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1.
云南丽江大气气溶胶的化学成分谱分析   总被引:1,自引:0,他引:1  
张仁健  邹捍  沈振兴  王玮 《高原气象》2007,26(6):1319-1323
对云南省丽江玉龙雪山地区大气气溶胶化学元素成分进行了观测和分析.结果表明,丽江玉龙雪山大气气溶胶以Mg、Al、Ca、Si、K和Fe等地壳元素为主,占总元素浓度的82%.丽江地区气溶胶Pb、Se、Br元素浓度均高于珠峰浓度值.丽江气溶胶S、As、Se、Br和Pb等与人类活动有关的气溶胶元素的富集因子很高.这表明丽江地区人类活动影响不容忽略.  相似文献   

2.
青海瓦里关大气气溶胶元素富集特征及其来源   总被引:15,自引:3,他引:15       下载免费PDF全文
利用中子活化及PIXE和可见光灰度仪, 对青海瓦里关大气本底基准监测站的大气气溶胶样品进行了测量。通过元素相对浓度、富集因子和主因子分析等数据统计分析, 并结合同期的气团后退轨迹分布资料, 讨论了瓦里关大气气溶胶元素的组成及来源。结果表明, 位于青藏高原偏远地区的瓦里关大气气溶胶以土壤及地壳等自然来源为主, 因子分析的方差百分数给出瓦里关气溶胶中自然源的贡献率平均在70%以上。燃煤、交通及冶炼等人为源也占有一定比例。大气黑碳气溶胶的观测也表明人类活动影响的存在。人为源的影响多与来自东部及河西走廊等经济发达地区的气流有关。  相似文献   

3.
北京秋季气溶胶化学成分的高分辨率观测及来源分析   总被引:2,自引:0,他引:2  
2001年9月30日~10月6日在北京北三环和北四环之间的中国科学院大气物理研究所气象塔院内使用步进采样仪对气溶胶进行了高分辨率连续采样(每2h采集1个样品),并对样品用PIXE方法进行了元素分析,得到20种元素的浓度。分析结果表明,气溶胶各元素浓度随时间的变化趋势基本一致,且日变化特征显著,早晚出现峰值。降雨期间Ti、Si、Fe等元素浓度急剧下降。S、Pb、Cl、Zn等与人类活动相关的气溶胶元素的富集因子很高。因子分析结果表明,北京秋季大气气溶胶主要源于土壤尘、燃煤尘、工业源和汽车尾气排放等。  相似文献   

4.
重庆冬季大气气溶胶的物理、化学特征   总被引:8,自引:2,他引:8  
利用2001—2002年重庆冬季大气气溶胶粒子观测资料,分析了气溶胶粒子的数浓度、质量浓度、谱分布、化学元素组成及其与气象因子的关系。结果表明,重庆冬季大气气溶胶数浓度与我国其他大城市处于同一水平,大于0.3μm气溶胶粒子的平均数浓度为225.3个/cm^3(最大337.8个/cm^3);冷空气入侵和降水是局地气溶胶的主要清除机制,雾的存在可以显著地改变气溶胶数浓度的一般日变化规律;PM10占TSP(Total Suspended Particles,总悬浮颗粒物)质量浓度的60%~80%;人为污染元素S、zn、As、Ph等在细粒子中富集较高。  相似文献   

5.
五道梁大气气溶胶的化学组成和浓度及其季节变化   总被引:4,自引:3,他引:4  
柳海燕  张小曳 《高原气象》1997,16(2):122-129
利用1993年9-10月和1994年4-5月及7-8月在青藏高原五道梁采集的大气气溶胶元素浓度资料,分析了气溶胶化学组成的总体特征和浓度及其季节变化。结果表明:五道梁低层大气中气溶胶在总体上保持自然大气的组成,以地壳土壤元素为主,由人类活动造成的污染轻微,春季的气溶胶浓度约为秋季的1.75倍,夏季可能与秋季接近,基本上反映了五道梁低层大气气溶胶浓度的季节变化特征。按元素质量深度的季节变化特征可将其  相似文献   

6.
北京地区夏季背景气溶胶的特征   总被引:3,自引:0,他引:3  
本文通过对观测资料的统计分析和比较研究,初步揭示了北京地区夏季背景气溶胶的一些特征,其中包括元素浓度及其变化、富集因子和气溶胶来源等。  相似文献   

7.
北京地区春末-秋初气溶胶理化特性的观测研究   总被引:10,自引:0,他引:10       下载免费PDF全文
分析了1997年5~9月和1998年4~9月北京整层大气气溶胶光学厚度、近地面气溶胶粒子数浓度的日变化、季节变化及其与气象要素的关系,还分析了 1997年5月16日、7月21日和8月2日收集的北京单个气溶胶粒子样品的形态、大小和化学元素组成.结果显示,北京地区春末-秋初整层大气气溶胶光学厚度在0.1~1.6之间变化;气溶胶数浓度(D>0.3μm)为几~几百个/cm3;整层大气气溶胶光学厚度的日变化型式与近地面气溶胶数浓度呈现相反的走向;气溶胶光学厚度和数浓度的日、季节变化显示了整层大气和近地面大气气溶胶与该地区气象、气候条件的关系.气溶胶数浓度与大气相对湿度呈正相关,与风向的关系是偏东风数浓度大,西、西南风数浓度小.电子显微镜分析的结果表明:颗粒物的形态以不规则形、丸形、液态滴形和方形为主;颗粒物化学元素组成有Si、K、S、Al、Mg、Ca、Fe等元素;人类活动排放的Zn、P、Ti、pb、Ba等元素也探测到;北京近地面粒子的一个显著特点是富含Ca和K元素,它们可能分别来自建筑粉尘和有机物的燃烧;给出了一个典型的碳黑粒子和一个粒子经过凝结过程的"卫星"滴环绕的矿物粒子的照片和元素谱图.  相似文献   

8.
中国西部大气清洁地区黑碳气溶胶的观测研究   总被引:48,自引:2,他引:46  
黑碳气溶胶是大气气溶胶中的重要成分,对可见光和红外光都具有强烈吸收作用,对气溶胶的局地及全球的气候效应有重要的贡献。本文给出了1994年7月到1995年底在瓦里关本底台进行的黑碳气溶胶观测结果,结合气象观测资料以及在我国东部地区的部分观测结果对该地区大气中的黑碳气溶胶浓度及其变化特点进行了讨论分析。瓦里关山地区的大气黑碳气溶胶月平均浓度为130~300 ng/m3,大大低于我国东部地区;该地区大气中黑碳气溶胶浓度的变化明显地与来自工业及人口集中地区的污染气团的影响有关,不同风向时的黑碳气溶胶浓度水平有明显的差异;由最大出现频数统计分析得出该地区大气黑碳气溶胶的本底浓度范围为50~120 ng/m3;冬季该地区大气黑碳气溶胶的平均浓度和本底浓度都较低,而春季较高。  相似文献   

9.
南京市大气细颗粒物化学成分分析   总被引:20,自引:3,他引:17  
为了解南京大气细粒子的污染水平和污染特征,在南京市中心鼓楼和北郊南京信息工程大学校内进行了连续1a、每季度5d的大气气溶胶同步采样。用称重法、离子色谱法和电感耦合等离子质谱法分别测得细颗粒物的质量浓度、水溶性离子和元素组成。结果表明,南京地区PM2.1污染比较严重,水溶性离子是细粒子的重要组分,所测6种离子质量浓度总和分别占市区和北郊PM2.1的46.99%、42.32%。PM2.1中的各离子最高浓度都出现在冬季。NH^+4与SO^2-4的相关性好,可能主要以(NH4)2SO4形式存在。温度对SOR和NOR的影响显著,温度升高时SOR值增大而NOR显著减小。通过计算NO^-3与SO^2-4的质量比发现,南京市SO2和NOx主要来自于固定源(如煤的燃烧)。分析细颗粒物中元素含量和富集因子结果表明,Pb、As、Zn、Hg、Cu、Cr、Ni元素的人为污染较明显,且北郊的污染重于市区。比较PM2.1和PM3.3中的离子成分发现,SO^2-4、NH^+4在PM2.1中占据绝对优势,F^-、Cl^-、NO^-2、NO^-3等不在细粒子中占明显优势。从元素组成来看,Pb、Zn在PM2.1细粒子中含量显著,而Ca、Mg、Na等在粗粒子中富集。  相似文献   

10.
2006-2007年冬春季在武汉市湖北大学校区连续采集气溶胶样品,测定气溶胶元素组成,分析气溶胶样品总悬浮颗粒物(TSP)质量浓度,再结合污染源的特征元素组成来确定污染物的来源构成。结果表明:湖北大学校区大气气溶胶污染程度较轻,气溶胶元素以地壳元素为主,其次是具有代表性的人为污染物元素,再次是盐类元素。通过因子载荷分析和相关性分析显示,湖北大学周边地区的建筑源、交通源和餐饮源是湖北大学校区大气的主要污染源。  相似文献   

11.
Observed daily precipitation data from the National Meteorological Observatory in Hainan province and daily data from the National Centers for Environmental Prediction/National Center for Atmospheric Research (NCEP/NCAR) reanalysis-2 dataset from 1981 to 2014 are used to analyze the relationship between Hainan extreme heavy rainfall processes in autumn (referred to as EHRPs) and 10–30 d low-frequency circulation. Based on the key low-frequency signals and the NCEP Climate Forecast System Version 2 (CFSv2) model forecasting products, a dynamical-statistical method is established for the extended-range forecast of EHRPs. The results suggest that EHRPs have a close relationship with the 10–30 d low-frequency oscillation of 850 hPa zonal wind over Hainan Island and to its north, and that they basically occur during the trough phase of the low-frequency oscillation of zonal wind. The latitudinal propagation of the low-frequency wave train in the middle-high latitudes and the meridional propagation of the low-frequency wave train along the coast of East Asia contribute to the ‘north high (cold), south low (warm)’ pattern near Hainan Island, which results in the zonal wind over Hainan Island and to its north reaching its trough, consequently leading to EHRPs. Considering the link between low-frequency circulation and EHRPs, a low-frequency wave train index (LWTI) is defined and adopted to forecast EHRPs by using NCEP CFSv2 forecasting products. EHRPs are predicted to occur during peak phases of LWTI with value larger than 1 for three or more consecutive forecast days. Hindcast experiments for EHRPs in 2015–2016 indicate that EHRPs can be predicted 8–24 d in advance, with an average period of validity of 16.7 d.  相似文献   

12.
Based on the measurements obtained at 64 national meteorological stations in the Beijing–Tianjin–Hebei (BTH) region between 1970 and 2013, the potential evapotranspiration (ET0) in this region was estimated using the Penman–Monteith equation and its sensitivity to maximum temperature (Tmax), minimum temperature (Tmin), wind speed (Vw), net radiation (Rn) and water vapor pressure (Pwv) was analyzed, respectively. The results are shown as follows. (1) The climatic elements in the BTH region underwent significant changes in the study period. Vw and Rn decreased significantly, whereas Tmin, Tmax and Pwv increased considerably. (2) In the BTH region, ET0 also exhibited a significant decreasing trend, and the sensitivity of ET0 to the climatic elements exhibited seasonal characteristics. Of all the climatic elements, ET0 was most sensitive to Pwv in the fall and winter and Rn in the spring and summer. On the annual scale, ET0 was most sensitive to Pwv, followed by Rn, Vw, Tmax and Tmin. In addition, the sensitivity coefficient of ET0 with respect to Pwv had a negative value for all the areas, indicating that increases in Pwv can prevent ET0 from increasing. (3) The sensitivity of ET0 to Tmin and Tmax was significantly lower than its sensitivity to other climatic elements. However, increases in temperature can lead to changes in Pwv and Rn. The temperature should be considered the key intrinsic climatic element that has caused the "evaporation paradox" phenomenon in the BTH region.  相似文献   

13.
Storms that occur at the Bay of Bengal (BoB) are of a bimodal pattern, which is different from that of the other sea areas. By using the NCEP, SST and JTWC data, the causes of the bimodal pattern storm activity of the BoB are diagnosed and analyzed in this paper. The result shows that the seasonal variation of general atmosphere circulation in East Asia has a regulating and controlling impact on the BoB storm activity, and the “bimodal period” of the storm activity corresponds exactly to the seasonal conversion period of atmospheric circulation. The minor wind speed of shear spring and autumn contributed to the storm, which was a crucial factor for the generation and occurrence of the “bimodal pattern” storm activity in the BoB. The analysis on sea surface temperature (SST) shows that the SSTs of all the year around in the BoB area meet the conditions required for the generation of tropical cyclones (TCs). However, the SSTs in the central area of the bay are higher than that of the surrounding areas in spring and autumn, which facilitates the occurrence of a “two-peak” storm activity pattern. The genesis potential index (GPI) quantifies and reflects the environmental conditions for the generation of the BoB storms. For GPI, the intense low-level vortex disturbance in the troposphere and high-humidity atmosphere are the sufficient conditions for storms, while large maximum wind velocity of the ground vortex radius and small vertical wind shear are the necessary conditions of storms.  相似文献   

14.
The spatial and temporal variations of daily maximum temperature(Tmax), daily minimum temperature(Tmin), daily maximum precipitation(Pmax) and daily maximum wind speed(WSmax) were examined in China using Mann-Kendall test and linear regression method. The results indicated that for China as a whole, Tmax, Tmin and Pmax had significant increasing trends at rates of 0.15℃ per decade, 0.45℃ per decade and 0.58 mm per decade,respectively, while WSmax had decreased significantly at 1.18 m·s~(-1) per decade during 1959—2014. In all regions of China, Tmin increased and WSmax decreased significantly. Spatially, Tmax increased significantly at most of the stations in South China(SC), northwestern North China(NC), northeastern Northeast China(NEC), eastern Northwest China(NWC) and eastern Southwest China(SWC), and the increasing trends were significant in NC, SC, NWC and SWC on the regional average. Tmin increased significantly at most of the stations in China, with notable increase in NEC, northern and southeastern NC and northwestern and eastern NWC. Pmax showed no significant trend at most of the stations in China, and on the regional average it decreased significantly in NC but increased in SC, NWC and the mid-lower Yangtze River valley(YR). WSmax decreased significantly at the vast majority of stations in China, with remarkable decrease in northern NC, northern and central YR, central and southern SC and in parts of central NEC and western NWC. With global climate change and rapidly economic development, China has become more vulnerable to climatic extremes and meteorological disasters, so more strategies of mitigation and/or adaptation of climatic extremes,such as environmentally-friendly and low-cost energy production systems and the enhancement of engineering defense measures are necessary for government and social publics.  相似文献   

15.
正AIMS AND SCOPE Atmospheric and Oceanic Science Letters (AOSL) publishes short research letters on all disciplines of the atmosphere sciences and physical oceanography. Contributions from all over the world are welcome.SUBMISSIONAll submitted  相似文献   

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17.
<正>With the support of specialized funds for national science institutions,the Guangzhou Institute of Tropical and Marine Meteorology,China Meteorological Administration set up in October 2008 an experiment base for marine meteorology and a number of observation systems for the coastal boundary layer,air-sea flux,marine environmental elements,and basic meteorological elements at Bohe town,Maoming city,Guangdong province,in the northern part of the South China Sea.  相似文献   

18.
《大气和海洋科学快报》2014,7(6):F0003-F0003
AIMS AND SCOPE
Atmospheric and Oceanic Science Letters (AOSL) publishes short research letters on all disciplines of the atmosphere sciences and physical oceanography. Contributions from all over the world are welcome.  相似文献   

19.
《大气和海洋科学快报》2014,(5):F0003-F0003
AIMS AND SCOPE Atmospheric and Oceanic Science Letters (AOSL) pub- lishes short research letters on all disciplines of the atmos- phere sciences and physical oceanography. Contributions from all over the world are welcome.  相似文献   

20.
正AIMS AND SCOPE Atmospheric and Oceanic Science Letters (AOSL) publishes short research letters on all disciplines of the atmosphere sciences  相似文献   

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