共查询到20条相似文献，搜索用时 15 毫秒
1.
膨胀云室可形成水汽、水面和冰面过饱和环境,是研究气溶胶粒子、人工影响天气冷暖催化剂核化过程和机理的重要实验设备。但长期以来,我国缺乏装备先进云雾粒子谱和图像测量系统的膨胀云室。2019年完成的我国自主研制的膨胀云室系统由云室主体、控制系统、通讯系统及环境和云雾测量系统4个子系统组成。该系统首次采用了国产云粒子谱仪和成像仪测量系统。测试结果表明:该云室具有良好的温度和压力控制能力,平均降温速率达到0.26℃·min-1,温度分布均匀,-40℃时舱内温差小于0.29℃;膨胀造雾过程4 min,雾可维持4 min,雾滴较小;可以实现从室温到-50℃低温环境的控制,具备压力膨胀成云雾模拟和微物理参数监测能力,解决了我国缺乏气溶胶粒子和暖云催化剂室内实验装备的状况,对验证暖云催化剂核化性能和提高暖云人工增雨科技水平有重要价值。 相似文献
2.
T. Sugita Y. Kondo M. Koike M. Kanada N. Toriyama H. Nakajima T. Deshler R. Imasu 《Journal of Atmospheric Chemistry》1999,32(1):183-204
A new balloon-borne optical particle counter has been developed to make in situ measurements of stratospheric aerosols. The intensity of light scattered at 60° from the forward direction by individual particles is measured. Aerosol number concentrations in seven size channels can be inferred. The counter has been calibrated using polystyrene and polyvinyl toluene latex spheres. There is good agreement between measured and calculated individual pulse intensities for aerosol with radii from 0.16 to 2.6 µm. The size resolution is limited by broadening of the pulse count/pulse height spectrum, arising mainly from the photoelectron statistics of photomultipliers. Stratospheric aerosol measurements have been made using this instrument at Kiruna (68°N, 21°E), Sweden, in February 1995, and at Aire sur l'Adour (44°N, 0°W), France, in 1992, 1993, and 1994. The uncertainties in the measurements are discussed. The retrieved aerosol concentrations and size distributions are presented, and shown to be broadly consistent with measurements made by the University of Wyoming optical particle counter. 相似文献
3.
A multifunctional HTDMA system with a robust temperature control 总被引：3，自引：0，他引：3
The hygroscopicity of atmospheric aerosols significantly influences their size distribution,
cloud condensation nuclei ability, atmospheric residence time, and climate forcing. In order to investigate
the hygroscopic behavior of aerosol particles and serious haze in China, a Hygroscopic Tandem Differential
Mobility Analyzers (HTDMA) system was designed and constructed at Fudan University. It can function as a
scanning mobility particle sizing system to measure particle size distribution in the range of 20--1000 nm
in diameter, as well as a hygroscopicity analyzer for aerosol particles with diameters between 20--400 nm
in the range of 20%--90% RH (relative humidity). It can also measure the effect of uptake of inorganic acids
or semi-VOCs on the hygroscopic behavior of aerosols, such as typical inorganic salts in atmospheric dust or
their mixtures. The performance tests show that the system measured particle size of the standard polystyrene
latex spheres (PSLs) is 197 nm, which is in excellent agreement with the certified diameter D=199±6 nm, as
well as a standard deviation of the repeated runs SD=8.9x10-4. In addition, the measured hygroscopic
growth factors of the model compounds, (NH4)2SO4 and NaNO3, agree with the Kohler theoretical
curves. The results indicate that the HTDMA system is an excellent and powerful tool for studying the
hygroscopic behavior of submicron aerosols and meets the demand required for laboratory research and
fieldwork on atmospheric aerosols in China. 相似文献
4.
H.-C. Hansson M. J. Rood S. Koloutsou-Vakakis K. Hämeri D. Orsini A. Wiedensohler 《Journal of Atmospheric Chemistry》1998,31(3):321-346
Organic compounds in the atmosphere can influence the activation, growth and lifetimes of haze, fog and cloud droplets by changing the condensation and evaporation rates of liquid water by these aqueous aerosol particles. Depending on the nature and properties of the organic compounds, the change can be to enhance or reduce these rates. In this paper we used a tandem differential mobility analyzer (TDMA) to examine the effect of tetracosane, octanoic acid, and lauric acid on the hygroscopic properties of NaCl aerosol particles at relative humidities (RH) between 30 and 95%. These organic compounds have been identified in ambient aerosol particle samples. A slight lowering of the deliquescence relative humidity (DRH) and suppression of hygroscopic growth for the NaCl-organic compound mixtures were observed when compared to pure NaCl particles. The growth of pure NaCl particles was 2.25 in diameter at 85% RH while the growth of the mixed particles was 1.3 to 1.7 in particle diameter at 85% RH with organic mass fraction of 30–50%. This shows that these organic compounds have to be present in rather large mass fractions to effect the hygroscopic behavior to a similar degree observed for ambient aerosol during field measurements. Despite the mixing of the organic material with NaCl, hysteresis was observed for decreasing RH histories, suggesting the formation of metastable droplets. These laboratory results are strikingly similar to ambient field results. For example, if the total organic mass fraction of the particles is between 0.30 and 0.50, the particle growth at 85% RH is about a factor of 1.4 for the laboratory and field measurements. Such reduction in growth compared to the pure inorganic salt is in contradiction to speculations concerning significant effects by organic compounds on cloud condensation nuclei and thus formation on clouds. 相似文献
5.
Assessment of the radiative forcing of aerosols in models still lacks sufficient input data for aerosol hygroscopicity. The light scattering enhancement factor [ f(RH, λ)] is a crucial parameter for describing aerosol hygroscopic growth properties.In this paper, we provide a survey of f(RH, λ) studies in China for the past seven years, including instrument developments of humidified nephelometers, ambient f(RH, λ) measurements in China, f(RH, λ) parameterization schemes, and f(RH, λ)applications in aerosol measurements. Comparisons of different f(RH, λ) parameterizations are carried out to check their performance in China using field measurement datasets. We also summary the parameterization schemes for predicting f(RH, λ)with aerosol chemical compositions. The recently developed methods to observe other aerosol properties using f(RH, λ)measurements, such as calculating the aerosol hygroscopicity parameter, cloud condensation nuclei number concentration,aerosol liquid water content, and aerosol asymmetry factor, are introduced. Suggestions for further research on f(RH, λ) in China are given. 相似文献
6.
海雾是一种常见的灾害性天气现象。以我国台湾海峡为示范研究区, 利用新一代卫星传感器MODIS的可见光和红外探测通道数据, 在分析海洋、中高云、低云和海雾等不同下垫面的MODIS光谱辐射特征基础上, 选择对海雾具有敏感反应的探测通道, 通过综合判识建立台湾海峡海雾遥感监测模型。利用该模型对2004-2007年我国台湾海峡海雾事件进行监测, 并用福建沿海5个地面气象观测站的能见度数据对监测结果进行验证分析。结果表明:基于MODIS数据的海雾遥感监测模型能够较准确地对台湾海峡海雾分布和发展过程进行监测, 从地面观测数据与卫星监测结果对比验证来看, 海雾监测的准确率可达80 %以上, 具有较高的业务化应用前景。 相似文献
7.
Richter David H. MacMillan Theodore Wainwright Charlotte 《Boundary-Layer Meteorology》2021,181(2-3):523-542
A large-eddy simulation model is coupled with a Lagrangian cloud model to study marine fog. In this model, aerosols and droplets are treated from a Lagrangian frame of reference, in contrast to the traditional bulk and bin microphysical models. Droplet growth via condensation is governed by Köhler theory and environmental conditions local to the droplet. Coupling to the vapour and temperature fields of the flow ensures mass, momentum, and energy conservation between the air and droplet phases. Based on the recent C-FOG field campaign, a simulation is performed which highlights the benefits and potential of this type of model. By initializing the simulation with the measured aerosol size distribution and making assumptions about the chemical composition of the multiple peaks, the simulations provide a clear explanation for the observed bimodal droplet distribution during C-FOG: high supersaturation levels cause condensational growth of nearly all coarse-mode aerosols (presumed to be composed of marine salt), as well as a large number of accumulation model aerosols (presumed to be of continental origin with a lower hygroscopicity). The largest peak in the resulting droplet distribution is created from coarse-mode aerosols with high hygroscopicity, while the secondary peak is only possible due to the limited impact of the largest peak on saturation levels inside the fog. Thus, for the simulated levels of supersaturation, it is the limited number of coarse-mode aerosols which is responsible for the emergence of a larger second peak.
相似文献8.
Jacqueline H. Carrillo Scott E. Emert D. Eli Sherman Pierre Herckes Jeffrey L. Collett Jr. 《Atmospheric Research》2008,87(3-4):259
A new, relatively low cost instrument has been developed to detect the presence of fog or cloud for fog/cloud sampling applications. The instrument uses attenuation of an 880 nm light emitting diode signal to detect cloud/fog drops in the optical path between a sending and receiving arm. Laboratory and field testing under a variety of conditions and fog types were carried out to determine the ability of the optical fog detector (OFD) to accurately detect cloud/fog presence as well as to provide some measure of liquid water content. Results indicated that the OFD provided a reliable estimate of fog presence as well as a reasonable estimate of liquid water content (LWC) under several different conditions. The OFD does appear to have an interference from rain, resulting in an overestimation of LWC during rainfall. This may occasionally give a false positive indication of fog presence. 相似文献
9.
南岭大瑶山高速公路浓雾的宏微观结构与能见度研究 总被引：20，自引：2，他引：20
南岭山地地处南亚热带湿润型季风气候区,每年9月至次年5月有华南准静止锋活动时均会有浓雾发生,每月浓雾日可高达15—18 d,尤其是中国目前最长的京珠高速公路通过南岭主脉大瑶山的乐昌—乳源段,路面海拔高度从200 m增至800多米,山地的抬升使雾害更加严重。在南岭大瑶山高速公路开展的两次多学科综合野外观测,内容包括目测能见度、器测能见度、雾滴谱、雾含水量、系留探空、双参数低空探空、雾层湍流扩散、气溶胶粒子谱、气溶胶成分谱、雾水样品成分、雨水样品成分。对典型个例进行了天气学分析,雾的宏观结构特征分析,雾的微物理特征分析。认识到南岭山地浓雾发生频率高,雾害十分严重,是典型的平流雾和上坡雾,实质上是出现在相对较高海拔高度上的低云,与华南锋面活动尤其是华南准静止峰的活动密切相关,局地地形的作用也非常重要。其特点是浓雾持续时间长、能见度极其恶劣、团块结构明显、雾滴尺度大、浓度不高、含水量较大、雾层内的湍流扩散能力比晴空区强,与中国过去研究较多的辐射雾差别较大。发现雾含水量与能见度呈明显的反相关关系,含水量较大时能见度较小;南岭山地雾含水量等微结构特征量的起伏变化,除与雾体本身的结构不均匀有关外,一个重要的原因是平流因素的影响,南岭山地下垫面的不均匀性,雾体随环境风的平移过程中,不规则的爬坡、翻越山坡的运动是造成雾体结构不均匀、振荡起伏变化的另一个重要原因。该地气溶胶粒子谱是呈单调下降的幂函数谱,次微米粒子浓度甚高,南岭山地气溶胶中含有高浓度的硫酸盐粒子,是优质凝结核,有利于雾的形成。雾的存在可以清除大气中的微量成分,雾滴可以包含浓度很高的污染物成分。同时,较之云滴而言,雾滴也很容易被地表物体(如植被、建筑物等)的垂直表面所截获,构成另一类清除过程。在南岭这样的大面积森林地区,这类清除过程可能是很重要的。研究本地区雾的特征变化,对建立本地区雾的预警预报系统有很大的现实意义,并为开展消雾试验提供了基本资料。 相似文献
10.
On the influence of the physico-chemical properties of aerosols on the life cycle of radiation fogs 总被引：3，自引：0，他引：3
Andreas Bott 《Boundary-Layer Meteorology》1991,56(1-2):1-31
A one-dimensional model of radiation fog with detailed microphysics is presented. Aerosols and cloud droplets are treated in a joint two-dimensional size distribution. Radiative fluxes are calculated as functions of the radiative properties of the time-dependent particle spectra. The droplet growth equation is solved by considering radiative effects. Turbulence is treated by means of a higher order closure model. The interaction between the atmosphere and the earth's surface is explicitly simulated.Three numerical sensitivity studies are performed to investigate the impact of the different physico-chemical properties of urban, rural and maritime aerosols on fog formation. Numerical results elucidate that depending on the aerosol type used, the resulting fog events are completely different. This is particularly true for the times of fog formation and dissipation as well as for the liquid water content and supersaturations within the fogs. In the activated part of the particle spectra, the aerosol mass is very inhomogeneously distributed. The maxima of the curves do not coincide with the maxima of the corresponding liquid water distributions. 相似文献
11.
针对自然界中雾天气向霾天气转化的现象,提出建立和发展雾环境气溶胶颗粒物多效应的动力学模型。基于离散系统的颗粒群平衡方程和多重Monte Carlo算法,分别对雾形成阶段（凝并、冷凝和成核3个动力学事件占主导）、雾发展阶段（凝并、破碎、沉积和成核4个动力学事件占主导）和雾消散阶段（破碎、蒸发和沉积3个动力学事件占主导）气溶胶颗粒物平均体积、颗粒数目随时间的演变过程进行研究。结果表明：气溶胶颗粒物的初始体积尺度为1,经过雾的生命周期进入消散阶段时,尺度为0.0156的细小气溶胶颗粒数目迅速增加,1000 s时间已发展至初始值的8.12倍。研究结果解释了自然界中雾天气向霾天气转化的过程和物理机制。 相似文献
12.
都市霾与雾的区分及粤港澳的灰霾天气观测预报预警标准 总被引：17，自引：16，他引：17
都市霾与雾的区分是迫切需要解决的问题。霾的出现有重要的空气质量指示意义,而雾的记录,有明确的天气指示意义。通常在平面时已达到饱和的水汽压,对相当于球面的云雾滴来讲就是未饱和的,云雾滴就会蒸发;在水汽条件不变时,云雾滴由于蒸发而变小,导致它的平衡水汽压升高,就更易蒸发掉。在不饱和大气中小于数μm的云雾滴必然蒸发,而且伴随着蒸发云雾滴尺度会进一步变小,导致曲率越来越大,蒸发速率越来越快。过去错误认为凝结核可以在低相对湿度(RH)情况下产生凝结生成雾滴的观点,是忽视了粒子曲率作用的结果,将实验室大颗粒(常常达mm量级)的吸湿性特征,延用至次μm粒子造成的。降温是达到饱和形成雾滴的重要物理过程,云雾是低温下饱和气块的可见标志。在云雾中必然存在凝结或凝华过程,因而必然伴随着潜热释放,这就使云雾内的温度高于环境,在云雾内必然盛行微弱的上升气流,不可能是下沉气流,这些宏观过程在霾层内是不存在的,因而成为识别雾与霾的重要的宏观动力条件。在对历史资料进行统计时,在排除降水、吹雪、雪暴、沙尘暴、扬沙、浮尘、烟幕等视程障碍现象的情况下,通过调试RH,使雾与轻雾反映自然的年际与年代际气候波动,而霾反映由于人类活动而引起的趋势性变化,其限值大体在90%左右,与美国和英国在讨论霾影响能见度(vis)的长期变化趋势中使用的限值RH<90%相同。20世纪80年代以来大幅增加的霾日,绝大部分是由于人类活动影响的气溶胶细粒子污染造成的。依据上述结果和以前的研究,给出了霾与雾区分的概念模型、霾与雾观测的标准和灰霾天气预警信号发布的标准,并介绍了相关的业务产品。 相似文献
13.
2016年11月13日在北京地区上空存在持续稳定的层状云天气背景下,利用飞机开展气溶胶粒径谱、化学组成、云滴谱等参量的垂直观测,研究该个例云底气溶胶的活化能力。结果表明:探测期间北京地区为轻度污染天气,地面气溶胶浓度(0.11~3 μm)达到4600 cm-3。云层高度为800~1200 m,云底气溶胶数浓度相对于近地面大幅度降低,有效粒径显著增大(0.3~0.6 μm)。同时,近地面气溶胶中疏水性的一次有机气溶胶贡献显著,而云底气溶胶中一次有机气溶胶的贡献大幅降低,无机组分和二次有机气溶胶的贡献明显增大,造成吸湿性参数κ由0.25(地面)增大至0.32(云底)。云中气溶胶和云滴的谱分布衔接较好,且两者的数浓度之和与云底气溶胶浓度一致,可分别代表未活化和已活化的粒子。基于云底气溶胶粒径谱和吸湿性参数计算得到不同过饱和比下云凝结核的活化率,通过与云中观测结果对比,反推得到云底过饱和度约为0.048%。 相似文献
14.
WU Dui DENG Xuejiao MAO Jietai MAO Weikang YE Yanxiang BI Xueyan 《Acta Meteorologica Sinica》2007,21(3):342-352
Belonging to the southern subtropical moist type of monsoon climate, the Nanling mountainous area
experiences heavy fogs whenever quasi-stationary fronts appear there from September to May. There can be as many as 15-18 days of heavy fogs per month. Fogs have more serious consequences in the Lechang-Ruyuan section of the Beijing-Zhuhai Expressway (the longest expressway in China) that passes through the main part of the Nanling Mts., where the road rises from 200 m to more than 800 m above sea level (ASL).For a major motorway in the mountainous areas of Nanling Mts., two multidisciplinary integrated field observations were carried out, which measured visibility by the naked eyes, visibility by instrument, spectrum of fogdrops, liquid water content (LWC) of fog, tethered sounding, dual-parameter low-level sounding, turbulence diffusion within fog layers, aerosol spectra of size and composition, sampled fog water compositions, and sampled rainwater compositions. Typical cases were probed for their analyses of synoptics, micro- and macro-structures and microphysics. It is understood that heavy fogs take place with high frequency in the area and bring about serious consequences. Being typical advection and upslope fogs, they are in essence low-lying clouds appearing at high altitudes,which are closely related with the activity of South China frontal processes, especially the South China quasi-stationary fronts, and reflect on the role of local terrain as well. The heavy fogs are characteristic of long duration, extremely low visibility, well-organized lump-shaped structure, large-size fog-drops, moderate concentration, high LWC, and stronger turbulent diffusion within the fog layers than in ne sky. They di er much from radiation fogs, which are better documented in previous study in China. It is found that fog LWC is in significant anti-correlation with visibility so that large LWC is associated with small visual range. It is also noted that one of the reasons for the fluctuation of characteristic quantities of micro-structure such as the LWC of fog in the area is, in addition to the inhomogeneous structure of the fog itself, the effect of advection and inhomogeneous underlying surface;during the translation of fog with the ambient wind, irregular upslope and cross-over movement is another reason for the inhomogeneous structure and fluctuation of fog. The spectrum of the aerosol size displays itself as the power function of monotonous descent. The concentration of submicrometer particles is even higher. The high-concentration sulfate particles found in the aerosols of Nanling Mts. are actually good
nuclei for condensation, which are favorable for the formation of fog. The presence of fog can help cleanse the trace compositions in the atmosphere so that fog droplets contain high levels of polluting elements. In the meantime, compared to cloud droplets, fog droplets are easier to be captured by the vertical surfaces of objects on the land surface, such as vegetation and buildings to constitute another kind of cleansing process.In vast stretches of forest like the Nanling Mts., this kind of cleansing may be quite important. Studying the characteristic variation of fogs in the area realistically assists in setting up a forecast and warning system for local fogs and provides basic information for fog dispersal experiments. 相似文献
15.
16.
714KaDP型云雾雷达具备30km内的低云和雾监测和预警能力,是专门针对影响机场运行的低云低能见度(两低)天气研制的国内首部毫米波脉冲多普勒雷达。昆明长水机场的试验验证表明,通过提供的云雾基本产品和二次产品,实现了机场两低天气生消演变的有效探测,显著提升了对严重影响空管正常运行的两低天气的监测预警能力。雷达探测发现,714KaDP型云雾雷达对机场及周边低云和雾的生消、演变、移动有着非常敏锐的捕捉能力,特别适合具有明显平流特征的低云和雾(锋面雾、低云平流、辐射雾平流等)的监测和预警,本文介绍了雷达特性、安装位置以及对锋面雾、平流低云和辐射平流混合雾过程的雷达产品分析方法,为提前预警、实时跟踪和云消雾散二次放行决策提供支撑提供了参考。 相似文献
17.
Belonging to the southern subtropical moist type of monsoon climate,the Nanling mountainous area experiences heavy fogs whenever quasi-stationary fronts appear there from September to May.There can be as many as 15-18 days of heavy fogs per month.Fogs have more serious consequences in the Lechang-Ruyuan section of the Beijing-Zhuhai Expressway(the longest expressway in China)that passes through the main part of the Nanling Mts.,where the road rises from 200m to more than 800m above sea level(ASL).For a major motorway in the mountainous areas of Nanling Mts.,two multidisciplinary integrated field observations were carried out,which measured visibility by the naked eyes,visibility by instrument,spectrum of fog- drops,liquid water content(LWC)of fog,tethered sounding,dual-parameter low-level sounding,turbulence diffusion within fog layers,aerosol spectra of size and composition,sampled fog water compositions,and sampled rainwater compositions.Typical cases were probed for their analyses of synoptics,micro- and macro-structures and microphysics.It is understood that heavy fogs take place with high frequency in the area and bring about serious consequences.Being typical advection and upslope fogs,they are in essence low-lying clouds appearing at high altitudes,which are closely related with the activity of South China frontal processes,especially the South China quasi-stationary fronts,and reflect on the role of local terrain as well.The heavy fogs are characteristic of long duration,extremely low visibility,well-organized lump- shaped structure,large-size fog-drops,moderate concentration,high LWC,and stronger turbulent diffusion within the fog layers than in fine sky.They differ much from radiation fogs,which are better documented in previous study in China.It is found that fog LWC is in significant anti-correlation with visibility so that large LWC is associated with small visual range.It is also noted that one of the reasons for the fluctuation of characteristic quantities of micro-structure such as the LWC of fog in the area is,in addition to the inhomogeneous structure of the fog itself,the effect of advection and inhomogeneous underlying surface; during the translation of fog with the ambient wind,irregular upslope and cross-over movement is another reason for the inhomogeneous structure and fluctuation of fog.The spectrum of the aerosol size displays itself as the power function of monotonous descent.The concentration of submicrometer particles is even higher.The high-concentration sulfate particles found in the aerosols of Nanling Mts.are actually good nuclei for condensation,which are favorable for the formation of fog.The presence of fog can help cleanse the trace compositions in the atmosphere so that fog droplets contain high levels of polluting elements.In the meantime,compared to cloud droplets,fog droplets are easier to be captured by the vertical surfaces of objects on the land surface,such as vegetation and buildings to constitute another kird of cleansing process. In vast stretches of forest like the Nanling Mts.,this kind of cleansing may be quite important.Studying the characteristic variation of fogs in the area realistically assists in setting up a forecast and warning system for local fogs and provides basic information for fog dispersal experiments. 相似文献
18.
南京冬季持续性强浓雾天气中三级分档雾水的理化特性分析 总被引：1，自引：0，他引：1
2013年12月7—9日南京出现持续性强浓雾天气过程。利用观测试验中获取的三级分档雾水和分粒径气溶胶的水溶性离子浓度,气溶胶数浓度谱、雾滴谱以及自动气象站获取的气象要素等资料,通过对比研究浓雾过程中4—16 μm（3级）、16—22 μm（2级）、>22 μm（1级）3个粒径范围雾滴（雾水）与分粒径气溶胶的微物理特征和化学特性,探讨不同粒径气溶胶粒子吸湿增长对雾滴的贡献以及气溶胶离子组分对不同尺度雾滴化学性质的影响。结果表明,在强浓雾天气中,能见度为50 m左右,短波辐射减弱形成稳定逆温层,有助于污染气溶胶的累积并吸湿增长向雾滴转化。雾滴的增加主要集中在小滴范围, 直径在0.5—1 μm的气溶胶粒子对其贡献最大。各粒径段气溶胶中阴离子NO3-和SO42-均表现出较高值,阳离子中Ca2+浓度最高。三档雾水中各阴、阳离子浓度均在4—16 μm小滴雾水中最高,16—22 μm中滴雾水和>22 μm大滴雾水的阴、阳离子浓度没有明显的高低之分。阳离子中Ca2+的浓度在第1级小滴雾水中最高,2级和3级雾水中NH4+的浓度最高,阴离子中NO3-和SO42-在各级雾水中浓度相差不大。雾水pH值2.7—6.9,呈酸性,小雾滴酸性更强。 相似文献
19.
Chunhong Zhou Xiaojing Shen Zirui Liu Yangmei Zhang Jinyuan Xin 《Acta Meteorologica Sinica》2018,32(2):265-278
A coupled aerosol–cloud model is essential for investigating the formation of haze and fog and the interaction of aerosols with clouds and precipitation. One of the key tasks of such a model is to produce correct mass and number size distributions of aerosols. In this paper, a parameterization scheme for aerosol size distribution in initial emission, which took into account the measured mass and number size distributions of aerosols, was developed in the GRAPES–CUACE [Global/Regional Assimilation and PrEdiction System–China Meteorological Administration (CMA) Unified Atmospheric Chemistry Environment model]—an online chemical weather forecast system that contains microphysical processes and emission, transport, and chemical conversion of sectional multi-component aerosols. In addition, the competitive mechanism between nucleation and condensation for secondary aerosol formation was improved, and the dry deposition was also modified to be in consistent with the real depositing length.Based on the above improvements, the GRAPES–CUACE simulations were verified against observational data during 1–31 January 2013, when a series of heavy regional haze–fog events occurred in eastern China. The results show that the aerosol number size distribution from the improved experiment was much closer to the observation, whereas in the old experiment the number concentration was higher in the nucleation mode and lower in the accumulation mode. Meanwhile, the errors in aerosol number size distribution as diagnosed by its sectional mass size distribution were also reduced. Moreover, simulations of organic carbon, sulfate, and other aerosol components were improved and the overestimation as well as underestimation of PM2.5 concentration in eastern China was significantly reduced, leading to increased correlation coefficient between simulated and observed PM2.5 by more than 70%. In the remote areas where bad simulation results were produced previously, the correlation coefficient grew from 0.35 to 0.61, and the mean mass concentration went up from 43% to 87.5% of the observed value. Thus, the simulation of particulate matters in these areas has been improved considerably. 相似文献
20.
高性能机载云粒子成像仪研制及应用 总被引：1，自引：0，他引：1
机载云粒子成像仪是目前直接观测云中粒子谱分布和形状特征的关键设备,在云物理结构探测、遥感反演验证、数值模式云物理过程改进和人工影响天气等领域具有十分重要的作用。因此,针对现有进口仪器性能和应用方面的不足,开发更高性能的云粒子探测仪器十分必要。通过2011年启动的国家重大科学仪器设备开发专项—机载云粒子谱仪与成像仪研制项目,研制出国产高性能机载云粒子测量系统。经过多年的研制和反复测试,解决和显著改进了激光光束均匀化、弱信号探测、多路并行处理及微粒消衍射等关键技术,从而提高了探测器像元的光功率均匀性和一致性,使光斑区域内平均光功率密度提高约3倍,从而改进了粒子成像能力。采用更高分辨率国产光电线阵探测器,测量响应时间明显缩短,对小云粒子的探测能力明显提高。研制的仪器通过一系列基础参数测试、系统优化、环境适应性实验和累计60多架次的飞行测试。对2018年11月5日进行的两架次对比探测结果的初步分析表明,新研制的云粒子成像仪对小粒子浓度的测量精度较进口仪器提高一个量级左右,测量数据起伏更小,稳定性更高,并且可正确获得更清晰可靠的云粒子形态特征。 相似文献