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1.
The results from a one-dimensional photochemical model of the troposphere representative of summertime conditions at Northern Hemisphere mid-latitudes are presented. A parameterization of mixing processes within the planetary boundary layer (PBL) has been incorporated into the model for both the daytime convective PBL and the formation of the nocturnal PBL. One result of the parameterized PBL is that the concentrations of some trace species in the free troposphere are 20–30% higher than when mixing processes are described by a vertical eddy diffusion coefficient which is held constant with respect to height and time.The calculations indicate that the lifetime of the oxides of nitrogen (NO x =NO+NO2) against photochemical conversion to nitric acid (HNO3) during summertime conditions is on the order of 6 h. This lifetime is short enough to deplete most of the NO x in the PBL, resulting in the finding that other reactive nitrogen species (HNO3 and peroxyacetyl nitrate) are more abundant than NO x throughout the free troposphere, even though NO x is the most abundant reactive nitrogen species at the surface. The effects of the inclusion of anthropogenic nonmethane hydrocarbon (NMHC) chemistry are also discussed. The inclusion of NMHC chemistry has a pronounced effect on the photochemistry of tropospheric oxone and increases thein situ column production by more than 30%.  相似文献   

2.
Summary This paper investigates the influence of the planetary boundary-layer (PBL) parameterization and the vertical distribution of model layers on simulations of an Alpine foehn case that was observed during the Mesoscale Alpine Programme (MAP) in autumn 1999. The study is based on the PSU/NCAR MM5 modelling system and combines five different PBL schemes with three model layer settings, which mainly differ in the height above ground of the lowest model level (z 1). Specifically, z 1 takes values of about 7 m, 22 m and 36 m, and the experiments with z 1 = 7 m are set up such that the second model level is located at z = 36 m. To assess if the different model setups have a systematic impact on the model performance, the simulation results are compared against wind lidar, radiosonde and surface measurements gathered along the Austrian Wipp Valley. Moreover, the dependence of the simulated wind and temperature fields at a given height (36 m above ground) on z 1 is examined for several different regions. Our validation results show that at least over the Wipp Valley, the dependence of the model skill on z 1 tends to be larger and more systematic than the impact of the PBL scheme. The agreement of the simulated wind field with observations tends to benefit from moving the lowest model layer closer to the ground, which appears to be related to the dependence of lee-side flow separation on z 1. However, the simulated 2 m-temperatures are closest to observations for the intermediate z 1 of 22 m. This is mainly related to the fact that the simulated low-level temperatures decrease systematically with decreasing z 1 for all PBL schemes, turning a positive bias at z 1 = 36 m into a negative bias at z 1 = 7 m. The systematic z 1-dependence is also observed for the temperatures at a fixed height of 36 m, indicating a deficiency in the self-consistency of the model results that is not related to a specific PBL formulation. Possible reasons for this deficiency are discussed in the paper. On the other hand, a systematic z 1-dependence of the 36-m wind speed is encountered only for one out of the five PBL schemes. This turns out to be related to an unrealistic profile of the vertical mixing coefficient. Correspondence: Günther Z?ngl, Meteorologisches Institut der Universitat München, 80333 München, Germany  相似文献   

3.
It is shown that K-theory has to be modified for chemical systems that react with time scales similar to the turbulence time scale. In such systems, the value of the exchange coefficient depends not only on the turbulence parameters, but also on the chemical reaction rates. As an example, the NO-O3-NO2 chemical system is studied. Using second-moment equations, new flux-gradient relationships for the neutral atmospheric surface layer are obtained which depend on the time scale ratios of turbulence ( t ) and chemical reactions ( ch), i.e., reactive K-theory. Within the framework of this reactive K-theory, the flux of a chemical species is both a function of the concentration gradients of the three chemical species involved and of the ratio of the time scale of turbulence to the time scale of chemistry. In the special case of slow chemistry ( t ch) inert K-theory is applicable.The reactive exchange coefficients are implemented in a surface-layer model that calculates the flux and concentration profiles of the three chemical species. The results of the calculations of the effective exchange coefficients are different for reactive K-theory and inert K-theory; the differences are largest for nitric oxide, but smaller for ozone and nitrogen dioxide.  相似文献   

4.
To understand and estimate wind speed differences across the coastal zone, two models, one theoretical and another semi-empirical, have been developed and verified by available data sets. Assuming that: (1) mean horizontal motion exists across the coastal zone; and (2) the geostrophic wind does not change appreciably at the top of the planetary boundary layer (PBL), the equation of motion in the direction of the wind can be reduced so that 341-01, where U, H, and C D are wind speed, height of PBL, and drag coefficient over the sea and land, respectively. For practice, C D SEA has been modified from a formula with U LAND as the only input. H SEA may be estimated routinely from known H D LAND LAND and the temperature difference between land and sea, which can be provided by such means as remote sensing from meteorological satellites. For a given coast, Cmay be estimated also. This formula is recommended for weather forecasters. The semiempirical formula is based mainly on the power law wind distribution with height in the PBL. The formula states that 341-02. Simultaneous offshore and onshore wind measurements made at stations ranging from Somalia, near the equator, to the Gulf of Alaska indicated that values of a and b are 2.98 and 0.34 with a correlation coefficient of -0.95. For oceanographic applications, a simplified equation, i.e., 341-03, is also proposed.  相似文献   

5.
A simple time-dependent one-dimensional model of the planetary boundary layer (PBL) is described and used to examine the degree to which model design decisions affect model output variables. The model's sensitivity to changes in the environmental conditions is also explored. Averages of the surface fluxes, near-ground wind speeds and other PBL properties from 48 h simulations are compared to control runs. The model-calculated surface fluxes are most sensitive, in decreasing order of importance, to the vertical grid spacing, the form of closure between the surface temperature and the atmosphere, the use of vertical diffusivity smoothing, the choice of maximum time step and choice of turbulence closure scheme. These fluxes are relatively insensitive to mixing-length scaling or choice of implicit time step weighting factor. Sensitivity to changes in soil type exceeds any of the design criteria tested. The modeled fluxes are moderately sensitive to small variations in the horizontal pressure gradient, to unsteadiness in the geostrophic wind and to variations in surface roughness. They are relatively insensitive to uncertainties in local vertical velocities and small (25%) variations applied separately to soil thermal diffusivity or heat capacity. The sensitivity of the average PBL depth (Z i ) to model and environmental changes are similar to those of surface fluxes except thatZ i is more sensitive to changes in mixing length, albedo and imposed vertical velocity then are the surface fluxes.  相似文献   

6.
Mesoscale models using a non-local K-scheme for parameterization of boundary-layer processes require an estimate of the planetary boundary layer (PBL) height z i at all times. In this paper, two-dimensional sea-breeze experiments are carried out to evaluate three different formulations for the advective contribution in the z i prognostic equation of Deardorff (1974).Poor representation of the thermal internal boundary layer in the sea breeze is obtained when z i is advected by the wind at level z i . However, significantly better results are produced if the mean PBL wind is used for the advecting velocity, or if z i is determined simply by checking for the first sufficiently stable layer above the ground.A Lagrangian particle model is used to demonstrate the effect of each formulation on plume dispersion by the sea breeze.  相似文献   

7.
精细PBL模式及其诊断应用   总被引：2，自引：0，他引：2  
在已建立的一种三维非静力细网格Ｅ－ε湍能闭合的动力学框架基础上,作了一些改进的技术处理和试验,包括：（１）利用ＧＩＳ提供的地形资料,较精确地计算太阳辐射,进而诊断地面温度;（２）引进位势流概念,处理稳定层结条件下初始内插风场的风向变化;（３）引入动力学调整项Ｇ（αｏｂｓ－α）。在此基础上,就地理信息系统（ＧＩＳ）提供的一个 ６０ｋｍ×４８ｋｍ区域作了边界层结构和湍流特征的数值模拟试验,并与实测作了比较,讨论了精细ＰＢＬ模式的模拟效果,结果表明,新建的ＰＢＬ模式能较好地模拟表征出复杂下垫面地域的陡峭地形和不规则海岸线对局地风场和湍流场的动力和热力学作用。  相似文献   

8.
A simple mixed-layer model is developed to describe evaporation into a convective planetary boundary layer (PBL). The model comprises volume budget equations for temperature and humidity, equations to describe transport through the surface layer which is treated as part of the lower boundary, and equations to describe entrainment at the top of the PBL. The ground surface is modelled as a canopy resistance. The model was integrated with canopy resistance, surface-layer resistance and available energy, (R n – G), input as given functions of time, and the simulated PBL was allowed to grow into an atmosphere with known temperature and humidity profiles.Two variants of the mixed-layer model were tested using data from the KNMI tower site at Cabauw in the Netherlands. These variants differed only in the formulation of entrainment: one used a formulation developed by Driedonks (1982) while the other was a simpler formulation. Simulated evaporation agreed very well with observations irrespective of which entrainment formulation was used, despite discrepancies between simulated and observed PBL height growth which were sometimes quite large for the simpler formulation. Sensitivity analysis of the model confirms that good PBL height-growth predictions are not always a prerequisite for good evaporation predictions.  相似文献   

9.
The formation of longitudinal vortex rolls in the planetary boundary layer (PBL) is investigated by means of perturbation analysis. The method is the same as that used by previous authors who have investigated the instability of a laminar Ekman layer. To study the instability of the turbulent boundary layer of the atmosphere, vertical profiles are needed of the eddy viscosity and of the two components of the basic flow. These profiles have been obtained by a numerical PBL-model; they are universal for zz 0. (However, the stability equations are not completely universal, i.e., independent of the external parameters). For each thermal stratification, expressed by the internal stratification parameter , one has a set of three consistent profiles.The numerical solution of the stability equations gives the critical values and the perturbation growth rates as functions of thermal stratification and of the surface Rossby number Ro0. This is in contrast to the case of a laminar Ekman layer, where the instability depends on a Reynolds number only, which makes atmospheric applications difficult. The most unstable perturbations are found for Ro0 = 1 × 106 approximately, which is in the range of surface Rossby numbers observed in the atmosphere. However, considering vortex rolls oriented in the direction of the surface stress, the instability is found to be universal, i.e., independent of the external parameters combined in the surface Rossby number. With respect to thermal stratification, the results show that the instability of the perturbations increases with increasing static stability.  相似文献   

10.
The effects of two soil datasets on planetary boundary layer (PBL) height are analyzed, using model simulations. Simulations are performed with the MM5 weather prediction system over the Carpathian Basin, with 6?km horizontal resolution, investigating three summer days, two autumn, and one winter day of similar synoptic conditions. Two soil datasets include that of the United States Department of Agriculture, which is globally used, and a regional Hungarian called Hungarian unsaturated soil database. It is shown that some hydraulic parameter values between the two datasets can differ up to 5–50%. These differences resulted in 10% deviations in the space–time-averaged PBL height (averaged over Hungary and over 12?h in the daytime period). Over smaller areas, these relative deviations could reach 25%. Daytime course changes in the PBL height for reference run conditions were significant (p?<?0.01) in ≈70% of the grid points covering Hungary. Ensemble runs using different atmospheric parameterizations and soil moisture initialization setups are also performed to analyze the sensitivity under changed conditions. In these cases, the sensitivity test showed that irrespective of the radiation and PBL scheme, the effect of different soil datasets on PBL height is roughly the same. PBL height is also sensitive to field capacity (Θf) and wilting point (Θw) changes. Θf changes seem to be more important for loamy sand, while Θw changes for the clay soil textural class.  相似文献   

11.
Relative dispersion in a neutrally stratified planetary boundary layer (PBL) is investigated by means of large-eddy simulations (LES). Despite the small extension of the inertial range of scales in the simulated PBL, our Lagrangian statistics turn out to be compatible with the Richardson t3 law for the average of square particle separation, where t is time. This emerges from the application of non-standard methods of analysis through which a precise measure of the Richardson constant was also possible. Its value is estimated as C2 0.5, in close agreement with recent experiments and three-dimensional direct numerical simulations.  相似文献   

12.
Functional forms of the universal similarity functions A, B (for wind components parallel and normal to the surface stress), and C (for potential temperature difference) are determined based on the generalized theory of the resistance laws for the Planetary Boundary Layer (PBL). The similarity-profile functions for the surface layer are matched with the velocity and temperature-defect profiles that are assumed to have shapes modified by certain powers of nondimensional height z/h, where h is the PBL height. The powers of the outer-layer profile functions are determined, so that the functions become negligible in the surface layer. To close the temperature defect law, an assumption that the temperature gradient across the top of the PBL is continuous with the stratification of the overlying atmosphere is used. The result of this assumption is that nondimensional momentum and temperature profiles in the PBL can be described in terms of four basic ratios: (1) roughness ratio = /h (2) scale-height ratio =|f|h/u*, (3) ambient stratification parameter =h/*, and (4) stability parameter =h/L, where L is the Monin-Obukhov length, z0 is the surface roughness, is the upper-air stratification, u * is the friction velocity, and * is the temperature scale at the surface. For stable conditions, the scale-height ratio can be related to the atmospheric stability and the upperair stratification, and the generalized similarity and Rossby number similarity theories become identical. Under appropriate boundary conditions, function A is explicitly dependent on the stability parameter , while B is a function of scale-height ratio , which in turn depends on the stability. Function C is shown to be dependent on the stability and the upper-air stratification, due to the closure assumption used for the temperature profile.The suggested functional forms are compared with other empirical approximations by several authors. The general framework used to determine the functional forms needs to be tested against good boundary-layer measurements.  相似文献   

13.
Three online coupled chemical transport model simulations were analyzed for three summer months of 2015 in Poland. One of them was run with default emission inventory, the other two with NOx and VOC emissions reduced by 30%, respectively. Obtained ozone concentrations were evaluated with data from air quality measurement stations and ozone sensitivity to precursor emissions was estimated by ozone concentration differences between simulations and with the use of indicator ratios. They were calculated based on modeled mixing ratios of ozone, total reactive nitrogen and its components, nitric acid and hydrogen peroxide. The results show that the model overestimates ozone concentrations with the largest errors in the morning and evening, which is primarily related to the way vertical mixing is resolved by the model. Better model performance for ozone is achieved in rural than urban environment, as PBL and mixing mechanisms play more significant role in urban areas. Modeled ozone shows mixed sensitivity to precursor concentrations, similarly to other European regions, but indicator ratios have different values than are found in literature, particularly H2O2/HNO3 is larger than in southern Europe. However, indicator ratios often differ between locations and transition values need to be established individually for a given region.  相似文献   

14.
气溶胶辐射效应在华东地区一次雾霾过程中的作用   总被引：3，自引：1，他引：2  
张悦  樊曙先  李皓  康博识 《气象学报》2016,74(3):465-478
利用WRF/Chem(Weather Research and Forecasting Model coupled with Chemistry)模拟了2013年12月华东地区一次雾、霾事件气溶胶辐射反馈效应对气象场和大气质量的影响。通过3个不同气溶胶浓度设置的试验区分气溶胶浓度不同辐射效应的影响。比较不同试验得出,本次雾、霾过程中,不论是气溶胶直接、半直接辐射效应还是间接效应均使污染地区短波辐射减少、2 m气温下降、大气边界层高度降低,不利于水汽与污染物的扩散,空气污染进一步加重,雾结构进一步稳定,并使雾的持续时间延长,发展高度更高;对于化学场来说,气溶胶直接、半直接辐射效应使污染地区PM_(2.5)浓度增大、消光系数增大、氮氧化物浓度增大,臭氧浓度降低;间接辐射效应使PM_(2.5)浓度和消光系数进一步增大,氮氧化物、臭氧浓度降低。综上所述,气溶胶辐射效应能使大气污染加重,并利于雾的发生、发展。  相似文献   

15.
A mean meridional circulation model of the stratosphere, incorporating radiative heating and photochemistry of the oxygen‐hydrogen‐nitrogen atmosphere, is used to simulate the meridional distributions of O3, HOX, N2O,NOX, temperature and the three components of mean motion for the summer and winter seasons under steady‐state conditions. The results are generally in good agreement with the available observations in the normal stratosphere. The model has been applied to assess the effects of water vapour and nitrogen oxide perturbations resulting from aircraft emissions in the stratosphere. It is found that a fleet of 500 Boeing‐type sst's, flying at 20 km and 45°N in the summer hemisphere and inserting NOx at a rate of 1.8 megatons per year, has the effect of reducing the global total ozone by 14.7%. Similar calculations for 342 Concorde/TU‐114's, cruising at 17 km and injecting NOx at a rate of 0.35 megatons per year, show a global‐average total‐ozone reduction of 1.85%. Although water vapour is considered important, because of its ability to convert NO2 into HNO3, the direct effect on global‐average total‐ozone reduction resulting from the 100% increase in the stratospheric water content is less than 1%. The changes in the chemical structure (HO^NO^), temperature, and mean motions associated with the ozone reduction are also investigated in the case of the 1.8‐megaton‐per‐year NOX perturbation. It is shown that the reduced meridional temperature gradient in the middle and upper stratosphere resulting from the NOx perturbation leads to the weakening of the tropical easterly jet in the summer hemisphere and mid‐latitude westerlies in the winter season.

The sensitivity of the model solutions to an alternate choice of input parameters (diffusion coefficients and solar photodissociation data) is tested and the main deficiency of the model is pointed out.  相似文献   

16.
The equations of motions are solved for concentric circular flow in the planetary boundary layer (PBL) under the assumption of K = l 2|?v/?z| and gradient wind independent of radius r. The theoretical distribution of wind is obtained for r ≥ 300 km. Other parameters of the PBL are also calculated. Finally, equilibrium of the forces in the PBL is analyzed.  相似文献   

17.
In this study, we used satellite data (GOME and MOPITT) together with a global chemical-transport-model of atmosphere (MOZART-2) to characterize the chemical/aerosol composition over eastern China. We then estimated the effects of local emissions in China on the chemical budgets in other regions of the world. Likewise, we also investigated the effects of air pollution from other regions on the chemical budget over eastern China. The study shows that the column CO and NO x concentrations are also high in eastern China. The high CO and NO x concentrations produce modest levels of O3 concentrations during summer (about 40 to 50 ppbv) and very low O3 during winter (about 10 to 20 ppbv) in eastern China. The calculated NO2 column is fairly consistent from the GOME measurement. The calculated CO column is underestimated from the MOPITT measurement. One of the reasons of the underestimation of the predicted CO is due to a fact that the CO emissions were taken without considering the rapid increase of emissions from 1990 to 2000. The calculated surface O3 is consistent with the measured values, with strong seasonal variations. However, the measurement is very limited, and more measurements in eastern China will be needed. The column NO2 has a very strong seasonal variation in eastern China, with the highest concentrations during winter and the lowest concentrations during summer. The cause of this seasonal variability is mainly due to the seasonal changes in the chemical loss of NO x , which is very high in summer and very low during winter. The effects of the local emissions in China and long-range transport from other regions on the chemical distributions in eastern China are studied. The results show that NO x concentrations in eastern China are mostly caused by the local emissions in China, especially during the winter. The CO concentration over eastern China is from both the local emissions (30% to 40%) and the transport from other regions. Likewise, the CO emissions in China have an important effect on the other regions of the world, but the effect is limited in the northern hemisphere. The local emissions in China also have an important effect on surface O3 concentrations. During winter, the local emissions reduce the surface O3 concentrations by 30 to 50%. During summer, the local emissions produce about 50 to 70% of the O3 concentration in eastern China.  相似文献   

18.
    
A new Lagrangian—Eulerian coupling model system is developed to study regional air quality. The system consists of mesoscale dynamical meteorological model (MM), Monte—Carlo model (MCM), parameterized model on planetary boundary layer (PBL) turbulent statistics, dry and wet removal model, and Eulerian nonlinear chemical model (ENCM). The physical, chemical and biological processes on air pollutants are considered comprehensively. 3—D distribution laws tor acidic gaseous pollutants (SO2 and NOx) emitted by Thai Mae Moh Power Plant and the secondary pollutants are studied in detail. The results simulated by the coupling model system are in good agreement with observational concentration data. The authors wish to express their thanks to Prof. Zeng Q. C. for his support to this research and to Dr. Han Z. W. and Zhang M. G. for their help in programming and numerical calculation of IAP, Chinese Academy of Sciences. Thanks are also due to NSTD and EGAT in Thailand for supporting this research.  相似文献   

19.
The logarithmic + polynomial approximation is suggested for vertical profiles of velocity components in a planetary boundary layer (PBL) at neutral and stable stratification. The resistance law functions A and B are determined on the basis of this approximation, using integral relations derived from the momentum equations, the Monin-Obukhov asymptotic formula for the wind profile in a stably stratified near-surface layer and the known expressions for the PBL depth. This result gives a realistic and convenient method for calculating the surface friction velocity and direction and the total dissipation rate of mean flow kinetic energy in terms of geostrophic velocity, buoyancy flux at the surface, the roughness parameter and the Coriolis parameter. In the course of these derivations a review is given of current views on the main problems of the neutral and stable PBL.  相似文献   

20.
This study investigates the influences of urban land cover on the extreme rainfall event over the Zhengzhou city in central China on 20 July 2021 using the Weather Research and Forecasting model at a convection-permitting scale [1-km resolution in the innermost domain(d3)]. Two ensembles of simulation(CTRL, NURB), each consisting of 11 members with a multi-layer urban canopy model and various combinations of physics schemes, were conducted using different land cover scenarios:(i) the real urban ...  相似文献   

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