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1.
运用完全在线耦合气溶胶—云—降水相互作用的WRF-Chem模式研究了污染气溶胶在2012年"7.21"极端降水事件中的作用,结果表明:在耦合人为排放源的情况下,通过与多种观测资料对比发现,WRF-Chem能较好地模拟此次极端降水事件中气象要素和气溶胶的发展趋势;不同水平的污染气溶胶在此次极端降水事件有不同的作用,相对于无污染气溶胶排放的情况,低排放水平的污染气溶胶对降水有激发作用,使降水增强,高排放水平污染气溶胶使降水更加的集中到降水中心,200 mm以上的降水区域增加了7倍以上,污染气溶胶对此次极端暴雨事件的形成有着重要作用;加入人为气溶胶的排放后,凝结核的增多、更加充沛的水汽条件及额外的凝结潜热的释放,使对流增强,降水粒子的含量增加是导致大暴雨更加强烈的原因。 相似文献
2.
周边地区对北京地面SO2影响的初步研究 总被引：15，自引：2，他引：15
采用Lagrangian传输、扩散、沉降模式计算了1994年9、10月份(非采暖期)、1995年1月和2000年1月(采暖期)北京地区SO2的变化规律,并分别计算了北京市不同类型的排放源以及周边地区污染源对平均地面SO2浓度的贡献.计算结果与实际观测资料对比表明,模式能够较好地模拟北京地区SO2的浓度量级和逐日变化趋势.北京地区地面SO2浓度受天气条件的影响较大.采暖期,北京当地排放源的影响相对较大;但在大气条件有利输送的背景下,来自周边地区污染排放源的影响不容忽视. 相似文献
3.
RMAPS_Chem V1.0系统是基于WRF_Chem模式建立的服务于华北区域雾霾等污染预报业务的模式系统,该研究着重针对系统中污染排放清单不确定性带来的SO2浓度预报偏差较大问题,采用EnKF源反演和误差统计订正相结合的方法对排放清单进行了改进,形成了一套优化后的华北区域SO2排放清单。通过输入初始清单和优化清单对2017年10月进行模拟,并与华北地区616个地面环境监测站观测值进行对比,结果表明:EnKF源反演结合误差统计订正的排放清单优化方法适用于SO2排放清单的改进,有效降低了清单系统性偏差,针对主要区域及重点城市的检验显示模拟结果接近观测值;排放清单优化后模拟误差显著降低,如河北南部、山东西部至北京一带模式预报均方根误差与归一化平均绝对误差明显下降,区域内站点模拟误差呈正态分布特征,误差分布范围、最大概率出现范围均明显变窄,且最大误差概率明显上升。 相似文献
4.
应用Models-3/CMAQ模式对华北地区一次强沙尘天气的研究初探 总被引：4，自引：1，他引：3
根据2002年在ACE-Asia和TRACE-P试验中获得的亚洲区域污染源排放资料,结合由MICAPS能见度观测资料估算而得的颗粒物排放资料,利用美国EPA最新发展的Models-3/CMAQ模式系统,模拟研究了2002年3月华北地区发生的一次强沙尘暴个例.结果表明,(1)模拟的各气态污染物的时空演变及相互关系与已有的观测结果基本一致.(2)颗粒污染物的模拟结果也反映了已有的观测事实,粗细颗粒物呈一致的先降后升日变化趋势;沙尘过程前期,颗粒物污染主要来源于近地面污染源;沙尘期间,颗粒物污染主要源自外界沙尘的高空输送,且粗颗粒物污染是此次过程的首要颗粒污染.(3)该模式系统可用于沙尘气溶胶研究的进一步开发与利用. 相似文献
5.
大气挥发性有机物（VOCs）是导致臭氧污染的关键前体物,是城市空气质量建模不可或缺的重要组成部分,但由于其非常复杂的构成和来源以及监测数据缺乏,目前对其模拟精度的了解仍非常有限。本文利用嵌套网格空气质量模式预报系统（NAQPMS）对珠江三角洲（简称珠三角）地区2017年9月21日至11月20日的VOCs开展了模拟试验,并利用光化学监测网8个地面站点的VOCs浓度监测数据,对模式模拟的关键VOCs组分进行了精度评估。结果发现,模式对强活性的甲苯、乙烯和二甲苯具有较高的模拟精度,模拟浓度偏差百分比为0.4%～26.6%,模拟能较好再现其日均浓度变化趋势和日变化的双峰特征。但是模式对化学反应活性强且与植物排放密切相关的异戊二烯具有很大的模拟偏差,偏差比近100%,无法再现其白天浓度高、夜间浓度低的观测日变化特征。通过分析发现,现有模拟系统主要考虑人为污染物排放而未考虑生物源排放,可能是导致这一模拟偏差的关键原因。同时,评估结果也表明模式在VOCs空间分布模拟上仍面临很大的不确定性。本文结果揭示了珠三角VOCs模拟面临的关键不确定性,表明融合VOCs观测数据来揭示并减小VOCs模拟的不确定性具有非常迫切的需求。 相似文献
6.
TRACE-P期间硫酸盐、硝酸盐和铵盐气溶胶的模拟研究 总被引：14，自引：7，他引：14
结合最新评估的东亚地区 1°× 1°污染源资料 ,利用由区域大气模式系统 (RAMS)和区域大气质量模式系统 (CMAQ)耦合的空气质量模式系统 ,对东亚地区 2 0 0 1年春季气溶胶的输送及其化学转化过程进行了研究。为了检验模式系统的模拟效果 ,我们将模拟的硫酸盐、硝酸盐和铵盐气溶胶的浓度与TRACE -P观测期间获取的观测值进行了比较。比较结果显示 ,模拟值与观测值具有相当好的一致性 ,模式很好地反映了气溶胶浓度的分布特征和变化规律 ,再现了许多观测到的重要特征。模拟结果表明 ,中国区域硫酸盐气溶胶浓度高值主要是人为排放的二氧化硫造成的 ,10 0°E以东的中国广大地区的硫酸盐气溶胶柱含量超过了 6mg·m- 2 ,最高值达到 2 4mg·m- 2 ,柱含量 >16mg·m- 2 的区域延伸到中国近海的广大海域。东亚地区的人类活动不仅使污染地区气溶胶柱含量显著增加 ,而且使近海无源区的广大海域的污染加重。本模式系统的建立为今后进一步研究区域大气污染物的变化机理提供了有效的手段。 相似文献
7.
京津冀地区一次雾霾过程的污染分布及来源分析 总被引：1，自引：0，他引：1
利用气象与化学模块在线耦合的模式WRF-Chem V3. 5(Weather Research and Forecasting Model coupled to Chemistry Version 3. 5)对2016年11月3-6日的一次京津冀污染过程展开了数值模拟,设计进行了包含人为排放源的实验,运用有效的模拟结果对过程进行分析。结果表明:大气稳定度指数能有效量化反映污染过程中的大气稳定状况,且K指数和TT指数相较其他两种指数的指示效果更为准确,是讨论雾霾发生发展原因的有力依据。本次污染高值中心有三个,分别为北京天津一带、河北东北部以及河北南部。PM_(2. 5)、PM_(10)以及SO_2污染物水平分布有明显日变化特征,CO和NO_2则变化不明显,污染从3日开始发展至6日结束,除NO_2外各项污染物都明显受到冷空气的影响,在6日浓度骤降。北京和天津地区的污染是主要来源于河北南部的工业和交通排放的外源型污染,而河北东北部和河北南部的污染则是主要受本地排放影响的内源型污染。污染物主要化学成分为CO,污染物颗粒PM_(2. 5)和PM_(10)量级相当且浓度差别不大,均对本次污染有较大贡献。 相似文献
8.
Parameterizing an agricultural production model for simulating nitrous oxide emissions in a wheat–maize system in the North China Plain 
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下载免费PDF全文 《大气和海洋科学快报》2016,(6)
农田土壤是大气氧化亚氮的一个重要排放源,农田氧化亚氮的排放同时受到气候环境和人为活动的复杂影响。本文基于中国华北平原的一个农田试验站的观测数据,对农业生产模拟器(APSIM)进行参数化,并检验该模型在不同时间尺度上模拟农田氧化亚氮排放的能力。结果表明,对消化系数(k_2)进行校正后,模型能够较好地模拟不同时间尺度和不同施肥处理下小麦-玉米系统的土壤氧化亚氮排放,但是对于一些较高的峰值排放模拟效果欠佳。 相似文献
9.
在北京城市气象环境的数值模拟中,人为热的设置是一个难点。人为热包括感热和潜热,人为潜热可以通过计算人为水汽排放获得。本文利用飞机观测资料对北京冬季人为水汽排放进行了定量估算。研究发现,在北京城区下风方向观测到相对周边区域更高的水汽摩尔分数,当观测到城市水汽过量信号时,水汽排放率的估计值在58～9539 kg/s,占城市大气边界层水汽总平流（背景+城市过量）的0.64%到13.12%。城市过量水汽排放的主要来源是天然气燃烧、水冷空调系统、城市交通等人为水汽的排放,中心城区和周边区域融雪率和蒸发率的差异可能也会有一定的贡献,但所占比例较小。 相似文献
10.
11.
T. Wang H. Guo D. R. Blake Y. H. Kwok I. J. Simpson Y. S. Li 《Journal of Atmospheric Chemistry》2005,52(3):295-317
We present a 16-month record of ozone (O3), carbon monoxide (CO), total reactive nitrogen (NOy), sulphur dioxide (SO2), methane (CH4), C2 – C8 non-methane hydrocarbons (NMHCs), C1 – C2 halocarbons, and dimethyl sulfide (DMS) measured at a southern China coastal site. The study aimed to establish/update seasonal
profiles of chemically active trace gases and pollution tracers in subtropical Asia and to characterize the composition of
the `background' atmosphere over the South China Sea (SCS) and of pollution outflow from the industrialized Pearl River Delta
(PRD) region and southern China. Most of the measured trace gases of anthropogenic origin exhibited a winter maximum and a
summer minimum, while O3 showed a maximum in autumn which is in contrast to the seasonal behavior of O3 in rural eastern China and in many mid-latitude remote locations in the western Pacific. The data were segregated into two
groups representing the SCS background air and the outflow of regional continental pollution (PRD plus southern China), based
on CO mixing ratios and meteorological conditions. NMHCs and halocarbon data were further analyzed to examine the relationships
between their variability and atmospheric lifetime and to elucidate the extent of atmospheric processing in the sampled air
parcels. The trace gas variability (S) versus lifetime (τ) relationship, defined by the power law, Slnx = Aτ− b, (where X is the trace gas mixing ratio) gives a fit parameter A of 1.39 and exponent b of 0.42 for SCS air, and A of 2.86 and b of 0.31 for the regional continental air masses. An examination of ln[n-butane]/ln[ethane] versus ln[propane]/ln[ethane] indicates that their relative abundance was dominated by mixing as opposed
to photochemistry in both SCS and regional outflow air masses. The very low ratios of ethyne/CO, propane/ethane and toluene/benzene
suggest that the SCS air mass has undergone intense atmospheric processing since these gases were released into the atmosphere.
Compared to the results from other polluted rural sites and from urban areas, the large values of these species in the outflow
of PRD/southern China suggest source(s) emitting higher levels of ethyne, benzene, and toluene, relative to light alkanes.
These chemical characteristics could be unique indicators of anthropogenic emissions from southern China. 相似文献
12.
Extensive ambient concentration and flux measurements have been performed in the heavily polluted region of Cubatão/Brazil. Substantial contribution of anthropogenic sources to the local reduced sulfur burden has been observed. As a result of this atmospheric sulfur burden average gas exchange between vegetated soils and the atmosphere shows net deposition. Based mainly on own field measurements a local budget for H2S, COS, and CS2 has been made up in order to calculate anthropogenic emissions. All major sources and sinks in the chosen atmospheric reservoir (24×20×1 km) have been taken into account. Due to the small reservoir size fluxes across its boundaries are dominant sources and sinks. The differences between outflux and influx therefore account for the unknown anthropogenic emissions which have been determined to be 80±10 (H2S), 66±15 (COS), and 29±6 Mmol year-1 (CS2). Other sources and sinks like natural emissions, chemical conversion, and dry deposition turned out to be of minor importance on a local scale. In fact, inside the investigated reservoir natural emissions were below 0.5% of anthropogenic emissions. Anthropogenic emissions of H2S, COS, and CS2 quantified in this work have been compared with global emission estimates for these compounds made by other authors. We conclude that global anthropogenic emissions of reduced sulfur compounds especially of COS and CS2 are currently under-estimated. 相似文献
13.
利用2005—2011年10次春季黄海海雾个例开展WRF模式参数化方案敏感性研究。结果表明:边界层方案对WRF模式雾区模拟结果起决定作用,而微物理方案影响较小,它主要影响海雾浓度和高度。边界层与微物理方案的最佳组合为YSU与Lin方案,最差为Mellor-Yamada与WSM5方案;Mellor-Yamada和QNSE方案模拟的近海面湍流过强,导致边界层过高,不利于海雾的发展与维持;而MYNN与YSU方案刻画的湍流强度与边界层高度合适,有利于海雾发展与维持。MYNN方案虽与YSU方案相当,但在大多数海雾个例中,后者明显优于前者,而在有些个例中却刚好相反。因此对于某一具体海雾个例而言,所用边界层方案仍需在它们之中选择最优者。这些信息可为黄海海雾WRF模式边界层与微物理方案的选择与改进提供参考。 相似文献
14.
Shanlan Li Mi-Kyung Park Chun Ok Jo Sunyoung Park 《Journal of Atmospheric Chemistry》2017,74(2):227-243
Methyl Chloride (CH3Cl) is a chlorine-containing trace gas in the atmosphere contributing significantly to stratospheric ozone depletion (Carpenter et al. 2014). In the global CH3Cl budget, the atmospheric CH3Cl emissions is predominantly maintained by natural sources, of which magnitudes have been relatively well-constrained. However, significant uncertainties still remain in the CH3Cl emission strengths from anthropogenic sources. High-frequency and high-precision in situ measurements of atmospheric CH3Cl concentrations obtained since 2008 at Gosan station (a remote background site in the East Asia) reveal significant pollution events superimposed on the seasonally varying regional background levels. Back trajectory statistics showed that air masses corresponding to the observed CH3Cl enhancement largely originated from regions of intensive industrial activities in China. Based on an inter-species correlation method, estimates of CH3Cl emissions from manufacturing industries including coal combustion, use of feedstocks, or process agents in chemical production for China (2008–2012) are 297 ± 71 Gg yr.?1 in 2008 to 480 ± 99 Gg yr.?1 in 2009, followed by a gradual decrease of about 25% between 2009 and 2012 (398 ± 92 Gg yr.?1 for 2010; 286 ± 68 Gg yr.?1 for 2011; 358 ± 92 Gg yr.?1 for 2012). The annual average of industrial CH3Cl emissions for 2008–2012 (363 ± 85 Gg yr.?1) in China is comparable to the known total global anthropogenic CH3Cl emissions accounting only for coal combustion and indoor biofuel use. This may suggest that unless emissions from the chemical industry are accounted for, global anthropogenic emissions of CH3Cl have been substantially underestimated. In particular, since industrial production and use of CH3Cl have not been regulated under the Montreal Protocol (MP) or its successor amendments, continuous monitoring of Chinese CH3Cl outflow is important to properly evaluate its anthropogenic emissions. 相似文献
15.
Wet deposition due to radiation fog is examined in this paper. The area where the reported measurements were performed, the Po Valley, northern Italy, is characterized by both a high fog occurrence during the fall-winter months and fog water solutions of high ionic concentration and acidity.Estimated wet deposition for NH
4
+
, NO
inf3
sup-
and SO
inf4
sup2-
ions due to fog droplet settling to the ground accounts for 13.2, 12.1 and 5.3 percent with respect to bulk precipitations over the same period: January–March and October–December (fog season).Fog deposition rates show that this process can be an important pathway of trace gases and particles loss from the air. First indicative results of fog removal efficiency with respect to air particulate matter are presented.Dry deposition parameters should be taken into account in evaluating the potential effect of fog droplet deposition on vegetation. 相似文献
16.
结合天气形势、高空风场、370m高塔、地面要素、激光云高仪、毫米波雷达等资料,对宁波北仑港区航道2018年2月15日海雾过程进行分析。结果表明,这是一次以锋前雾为主的海雾过程,在上暖下冷的锋面背景下,地面水汽充沛、风力温和,近地层逆温结构,都为海雾的形成和维持提供了有利条件。上下大气风向不一致,不利于垂直方向空气交换,有利于雾霾的产生。激光云高仪后向散射系数、颗粒物的消光系数及退偏振比,可以比较清晰地得出雾滴粒子的光学特性和过程演变趋势。随着海雾的生成、发展、消散,后向散射系数强度也呈增强、强、逐渐减弱的变化。雾天气现象下雾滴粒子小且轻,波动幅度比较大,某一高度粒子的傅里叶变换频率谱对应频率较高,高频所占比多数大于50%。 相似文献
17.
Examination of Microphysical Relationships and Corresponding Microphysical Processes in Warm Fogs 总被引：1，自引：0，他引：1
LU Chunsong LIU Yangang NIU Shengjie ZHAO Lijuan YU Huaying CHENG Muning 《Acta Meteorologica Sinica》2013,27(6):832-848
In this paper, the microphysical relationships of 8 dense fog events collected from a comprehensive fog observation campaign carried out at Pancheng（32.2 N, 118.7 E） in the Nanjing area, China in the winter of 2007 are investigated. Positive correlations are found among key microphysical properties（cloud droplet number concentration, droplet size, spectral standard deviation, and liquid water content） in each case, suggesting that the dominant processes in these fog events are likely droplet nucleation with subsequent condensational growth and/or droplet deactivation via complete evaporation of some droplets. The abrupt broadening of the fog droplet spectra indicates the occurrence of the collision-coalescence processes as well, although not dominating. The combined efects of the dominant processes and collision-coalescence on microphysical relationships are further analyzed by dividing the dataset according to visibility or autoconversion threshold in each case. The result shows that the specific relationships of number concentration to volume-mean radius and spectral standard deviation depend on the competition between the compensation of small droplets due to nucleation-condensation and the loss of small droplets due to collision-coalescence. Generally, positive correlations are found for diferent visibility or autoconversion threshold ranges in most cases, although negative correlations sometimes appear with lower visibility or larger autoconversion threshold. Therefore, the compensation of small droplets is generally stronger than the loss, which is likely related to the sufcient fog condensation nuclei in this polluted area. 相似文献
18.
Analysis of the Microphysical Structure of Heavy Fog Ｕsing a Droplet Spectrometer: A Case Study 总被引：15，自引：0，他引：15
The microphysical properties of a long-lasting heavy fog event are examined based on the results from a comprehensive field campaign conducted during the winter of 2006 at Pancheng (32.2°N, 118.7°E), Jiangsu Province, China. It is demonstrated that the key microphysical properties (liquid water content, fog droplet concentration, mean radius and standard deviation) exhibited positive correlations with one another in general, and that the 5-min-average maximum value of fog liquid water content was sometimes ... 相似文献
19.
Y. S. Chung Hak-Sung Kim Youngsin Chun 《Asia-Pacific Journal of Atmospheric Sciences》2014,50(3):345-354
Dust air pollution has been routinely monitored in central Korea for the last two decades. In 2009, there were eight typical episodes of significant dust loadings in the air: four were caused by dust storms from deserts in Mongolia and Northern China, while the remaining were typical cases of anthropogenic air pollution masses arriving from the Yellow Sea and East China. These natural dust loadings occurred with cool northwesterly airflows in the forward side of an intense anticyclone coming from Mongolia and Siberia. The mean concentrations of the four natural dustfall cases for TSP, PM10 and PM2.5 were 632, 480 and 100 μg m?3, respectively. In contrast, the anthropogenic dust-pollution episodes occurred with the warm westerly and southwesterly airflows in the rear side of an anticyclone. This produced a favorable atmospheric and chemical condition for the build-up of anthropogenic dust air pollution in the Yellow Sea. The mean concentrations of the four anthropogenic dust loadings for TSP, PM10 and PM2.5 were 224, 187 and 137 μg m?3, respectively. The contents of fine dust loadings of PM2.5 were comparatively high in the cases of anthropogenic air pollution. High atmospheric concentrations of fine particles in the atmosphere cause poor visibility and constitute a health hazard. Satellite observations clearly showed the movement of dust-pollution masses from Mongolia and Northern China and from the Yellow Sea and East China that caused these dust pollution episodes in Korea. 相似文献
20.
南京冬季浓雾的演变特征及爆发性增强研究 总被引：5，自引：2，他引：3
2007年12月18—19日,南京地区出现了一次持续20h的浓雾过程,其中能见度低于50m的强浓雾几乎占到整个雾过程的1／3。利用同期在南京市北郊的外场观测数据,结合NCEP再分析资料,分析了该次雾的演变过程、微物理结构及边界层特征,探讨了地面雾爆发性增强的成因。结果表明：本次雾在西南平流的增湿作用下触发生成;日出后,平流输送和地表蒸发提供了充足水汽来源,贴地层逆温因高空下沉增温而向上抬升且稳定存在,因此大雾得以维持;整个雾过程中雾滴数浓度、平均直径、含水量随时间的变化趋势基本一致,平均谱曲线均呈指数下降分布,雾滴集中在小滴端;两次地面雾爆发性增强均发生在夜间,其特征为各微物理参量明显增大,滴谱上抬拓宽;爆发性增强的原因是地表气温陡降、贴地层逆温增强及可充当雾滴凝结核的气溶胶大粒子数增多。 相似文献