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1.
The rainwater composition in the vicinity of Mainz, FRG, has been investigated with special emphasis on insoluble constituents. The number size distribution was determined in the range from 0.1 m up to 100 m radius. For particles with r>0.5 m radius the shape of the size distribution of insoluble particles in rain follows the shape of the average urban and rural aerosol. In this particular size range no major size selective removal processes could be seen. For r<0.5 m the number size distribution tends to flatten compared to the average aerosol. This might be the indication of a size selective removal process (Greenfield Gap).  相似文献   

2.
Airborne measurements of the emissions from natural fires, fueled by pyrites and organic materials, at the Smoking Hills in the Northwest Territories, show that they are a regionally significant source of SO2 (0.3 kg s–1 or 104 T yr–1) and particles (0.3 kg s–1). It appears likely that the Smoking Hills are a source for some of the dense, lower-level, haze layers that occur in the North American Arctic.  相似文献   

3.
A liquid jet of 90 m diameter and variable length has been utilized to determine absorption rates and, hence, mass accommodation coefficients , of atmospheric trace gases. The compounds investigated are HCl (0.01), HNO3 (0.01), N2O5 (0.005), peroxyacetyl nitrate (>0.001), and HONO (0.005). It is concluded that the absorption of these trace gases by liquid atmospheric water is not significantly retarded by interfacial mass transport. The strengths and limitations of the liquid jet technique for measuring mass accommodation coefficients are explored.  相似文献   

4.
A method for determining the distribution of supermicrometer nitrate between size-segregated sea-salt and soil derived particles is presented. The analysis is based on field data from six measurements at a coastal site in southern Finland, and on a theoretical treatment taking into account the transfer of gaseous species onto particle surfaces and their subsequent reaction. Significant amounts of nitrate were found in both the particle types, with the fraction of nitrate associated with soil particles varying from 20–50% in the 1–2 m size to near 90% in particles larger than 10 m. Overall, the nitrate accumulation followed closely the relative abundances of these two particle types. Two overlapping modes in supermicron nitrate mass size distributions could be identified. The lower mode, associated with sea-salt, was located between the surface-area and volume distribution of sodium peaking at about 2–3 m of EAD. The upper mode peaked at 3–5 m and followed more closely the surface-area distribution of calcium in all samples. At our site, the accumulation of nitrate into both particle types was shown to be limited by an effective surface reaction rate rather than by gas-phase diffusion. This rate was estimated to be considerably larger for sea-salt particles. Strong evidence in support of the saturation of nitrate in sea-salt particles were obtained.  相似文献   

5.
Thermal and optical techniques were used at Barrow, Alaska during AGASP II (3/20/86–4/7/86) to measure in-situ variability of major aerosol components present in Arctic Haze. The experiment provided continuous data on the concentration, size distribution and relative proportions of sulfate species and refractory aerosol for particle diameters of 0.15 to 5 m. Filter samples were also taken for determination of aerosol optical absorption due to soot (EC-elemental carbon). Although pronounced haze events were absence during this period the haze aerosol present varied in concentration between 2 and 6 g/m3 but showed little change in relative constituents. Apart from local influences, the optical data indicated a persistent fine-mode sulfate aerosol with a NH4 +/SO4 – molar ratio of about 0.4 and a refractory component of somewhat less than 10% by mass. A preliminary comparison of soot estimates determined from the light absorption data with the size distributions of refractory aerosol observed independently by the optical particle counter showed good agreement during the sample period. In the absence of local pollution, values of single scatter albedo derived from light scattering and light absorption showed similar variation about the average value of 0.86 found by us during flights north of Barrow three years earlier during AGASP I.  相似文献   

6.
We present the first application of a multi-stage impactor to study volcanic particle emissions to the troposphere from Masaya volcano, Nicaragua. Concentrations of soluble SO4 2–,Cl–, F–, NO3 –, K+, Na+,NH4 +, Ca2+ and Mg2+ were determined in 11 size bins from 0.07 m to >25.5 m. The near-source size distributions showed major modes at 0.5m (SO4 2–, H+,NH4 +); 0.2 m and 5.0 m (Cl–) and 2.0–5.0 m(F–). K+ and Na+ mirrored the SO4 2– size-resolvedconcentrations closely, suggesting that these were transported primarily asK2SO4 and Na2SO4 in acidic solution, while Mg2+ andCa2+ presented modes in both <1 m and >1 m particles. Changes in relative humidity were studied by comparing daytime (transparent plume) and night-time (condensed plume) results. Enhanced particle growth rates were observed in the night-time plume as well as preferential scavenging of soluble gases, such as HCl, by condensed water. Neutralisation of the acidic aerosol by background ammonia was observed at the crater rim and to a greater extent approximately 15 km downwind of the active crater. We report measurements of re-suspended near-source volcanic dust, which may form a component of the plume downwind. Elevated levels ofSO4 2–, Cl–, F–,H+, Na+, K+ and Mg2+ were observed around the 10 m particle diameter in this dust. The volcanic SO4 2– flux leaving the craterwas 0.07 kg s–1.  相似文献   

7.
Eighteen soil samples from central Sudan were fractionated by dry sieving ina size fraction from <45 m to >300 m while aerosols generatedfrom these soils were fractionated in the particle size range from 0.25 mto >16 m. The elemental concentrations of soil samples were determinedby energy-dispersive X-ray fluorescence, while the elemental concentrationsof generated aerosols were analysed by particle-induced X-ray emission. Theelements Al, K and Rb show a slight positive fractionation with decreasingparticle size throughout the particle size range studied. The concentrationsof Ca, Mn, Fe, Sr and Y are maximum in the small soil size fraction (<45m) and decrease for the coarse soil size fractions, while in the mineralaerosol particle sizes (0.25– > 16 m) the concentrations remainmore or less constant. The size distributions for Cr, Ti and Zr show a maximumin the particle size range 45–100 m and the concentrations of theseelements decrease sharply in the aerosol fraction down to 16 m to remainconstant in the smaller aerosol fractions.Enrichment factors for the elements were calculated relative to five referencematerials: average crustal rock, average soil, the investigated Sahara bulksoil, the finest fraction of this soil and the aerosol generated from thissoil, and using four reference elements: Al, Si, Ti and Fe. The enrichmentfactors were found to vary significantly depending on the choice of thereference material or the reference element. The enrichment factors for theSudan mineral aerosol were almost identical to those for Khartoum atmosphericaerosol but different from those for Namib mineral aerosol and Israelatmospheric aerosol following dust storms. Multivariate display methods(cluster analysis, principal component analysis and linear discriminantanalysis) were applied to the element ratios in the mineral aerosol from theSahara and Namib and this showed that these mineral aerosol can bedifferentiated into different groups. An attempt was also made to relate themineral aerosol to its parent soil through the use of these multivariatetechniques and the elemental ratios in both the mineral aerosols and the bulksoils (Namib and Sahara). It was also possible using the elemental ratios andthe multivariate display methods to associate the crustal component to themineral aerosol generated from the Sahara.  相似文献   

8.
Results from measurements of the composition and size distribution of aerosol particles advected into central Alaska are reported. It is argued that the aerosol predominant in number, but not necessarily in mass, consists of submicron droplets of sulfuric acid. The major aerosol by mass in arctic air is a removal-resistant accumulation mode (radius 0.3 m) probably to large extent originating from pollution sources 103 km upstream (mostly in central Eurasia) from the site in Alaska. The accumulation mode aerosol disappears when arctic air masses are replaced with relatively warmer air masses flowing in from the northern Pacific. The latter air mass systems have been strongly scavenged by clouds and precipitation associated with the Aleutian low pressure system and with forced orographic uplifting over the Alaska Mountain Range; nevertheless the Pacific air masses contain substantial (i.e., 500–1000 cm-3) quantities of small (several hundredths of a micron in radius) particles. Arctic-derived air masses are enriched in large (i.e, 0.3 ) particles compared to Pacific Marine air masses, whereas the opposite trend is found for smaller, Aitken, particles. The smaller particles are found in greatest abundance in warmer air mass systems, presumably because of the relatively brief time since such air masses were last exposed to sunlight with attendant production of small particles from the gas phase.  相似文献   

9.
Radiative Heat Transfer and Hydrostatic Stability in Nocturnal Fog   总被引：1，自引：0，他引：1  
We have performed a one-dimensional and transient radiative heat transfer analysis in order to investigate interaction between atmospheric radiation and convective instability within a nocturnal fog. The radiation element method using the Ray Emission Model (REM2), which is a generalized numerical method, in conjunction with a line-by-line (LBL) method, is employed to attain high spectral resolution calculations for anisotropically scattering fog. The results show that the convective instability has a strong dependence on radiative properties of the fog. For the condition of a 20-m droplet diameter and liquid water content of 0.1 × 10–3 kg m–3;, the temperature profile within the fog becomes S shaped, and a convective instability layer forms in the middle or lower level of the fog. However, for the same water content and a 40-m diameter droplet, no strong convective instability layer forms, whereas for a 10-m diameter droplet a strong convective instability is observed.  相似文献   

10.
Weekly bulk aerosol samples collected at Funafuti, Tuvalu (8°30S, 179°12E), American Samoa (14°15S, 170°35W), and Rarotonga (21°15S, 159°45W), from 1983 through most of 1987 have been analyzed for nitrate and other constituents. The mean nitrate concentration is about 0.11 g m–3 at each of these stations: 0.107±0.011 g m–3 at Funafuti; 0.116±0.008 at American Samoa; and 0.117±0.010 at Rarotonga. Previous measurements of mineral aerosol and trace metal concentrations at American Samoa are among the lowest ever recorded for the near-surface troposphere and indicate that this region is minimally affected by transport of soil material and pollutants from the continents. Consequently, the nitrate concentration of 0.11 g m–3 can be regarded as the natural level for the remote marine boundary layer of the tropical South Pacific Ocean. In contrast, over the tropical North Pacific which is significantly impacted by the transport of material from Asia and North America, the mean nitrate concentrations are about three times higher, 0.29 and 0.36 g m–3 at Midway and Oahu, respectively. The major sources of the nitrate over the tropical South Pacific are still very uncertain. A very significant correlation between the nitrate concentrations at American Samoa and the concentrations of 210Pb suggests that transport from continental sources might be important. This continental source could be lightning, which occurs most frequently over the tropical continents. A near-zero correlation with 7Be indicates that the stratosphere and upper troposphere are probably not the major sources. A significant biogenic source would be consistent with the higher mean nitrate concentrations, 0.16 to 0.17 g m–3, found over the equatorial Pacific at Fanning Island (3°55N, 159°20W) and Nauru (0°32S, 166°57E). The lack of correlation between nitrate and nss sulfate at American Samoa does not necessarily preclude an important role for marine biogenic sources.  相似文献   

11.
Data collected during the french VOVES-1977 experiment are used for the determination of the functionsA() andB() of the stability parameter . It is found that, although pertaining to different geographic conditions, they lead to the same kind of dependency ofA andB upon as found previously considered data. The influence of baroclinicity onA andB is also studied and it is found in that, statistically, consideration of this parameter does not lead either to a decrease of the large scatter of experimental points or to a significant improvement of the similarity theory. It is also shown that a satisfactory estimation of the surface geostrophic wind can be made from the network of meteorological stations, to compute such functions.  相似文献   

12.
Summary The flux of radiation emerging at the top and bottom of a realistic model of a cloud-free, plane-parallel, vertically inhomogeneous turbid atmosphere has been computed for different values of atmospheric turbidity and surface albedo in 83 unequal spectral intervals over the short-wave or solar radiation (0.285–2.5 m) regime. These computations have been utilized to determine the diffusely reflected radiation at the top of the atmosphere in the spectral interval 0.535–0.7035 m (which covers the visible channels of the radiometers onboard the Geosynchronous Operational Environmental Satellites and the NOAA polar orbiting satellites) and in the spectral interval 0.375–0.7035 m. The total global solar radiation (0.285–2.5 m) reaching the surface has also been determined. Simple linear regression relationships have been established between (i) the reflected radiation at the top and atmospheric turbidity and (ii) between the global radiation at the surface and the reflected radiation at the top. These regression relationships yield coefficients of determination very close to unity. The implications of this strong linear dependence of the reflected radiation on atmospheric turbidity and of the global radiation at the surface on the reflected radiation at the top to satellite-based studies of the feasibility of estimation of the insolation (global radiation) at the surface are briefly mentioned.With 3 Figures  相似文献   

13.
Turbulence measurements from a 30 m tower in the stably stratifiedboundary layer over the Greenland ice sheet are analyzed. The observationsinclude profile and eddy-correlation measurements at various levels. Atfirst, the analysis of the turbulence data from the lowest level (2 m aboveground) shows that the linear form of the non-dimensional wind profile(m) is in good agreement with the observations for z/L <0.4, whereL represents the Obukhov length. A linear regression yieldsm=1+5.8z/L. The non-dimensional temperature profile (h) at the2m level shows no tendency to increase with increasing stability. The datafrom the upper levels of the tower are analyzed in terms of both localscaling and surface-layer scaling. The m and the h values show atendency to level off at large stability (z/>0.4) where represents the local Obukhov length. Hence, the linear form of the functions is no longer appropriate under such conditions. The bestcorrespondence to the data can be achieved when using the expression ofBeljaars and Holtslag for m and h. The vertical profiles of theturbulent fluxes, the wind velocity variances and temperature variance arealso determined. The momentum flux profile and the profiles of wind speedvariances are in general agreement with other observations if a welldeveloped low-level wind maximum occurs, and the height of this maximum isused as a height scale.  相似文献   

14.
Zusammenfassung Auf dem Feldberg (1493 m NN) im südlichen Schwarzwald wurden von Januar 1953 bis Mai 1953 und von September 1954 bis Februar 1955 Messungen von Tropfengröße, Wassergehalt und Sichtweite in Wolken durchgeführt. Die Tropfen der einzelnen Spektren haben einen mittleren Durchmesser zwischen 6 und 30 ; die Durchmesser der größten gemessenen Tropfen liegen zwischen 50 und 60 . Der Wassergehalt hat Werte zwischen 0,003 und 1,54 g/m3, wobei über 90% aller Messungen einen Wassergehalt unter 0,50 g/m3 zeigen. Ein einfacher Zusammenhang zwischen Sichtweite, Tropfengröße und Wassergehalt nach derTrabertschen Formel besteht nicht.Eine enge beziehung wurde zwischen der Form der Spektren und dem Niederschlag gefunden. In Zeiten ohne Niederschlag und bei geringfügigem Niederschlag überwiegen schmale ( < 12,0 ), in Zeiten mit länger andauerndem Niederschlag breite Spektren ( > 12,0 ). Eine Ausnahme machen alle Messungen in Hochnebel, die breite Spektren mit zwischen 13 und 17 zeigen, ohne daß Niederschlag fällt.Das gleichzeitige Vorhandensein der drei Phasen Wasserdampf, flüssiges Wasser und Eisteilchen über längere Zeiträume hinweg wurde festgestellt; somit kann die Eiskristall-Niederschlagstheorie vonBergeron und vonFindeisen für den Mechanismus der Niederschlagsbildung nicht im allgemein angenommenen Ausmaß zutreffen. Es erscheint notwendig, die Frage der Wolkenphysik nicht nur thermodynamisch, sondern auch in vermehrtem maß kolloidphysikalisch im Sinne vonSchmauss zu untersuchen.
Summary Measurements of drop size, water content and visibility in clouds have been carried out from January till May 1953 and from September 1954 to February 1955 on the Feldberg (1493 m. a. s. 1.) in the southern Black Forest. The drops of the different spectra have a mean diameter between 6 and 30 ; the diameters of the largest measured drops lie between 50 and 60 . The water content shows values between 0.003 and 1.54g/m3 whereby more than 90 per cent of all measurements lead to a water content below 0.50 g/m3. A simple relation between visibility, drop size and water content according to the formula ofTrabert does not exist.A closed connection between the form of the spectra and the precipitations has been found. In periods without or with only slight precipitation narrow spectra ( < 12.0 ) prevail, in periods with persistent precipitation broad ones ( > 12.0 ). All measurements in elevanted fog make an exception, showing broad spectra with between 13 and 17 without any precipitation.The simultaneous existance of the 3 phases: water vapour, liquid water and ice particles over alonger periods has been stated; the ice crystall precipitation theory ofBergeron andFindeisen for the mechanism of precipitation can therefore not hold in the generally accepted extent. The examination of the problems of cloud physics appears to be necessary, not only in thermodynamical respect, but also in the sense of coloid physics according toSchmauss.
Résumé On a effectué de janvier à mai 1953 et de septembre 1954 à février 1955 au Feldberg (1493 m.) en Forêt-Noire des mesures de grosseur de gouttelettes, de teneur en eau et de visibilité dans les nuages. Les gouttelettes ont und diamètre moyen compris entre 6 et 30 ; les plus grosses mesurent 50 à 60 . La teneur en eau varie de 0,003 à 1,54 g/m3; dans plus de 90% des mesures, elle reste inférieure a 0,5g/m3. Il n'y a pas de relation simple, qui suivrait la formula deTrabert, entre visibilité, grosseur des gouttelettes et teneur en eau.Il existe par contre une relation étroite entre la forme du spectre de fréquence et les précipitations. Lorsque celles-ci sont nulles ou très faibles ce sont les spectres étroit ( < 12,0 ) qui dominent; par précipitations durables, ce sont les spectres larges ( > ). Dans le stratus, sans pluie, les spectres larges ( entre 13 et 17 ) prédominent.On a constaté l'existence simultanée des trois phases solide, liquide et gazeuse pendant d'assez longs intervalles de temps, de sorte que le théorie deBergeron et deFindeisen concernant la genène des précipitations n'a pas la généralité qu'on lui prête. Il apparaît nécessaire d'aborder les problèmes de la physique des nuages non seulement du point de vue thermodynamique, mais aussi de celui de l'état colloïdal au sens deSchmauss.

Mit 9 Textabbildungen.

Hinsichtlich der Wiedergabe von Tabellen und Tropfenspektren stark verkürzte Fassung einer bei der Technischen Hochschule in Karlsruhe eingereichten und genehmigten Dissertation; die hier weggelssene Dokumentation kann zur Einsichtnahme bezogen werden bei den Bibliotheken der Technischen Hochschule Karlsruhe und des Deutschen Wetterdienstes, Offenbach (Main).  相似文献   

15.
A dynamical model for the late-Quaternary global variations of 18O, mean ocean surface tempeature , ice mass I, deep ocean temperature , and atmospheric carbon dioxide concentration , is constructed. This model consists of two diagnostic equations (for 18O and ), and three prognostic equations (for I, , and ) of a form studied extensively in previous articles. The carbon dioxide equation includes forcing by a representation of the Milankovitch earth-orbital radiation effects, and contains a basic instability that drives a free oscillation of period near 100,000 years. The system is constrained to conserve mass and energy, contain physically plausible feedbacks including a system time constant no greater than 10.000 years, and be robust (i. e., structurally stable in the presence of expected noise levels and uncertainties in values of coefficients). Within the limits of these constraints, coefficients are chosen such that (i) the solution gives a good fit to the observed SPECMAP 18O variations, and (ii) the ice mass variations are qualitatively similar to the 18O variations. The predicted long term variations of sea surface temperature and atmospheric carbon dioxide are in reasonably good agreement with the limited observational evidence available for these quantities, while the predicted variations of deep ocean temperature remain to be verified when paleoclimatic estimates of this quantity become available. The relative contributions of ice mass changes and surface water temperature changes to the variations of 18O at any time are given by the model.  相似文献   

16.
Summary ¶In order to better understand land-atmosphere interactions and increase the predictability of climate models, it is important to investigate the role of forest representation in climate modeling. Corresponding to the big-leaf model commonly employed in land surface schemes to represent the effects of a forest, a so called big-tree model, which uses multi-layer vegetation to represent the vertical canopy heterogeneity, was introduced and incorporated into the National Center for Atmospheric Research (NCAR) regional climate model RegCM2, to make the vegetation model more physically based. Using this augmented RegCM2 and station data for China during 1991 Meiyu season, we performed 10 experiments to investigate the effects of the application of the big-tree model on the summer monsoon climate.With the big-tree model incorporated into the regional climate model, some climate characteristics, e.g. the 3-month-mean surface temperature, circulation, and precipitation, are significantly and systematically changed over the model domain, and the change of the characteristics differs depending on the area. Due to the better representation of the shading effect in the big-tree model, the temperature of the lower layer atmosphere above the plant canopy is increased, which further influences the 850hPa temperature. In addition, there are significant decreases in the mean latent heat fluxes (within 20–30W/m2) in the three areas of the model domain.The application of the big-tree model influences not only the simulated climate of the forested area, but also that of the whole model domain, and its impact is greater on the lower atmosphere than on the upper atmosphere. The simulated rainfall and surface temperature deviate from the originally simulated result and are (or seem to be) closer to the observations, which implies that an appropriate representation of the big-tree model may improve the simulation of the summer monsoon climate.We also find that the simulated climate is sensitive to some big-tree parameter values and schemes, such as the shape, height, zero-plane displacement height and mixing-length scheme. The simulated local/grid differences may be very large although the simulated areal-average differences may be much lower. The area-average differences in the monthly-mean surface temperature and heat fluxes can amount to 0.5°C and 4W/m2, respectively, which correspond to maximum local/grid differences of 3.0°C and 40W/m2 respectively. It seems that the simulated climate is most sensitive to the parameter of the zero-plane displacement among the parameters studied.  相似文献   

17.
On the determination of the height of the Ekman boundary layer   总被引：1，自引：1，他引：1  
The heighth of the Ekman turbulent boundary layer determined by the momentum flux profile is estimated with the aid of considerations of similarity and an analysis of the dynamic equations. Asymptotic formulae have been obtained showing that, with increasing instability,h increases as ¦¦1/2 (where is the non-dimensional stratification parameter); with increasing stability, on the other hand,h decreases as –1/2. For comparison, a simple estimate of the boundary-layer heighth u determined by the velocity profile is given. As is shown, in unstable stratification,h u behaves asymptotically as ¦¦–1, i.e., in a manner entirely different from that ofh .  相似文献   

18.
Summary A 25-year (1966–1990) record of measurements of the broadband direct solar irradiances performed in Athens, has been utilized to determine the radiant energy distribution in several spectral bands. Using these data the year-to-year trend of the time sequences of the mean values of the irradiation ratios in the various spectral intervals, viz. blue, green/orange, red, and photosynthetically active radiation (PAR) and the total direct irradiance for the whole spectrum, are evaluated.From this trend the following can be concluded: the blue spectral band (0.380–0.525 m) decreased from the beginning of the examined period until the mid-seventies and then increased gradually; the red band (0.630–0.710 m) shows similar trend but opposite in sense. The PAR band (0.380–0.710 m) decreased slightly until 1985 and then increases. In the green/orange band (0.525–0.630 m) the trend can be considered as nearly constant throughout the examined period. This trend of the irradiation ratios is related to the aerosol and gaseous pollutant content of the atmosphere, which probably reflects the urbanization, industrialization and heavy traffic conditions of the Athens area, during the last three decades.With 2 Figures  相似文献   

19.
Measurements at Barrow during the second Arctic Gas and Aerosol Sampling Program (AGASP-II), conducted in April 1986, showed no rapid long-range transport from lower-latitude source regions to Barrow, and only limited vertical transport from above the boundary layer to the surface. New aerosol size distribution measurements in the 0.005–0.1 m diameter size range using a Nuclepore-filter diffusion battery apparatus showed a median diameter of about 0.01 m during times of high condensation nucleus (CN) concentrations. Aerosol black carbon concentrations exceeding 400 ng m–3 were detected at the surface and were more strongly correlated with CN concentrations than with aerosol scattering extinction (sp), suggesting that aerosol carbon was generally associated with small particles rather than large particles. Measurements at Barrow during AGASP-I, conducted in March–April 1983, showed a series of aerosol events detected at the ground that were caused by rapid long-range transport paths to the vicinity of Barrow from Eurasia. These events were strongly correlated with aerosol loading in the vertical column (optical depth).  相似文献   

20.
Summary The Earths local fair-weather electric field is significantly affected by small ions present in the atmosphere. These ions are typically smaller than 0.001µm and occur in concentrations from 500 to 600cm–3 in air. Attachment to larger aerosol particles may severely decrease the mobility of these atmospheric ions resulting in an increased local electric field. The number concentration of environmental aerosol particles in the size range 0.1 to 5.0µm was measured with two automatic laser scattering particle counters. The Earths electric field was monitored with an electric fieldmeter. Measurements were made in clean air and in an environment highly polluted by wood smoke. The electric field was found to be positively correlated to the aerosol number concentration. During one 24-hour period of measurement, the electric field increased from 180 to about 280Vm–1 as the number concentration of aerosols larger than 0.1µm increased from about 2000 to 9000cm–3. The number concentrations of aerosols larger than 0.1 and 0.3µm were both found to be positively correlated with the Earths electric field with correlation coefficients of 70% and 61%, respectively.Present address: School of Physical Sciences, Queensland University of Technology, Brisbane 4001, Australia.  相似文献   

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