共查询到19条相似文献，搜索用时 109 毫秒
1.
平流层对对流层的作用是准确评估、预测对流层气候变化的一个重要方面。其中平流层成分尤其是臭氧的变化,可以改变平流层乃至对流层的辐射平衡,从而影响平流层、对流层的热动力过程。本文从辐射、动力2个角度介绍了平流层臭氧影响对流层气候变化的若干研究进展。平流层臭氧可以通过长短波辐射的方式对对流层大气造成辐射强迫,利用大气化学气候模式可以定量计算平流层臭氧变化引起的辐射强迫,但是辐射强迫的估算受模式中辐射传输模块本身缺陷的影响存在不确定性。动力方面,平流层臭氧变化产生的辐射效应可以改变温度的垂直和经向梯度,造成波折射指数的变化,进而影响平流层甚至对流层内波的折射与反射,通过上对流层下平流层区域内的波—流相互作用,对对流层气候产生影响。另外,南极臭氧损耗可通过大气环状模影响冬春季中高纬度对流层的天气气候,但是其影响的强度大小以及物理机制仍需进一步的确认。值得注意的是,北极平流层臭氧的变化与北半球中高纬度气候变化之间的关系相比南半球要更加复杂,需要更为深入的研究。 相似文献
2.
文中使用欧洲中期天气预报中心臭氧柱总量资料分析了西北太平洋地区大气臭氧柱总量的时空分布特征,结果表明:低纬度地区是臭氧柱总量最低的地区,纬向分布明显,臭氧柱总量随着纬度向北极的增加而增大;夏季臭氧柱总量最大值出现在北半球高纬度约80°N的地区,最低值出现在热带地区;秋季臭氧柱总量最大值出现在55°N左右的地区;最小值出现在赤道地区。冬春季,臭氧柱总量的最低值均出现在热带地区,最高值出现在北半球约50°～60°N的高纬度地区。 相似文献
3.
利用观测和再分析资料通过合成分析方法,研究了中部型ENSO和平流层准两年振荡（QBO）对冬季北半球平流层臭氧的独立影响和联合调制作用。研究表明,北半球平流层臭氧在中部型厄尔尼诺年增加,而在中部型拉尼娜年减少;准两年振荡东风位相年份,北半球平流层臭氧增加,准两年振荡西风位相结果则相反。相比之下,北半球中、高纬度平流层臭氧异常对准两年振荡活动的响应明显小于其对ENSO活动的响应。进一步研究发现,准两年振荡东风位相会加强中部型厄尔尼诺事件引起的北半球平流层臭氧的增加,而减弱中部型拉尼娜事件造成的平流层臭氧的减少。在准两年振荡西风位相下,中部型厄尔尼诺事件仅导致北半球平流层臭氧含量少量升高,而中部型拉尼娜事件期间臭氧会大幅度减少。因此,准两年振荡东风位相会加强中部型厄尔尼诺事件对北半球平流层臭氧的影响,而减弱中部型拉尼娜事件对北半球平流层臭氧的影响。准两年振荡西风位相会减弱中部型厄尔尼诺而加强中部型拉尼娜事件对北半球平流层臭氧的影响。 相似文献
4.
利用2003—2013年北京地区臭氧探空资料和多种再分析资料,结合CAM-chem模式模拟分析了北京地区对流层臭氧的长期变化趋势及影响因子。结果表明:近11 a来,北京地区对流层臭氧整体呈明显增加趋势,对流层臭氧总量每年增加约0.98 DU,且地表排放对该地区对流层臭氧增加的贡献相比动力过程更大。其中,由平流层向下输送造成的对流层臭氧总量每年增加约为0.13×10~(-3)~0.17×10~(-3)Tg,对北京地区对流层臭氧总量的增加贡献约20%;由水平输送造成的臭氧增加每年约为0.06×10~(-3)Tg,对臭氧总量增加贡献约10%;而由地表排放造成的对流层臭氧增加约占该地区对流层臭氧总增加量的60%。 相似文献
5.
臭氧和平流层动力学的相互作用 总被引：1，自引：0，他引：1
讨论了给定的南极春季臭氧洞(取自1979—1985年臭氧减少的观测结果)对二维平流层—对流层模式中温度和环流的影响。11月份,南极上空约17km处,温度最多可降低6℃。这种温度变化引起的平均经向环流对臭氧洞起填塞作用,不过,这种影响很小,每年仅产生14DU的变化。观测事实表明,近年来10月份,南半球波活动减弱。为此,我们作了南半球波作用全年都减少一半,并考虑了臭氧洞的数值试验。结果表明,臭氧柱在11月份76°S减少了44DU,在赤道却增加了12DU。 相似文献
6.
通过WACCM-3模式中气溶胶光学厚度与卫星资料的对比发现,模式可以很好地再现全球气溶胶的主要分布特征,但在一些区域还存在数值上的差异。利用数值试验研究对流层气溶胶的直接气候效应对平流层气候的影响,结果表明:对流层气溶胶对平流层气候有明显影响,平流层化学过程在这一影响中起重要作用,而对流层气溶胶对平流层辐射的影响不是其直接气候效应对平流层影响的主要原因。其机制可能是对流层气溶胶改变对流层的辐射平衡,影响对流层的温度和大气环流,进而影响行星波的上传,使得平流层气候发生变化;影响区域主要位于高纬度和极地地区,南半球的变化比北半球大,温度变化最大达10 K,纬向风变化最大可达12 m/s,臭氧体积分数最多减少0.8×10-6。 相似文献
7.
利用卫星和台站观测的南极臭氧资料和NCEP/NCAR再分析资料,分析了南极臭氧近年来的变化特征和影响因子,探讨了南极臭氧洞期间中山站臭氧突变过程与大气动力的作用。结果显示,平流层氯和溴的卤化物当量（EESC）和平流层温度是影响南极臭氧洞面积的关键因子。臭氧总量与EESC和平流层温度均具有显著相关,表明两站虽然都位于臭氧洞边缘,EESC和平流层温度对臭氧总量的变化仍然可以起决定性的作用,同时也验证了EESC参数在东南极大陆沿岸具有适用性。 EESC的年代际变化与臭氧变化趋势相似,臭氧的年际变化与平流层温度关系密切。回归结果表明,2010年后臭氧洞面积逐渐减小,在2070年左右可能恢复到1980年前的水平,但其结果存在很大的不确定性。 相似文献
8.
1.引言极地平流层云(PSCs)对南极臭氧洞的形成及北半球臭氧的耗减是至关重要的.首先,极地平流层云通过沉降作用清除平流层中作为云的成分的氮化物.云层内低的氮化物含量,对高水平的活性氯物质的存在是极 相似文献
9.
《高原气象》2016,(5)
为全面了解冬季北半球中高纬度地区臭氧与同期北极极涡强度变化的相关关系,利用1979年1月至2011年12月欧洲中心再分析资料,选取了4个关键区(北极、东亚、北美和西欧),采用相关分析和E-P通量计算方法,分析了两者之间的相关关系并进行了机制研究。结果表明:(1)冬季北极平流层臭氧总量与极涡强度的负相关关系较好;(2)当极涡强(弱)年,极圈内和外围的北美部分地区臭氧总量显著减少(增加);(3)极涡强度弱时,上传到平流层的涡动热通量强,北半球中高纬地区E-P通量散度辐合增强,剩余环流加强,将导致该地区得到低纬高浓度臭氧的补充而使得臭氧含量增多;(4)1979-2011年上传到中高纬平流层的波动通量增加,造成极区温度增加,进而抑制非均相反应发生而使得极区臭氧含量增加。 相似文献
10.
2000年北半球平流层、对流层质量交换的季节变化 总被引：21，自引：6，他引：15
用2000年NCEP资料,P坐标下Wei公式诊断北半球平流层、对流层交换的季节变化.主要结论:(1)热带西太平洋是物质由对流层向平流层输送的主要通道,并有明显的季节性东西移动.由于2000年赤道辐合带偏弱,因此秋季通量最大.(2)中高纬度地区同时存在向上、向下的通量,大尺度槽区伴随着平流层向下的输送.一年中冬春季向下的输送强,夏秋季较弱,其季节变化与大尺度环流的季节性变化一致.(3)东亚地区存在很强的平流层向下输送,且中心位置移动不大.只占北半球5.6%面积的东亚其年净交换量竟占北半球的29%,这说明东亚地区的平流层与对流层之间的质量交换对北半球平流层、对流层交换研究的重要性. 相似文献
11.
Impact of increasing stratospheric water vapor on ozone depletion and temperature change 总被引：2，自引：0，他引：2
Using a detailed, fully coupled chemistry climate model (CCM), the effect of increasing
stratospheric H2O on ozone and temperature is investigated. Different CCM time-slice runs have
been performed to investigate the chemical and radiative impacts of an assumed 2 ppmv increase in
H2O. The chemical effects of this H2O increase lead to an overall decrease of the total column ozone
(TCO) by ～1% in the tropics and by a maximum of 12% at southern high latitudes. At northern high
latitudes, the TCO is increased by only up to 5% due to stronger transport in the Arctic. A 2-ppmv H2O
increase in the model's radiation scheme causes a cooling of the tropical stratosphere of no more than 2 K,
but a cooling of more than 4 K at high latitudes. Consequently, the TCO is increased by about 2%--6%.
Increasing stratospheric H2O, therefore, cools the stratosphere both directly and indirectly, except in
the polar regions where the temperature responds differently due to feedbacks between ozone and H2O changes.
The combined chemical and radiative effects of increasing H2O may give rise to more cooling in the tropics
and middle latitudes but less cooling in the polar stratosphere. The combined effects of H2O increases on
ozone tend to offset each other, except in the Arctic stratosphere where both the radiative and chemical
impacts give rise to increased ozone. The chemical and radiative effects of increasing H2O cause dynamical
responses in the stratosphere with an evident hemispheric asymmetry. In terms of ozone recovery, increasing
the stratospheric H2O is likely to accelerate the recovery in the northern high latitudes and delay it in
the southern high latitudes. The modeled ozone recovery is more significant between 2000--2050 than between
2050--2100, driven mainly by the larger relative change in chlorine in the earlier period. 相似文献
12.
To analyze the mechanism by which water vapor increase leads to cooling in the stratosphere, the effects of water-vapor increases on temperature in the stratosphere were simulated using the two-dimensional, interactive chemical dynamical radiative model (SOCRATES) of NCAR. The results indicate that increases in stratospheric water vapor lead to stratospheric cooling, with the extent of cooling increasing with height, and that cooling in the middle stratosphere is stronger in Arctic regions. Analysis of the radiation process showed that infrared radiative cooling by water vapor is a pivotal factor in middle-lower stratospheric cooling. However, in the upper stratosphere (above 45 km), infrared radiation is not a factor in cooling; there, cooling is caused by the decreased solar radiative heating rate resulting from ozone decrease due to increased stratospheric water vapor. Dynamical cooling is important in the middle-upper stratosphere, and dynamical feedback to temperature change is more distinct in the Northern Hemisphere middle-high latitudes than in other regions and signiffcantly affects temperature and ozone in winter over Arctic regions. Increasing stratospheric water vapor will strengthen ozone depletion through the chemical process. However, ozone will increase in the middle stratosphere. The change in ozone due to increasing water vapor has an important effect on the stratospheric temperature change. 相似文献
13.
AbstractTo evaluate future climate change in the middle atmosphere and the chemistry–climate interaction of stratospheric ozone, we performed a long-term simulation from 1960 to 2050 with boundary conditions from the Intergovernmental Panel on Climate Change A1B greenhouse gas scenario and the World Meteorological Organization Ab halogen scenario using the chemistry–climate model ECHAM5/MESSy Atmospheric Chemistry (EMAC). In addition to this standard simulation we performed five sensitivity simulations from 2000 to 2050 using the rerun files of the simulation mentioned above. For these sensitivity simulations we used the same model setup as in the standard simulation but changed the boundary conditions for carbon dioxide (CO2), methane (CH4), nitrous oxide (N2O), and ozone-depleting substances (ODS). In the first sensitivity simulation we fixed the mixing ratios of CO2, CH4, and N2O in the boundary conditions to the amounts for 2000. In each of the four other sensitivity simulations we fixed the boundary conditions of only one of CO2, CH4, N2O, or ODS to the year 2000.In our model simulations the future evolution of greenhouse gases leads to significant cooling in the stratosphere and mesosphere. Increasing CO2 mixing ratios make the largest contributions to this radiative cooling, followed by increasing stratospheric CH4, which also forms additional H2O in the upper stratosphere and mesosphere. Increasing N2O mixing ratios makes the smallest contributions to the cooling. The simulated ozone recovery leads to warming of the middle atmosphere.In the EMAC model the future development of ozone is influenced by several factors. 1) Cooler temperatures lead to an increase in ozone in the upper stratosphere. The strongest contribution to this ozone production is cooling due to increasing CO2 mixing ratios, followed by increasing CH4. 2) Decreasing ODS mixing ratios lead to ozone recovery, but the contribution to the total ozone increase in the upper stratosphere is only slightly higher than the contribution of the cooling by greenhouse gases. In the polar lower stratosphere a decrease in ODS is mainly responsible for ozone recovery. 3) Higher NOx and HOx mixing ratios due to increased N2O and CH4 lead to intensified ozone destruction, primarily in the middle and upper stratosphere, from additional NOx; in the mesosphere the intensified ozone destruction is caused by additional HOx. In comparison to the increase in ozone due to decreasing ODS, ozone destruction caused by increased NOx is of similar importance in some regions, especially in the middle stratosphere. 4) In the stratosphere the enhancement of the Brewer-Dobson circulation leads to a change in ozone transport. In the polar stratosphere increased downwelling leads to additional ozone in the future, especially at high northern latitudes. The dynamical impact on ozone development is higher at some altitudes in the polar stratosphere than the ozone increase due to cooler temperatures. In the tropical lower stratosphere increased residual vertical upward transport leads to a decrease in ozone. 相似文献
14.
利用2010—2012年对流层臭氧（O3）及其多种前体物的卫星遥感资料和全球水汽再分析资料,研究东亚区域O3及其前体物的时空分布,以及在中国东部（分为南、北两部分）相关性的季节变化。结果表明:东亚区域NO2与CO的对流层柱含量均表现为冬季高、夏季低的时空变化形式。O3对流层柱含量夏季达到峰值,冬季为谷值。中国东部的北部与南部地区O3与NO2均在夏秋季呈正相关,冬春季呈负相关。夏季大部分地区NOx的光化学循环反应对O3生成有积极的促进作用,冬季大部分地区O3的光化学循环生成受到抑制。O3与CO在北部地区夏秋季和南部地区夏季正相关性最大,无论是在北部还是南部地区,O3与CO的相关性在轻污染情况下最大,而在重污染和背景情况下较小,表明重污染气团向下风方的输送更有利于O3的光化学生成。O3与水汽在北部和南部地区的多数时间均呈较显著的正相关性,而在南部地区夏季和北部地区冬季具有较大的负相关性,反映出不同的环流形式、气团来源及伴随的天气条件变化对O3分布的影响。 相似文献
15.
Kequan ZHANG Jiakang DUAN Siyi ZHAO Jiankai ZHANG James KEEBLE Hongwen LIU 《大气科学进展》2022,39(7):1167-1183
Total column ozone (TCO) over the Tibetan Plateau (TP) is lower than that over other regions at the same latitude, particularly in summer. This feature is known as the “TP ozone valley”. This study evaluates long-term changes in TCO and the ozone valley over the TP from 1984 to 2100 using Coupled Model Intercomparison Project Phase 6 (CMIP6). The TP ozone valley consists of two low centers, one is located in the upper troposphere and lower stratosphere (UTLS), and the other is in the middle and upper stratosphere. Overall, the CMIP6 models simulate the low ozone center in the UTLS well and capture the spatial characteristics and seasonal cycle of the TP ozone valley, with spatial correlation coefficients between the modeled TCO and the Multi Sensor Reanalysis version 2 (MSR2) TCO observations greater than 0.8 for all CMIP6 models. Further analysis reveals that models which use fully coupled and online stratospheric chemistry schemes simulate the anticorrelation between the 150 hPa geopotential height and zonal anomaly of TCO over the TP better than models without interactive chemistry schemes. This suggests that coupled chemical-radiative-dynamical processes play a key role in the simulation of the TP ozone valley. Most CMIP6 models underestimate the low center in the middle and upper stratosphere when compared with the Microwave Limb Sounder (MLS) observations. However, the bias in the middle and upper stratospheric ozone simulations has a marginal effect on the simulation of the TP ozone valley. Most CMIP6 models predict the TP ozone valley in summer will deepen in the future. 相似文献
16.
17.
BCC_AGCM2.1模式对平流层环流变化特征的数值模拟及其模式评估 总被引：2，自引：1，他引：1
使用国家气候中心大气环流模式BCC_AGCM2.1的30年模拟试验资料,对平流层纬向环流场、高空急流、极涡及爆发性增温过程进行了数值模拟研究,并使用欧洲中期天气预报中心（ECMWF）和美国国家环境预报中心（NCEP）的再分析资料对模式输出结果进行了对比、分析。结果表明：（1） 在观测海温、二氧化碳、气溶胶等外强迫地驱动下,BCC模式能够很好地再现出与再分析资料一致的平流层纬向平均风场、温度场的分布特征和季节变化过程;模拟得到的温度廓线和高空急流与再分析资料的主要差别出现在南、北半球冬季的中高纬度地区;模拟得到的平流层温度普遍偏低,主要的差异位于对流层顶区域和平流层高层。（2） 模拟的对流层上层的副热带急流位置偏南、强度也偏弱,而平流层中的绕极极夜急流则位置偏北、强度更大。这样的急流分布特征使模拟的行星波向赤道的波导更强,向极的波导偏弱;同时由于模式中本身可以形成的行星波就比再分析资料弱,因此导致模拟结果中北半球冬季的平流层极涡更加稳定、极区温度更低。（3） BCC模式对于平流层极涡的季节变化特征模拟得较好,但对强极涡扰动过程,即北半球冬季的平流层爆发性增温（SSW）事件则模拟效果不佳,不论是增温事件出现的频率,还是增温的时间、强度,模拟结果和再分析资料都还存在一定偏差,需要在今后的工作中逐步改善。 相似文献
18.
AbstractThe solar backscattered ultraviolet (SBUV/SBUV-2) merged ozone datasets, version 8.6, including column ozone and ozone profiles for the 1979–2012 period are examined for the 35°N–60°N zonal belt in the northern hemisphere mid-latitudes and four sub-regions: central Europe, continental Europe, North America, and East Asia. The residual long-term patterns for total ozone and ozone profiles are extracted by smoothing the time series of differences between the original and the modelled ozone time series. Modelled ozone is obtained using the standard trend model accounting for ozone variability due to changes in stratospheric halogens and various dynamical factors commonly used in previous ozone trend analyses. Since about 2005 spring and summer total ozone in the troposphere and lower stratosphere has decreased in some regions (central and continental Europe, North America, and the 35°N–60°N zonal belt) compared with modelled ozone. The negative departure from modelled ozone in 2010 is approximately 2–3% of the overall 1979–2012 monthly mean level. It seems that this decrease is a result of yet unknown dynamical processes rather than to chemical destruction because the differences have a longitudinal structure, and total ozone in the upper stratosphere still follows changes in stratospheric halogen loading. 相似文献
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A review of global stratospheric aerosol: Measurements, importance, life cycle, and local stratospheric aerosol 总被引：1，自引：0，他引：1
Stratospheric aerosol, noted after large volcanic eruptions since at least the late 1800s, were first measured in the late 1950s, with the modern continuous record beginning in the 1970s. Stratospheric aerosol, both volcanic and non-volcanic are sulfuric acid droplets with radii (concentrations) on the order of 0.1–0.5 µm (0.5–0.005 cm− 3), increasing by factors of 2–4 (10–103) after large volcanic eruptions. The source of the sulfur for the aerosol is either through direct injection from sulfur-rich volcanic eruptions, or from tropical injection of tropospheric air containing OCS, SO2, and sulfate particles. The life cycle of non-volcanic stratospheric aerosol, consisting of photo-dissociation and oxidation of sulfur source gases, nucleation/condensation in the tropics, transport pole-ward and downward in the global planetary wave driven tropical pump, leads to a quasi steady state relative maximum in particle number concentration at around 20 km in the mid latitudes. Stratospheric aerosol have significant impacts on the Earth's radiation balance for several years following volcanic eruptions. Away from large eruptions, the direct radiation impact is small and well characterized; however, these particles also may play a role in the nucleation of near tropopause cirrus, and thus indirectly affect radiation. Stratospheric aerosol play a larger role in the chemical, particularly ozone, balance of the stratosphere. In the mid latitudes they interact with both nitrous oxides and chlorine reservoirs, thus indirectly affecting ozone. In the polar regions they provide condensation sites for polar stratospheric clouds which then provide the surfaces necessary to convert inactive to active chlorine leading to polar ozone loss. Until the mid 1990s the modern record has been dominated by three large sulfur-rich eruptions: Fuego (1974), El Chichón (1982) and Pinatubo (1991), thus definitive conclusions concerning the trend of non-volcanic stratospheric aerosol could only recently be made. Although anthropogenic emissions of SO2 have changed somewhat over the past 30 years, the measurements during volcanically quiescent periods indicate no long term trend in non-volcanic stratospheric aerosol. 相似文献