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1.
Sergio Pacca 《Climatic change》2007,84(3-4):281-294
Greenhouse gas (GHG) emissions from hydroelectric dams are often portrayed as nonexistent by the hydropower industry and have been largely ignored in global comparisons of different sources of electricity. However, the life cycle assessment (LCA) of any hydroelectric plant shows that GHG emissions occur at different phases of the power plant’s life. This work examines the role of decommissioning hydroelectric dams in greenhouse gas emissions. Accumulated sediments in reservoirs contain noticeable levels of carbon, which may be released to the atmosphere upon decommissioning of the dam. The rate of sediment accumulation and the sediment volume for six of the ten largest United States hydroelectric power plants is surveyed. The amount of sediments and the respective carbon content at the moment of dam decommissioning (100 years after construction) was estimated. The released carbon is partitioned into CO2 and CH4 emissions and converted to CO2 equivalent emissions using the global warming potential (GWP) method. The global warming effect (GWE) due to dam decommissioning is normalized to the total electricity produced over the lifetime of each power plant. The estimated GWE of the power plants range from 128–380 g of CO2eq./kWh when 11% of the total available sediment organic carbon (SOC) is mineralized and between 35 and 104 g of CO2eq./kWh when 3% of the total SOC is mineralized. Though these values are below emission factors for coal power plants (890 g of CO2eq./kWh), the amount of greenhouse gases emitted by the sediments upon dam decommissioning is a notable amount that should not be ignored and must be taken into account when considering construction and relicensing of hydroelectric dams.  相似文献   

2.
Substitution of natural gas for coal is one means of reducing carbon dioxide (CO2) emissions. However, natural gas and coal use also results in emissions of other radiatively active substances including methane (CH4), sulfur dioxide (SO2), a sulfate aerosolprecursor, and black carbon (BC) particles. Will switching from coal to gas reduce the net impact of fossil fuel use on global climate? Using the electric utility sector as an example, changes in emissions of CO2, CH4,SO2 and BC resulting from the replacement of coal by natural gas are evaluated, and their modeled net effect on global mean-annual temperature calculated. Coal-to-gas substitution initially produces higher temperatures relative to continued coal use. This warming is due to reduced SO2 emissionsand possible increases in CH4 emissions, and can last from 1 to 30years, depending on the sulfur controls assumed. This is followed by a net decrease in temperature relative to continued coal use, resulting from lower emissions of CO2 and BC. The length of this period and the extent of the warming or cooling expected from coal-to-gas substitution is found to depend on key uncertainties and characteristics of the substitutions, especially those related to: (1) SO2 emissions and consequentsulphate aerosol forcing; and (2) the relative efficiencies of the power plantsinvolved in the switch.  相似文献   

3.
Carbon dioxide, methane, and carbon monoxide are the carbon cycle gases, the data on their emissions are needed when monitoring air pollution and developing methods for reducing anthropogenic emissions to the atmosphere and for climate forecasting. The estimates of nocturnal area fluxes for CO2, CH4, and CO presented for a suburb of Saint Petersburg (Peterhof) are obtained using the box model and continuous observations of concentration of these gases. The mean values of CH4, CO2, and CO fluxes estimated for Peterhof for 2014–2015 are 44 ± 27, 6100 ± 4000, and 90 ± 100 t/(km2 year), respectively. The intensity of the CO area flux has pronounced seasonal variations characterized by the maximum of ~(160 ± 120) t/(km2 year) in November—February and by the minimum of ~(30 ± 20) t/(km2 year) in June-July. The analysis of the ratio of CO/CO2 fluxes identified the main types of anthropogenic sources typical of Peterhof: motor transport, natural gas combustion, and the use of wood stoves for the heating of private low-rise buildings (in the cold season).  相似文献   

4.
We use recent advances in time series econometrics to estimate the relation among emissions of CO2 and CH4, the concentration of these gases, and global surface temperature. These models are estimated and specified to answer two questions; (1) does human activity affect global surface temperature and; (2) does global surface temperature affect the atmospheric concentration of carbon dioxide and/or methane. Regression results provide direct evidence for a statistically meaningful relation between radiative forcing and global surface temperature. A simple model based on these results indicates that greenhouse gases and anthropogenic sulfur emissions are largely responsible for the change in temperature over the last 130 years. The regression results also indicate that increases in surface temperature since 1870 have changed the flow of carbon dioxide to and from the atmosphere in a way that increases its atmospheric concentration. Finally, the regression results for methane hint that higher temperatures may increase its atmospheric concentration, but this effect is not estimated precisely.  相似文献   

5.
Fifty flask air samples were taken during April 1986 from a NOAA WP-3D Orion aircraft which flew missions across a broad region of the Arctic as part of the second Arctic Gas and Aerosol Sampling Program (AGASP II). The samples were subsequently analyzed for both carbon dioxide (CO2) and methane (CH4). The samples were taken in well-defined layers of Arctic haze, in the background troposphere where no haze was detected, and from near the surface to the lower stratosphere. Vertical profiles were specifically measured in the vicinity of Barrow, Alaska to enable comparisons with routine surface measurements made at the NOAA/GMCC observatory. Elevated levels of both methane and carbon dioxide were found in haze layers. For samples taken in the background troposphere we found negative vertical gradients (lower concentrations aloft) for both gases. For the entire data set (including samples collected in the haze layers) we found a strong positive correlation between the methane and carbon dioxide concentrations, with a linear regression slope of 17.5 ppb CH4/ppm CO2, a standard error of 0.6, and a correlation coefficient (r2) of 0.95. This correlation between the two gases seen in the aircraft samples was corroborated by in situ surface measurements of these gases made at the Barrow observatory during March and April 1986. We also find a similar relationship between methane and carbon dioxide measured concurrenty for a short period in the moderately polluted urban atmosphere of Boulder, Colorado. We suggest that the strong correlation between methane and carbon dioxide concentrations reflects a common source region for both, with subsequent long-range transport of the polluted air to the Arctic.  相似文献   

6.
Minimizing the future impacts of climate change requires reducing the greenhouse gas (GHG) load in the atmosphere. Anthropogenic emissions include many types of GHG’s as well as particulates such as black carbon and sulfate aerosols, each of which has a different effect on the atmosphere, and a different atmospheric lifetime. Several recent studies have advocated for the importance of short timescales when comparing the climate impact of different climate pollutants, placing a high relative value on short-lived pollutants, such as methane (CH4) and black carbon (BC) versus carbon dioxide (CO2). These studies have generated confusion over how to value changes in temperature that occur over short versus long timescales. We show the temperature changes that result from exchanging CO2 for CH4 using a variety of commonly suggested metrics to illustrate the trade-offs involved in potential carbon trading mechanisms that place a high value on CH4 emissions. Reducing CH4 emissions today would lead to a climate cooling of approximately ~0.5 °C, but this value will not change greatly if we delay reducing CH4 emissions by years or decades. This is not true for CO2, for which the climate is influenced by cumulative emissions. Any delay in reducing CO2 emissions is likely to lead to higher cumulative emissions, and more warming. The exact warming resulting from this delay depends on the trajectory of future CO2 emissions but using one business-as usual-projection we estimate an increase of 3/4 °C for every 15-year delay in CO2 mitigation. Overvaluing the influence of CH4 emissions on climate could easily result in our “locking” the earth into a warmer temperature trajectory, one that is temporarily masked by the short-term cooling effects of the CH4 reductions, but then persists for many generations.  相似文献   

7.
Carbon dioxide (CO2) emissions from fossil fuel combustion may be reduced by using natural gas rather than coal to produce energy. Gas produces approximately half the amount of CO2 per unit of primary energy compared with coal. Here we consider a scenario where a fraction of coal usage is replaced by natural gas (i.e., methane, CH4) over a given time period, and where a percentage of the gas production is assumed to leak into the atmosphere. The additional CH4 from leakage adds to the radiative forcing of the climate system, offsetting the reduction in CO2 forcing that accompanies the transition from coal to gas. We also consider the effects of: methane leakage from coal mining; changes in radiative forcing due to changes in the emissions of sulfur dioxide and carbonaceous aerosols; and differences in the efficiency of electricity production between coal- and gas-fired power generation. On balance, these factors more than offset the reduction in warming due to reduced CO2 emissions. When gas replaces coal there is additional warming out to 2,050 with an assumed leakage rate of 0%, and out to 2,140 if the leakage rate is as high as 10%. The overall effects on global-mean temperature over the 21st century, however, are small.  相似文献   

8.
Strategies for mitigating the increasing concentration of carbon dioxide (CO2) in the atmosphere include sequestering carbon (C) in soils and vegetation of terrestrial ecosystems. Carbon and nitrogen (N) move through terrestrial ecosystems in coupled biogeochemical cycles, and increasing C stocks in soils and vegetation will have an impact on the N cycle. We conducted simulations with a biogeochemical model to evaluate the impact of different cropland management strategies on the coupled cycles of C and N, with special emphasis on C-sequestration and emission of the greenhouse gases methane (CH4) and nitrous oxide (N2O). Reduced tillage, enhanced crop residue incorporation, and farmyard manure application each increased soil C-sequestration, increased N2O emissions, and had little effect on CH4 uptake. Over 20 years, increases in N2O emissions, which were converted into CO2-equivalent emissions with 100-year global warming potential multipliers, offset 75–310% of the carbon sequestered, depending on the scenario. Quantification of these types of biogeochemical interactions must be incorporated into assessment frameworks and trading mechanisms to accurately evaluate the value of agricultural systems in strategies for climate protection.  相似文献   

9.
Anthropogenic emissions of methane (CH4) and nitrous oxide (N2O) from livestock agriculture (enteric fermentation, animal waste management systems, and pasture manure) and plant growing of the Russia (CH4 emissions from rice fields, direct and indirect N2O emissions from agricultural lands) are considered. In 2004, the total emissions of these greenhouse gases in the agricultural sector amounted to 1.4 × 105 thousand t CO2-equivalent, which corresponds to 45% of the 1990 level (3.1 × 105 thousand t CO2-equivalent). In 2004, the contribution of N2O to the total agricultural emissions was approximately twice (67.0%) that of CH4 (33.0%). Direct N2O emissions from agricultural soils (0.5 × 105 thousand t CO2-equivalent) and CH4 emissions from the internal fermentation of domestic animals (0.4 × 105 thousand t CO2-equivalent) are the most significant sources in the agricultural sector of the Russian Federation. In 2004, all these agricultural sources emitting methane and nitrous oxide contributed about 7% CO2-equivalent to the total emission of the anthropogenic greenhouse gases in Russia.  相似文献   

10.
Presented is the assessment of the contribution that such major types of the land use in Russia as arable lands, forage lands, settlements, and peatery make to anthropogenic fluxes of carbon dioxide CO2, methane CH4, and nitrogen oxide N2O, The assessment is based on the methods of computation monitoring carried out in the period from 2000 to 2011. The results of the study demonstrated that every year arable lands cause the emission of CO2 and N2O of about 117.0 and 74.9 million t CO2 equiv, and peatery, 0.54 and 105.4 thousand t CO2 equiv, respectively. The balance of soil carbon in hayfields and pastures is close to zero. The average emissions of CH4 and N2O from the manure of pasture animals amount to 0.2 and 5.0 million t CO2 equiv/year, and those from grass fires, 276.1 and 372.5 thousand t CO2 equiv/year, respectively. The carbon balance in permanent soils of settlements is also almost close to zero, and newly built-up lands are the source of CO2 (9.5 million t/year). The natural overgrowing of fallow lands leads to the accumulation of the soil carbon (about 92.4 million t CO2/year). It was revealed that the intensity of CO2 emission is defined by the soil carbon balance and that of other gases, by the amount of nitrogen fertilizers, plant residues, and manure coming to the soil. The total emission from the land use is 106.9 million t CO2 equiv/year that makes up 4.9% of the total anthropogenic emission of greenhouse gases in the Russian Federation.  相似文献   

11.
Emissions from Russian domestic civil aviation for the period of 2000–2012 are assessed for the following gases: carbon dioxide, methane, nitrous oxide, carbon monoxide, nitrogen oxides, and sulfur dioxide. The integrated assessment of their impact on the climate system is performed using the values of the global warming potential. The CO2 equivalent was used as a common measure of emissions. It is established that the modern impact of Russian civil aviation on the Earth climate is insignificant.  相似文献   

12.
The greenhouse gases emission (CO2, CH4, and N2O) from domestic and international aviation in the Russian Federation is assessed. In 2007, the total emission of CO2, CH4, and N2O amounted to 18.4 million tons of CO2-equivalent, which is 21% below the 1990 level. Carbon dioxide dominates in the component composition of the emissions, its part in 2007 accounted for 99.1% of the emission. Taking into account the tendency towards increasing fuel consumption due to intense aircraft traffic it can be expected that compared to the present level the greenhouse gases emissions in 2012 and 2020 will increase by 15 and 45%, respectively. Accounting for the increased aircraft emissions as well as plans of foreign countries to include the international aviation into the scheme of greenhouse gases emission allowance (trade credits) it is expedient to make more precise the greenhouse gases emissions from the Russian aviation based on the detailed flight data for all types of the aircraft.  相似文献   

13.
Richard Heede 《Climatic change》2014,122(1-2):229-241
This paper presents a quantitative analysis of the historic fossil fuel and cement production records of the 50 leading investor-owned, 31 state-owned, and 9 nation-state producers of oil, natural gas, coal, and cement from as early as 1854 to 2010. This analysis traces emissions totaling 914 GtCO2e—63 % of cumulative worldwide emissions of industrial CO2 and methane between 1751 and 2010—to the 90 “carbon major” entities based on the carbon content of marketed hydrocarbon fuels (subtracting for non-energy uses), process CO2 from cement manufacture, CO2 from flaring, venting, and own fuel use, and fugitive or vented methane. Cumulatively, emissions of 315 GtCO2e have been traced to investor-owned entities, 288 GtCO2e to state-owned enterprises, and 312 GtCO2e to nation-states. Of these emissions, half has been emitted since 1986. The carbon major entities possess fossil fuel reserves that will, if produced and emitted, intensify anthropogenic climate change. The purpose of the analysis is to understand the historic emissions as a factual matter, and to invite consideration of their possible relevance to public policy.  相似文献   

14.
A global two-dimensional (altitude-latitude) chemistry transport model is used to follow the changes in the tropospheric distribution of the two major radiatively active trace gases, methane and ozone, following step changes to the sustained emissions of the short-lived trace gases methane, carbon monoxide and non-methane hydrocarbons. The radiative impacts were dependent on the latitude chosen for the applied change in emissions. Step change global warming potentials (GWPs) were derived for a range of short-lived trace gases to describe their time-integrated radiative forcing impacts for unit emissions relative to that of carbon dioxide. The GWPs show that the tropospheric chemistry of the hydrocarbons can produce significant indirect radiative impacts through changing the tropospheric distributions of hydroxyl radicals, methane and ozone. For aircraft, the indirect radiative forcing impact of the NO x emissions appears to be greater than that from their carbon dioxide emissions. Quantitative results from this two-dimensional model study must, however, be viewed against the known inadequacies of zonally-averaged models and their poor representation of many important tropospheric processes.  相似文献   

15.
The MAGICC (Model for the Assessment of Greenhouse gas Induced Climate Change) model simulation has been carried out for the 2000–2100 period to investigate the impacts of future Indian greenhouse gas emission scenarios on the atmospheric concentrations of carbon dioxide, methane and nitrous oxide besides other parameters like radiative forcing and temperature. For this purpose, the default global GHG (Greenhouse Gases) inventory was modified by incorporation of Indian GHG emission inventories which have been developed using three different approaches namely (a) Business-As-Usual (BAU) approach, (b) Best Case Scenario (BCS) approach and (c) Economy approach (involving the country’s GDP). The model outputs obtained using these modified GHG inventories are compared with various default model scenarios such as A1B, A2, B1, B2 scenarios of AIM (Asia-Pacific Integrated Model) and P50 scenario (median of 35 scenarios given in MAGICC). The differences in the range of output values for the default case scenarios (i.e., using the GHG inventories built into the model) vis-à-vis modified approach which incorporated India-specific emission inventories for AIM and P50 are quite appreciable for most of the modeled parameters. A reduction of 7% and 9% in global carbon dioxide (CO2) emissions has been observed respectively for the years 2050 and 2100. Global methane (CH4) and global nitrous oxide (N2O) emissions indicate a reduction of 13% and 15% respectively for 2100. Correspondingly, global concentrations of CO2, CH4 and N2O are estimated to reduce by about 4%, 4% and 1% respectively. Radiative forcing of CO2, CH4 and N2O indicate reductions of 6%, 14% and 4% respectively for the year 2100. Global annual mean temperature change (incorporating aerosol effects) gets reduced by 4% in 2100. Global annual mean temperature change reduces by 5% in 2100 when aerosol effects have been excluded. In addition to the above, the Indian contributions in global CO2, CH4 and N2O emissions have also been assessed by India Excluded (IE) scenario. Indian contribution in global CO2 emissions was observed in the range of 10%–26%, 6%–36% and 10%–38% respectively for BCS, Economy and BAU approaches, for the years 2020, 2050 and 2100 for P50, A1B-AIM, A2-AIM, B1-AIM & B2-AIM scenarios. CH4 and N2O emissions indicate about 4%–10% and 2%–3% contributions respectively in the global CH4 and N2O emissions for the years 2020, 2050 and 2100. These Indian GHG emissions have significant influence on global GHG concentrations and consequently on climate parameters like RF and ∆T. The study reflects not only the importance of Indian emissions in the global context but also underlines the need of incorporation of country specific GHG emissions in modeling to reduce uncertainties in simulation of climate change parameters.  相似文献   

16.
The ongoing human-induced emission of carbon dioxide (CO2) threatens to change the earth's climate. One possible way of decreasing CO2 emissions is to apply CO2 removal, which involves recovering of carbon dioxide from energy conversion processes and storing it outside the atmosphere. Since the 1980's, the possibilities for recovering CO2 from thermal power plants received increasing attention.In this study possible techniques of recovering CO2 from large-scale industrial processes are assessed.In some industrial processes, e.g. ammonia production, CO2 is recovered from the process streams to prevent it from interfering with the production process. The CO2 thus recovered can easily be dehydrated and compressed, at low cost. In the iron and steel industry, carbon dioxide can be recovered from blast furnace gas. In the petrochemical industry CO2 can be recovered from flue gases, using low-temperature heat for the separation process.Carbon dioxide can be recovered from large-scale industrial processes and in some cases the cost of recovery is significantly less than CO2 recovery from thermal power plants. Therefore this option should be studied further and should be considered if carbon dioxide removal is introduced on a wide scale.  相似文献   

17.
A complex approach is considered to the estimation of emissions of carbon gases formed during wildfires in the middle taiga subzone in the Yenisei region of Siberia. Based on the large-scale Siberian wildfires in 2012, the relative contribution of emissions to the values of background concentration of carbon gases (CO2, CH4, CO) in the atmospheric boundary layer measured at the 300-m ZOTTO tall tower is assessed. The degree of ecosystem damage caused by wildfires is estimated depending on their intensity and combustion phase (flame or flameless). Emission factors are calculated for the major carbon gases in wildfire plumes which are the key component for assessing wildfire emissions to the atmosphere.  相似文献   

18.
This paper identifies a critical systematic error in greenhouse gas accounting in renewable biomass systems. While CO2 emissions from renewable biomass energy systems are generally considered to have a net impact of 0, no similar adjustment is made for carbon-based products of incomplete combustion, such as methane, in renewable systems. This results in an under- or overestimation of the impact of CH4 by 12.3% and CO by ∼478% in renewable systems. This error is propagated both in scientific studies and in carbon accounting policies. We advocate first for full-carbon accounting of biomass-derived emissions, but also provide adjusted global warming impacts for emissions from proven renewable systems.  相似文献   

19.
Measurements of carbon dioxide(CO2), methane(CH4), and carbon monoxide(CO) are of great importance in the Qinghai-Tibetan region, as it is the highest and largest plateau in the world affecting global weather and climate systems. In this study, for the first time, we present CO2, CH4, and CO column measurements carried out by a Bruker EM27/SUN Fourier-transform infrared spectrometer(FTIR) at Golmud(36.42°E, 94.91°N, 2808 m) in August 2021. The mean and...  相似文献   

20.
Biotic Feedbacks in the Warming of the Earth   总被引：16，自引：0，他引：16  
A positive correlation exists between temperature and atmospheric concentrations of carbon dioxide and methane over the last 220,000 years of glacial history, including two glacial and three interglacial periods. A similar correlation exists for the Little Ice Age and for contemporary data. Although the dominant processes responsible may be different over the three time periods, a warming trend, once established, appears to be consistently reinforced through the further accumulation of heat-trapping gases in the atmosphere; a cooling trend is reinforced by a reduction in the release of heat-trapping gases. Over relatively short periods of years to decades, the correspondence between temperature and greenhouse gas concentrations may be due largely to changes in the metabolism of terrestrial ecosystems, whose respiration, including microbial respiration in soils, responds more sensitively, and with a greater total effect, to changes in temperature than does gross photosynthesis. Despite the importance of positive feedbacks and the recent rise in surface temperatures, terrestrial ecosystems seem to have been accumulating carbon over the last decades. The mechanisms responsible are thought to include increased nitrogen mobilization as a result of human activities, and two negative feedbacks: CO2 fertilization and the warming of the earth, itself, which is thought to lead to an accumulation of carbon on land through increased mineralization of nutrients and, as a result, increased plant growth. The relative importance of these mechanisms is unknown, but collectively they appear to have been more important over the last century than a positive feedback through warming-enhanced respiration. The recent rate of increase in temperature, however, leads to concern that we are entering a new phase in climate, one in which the enhanced greenhouse effect is emerging as the dominant influence on the temperature of the earth. Two observations support this concern. One is the negative correlation between temperature and global uptake of carbon by terrestrial ecosystems. The second is the positive correlation between temperature and the heat-trapping gas content of the atmosphere. While CO2 fertilization or nitrogen mobilization (either directly or through a warming-enhanced mineralization) may partially counter the effects of a warming-enhanced respiration, the effect of temperature on the metabolism of terrestrial ecosystems suggests that these processes will not entirely compensate for emissions of carbon resulting directly from industrial and land-use practices and indirectly from the warming itself. The magnitude of the positive feedback, releasing additional CO2, CH4, and N2O, is potentially large enough to affect the rate of warming significantly.  相似文献   

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