWTP-derived compounds. Quantification of GW inflow with the finite element model FINIFLUX, based on observed in-stream Rn activities led to plausible fluxes along the investigated river reaches (0.265 m3 s−1), while observations of other natural or anthropogenic environmental tracers produced less plausible water fluxes. Important point sources of groundwater exfiltration can be ascribed to locations where the river crosses geological fault lines. This indicates that commonly applied concepts describing groundwater–surface water interactions assuming diffuse flow in porous media are difficult to transfer to karstic river systems whereas concepts from fractured aquifers may be more applicable. In general, this study helps selecting the best suited hydrological tracer for GW exfiltration and leads to a better understanding of processes controlling groundwater inflow into karstic river systems.  相似文献   

7.
Mountainous areas are characterized by steep slopes and rocky landforms, with hydrological conditions varying rapidly from upstream to downstream, creating variable interactions between groundwater and surface water. In this study, mechanisms of groundwater–surface water interactions within a headwater catchment of the North China Plain were assessed along the stream length and during different seasons, using hydrochemical and stable isotope data, and groundwater residence times estimated using chlorofluorocarbons. These tracers indicate that the river is gaining, due to groundwater discharge in the headwater catchment both in the dry and rainy seasons. Residence time estimation of groundwater using chlorofluorocarbons data reveals that groundwater flow in the shallow sedimentary aquifer is dominated by the binary mixing of water approximating a piston flow model along 2 flow paths: old water, carried by a regional flow system along the direction of river flow, along with young water, which enters the river through local flow systems from hilly areas adjacent to the river valley (particularly during the rainy season). The larger mixing ratio of young water from lateral groundwater recharge and return flow of irrigation during the rainy season result in higher ion concentrations in groundwater than in the dry season. The binary mixing model showed that the ratio of young water versus total groundwater ranged from 0.88 to 0.22 and 1.0 to 0.74 in the upper and lower reaches, respectively. In the middle reach, meandering stream morphology allows some loss of river water back into the aquifer, leading to increasing estimates of the ratio of young water (from 0.22 to 1). This is also explained by declining groundwater levels near the river, due to groundwater extraction for agricultural irrigation. The switch from a greater predominance of regional flow in the dry season, to more localized groundwater flow paths in the wet season is an important groundwater–surface water interactions mechanism, with important catchment management implications.  相似文献   

8.
Understanding groundwater–surface water exchange in river banks is crucial for effective water management and a range of scientific disciplines. While there has been much research on bank storage, many studies assume idealized aquifer systems. This paper presents a field‐based study of the Tambo Catchment (southeast Australia) where the Tambo River interacts with both an unconfined aquifer containing relatively young and fresh groundwater (<500 μS/cm and <100 years old) and a semi‐confined artesian aquifer containing old and saline groundwater (electrical conductivity > 2500 μS/cm and >10 000 years old). Continuous groundwater elevation and electrical conductivity monitoring within the different aquifers and the river suggest that the degree of mixing between the two aquifers and the river varies significantly in response to changing hydrological conditions. Numerical modelling using MODFLOW and the solute transport package MT3DMS indicates that saline water in the river bank moves away from the river during flooding as hydraulic gradients reverse. This water then returns during flood recession as baseflow hydraulic gradients are re‐established. Modelling also indicates that the concentration of a simulated conservative groundwater solute can increase for up to ~34 days at distances of 20 and 40 m from the river in response to flood events approximately 10 m in height. For the same flood event, simulated solute concentrations within 10 m of the river increase for only ~15 days as the infiltrating low‐salinity river water drives groundwater dilution. Average groundwater fluxes to the river stretch estimated using Darcy's law were 7 m3/m/day compared with 26 and 3 m3/m/day for the same periods via mass balance using Radon (222Rn) and chloride (Cl), respectively. The study shows that by coupling numerical modelling with continuous groundwater–surface water monitoring, the transient nature of bank storage can be evaluated, leading to a better understanding of the hydrological system and better interpretation of hydrochemical data. Copyright © 2015 John Wiley & Sons, Ltd.  相似文献   

9.
Flow regulation and water diversion for irrigation have considerably impacted the exchange of surface water between the Murray River and its floodplains. However, the way in which river regulation has impacted groundwater–surface water interactions is not completely understood, especially in regards to the salinization and accompanying vegetation dieback currently occurring in many of the floodplains. Groundwater–surface water interactions were studied over a 2 year period in the riparian area of a large floodplain (Hattah–Kulkyne, Victoria) using a combination of piezometric surface monitoring and environmental tracers (Cl−, δ2H, and δ18O). Despite being located in a local and regional groundwater discharge zone, the Murray River is a losing stream under low flow conditions at Hattah–Kulkyne. The discharge zone for local groundwater, regional groundwater and bank recharge is in the floodplain within ∼1 km of the river and is probably driven by high rates of transpiration by the riparian Eucalyptus camaldulensis woodland. Environmental tracers data suggest that the origin of groundwater is principally bank recharge in the riparian zone and a combination of diffuse rainfall recharge and localized floodwater recharge elsewhere in the floodplain. Although the Murray River was losing under low flows, bank discharge occurred during some flood recession periods. The way in which the water table responded to changes in river level was a function of the type of stream bank present, with point bars providing a better connection to the alluvial aquifer than the more common clay‐lined banks. Understanding the spatial variability in the hydraulic connection with the river channel and in vertical recharge following inundations will be critical to design effective salinity remediation strategies for large semi‐arid floodplains. Copyright © 2005 John Wiley & Sons, Ltd.  相似文献   

10.
Peter G. Cook 《水文研究》2013,27(25):3694-3707
Environmental tracer methods have been used to quantify groundwater discharge to rivers for the past few decades. A number of different tracers have been used in these studies, including individual ion concentrations, electrical conductivity, stable isotopes 2H and 18O, and the dissolved gases helium, chlorofluorocarbons and radon. This paper discusses the assumptions of the method, as well as its resolution and accuracy. The method will be most accurate when the tracer concentration in groundwater is very distinct from that in the river. On the basis of typical parameters, groundwater inflow rates as low as 5 mm/day can usually be estimated with electrical conductivity and ion tracers. A lower limit of resolution of approximately 2 mm/day is usually possible with radon, principally because the ratio of the river concentration to the groundwater concentration will be higher. However, hyporheic exchange can also contribute radon to the river. Where this process is significant, it is more difficult to estimate groundwater inflow from radon activities in the river, thus reducing the accuracy of the method. For CFCs, the lower limit of resolution is approximately 30 mm/day. Helium has not been widely used but can potentially be very accurate if the groundwater is old. The method assumes steady‐state conditions and so can only be applied when river flows are stable. Sampling resolution is also particularly important for dissolved gases, and uncertainty in where groundwater inflow occurs between sampling points can cause large uncertainty in inflow rates if the distance between sample locations is large. Poor mixing of solutes within the river can limit the method if the river is wide and shallow. When correctly applied, however, the environmental tracer method is able to provide robust estimates of groundwater discharge at a scale and accuracy that is not possible with most other methods. Copyright © 2012 John Wiley & Sons, Ltd.  相似文献   

11.
Groundwater discharges in the western Canadian oil sands region impact river water quality. Mapping groundwater discharges to rivers in the oil sands region is important to target water quality monitoring efforts and to ensure injected wastewater and steam remain sequestered rather than eventually resurfacing. Saline springs composed of Pleistocene‐aged glacial meltwater exist in the region, but their spatial distribution has not been mapped comprehensively. Here we show that formation waters discharge into 3 major rivers as they flow through the Athabasca Oil Sands Region adjacent to many active oil sands projects. These discharges increase river chloride concentrations from river headwaters to downstream reaches by factors of ~23 in the Christina River, ~4 in the Clearwater River, and ~5 in the Athabasca River. Our survey provides further evidence for the substantial impact of formation water discharges on river water quality, even though they comprise less than ~2% of total streamflow. Geochemical evidence supporting formation water discharges as the leading control on river salinity include increases in river chloride concentrations, Na/(Na + Ca) ratios, Cl/(Cl + SO4) ratios and decreases in 87Sr/86Sr ratios; each mixing trend is consistent with saline groundwater discharges sourced from Cretaceous or Devonian aquifers. These regional subsurface‐to‐surface connections signify that injected wastewater or steam may potentially resurface in the future, emphasizing the critical importance of mapping groundwater flow paths to understand present‐day streamflow quality and to predict the potential for injected fluids to resurface.  相似文献   

12.
Riverbank filtration (RBF) has been widely used throughout the world as an effective means to regulate surface water and groundwater resources and pretreat raw water for municipal water supply. The quality of the water from a riverside well field and the mixing ratios of surface water and groundwater is primarily impacted by the hydrodynamic processes in the RBF system. The RBF system is largely controlled by the water exploiting system in addition to the natural hydrologic condition of the river–aquifer system. As one of the most important design parameters of the riverside well field, the drawdown of groundwater level greatly determines the water head differences between the river water and groundwater as well as the field flow net, which subsequently impacts the mixing of river water and groundwater and water quality significantly. This study aimed to improve the understanding of the mixing process between the surface water and groundwater and estimate the impact of the RBF on the mixing ratio of surface water–groundwater and water quality quantitatively. A set of field pumping tests with various groundwater level drawdowns were carried out independently and successively at a riverside field with a single pumping well near the Songhua River in Northeast China in August 2017. During these tests, the water levels and hydrochemical parameters of the Songhua River, the adjacent aquifer, and the pumping well were monitored. The dynamic mixing process of the river water and groundwater and water quality under various drawdown conditions were analysed systematically using analytical methods. The results obtained from Dupuit method and the Mirror Image method in conjunction with the Hydrochemical Tracing method showed that the pumping water directly from the river water reached 60% ± 10% after a steady flow net was established. The larger the proportion of the pumping water captured from the river, the better quality of the pumping water was, because the quality of the river water (only limited to some water quality parameters monitored which were minority) was better than that of the groundwater. The results also showed that total Fe, TDS, total hardness, CODMn, and K+ were relatively sensitive to the changes of groundwater drawdown, and their concentrations decreased with an increase in the groundwater drawdown. It can be concluded that both the mixing ratio of the surface water and the groundwater and the water quality of the riverside well field can be regulated through adjusting the designed drawdown of the groundwater level, which is helpful for the design and the optimization of the riverside well water intake engineering.  相似文献   

13.
This paper examines groundwater hydrochemical characteristics during mixing between thermal and non-thermal groundwater in low-to-medium temperature geothermal fields. A case study is made of Daying and Qicun geothermal fields in the Xinzhou basin of Shanxi province, China. The two geothermal fields have similar flow patterns, with recharge sourced from precipitation in mountain areas heated through a deep cycle, before flowing into overlying Quaternary porous aquifers via fractures. Hydrochemical features of 60 ground- and surface water samples were examined in the context of hydrogeologic information. The average temperatures of the deep geothermal reservoirs are estimated to be 125 °C in Daying field, and 159 °C in Qicun field, based on Na–K–Mg geothermometry, while slightly lower estimates are obtained using silica geothermometers. Hydrochemical features of thermal water are distinct from cold water. Thermal groundwater is mainly Cl·SO4–Na type, with high TDS, while non-thermal groundwater is mostly HCO3–Ca·Mg and HCO3–Ca type in the Daying and Qicun regions, respectively. Hydrogeochemical processes are characterized by analyzing ion ratios in various waters. Higher contents of some minor elements in thermal waters, such as F, Si, B and Sr, are probably derived from extended water–rock interaction, and these elements can be regarded as indicators of flow paths and residence times. Mixing ratios between cold and thermal waters were estimated with Cl, Na, and B concentrations, using a mass balance approach. Mixing between ascending thermal waters and overlying cold waters is extensive. The proportion of water in the Quaternary aquifer derived from a deep thermal source is lower in Daying geothermal field than in Qicun field (5.3–7.3% vs. 6.3–49.3%). Mixing between thermal and non-thermal groundwater has been accelerated by groundwater exploitation practices and is enhanced near faults. Shallow groundwater composition has also been affected by irrigation with low-temperature thermal water.  相似文献   

14.
Models simulating stream flow and conservative tracers can provide a representation of flow paths, storage distributions and mixing processes that is advantageous for many predictive purposes. Compared with models that only simulate stream flow, tracer data can be used to investigate the internal consistency of model behaviour and to gain insight into model performance. Here, we examine the strengths and weaknesses of a data‐driven, spatially distributed tracer‐aided rainfall‐runoff model. The model structure allowed us to assess the influence of landscape characteristics on the routing and mixing of water and tracers. The model was applied to a site in the Scottish Highlands with a unique tracer data set; ~4 years of daily isotope ratios in stream water and precipitation were available, as well as 2 years of weekly soil and ground water isotopes. The model structure was based on an empirically based, lumped tracer‐aided model previously developed for the catchment. The best model runs were selected from Monte Carlo simulations based on dual calibration criteria using objective functions for both stream isotopes and discharge at the outlet. Model performance for these criteria was reasonable (Nash–Sutcliffe efficiencies for discharge and isotope ratios were ~0.4–0.6). The model could generally reproduce the variable isotope signals in the soils of the steeper hill slopes where storage was low, and damped isotope responses in valley bottom cells with high storage. The model also allowed us to estimate the age distributions of internal stores, water fluxes and stream flow. Average stream water age was ~1.6 years, integrating older groundwater in the valley bottom and dynamic younger soil waters. By tracking water ages and simulating isotopes, the model captured the changes in connectivity driven by distributed storage dynamics. This has substantially improved the representation of spatio‐temporal process dynamics and gives a more robust framework for projecting environmental change impacts. Copyright © 2016 The Authors Hydrological Processes Published by John Wiley & Sons Ltd.  相似文献   

15.
A key parameter used in the assessment of bank filtration is the travel time of the infiltrated river water during the passage through groundwater. We analyze time series of electrical conductivity (EC) in the river and adjacent groundwater observation wells to investigate travel times of young hyporheic groundwater in adjoining channelized and restored sections of River Thur in North-East Switzerland. To quantify mixing ratios and mean residence times we perform cross-correlation analysis and non-parametric deconvolution of the EC time series. Measurements of radon-222 in the groundwater samples validate the calculated residence times. A simple relationship between travel time and distance to the river has not been observed. Therefore, we speculate that the lateral position and depth of the thalweg as well as the type of bank stabilization might control the infiltration processes in losing rivers. Diurnal oscillations of EC observed in the river and in nearby observation wells facilitate analyzing the temporal variation of infiltration. The diurnal oscillations are particularly pronounced in low flow situations, while the overall EC signal is dominated by individual high-flow events. Differences in travel times derived from diurnal and overall EC signals thus reflect different infiltration regimes.  相似文献   

16.
Critical zone influences on hydrologic partitioning, subsurface flow paths and reactions along these flow paths dictate the timing and magnitude of groundwater and solute flux to streams. To isolate first‐order controls on seasonal streamflow generation within highly heterogeneous, snow‐dominated basins of the Colorado River, we employ a multivariate statistical approach of end‐member mixing analysis using a suite of daily chemical and isotopic observations. Mixing models are developed across 11 nested basins (0.4 to 85 km2) spanning a gradient of climatological, physical, and geological characteristics. Hydrograph separation using rain, snow, and groundwater as end‐members indicates that seasonal contributions of groundwater to streams is significant. Mean annual groundwater flux ranges from 12% to 33% whereas maximum groundwater contributions of 17% to 50% occur during baseflow. The direct relationship between snow water equivalent and groundwater flux to streams is scale dependent with a trend toward self‐similarity when basins exceed 5.5 km2. We find groundwater recharge increases in basins of high relief and within the upper subalpine where maximum snow accumulation is coincident with reduced conifer cover and lower canopy densities. The mixing model developed for the furthest downstream site did not transfer to upstream basins. The resulting error in predicted stream concentrations points toward weathering reactions as a function of source rock and seasonal shifts in flow path. Additionally, the potential for microbial sulfate reduction in floodplain sediments along a low‐gradient, meandering portion of the river is sufficient to modify hillslope contributions and alter mixing ratios in the analysis. Soil flushing in response to snowmelt is not included as an end‐member but is identified as an important mechanism for release of solutes from these mountainous watersheds. End‐member mixing analysis used in combination with high‐frequency observations reveals important aspects of catchment hydrodynamics across scale.  相似文献   

17.
Understanding rainfall‐runoff processes is crucial for prevention and prediction of water‐related natural disasters. Sulfur hexafluoride (SF6) is a potential tracer, but few researches have applied it for rainfall‐runoff process studies. We observed multiple tracers including SF6 in spring water at 1‐ to 2‐hr intervals during rainstorm events to investigate the effectivity of SF6 tracer in rainfall–runoff studies through the clarification of rainfall–runoff process. The target spring is a perennial spring in a forested headwater catchment with an area of 0.045 km2 in Fukushima, Japan. The relationship between the SF6 concentration in spring water and the spring discharge volume was negative trend; the SF6 concentration in spring water becomes low as the spring discharge volume increases especially during rainstorms. The hydrograph separation using SF6 and chloride ion tracers was applied for determining the contribution of principal sources on rainfall–runoff water. It suggested more than 60% contribution of bedrock groundwater at the rainfall peak and high percentage contribution continued even in the hydrograph recession phase. Based on observed low SF6 concentration in groundwater after heavy rainfall, the replacement of groundwater near the spring with bedrock groundwater is indicated as a mechanism for water discharge with low SF6 concentration during rainfall events. Consequently, rainstorm events play an important role as triggers in discharging water stored in the deeper subsurface area. In addition, SF6 tracer is concluded as one of the strongest tracers for examining rainfall–runoff process studies. And, therefore, this study provided new insights into the dynamics of groundwater and its responses to rainfall in terms of SF6 concentration variance in water in headwater regions.  相似文献   

18.
Soil water, stream water, groundwater and rain water were sampled through a storm event in a moorland catchment. Samples were analysed for major ions and deuterium. Chloride and deuterium are used as tracers to enable separation of the stream runoff hydrograph into three components: rain, soil and groundwater. The results indicate that rain water arrives in the stream quickly during the event and contributes a significant volume to the runoff peak. The chemical signal in the rain water is, however, significantly damped, apparently due to mixing with soil water held in the catchment before the event. This is further modified before reaching the stream, apparently through mixing with a deeper groundwater component. Interpretation of tracer, chemistry and hydrological data to present an integrated picture of catchment hydrochemical response is difficult due to problems in the chemical and conceptual definition of the flow components.  相似文献   

19.
The artificial sweetener acesulfame (ACE) is a potentially useful tracer of waste water contamination in groundwater. In this study, ACE concentrations were measured in waste water and impacted groundwater at 12 septic system sites in Ontario, Canada. All samples of septic tank effluent (n = 37) had ACE >6 µg/L, all samples of groundwater from the proximal plume zones (n = 93) had ACE >1 µg/L and, almost all samples from the distal plume zones had ACE >2 µg/L. Mean mass ratios of total inorganic nitrogen/ACE at the 12 sites ranged from 680 to 3500 for the tank and proximal plume samples. At five sites, decreasing ratio values in the distal zones indicated nitrogen attenuation. These ratios were applied to three aquifers in Canada that are nitrate‐stressed and an urban stream where septic systems are present nearby to estimate the amount of waste water nitrate contamination. At the three aquifer locations that are agricultural, low ACE values (<0.02‐0.15 µg/L) indicated that waste water contributed <15% of the nitrate in most samples. In groundwater discharging to the urban stream, much higher ACE values (0.2‐11 µg/L) indicated that waste water was the likely source of >50% of the nitrate in most samples. This study confirms that ACE is a powerful tracer and demonstrates its use as a diagnostic tool for establishing whether waste water is a significant contributor to groundwater contamination or not.  相似文献   

20.
The three-dimensional groundwater flow patterns in a gravel bar at the Danube east of Vienna were investigated and are discussed in this paper. The observed groundwater level gradients are highly dynamic and respond very quickly to changes in the river water levels. A variably saturated groundwater model was calibrated to the data to describe the complex dynamics of flow in the gravel bar. The model results suggest that short-term (6–48 h) fluctuations of river water levels cause variations in the exchange flow rates from − 35 l/s to 82 l/s. The highest rates occur during brief infiltration after rapidly rising river water levels. Simulations of different scenarios indicate that riverbank clogging will decrease the exchange fluxes by up to 80%, while clogging of both riverbank and riverbed essentially stops the flow exchange. The groundwater model is also used to simulate the transport of a conservative tracer. The variation of river water levels over time is shown to increase the extent of the active river–aquifer mixing zone in the gravel bar. These dynamic factors significantly enhance the dilution of conservative tracer concentrations in this zone.  相似文献   

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