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1.
The studies on the effect of atmospheric aerosol on climate and environment are hot issues in the current circle of international science and technology. In recent years the pollution of aerosol is getting worse and worse over the Pearl River Delta. The clouds of aerosol occur all year round, with heavy pollution area located at the western side at the mouth of Pearl River. The haze weather mainly occurs from October to April next year, resulting in visibility deterioration. From the beginning of 1980s, visibility dramatically deteriorated, obviously increasing haze weather, in which there are three big fluctuations, showing the periods of pollutions of dust, sulphate and dust, fine particle from photochemical process and sulphate and dust accompanying with the development of economy respectively. The long-term tendency of visibility caused by fog and light fog does not show a tendency due to human activities or economic development, which mainly shows the interannual and interdecadal variation of climate. The deterioration of visibility has close relation to the fine particles over Pearl River Delta, with half of PM10 overpass the limited value set by national second graded standard (150μg m-3), meanwhile, all values of PM2.5 overpass the day-mean limited value of American national standard (65μg m-3), especially from October to January next year, monthly mean values of PM2.5 almost reach two times of standard value, indicating the fine particle concentration is very high. The ratio of PM2.5 to PM10 is also very high, reaching 58%-77%, higher especially in dry season than in rainy season. Thus it is the fine particle pollution in aerosol pollution over the Pearl River Delta. Compared with the data of 15 years ago, the ratio of fine particle to aerosol has obviously increased.  相似文献   

2.
A comparative study on the vertical distributions of aerosol optical properties during haze and floating dust weather in Shanghai was conducted based on the data obtained from a micro pulse lidar.There was a distinct difference in layer thickness and extinction coefficient under the two types of weather conditions.Aerosols were concentrated below 1 km and the aerosol extinction coefficients ranged from 0.25 to 1.50km-1 on haze days.In contrast,aerosols with smaller extinction coefficients(0.20 0.35 km-1) accumulated mainly from the surface to 2 km on floating dust days.The seasonal variations of extinction and aerosol optical depth（AOD） for both haze and floating dust cases were similar greatest in winter,smaller in spring,and smallest in autumn.More than 85%of the aerosols appeared in the atmosphere below 1 km during severe haze and floating dust weather.The diurnal variation of the extinction coefficient of haze exhibited a bimodal shape with two peaks in the morning or at noon,and at nightfall,respectively.The aerosol extinction coefficient gradually increased throughout the day during floating dust weather.Case studies showed that haze aerosols were generated from the surface and then lifted up,but floating dust aerosols were transported vertically from higher altitude to the surface.The AOD during floating dust weather was higher than that during haze.The boundary layer was more stable during haze than during floating dust weather.  相似文献   

3.
This paper explores the role of the secondary inorganic aerosol （SIA） species ammonium,NH4＋,nitrate,NO3-,and sulfate,SO24-,during haze and fog events using hourly mass concentrations of PM2.5 measured at a suburban site in Hangzhou,China.A total of 546 samples were collected between 1 April and 8 May 2012.The samples were analyzed and classified as clear,haze or fog depending on visibility and relative humidity （RH）.The contribution of SIA species to PM2.5 mass increased to ～50％ during haze and fog.The mass contribution of nitrate to PM2.5 increased from 11％ during clear to 20％ during haze episodes.Nitrate mass exceeded sulfate mass during haze,while near equal concentrations were observed during fog episodes.The role of RH on the correlation between concentrations of SIA and visibility was examined,with optimal correlation at 60％-70％ RH.The total acidity during clear,haze and fog periods was 42.38,48.38 and 45.51 nmol m-3,respectively,indicating that sulfate,nitrate and chloride were not neutralized by ammonium during any period.The nitrate to sulfate molar ratio,as a function of the ammonium to sulfate molar ratio,indicated that nitrate formation during fog started at a higher ammonium to sulfate molar ratio compared to clear and haze periods.During haze and fog,the nitrate oxidation ratio increased by a factor of 1.6-1.7,while the sulfur oxidation ratio increased by a factor of 1.2-1.5,indicating that both gaseous NO2 and SO2 were involved in the reduced visibility.  相似文献   

4.
Haze-to-fog transformation during a long lasting, low visibility episode was examined using the observations from a comprehensive field campaign conducted in Nanjing, China during 4-9 December 2013. In this episode, haze was transformed into fog and the fog lasted for dozens of hours. The impacts of meteorological factors such as wind, temperature (T) and relative humidity (RH) on haze, transition and fog during this episode were investigated. Results revealed significant differences between haze and fog days, due to their different formation mechanisms. Comparison was made for boundary-layer conditions during hazy days, haze-to-fog days and foggy days. Distributions of wind speed and wind direction as well as synoptic weather conditions around Nanjing had determinative impacts on the occurrences and characteristics of haze and fog. Weakened southerly wind in southern Nanjing resulted in high concentration of pollutants, and haze events occurred frequently during the study period. The wind speed was less than 1 m s-1 in the haze event, which resulted in a stable atmospheric condition and weak dispersion of the pollutants. The height of the temperature inversion was about 400 m during the period. The inversion intensity was weak and the temperature-difference was 4°C km-1 or less in haze, while the inversion was stronger, and temperature-difference was about 6°C km-1, approaching the inversion layer intensity in the fog event. Haze event is strongly influenced by ambient RH. RH values increased, which resulted in haze days evidently increased, suggesting that an increasing fraction of haze events be caused by hygroscopic growth of aerosols, rather than simply by high aerosol loading. When RH was above 90%, haze aerosols started to be transformed from haze to fog. This study calls for more efforts to control emissions to prevent haze events in the region.  相似文献   

5.
Using the composite field observational data collected in the area south of the Nanling Mts. and numerical modeling, the seasonal features of dense fog and visibility, fog drop spectrum and physical concept of fog forming have been analyzed. The occurring frequency of low visibility（≤200 m） is very high with a mean of 24.7%, a maximum of 41.8% from the end of autumn to winter and next spring. The fog processes that occur in the area south of the Nanling Mts. in spring and winter result from the interactions of complicated micro-physical processes, the local terrain, water vapor transportation and the influencing weather system. The fog processes are arisen from advection or windward slope, which is much different from the radiation fog. Cooling condensation due to the air lifted by the local mountain plays an important role in fog formation. Windward slope of the mountain is favorable to the fog formation. Dense fog can occur at lower altitudes in the windward slope of mountain, resulting in the lower visibility. The fog is mainly of small-drop spectrum with smaller number-density than that of urban fog, and its drop spectrum has descending trend in the section of smaller diameter. The inverse relationship between fog water content and visibility is the best among several relationships of micro-variables. In addition to micro-physical processes of fog body itself, the motion of irregular climbing and crossing over hillside while the fog body is being transported by the wind are also important reasons for the fluctuation of micro-physical parameters such as fog water content.  相似文献   

6.
Continuous observations of mass concentration and elemental composition of aerosol particles （PM2.5） were conducted at Tongyu, a semi-arid site in Northeast China in the spring of 2006. The average mass concentration of PM2.5 at Tongyu station was 260.9±274.4 μg m^-3 during the observation period. Nine dust events were monitored with a mean concentration of 528.0±302.7 μgm^-3. The PM2.5 level during non- dust storm （NDS） period was 111.65±63.37 μg m^-3. High mass concentration shows that fine-size particles pollution was very serious in the semi-arid area in Northeast China. The enrichment factor values for crust elements during the dust storm （DS） period are close to those in the NDS period, while the enrichment factor values for pollution elements during the NDS period are much higher than those in the DS period, showing these elements were from anthropogenic sources. The ratios of dust elements to Fe were relative constant during the DS period. The Ca/Fe ratio in dust aerosols at Tongyu is remarkably different from that observed in other source regions and downwind regions. Meteorological analysis shows that dust events at Tongyu are usually associated with dry, low pressure and high wind speed weather conditions. Air mass back-trajectory analysis identified three kinds of general pathways were associated with the aerosol particle transport to Tongyu, and the northwest direction pathway was the main transport route.  相似文献   

7.
Urban aerosols have a large effect on the deterioration of air quality and the degradation of atmospheric visibility.Characterization of the chemical composition of PM 2.5 and in situ measurements of the optical properties of aerosols were conducted in July 2008 at an urban site in Guangzhou,Southern China.The mean PM 2.5 concentration for the entire period was 53.7±23.2 μg m 3.The mean PM 2.5 concentration (82.7±25.4 μg m 3) on hazy days was roughly two times higher than that on clear days (38.8±8.7 μg m 3).The total water-soluble ion species and the total average carbon accounted for 47.9%±4.3% and 35.2%±4.5%,respectively,of the major components of PM 2.5.The increase of secondary and carbonaceous aerosols,in particular ammonium sulfate,played an important role in the formation of haze pollution.The mean absorption and scattering coefficients and the single scattering albedo over the whole period were 53±20 M m 1,226±111 M m 1,and 0.80±0.04,respectively.PM 2.5 had a high linear correlation with the aerosol extinction coefficient,elemental carbon (EC) was correlated with aerosol absorption,and organic carbon (OC) and SO 4 2 were tightly linked to aerosol scattering.  相似文献   

8.
A Novel Four-Wavelength Transmissometer for Distinguishing Haze and Fog   总被引：1，自引：1，他引：0  
Haze and fog exhibit different microphysical and optical properties according to Mie scattering theory. Haze particles are smaller than fog droplets. Light of a shorter wavelength is reduced more than that of a longer wavelength during haze events. In fog, the differences between the extinction coefficients at different wavelengths are not as apparent. On the basis of the different light extinction characteristics of haze and fog, a novel four-wavelength transmissometer based on charge-coupled device （CCD） imaging was designed to distinguish haze from fog with central wavelengths at 415, 516, 650, and 850 nm. The four-wavelength transmissometer was tested in an insitu experiment during the winter of 2009. Fog was determined when the differences of the extinction coefficients at the four wavelengths were not notable, whereas haze was determined when the light at shorter wavelengths was significantly more reduced than that at longer wavelengths. A threshold which describes the relative size of the extinction coefficients at the four wavelengths was defined to distinguish between fog and haze. The four-wavelength transmissometer provided results consistent with the commercial fog monitor during several measurements made in fog and haze events, especially under conditions of low visibility and high relative humidity.  相似文献   

9.
A set of micro pulse lidar(MPL)systems operating at 532 nm was used for ground-based observation of aerosols in Shanghai in 2011.Three typical particulate pollution events(e.g.,haze)were examined to determine the evolution of aerosol vertical distribution and the planetary boundary layer(PBL)during these pollution episodes.The aerosol vertical extinction coefficient(VEC)at any given measured altitude was prominently larger during haze periods than that before or after the associated event.Aerosols originating from various source regions exerted forcing to some extent on aerosol loading and vertical layering,leading to different aerosol vertical distribution structures.Aerosol VECs were always maximized near the surface owing to the potential influence of local pollutant emissions.Several peaks in aerosol VECs were found at altitudes above 1 km during the dust-and bioburning-influenced haze events.Aerosol VECs decreased with increasing altitude during the local-polluted haze event,with a single maximum in the surface atmosphere.PM2.5 increased slowly while PBL and visibility decreased gradually in the early stages of haze events;subsequently,PM2.5 accumulated and was exacerbated until serious pollution bursts occurred in the middle and later stages.The results reveal that aerosols from different sources impact aerosol vertical distributions in the atmosphere and that the relationship between PBL and pollutant loadings may play an important role in the formation of pollution.  相似文献   

10.
Visibility is one of the parameters for indicating air pollution.In this study,visibility variation in Hong Kong during summer and winter is investigated.Visibility in Hong Kong has clear intraseasonal variation.Examination of different environmental parameters suggests that the intraseasonal component dominates the overall circulation anomalies in both summer and winter.Associated with the intraseasonal variation of environmental parameters,obvious variation in visibility impairment is found in both summer and winter.In summer,local visibility and air quality are found to be significantly affected by the(MJO)and the 10–30-day intraseasonal oscillation(ISO)through modulation of associated atmospheric circulations.In winter,the modulation effects appear to be weaker due to the southward shift of the associated convection.The results in this study highlight the importance of the ISO in contributing to the overall variation in visibility in Hong Kong,and provide useful implications for the development of possible mitigation strategies associated with visibility impairment and air pollution in Hong Kong.  相似文献   

11.
2014年,中国气象局将地面人工观测业务调整为自动仪器观测的方式,这一改变明显提高了工作效率,但对观测结果,特别是视程障碍类观测产生了一定的影响。为了完善内蒙古地区霾和沙尘天气判别标准,获得准确可信的气象资料,本文选取了2001-2019年内蒙古12个站点逐三小时的气象观测资料,从时空分布特征和判别方法研究了内蒙古地区沙尘和霾自动气象观测数据的可靠性和判别标准的适用性。结合PM2.5和PM10两个空气质量指数,通过修正错误记录,将沙尘中误判的霾和无天气、霾中误判的沙尘、雾和无天气等分离出来。对比结果来看,修正前,霾和沙尘分别占总频次的95%和5%；修正后,霾、沙尘、雾和无天气分别占总频次的55%、17%、1%、27%。对比呼和浩特单站一次沙尘和一次霾天气过程中气象要素和空气质量指数的连续变化可以看出,相对湿度与PM2.5的相关性均达到了0.5以上。沙尘期,能见度与PM10负相关,PM2.5和PM10相关性较差；而霾期,能见度与PM2.5和PM10的相关性较差,PM2.5和PM10相关性达到了0.8以上,即不同相对湿度环境下影响能见度的因素不同。  相似文献   

12.
天津一次持续低能见度事件的影响因素分析   总被引：7，自引：2，他引：5  
姚青  韩素芹  蔡子颖 《气象》2012,38(6):688-694
2009年1月天津发生了一次持续低能见度事件,从气象条件、污染演化过程和气流后向轨迹等方面分析该次事件是由以细粒子为主的灰霾天气所引起。分析表明,细粒子质量浓度是影响大气能见度的主要因素;细粒子在可吸人颗粒物中的富集,是造成持续性污染和能见度连续下降的主要原因;西南暖湿气流控制下的静稳天气有利于污染物聚集,而以大风降温为标志的冷锋过境是细粒子清除的重要机制;能见度的周期性变化主要依赖于细粒子的富集和污染物的快速清除,并且这一过程受到周期性天气系统的影响。  相似文献   

13.
沿海工业城市灰霾天气增多与海盐气溶胶粒子的关系   总被引：13，自引：1，他引：12  
吴兑 《广东气象》2009,31(2):1-3
我国28年前在粉尘污染时代建立的空气质量评价体系,已经远远不能描述新型复合空气污染类型,尤其是不能描述细粒子污染的情况,能见度（vis）的恶化主要与细粒子的质量浓度关系比较大,而与气溶胶的质量浓度关系不大。vis与PM2.5,尤其是PM1有非常好的关系,因而目前用vis来描述灰霾天气是最好的指标。2008年珠三角灰霾的减少与大气环流形势有关,东亚环流径向度较大,冷空气影响岭南地区较为频繁;与2008年下半年爆发的金融海啸引发的加工业开工不足、物流减少亦有关联;另外各级政府对大气环境的治理收到成效也是灰霾天气减少的重要原因。尤其值得注意的是沿海工业城市灰霾天气增长较快,沿海工业城市灰霾天气增多与海盐气溶胶粒子的氯损耗机制关系密切。  相似文献   

14.
利用多尺度空气质量模式系统（Models-3/CMAQ）对2002年12月1—3日北京及周边地区发生的一次大雾天气进行数值模拟,分析了大雾天气下PM2.5二次无机粒子的演变及其影响。结果表明,白天相对湿度降低,雾滴蒸发脱水后PM2.5二次无机粒子会悬浮在大气中;夜间在水汽凝结成雾滴的过程中,大量的PM2.5二次无机粒子提供了充足的凝结核,促进大雾天气的进一步发展。午后PM2.5二次无机粒子积聚及较高的相对湿度是造成北京及周边地区低能见度的重要原因,并推断该区域很可能是霾天气。  相似文献   

15.
沙尘天气是造成我国北方春季区域性沙尘型重污染的主要原因,然而目前对此研究并不多见。因此,本文利用中国环保网2014年1月1日-2016年12月31日内蒙古11个城市环境监测站的颗粒物浓度的逐日和逐时资料,首先分析近3年该地区颗粒物污染浓度的年变化特征,然后对比这3年沙尘天气发生的次数及时段,探究颗粒物污染的年变化特征及其与沙尘天气之关系。统计结果表明,近3年春季内蒙古沙尘天气的发生次数是逐年增加的,中西部是沙尘天气频发区,与之相对应,西部颗粒物浓度的年变化高于东部,且造成内蒙古主要城市PM10浓度春季出现全年的最高值,表明沙尘天气频繁发生对当地粗颗粒物污染有显著的影响。对比内蒙古全年3个时间段的PM10浓度值,其排序是：春季沙尘期间＞春季非沙尘期间＞其他季节;即春季沙尘期间PM10浓度比非沙尘期间高69%,比其他季节高101%。有所不同的是,3个时间段平均PM2.5浓度排序则为：春季沙尘期间＞其他季节＞春季非沙尘期间;春季沙尘期间PM2.5的平均浓度比其他季节高16%,比春季非沙尘期间高29%;可见,春季沙尘天气对相关城市PM10浓度的影响明显大于对PM2.5浓度的影响。最后对内蒙古地区典型沙尘暴和扬沙个例进行细致研究, 发现沙尘暴个例中PM10浓度的增加倍数在2.3~15.1之间,而扬沙过程PM10浓度的增加倍数在0.8~5.6之间,两者相比可看出,沙尘暴过程对颗粒物污染的影响显著大于扬沙过程。  相似文献   

16.
利用中国国家地面站逐小时气象观测资料、中国环境监测总站空气质量逐时监测数据、ECMWF 0.125°（纬度）×0.125°（经度）再分析资料及青岛市八关山自动站常规要素逐小时数据,对2018年1月15~22日青岛市一次重度污染雾—霾天气过程的特征及其影响因子进行分析。结果表明:PM10为首要污染物,污染过程中青岛市48 h 输入污染源前期主要为北方干冷气团与江淮湿空气在山东半岛北部汇聚堆积,后期则主要包括山东省内局地大气污染物排放。雾—霾期间,500 hPa中高纬地区受乌拉尔山阻塞高压和中西伯利亚冷低压控制,宽广的东亚横槽稳定维持,青岛上空以平直西风气流为主,地面等压线稀疏,风速小;随着横槽转竖,纬向型环流转为经向型,冷空气大举南下,风速急增,降雪发生,雾—霾迅速消散。在静稳的大气环流背景下,当近地逆温层内弱风或持续吹陆风,对流层低层上升和下沉运动较弱,水汽条件较好时,有利于雾—霾维持。综合分析雾—霾各阶段PM2.5浓度和相对湿度与能见度间的关系发现,霾阶段两因子影响力相当;雾阶段能见度主要受相对湿度的影响;静稳条件下PM2.5浓度累积增加是影响雾、霾混合阶段能见度的主要因子。  相似文献   

17.
导致空气质量变差的天气,并非只有雾和霾,还有沙尘暴、扬沙、浮尘等天气。为更好地掌握咸阳地区空气质量的时空变化特征,从而为政府治污降霾提供有力依据,将气象观测中能见度小于10 km的雾、霾、沙尘暴、扬沙、浮尘等影响空气质量的天气,统一定义为“广义雾霾日”,并将其划分为轻微、轻度、中度和重度4个等级。通过研究发现,咸阳市区“广义雾霾日”与实际污染日数的相关性比普通雾霾日的相关性更好,能更好地反映空气质量的变化状况。咸阳市区能见度与空气质量监测数据之间存在较明显的对数负相关关系,即能见度越小空气质量越差,能见度越大空气质量越好,故“广义雾霾日”可在一定程度上反映咸阳地区的空气质量状况。空间变化上,咸阳地区的“广义雾霾日”空间分布呈现由南向北递减的趋势,兴平的最多,旬邑的最少。时间变化上,市区和旬邑“广义雾霾日”年际变化呈现减少的趋势,兴平的年际变化不明显,乾县的年际变化呈现增多的趋势。市区的“广义雾霾日”在10月至次年1月间较多,此期间恰好是市区风速较小、降水较少的时段;而“广义雾霾日”较少的时段内,市区的风速较高,降水较多。在“广义雾霾日”出现较多的时段内,重度等级日数明显增多。  相似文献   

18.
一次持续性雾霾天气过程的阶段性特征及影响因子分析   总被引：4，自引：0，他引：4  
苗爱梅  李苗  王洪霞 《干旱气象》2014,32(6):947-953
应用常规与非常规气象观测资料及PM2.5浓度监测资料,对2013年1月20~24日山西区域一次持续性雾霾天气过程进行分析。研究发现：（1）本次雾霾天气过程具有明显的阶段性特征。2013年1月20日14时至23日11时,由于相对湿度的变化导致了3次轻雾转大雾过程;23日14~20时,由于PM2.5浓度的增大经历了1次轻雾转霾的天气过程。（2）地面弱的气压场和较小的风速以及PM2.5浓度的上升和相对湿度的增大为本次持续性雾霾天气过程的形成和发展提供了有利条件。（3）边界层逆温的存在是雾霾低能见度过程形成的必要条件,边界层有逆温层而不出现雾霾天气的条件是：相对湿度〈50%,PM2.5日均值浓度〈75μg·m-3;逆温层下相对湿度的大小是区别雾和霾天气的指标。（4）相对湿度和PM2.5是决定能见度大小的关键因子,其对能见度的影响体现出明显的阶段性特征,当相对湿度〈90%时,PM2.5浓度对能见度的作用强于相对湿度,是影响能见度变化的主要因子,但随着相对湿度的增大,其对能见度的影响相对增强,当能见度降至1 km以下时,相对湿度成为影响能见度变化的主要因子。  相似文献   

19.
霾与雾的区别和灰霾天气预警建议   总被引：44，自引：13，他引：44  
霾与雾的区分是目前一个非常现实 ,又迫切需要解决的问题。而过去东南沿海各省不成文规定的用相对湿度区分的标准普遍偏低 ,区分霾和雾 ,应该根据影响天气系统的变化 ,结合各种判据来确定。考虑到近几年对气溶胶研究的新成果 ,大气中 0 .1μm以下的水溶性粒子主要是 (NH4) 2 SO4等组成的 ,>1μm的粒子主要是NaCl等组成的。这些物质的相变湿度大都在 80 %左右。建议将相对湿度<80 %时的大气混浊视野模糊导致的能见度恶化的天气现象确定为霾 ,相对湿度 >90 %时的大气混浊视野模糊导致的能见度恶化确定为雾 ,相对湿度介于 80～ 90 %之间时的大气混浊视野模糊导致的能见度恶化是霾和雾的混合物共同造成的 ,但其主要成分应该是霾。建议尽快制定灰霾指数和预警办法 ,开展灰霾天气预测预报预警方法的研究和业务平台建设 ,拓展气象服务领域 ,使环境气象产品更好地为社会公众服务 ,为政府实行动态调控的环保措施的决策服务。  相似文献   

20.
北京市持续重污染天气分析   总被引：7，自引：0，他引：7  
通过对2004-2008年北京市空气持续重污染过程的统计及其对非沙尘型持续重污染天气形势的特征分析,得到以下结论：持续重污染过程具有明显的季节分布特征,主要包括春季沙尘型污染和秋冬季节非沙尘型污染;非沙尘型持续重污染过程期间多对应着大雾、轻雾、霾、烟等低能见度天气,过程后期对应的天气现象多为大风或降水天气。其中大雾天气更易引发长时间持续的空气重污染事件。非沙尘型持续重污染的天气形势特点为：高空多为纬向环流,850 hPa多为暖脊控制,地面多处于弱气压场,鞍形场型污染尤为严重。北京持续重污染多对应区域性污染。  相似文献   

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