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1.
An improved stratospheric representation has been included in simulations with the Hadley Centre HadGEM1 coupled ocean atmosphere model with natural and anthropogenic forcings for the period 1979–2003. An improved stratospheric ozone dataset is employed that includes natural variations in ozone as well as the usual anthropogenic trends. In addition, in a second set of simulations the quasi biennial oscillation (QBO) of stratospheric equatorial zonal wind is also imposed using a relaxation towards ERA-40 zonal wind values. The resulting impact on tropospheric variability and trends is described. We show that the modelled cooling rate at the tropopause is enhanced by the improved ozone dataset and this improvement is even more marked when the QBO is also included. The same applies to warming trends in the upper tropical troposphere which are slightly reduced. Our stratospheric improvements produce a significant increase of internal variability but no change in the positive trend of annual mean global mean near-surface temperature. Warming rates are increased significantly over a large portion of the Arctic Ocean. The improved stratospheric representation, especially the QBO relaxation, causes a substantial reduction in near-surface temperature and precipitation response to the El Chichón eruption, especially in the tropical region. The winter increase in the phase of the northern annular mode observed in the aftermath of the two major recent volcanic eruptions is partly captured, especially after the El Chichón eruption. The positive trend in the southern annular mode (SAM) is increased and becomes statistically significant which demonstrates that the observed increase in the SAM is largely subject to internal variability in the stratosphere. The possible inclusion in simulations for future assessments of full ozone chemistry and a gravity wave scheme to internally generate a QBO is discussed.  相似文献   

2.
Abstract

To evaluate future climate change in the middle atmosphere and the chemistry–climate interaction of stratospheric ozone, we performed a long-term simulation from 1960 to 2050 with boundary conditions from the Intergovernmental Panel on Climate Change A1B greenhouse gas scenario and the World Meteorological Organization Ab halogen scenario using the chemistry–climate model ECHAM5/MESSy Atmospheric Chemistry (EMAC). In addition to this standard simulation we performed five sensitivity simulations from 2000 to 2050 using the rerun files of the simulation mentioned above. For these sensitivity simulations we used the same model setup as in the standard simulation but changed the boundary conditions for carbon dioxide (CO2), methane (CH4), nitrous oxide (N2O), and ozone-depleting substances (ODS). In the first sensitivity simulation we fixed the mixing ratios of CO2, CH4, and N2O in the boundary conditions to the amounts for 2000. In each of the four other sensitivity simulations we fixed the boundary conditions of only one of CO2, CH4, N2O, or ODS to the year 2000.

In our model simulations the future evolution of greenhouse gases leads to significant cooling in the stratosphere and mesosphere. Increasing CO2 mixing ratios make the largest contributions to this radiative cooling, followed by increasing stratospheric CH4, which also forms additional H2O in the upper stratosphere and mesosphere. Increasing N2O mixing ratios makes the smallest contributions to the cooling. The simulated ozone recovery leads to warming of the middle atmosphere.

In the EMAC model the future development of ozone is influenced by several factors. 1) Cooler temperatures lead to an increase in ozone in the upper stratosphere. The strongest contribution to this ozone production is cooling due to increasing CO2 mixing ratios, followed by increasing CH4. 2) Decreasing ODS mixing ratios lead to ozone recovery, but the contribution to the total ozone increase in the upper stratosphere is only slightly higher than the contribution of the cooling by greenhouse gases. In the polar lower stratosphere a decrease in ODS is mainly responsible for ozone recovery. 3) Higher NOx and HOx mixing ratios due to increased N2O and CH4 lead to intensified ozone destruction, primarily in the middle and upper stratosphere, from additional NOx; in the mesosphere the intensified ozone destruction is caused by additional HOx. In comparison to the increase in ozone due to decreasing ODS, ozone destruction caused by increased NOx is of similar importance in some regions, especially in the middle stratosphere. 4) In the stratosphere the enhancement of the Brewer-Dobson circulation leads to a change in ozone transport. In the polar stratosphere increased downwelling leads to additional ozone in the future, especially at high northern latitudes. The dynamical impact on ozone development is higher at some altitudes in the polar stratosphere than the ozone increase due to cooler temperatures. In the tropical lower stratosphere increased residual vertical upward transport leads to a decrease in ozone.  相似文献   

3.
The paper presents a coupled chemical-radiative one-dimensional model which is used to assess the steady-state and time-dependent composition and temperature changes in relation to the release in the atmosphere of chemicals such as CO2, N2O, CH4, NO x and chlorofluorocarbons.The model indicates that a doubling in CO2 leads to an increase in temperature of 12.7 K near the stratopause and to an increase in total ozone of 3.3% with a local enhancement of 17% at 40 km altitude. Additional release of N2O leads to an ozone reduction in the middle stratosphere. The reduction in the ozone column is predicted to be equal to 8.8% when the amount of N2O is doubled. The chemical effect of CH4 on ozone is particularly important in the troposphere. A doubling in the mixing ratio of this gas enhances the O3 concentration by 11% at 5 km. The predicted increase of the ozone column is equal to 1.4%. A constant emission of CFCl3 (230 kT/yr) and CF2Cl2 (300 kT/yr) leads to a steady-state reduction in the ozone column of 1.9% compared to the present-day situation. The effect of some uncertainties in the chemical scheme as well as the impact of a high chlorine perturbation are briefly discussed.Finally the results of a time dependent calculation assuming a realistic scenario for the emission of chemical species are presented and analyzed.  相似文献   

4.
Abstract

The first substantial radiative effects of the El Chichón volcanic cloud were observed in Fairbanks in the winter of 1982/83. Winter is the time when stratospheric temperatures can vary widely owing to sudden stratospheric warmings, and interannual variations are large. Mean monthly temperatures of the stratosphere were analysed for the 50‐, 40‐, 30‐, 25‐, 20‐, 15‐, and 10‐mb levels, with the greatest density of the volcanic cloud expected to be around the 20‐mb level. For the four winter months, December 1982 to March 1983, an increase in temperature was observed. This increase was not only observed in Fairbanks, but also for two other stations (McGrath and Anchorage) close by, for which we also analysed the stratospheric temperatures.

Further, the interdiurnal variation of temperature (the radiosonde ascents are made at 0200 and 1400 local time) showed marked and significant increases for all three stations. This can be explained by the fact that during daytime the volcanic cloud is warmed by absorption of solar radiation, while at night no substantial temperature effect for this layer was detected.  相似文献   

5.
The paper discusses the potential effects on the ozone layer of gases released by the engines of proposed high altitude supersonic aircraft. The major problem arises from the emissions of nitrogen oxides which have the potential to destroy significant quantities of ozone in the stratosphere. The magnitude of the perturbation is highly dependent on the cruise altitude of the aircraft. Furthermore, the depletion of ozone is substantially reduced when heterogeneous conversion of nitrogen oxides into nitric acid on sulfate aerosol particles is taken into account in the calculation. The sensitivity of the aerosol load on stratospheric ozone is investigated. First, the model indicates that the aerosol load induced by the SO2 released by aircraft is increased by about 10–20% above the background aerosols at mid-high latitude of the Northern Hemisphere at 15 km for the NASA emission scenario A (the NASA emission scenarios are explained in Tables I to III). This increase in aerosol has small effects on stratospheric ozone. Second, when the aerosol load is increased following a volcanic eruption similar to the eruption of El Chichon (Mexico, April 1982), the ozone column in spring increases by as much as 9% in response to the injection of NO x from the aircraft with the NASA emission scenario A. Finally, the modeled suggests that significant ozone depletion could result from the formation of additional polar stratospheric clouds produced by the injection of H2O and HNO3 by the aircraft engines.  相似文献   

6.
A one-dimensional coupled climate and chemistry model has been developed to estimate past and possible future changes in atmospheric temperatures and chemical composition due to human activities. The model takes into account heat flux into the oceans and uses a new tropospheric temperature lapse rate formulation. As found in other studies, we estimate that the combined greenhouse effect of CH4, O3, CF2Cl2, CFCl3 and N2O in the future will be about as large as that of CO2. Our model calculates an increase in average global surface temperatures by about 0.6°C since the start of the industrial era and predicts for A.D. 2050 a twice as large additional rise. Substantial depletions of ozone in the upper stratosphere by between 25% and 55% are calculated, depending on scenario. Accompanying temperature changes are between 15°C and 25°C. Bromine compounds are found to be important, if no rigid international regulations on CFC emissions are effective. Our model may, however, concivably underestimate possible effects of CFCl3, CF2Cl2, C2F3Cl3 and other CFC and organic bromine emissions on lower stratospheric ozone, because it can not simulate the rapid breakdown of ozone which is now being observed worldwide. An uncertainty study regarding the photochemistry of stratospheric ozone, especially in the region below about 25 km, is included. We propose a reaction, involving excited molecular oxygen formation from ozone photolysis, as a possible solution to the problem of ozone concentrations calculated to be too low above 45 km. We also estimate that tropospheric ozone concentrations have grown strongly in the northern hemisphere since pre-industrial times and that further large increases may take place, especially if global emissions of NOx from fossil fuel and biomass burning were to continue to increase. Growing NOx emissions from aircraft may play an important role in ozone concentrations in the upper troposphere and low stratosphere.  相似文献   

7.
The effects of E1Nifio Modoki events on global ozone concentrations are investigated from 1980 to 2010 E1 Nifio Modoki events cause a stronger Brewer-Dobson (BD) circulation which can transports more ozone-poor air from the troposphere to stratosphere, leading to a decrease of ozone inthe lower-middle stratosphere from 90~S to 90~N. These changes in ozone concentrations reduce stratospheric column ozone. The reduction in stratospheric column ozone during E1 Nifio Modoki events is more pronounced over the tropical eastern Pacific than over other tropical areas because transport of ozone-poor air from middle-high latitudes in both hemispheres to low latitudes is the strongest between 60°W and 120°W. Because of the decrease in stratospheric column ozone during E1 Nifio Modoki events more UV radiation reaches the tropical troposphere leading to significant increases in tropospheric column ozone An empirical orthogonal function (EOF) analysis of the time series from 1980 to 2010 of stratospheric and tropospheric ozone monthly anomalies reveals that: E1 Nifio Modoki events are associated with the primary EOF modes of both time series. We also found that E1 Nifio Modoki events can affect global ozone more significantly than canonical E1 Nifio events. These results imply that E1 Nifio Modoki is a key contributor to variations in global ozone from 1980 to 2010.  相似文献   

8.
This paper describes a diagnostic study of the feedback mechanism in greenhouse effects of increased CO_2 and oth-er trace gases(CH_4,N_2O and CFCs),simulated by general circulation model.The study is based on two sensitivity exper-iments for doubled CO_2 and the inclusion of other trace gases,respectively,using version one of the community climatemodel(CCM1)developed at the National Centre for Atmospheric Research.A one-dimensional(1-D)and atwo-dimensional(2-D)radiative-convective models are used to diagnose the feedback effect.It shows that thefeedback factors in global and annual mean conditions are in the sequence of surface albedo,water vapor amount,watervapor distribution,cloud height,critical lapse rate and cloud cover,while in zonal and annual mean conditions in thetropical region the above sequence does not change except the two water vapor terms being the largest feedback compo-nents.Among the feedback components,the total water vapor feedback is the largest(about 50%).The diagnosis alsogives a very small feedback of either the cloud cover or the lapse rate,which is substantially different from the 1-Dfeedback analysis by Hansen et al.(1984).The small lapse rate feedback is considered to be partly caused by theconvective adjustment scheme adopted by CCM1 model.The feedback effect for doubled CO_2 is very different from that of the addition of other trace gases because of theirdifferent vertical distributions of radiative forcing although the non-feedback responses of surface air temperature forboth cases are almost the same.For instance,the larger forcing at surface by the addition of other trace gases can causestronger surface albedo feedback than by doubled CO_2.Besides,because of the negative forcing of doubled CO_2 in thestratosphere,cloud height feedback is more intense.The larger surface forcing in the case of other trace gases can also in-fluence atmospheric water vapor amount as well as the water vapor distribution,which will in turn have strongerfeedback effects.All these indicate that it is incorrect to use“effective CO_2”to replace other trace gases in the generalcirculation model.  相似文献   

9.
A mean meridional circulation model of the stratosphere, incorporating radiative heating and photochemistry of the oxygen‐hydrogen‐nitrogen atmosphere, is used to simulate the meridional distributions of O3, HOX, N2O,NOX, temperature and the three components of mean motion for the summer and winter seasons under steady‐state conditions. The results are generally in good agreement with the available observations in the normal stratosphere. The model has been applied to assess the effects of water vapour and nitrogen oxide perturbations resulting from aircraft emissions in the stratosphere. It is found that a fleet of 500 Boeing‐type sst's, flying at 20 km and 45°N in the summer hemisphere and inserting NOx at a rate of 1.8 megatons per year, has the effect of reducing the global total ozone by 14.7%. Similar calculations for 342 Concorde/TU‐114's, cruising at 17 km and injecting NOx at a rate of 0.35 megatons per year, show a global‐average total‐ozone reduction of 1.85%. Although water vapour is considered important, because of its ability to convert NO2 into HNO3, the direct effect on global‐average total‐ozone reduction resulting from the 100% increase in the stratospheric water content is less than 1%. The changes in the chemical structure (HO^NO^), temperature, and mean motions associated with the ozone reduction are also investigated in the case of the 1.8‐megaton‐per‐year NOX perturbation. It is shown that the reduced meridional temperature gradient in the middle and upper stratosphere resulting from the NOx perturbation leads to the weakening of the tropical easterly jet in the summer hemisphere and mid‐latitude westerlies in the winter season.

The sensitivity of the model solutions to an alternate choice of input parameters (diffusion coefficients and solar photodissociation data) is tested and the main deficiency of the model is pointed out.  相似文献   

10.
Airborne measurements of stratospheric ozone and N2O from the SCIAMACHY (Scanning Imaging Absorption Spectrometer) Validation and Utilization Experiment (SCIA-VALUE) are presented. The campaign was conducted in September 2002 and February–March 2003. The Airborne Submillimeter Radiometer (ASUR) observed stratospheric constituents like O3 and N2O, among others, spanning a latitude from 5°S to 80°N during the survey. The tropical ozone source regions show high ozone volume mixing ratios (VMRs) of around 11 ppmv at 33 km altitude, and the altitude of the maximum VMR increases from the tropics to the Arctic. The N2O VMRs show the largest value of 325 ppbv in the lower stratosphere, indicating their tropospheric origin, and they decrease with increasing altitude and latitude due to photolysis. The sub-tropical and polar mixing barriers are well represented in the N2O measurements. The most striking seasonal difference found in the measurements is the large polar descent in February–March. The observed features are interpreted with the help of SLIMCAT and Bremen Chemical Transport Model (CTMB) simulations. The SLIMCAT simulations are in good agreement with the measured O3 and N2O values, where the differences are within 1 ppmv for O3 and 15 ppbv for N2O. However, the CTMB simulations underestimate the tropical middle stratospheric O3 (1–1.5 ppmv) and the tropical lower stratospheric N2O (15–30 ppbv) measurements. A detailed analysis with various measurements and model simulations suggests that the biases in the CTMB simulations are related to its parameterised chemistry schemes.  相似文献   

11.
The climate response to an increase in carbon dioxide and sea surface temperatures is examined using the Météo-France climate model. This model has a high vertical resolution in the stratosphere and predicts the evolution of the ozone mixing ratio. This quantity is fully interactive with radiation and photochemical production and loss rates are accounted for. Results from a 5-year control run indicate a reasonable agreement with observed climatologies. A 5-year simulation is performed with a doubled CO2 concentration using, as lower boundary conditions, mean surface temperatures anomalies and sea ice limits predicted for the years 56–65 of a 100-year transient simulation performed at Hamburg with a global coupled atmosphere-ocean model. The perturbed simulation produces a global mean surface air warming of 1.4 K and an increase in global mean precipitation rate of 4%. Outside the high latitudes in the Northern Hemisphere, the model simulates a strong cooling in the stratosphere reaching 10 K near the stratopause. Temperature increases are noticed in the lower polar stratosphere of the Northern Hemisphere caused by an intensification in the frequency of sudden warmings in the perturbed simulation. The low and mid-latitude stratospheric cooling leads to an ozone column enhancement of about 5%. Other features present in similar studies are exhibited in the troposphere such as the stronger surface warming over polar regions of the Northern Hemisphere, the summer time soil moisture drying in mid-latitudes and the increase in high convective cloudiness in tropical regions.This paper was presented at the Second International Conference on Modelling of Global Climate Variability, held in Hamburg 7–11 September 1992 under the auspices of the Max Planck Institute for Meteorology. Guest Editor for these papers is L. Dümenil Correspondence to: JF Mahfouf  相似文献   

12.
Previous studies (e.g., Dessler et al., 1996; Haigh, 1984) have discussed the effect of cloud on modelled ozone distribution through changes in the radiative heating in the lower stratosphere. Here the relationship is investigated using an interactive chemical-radiative- transport 2D model. It is shown that, while similar cooling in the lower stratosphere due to high cloud is found, the effect on ozone is not as previously expected. The inclusion of high cloud is found to bring about a warming of the troposphere, resulting in a net heating in the lower stratosphere. This strengthens the circulation, leading to a decrease in total tropical ozone. Importantly, the effect of the cloud-induced temperature changes on heating rates does not combine linearly with the direct radiative effect of cloud changes. The possibility of a link between the high cloud increases and total ozone decreases observed in some regions during strong El Niño episodes is investigated. The possible impact on ozone of a global trend in high cloud cover is also discussed.  相似文献   

13.
未来甲烷排放增加对平流层水汽和全球臭氧的影响   总被引:3,自引:0,他引:3  
利用一个耦合的大气化学-气候模式(WACCM3)研究了地表甲烷排放增加对平流层水汽和全球臭氧变化的影响.结果表明,如果地表甲烷的排放量在2000年的基础上增加50%(达到政府间气候变化专门委员会A1B排放情景中2050年的值),平流层水汽体积分数将平均增加约0.8×10-6.南半球平流层甲烷转化为水汽的效率比北半球高.在北半球平流层中,1mol甲烷分子可以转化为约1.63mol的水汽分子,而在南半球1mol甲烷分子大概可以转化为约1.82mol的水汽分子.甲烷排放增加50%将使全球中低纬度地区以及北半球高纬度地区的臭氧柱总量增加1%-3%,使南半球高纬度地区臭氧柱总量增加近8%,而秋季(南半球春季)南极地区臭氧柱总量增加幅度可高达20%,南极臭氧的这种显着增加主要是由于甲烷增加造成的化学反馈所致.在北半球中高纬度地区,甲烷增加引起的臭氧变化主要与甲烷氧化导致的水汽增加有关.研究还表明,未来甲烷排放增加对臭氧的恢复作用其实与溴化物排放的减少一样重要.  相似文献   

14.
To analyze the mechanism by which water vapor increase leads to cooling in the stratosphere, the effects of water-vapor increases on temperature in the stratosphere were simulated using the two-dimensional, interactive chemical dynamical radiative model (SOCRATES) of NCAR. The results indicate that increases in stratospheric water vapor lead to stratospheric cooling, with the extent of cooling increasing with height, and that cooling in the middle stratosphere is stronger in Arctic regions. Analysis of the radiation process showed that infrared radiative cooling by water vapor is a pivotal factor in middle-lower stratospheric cooling. However, in the upper stratosphere (above 45 km), infrared radiation is not a factor in cooling; there, cooling is caused by the decreased solar radiative heating rate resulting from ozone decrease due to increased stratospheric water vapor. Dynamical cooling is important in the middle-upper stratosphere, and dynamical feedback to temperature change is more distinct in the Northern Hemisphere middle-high latitudes than in other regions and signiffcantly affects temperature and ozone in winter over Arctic regions. Increasing stratospheric water vapor will strengthen ozone depletion through the chemical process. However, ozone will increase in the middle stratosphere. The change in ozone due to increasing water vapor has an important effect on the stratospheric temperature change.  相似文献   

15.
Abstract

Solar radiation data for Vancouver, B.C. were used to determine the increase in aerosol optical depth and the changes in the total, direct, diffuse and net short‐wave radiation fluxes associated with the presence of aerosol that originated from the eruption of El Chichón (Mexico) in April 1982. The aerosol optical depth increased by 400% resulting in reductions of 33% in the direct and increases of 80% in the diffuse short‐wave radiation. These maximum changes were experienced some 9 months following the eruption. The relative insensitivity of the total short‐wave radiation (maximum reduction was 6%) suggests that the volcanic cloud was a strong forward scatterer rather than an absorber or back scatterer. Moreover, interannual variability in the surface albedo and a negative feedback associated with the dependence of the surface albedo on the directionality of the incident radiation resulted in no consistent change in the amount of short‐wave radiation absorbed by the Earth's surface.  相似文献   

16.
Wintertime temperature and ozone in the Northern Hemisphere stratosphere vary significantly between years. Largely random, those variations are marked by compensating changes at high and low latitudes, a feature that reflects the residual mean circulation of the stratosphere. Interannual changes of temperature and ozone each track anomalous forcing of the residual circulation. This relationship is shown to be obeyed even over the Arctic, where transport is augmented by heterogeneous chemical processes that destroy ozone. Chlorine activation obeys a similar relationship, reflecting feedback between changes of the residual circulation and anomalous photochemistry.Changes of stratospheric dynamical and chemical structure are found be accompanied by coherent changes in the troposphere. Vertically extensive, they reflect inter-dependent changes in the stratosphere and troposphere, which are coupled by the residual circulation through transfers of mass. The corresponding structure is shown to share major features with empirical modes of interannual variability associated with the AO and its cousin, the NAO.A 3D model of dynamics and photochemistry is used to simulate anomalous temperature and ozone. Driven by anomalous wave activity representative of that observed, the model reproduces the salient structure of observed interannual changes. Anomalous temperature and ozone follow in the integrations from anomalous downwelling, which, under disturbed conditions, renders temperature over the Arctic anomalously warm, and from anomalous poleward transport, which renders Arctic ozone anomalously rich.Accompanying random interannual changes in the observed record was a systematic decline of Northern Hemisphere temperature and ozone during the 1980s and early 1990s. Comprising decadal trends, these systematic changes are shown to have the same essential structure and seasonality as random changes, which, in turn, vary coherently with anomalous forcing of the residual circulation. Implications of the findings to the interpretation of stratospheric trends are discussed in light of anomalous residual motion, photochemistry, and feedback between them.  相似文献   

17.
Factors influencing the18O content of stratospheric H2O are reviewed in order to provide a theoretical framework for the interpretation of measurements of this quantity, which are now becoming available. Depletions in18O of 5–10% in stratospheric H2O are expected based on the known correlation between that of D and18O in tropospheric H2O and observed measurements of large (typically 50%) depletions of D in stratospheric H2O. H2O formed in the stratosphere as a result of oxidation of CH4 can be expected to reflect primarily the18O content of stratospheric O2, which is the same as that of tropospheric O2 (slightly enhanced with respect to standard mean ocean water). Thus, a reduction in the18O depletion is expected with increasing altitude, but not a large enhancement in18O in upper stratospheric H2O as found in recent far infrared measurements. The observed large enhancement of18O in stratospheric O3 is not expected to be reflected in stratospheric H2O. Necessary laboratory data for the improved quantification of these effects are reviewed.  相似文献   

18.
Time sclice experiments are performed with the atmospheric GCM ARPEGE, developed at Météo-France, to study the impact to increases in the atmospheric carbon dioxide. This spectral model runs at T42 horizontal resolution with 30 vertical layers including a comprehensive tropospheric and stratospheric resolution and a prognostic parameterization of the ozone mixing ratio. The model is forced in a 5-year control run by climatological SSTs and sea-ice extents in order to obtain an accurate simulation of the present-day climate. Two perturbed runs are performed using SSTs and sea-ice extents for doubled CO2 concentration, obtained from transient runs performed by two coupled atmospheric-oceanic models run at the Max Planck Institute (MPI) in Hamburg and the Hadley Centre (HC). A global surface temperature warming of 1.6 K is obtained with the MPI SST anomalies and 1.9 K with the HC SST anomalies. The precipitation rate increases by 4.2% (and 4.7%). The features obtained in the stratosphere (a cooling increasing with the altitude and an increase in the ozone mixing ratio) are not sensitive to the oceanic forcing. On the contrary, the anomalies in the troposphere such as a warming increasing with altitude, an acceleration of westerly jets and a raised cloud height, depend on the oceanic forcing imposed in the two perturbed runs. Special attention is given to continental areas where the impact of the oceanic forcing is studied over eight regions around the globe. Regions sensitive to oceanic forcing such as Europe are identified in contrast with areas where the patterns are driven by land-surface physical processes, such as over continental Asia. Finally, the Köppen classification is applied to the climate simulated in the three experiments. Both doubled CO2 runs show the same predominance of global warming over precipitation changes in the Kbppen analyses.  相似文献   

19.
Wilhelm May 《Climate Dynamics》2008,31(2-3):283-313
In this study, concentrations of the well-mixed greenhouse gases as well as the anthropogenic sulphate aerosol load and stratospheric ozone concentrations are prescribed to the ECHAM5/MPI-OM coupled climate model so that the simulated global warming does not exceed 2°C relative to pre-industrial times. The climatic changes associated with this so-called “2°C-stabilization” scenario are assessed in further detail, considering a variety of meteorological and oceanic variables. The climatic changes associated with such a relatively weak climate forcing supplement the recently published fourth assessment report by the IPCC in that such a stabilization scenario can only be achieved by mitigation initiatives. Also, the impact of the anthropogenic sulphate aerosol load and stratospheric ozone concentrations on the simulated climatic changes is investigated. For this particular climate model, the 2°C-stabilization scenario is characterized by the following atmospheric concentrations of the well-mixed greenhouse gases: 418 ppm (CO2), 2,026 ppb (CH4), and 331 ppb (N2O), 786 ppt (CFC-11) and 486 ppt (CFC-12), respectively. These greenhouse gas concentrations correspond to those for 2020 according to the SRES A1B scenario. At the same time, the anthropogenic sulphate aerosol load and stratospheric ozone concentrations are changed to the level in 2100 (again, according to the SRES A1B scenario), with a global anthropogenic sulphur dioxide emission of 28 TgS/year leading to a global anthropogenic sulphate aerosol load of 0.23 TgS. The future changes in climate associated with the 2°C-stabilization scenario show many of the typical features of other climate change scenarios, including those associated with stronger climatic forcings. That are a pronounced warming, particularly at high latitudes accompanied by a marked reduction of the sea-ice cover, a substantial increase in precipitation in the tropics as well as at mid- and high latitudes in both hemispheres but a marked reduction in the subtropics, a significant strengthening of the meridional temperature gradient between the tropical upper troposphere and the lower stratosphere in the extratropics accompanied by a pronounced intensification of the westerly winds in the lower stratosphere, and a strengthening of the westerly winds in the Southern Hemisphere extratropics throughout the troposphere. The magnitudes of these changes, however, are somewhat weaker than for the scenarios associated with stronger global warming due to stronger climatic forcings, such as the SRES A1B scenario. Some of the climatic changes associated with the 2°C-stabilization are relatively strong with respect to the magnitude of the simulated global warming, i.e., the pronounced warming and sea-ice reduction in the Arctic region, the strengthening of the meridional temperature gradient at the northern high latitudes and the general increase in precipitation. Other climatic changes, i.e., the El Niño like warming pattern in the tropical Pacific Ocean and the corresponding changes in the distribution of precipitation in the tropics and in the Southern Oscillation, are not as markedly pronounced as for the scenarios with a stronger global warming. A higher anthropogenic sulphate aerosol load (for 2030 as compared to the level in 2100 according to the SRES A1B scenario) generally weakens the future changes in climate, particularly for precipitation. The most pronounced effects occur in the Northern Hemisphere and in the tropics, where also the main sources of anthropogenic sulphate aerosols are located.  相似文献   

20.
Radiative forcing has been widely used as a metric of climate change, i.e. as a measure by which various contributors to a net surface temperature change can be quantitatively compared. The extent to which this concept is valid for spatially inhomogeneous perturbations to the climate system is tested. A series of climate model simulations involving ozone changes of different spatial structure reveals that the climate sensitivity parameter is highly variable: for an ozone increase in the northern hemisphere lower stratosphere, it is more than twice as large as for a homogeneous CO2 perturbation. A global ozone perturbation in the upper troposphere, however, causes a significantly smaller surface temperature response than CO2. The variability of the climate sensitivity parameter is shown to be mostly due to the varying strength of the stratospheric water vapour feedback. The variability of the sea-ice albedo feedback modifies climate sensitivity of perturbations with the same vertical structure but a different horizontal structure. This feedback is also the origin of the comparatively larger climate sensitivity to perturbations restricted to the northern hemisphere extratropics. As cloud feedback does not operate independently from the other feedbacks, quantifying its effect is rather difficult. However, its effect on the variability of for horizontally and vertically inhomogeneous perturbations within one model framework seems to be comparatively small.This revised version was published online March 2005 with corrections to table 5.  相似文献   

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