共查询到19条相似文献，搜索用时 125 毫秒
1.
双差分吸收激光雷达:-种能有效减小气溶胶对臭氧测量影响的方法 总被引：3，自引：1，他引：3
文中提出了一种新的激光雷达测量臭氧的方法：双差分吸收方法。理论分析和数值模拟表明这种方法可以有效减小气溶胶消光和后向散射对臭氧测量的影响，从而使激光雷达在气溶胶影响严重地区测量的臭氧精度比传统差分吸收激光雷达大大提高。利用（２８９，３１３；２７７．１，２９９．１ｎｍ）或（２６８．４，２８９；２７７．１，２９９．１ｎｍ）４波长进行双差分吸收可以用于对流层大气气溶胶含量丰富或分布不均匀地区臭氧的测量。利用（２９９．１，３４１．５；３０８，３５３ｎｍ）４波长进行双差分吸收可以对火山爆发后平流层臭氧进行较精确的测量。 相似文献
2.
通过WACCM-3模式中气溶胶光学厚度与卫星资料的对比发现,模式可以很好地再现全球气溶胶的主要分布特征,但在一些区域还存在数值上的差异。利用数值试验研究对流层气溶胶的直接气候效应对平流层气候的影响,结果表明:对流层气溶胶对平流层气候有明显影响,平流层化学过程在这一影响中起重要作用,而对流层气溶胶对平流层辐射的影响不是其直接气候效应对平流层影响的主要原因。其机制可能是对流层气溶胶改变对流层的辐射平衡,影响对流层的温度和大气环流,进而影响行星波的上传,使得平流层气候发生变化;影响区域主要位于高纬度和极地地区,南半球的变化比北半球大,温度变化最大达10 K,纬向风变化最大可达12 m/s,臭氧体积分数最多减少0.8×10-6。 相似文献
3.
利用TUV模式计算分析了银川光化辐射通量变化特征,探讨了云、气溶胶、臭氧柱浓度、NO_(2)柱浓度等因子对银川光化辐射通量的影响。结果表明:2019年7—9月银川月平均光化辐射通量分别为6.5E+16光子数·cm^(-2)·s^(-1)、5.6E+16光子数·cm^(-2)·s^(-1)和4.7E+16光子数·cm^(-2)·s^(-1),日最大值出现在13:00;波长小于325 nm时,光化辐射通量随波长增加缓慢上升,波长在325—480 nm之间时,光化辐射通量迅速升高,波长大于480 nm时,光化辐射通量随波长增加变化较小,此特征在中午前后较早晚表现更明显;云光学厚度和气溶胶光学厚度对光化辐射通量的衰减作用具有明显的“U”型日变化特征,比较而言,气溶胶光学厚度对光化辐射通量衰减作用的“U”型波形更为宽广;光化辐射通量衰减率对较低的云光学厚度的变化更敏感;光化辐射通量随气溶胶光学厚度增加而减小的变率要比随云光学厚度增加而减小的变率小;光化辐射通量对单次散射反照比大于0.6的强散射性气溶胶的变化更敏感,且气溶胶光学厚度越大,此特性整体表现越明显;波长指数对光化辐射通量的影响相对较小。 相似文献
4.
大气臭氧与气溶胶垂直分布的高空气球探测 总被引：17，自引：2，他引：17
本文给出了1993年9月12日利用高空科学气球在河北省香河地区探测到的大气臭氧和气溶胶的垂直分布。结果发现:(1) 大气臭氧的数密度在整个对流层较低(～10[12]mol/cm3)，并从地面到对流层顶略有下降；对流层顶以上开始快速增加，极值层高度在～24 km，其值为4.78×10[12]mol/cm3；臭氧分压有类似的分布特征，极值146×10[-4]Pa，位于同一高度；(2) 在平流层低层，臭氧分压有一个次极值62×10[-4]Pa，位于15～16 km；(3) 0～30 km大气气溶胶数密度呈现出三个峰值:143，8和1.1 个/cm[3]，分别位于近地面、5 km和21 km；（4）气溶胶的数密度谱在对流层为双模态；在平流层，次峰消失。同时，我们还与其他观测结果作了比较分析。 相似文献
5.
双偏振多普勒天气雷达差分反射率因子的测量误差 总被引：1，自引：1，他引：0
针对同时发射、同时接收体制双偏振多普勒天气雷达,论述了测量差分反射率因子时雷达应满足的基本要求,提出了测量差分反射率因子时能够引入误差的3类因素,即雷达测量基本要求不满足、接收机噪声和散射粒子相对运动引起的回波功率起伏、云雨目标对水平极化波和垂直极化波衰减的不同,并分别对影响差分反射率因子测量误差的各种因素及其影响程度,进行了深入研究和分析. 相似文献
6.
利用2019年1月1—7日AIRS观测的(80°—100°W,30°—45°N)范围内0—45 km高度的大气温度剖面数据,根据重力波的线性理论,分别采用垂直滑动窗口法、双滤波器法、单滤波器法对温度廓线数据进行处理,从中得到初始扰动剖面,再使用分离出来的对流层到平流层低层的背景温度和重力波扰动剖面计算重力波势能,最后根据提取结果比较三种方法的差异。结果表明:1) 采用垂直滑动窗口法提取的重力波势能对波长较小的波动有很好的反映,在对流层顶区域重力波势能异常偏大。2) 采用双滤波器法提取的重力波势能很好地反映各个波长的波动,更符合真实情况。3) 采用单滤波器法能够提取波长较大的重力波扰动,且扰动在对流层贡献更大;而采用双滤波器提取的重力波扰动分别在对流层顶和平流层贡献更大。 相似文献
7.
北京地区对流层中上部云和气溶胶的激光雷达探测 总被引：39，自引：8，他引：39
介绍了近年来研制的一台多波长激光雷达及其探测对流层高云和气溶胶的实验,并依据探测结果重点分析了北京2000年1月至4月对流层上部云和气溶胶在532 nm波长的消光系数分布特征.结果表明:从6 km至11 km的气溶胶光学厚度值在0.0152至0.0284之间变化,均值为0.0192.从6 km至11 km的云光学厚度值在0.014至0.23之间变化.观测到的单层高云的厚度最大为6 km.4月6日,近年来最强的一次沙尘暴袭击北京.4月7日北京地区无可见云,激光雷达探测结果表明,从4 km至10 km高度范围内,存在一层厚度约为6 km的气溶胶粒子层,消光系数峰值处于8 km附近,比晴天无云时的消光系数值约大一个数量级.估计这是一层沙尘气溶胶,系由远距离输送至北京形成的. 相似文献
8.
9.
介绍了以太阳散射光为光源的多轴差分吸收光谱技术（Multi-Axis Differential Optical Absorption Spectroscopy,简称MAX-DOAS）,以及MAX-DOAS仪器试验应用.试验中选取中午仪器测量的天顶散射光光谱为参考光谱即Fraunhofer参考光谱,并将测量光谱进行消噪、波长校准以及去除Fraunhofer结构处理.利用分子吸收光学厚度和Ring效应光学厚度对处理后的测量光谱进行最小二乘法拟合,反演出了大气NO2差分斜柱浓度（Differential Slant Column Densities,简称DSCD）.分析了天津武清NO2的差分斜柱浓度反演结果,用简单快捷的几何法将NO2差分斜柱浓度转化成对流层垂直柱浓度（Vertical Column Densities,简称VCD）.研究表明,MAX-DOAS可以有效地监测污染地区对流层NO2的垂直柱浓度. 相似文献
10.
东亚地区平流层、对流层交换对臭氧分布影响的模拟研究 总被引：13，自引：2，他引：11
首先将区域酸沉降模式(RADM)进行改造,加入平流层化学模块以替代对流层模块.然后用MM5单向耦合改造后的化学模式M-RADM,对东亚地区一次切断低压(2000年4月8～12日)引起的对流层顶折叠对上对流层、下平流层臭氧分布形式的影响进行模拟.结果显示:(1)随着高空槽的发展与切断,高空槽的底部及切断低压四周臭氧有显著增加.对流层顶折叠使高空臭氧向下输送,这种向下的输送可以到达对流层中部,对上对流层的臭氧影响最大.(2)模式可以成功地模拟出在北京地区探测到的臭氧垂直廓线的双峰结构.250 hPa处的臭氧分压比背景值增加近5倍.模拟表明改造后的区域化学模式M-RADM可以用于研究天气过程引起的对流层顶附近臭氧的演变情况.(3)上对流层臭氧分布形势的变化主要是由动力过程中的水平平流作用引起的,但是对流层顶附近臭氧的化学过程是不可忽略的. 相似文献
11.
In this paper the effects of aerosol on tropospheric ozone measurements by three-wavelength (266-289-308nm) dual differential absorption lidar (DIAL) and two-wavelength (266-289 nm and 266-308 nm) DIAL are simulated.By using the two kinds of DIAL.vertical profiles of ozone density from 2 to 3.6 km altitude range are measured.Both simulation and observation results show that the three-wavelength dual-DIAL method is more effective to reduce the effects of aerosol than the two-wavelength DIAL method.Therefore,accurate ozone density distributions can be retrieved by the three wavelength dual DIAL method. 相似文献
12.
胡顺星 naol.hfcas.ac.cn 胡欢陵 naol.hfcas.ac.cn 周军 naol.hfcas.ac.cn 吴永华 naol.hfcas.ac.cn 《Acta Meteorologica Sinica》2002,(2)
In this paper the effects of aerosol on tropospheric ozone measurements by three-wavelength(266-289-308nm) dual differential absorption lidar (DIAL) and two-wavelength (266-289 nmand 266-308 nm) DIAL are simulated.By using the two kinds of DIAL.vertical profiles of ozonedensity from 2 to 3.6 km altitude range are measured.Both simulation and observation resultsshow that the three-wavelength dual-DIAL method is more effective to reduce the effects of aerosolthan the two-wavelength DIAL method.Therefore,accurate ozone density distributions can beretrieved by the three wavelength dual DIAL method. 相似文献
13.
We describe here a DIAL lidar system for atmospheric ozone measurements atAberystwyth, Wales, together witha method for deriving a stratospheric ozone profile from a single laserwavelength. Lidar measurements are used todepict the passage of three mesoscale ozone disturbances in the troposphereand stratosphere. In the troposphere, twosmall fold-like structures are shown beneath and at the edge of streamers ofhigh potential vorticity in ECMWFanalyses. MST radar measurements at the same time show that one of these foldswas actively turbulent, causingmixing of stratospheric and tropospheric air. In the stratosphere, a streamerof low-latitude air drawn into a filamentby a breaking Rossby wave event was observed crossing the lidar site. 相似文献
14.
Fabien Gibert Irène Xuéref-Rémy Lilian Joly Martina Schmidt Juan Cuesta Kenneth J. Davis Michel Ramonet Pierre H. Flamant Bertrand Parvitte Virginie Zéninari 《Boundary-Layer Meteorology》2008,128(3):381-401
A network of remote and in-situ sensors was deployed in a Paris suburb in order to evaluate the mesoscale evolution of the
daily cycle of CO2 and related tracers in the atmospheric boundary layer (ABL) and its relation to ABL dynamics and nearby natural and anthropogenic
sources and sinks. A 2-μm heterodyne Doppler differential absorption lidar, which combines measurements of, (1) structure
of the atmosphere, (2) radial velocity, and (3) CO2 differential absorption was a particularly unique element of the observational array. We analyse the differences in the diurnal
cycle of CO, CO2, lidar reflectivity (a proxy for aerosol content) and H2O using the lidar, airborne measurements in the free troposphere and ground-based measurements made at two sites located few
kilometres apart. We demonstrate that vertical mixing dominates the early morning drawdown of CO and aerosol content trapped
in the former nocturnal layer but not the H2O and CO2 mixing ratio variations. Surface fluxes, vertical mixing and advection all contribute to the ABL CO2 mixing ratio decrease during the morning transition, with the relative importance depending on the rate and timing of ABL
rise. We also show evidence that when the ABL is stable, small-scale (0.1-km vertical and 1-km horizontal) gradients of CO2 and CO are large. The results illustrate the complexity of inferring surface fluxes of CO2 from atmospheric budgets in the stable boundary layer. 相似文献
15.
A state-of-the art Rayleigh and Mie backscattering lidar was set up at Gadanki (13.5N, 79.2E) in the Tropics in India. Using this system, regular observations of upper tropospheric clouds, aerosols at stratospheric heights and atmospheric temperatures in the range from 30 to 80 km were made. In this paper, the data collected during the period of 1998–99 were selected for systematic investigation and presentation. The Mie scattering lidar system is capable of measuring the degree of depolarization in the laser backscattering. Several tropical cirrus cloud structures have been identified with low to moderate ice content. Occasionally, thin sub-visible cirrus clouds in the vicinity of the tropical tropopause have also been detected. The aerosol measurements in the upper troposphere and lower stratosphere show low aerosol content with a vertical distribution up to 35 km altitude. Rayleigh-scattering lidar observations reveal that at the tropical site, temperature inversion occurs at mesospheric heights. Atmospheric waves have induced perturbations in the temperatures for several times at the upper stratospheric heights. A significant warming in the lower mesosphere associated with a consistent cooling in the upper stratospheric heights is observed particularly in the winter season during the events of sudden stratospheric warming (SSW). 相似文献
16.
The role of atmospheric ozone to protect the living organisms and vegetation from the harmful effects of ultraviolet irradiation is well known. Depletion of the ozone layer is a great threat to the human society. In this paper we have discussed the lethal effects of ozone depletion and have presented the ozone and UV-B scenarios from 1979 to 2005 at different Indian latitudes using satellite data. The erythemal UV irradiance data obtained from Nimbus-7 and Earth probe total ozone mapping spectrometer (TOMS) and the tropospheric and stratospheric ozone data obtained from the convective cloud differential (CCD) method have been used to study the variability of erythemal UV irradiance and the stratospheric and tropospheric column ozone, respectively, over a period from 1979 to 2005. The observed results along with the expected upper and lower tolerance limits for tropospheric and stratospheric ozone, respectively, for different Indian latitudes, which have been estimated statistically using monthly mean CCD ozone data from 1979 to 2005 have been discussed in detail. 相似文献
17.
J. Keder M. Střižík P. Berger A. Černý P. Engst I. Němcová 《Meteorology and Atmospheric Physics》2004,85(1-3):155-164
Summary Air pollution problem in the Czech Republic is very complex due to large number of factors as turbulent dispersion and chemical reactions concurring in the status of the PBL. For this 3D distribution of pollutants is a key information that cannot be given by conventional monitoring stations. Combined use of DIAL lidar and sodar can give access to such information. Case studies of air pollutants transport are presented using 3D concentration fields of NO2 and ozone measured by lidar and meteorological conditions monitored by Doppler Sodar. 相似文献
18.
X. Tie S. Chandra J. R. Ziemke C. Granier G. P. Brasseur 《Journal of Atmospheric Chemistry》2007,56(2):105-125
Satellite measurements of tropospheric column O3 and NO2 in eastern and southeastern Asia are analyzed to study the spatial and seasonal characteristics of pollution in these regions.
Tropospheric column O3 is derived from differential measurements of total column ozone from Total Ozone Mapping Spectrometer (TOMS), and stratospheric
column ozone from the Microwave Limb Sounder (MLS) instrument on the Upper Atmosphere Research Satellite (UARS). The tropospheric
column NO2 is measured by Global Ozone Monitoring Experiment (GOME). A global chemical and transport model (Model of Ozone and Related
Chemical Tracers, version 2; MOZART-2) is applied to analyze and interpret the satellite measurements. The study, which is
based on spring, summer, and fall months of 1997 shows generally good agreement between the model and satellite data with
respect to seasonal and spatial characteristics of O3 and NO2 fields. The analysis of the model results show that the industrial emission of NOx (NO + NO2) contributes about 50%–80% to tropospheric column NO2 in eastern Asia and about 20%–50% in southeastern Asia. The contribution of industrial emission of NOx to tropospheric column O3 ranges from 10% to 30% in eastern Asia. Biomass burning and lightning NOx emissions have a small effect on tropospheric O3 in central and eastern Asia, but they have a significant impact in southeastern Asia. The varying effects of NOx on tropospheric column ozone are attributed to differences in relative abundance of volatile organic compounds (VOCs) with
respect to total nitrogen in the two regions. 相似文献
19.
Climatic effects of air pollutants over china: A review 总被引：3，自引：0，他引：3
Tropospheric ozone(O3) and aerosols are major air pollutants in the atmosphere. They have also made significant contributions to radiative forcing of climate since preindustrial times. With its rapid economic development, concentrations of air pollutants are relatively high in China; hence, quantifying the role of air pollutants in China in regional climate change is especially important. This review summarizes existing knowledge with regard to impacts of air pollutants on climate change in China and defines critical gaps needed to reduce the associated uncertainties. Measured monthly, seasonal, and annual mean surface-layer concentrations of O3 and aerosols over China are compiled in this work, with the aim to show the magnitude of concentrations of O3 and aerosols over China and to provide datasets for evaluation of model results in future studies. Ground-based and satellite measurements of O3 column burden and aerosol optical properties, as well as model estimates of radiative forcing by tropospheric O3 and aerosols are summarized. We also review regional and global modeling studies that have investigated climate change driven by tropospheric O3and/or aerosols in China; the predicted sign and magnitude of the responses in temperature and precipitation to O3/aerosol forcings are presented. Based on this review, key priorities for future research on the climatic effects of air pollutants in China are highlighted. 相似文献