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1.
气溶胶对环境、气象和人体健康都有较大影响,这些影响与气溶胶理化特性(粒子尺度谱、化学组分、混合状态等)密切相关。为了深入研究气溶胶的环境和气候效应,发展了一套气溶胶在线综合观测系统。本文介绍了利用该系统在北京、上海、广州三个超大城市开展的综合观测实验结果。通过对比分析发现,广州气溶胶数浓度最高,其粒子尺度谱分布特征与北京特征相似,均以核模态为主,上海气溶胶数浓度则整体较低。对比三个超大城市的新粒子生成(New Particle Formation,NPF)特征发现,北京NPF的发生频率低于广州,主要由于北京地区大气中大粒径气溶胶更多,较高的碰并汇抑制了NPF的发生和发展。研究发现,观测期间北京和上海站点气溶胶的吸湿性强于广州,人为一次性排放气溶胶吸湿性较弱。气溶胶吸湿性日变化特征与人为活动、气溶胶老化程度密切相关。此外,三个超大城市中气溶胶光吸收系数的日变化特征存在明显差别,北京站点的气溶胶吸收系数呈现白天高、夜间低的特点,而广州站点气溶胶的吸收系数呈现相反的日变化趋势,这可能是由观测站周边的环境差异及大气边界层的变化特征差异造成的。  相似文献   

2.
As part of a series of studies on laser propagation for terrestrial free space optical (FSO) telecommunications or laser telecommunications, an experiment was conducted to determine the relationship between visibility in fog and optical attenuation (dB/km) at a laser wavelength of 1.55 μm. In the telecommunications industry, a semi-empirical equation, called the Kruse formula [Kruse, P.W., McGlauchlin, L., McQuistan, R.B., 1962. Elements of infrared technology: generation, transmission, and detection. John Wiley and Sons, New York] is typically used to calculate expected attenuation for a given meteorological visibility. The Kruse formula, however, was developed to relate meteorological visibility to optical attenuation over wavelengths from the visible to the near infrared (IR), and for dust and small particle aerosols with dimensions much smaller than the wavelength. Typically, suspended small aerosols have diameters that average about 0.1 μm while fog droplets have diameters that range upward from 2.5 μm with mean diameters that exceed 10 μm in some fogs. Therefore, application of the Kruse formula to attenuation in fog is not appropriate since fogs consist mainly of particles much larger than the laser wavelength. As part of the experiment, a transmissometer with an 85-m baseline and a dynamic range of 60 dB operated for thirteen months in an area prone to radiation fog. A commercial visibility sensor, similar to those used at airports, was located near the middle of the optical path of the transmissometer and operated over the same period. The largest attenuation measured at this site was just over 300 dB/km, corresponding to a visibility of 32 m. The key finding of the study is that the generally accepted Kruse formula relating visibility and optical attenuation may be too pessimistic at low visibilities, and actual attenuation values for a given visibility may be more than 20% lower than previously thought. At visibilities exceeding about 650 m, the Kruse formula gives a good estimate of optical attenuation.  相似文献   

3.
基于1980~2014年上甸子国家级地面气象台站人工观测的大气水平能见度数据和大气成分站资料,采用Mann-Kendall趋势分析及突变检验法对大气能见度进行分析,并结合气象和污染要素进行相关性检验,以了解华北背景地区大气能见度的变化趋势及其影响因素。结果表明:上甸子地区年均能见度呈下降趋势,能见度最大和最小变率出现在夏季和春季,分别为3.4 km（10 a）-1和1.7 km（10 a）-1;冬季能见度（38.1 km）最高,秋季（36.2 km）次之,春季（32.8 km）和夏季（31.4 km）较低;突变分析表明上甸子地区的年均能见度未出现明显突变。能见度受各类气象因子的综合影响。根据Person相关和偏相关的统计结果,能见度与相对湿度和风速均呈明显负相关;与气压呈明显的正相关;而与气温的相关系数时正时负,表明气温对能见度的影响具有两面性。能见度下降的主要原因为大气污染,能见度随着大气细颗粒物增加呈幂指数降低（决定系数R2=0.98,显著性水平p < 0.01）;能见度为10 km时对应的细颗粒物（PM2.5）的边界浓度为74 μg/m3;在现行的国家环境空气质量标准二级标准（75μg/m3）下,可以使华北背景地区保持较高的大气能见度（≥ 10 km）。  相似文献   

4.
Trends in fog frequencies in the Los Angeles Basin   总被引：1，自引：0，他引：1  
Data from throughout the Los Angeles area were examined to determine the horizontal distribution of dense fog (visibility < 400 m) in the region and trends over time. The relationship between the occurrence of dense fog to the phase of two atmosphere–ocean cycles: the Pacific Decadal Oscillation (PDO) measured by the PDO Index and the Southern Oscillation measured by the Southern Oscillation Index (SOI) was investigated. In addition, the influence of the urban heat island and the amount of suspended particulate matter were assessed. For the three stations that had 22 or more years of data, we examined trends and the relation to atmosphere–ocean cycles. Results show a decrease in the occurrence of very low visibilities (< 400 m) at the stations in close proximity to the Pacific Ocean, Los Angeles International Airport (LAX) and Long Beach International Airport (LGB). Occurrence of the frequency of low visibilities at these two locations was also highly correlated with the phase of the PDO. Only a weak, non-statistically significant relationship was seen with the SOI. At Burbank, a reporting station about 30 km from the ocean, no trends were noted, and there was no evidence of a correlation with either the PDO Index or the SOI. In the Los Angeles Central Business District (CBD) when comparing dense fog occurrence in the early 1960s to a similar period in the early 2000s we saw a decrease in dense fog from a mean of 10 h per year to a mean of 3 h per year. Also contributing to the decrease was decreasing particulate pollution and increased urban warming. A downward trend in particulate concentrations coupled with an upward trend in urban temperatures were associated with a decrease in dense fog occurrence at both LAX and LGB. These trends were evident for the period 1966–1997, but appear to have ended by the late 1990s.  相似文献   

5.
A data set acquired by eight particle-dedicated instruments set up on the SIRTA (Site Instrumental de Recherche par Télédétection Atmosphérique, which is French for Instrumented Site for Atmospheric Remote Sensing Research) during the ParisFog field campaign are exploited to document microphysical properties of particles contributing to extinction of visible radiation in variable situations. The study focuses on a 48-hour period when atmospheric conditions are highly variable: relative humidity changes between 50 and 100%, visibility ranges between 65 and 35 000 m, the site is either downwind the Paris area either under maritime influence. A dense and homogeneous fog formed during the night by radiative cooling. In 6 h, visibility decreased down from 30 000 m in the clear-sky regime to 65 m within the fog, because of advected urban pollution (factor 3 to 4 in visibility reduction), aerosol hydration (factor 20) and aerosol activation (factor 6). Computations of aerosol optical properties, based on Mie theory, show that extinction in clear-sky regime is due equally to the ultrafine modes and to the accumulation mode. Extinction by haze is due to hydrated aerosol particles distributed in the accumulation mode, defined by a geometric mean diameter of 0.6 μm and a geometric standard deviation of 1.4. These hydrated aerosol particles still contribute by 20 ± 10% to extinction in the fog. The complementary extinction is due to fog droplets distributed around the geometric mean diameter of 3.2 μm with a geometric standard deviation of 1.5 during the first fog development stage. The study also shows that the experimental set-up could not count all fog droplets during the second and third fog development stages.  相似文献   

6.
Shanghai is the largest industrial and commercial city in China, and its air quality has been deteriorating for several decades. However, there are scarce researches on the level and seasonal variation of fine particle (PM2.5) as well as the carbonaceous fractions when compared with other cities in China and around the world. In the present paper, abundance and seasonal characteristics of PM2.5, organic carbon (OC) and elemental carbon (EC) were studied at urban and suburban sites in Shanghai during four season-representative months in 2005–2006 year. PM2.5 samples were collected with high-vol samplers and analyzed for OC and EC using thermal-optical transmittance (TOT) protocol. Results showed that the annual average PM2.5 concentrations were 90.3–95.5 μg/m3 at both sites, while OC and EC were 14.7–17.4 μg/m3 and 2.8–3.0 μg/m3, respectively, with the OC/EC ratios of 5.0–5.6. The carbonaceous levels ranked by the order of Beijing > Guangzhou > Shanghai > Hong Kong. The carbonaceous aerosol accounted for  30% of the PM2.5 mass. On seasonal average, the highest OC and EC levels occurred during fall, and they were higher than the values in summer by a factor of 2. Strong correlations (r = 0.79–0.93) between OC and EC were found in the four seasons. Average level of secondary organic carbon (SOC) was 5.7–7.2 μg/m3, accounting for  30% of the total OC. Strong seasonal variation was observed for SOC with the highest value during fall, which was about two times the annual average.  相似文献   

7.
选用2007年1月8—30日期间8个无云天的激光雷达资料进行分析。基于Fernald方法反演得到气溶胶消光系数廓线,结合无线电探空资料分析了边界层内气溶胶时空分布,并将反演的激光雷达最低观测高度处(180 m)的气溶胶消光系数与地面PM10、能见度资料进行对比分析。结果表明：冬季大连市区气溶胶主要分布在2 km以下区域,早晨和夜间在0.5 km以下区域经常存在一个气溶胶层;气溶胶消光系数廓线与探空资料较吻合;反演激光雷达最低观测高度处(180 m)的气溶胶消光系数与地面的PM10浓度呈正相关,与能见度呈负相关,相关性较好。  相似文献   

8.
天津夏季大气消光性质的研究   总被引：2，自引：0，他引：2  
利用2010年夏季天津城市边界层观测站颗粒物、黑碳气溶胶、氮氧化物(NOX)浓度、地面能见度和气象梯度观测资料,分析了天津夏季大气消光特性及低能见度事件产生的原因。结果表明,天津夏季主要污染物为PM10和PM2.5,大气气溶胶消光系数为529.06M.m-1,其中,吸收系数为50.17M.m-1,散射系数为478.89M.m-1,气体吸收系数为7.74M.m-1,气溶胶单次散射反射率为0.87。天津夏季边界层大气状态有近一半的时间为中性或偏稳定层结,当出现中性或偏稳定层结大气时则有接近一半的情况出现低能见度事件(能见度<5km),影响人们的日常生活。  相似文献   

9.
Measurements from July 4 to July 8, 2005 by a high resolution visible radiometer, a Raman lidar, a ground particulate matter sampler, and ground meteorological sensors have been combined in synergy to infer the intrusion over south-east Italy, of air masses from north-west Sahara, the Atlantic Ocean, and the continental Europe. It is shown that backscatter coefficient, depolarization-ratio, and lidar ratio vertical profiles represent the best tools to detect the intrusion of long range transported air masses and to monitor their effects on the vertical distribution of aerosol optical and microphysical properties. High resolution radiometers are instead important tools to monitor changes on columnar aerosol properties and size distributions.Backscatter coefficient, depolarization-ratio, and lidar ratio vertical profiles have revealed that aerosol optical and microphysical properties significantly changed with time and space during African dust outbreaks: the intrusion of dust particles that at first occurred above 2 km of altitude extending up to 6 km, affected the all aerosol load down to ground within few hours. Aerosol size distributions showed during dust events a clear bimodality with an accumulation mode maximum at 0.24 µm and a coarse mode maximum at 0.94 μm. Conversely, we have found that during the advection of air masses from the Atlantic and continental Europe, aerosol particles were mainly located below 2 km, their optical and microphysical properties were affected by smaller changes in time and space, and were characterized by depolarization ratios rather close to those due to a pure molecular atmosphere. In this case bimodal size distributions with an accumulation mode showing two sub-modes at 0.16 μm and 0.24 μm, respectively and a coarse mode centred at 0.94 μm have also been observed.  相似文献   

10.
This study analyzes and compares aerosol properties and meteorological conditions during two air pollution episodes in 19–22 (E1) and 25–26 (E2) December 2016 in Northeast China. The visibility, particulate matter (PM) mass concentration, and surface meteorological observations were examined, together with the planetary boundary layer (PBL) properties and vertical profiles of aerosol extinction coefficient and volume depolarization ratio that were measured by a ground-based lidar in Shenyang of Liaoning Province, China during December 2016–January 2017. Results suggest that the low PBL height led to poor pollution dilution in E1, while the high PBL accompanied by low visibility in E2 might have been due to cross-regional and vertical air transmission. The PM mass concentration decreased as the PBL height increased in E1 while these two variables were positively correlated in E2. The enhanced winds in E2 diffused the pollutants and contributed largely to the aerosol transport. Strong temperature inversion in E1 resulted in increased PM2.5 and PM10 concentrations, and the winds in E2 favoured the southwesterly transport of aerosols from the North China Plain into the region surrounding Shenyang. The large extinction coefficient was partially attributed to the local pollution under the low PBL with high ground-surface PM mass concentrations in E1, whereas the cross-regional transport of aerosols within a high PBL and the low PM mass concentration near the ground in E2 were associated with severe aerosol extinction at high altitudes. These results may facilitate better understanding of the vertical distribution of aerosol properties during winter pollution events in Northeast China.  相似文献   

11.
利用MODIS光学厚度遥感产品研究北京及周边地区的大气污染   总被引：53，自引：2，他引：53  
对2001年在北京地区利用太阳光度计观测的气溶胶光学厚度和NASA发布的MODIS气溶胶产品进行了比较,验证了这一卫星遥感产品的可靠性;比较了2001年MODIS气溶胶光学厚度(AOD)产品和由空气污染指数(API)计算的每日平均可吸入颗粒物(PM10)浓度,得到了比较高的相关系数,证实该气溶胶产品可用于污染分析.将北京地区AOD与气象能见度观测资料进行比较,得到了不同季节的气溶胶"标高".利用统计的不同季节的气溶胶标高,从光学厚度的季节分布得到了能见度(能见距离)的季节分布.气溶胶光学厚度图像的个例分析表明,除局地排放外,周边区域(主要为西南和南向)的输送对北京市区的空气污染贡献份额较大.卫星遥感气溶胶可以比较直观地再现污染物的区域分布和输送,不仅为研究全球气候变化也为研究区域环境的空气质量提供了一种有效手段.  相似文献   

12.
南京大气能见度变化规律及影响因子分析   总被引：7，自引：1，他引：6       下载免费PDF全文
利用累积百分率法、Ridit中值分析法、"非常好"能见度出现频率法以及平均能见度年际和季节变化法,对1980—2005年南京大气能见度年际变化趋势进行分析,发现1980—1984年能见度呈上升趋势,1985年以后则在波动中呈明显下降趋势。26 a中,日均大气能见度最小值为0.55 km,最大值为29.25 km,平均值为8.59 km。大气能见度具有明显的日变化和季节变化特征,一日之中,14时最好,08时最差;一年之中,冬季能见度最低,夏季最高。能见度与相对湿度呈负相关,与风速呈正相关,与温度和气压的相关性相对较小。PM10是影响南京地区大气能见度的首要污染物,通过对能见度与PM10平均质量浓度进行曲线拟合发现,二者呈负相关,复相关系数在秋季最高,夏季最低。由统计预报方程可知,空气污染和气象条件协同作用对能见度的影响在春季、秋季、冬季较为明显,夏季则相对较差。  相似文献   

13.
利用中国太阳分光观测网的观测资料结合MODIS(中分辨率成像光谱仪)的气溶胶产品分析了北京、兰州、上海3个典型区域城市的气溶胶光学特性。结果表明:北京AOD(气溶胶光学厚度)年平均为0.41±0.35,春夏高,秋冬低,Angstrm波长指数α年平均为1.40±0.85表现为细模态粒子,MODIS的光学厚度为0.52±0.39与地面观测相关系数为0.91,存在系统性高估;兰州AOD年平均为0.55±0.21,夏季最低,秋冬较高,α年平均为0.95±0.20表现为粗模态粒子,MODIS光学厚度为0.43±0.21与地面观测相关系数仅为0.07,存在系统性低估;上海AOD年平均为0.55±0.21,无明显季节变化,α平均为1.03±0.25,MODIS光学厚度为0.74±0.30与地面观测相关系数为0.75,存在系统性高估。城市地理位置和复杂地表等原因造成反照率的不确定,MODIS气溶胶产品在这3个城市的反演效果仍有很大提升空间。  相似文献   

14.
辽宁旅顺与山东龙口能见度对比分析   总被引：1，自引：0，他引：1       下载免费PDF全文
利用2002-2011年渤海海峡两岸辽宁旅顺和山东龙口地面气象站能见度逐时观测资料,采用等级分析法,统计分析两地平均和分级能见度的年、月、日变化特征。结果表明：位于渤海北岸旅顺的年均能见度值高于渤海南岸的龙口,近10 a两地年均能见度均呈下降趋势,龙口年均能见度降低速度高于旅顺;各级能见度的时间百分比旅顺年际变化较大,而龙口相对稳定;一年中两地10月份月均能见度最高,旅顺月均最低能见度出现在7月,龙口出现在6月,两地能见度日变化特征基本一致,呈一波峰一波谷形势。通过分析天气现象及相关气象因子发现,两地出现低能见度（0-1 km）时,风场、温湿场特征均存在明显区域性差异。  相似文献   

15.
北京地区对流层中上部云和气溶胶的激光雷达探测   总被引：39，自引：8，他引：39  
介绍了近年来研制的一台多波长激光雷达及其探测对流层高云和气溶胶的实验,并依据探测结果重点分析了北京2000年1月至4月对流层上部云和气溶胶在532 nm波长的消光系数分布特征.结果表明:从6 km至11 km的气溶胶光学厚度值在0.0152至0.0284之间变化,均值为0.0192.从6 km至11 km的云光学厚度值在0.014至0.23之间变化.观测到的单层高云的厚度最大为6 km.4月6日,近年来最强的一次沙尘暴袭击北京.4月7日北京地区无可见云,激光雷达探测结果表明,从4 km至10 km高度范围内,存在一层厚度约为6 km的气溶胶粒子层,消光系数峰值处于8 km附近,比晴天无云时的消光系数值约大一个数量级.估计这是一层沙尘气溶胶,系由远距离输送至北京形成的.  相似文献   

16.
能见度可以直观反映空气污染程度,通过卫星反演获取能见度可以实现大面积同步观测,弥补地面观测在此方面的不足。基于安徽省池州市2015年Terra/MODIS的气溶胶产品(AOD)和池州市一区三县4个国家观测站的能见度观测资料,分析研究MODIS气溶胶产品与能见度的关系。通过拟合池州市四季气溶胶标高,建立不同季节能见度回归模型,并利用标高数据和AOD的季节分布,反演出池州能见度的季节变化,研究了近地层大气气溶胶与地面能见度的关系,最终获取了池州市2015年四季能见度时空分布并对其特征进行分析。结果表明:池州市夏季气溶胶标高最高,冬季的最低;能见度模型估算值与观测值整体较为一致,季节平均值相对误差为18. 15%;池州市2015年四季平均能见度为13. 8 km,整体呈从东南向西北逐渐减小的趋势,空间分布不均;季节平均能见度夏季最高,为19. 3 km,冬季最低,为9. 9 km,其中石台县各季能见度均明显好于其他地区的,且四季变化小而平稳;月平均能见度7月的最好,2月、5月和9月的较差;经济社会发展状况、生态环境和气候状况是影响池州市能见度分布时空变化的主要因素。  相似文献   

17.
Aerosol depolarization ratio and aerosol optical depth (AOD) were measured at Chungli (24.58° N, 121.1° E), Taiwan during the period from 2002–2004. The depolarization ratios of background aerosol have values mostly less than 0.06. The maximum AOD in the altitude range of 0.7 to 2km occurs in the summer (June–August) while between 2 and 5km, the spring (March–May) shows the maximum. The former is mainly related to strong convection and humidity; however the latter is due to anthropogenic aerosols transported from East China and Southeast Asia based on calculations of backward trajectories. This seasonal variation of AOD inferred from different transport mechanisms and aerosol compositions which are supported by the height distributions of aerosol extinction and origins.  相似文献   

18.
Aerosol observational data at 8 ground-based observation sites in the Chinese Sun Hazemeter Network(CSHNET)were analyzed to characterize the optical properties of aerosol particles during the strong dust storm of 16-21 April 2005.The observational aerosol optical depth(AOD)increased significantly during this dust storm at sites in Beijing city(86%),Beijing forest(84%),Xianghe(13%),Shapotou(27%),Shenyang(47%),Shanghai(23%),and Jiaozhou Bay(24%).The API(air pollution index)in Beijing and Tianjin also had a similar rise during the dust storm,while the Angstrm exponent(α)declined evidently at sites in Beijing city(21%),Beijing forest(39%),Xianghe(19%),Ordos(77%),Shapotou(50%),Shanghai(12%),and Jiaozhou Bay(21%),respectively.Furthermore,The observational AOD andαdemonstrated contrary trends during all storm stages(pre-dust storm,dust storm,and post-dust storm),with the AOD indicating an obvious"Valley-Peak-Valley"pattern of variation,whileαdemonstrated a"Peak-Valley-Peak"pattern. In addition,the dust module in a regional climate model(RegCM3)simulated the dust storm occurrence and track accurately and RegCM3 was able to basically simulate the trends in AOD.The simulation results for the North China stations were the best,and the simulation for dust-source stations was on the high side,while the simulation was on the low side for coastal sites.  相似文献   

19.
赵胡笳  马雁军 《气象科技》2011,39(4):468-472
利用2009年5月至2009年11月鞍山、沈阳、本溪、抚顺4个市区的器测能见度和人工观测能见度资料,分别按照不同气象要素和天气现象等情形下,对两种观测数据资料的差异进行了详细的统计分析.结果表明:与无视程障碍天气情形相比,出现具有视程障碍天气情形时,器测、目测能见度差异较小;总云量越多,两种观测值差异越小;PM10质量...  相似文献   

20.
A comparative study on the vertical distributions of aerosol optical properties during haze and floating dust weather in Shanghai was conducted based on the data obtained from a micro pulse lidar.There was a distinct difference in layer thickness and extinction coefficient under the two types of weather conditions.Aerosols were concentrated below 1 km and the aerosol extinction coefficients ranged from 0.25 to 1.50km-1 on haze days.In contrast,aerosols with smaller extinction coefficients(0.20 0.35 km-1) accumulated mainly from the surface to 2 km on floating dust days.The seasonal variations of extinction and aerosol optical depth（AOD） for both haze and floating dust cases were similar greatest in winter,smaller in spring,and smallest in autumn.More than 85%of the aerosols appeared in the atmosphere below 1 km during severe haze and floating dust weather.The diurnal variation of the extinction coefficient of haze exhibited a bimodal shape with two peaks in the morning or at noon,and at nightfall,respectively.The aerosol extinction coefficient gradually increased throughout the day during floating dust weather.Case studies showed that haze aerosols were generated from the surface and then lifted up,but floating dust aerosols were transported vertically from higher altitude to the surface.The AOD during floating dust weather was higher than that during haze.The boundary layer was more stable during haze than during floating dust weather.  相似文献   

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