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1.
面对日益严峻的大气污染形势,针对卫星气溶胶光学厚度（AOD）资料在灰霾数值预报领域的合理有效利用问题,使用WRF-Chem（WRF coupled with Chemistry）大气化学模式以及GSI（Gridpoint Statistical Interpolation）三维变分同化系统,利用MODIS和FY-3A/MERSI AOD资料,对一次灰霾天气过程进行了同化预报试验。试验结果显示,同化卫星AOD资料有效改善了模式初始场,MODIS和MERSI同化试验分别在AOD分析场的中心强度和空间分布各具优势,且对PM2.5和PM10的后续预报改进明显;从统计分析上看,同化试验的预报效果整体上好于控制试验,同化试验中PM2.5和PM10预报值的平均值、中值、平均偏差、均方根误差等指标均明显优于控制试验,且MODIS和MERSI同化试验分别在PM2.5和PM10预报统计结果中体现出了优势;卫星AOD资料同化能明显降低污染事件的空报率和漏报率,提高预报的TS评分和ETS评分。不同卫星AOD资料的差异对分析场中AOD的分布和强度产生了相应影响,进而影响了模式的灰霾预报效果;本次试验中,MODIS和MERSI AOD同化试验分别在PM2.5和PM10预报的评分上表现更佳。结果表明,卫星AOD资料同化对数值预报产生了积极的效果。 相似文献
2.
准确获取气溶胶光学厚度对于气候变化研究和大气环境监测具有重要意义。通过波长插值和时空匹配方法,利用气溶胶自动观测站网（AERONET）观测的气溶胶光学厚度（AOD）对风云3A/中分辨率光谱成像仪（FY-3A/MERSI）、Terra（Aqua）/MODIS的C5.1（Collections 5.1）和C6（Collections 6）气溶胶光学厚度产品在中国区域的反演精度进行验证分析。结合一次发生在中国境内的沙尘天气与一次严重雾霾天气个例,分析上述卫星气溶胶光学厚度的分布特征。研究结果表明,（1）FY-3A/MERSI AOD的反演精度较高（R=0.887,RMSE=0.234）,其值低于AERONET的观测值（Bias=-0.293）。（2）在不同的下垫面下,各种卫星暗像元算法AOD产品反演精度有差异,植被覆盖情况越好,反演精度越高,而植被很少的地区,即亮地表甚至没有反演值。（3）MODIS C5.1深蓝算法产品能在亮地表地区反演AOD,但效果不佳。MODIS C6中的深蓝算法产品在不同下垫面的反演精度都很高（RMSE为0.096-0.127）。（4）在不同季节的对比中,各种卫星AOD产品在夏季的反演精度最差,而反演最好的季节各有不同。（5）在一次沙尘天气污染与一次严重雾霾天气个例中,中国西部与北部区域,MODIS C6深蓝算法AOD的监测效果优于其他算法AOD;MERSI AOD产品在此区域的分布不连续。总体而言,MODIS C6 AOD分布比MODIS C5.1产品连续,MODIS 3 km产品在相同区域的AOD值高于其他产品。以上结论可为卫星AOD产品在中国区域的使用提供参考。 相似文献
3.
The Moderate Resolution Imaging Spectroradiometer(MODIS) sensor onboard NASA's Aqua satellite has been collecting valuable data about the Earth system for more than 14 years, and one of the benefits of this is that it has made it possible to detect the long-term variation in aerosol loading across the globe. However, the long-term aerosol optical depth(AOD)trends derived from MODIS need careful validation and assessment, especially over land. Using AOD products with at least 70 months' worth of measurements collected during 2002–15 at 53 Aerosol Robotic Network(AERONET) sites over land,Mann–Kendall(MK) trends in AOD were derived and taken as the ground truth data for evaluating the corresponding results from MODIS onboard Aqua. The results showed that the AERONET AOD trends over all sites in Europe and North America, as well as most sites in Africa and Asia, can be reproduced by MODIS/Aqua. However, disagreement in AOD trends between MODIS and AERONET was found at a few sites in Australia and South America. The AOD trends calculated from AERONET instantaneous data at the MODIS overpass times were consistent with those from AERONET daily data, which suggests that the AOD trends derived from satellite measurements of 1–2 overpasses may be representative of those from daily measurements. 相似文献
4.
This study evaluates the spatial and temporal variation of the aerosol optical depth (AOD), the particle size characteristics (Ångström coefficients) and single scattering albedos during selected episodes over the Mediterranean area in 2006, based on independent observational datasets. We compare the satellite data of MODIS and MISR with those of the ground-based AERONET and in situ measurements. In general the yearly mean MODIS and MISR AODs as well as their temporal variation are in good agreement with AERONET. The highest AODs are caused by mineral dust outbreaks and the accumulation of anthropogenic aerosols during stagnant meteorological conditions. The comparison of MODIS with MISR aerosol optical properties for June corroborates that the AODs, Ångström coefficients and single scattering albedos agree well, and indicates the presence of high dust loads over the Mediterranean. Later in summer, however, MISR AOD is generally lower than MODIS, which is consistent with previous studies that show that MISR tends to underestimate and MODIS tends to overestimate AOD over land when compared to AERONET observations. Comparing MODIS Aqua Deep Blue with MISR for June over the Saharan desert reveals some differences in the location and the maxima of the AODs. Over the eastern Mediterranean highest dust loads occur during spring and autumn. Biomass burning activities around the Black Sea during July and August cause high AODs (e.g. by agricultural waste burning), and the particulate pollution is transported to the eastern Mediterranean and the Middle East by the prevailing northerly Etesian winds. 相似文献
5.
Hak-Sung Kim Yong-Seung Chung Joon-Tae Kim 《Asia-Pacific Journal of Atmospheric Sciences》2014,50(2):191-200
Long-term variations and trends of atmospheric aerosols in the East Asian region were analyzed by using aerosol optical depth (AOD or τ), and ångström exponent (AE or α) obtained from the Moderate Resolution Imaging Spectroradiometer (MODIS) from 2001 to 2010. The increased emission of anthropogenic fine aerosols in east China resulted in the high AOD in this region during summer. The steady increasing emission of anthropogenic fine aerosols caused an increasing trend of AOD in east China, and the large-scale transport of sandstorms and smoke plume caused by forest fires affected intense inter-annual variations of AOD in the East Asian region. While in the central part of South Korea, located in the lee side of the East Asian continent, AE tended to rise to a level higher than in east China, the ground-based mass concentrations continued to decline. A noticeable decrease of PM10 mass concentration in spring and winter in central Korea is most likely attributable to decreases in sandstorms in the source region of East Asia. However, the ratio of PM2.5 mass concentration to PM10 increases overall with a high level in summer. Aerosol types were classified into dust, smoke plume, and sulphate by using satellite data over Cheongwon in central Korea. The columnar AOD, with different aerosol types, was compared with the ground-based mass concentrations at Cheongwon, and the relatively high level of the correlations presented between PM2.5 and AOD produced in sulphate. Growth and increases of fine hygroscopic aerosols generated as gas-to-particle conversion particularly in summer contribute to increases of columnar AOD in the East Asian region. 相似文献
6.
气溶胶已是东亚地区最主要的大气污染物之一,其时空分布会受到东亚季风气候的影响。利用2000～2014年MODIS/AOD（Moderate-resolution Imaging Spectroradiometer/Aerosol Optical Depth）和NCEP月平均气象场再分析资料,本研究分析了东亚冬季风长期变化趋势、气溶胶年际变化规律,探讨了东亚冬季风强度变化对气溶胶分布的影响。基于MODIS/AOD,发现近10年东亚地区冬季AOD呈现上升趋势,最大值为2007年的0.44,高值区覆盖四川盆地、华北平原及长江中下游大部分地区。风场特征类冬季风指数分析表明,东亚冬季风存在明显的年际和年代际差异,近年出现逐渐减弱的趋势。强冬季风年,海陆气压差增大、东亚大槽加深增强,东亚地区偏北风异常,风场的增强将引导更多冷空气南下,从而给东亚大部分地区带来明显的降温天气;弱年相反。气象场差异引起气溶胶分布变化,强年较强的偏北风将气溶胶向南方输送,东亚地区AOD出现“北低南高”的空间分布;弱年偏北风较弱,导致气溶胶集中在华北平原一带,AOD出现“北高南低”的空间分布。 相似文献
7.
Soil dust aerosol is the largest contributor to aerosol mass concentrations in the troposphere and has considerable effects on air quality and climate. Arid and semi-arid areas of East Asia are one of the important dust source regions thus it is crucial to understand dust mobilization and accurately estimate dust emissions in East Asia. However, present dust models still contain large uncertainties with dust emissions that remain a significant contributor to the overall uncertainties in the model. In this study, we attempt to reduce these uncertainties by using an inverse modeling technique and obtain optimized dust emissions. We use Moderate Resolution Imaging Spectrometer (MODIS) aerosol optical depths (AODs) and groundbased mass concentrations of particles less than 10 μm in aerodynamic diameter (PM10) observations over East Asia in May 2007. The MODIS AODs are validated with AErosol RObotic NETwork (AERONET) AODs. The inversion uses the maximum a posteriori method and the GEOS-Chem chemical transport model (CTM) as a forward model. The model error is large over dust source regions including the Gobi Desert and Mongolia. We find that inverse modeling analyses from the MODIS and PM10 observations consistently result in decrease of dust emissions over Mongolia and the Gobi Desert. Whereas over the Taklamakan Desert and Manchuria, the inverse modeling analyses from both observations yield contrast results such as increase of dust sources using MODIS AODs, while decrease of those using PM10 observations. We discuss some limitations of both observations to obtain the optimized dust emissions and suggest several strategies for the improvement of dust emission estimates in the model. 相似文献
8.
开发AVHRR可见光通道反演陆地气溶胶光学厚度 (AOD) 的算法对于研究长时间序列AOD的变化有重要意义。AVHRR由于缺少2.1 μm通道而不能采用MODIS的暗背景算法,该文利用背景合成算法进行陆地AOD反演。背景合成算法是指假设一段时间内地表反射率变化不大且会出现相对清洁大气, 采用最小值合成即可得到地表反射率,再通过辐射传输模式6S制作的查算表查算得到AOD的反演结果。将此算法应用到2009年AVHRR中国部分陆地区域 (15°~45°N,75°~135°E) 得到AOD的时空分布,将反演结果与同期Aqua/MODIS的MOD04 AOD产品进行对比分析表明,华北和华东地区的反演效果较好,西北地区结果较差。以长江三角洲地区为例可知,AVHRR AOD产品与MODIS AOD产品以及AERONET观测的AOD相比相关系数基本在0.6以上,从时间变化规律来看,AVHRR AOD和MODIS AOD产品年变化趋势具有很好的一致性。该文为建立长时间序列AVHRR AOD数据集提供了一个较为可行的方法。 相似文献
9.
华东区域夏季行星边界层大气稳定度的气候特征及其与气溶胶的联系 总被引：2，自引：1，他引：1
利用1979-2008年夏季（6—8月）逐日NCEP／NACR再分析资料、MODIS卫星的气溶胶资料等,研究了华东区域夏季行星边界层大气稳定度的气候特征与年际变化,分析了大气稳定度和相应的加热场与气溶胶光学厚度（aerosol optical depth,AOD）的联系。结果表明：华东区域夏季行星边界层大气稳定度在空间上分布不均匀,时间上具有明显的年际变化。边界层中的非绝热加热率、大气稳定度及气溶胶光学厚度三者之间可能存在密切联系。利用经验正交函数分析了华东区域总体理查森数Rib的距平场,得到了边界层稳定度分布的3个主要模态,这3个模态所代表的边界层大气稳定度异常与夏季风环流异常密切相关,特别是P-J型遥相关波列和西太平洋副热带高压在中国东部大气边界层稳定度变化中可能起着非常重要的作用。 相似文献
10.
Modeling Study of the Impact of Heterogeneous Reactions on Dust Surfaces on Aerosol Optical Depth and Direct Radiative Forcing over East Asia in Springtime 
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下载免费PDF全文 The spatial distributions and interannual variations of aerosol concentrations,aerosol optical depth(AOD) ,aerosol direct radiative forcings,and their responses to heterogeneous reactions on dust surfaces over East Asia in March 2006-10 were investigated by utilizing a regional coupled climate-chemistry/aerosol model. Anthropogenic aerosol concentrations(inorganic+carbonaceous) were higher in March 2006 and 2008,whereas soil dust reached its highest levels in March 2006 and 2010,resulting in stronger aerosol radiative forcings in these periods.The domain and five-year(2006-10) monthly mean concentrations of anthropogenic and dust aerosols,AOD,and radiative forcings at the surface(SURF) and at the top of the atmosphere(TOA) in March were 2.4μg m-3,13.1μg m-3,0.18,-19.0 W m-2,and-7.4 W m-2,respectively.Heterogeneous reactions led to an increase of total inorganic aerosol concentration;however,the ambient inorganic aerosol concentration decreased,resulting in a smaller AOD and weaker aerosol radiative forcings.In March 2006 and 2010,the changes in ambient inorganic aerosols,AOD,and aerosol radiative forcings were more evident.In terms of the domain and five-year averages,the total inorganic aerosol concentrations increased by 13.7%(0.17μg m-3) due to heterogeneous reactions,but the ambient inorganic aerosol concentrations were reduced by 10.5%(0.13μg m-3) .As a result,the changes in AOD,SURF and TOA radiative forcings were estimated to be-3.9%(-0.007) ,-1.7%(0.34 W m-2) ,and-4.3%(0.34 W m-2) ,respectively,in March over East Asia. 相似文献
11.
Dust storm, which has a significant impact on regional air quality, is one of the most hazardous meteorological phenomena in the arid areas. Yazd province is one of the arid areas in Iran that is exposed to dust storms. In this study, two cases of dust storms of Yazd province are studied with the use of coupling numerical models and aerosol optical depth (AOD) from MODIS data. We investigated synoptic condition of such dust storms that were formed downstream of upper level through in the area by focusing on two storms, on May 24 and 25, 2014. For this purpose, a dynamic coupling of this case is done using WRF output the HYSPLIT model. This model was implemented to investigate the sources of the dust storms by calculating the back trajectories from the receptor sites. The trajectories indicated that the first and the second case storms occurred in the northeast and the south of Yazd respectively. These results also showed a good agreement with MODIS aerosol optical depth data and HYSPLIT back trajectories paths. 相似文献
12.
The air quality model system RAMS (Regional Atmospheric Modeling System)-CMAQ (Models-3 Community Multi-scale Air Quality) coupled with an aerosol optical/radiative module was applied to investigate the impact of different aerosol mixing states (i.e., externally mixed, half externally and half internally mixed, and internally mixed) on radiative forcing in East Asia. The simulation results show that the aerosol optical depth (AOD) generally increased when the aerosol mixing state changed from externally mixed to internally mixed, while the single scattering albedo (SSA) decreased. Therefore, the scattering and absorption properties of aerosols can be significantly affected by the change of aerosol mixing states. Comparison of simulated and observed SSAs at five AERONET (Aerosol Robotic Network) sites suggests that SSA could be better estimated by considering aerosol particles to be internally mixed. Model analysis indicates that the impact of aerosol mixing state upon aerosol direct radiative forcing (DRF) is complex. Generally, the cooling effect of aerosols over East Asia are enhanced in the northern part of East Asia (Northern China, Korean peninsula, and the surrounding area of Japan) and are reduced in the southern part of East Asia (Sichuan Basin and Southeast China) by internal mixing process, and the variation range can reach 5 W m－2. The analysis shows that the internal mixing between inorganic salt and dust is likely the main reason that the cooling effect strengthens. Conversely, the internal mixture of anthropogenic aerosols, including sulfate, nitrate, ammonium, black carbon, and organic carbon, could obviously weaken the cooling effect. 相似文献
13.
Kuwait was exposed to a severe dust storm on 19 March 2003, the eve of operation ??Iraqi Freedom??. Three days of dust events (19, 26, 27 March) were analyzed for their aerosol optical and physical properties using ground-based and satellite-retrieved measurements. Ground-based measurements of aerosol optical depth (or thickness; AOD or AOT) at 675?nm, ?? 657, ?ngstrom coefficient ?? 936/657, particulate matter of diameter 10???m or less, PM10 (??g/m3), and meteorological parameters were analyzed for March 2003. AOT exceeded 3 for the 3?days of interest and PM10 concentrations reached as high value as 2,457???g/m3 on 19 March dust storm day. Retrieved aerosol characteristics from space using Moderate Resolution Imaging Spectrometer (MODIS) on board Terra and Aqua satellite were examined against ground-based measurements. A strong correlation was found between ground-based measurements of ?? 675 and the Terra-MODIS retrieved AOD550. The synoptic of the dust storm were analyzed and source regions were identified using back trajectory analysis and Total Ozone Mapping Spectrometer Aerosol Index. 相似文献
14.
近10年东亚沙尘气溶胶时空分布与起尘通量的数值研究 总被引：2，自引：0，他引：2
利用一个耦合了沙尘模型的区域气候模式RegCM3和NCEP再分析资料,对近10年(2000-2009年)东亚地区沙尘气溶胶(直径≤20μm)时空分布特征和起尘通量进行了数值模拟。结果表明,(1)耦合模式能较好地模拟东亚地区沙尘气溶胶的时空分布特点。东亚地区沙尘气溶胶光学厚度、柱含量高值区主要位于塔克拉玛干沙漠和巴丹吉林沙漠。沙尘气溶胶柱含量的季节变化特征明显,春季最大,冬季次之,秋季最小。东亚地区110°E以东,沙尘主要以700hPa高度为中心向东传输。(2)东亚地区起沙源区主要位于塔克拉玛干沙漠、巴丹吉林沙漠、藏北沙漠化地区及蒙古国西南部,起沙强度存在明显的季节变化。2000-2009年东亚地区年平均起沙通量为1015.34mg.m-2.d-1,其中62.4%和2.3%分别通过干、湿过程重新沉降在东亚地区,其余35.3%被净释放进入大气或进行远距离传输。 相似文献
15.
利用MODIS卫星资料对中国中东部和印度次大陆气溶胶特性的分析 总被引：1，自引：1，他引：0
利用Terra和Aqua卫星上的MODIS探测反演气溶胶产品,比较分析了中国中东部和印度次大陆地区的气溶胶物理特性的异同。研究结果表明:中国中东部气溶胶类型以烟尘为主,印度次大陆地区东、西部分别以烟尘和沙尘为主。两地气溶胶光学厚度均有明显的年际变化,冬季低,夏季高。在夏季,两地烟尘所占比例都很大,且光学厚度也大,故两地污染状况都比较严重。总体来说,中国中东部地区污染程度要高于印度次大陆地区。 相似文献
16.
Aerosol optical depth (AOD) is a common indicator applied in monitoring aerosols in the atmosphere. The hilly landscape and rapid economic growth of the megacity Chongqing have facilitated increased aerosol concentration, and it is meaningful to accurately retrieve AOD over Chongqing. The HJ-1A/B satellite of China carries a sensor/camera called the Charge Coupled Device (CCD), the spatial resolution of which meets the requirement for retrieving high resolution AOD. In this paper, analysis of the AOD retrievals from different methods using the HJ-1 satellite data revealed the most suitable algorithm. Through comparison with the AOD product of Moderate Resolution Imaging Spectroradiometer (MODIS), the AOD retrieval results using enhanced vegetation index (EVI) to estimate dark pixels showed the highest correlation. The continental aerosol model was used to build a lookup table that was able to facilitate a good AOD retrieval for both city and rural areas. Finally, the algorithm that combined dark pixels, buffer areas, and the deep blue algorithm was found to be most suitable for AOD retrieval. The AOD retrieval results based on the HJ-1 data were consistent with MODIS products, and our algorithm yields reasonable results in most cases. The results were also compared with ground-based PM10 measurements synchronized with the overpass time of the HJ-1 satellite, and high correlation was found. The findings are relevant to other Chinese satellite data used for retrieving AOD on the same channels. 相似文献
17.
基于新耦合气溶胶气候模式FGOALS-f3-L模拟分析了2002-2011年青藏高原地区气溶胶时空分布特征.结果表明:青藏高原地区,沙尘,硫酸盐,碳质气溶胶(包括黑碳,有机碳和混合碳)地表质量浓度分别占比为53.6％,32.2％,14.2％;在拉萨站点,模拟的气溶胶地表质量浓度被低估,尤其是黑碳和有机碳气溶胶;模拟的气溶胶光学厚度(AOD)时空分布与卫星观测结果较为一致,均方根误差和偏差分别为0.081和0.036;由于模式中沙尘排放参数化的不确定性,模式对AOD的模拟效果在夏季和秋季优于春季. 相似文献
18.
19.
Seasonal variation features of aerosol optical depth (AOD) over East China and India in association with the Asian monsoon system are investigated, based on the latest AOD data derived from the Moderate Resolution Imaging Spectroradiometer (MODIS) aboard the Terra satellite, the NCEP Final (FNL) Operational Global Analysis data, the Climate Prediction Center (CPC) Merged Analysis of Precipitation (CMAP) data, and the NCEP/NCAR reanalysis data from March 2000 to February 2017. The results indicate that AOD in East China is significantly larger than that in India, especially in spring. The seasonal mean AOD in East China is high in both spring and summer but low in fall and winter. However, the AOD averaged over India is highest in summer and lower in spring, fall, and winter. Analysis reveals that AOD is more closely related to changes in surface wind speed in East China, while no obvious relation is found between precipitation and the AOD distribution on the seasonal timescale. As aerosols are mainly distributed in the atmospheric boundary layer (ABL), the stability of the ABL represented by Richardson number (Ri) is closely correlated with spatial distribution of AOD. The upper and lower tropospheric circulation patterns significantly differ between East China and India, resulting in different effects on the AOD. The effect of advection associated with lower tropospheric circulation on the AOD and the influence of convergence and divergence on the AOD distribution play different roles in maintaining the AOD in East China and India. These results improve our understanding of the mechanism responsible for and differences among the aerosol changes in East China and India. 相似文献
20.
Aerosol observational data at 8 ground-based observation sites in the Chinese Sun Hazemeter Network(CSHNET)were analyzed to characterize the optical properties of aerosol particles during the strong dust storm of 16-21 April 2005.The observational aerosol optical depth(AOD)increased significantly during this dust storm at sites in Beijing city(86%),Beijing forest(84%),Xianghe(13%),Shapotou(27%),Shenyang(47%),Shanghai(23%),and Jiaozhou Bay(24%).The API(air pollution index)in Beijing and Tianjin also had a similar rise during the dust storm,while the Angstrm exponent(α)declined evidently at sites in Beijing city(21%),Beijing forest(39%),Xianghe(19%),Ordos(77%),Shapotou(50%),Shanghai(12%),and Jiaozhou Bay(21%),respectively.Furthermore,The observational AOD andαdemonstrated contrary trends during all storm stages(pre-dust storm,dust storm,and post-dust storm),with the AOD indicating an obvious"Valley-Peak-Valley"pattern of variation,whileαdemonstrated a"Peak-Valley-Peak"pattern. In addition,the dust module in a regional climate model(RegCM3)simulated the dust storm occurrence and track accurately and RegCM3 was able to basically simulate the trends in AOD.The simulation results for the North China stations were the best,and the simulation for dust-source stations was on the high side,while the simulation was on the low side for coastal sites. 相似文献