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1.
Past studies based on the NOAA/AVHRR and GOES I-M imager instruments have documented the link between certain storm top features referred to as the “cold-U/V” shape in the 10–12 μm IR band imagery and plumes of increased 3.7/3.9 μm band reflectivity. Later, similar features in the 3.7/3.9 μm band have been documented in the AVHRR/3 1.6 μm band imagery.The present work focuses on storm top observations utilizing the MODIS data. The MODIS instrument (available onboard NASA's EOS Terra and Aqua satellites) provides image data with significantly better geometrical resolution (in some of its bands) and broader range of spectral bands as compared to that from AVHRR/3 observations. One of the goals of this study is to evaluate the contribution of this new instrument to observations of convective storm tops. Besides the cloud top features linked to storm top microphysics and morphology, the paper also addresses the possibility of detection of lower stratospheric water vapor above cold convective storm tops. This issue is explored utilizing MODIS as well as GOES and MSG imagery.In addition, the paper discusses an alternative interpretation of the “cold-U/V” patterns at the top of intense storms by a mechanism of “plume masking” as suggested by some of the observations.  相似文献   

2.
The changing chemical composition of cloud water and precipitation in the Western Sudety Mountains are discussed against the background of air-pollution changes in the Black Triangle since the 1980s until September 2004. A marked reduction of sulphur dioxide emissions between the early 1990's and the present (from almost 2 million tons to around 0.2 million tons) has been observed, with a substantial decline of sulphate and hydrogen concentration in cloud water (SO42− from more than 200 to around 70 μmol l− 1; H+ from 150 to 50 μmol l− 1) and precipitation (SO42− from around 80 to 20–30 μmol l− 1; H+ from around 60 to 10–15 μmol l− 1) samples. At some sites, where fog/cloud becomes the major source of pollutants, deposition hot spots are still observed where, for example, nitrogen deposition can exceed 20 times the relevant critical load. The results show that monitoring of cloud water chemistry can be a sensitive indicator of pollutant emissions.  相似文献   

3.
On February 8, 1993, the NASA DC-8 aircraft profiled from 10,000 to 37,000 feet (3.1–11.3 km) pressure altitude in a stratified section of tropical cyclone “Oliver” over the Coral Sea northeast of Australia. Size, shape and phase of cloud and precipitation particles were measured with a 2-D Greyscale probe. Cloud/ precipitation particles changed from liquid to ice as soon as the freezing level was reached near 17,000 feet (5.2 km) pressure altitude. The cloud was completely glaciated at −5°C. There was no correlation between ice particle habit and ambient temperature. In the liquid phase, the precipitation-cloud drop concentration was 4.0 × 103 m−3, the geometric mean diameter Dg=0.5−0.7 mm, and the liquid water content 0.7−1.9 g m−3. The largest particles anywhere in the cloud, dominated by fused dendrites at concentrations similar to that of raindrops (2.5 × 103 m−3) but a higher condensed water content (5.4 g m−3 estimated) were found in the mixed phase; condensed water is removed very effectively from the mixed layer due to high settling velocities of the large mixed particles. The highest number concentration (4.9 × 104 m−3), smallest size (Dg=0.3−0.4 mm), largest surface area (up to 2.6 × 102 cm2 m−3 at 0.4−1.0 g m−3 of condensate) existed in the ice phase at the coldest temperature (−40°C) at 35,000 feet (10.7 km). Each cloud contained aerosol (haze particles) in addition to cloud particles. The aerosol total surface area exceeded that of the cirrus particles at the coldest temperature. Thus, aerosols must play a significant role in the upscattering of solar radiation. Light extinction (6.2 km−1) and backscatter (0.8 sr−1 km−1) was highest in the coldest portion of the cirrus cloud at the highest altitude.  相似文献   

4.
Physical experiments designed to explore the potential of rain augmentation through airborne glaciogenic seeding on small, isolated non-precipitating cumuliform clouds near Red Deer, Alberta were carried out during the period 1982–1985. The microstructure of 90 cumulus congestus clouds have been documented through repeated in-situ sampling using a cloud physics instrumented aircraft platform. Observations from the inspection passes of 57 clouds seeded with either dry ice pellets or silver iodide pyrotechnics, and all the passes of 33 natural clouds are presented.Measurements of the cloud droplet concentration indicate that Alberta cumulus clouds are typically continental in nature, with an average droplet concentration of 535 cm−3 and an average droplet diameter of 10.6 μm. Alberta clouds have average liquid water contents of 0.57 g m−3, with a peak 1-sec value of 3.17 g m−3. The 1-km average liquid water contents are 0.83 g m−3, with a peak value of 2.81 g m−3. Cloud lifetimes vary between 11 and 20 minutes. Concentrations of naturally occurring ice crystals are found to be low. The average maximum 1-km ice concentration was 31−1, and the peak 1-km concentration was 73.11−1 in the natural cloud dataset. Evidence of precipitation-sized particles was detected in 21% (7 of 33) of the clouds, and precipitation below cloud base was detected in 6% (2 of 33) of the clouds.A comparison of the Alberta cloud characteristics to the cumulus clouds from different locations showed that there are some distinct differences between Alberta clouds and the clouds from the other regions.  相似文献   

5.
Influence of drizzle on Z–M relationships in warm clouds   总被引：1，自引：0，他引：1  
This paper addresses the sensitivity of the relationships between radar reflectivity (Z) and liquid water content (M) for liquid water clouds to microphysical drizzle parameters by means of simulated radar observation at a frequency of 3 GHz of modeled cumulus clouds. A power law relationship for non drizzling clouds with water content as high as 3 gm− 3: Zc = 0.026 Mc1.61 is numerically derived and agreed with previous empirical relationships relative to cumulus and stratocumulus. This relationship is then used to explore the influence of drizzle on the correlation between radar reflectively and water content. Due to their large diameters with respect to cloud droplets, drizzle sized drops dominate radar reflectivity but do not carry the cloud water content so that reflectivity and liquid water content are expected to be not correlated in clouds containing drizzle. It is shown that for congestus or extreme congestus cumuli, microphysical conditions for which the Zc–Mc relationship can be used with a tolerance of 5 and 10% are provided whereas for humilis or mediocris cumuli, the presence of drizzle breaks down the Zc–Mc relationship whatever the situations.  相似文献   

6.
We present a parameterization for numbers of water and ammonia molecules in an equilibrium droplet with fixed number of sulfuric acid molecules at known relative humidity, ammonia mixing ratio and temperature. The radius of the droplet is also parameterized. The parameterizations are based on macroscopic model of solution droplets and up-to-date thermodynamics. The binary parameterizations are valid for temperatures 190–330 K and relative humidities 1–99%. The ternary parameterization can be used at temperatures 240–300 K, relative humidities 5–95%, and ammonia mixing ratios 10− 4–100 ppt. In both cases the parameterizations are valid for droplets containing up to 1011 sulfuric acid molecules. The droplet composition is always between the limits of pure ammonium bisulfate and pure ammonium sulfate.  相似文献   

7.
This paper documents a study to examine the sensitivity to cloud droplet effective radius and liquid water path and the alleviation the energy imbalance at the top of the atmosphere and at the surface in the latest version of the Grid-point Atmospheric Model of the State Key Laboratory of Numerical Modeling for Atmospheric Sciences and Geophysical Fluid Dynamics （LASG）, Institute of Atmospheric Physics （IAP） （GAMIL1.1.0）. Considerable negative biases in all flux components, and thus an energy imbalance, are found in GAMIL1.1.0. In order to alleviate the energy imbalance, two modifications, namely an increase in cloud droplet effective radius and a decrease in cloud liquid water path, have been made to the cloud properties used in GAMIL. With the increased cloud droplet effective radius, the single scattering albedo of clouds is reduced, and thus the reflection of solar radiation into space by clouds is reduced and the net solar radiation flux at the top of the atmosphere is increased. With the reduced cloud optical depth, the net surface shortwave radiation flux is increased, causing a net warming over the land surface. This results in an increase in both sensible and latent heat fluxes over the land regions, which is largely balanced by the increased terrestrial radiation fluxes. Consequently, the energy balance at the top of atmosphere and at the surface is achieved with energy flux components consistent with available satellite observations.  相似文献   

8.
Based on 1-year cloud measurements with radar and microwave radiometer broadband solar radiative transfer simulations were performed to quantify the impact of different ice crystal shapes of Arctic mixed-phase clouds on their radiative properties (reflectance, transmittance and absorptance). The ice crystal shape effects were investigated as a function of microphysical cloud properties (ice volume fraction fi, ice and liquid water content IWC and LWC, mean particle diameter DmI and DmW of ice/water particle number size distributions, NSDs).The required NSDs were statistically derived from radar data. The NSD was composed of a liquid and a solid mode defined by LWC, DmW (water mode) and IWC, DmI (ice mode). It was found that the ratio of DmI and DmW determines the magnitude of the shape effect. For mixed-phase clouds with DmI ≤ 27 μm a significant shape effect was obtained. The shape effect was almost insensitive with regard to the solar zenith angle, but highly sensitive to the ice volume fraction of the mixed-phase cloud. For mixed-phase clouds containing small ice crystals (DmI ≤ 27 μm) and high ice volume fractions (fi > 0.5) crystal shape is crucial. The largest shape effects were observed assuming aggregates and columns. If the IWC was conserved the shape effect reaches values up to 0.23 in cloud reflectance and transmittance. If the ice mode NSD was kept constant only a small shape effect was quantified (≤ 0.04).  相似文献   

9.
We examined microsecond- and submicrosecond-scale pulses in electric field records of cloud and cloud-to-ground lightning discharges acquired in summer 2006, in Gainesville, Florida. A total of 12 cloud and 12 ground flashes were analyzed in detail, with the electric field record length being 96 or 200 ms and sampling interval being 4 or 10 ns. The majority of pulses in both cloud and ground discharges analyzed in this study were associated with the initial breakdown process and were relatively small in amplitude and duration. The typical durations were an order of magnitude smaller than tens of microseconds characteristic of “classical” preliminary breakdown pulses. We estimated that 26% of the pulses in the 12 cloud discharges and 22% of the pulses in the 12 cloud-to-ground discharges had total durations less that 1 µs.  相似文献   

10.
Aqueous concentrations of ionic species observed in cloud water studies often have been in conflict with expectations from model predictions. These inconsistencies result from the size-dependent chemical composition of cloud drops during different stages in the lifetime of a cloud. To study this phenomenon, droplets of clouds need to be collected in different size ranges with high resolution in space and time. The only possibility for this kind of study is the use of an aircraft. Therefore, during the last several years, an attempt was made to develop a mobile cascade impactor, which can be installed outside an aircraft. The cloud water sampled in different size fractions can be transferred into the interior of the aircraft during the measuring flight. The collector is able to sample two size fractions. For continental clouds, the cutoffs are chosen to be >5 and >13.5 μm in diameter. For maritime clouds, the cutoff for the first stage could be shifted to 18.6 μm by lowering the nozzle speed. Prior to field application, the collector was characterized with the aid of “calibration fogs” produced in the laboratory with different drop sizes and different chemical compositions. The characterization included the examination of the cutoffs and the reliability of the sampling procedure with regard to the subsequent chemical analysis. With a collection period of 2 min, collection rates in the order of 0.1–1 cm3 min−1 can be obtained. The collector characterized in this manner was successfully used during measuring flights in clouds over northern Germany. Preliminary concentrations of NH4+, SO42− and Cl− found in the two size fractions of the cloud drops are presented.  相似文献   

11.
A two-dimensional cloud model with bin microphysics was used to investigate the effects of cloud condensation nuclei (CCN) concentrations and thermodynamic conditions on convective cloud and precipitation developments. Two different initial cloud droplet spectra were prescribed based on the total CCN concentrations of maritime (300 cm− 3) and continental (1000 cm− 3) air masses, and the model was run on eight thermodynamic conditions obtained from observational soundings. Six-hourly sounding data and 1-hourly precipitation data from two nearby weather stations in Korea were analyzed for the year 2002 to provide some observational support for the model results.For one small Convective Available Potential Energy (CAPE) ( 300 J kg− 1) sounding, the maritime and continental differences were incomparably large. The crucial difference was the production of ice phase hydrometeors in the maritime cloud and only water drops in the continental cloud. Ice phase hydrometeors and intrinsically large cloud drops of the maritime cloud eventually lead to significant precipitation. Meanwhile negligible precipitation developed from the continental cloud. For the three other small CAPE soundings, generally weak convective clouds developed but the maritime and continental clouds were of the same phases (both warm or both cold) and their differences were relatively small.Model runs with the four large CAPE ( 3000 J kg− 1) soundings demonstrated that the depth between the freezing level (FL) and the lifting condensation level (LCL) was crucial to determine whether a cloud becomes a cold cloud or not, which in turn was found to be a crucial factor to enhance cloud invigoration with the additional supply of freezing latent heat. For two large CAPE soundings, FL–LCL was so deep that penetration of FL was prohibitive, and precipitation was only mild in the maritime clouds and negligible in the continental clouds. Two other soundings of similarly large CAPE had small FL–LCL, and both the maritime and continental clouds became cold clouds. Precipitation was strong for both but much more so in the maritime clouds, while the maximum updraft velocity and the cloud top were slightly higher in continental clouds. Although limited to small CAPE cases, more precipitation for smaller FL–LCL for a selected group of precipitation and thermodynamic sounding data from Korea was in support of these model results in its tendency.These results clearly demonstrated that the CCN effects on cloud and precipitation developments critically depended on the given thermodynamic conditions and not just the CAPE but the entire structure of the thermodynamic profiles had to be taken into account.  相似文献   

12.
Analyses of cloud condensation nuclei (CCN) number concentrations (cm− 3) measured at the Mace Head Atmospheric Research Station, near Carna, County Galway, Ireland, using a DH Associates Model M1 static thermal diffusion cloud chamber over the period from March 1994 to September 2002 are presented in this work. Air masses are defined as being ‘marine’ if they originate from a wind direction of 180–300° and ‘continental’ air masses are defined as originating from a wind direction of 45–135°. Air masses without such filtering were classified as ‘undefined’ air masses. Air masses were found to be dominated by marine sector air, re-affirming Mace Head as a baseline atmospheric research station. CCN levels for specific air masses at Mace Head were found to be comparable with earlier studies both at Mace Head and elsewhere. Monthly averaged clean marine (wind direction of 180–300° and black carbon absorption coefficient < 1.425 Mm− 1) CCN and marine CCN varied between 15–247 cm− 3 and 54–670 cm− 3, respectively. As expected, significant increases in number concentration were found in continentally sourced CCN over that of marine CCN and were found to follow a log-normal distribution significantly tighter than that of clean marine air masses. No significant trend was found for CCN over the 9-year period. While polluted continental air masses showed a slight increase in CCN concentrations over the winter months, most likely due to increased fuel usage and a lower mixed boundary layer, the dominance of marine sector air arriving at Mace Head, which generally consists of background CCN concentrations, reduced seasonal differences for polluted air. Marine air showed a distinct seasonal pattern, with elevated values occurring over the spring and summer seasons. This is thought to be due to enhanced biogenic aerosol production as a result of phytoplankton bloom activity in the North Atlantic.  相似文献   

13.
In November 1993 an airborne field study was performed in order to investigate the microphysical and radiative properties of cooling tower water clouds initiated by water vapour emissions and polluted by the exhaust from coal-fired power plants. The number-median diameter of the droplet size distributions of these artificial clouds was in the range of 13 μm. The concentration of smaller droplets (diameters dD < 10 μm) increased with height and horizontal distance from the cooling towers. Close to the cooling towers, bimodal spectra were found with a second mode at 19 μm. The liquid water content (LWC) ranged between 2 and 5 g/m3 and effective droplet radii (Re) between 6 and 9 μm were measured. LWC and Re decreased with altitude, whereas the droplet concentration (ND) remained approximately constant (about 2000 cm−3 ). An enrichment of interstitial aerosol particles with particle diameters (dp) smaller 0.2 μm compared to the power plant plume in the vicinity of the clouds was observed. Particle activation for dm > 0.3 μm. was evident, especially in cooling tower clouds further apart and separated from their sources. Furthermore, radiation measurements were performed, which revealed differences in the vertical profiles of downwelling solar and UV radiation flux densities inside the clouds.The effective droplet radius Re was parameterized in terms of LWC and ND using equations known from literature. The close agreement between measured and parameterized Re indicates a similar coupling of Re, LWC and ND as in natural clouds.By means of Mie calculations, volume scattering coefficients and asymmetry factors are derived for both the cloud droplets and the aerosol particles. For the cloud droplets, the optical parameters were described by parameterizations from the literature. The results show, that the link between radiative and microphysical properties of natural clouds is not changed by the extreme pollution of the artificial clouds.  相似文献   

14.
The uppermost surface of the ocean forms a peculiarly important ecosystem, the sea surface microlayer (SML). Comprising the top 1–1000 μm of the ocean surface, the SML concentrates many chemical substances, particularly those that are surface active. Important economically as a nursery for fish eggs and larvae, the SML unfortunately is also especially vulnerable to pollution. Contaminants that settle out from the air, have low solubility, or attach to floatable matter tend to accumulate in the SML.Bubbles contribute prominently to the dynamics of air–sea exchanges, playing an important role in geochemical cycling of material in the upper ocean and SML. In addition to the movement of bubbles, the development of a bubble cloud interrelates with the single particle dynamics of all other bubbles and particles. In the early sixties, several in situ oceanographic techniques revealed an “unbelievably immense” number of coastal bubbles of radius 15–300 μm. The spatial and temporal variation of bubble numbers were studied; acoustical oceanographers now use bubbles as tracers to determine ocean processes near the ocean surface. Sea state and rain noises have both been definitively ascribed to the radiation from huge numbers of infant micro bubbles [The Acoustic Bubble. Academic Press, San Diego].Our research programme aims at constructing a hydrodynamic model for particle transport processes occurring at the microscale, in multi-phase flotation suspensions. Current research addresses bubble and floc microhydrodynamics as building blocks for a microscale transport model. This paper reviews sea surface transport processes in the microlayer and the lower atmosphere, and identifies those amenable to microhydrodynamic modelling and simulation. It presents preliminary simulation results including the multi-body hydrodynamic mobility functions for the modelling of “dynamic bubble filters” and floc suspensions. Hydrodynamic interactions versus spatial anisotropy and size of particle clouds are investigated.  相似文献   

15.
In a first attempt to assess a proposed climatic change feedback process involving cloud condensation nuclei (CCN) and cloud albedo, CCN concentrations N as a function of supersaturation S were measured on a voyage from latitude 43 to 65°S in October–November 1988. The usual relationship N=CSk, with k=0.5 and C a constant was a fair apprraximation for S in the range 0.3–0.7% implying that CCN concentrations should largely determine cloud drop concentrations and hence albedo for clouds with S in that range. South of latitude 50°S and at smaller S,k was 1 or larger on average, which would lead to reduced dependence of albedo on CCN for the relevant clouds. N varied very widely for separations of the order of 100 km or 6 hours in time, particularly when the sea was partly ice-covered, suggesting strong local influences. During a large increase in N 60°S, unaccompanied by an increase in condensation nuclei (CN), cloud drops grew more rapidly than usual. In a subsidiary experiment particles were collected and examined by transmission electron microscopy. For particles less than 0.2 μm diameter, 80–90% appeared to consist of ammonium sulfate, the remainder being sea salt or an unknown substance which was more liquid and heat-resistant. Dialysis showed that the sulfate particles contained a few percent of insoluble material. Particles which formed cloud drops in vapours other water, were also studied. Comparison of these and water CCN and the rates of droplet suggested that the water insoluble portion of the particles was ethanol-soluble and surface-active. CN concentrations decreased by a factor of about 2 between 43 and 65°S, a change closely paralleled by ethanol CCN concentrations.  相似文献   

16.
A field study was conducted at a mountain-top site in northwestern Colorado. Supercooled cloud water, collected as a function of droplet size, was analyzed for anions, cations and trace elements. Enrichment factors (EF) of SO 4 2– , K+, Na+ and Cl– relative to crustal and marine reference elements (Al and Na) were calculated to determine whether chemical fractionation of the aerosol occurs during cloud droplet formation. The largest EF's for all ions were found for droplets less than 10–15 µm diameter. Ratios of the small to large droplet mean EF's ranged from 1 to 2, for SO 4 2– relative to both Al and Na+, to 10 to 12 for Na+, Cl– and K+, relative to Al. EF's of K+ and Cl– in the bulk cloud water were in crustal and marine proportions, respectively. It was concluded that although bulk could chemistry may indicate a lack of enrichment of a species, this may not be true throughout the droplet size distribution. The higher enrichments in small droplets is likely a result of their formation on small aerosol particles whereas the large droplets form on the largest aerosol particles. This may suppress EF's in precipitation relative to the total aerosol.  相似文献   

17.
In this paper warm cloud microphysical parameters including cloud droplet number concentration (Nc), liquid water content (ql) and effective radius (re) from 75 flights around the Beijing area during 2005 and 2006 are summarized. Average Nc (cm− 3) for Cu, Sc, Ac, As and Ns are 376 ± 290, 257 ± 226, 147 ± 112, 60 ± 35 and 60 ± 84, respectively. Many records of high Nc above 1000 cm− 3 are observed. The large standard deviations indicate a large variation of Nc and ql in this region. The maxima of ql reach 1.4 g m− 3 in Cu and 1.0 g m− 3 in Sc, respectively. Different parameterizations of effective radius are examined with the in-situ data in this area. There are different ways to obtain the prefactor representing the relationship between effective radius and mean volume radius. Significant systematic errors are found to be at the large sizes when the prefactor is expressed with relative dispersion under the Gamma Distribution. Fixed prefactor of 1, which was widely used, even produces much larger error. A prefactor of 1.22 is found to be better than the former two methods by fitting with the observed data. The effective radius is further parameterized as functions of mean volume radius, liquid water content and cloud droplet number concentration. We suggest that the effective radius can be parameterized as re,p ≈ 1.20rv + 0.22–1.28/rv2, which is a practical and more accurate scheme without too much computation complexity.  相似文献   

18.
An index for fast thermodynamic cloud phase retrievals, the cloud phase index (CPI), is presented. The index is calculated by fitting the spectral slope of the reflectance around 1.6 μm. It is normalized with the reflectance at 1.64 μm in order to make the index insensitive to calibration constants. A selected set of observations by the Scanning Imaging Absorption Spectrometer for Atmospheric Chartography (SCIAMACHY), an instrument on board the ENVISAT platform, is used. Preliminary results are encouraging, showing a positive index between ≈25 and 50 for ice clouds.  相似文献   

19.
A falling droplet reactor was used to study the heterogeneous oxidation of gaseous PAH molecules adsorbed on a 92 μm diameter water droplet by ozone. The dynamic partition constant for the PAH between the droplet and air and the first-order surface rate constant was measured. The increase in uptake with ozone concentration was due to increased mass transfer via surface reaction of co-adsorbed ozone and PAH. The surface rate constant was rationalized through the Langmuir–Hinshelwood mechanism. The rate constant was smaller for phenanthrene than naphthalene. The main reaction products identified in the aqueous phase indicated the peroxidic route for surface reaction of ozone with PAH. The heterogeneous reaction rate of ozone with adsorbed phenanthrene at the air–water interface of a 92-μm droplet was estimated to be 9300 times larger than the homogeneous reaction of ozone with phenanthrene in the gas phase and it was 76 times larger than the homogeneous oxidation by hydroxyl radical in the gas phase. For naphthalene that is more volatile, however, the homogeneous reaction with hydroxyl was more important. Increased organic carbon added to the droplet increased both the partition constant for phenanthrene and surface reaction with ozone. The partition constant for a droplet formed from actual fog water was much larger than for pure distilled water.  相似文献   

20.
Transport safety is a major goal in the European Union. Low visibility conditions, especially due to fog, increase the risk of major accidents (chain collision). Innovative products have been developed by the automotive industry, including equipment manufacturers, to increase the level of safety of car passengers and drivers. Testing of these products requires the simulation or artificial reproduction of low visibility (fog) conditions with good stability and reproducibility characteristics. We report on the results of the European Union funded “FOG” project to improve road transport safety through fog production in an experimental test chamber located at the Clermont-Ferrand laboratory for research on road safety and visibility. The project developed a prototype of a small-scale climatic chamber, an improved fog production spraying device, a laser-based visibility measurement device, a reduced scale transmissometer, and a combined indoor climate-fog production simulation software. The ability of the fog chamber to test for driver reaction was also investigated. Recent developments include a device able to produce stable visibility levels and homogeneous fog, representative of various types of natural water droplet distribution. The fog characteristics were determined and compared to natural fog. Results are presented for a selection of conditions including stabilized visibility levels for dense fog and two kinds of droplet distributions.  相似文献   

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