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1.
基于CLDAS大气驱动数据驱动CLM3.5陆面模式和3种不同参数化方案下的Noah-MP陆面模式模拟得到的地表温度,利用中国气象局2009-2013年2000多个国家级地面观测站地表温度进行质量评估。结果表明:从时间分布看,模拟地表温度与观测的偏差及均方根误差均呈季节性波动;从空间分布看,模拟地表温度与观测的偏差及均方根误差在中国东部地区相对于中国西部地区更小。选择Noah-MP陆面模式3种不同参数化方案模拟结果进行对比,结果表明:Noah-MP模式的非动态植被方案不变时,考虑植被覆盖度的二流近似辐射传输方案的Noah-MP陆面模式模拟的地表温度优于考虑太阳高度角和植被三维结构的二流近似辐射传输方案Noah-MP陆面模式模拟的地表温度;选择动态植被方案的Noah-MP陆面模式模拟的地表温度优于选择非动态植被方案的Noah-MP陆面模式;总体而言,考虑动态植被方案的Noah-MP陆面模式模拟的地表温度优于其他两种参数化方案的Noah-MP陆面模式以及CLM3.5陆面模式模拟的地表温度。 相似文献
2.
我国对流层大气臭氧的数值模拟 总被引：7，自引：2，他引：7
本文建立了一个用于对流层大气臭氧模拟的三维欧拉模式,针对影响臭氧光化学转化的各种因素及我国城市光化学污染的特点,模式中简化了光化学项的计算。根据实际观测资料,提出了模拟云雾对臭氧影响的参数化方法,并确定了云雾作用系数,通过模式的数值模拟,得出了我国对流层大气臭氧,特别是近地面层大气臭氧的分布状况、我国城市光化学污染的分布特征以及它们的季节变化规律. 相似文献
3.
以2010年8月发生在太湖地区的一次雷暴过程为例,利用WRF模式进行48 h的短期天气模拟,分析两个陆面参数化方案(Noah方案和RUC方案)对雷暴过程模拟的影响。对比模式结果与实况降水以及太湖地区两个站点的近地面要素表明:雷暴过程对陆面参数化方案的选取较为敏感,不同陆面参数化方案可影响雷暴发生的时间、地点及强度,两种方案的降水中心值差达40 mm以上,其中Noah方案所模拟的降水与实况更为接近。通过对两个方案模拟的物理量场的对比分析发现,RUC方案中对流发展滞后于Noah方案2 h;这表明陆面过程对雷暴等中尺度对流过程有显著的反馈作用,不同陆面参数化方案的使用影响雷暴发生的动力和热力作用,并改变雷暴的时空分布特征。陆面过程通过改变地面热通量输送影响边界层结构,使得水平和垂直方向上的风和温度等发生变化并产生辐合辐散,进而影响对流的启动时间和对流发展强度。由于对不同植被的参数化处理的差异,Noah方案对下垫面特征的描述能力优于RUC方案,尤其是对城市下垫面的处理,这也使得之后该方案模拟的雷暴发生时间更加接近于实况且雷暴过程更加强烈。 相似文献
4.
霍文 《沙漠与绿洲气象(新疆气象)》2016,10(5):87-96
陆面过程是影响大气环流和气候变化的基本物理、生化过程之一。沙漠陆面过程及相应的小气候效应已经成为当前沙漠气象研究的热门问题。近年来,在沙漠陆面过程野外观测、陆面过程特征及参数化、陆面过程模拟、小气候及陆面过程对小气候影响等方面已取得重大进展。本文对于沙漠小气候、沙漠陆面过程及沙漠陆面过程参数化进行了简要概述,重点总结了国内外在沙漠地区气候考察、沙漠边界层高度、沙漠热力环流、绿洲效应、塔克拉玛干沙漠气候特征、沙漠陆面过程野外观测试验及结果、沙漠陆面过程对气候的影响、沙漠陆面过程参数化方案方面的成果,回顾了近年来利用地面观测设备和数值模式等对气候效应和陆面过程直接观测和数值模拟所获得的观测事实和模拟试验,并讨论了其陆面过程参数化对模拟的影响,在总结前人研究成果的基础上对未来的研究方向进行了讨论。 相似文献
5.
SHAW模式的改进及其在黄土高原半干旱区的模拟研究 总被引：1，自引：0，他引：1
陆面过程模拟研究中的一个关键问题是如何准确的计算陆气间能量交换,但现有的陆面过程模式模拟的湍流通量与观测值间仍然存在较大偏差,因此改进湍流通量的参数化方案对于提高陆面过程模式模拟能力有重要意义。本研究通过改进陆面过程模式SHAW中的热力粗糙度方案,以及引入干表层蒸发方案,以期改善湍流通量的模拟能力。在此基础上利用黄土高原半干旱区SACOL站观测资料,进行模式改进前后的单点模拟对比试验,研究其参数化方案改进对陆面过程模拟的影响。结果表明:改进后的SHAW模式能够合理地模拟黄土高原半干旱区陆面特征的变化趋势,模拟值与观测值偏差较小。与原来的SHAW模式模拟结果相比,改进后的SHAW_MOD模式显著提高了湍流通量的模拟能力,并改善了净辐射和深层土壤温度的模拟,但对土壤湿度的改进并不明显,这可能与土壤内部水热传输过程及相关参数化方案有关,还有待做进一步研究。 相似文献
6.
7.
陆面水文过程研究进展 总被引：11，自引：2，他引：9
本文回顾了近年来中国科学院大气物理研究所在陆面水文过程的观测、模式发展以及陆气相互作用研究等方面所取得的重要研究成果。首先概述了近年来在中国区域所开展的陆气相互作用野外观测试验,通过资料分析揭示了国际上现有陆面模式对干旱／半干旱地区陆气相互作用模拟的偏差,指出典型干旱／半干旱区陆面过程参数修正的必要性;随后重点描述了陆面过程模式中积雪覆盖度和冻土参数化方案的发展,中国区域土壤湿度的时空分布特征及其对区域气候的影响,以及中国区域大尺度水文模式的研制和应用等;最后给出了陆面水文过程研究的趋势和发展方向的展望。 相似文献
8.
《高原气象》2015,(6)
利用由国家气候中心最近研发的全球大气环流化学模式BCC-AGCM-ChemO对1871-1999年全球大气O_3浓度进行了模拟,并利用全球臭氧和紫外线辐射数据中心(WOUDC)提供的O_3台站观测资料以及第5次耦合模式国际比较计划(CMIP5)整理的一套全球O_3分析资料对BCC-AGCM-ChemO模拟的O_3的气候平均态及季节变化特征进行了评估。结果表明:(1)BCC-AGCM-ChemO模式模拟出了全球年平均的O_3空间分布特征,表现为北半球O_3浓度高于南半球,O_3的经向分布大致呈由低纬向高纬递增;模式可以再现台站观测的O_3浓度垂直分布结构;相对于CMIP5分析数据,BCC-AGCM-ChemO模拟的O_3气柱总量在40°S以南的南大洋区域,模拟值偏低3~6 DU,在40°S-50°N中低纬地区略偏高3~6DU,陆地地区差异明显大于海洋地区,这些模拟偏差与地面排放和模式中O_3水平和垂直平流输送的影响有关。(2)BCC-AGCM-ChemO模式对全球O_3浓度的季节变化特征也有较好的模拟能力,模拟的O_3柱浓度与CMIP5资料的结果在1、4、7和10月的全球格点空间相关系数分别达到0.89,0.97,0.86和0.91;模式再现了南、北半球O_3浓度春季偏大、秋季偏小的特点;(3)从模式模拟和台站观测的对比分析来看,500 hPa以上的对流层中高层与以下的对流层中低层的O_3季节变化峰值存在明显的不一致性,表明500 hPa以下的中低层区域O_3变化可能受地面排放和干、湿等过程的影响较大,而对流层中高层的O_3变化可能与化学过程和平流层向下的输送影响较大有关。 相似文献
9.
不同边界层参数化方案和陆面过程参数化方案对一次梅雨锋暴雨显式对流模拟的影响分析 总被引：1，自引：0，他引：1
利用WRF模式对2007年7月8日淮河地区特大暴雨过程开展显式对流(1.1 km)模拟试验,比较两种边界层参数化方案和三种陆面过程参数化方案对降水模拟的影响。结果表明,不同边界层参数化方案和陆面过程参数化方案主要影响模拟的强降水位置和强度,而对雨带位置的影响不大。采用MYJ边界层方案模拟的强降水更接近观测,采用YSU方案模拟的强降水偏弱;陆面过程参数化方案对比,简单的热扩散方案模拟的强降水最强、最接近观测,而RUC方案模拟的强降水最弱,Noah方案居中;同时改变陆面方案和边界层方案比单一改变其中一种方案对模拟降水的影响更大。造成强降水模拟差异的主要原因是模拟的近地面(约1 km以下)大气的湿度和温度不同,导致支持对流发生发展的入流空气的对流有效位能(CAPE)不同,进而影响模拟的对流强度和地面降水量。对强降水模拟较好的试验模拟的近地面大气湿度更大,环境入流空气的CAPE更大,对流发展更强,地面降水也更强。 相似文献
10.
积雪季节变化特征的数值模拟及其敏感性试验 总被引：4，自引：0，他引：4
文中利用综合陆面模式 (ComprehensiveLandSurfaceModel,CLSM )对法国ColdePorte 1 993/ 1 994 ,1 994 / 1 995年及BOREASSSA OJP 1 994 / 1 995年积雪个例进行了模拟试验 ,通过模拟结果与观测资料的对比 ,检验了CLSM对积雪变化特征的模拟能力 ,并通过敏感性试验探讨了降雪密度、积雪持水量等积雪参数化方案及植被对积雪模拟可能产生的影响。结果表明 :(1 )CLSM能够准确地模拟出积雪的变化过程 ,对积雪的演变特征作出了合理的描述 ;(2 )降雪密度、积雪持水量参数化方案对积雪模拟结果均具有一定的影响 :降雪密度参数化主要对积雪深度的模拟产生影响 ;而积雪持水量参数化方案对积雪的演变过程 ,尤其是积雪的消融 ,具有重要的作用 ;(3)有、无植被存在的情况下 ,积雪 土壤系统的变化过程存在显著的差别 ,植被通过改变积雪 /土壤表面的能量平衡 ,对积雪及土壤的变化过程产生重要影响 :植被的存在有利于积雪的维持 ,使得积雪融化进程推迟 ,冻结土壤的增温明显偏慢 相似文献
11.
In conversion of the integrated slant column amount of atmospheric ozone(O3) measured by the ground-based spectrometer technique during twilight to the vertical quantity,the air-mass factor(AMF) is an important parameter.In this work,calculations of AMF for ozone were performed for different atmospheres.It is shown that the O3 AMF has seasonal variations with the minimum at the beginning of spring and the maximum in summer due to the seasonal change in the vertical distributions of O3.A parameterization relation is obtained between O3 AMF and optical thickness of stratospheric volcanic aerosols based on the Monte-Carlo radiative transfer simulations. 相似文献
12.
The effect of clouds and cloud chemistry on tropospheric ozone chemistry is tested out in a two-dimensional channel model covering a latitudinal band from 30 to 60° N. Three different methods describing how clouds affect gaseous species are applied, and the results are compared. The three methods are: ?A first order parameterization scheme for the removal of sulphur and other soluble gases by liquid droplets. ?A parameterization scheme for SO2, O3, and H2O2 removal is constructed. The scheme is based on the solubility of gases in liquid droplets, cycling times of air masses between clouds and cloud free areas and on the chemical interaction of SO2 with H2O2 and O3 in the liquid phase. ?Gas-aqueous-phase interactions and aqueous-phase chemical reactions are included in the reaction scheme for a number of components in areas where clouds are present. In all three methods, a full gas-phase chemistry scheme is used. Particular emphasis is given to the study of how the ozone and hydrogen peroxide levels are affected. Significant changes in the distributions are found when aqueous-phase chemical reactions are included. The result is loss of ozone in the aqueous phase, with pronounced reductions in ozone levels in the middle and lower troposphere. Ozone levels are reduced by 10 to 30% with the largest reductions in the remote middle troposphere, bringing the values in better agreement with observations. Changes in H2O2 are harder to predict. Although, in one case study, hydrogen peroxide is produced within the aqueous phase, concentrations are mostly comparable or even lower than in the other cases. Hydrogen peroxide levels are, however, shown to be very pH sensitive. pH values around 5 seem to favour high H2O2 levels. High H2O2 concentrations may be found particularly in the upper part of the clouds under favourable conditions. 相似文献
13.
本文将四个常见陆面模式CLM3.5（Community Land Model Version 3.5）、Noah_LSM（The Noah Land Surface Model）、VIC（Variable Infiltration Capacity）以及SSiB（The Simplified Simple Biosphere Model）中土壤湿度影响蒸散的参数化方案进行简化,并利用实验观测资料对不同参数化方案进行评估,探究不同陆面模式对土壤湿度与蒸散关系的模拟差异,从而为提高模式的模拟能力提供依据。结果表明,（1）CLM与SSiB中计算土壤湿度影响裸土蒸发的参数化方案较Noah_LSM和VIC更接近真实的物理过程,同时CLM与SSiB模式中土壤湿度对蒸发的影响程度较Noah_LSM和VIC大;而对于下垫面有植被条件下的蒸散而言,CLM中包含了植被光合作用、呼吸作用等生物物理学过程,与实际情况更为接近,并且CLM与SSiB中土壤湿度对植被蒸散的影响程度大于VIC,Noah_LSM最低;（2）根据干旱区、半干旱区、半湿润区以及湿润区各站点的分析可知,CLM、SSiB与Noah_LSM中土壤湿度影响蒸散的参数化方案的拟合效果较VIC好,同时在部分站点CLM与SSiB的参数化方案稍优于Noah_LSM。区域之间比较说明,四个模式对干旱半干旱区的模拟效果明显较半湿润区和湿润区好。 相似文献
14.
Dr. R. Reiter Dr. R. Sladkovic Dr. H. -J. Kanter 《Meteorology and Atmospheric Physics》1987,37(1):27-47
Summary Long-term ozone recordings at different altitude levels, conducted in remote areas, can make a valuable contribution to an understanding of the background level of ozone, its periodical variations and possible long-term trends.The measuring stations (three high mountain stations between 740 and nearly 3000 m a.s.l. with small horizontal distance) are described together with recording and calibration procedures. Information is provided on the time history of all recordings since 1978, considering not only the annual means but also the monthly and 10-day means as a function of height. An analysis is presented of the annual variations which differ considerably in the respective height levels and—in three-dimensional diagrams—the correlation between daily and annual variation is shown as a function of height. Then follows a careful parameterization: analysis of the frequency distribution of the ozone concentration, correlation with relative humidity, relative sunshine duration, and temperature. It can be seen that the correlations are very different and partly inverse, depending on the altitude level.Many ozone profiles obtained between valley level and nearly 3000 m a.s.l. (cable car O3 radiosonde) give a picture of the typical ozone profile for different meteorological situations and for the case of stratospheric intrusions of ozone into the troposphere. The stratospheric contribution of ozone to the tropospheric ozone budget is discussed.Since obviously a very high photochemical production rate can be established for ozone in the lowest layer above ground (correlation of O3 with the daily variation of the sunshine duration) it was examined if this O3 variation might be caused only by horizontal transport of ozone from remote areas with high anthropogenic activity by the daily quasiperiodical currents near the ground. But this is not the case.The correlation between ozone concentration, other trace gases such as nitrogen-oxygen compounds and hydrocarbons is shown.With 29 Figures 相似文献
15.
Halogens in the atmosphere chemically destroy ozone. In the troposphere, bromine has higher ozone destruction efficiency than chlorine and is the halogen species with the widest geographical spread of natural sources. We investigate the relative strength of various sources of reactive tropospheric bromine and the influence of bromine on tropospheric chemistry using a 6-year simulation with the global chemistry transport model MOZART4. We consider the following sources: short-lived bromocarbons (CHBr3, CH2BrCl, CHBr2Cl, CHBrCl2, and CH2Br2) and CH3Br, bromine from airborne sea salt particles, and frost flowers and sea salt on or in the snowpack in polar regions. The total bromine emissions in our simulations add up to 31.7 Gmol(Br)/yr: 63 % from polar sources, 24.6 % from short-lived bromocarbons and 12.4 % from airborne sea salt particles. We conclude from our analysis that our global bromine emission is likely to be on the lower end of the range, because of too low emissions from airborne sea salt. Bromine chemistry has an effect on the oxidation capacity of the troposphere, not only due to its direct influence on ozone concentrations, but also by reactions with other key chemical species like HO x and NO x . Globally, the impact of bromine chemistry on tropospheric O3 is comparable to the impact of gas-phase sulfur chemistry, since the inclusion of bromine chemistry in MOZART4 leads to a decrease of the O3 burden in the troposphere by 6 Tg, while we get an increase by 5 Tg if gas-phase sulfur chemistry is switched off in the standard model. With decreased ozone burden, the simulated oxidizing capacity of the atmosphere decreases thus affecting species associated with the oxidation capacity of the atmosphere (CH3OOH, H2O2). 相似文献
16.
A 2-D global chemistry-transport model is set up in this paper.The model simulates the atmospheric ozone distributions well with specified dynamical conditions.The analysis of ozone variation mechanism shows that ozone is chemically in quasi-equilibrium except for the polar night region where the variation of ozone concentration is under the control of dynamical processes,that the oxygen atoms which produce ozone are mainly provided by the photolysis of O2 in the upper stratosphere and by the photolysis of NO2 in the lower stratosphere and the troposphere.and that the ozone is destroyed mainly by NOx:the reactions between NOx and O3 and the odd oxygen cycle contribute 80% to more than 90% of the ozone destruction. 相似文献
17.
A one-dimensional coupled climate and chemistry model has been developed to estimate past and possible future changes in atmospheric temperatures and chemical composition due to human activities. The model takes into account heat flux into the oceans and uses a new tropospheric temperature lapse rate formulation. As found in other studies, we estimate that the combined greenhouse effect of CH4, O3, CF2Cl2, CFCl3 and N2O in the future will be about as large as that of CO2. Our model calculates an increase in average global surface temperatures by about 0.6°C since the start of the industrial era and predicts for A.D. 2050 a twice as large additional rise. Substantial depletions of ozone in the upper stratosphere by between 25% and 55% are calculated, depending on scenario. Accompanying temperature changes are between 15°C and 25°C. Bromine compounds are found to be important, if no rigid international regulations on CFC emissions are effective. Our model may, however, concivably underestimate possible effects of CFCl3, CF2Cl2, C2F3Cl3 and other CFC and organic bromine emissions on lower stratospheric ozone, because it can not simulate the rapid breakdown of ozone which is now being observed worldwide. An uncertainty study regarding the photochemistry of stratospheric ozone, especially in the region below about 25 km, is included. We propose a reaction, involving excited molecular oxygen formation from ozone photolysis, as a possible solution to the problem of ozone concentrations calculated to be too low above 45 km. We also estimate that tropospheric ozone concentrations have grown strongly in the northern hemisphere since pre-industrial times and that further large increases may take place, especially if global emissions of NOx from fossil fuel and biomass burning were to continue to increase. Growing NOx emissions from aircraft may play an important role in ozone concentrations in the upper troposphere and low stratosphere. 相似文献
18.
A one-dimensional, time-dependent model of the physics and chemistry of a warm stratiform cloud is used to study the possible impact of chemical inhomogeneity among cloud and raindrops on the oxidation of SO2 in clouds. The effects of chemical inhomogeneity are examined using two contrasting models: In Model 1 a bulk-solution parameterization is adopted which effectively treats all cloud and raindrops as if they are chemically homogeneous; in Model 2 we allow the cloud and raindrops to have a dichotomous distribution. The dichotomous distribution in Model 2 is simulated by assuming that the two groups of cloud droplets nucleate from two chemically distinct populations of condensation nuclei; one being acidic and the other being alkaline. While the two models yield essentially identical results when the ambient levels of H2O2 are greater than the ambient levels of SO2, the rate of conversion of SO2 to sulfuric acid and the amount of sulfate removed in the precipitation can be significantly enhanced in Model 2 over that of Model 1 under conditions of oxidant limitation (i.e., H2O2 < SO2). This enhancement is critically dependent upon the fraction of alkaline nuclei assumed to be present in Model 2 and arises from the rapid increase in the aqueous-phase reaction between O3+SIV at high pH. Our results suggest that cloud models which adopt a bulk-solution parameterization for cloud droplet chemistry, may underestimate the amount of in-cloud SO2 oxidation under oxidant-limited conditions. 相似文献
19.
K.-Y. Wang J. A. Pyle D. E. Shallcross D. J. Larry 《Journal of Atmospheric Chemistry》2001,38(1):31-71
In part two of this series of papers on the IMS model, we present the chemistry reaction mechanism usedand compare modelled CH4, CO, and O3 witha dataset of annual surface measurements. The modelled monthly and 24-hour mean tropospheric OH concentrationsrange between 5–22 × 105 moleculescm–3, indicating an annualaveraged OH concentration of about 10 × 105 moleculescm–3. This valueis close to the estimated 9.7 ± 0.6 × 105 moleculescm–3 calculated fromthe reaction of CH3CCl3 with OH radicals.Comparison with CH4 generally shows good agreementbetween model and measurements, except for the site at Barrow where modelledwetland emission in the summer could be a factor 3 too high.For CO, the pronounced seasonality shown in the measurements is generally reproduced by the model; however, the modelled concentrations are lower thanthe measurements. This discrepancy may due to lower the CO emission,especially from biomass burning,used in the model compared with other studies.For O3, good agreement between the model and measurements is seenat locations which are away from industrial regions. The maximum discrepancies between modelled results and measurementsat tropical and remote marine sites is about 5–10 ppbv,while the discrepancies canexceed 30 ppbv in the industrial regions.Comparisons in rural areas at European and American continental sites arehighly influenced by the local photochemicalproduction, which is difficult to model with a coarse global CTM.The very large variations of O3 at these locations vary from about15–25 ppbv in Januaryto 55–65 ppbv in July–August. The observed annual O3amplitude isabout 40 ppbv compared with about 20 ppbv in the model. An overall comparison of modelled O3 with measurements shows thatthe O3seasonal surface cycle is generally governed bythe relative importance of two key mechanisms that drivea springtime ozone maximum and asummertime ozone maximum. 相似文献
20.
X. Tie S. Chandra J. R. Ziemke C. Granier G. P. Brasseur 《Journal of Atmospheric Chemistry》2007,56(2):105-125
Satellite measurements of tropospheric column O3 and NO2 in eastern and southeastern Asia are analyzed to study the spatial and seasonal characteristics of pollution in these regions.
Tropospheric column O3 is derived from differential measurements of total column ozone from Total Ozone Mapping Spectrometer (TOMS), and stratospheric
column ozone from the Microwave Limb Sounder (MLS) instrument on the Upper Atmosphere Research Satellite (UARS). The tropospheric
column NO2 is measured by Global Ozone Monitoring Experiment (GOME). A global chemical and transport model (Model of Ozone and Related
Chemical Tracers, version 2; MOZART-2) is applied to analyze and interpret the satellite measurements. The study, which is
based on spring, summer, and fall months of 1997 shows generally good agreement between the model and satellite data with
respect to seasonal and spatial characteristics of O3 and NO2 fields. The analysis of the model results show that the industrial emission of NOx (NO + NO2) contributes about 50%–80% to tropospheric column NO2 in eastern Asia and about 20%–50% in southeastern Asia. The contribution of industrial emission of NOx to tropospheric column O3 ranges from 10% to 30% in eastern Asia. Biomass burning and lightning NOx emissions have a small effect on tropospheric O3 in central and eastern Asia, but they have a significant impact in southeastern Asia. The varying effects of NOx on tropospheric column ozone are attributed to differences in relative abundance of volatile organic compounds (VOCs) with
respect to total nitrogen in the two regions. 相似文献