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1.
The infrared radiative effect of methane was analyzed using the 2D, interactive chemical dynamical radiative SOCRATES model of the National Center for Atmospheric Research. Then, a sensitivity experi ment, with the methane volume mixing ratio increased by 10%, was carried out to study the influence of an increase of methane on air temperature. The results showed that methane has a heating effect through the infrared radiative process in the troposphere and a cooling effect in the stratosphere. However, the cooling effect of the methane is much smaller than that of water vapor in the stratosphere and is negligible in the mesosphere. The simulation results also showed that when methane concentration is increased by 10%, the air temperature lowers in the stratosphere and mesosphere and increases in the troposphere. The cooling can reach 0.2 K at the stratopause and can vary from 0.2-0.4 K in the mesosphere, and the temperature rise varies by around 0.001-0.002 K in the troposphere. The cooling results from the increase of the infrared radiative cooling rate caused by increased water vapor and O3 concentration, which are stimulated by the increase in methane in most of the stratosphere. The infrared radiation cooling of methane itself is minor. The depletion of O3 stimulated by the methane increase results indirectly in a decrease in the rate of so- lar radiation heating, producing cooling in the stratopause and mesosphere. The tropospheric warming is mainly caused by the increase of methane, which produces infrared radiative heating. The increase in H2O and O3 caused by the methane increase also contributes to a rise in temperature in the troposphere. 相似文献
2.
Impact of increasing stratospheric water vapor on ozone depletion and temperature change 总被引：2，自引：0，他引：2
Using a detailed, fully coupled chemistry climate model (CCM), the effect of increasing
stratospheric H2O on ozone and temperature is investigated. Different CCM time-slice runs have
been performed to investigate the chemical and radiative impacts of an assumed 2 ppmv increase in
H2O. The chemical effects of this H2O increase lead to an overall decrease of the total column ozone
(TCO) by ～1% in the tropics and by a maximum of 12% at southern high latitudes. At northern high
latitudes, the TCO is increased by only up to 5% due to stronger transport in the Arctic. A 2-ppmv H2O
increase in the model's radiation scheme causes a cooling of the tropical stratosphere of no more than 2 K,
but a cooling of more than 4 K at high latitudes. Consequently, the TCO is increased by about 2%--6%.
Increasing stratospheric H2O, therefore, cools the stratosphere both directly and indirectly, except in
the polar regions where the temperature responds differently due to feedbacks between ozone and H2O changes.
The combined chemical and radiative effects of increasing H2O may give rise to more cooling in the tropics
and middle latitudes but less cooling in the polar stratosphere. The combined effects of H2O increases on
ozone tend to offset each other, except in the Arctic stratosphere where both the radiative and chemical
impacts give rise to increased ozone. The chemical and radiative effects of increasing H2O cause dynamical
responses in the stratosphere with an evident hemispheric asymmetry. In terms of ozone recovery, increasing
the stratospheric H2O is likely to accelerate the recovery in the northern high latitudes and delay it in
the southern high latitudes. The modeled ozone recovery is more significant between 2000--2050 than between
2050--2100, driven mainly by the larger relative change in chlorine in the earlier period. 相似文献
3.
DEVELOPMENT OF THE 2-D COUPLED STRATOSPHERICTROPOSPHERIC DYNAMICAL-RADIATIVE-CHEMICAL MODEL—PART Ⅱ:THE RESULTS AND DISCUSSION OF SENSITIVITY EXPERIMENTS 
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下载免费PDF全文 By using the 2-D stratospheric-tropospheric dynamic-radiative-chemical coupled model,somesensitivity experiments have been done,which are interactions among ozone,radiation andtemperature,vapor effects,as well as effects of source and sink.The result of temperatureexperiment shows that feedback interaction among ozone,radiation and temperature,mainlyoccurs in the upper and middle stratosphere,the maximum of ozone concentration decrease is 1ppm,the maximum of temperature change is 6 K,and the maximum of total ozone change is 20DU.From the experiment of water vapor,we can see that the area of the middle and high latitudesof the Northern Hemisphere is sensitive to vapor change.When the maximum difference betweenboth surface sources is in the Antarctic,the maximum of ozone change is also there.Because thecharacter of surface varies with latitude,dry deposition is different in different latitudes.Thechange of dry deposition makes ozone in boundary layer quite obvious,especially in both poles.The maximum change of total volume ozone in experiments of vapor,source and sink is more than12 DU. 相似文献
4.
Both water vapor and heat processes play key roles in producing surface rainfall.While the water vapor effects of sea surface temperature and cloud radiative and microphysical processes on surface rainfall have been investigated in previous studies,the thermal effects on rainfall are analyzed in this study using a series of two-dimensional equilibrium cloud-resolving model experiments forced by zonally-uniform,constant,large-scale zonal wind and zero large-scale vertical velocity.The analysis of thermally-related surface rainfall budget reveals that the model domain mean surface rain rate is primarily associated with the mean infrared cooling rate.Convective rainfall and transport of hydrometeor concentration from convective regions to raining stratiform regions corresponds to the heat divergence over convective regions,whereas stratiform rainfall corresponds to the transport of hydrometeor concentration from convective regions and heat divergence over raining stratiform regions.The heat divergence over convective regions is mainly balanced by the heat convergence over rainfall-free regions,which is,in turn,offset by the radiative cooling over rainfall-free regions.The sensitivity experiments of rainfall to the effects of sea surface temperature and cloud radiative and microphysical processes show that the sea surface temperature and cloud processes affect convective rainfall through the changes in infrared cooling rate over rainfall-free regions and transport rate of heat from convective regions to rainfall-free regions. 相似文献
5.
Increasing greenhouse gases and likely ozone recovery will be the two most important factors influencing changes in stratospheric temperatures in the 21st century. The radiative effect of increasing greenhouse gases will cause cooling in the stratosphere, while ozone recovery will lead to stratospheric warming. To investigate how stratospheric temperatures change under the two opposite forcings in the 21st century, we use observed ozone and reanalysis data as well as simulation results from four coupled oceanic and atmo- spheric general circulation models （GISS-ER, GFDL-CM20, NCAR-CCSM3, and UKMO-HadCM3） used in the IPCC （Intergovernment Panel for Climate Change） Fourth Assessment Report （AR4）. Observational analysis shows that total column ozone and lower stratospheric temperatures all show increasing in the past 10 years, while middle stratospheric temperatures demonstrate cooling. IPCC AR4 simulations show that greenhouse forcing alone will lead to stratospheric cooling. However, with forcing of both increasing greenhouse gases and ozone recovery, the middle stratosphere will be cooled, while the lower stratosphere will be warmed. Warming magnitudes vary from one model to another. UKMO-HadCM3 generates relatively strong warming for all three greenhouse scenarios, and warming extends to 40 hPa. GFDL-CM20 and NCAR-CCSM3 produce weak warming, and warming mainly exists at lower levels, below about 60 hPa. In addition, we also discuss the effect of temperature changes on ozone recovery. 相似文献
6.
Air Temperature Changes over the Tibetan Plateau and Other Regions in the Same Latitudes and the Role of Ozone Depletion 总被引：3，自引：0，他引：3 下载免费PDF全文
下载免费PDF全文 Using radiosonde and satellite observations, we investigated the trends of air temperature changes over the Tibetan Plateau （TP） in comparison with those over other regions in the same latitudes from 1979 to 2002. It is shown that Over the TP, the trends of air temperature changes in the upper troposphere to lower stratosphere were out of phase with those in the lower to middle troposphere. Air temperature decreased and a decreasing trend appeared in the upper troposphere to lower stratosphere. The amplitude of the annual or seasonal mean temperature decreases over the TP was larger than that over the whole globe. In the lower to middle troposphere over the TP, temperature increased, and the increasing trend was stronger than that over the non-plateau regions in the same latitudes in the eastern part of China. Meanwhile, an analysis of the satellite observed ozone data in the same period of 1979-2002 shows that over the TP, the total ozone amount declined in all seasons, and the ozone depleted the most compared with the situations in other regions in the same latitudes. It is proposed that the difference between the ozone depletion over the TP and that over other regions in the same latitudes may lead to the difference in air temperature changes. Because of the aggravated depletion of ozone over the TP, less （more） ultraviolet radiation was absorbed in the upper troposphere to lower stratosphere （lower to middle troposphere） over the TP, which favored a stronger cooling in the upper troposphere to lower stratosphere, and an intenser heating in the lower to middle troposphere over the TP. Therefore, the comparatively more depletion of ozone over the TP is possibly a reason for the difference between the air temperature changes over the TP and those over other regions in the same latitudes. 相似文献
7.
Recent studies demonstrate that the Antarctic Ozone Hole has important influences on Antarctic sea ice.While most of these works have focused on effects associated with atmospheric and oceanic dynamic processes caused by stratospheric ozone changes,here we show that stratospheric ozone-induced cloud radiative effects also play important roles in causing changes in Antarctic sea ice.Our simulations demonstrate that the recovery of the Antarctic Ozone Hole causes decreases in clouds over Southern Hemisphere(SH)high latitudes and increases in clouds over the SH extratropics.The decrease in clouds leads to a reduction in downward infrared radiation,especially in austral autumn.This results in cooling of the Southern Ocean surface and increasing Antarctic sea ice.Surface cooling also involves ice-albedo feedback.Increasing sea ice reflects solar radiation and causes further cooling and more increases in Antarctic sea ice. 相似文献
8.
Middle Stratospheric Polar Vortex Ozone Budget during the Warming Arctic Winter, 2002--2003 总被引：1，自引：0，他引：1
The ozone budget inside the middle stratospheric polar vortex(24-36 km) during the 2002-2003 Arctic winter is studied by analyzing Michelson Interferometer for Passive Atmospheric Sounding(MIPAS) satellite data.A comprehensive global chemical transport model(Model for Ozone and Related Chemical Tracers,MOZART-3) is used to analyze the observed variation in polar vortex ozone during the stratospheric sudden warming(SSW) events.Both MIPAS measurement and MOZART-3 calculation show that a pronounced increase(26-28 DU) in the polar vortex ozone due to the SSW events.Due to the weakening of the polar vortex,the exchange of ozone mass across the edge of the polar vortex increases substantially and amounts to about 3.0× 107 kg according to MOZART-3 calculation.The enhanced downward transport offsets about 80% of polar vortex ozone mass increase by horizontal transport.A "passive ozone" experiment shows that only ～55% of the vertical ozone mass flux in February and March can be attributed to the variation in vertical transport.It is also shown that the enhanced downward ozone above ～32 km should be attributed to the springtime photochemical ozone production.Due to the increase of air temperature,the NOx reaction rate increases by 40%-80% during the SSW events.As a result,NOx catalytic cycle causes another 44% decrease in polar vortex ozone compared to the net ozone changes due to dynamical transport.It is also shown that the largest change in polar vortex ozone is due to horizontal advection by planetary waves in January 2003. 相似文献
9.
Using the measurements from the Halogen Occultation Experiment(HALOE) and the European Centre for Medium-Range Weather Forecasts(ECMWF) Interim reanalysis data for the period 1994-2005, we analyzed the relationship between tropical tropopause temperature anomalies and stratospheric water vapor anomalies. It is found that tropical tropopause temperature is correlated with stratospheric water vapor, i.e., an anomalously high(low) tropical tropopause temperature corresponds to anomalously high(low) stratospheric water vapor during the period 1994-2005,except for 1996. The occurrence frequency and strength of deep convective activity during the‘mismatched'months is less and weaker than that during the‘matched'months in 1996. However, the instantaneous intensity of four short periods of deep convective activity, caused by strong surface cyclones and high sea surface temperatures, are greater during the ‘mismatched'months than during the ‘matched'months. Water vapor is transported from the lower troposphere to the lower stratosphere through a strong tropical upwelling, leading to an increase in stratospheric water vapor. On the other hand, deep convective activity can lift the tropopause and cool its temperature. In short, the key factor responsible for the poor correlation between tropical tropopause temperature and stratospheric water vapor in1996 is the instantaneous strong deep convective activity. In addition, an anomalously strong Brewer-Dobson circulation brings more water vapor into the stratosphere during the‘mismatched'months in 1996, and this exacerbates the poor correlation between tropical tropopause temperature and stratospheric water vapor. 相似文献
10.
The longwave (0-2380 cm-1) cooling rate due to water vapor in the troposphere and the stratosphere has been calculated by a new infrared transmission model in this paper. An exact scheme is used for treating the integration over wavenumber and the inhomogeneous path in the atmosphere. It is shown that the atmospheric window region (730-1200 cm-1) (mainly water vapor continuum) plays an important role in the total cooling near the surface, about 72% of the total cooling lying in this region at the height of 1 km; the CG approximation used for an inhomogeneous path is fairly applicable for calculating the cooling rate due to water vapor, with a maximum error of 0.16 K/day throughout the troposhere and the stratosphere; on the other hand, the error due to the diffusivity factor of 1.66 appears to be slightly larger near the surface. In this study, the influences on the calculation of above infrared cooling rate, of the temperature-dependence of the absorption coefficients of water vapor, the upper level cu 相似文献
11.
平流层对对流层的作用是准确评估、预测对流层气候变化的一个重要方面。其中平流层成分尤其是臭氧的变化,可以改变平流层乃至对流层的辐射平衡,从而影响平流层、对流层的热动力过程。本文从辐射、动力2个角度介绍了平流层臭氧影响对流层气候变化的若干研究进展。平流层臭氧可以通过长短波辐射的方式对对流层大气造成辐射强迫,利用大气化学气候模式可以定量计算平流层臭氧变化引起的辐射强迫,但是辐射强迫的估算受模式中辐射传输模块本身缺陷的影响存在不确定性。动力方面,平流层臭氧变化产生的辐射效应可以改变温度的垂直和经向梯度,造成波折射指数的变化,进而影响平流层甚至对流层内波的折射与反射,通过上对流层下平流层区域内的波—流相互作用,对对流层气候产生影响。另外,南极臭氧损耗可通过大气环状模影响冬春季中高纬度对流层的天气气候,但是其影响的强度大小以及物理机制仍需进一步的确认。值得注意的是,北极平流层臭氧的变化与北半球中高纬度气候变化之间的关系相比南半球要更加复杂,需要更为深入的研究。 相似文献
12.
The interactively coupled chemistry-climate model ECHAM4.L39(DLR)/CHEM is employed in sensitivity calculations to investigate feedback mechanisms of dynamic, chemical, and radiative processes. Two multi-year model simulations are carried out, which represent recent atmospheric conditions. It is shown that the model is able to reproduce observed features and trends with respect to dynamics and chemistry of the troposphere and lower stratosphere. In polar regions it is demonstrated that an increased persistence of the winter vortices is mainly due to enhanced greenhouse gas mixing ratios and to reduced ozone concentration in the lower stratosphere. An additional sensitivity simulation is investigated, concerning a possible future development of the chemical composition of the atmosphere and climate. The model results in the Southern Hemisphere indicate that the adopted further increase of greenhouse gas mixing ratios leads to an intensified radiative cooling in the lower stratosphere. Therefore, Antarctic ozone depletion slightly increases due to a larger PSC activity, although stratospheric chlorine is reduced. Interestingly, the behavior in the Northern Hemisphere is different. During winter, an enhanced activity of planetary waves yields a more disturbed stratospheric vortex. This "dynamical heating" compensates the additional radiative cooling due to enhanced greenhouse gas concentrations in the polar region. In connection with reduced stratospheric chlorine loading, the ozone layer clearly recovers. 相似文献
13.
本论文基于WACCM（Whole Atmosphere Community Climate Model）模式最新版本WACCM6和DART（Data Assimilation Research TestBed）同化工具最新版本Manhattan,开发了中高层大气温度、臭氧和水汽卫星资料的同化接口,搭建了一个包含完整平流层过程的数值同化、天气预报和短期气候预测模型（此后简称模型）;本模型对2020年3～4月平流层大气变化进行了同化观测资料的模拟,并以同化试验输出的分析场作为初值,对5～6月的平流层大气进行了0～30天天气尺度预报以及31～60天短期气候尺度预测的回报试验。结果表明:本模型能较好地重现2020年3、4月北极平流层出现的大规模臭氧损耗事件随时间的演变特征,模拟结果和Microwave Limb Sounder（MLS）卫星观测结果很接近;而未进行同化的模拟试验,虽然可以模拟出北极臭氧损耗现象,但是模拟的臭氧损耗规模相比MLS卫星观测结果要低很多;利用同化试验4月末输出的分析场作为初值,预报的5月北极平流层臭氧体积混合比变化与MLS卫星观测值的差值小于0.5,预测的6月北极平流层臭氧变化只在10～30 hPa之间的区域,与观测之间的差异达到了1 ppm（ppm=10?6）。本模型不但改善了北极平流层化学成分变化的模拟,也显著地提升了北极平流层温度和环流的模拟。本模型同化模拟的3～4月、预报预测的5～6月北极平流层温度和纬向风变化与Modern-Era Retrospective analysis for Research and Applications, Version 2 （MERRA2）再分析资料结果具有很好的一致性,仅在北极平流层顶部,预报预测的温度和纬向风分别与再分析资料之间的均方根误差（RMSE）约为3 K和4 m s?1。未进行同化的试验模拟的3～4月、预报预测的5～6月北极平流层的温度和纬向风与MERRA2再分析资料之间的RMSE在大部分区域都达到6 K及5 m s?1以上。从全球范围来看,本模型对平流层中低层模拟性能改善最为显著,其预报预测结果与观测值之间的差异,比未进行同化试验的结果,减少了50%以上。 相似文献
14.
通过WACCM-3模式中气溶胶光学厚度与卫星资料的对比发现,模式可以很好地再现全球气溶胶的主要分布特征,但在一些区域还存在数值上的差异。利用数值试验研究对流层气溶胶的直接气候效应对平流层气候的影响,结果表明:对流层气溶胶对平流层气候有明显影响,平流层化学过程在这一影响中起重要作用,而对流层气溶胶对平流层辐射的影响不是其直接气候效应对平流层影响的主要原因。其机制可能是对流层气溶胶改变对流层的辐射平衡,影响对流层的温度和大气环流,进而影响行星波的上传,使得平流层气候发生变化;影响区域主要位于高纬度和极地地区,南半球的变化比北半球大,温度变化最大达10 K,纬向风变化最大可达12 m/s,臭氧体积分数最多减少0.8×10-6。 相似文献
15.
The effect of the stratospheric ozone depletion on the thermal and dynamical structure of the middle atmosphere is assessed using two 5-member ensembles of transient GCM simulations; one including linear trends in ozone, the other not, for the 1980–1999 period. Simulated temperatures and observations are in good agreement in terms of mean values, autocorrelations and cross correlations. Annual-mean and seasonal temperature trends have been calculated using the same statistical analysis. Simulations show that ozone trends are responsible for reduced wave activity in the Arctic lower stratosphere in February and March, confirming both the role of dynamics in controlling March temperatures and a recently proposed mechanism whereby Arctic ozone depletion causes the reduction in wave activity entering the lower stratosphere. Changes in wave activity are consistent with an intensification of the polar vortex at the time of ozone depletion and with a weakened Brewer–Dobson circulation: A decrease of the dynamical warming/cooling associated with the descending/ascending branch of the wintertime mean residual circulation at high/low latitudes has been obtained through the analysis of temperature observations (1980–1999). Ozone is responsible of about one third of the decrease of this dynamical cooling at high latitudes. An increase in the residual mean circulation is seen in the observations for the 1965–1980 period. 相似文献
16.
The radiative impacts of the stratosphere in global warming simulations are investigated using abrupt CO2 quadrupling experiments of the Coupled Model Inter-comparison Project phase 5 (CMIP5), with a focus on stratospheric temperature and water vapor. It is found that the stratospheric temperature change has a robust bullhorn-like zonal-mean pattern due to a strengthening of the stratospheric overturning circulation. This temperature change modifies the zonal mean top-of-the-atmosphere energy balance, but the compensation of the regional effects leads to an insignificant global-mean radiative feedback (?0.02 ± 0.04 W m?2 K?1). The stratospheric water vapor concentration generally increases, which leads to a weak positive global-mean radiative feedback (0.02 ± 0.01 W m?2 K?1). The stratospheric moistening is related to mixing of elevated upper-tropospheric humidity, and, to a lesser extent, to change in tropical tropopause temperature. Our results indicate that the strength of the stratospheric water vapor feedback is noticeably larger in high-top models than in low-top ones. The results here indicate that although its radiative impact as a forcing adjustment is significant, the stratosphere makes a minor contribution to the overall climate feedback in CMIP5 models. 相似文献
17.
Wintertime temperature and ozone in the Northern Hemisphere stratosphere vary significantly between years. Largely random, those variations are marked by compensating changes at high and low latitudes, a feature that reflects the residual mean circulation of the stratosphere. Interannual changes of temperature and ozone each track anomalous forcing of the residual circulation. This relationship is shown to be obeyed even over the Arctic, where transport is augmented by heterogeneous chemical processes that destroy ozone. Chlorine activation obeys a similar relationship, reflecting feedback between changes of the residual circulation and anomalous photochemistry.Changes of stratospheric dynamical and chemical structure are found be accompanied by coherent changes in the troposphere. Vertically extensive, they reflect inter-dependent changes in the stratosphere and troposphere, which are coupled by the residual circulation through transfers of mass. The corresponding structure is shown to share major features with empirical modes of interannual variability associated with the AO and its cousin, the NAO.A 3D model of dynamics and photochemistry is used to simulate anomalous temperature and ozone. Driven by anomalous wave activity representative of that observed, the model reproduces the salient structure of observed interannual changes. Anomalous temperature and ozone follow in the integrations from anomalous downwelling, which, under disturbed conditions, renders temperature over the Arctic anomalously warm, and from anomalous poleward transport, which renders Arctic ozone anomalously rich.Accompanying random interannual changes in the observed record was a systematic decline of Northern Hemisphere temperature and ozone during the 1980s and early 1990s. Comprising decadal trends, these systematic changes are shown to have the same essential structure and seasonality as random changes, which, in turn, vary coherently with anomalous forcing of the residual circulation. Implications of the findings to the interpretation of stratospheric trends are discussed in light of anomalous residual motion, photochemistry, and feedback between them. 相似文献