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1.
《Atmospheric Research》2009,91(2-4):211-222
The microphysical structure, chemical composition and prehistory of aerosol are related to the aerosol optical properties and radiative effect in the UV spectral range. The aim of this work is the statistical mapping of typical aerosol scenarios and adjustment of regional aerosol parameters. The investigation is based on the in situ measurements in Preila (55.55° N, 21.00° E), Lithuania, and the AERONET data from the Gustav Dalen Tower (58 N, 17 E), Sweden.Clustering of multiple characteristics enabled to distinguish three aerosol types for clear-sky periods: 1) clean maritime–continental aerosol; 2) moderately polluted maritime–continental aerosol; 3) polluted continental aerosol. Differences between these types are due to significant differences in aerosol number and volume concentration, effective radius of volume distribution, content of SO4− ions and Black Carbon, as well as different vertical profiles of atmospheric relative humidity. The UV extinction, aerosol optical depth (AOD) and the Ångstrom coefficient α increased with the increasing pollution. The value α = 1.96 was observed in the polluted continental aerosol that has passed over central and eastern Europe and southern Russia. Reduction of the clear-sky UV index against the aerosol-free atmosphere was of 4.5%, 27% and 41% for the aerosol types 1, 2 and 3, respectively.  相似文献   

2.
We present results of direct aerosol radiative forcing over a French Mediterranean coastal zone based on one year of continuous observations of aerosol optical properties during 2005–2006. Monthly-mean aerosol optical depth at 440 nm ranged between 0.1 and 0.34, with high Angstrom coefficient (α > 1.2). The single scattering albedo (at 525 nm) estimated at the surface ranged between 0.7 and 0.8, indicating significant absorption. The presence of aerosols over the Mediterranean zone during summer decreases the shortwave radiation reaching the surface by as much as 26 ± 3.9 W m− 2, and increases the top of the atmosphere reflected radiation by as much as 5.2 ± 1.0 W m− 2. The shortwave atmospheric absorption translates to an atmospheric heating of 2.5 to 4.6 K day− 1. Concerted efforts are needed for investigating the possible impact of the increase in heating rate on the maintenance of heat-waves frequently occurring over this coastal region during summer time.  相似文献   

3.
Analyses of cloud condensation nuclei (CCN) number concentrations (cm− 3) measured at the Mace Head Atmospheric Research Station, near Carna, County Galway, Ireland, using a DH Associates Model M1 static thermal diffusion cloud chamber over the period from March 1994 to September 2002 are presented in this work. Air masses are defined as being ‘marine’ if they originate from a wind direction of 180–300° and ‘continental’ air masses are defined as originating from a wind direction of 45–135°. Air masses without such filtering were classified as ‘undefined’ air masses. Air masses were found to be dominated by marine sector air, re-affirming Mace Head as a baseline atmospheric research station. CCN levels for specific air masses at Mace Head were found to be comparable with earlier studies both at Mace Head and elsewhere. Monthly averaged clean marine (wind direction of 180–300° and black carbon absorption coefficient < 1.425 Mm− 1) CCN and marine CCN varied between 15–247 cm− 3 and 54–670 cm− 3, respectively. As expected, significant increases in number concentration were found in continentally sourced CCN over that of marine CCN and were found to follow a log-normal distribution significantly tighter than that of clean marine air masses. No significant trend was found for CCN over the 9-year period. While polluted continental air masses showed a slight increase in CCN concentrations over the winter months, most likely due to increased fuel usage and a lower mixed boundary layer, the dominance of marine sector air arriving at Mace Head, which generally consists of background CCN concentrations, reduced seasonal differences for polluted air. Marine air showed a distinct seasonal pattern, with elevated values occurring over the spring and summer seasons. This is thought to be due to enhanced biogenic aerosol production as a result of phytoplankton bloom activity in the North Atlantic.  相似文献   

4.
Aerosol size spectra (d=10 nm–10 μm) were measured with an electrical aerosol spectrometer (EAS) at Mace Head on the west coast of Ireland. Several small aerosol particle (diameter 10–32 nm) concentration bursts were observed during the measurement period. Relationships between the events, air mass trajectories, tide height, and meteorological parameters are examined. Series of bursts were observed when a spectral transformation due to subsequent particle growth from 10 to 56–100 nm can be identified in an Eulerian experiment. Particle growth rates of between 1 and 3 nm/h were determined. These bursts appear in cold and comparatively clean arctic or polar air masses with temperature and relative humidity fluctuations, and do not correlate with low tide in some cases. These episodes, similar to those frequently found in the continental boundary layer, are thought to occur over a wide area and, for clear detection, require stable airflow for a few days. Elevated small-particle concentration events are more common during low tide or shortly after, and are typically associated with low wind speeds. Here, the increased shore exposure during low tide is thought to influence the nucleation and the subsequent growth of these aerosol particles. The occurrences of the bursts are found to depend on local wind direction. The highest d=10–32 nm particle concentrations appeared for wind sectors furthest from the tidal regions when the wind direction was 150–160°(south-easterly). Most of the events occurred during daytime when solar irradiation is most intense.  相似文献   

5.
Aerosol depolarization ratio and aerosol optical depth (AOD) were measured at Chungli (24.58° N, 121.1° E), Taiwan during the period from 2002–2004. The depolarization ratios of background aerosol have values mostly less than 0.06. The maximum AOD in the altitude range of 0.7 to 2km occurs in the summer (June–August) while between 2 and 5km, the spring (March–May) shows the maximum. The former is mainly related to strong convection and humidity; however the latter is due to anthropogenic aerosols transported from East China and Southeast Asia based on calculations of backward trajectories. This seasonal variation of AOD inferred from different transport mechanisms and aerosol compositions which are supported by the height distributions of aerosol extinction and origins.  相似文献   

6.
Characterization of aerosol optical properties, such as aerosol optical depth, Angstrom exponent, and volume size distribution at the semiarid site of Tombstone Arizona (31°23′N, 110°05′W, 1408 m) will be presented for one annual cycle. In this region, extensive observations of selected optical parameters such as aerosol optical depth (AOD) have been made in the past and reported on in the literature. Less is known about other optical characteristics that are important in climate modeling and remote sensing. New observational techniques and inversion methods allow for the expansion of the earlier information. Observations have been taken with a state of the art sun photometer for a 1-year period and their analysis will be presented here. Monthly mean AODs at 500 nm were found to be in the range of 0.03–0.12; the monthly mean Angstrom exponent ranged from 0.9 to 1.6, being higher in spring and summer and lower in late fall and winter. Volume size distributions exhibit clear dominance of smaller particles, with a gradual increase in size from winter to spring and into summer. Annual variation of the radii of the smaller and the larger particles ranged between 0.05–0.4 and 4–8 μm, respectively. Radiance measurements at 940 nm were used to estimate precipitable water. The retrieved values compared within limits of uncertainty with independently derived estimates from the National Center for Environmental Prediction (NCEP) regional weather forecast model. An interesting outcome from this study was the consistency found in aerosol optical depths as observed in this study and those derived about two decades ago.  相似文献   

7.
Balloon-borne aerosol measurements were performed with an optical particle counter between 1994 and 2000 at Ny-Ålesund (79°N), Svarbard. Throughout the observation period, continuous decay was found in the concentrations of particles with 0.4–0.6 μm in radius in the Arctic stratosphere, suggesting that Pinatubo aerosols remained even at the end of the 1990s. The decay rate was clearly higher for larger particle sizes, and higher at higher altitude (e-folding time of 970–526 days), suggesting a gravitational sedimentation effect. For smaller particles with R<0.4 μm, slight increases in concentration with time were found, which agreed with the measurements at mid-latitude. The sulfate mass mixing ratio in the Arctic stratosphere before 1998 showed values higher than those at middle latitude, while values were almost the same in both regions after 1998. A possible explanation of the latitudinal difference is a time lag (of 0.5–1 year) in the arrival of Pinatubo aerosols in the Arctic.  相似文献   

8.
Summary One of the great unknowns in climate research is the contribution of aerosols to climate forcing and climate perturbation. In this study, retrievals from AERONET are used to estimate the direct clear-sky aerosol top-of-atmosphere and surface radiative forcing effects for 12 multi-site observing stations in Europe. The radiative transfer code sdisort in the libRadtran environment is applied to accomplish these estimations. Most of the calculations in this study rely on observations which have been made for the years 1999, 2000, and 2001. Some stations do have observations dating back to the year of 1995. The calculations rely on a pre-compiled aerosol optical properties database for Europe. Aerosol radiative forcing effects are calculated with monthly mean aerosol optical properties retrievals and calculations are presented for three different surface albedo scenarios. Two of the surface albedo scenarios are generic by nature bare soil and green vegetation and the third relies on the ISCCP (International Satellite Cloud Climatology Project) data product. The ISCCP database has also been used to obtain clear-sky weighting fractions over AERONET stations. The AERONET stations cover the area 0° to 30° E and 42° to 52° N. AERONET retrievals are column integrated and this study does not make any seperation between the contribution of natural and anthropogenic components. For the 12 AERONET stations, median clear-sky top-of-atmosphere aerosol radiative forcing effect values for different surface albedo scenarios are calculated to be in the range of −4 to −2 W/m2. High median radiative forcing effect values of about −6 W/m2 were found to occur mainly in the summer months while lower values of about −1 W/m2 occur in the winter months. The aerosol surface forcing also increases in summer months and can reach values of −8 W/m2. Individual stations often have much higher values by a factor of 2. The median top-of-atmosphere aerosol radiative forcing effect efficiency is estimated to be about −25 W/m2 and their respective surface efficiency is around −35 W/m2. The fractional absorption coefficient is estimated to be 1.7, but deviates significantly from station to station. In addition, it is found that the well known peak of the aerosol radiative forcing effect at a solar zenith angle of about 75° is in fact the average of the peaks occurring at shorter and longer wavelengths. According to estimations for Central Europe, based on mean aerosol optical properties retrievals from 12 stations, the critical threshold of the aerosol single scattering albedo, between cooling and heating in the presence of an aerosol layer, is close between 0.6 and 0.76.  相似文献   

9.
Surface irradiance measurements with high temporal resolution can be used to detect clear skies, which is a critical step for further study, such as aerosol and cloud radiative effects. Twenty-one clear-sky detection (CSD) methods are assessed based on five years of 1-min surface irradiance data at Xianghe—a heavily polluted station on the North China Plain. Total-sky imager (TSI) discrimination results corrected by manual checks are used as the benchmark for the evaluation. The performance heavily relies on the criteria adopted by the CSD methods. Those with higher cloudy-sky detection accuracy rates produce lower clear-sky accuracy rates, and vice versa. A general tendency in common among all CSD methods is the detection accuracy deteriorates when aerosol loading increases. Nearly all criteria adopted in CSD methods are too strict to detect clear skies under polluted conditions, which is more severe if clear-sky irradiance is not properly estimated. The mean true positive rate (CSD method correctly detects clear sky) decreases from 45% for aerosol optical depth (AOD) ≤ 0.2% to 6% for AOD > 0.5. The results clearly indicate that CSD methods in a highly polluted region still need further improvements.摘要根据位于华北平原的重污染站点——香河5年的分钟级别地表太阳辐射和人工订正的全天空成像仪数据, 对21种晴空识别 (CSD) 方法进行了评估:晴空识别准确率较高的方法云天识别准确率较低, 反之亦然;由于CSD 方法采用的参数阈值不适用于污染情况, 当气溶胶含量增加时, 识别准确率呈下降趋势.研究结果显示, 利用太阳辐射数据识别晴空的方法在高污染地区使用时需进行改进.  相似文献   

10.
Summary This study reports a 37-year long record of direct beam spectral irradiance measurements made in Athens, Greece. An analysis of aerosol effects on the spectral distribution of solar radiation through effective optical depths, are presented. Thus, spectrally resolved aerosol optical depths were calculated and analyzed for the period 1954–1990. Summertime aerosol optical depths were found to be larger than winter values, while their seasonal variations were related to varying weather conditions throughout the year. The interrelationships between effective optical depths were found to be linear and were related strongly to microphysics of aerosol loading in the atmosphere. For the period 1962–1983 as wavelength exponent 0 values ranged between 0.76–1.14 the spectrally resolved optical depths were found to increase markedly with respect to remaining periods 1954–1961 and 1984–1990 in which 0 values ranged between 1.16–1.39. A minimum in aerosol optical depths, believed to be near background levels, was reached during period 1954–1957, while there was some indication that both optical depths continued to decrease reaching background levels at the end of the study period. From the long-term variation of aerosol effective optical depths some interesting information on the time evolution of air quality in Athens was gained. In addition, their frequency distribution, temporal daily variations and some remarks on photosynthetically active radiation for plant development, are presented and discussed.With 7 Figures  相似文献   

11.
Direct physical measurements of particle mass and number concentration indicate an increase in overall aerosol mass resulting from cloud processing, most likely through aqueous-phase chemistry (e.g., SO2 oxidation). Measurements conducted in the Pennines of Northern England reveal an average increase of 14 to 20% in dry aerosol mass (0.003<particle diameter<0.9 μm) after aerosol passage through an orographic cloud. The rate of in-cloud mass production is most sensitive to changes in upwind particle size distributions, SO2 concentration, and cloud water acidity. Newly-formed mass appears in size range between 200 and 600 nm and enhances the bimodality of the particle number distribution after cloud processing. Furthermore, the cloud-produced mass is estimated to increase total light scattering, bsp, by 18 to 24%. The scattering efficiency of the dry, cloud-generated aerosol is 5.0±0.3 m2 g−1 and increases to 7.4±0.7 m2 g−1 when adjusted to 90% relative humidity by incorporating particle hygroscopicity data.  相似文献   

12.
Aerosol optical properties are simulated using the Spectral Radiation Transport Model for Aerosol Species(SPRINTARS)coupled with the Non-hydrostatic ICosahedral Atmospheric Model(NICAM). The 3-year global mean all-sky aerosol optical thickness(AOT) at 550 nm, the ngstr m Exponent(AE) based on AOTs at 440 and 870 nm, and the single scattering albedo(SSA) at 550 nm are estimated at 0.123, 0.657 and 0.944, respectively. For each aerosol species, the mean AOT is within the range of the Aero Com models. Both the modeled all-sky and clear-sky results are compared with observations from the Moderate Resolution Imaging Spectroradiometer(MODIS) and the Aerosol Robotic Network(AERONET). The simulated spatiotemporal distributions of all-sky AOTs can generally reproduce the MODIS retrievals, and the correlation and model skill can be slightly improved using the clear-sky results over most land regions. The differences between clear-sky and all-sky AOTs are larger over polluted regions. Compared with observations from AERONET, the modeled and observed all-sky AOTs and AEs are generally in reasonable agreement, whereas the SSA variation is not well captured. Although the spatiotemporal distributions of all-sky and clear-sky results are similar, the clear-sky results are generally better correlated with the observations. The clear-sky AOT and SSA are generally lower than the all-sky results, especially in those regions where the aerosol chemical composition is contributed to mostly by sulfate aerosol. The modeled clear-sky AE is larger than the all-sky AE over those regions dominated by hydrophilic aerosol, while the opposite is found over regions dominated by hydrophobic aerosol.  相似文献   

13.
A data set acquired by eight particle-dedicated instruments set up on the SIRTA (Site Instrumental de Recherche par Télédétection Atmosphérique, which is French for Instrumented Site for Atmospheric Remote Sensing Research) during the ParisFog field campaign are exploited to document microphysical properties of particles contributing to extinction of visible radiation in variable situations. The study focuses on a 48-hour period when atmospheric conditions are highly variable: relative humidity changes between 50 and 100%, visibility ranges between 65 and 35 000 m, the site is either downwind the Paris area either under maritime influence. A dense and homogeneous fog formed during the night by radiative cooling. In 6 h, visibility decreased down from 30 000 m in the clear-sky regime to 65 m within the fog, because of advected urban pollution (factor 3 to 4 in visibility reduction), aerosol hydration (factor 20) and aerosol activation (factor 6). Computations of aerosol optical properties, based on Mie theory, show that extinction in clear-sky regime is due equally to the ultrafine modes and to the accumulation mode. Extinction by haze is due to hydrated aerosol particles distributed in the accumulation mode, defined by a geometric mean diameter of 0.6 μm and a geometric standard deviation of 1.4. These hydrated aerosol particles still contribute by 20 ± 10% to extinction in the fog. The complementary extinction is due to fog droplets distributed around the geometric mean diameter of 3.2 μm with a geometric standard deviation of 1.5 during the first fog development stage. The study also shows that the experimental set-up could not count all fog droplets during the second and third fog development stages.  相似文献   

14.
As a component of the Canadian Arctic Haze Study, held coincident with the second Arctic Gas and Aerosol Sampling Program (AGASP II), vertical profiles of aerosol size distribution (0.17 m), light scattering parameters and cloud particle concentrations were obtained with an instrumented aircraft and ground-based lidar system during April 1986 at Alert. Northwest Territories. Average aerosol number concentrations range from about 200 cm–3 over the Arctic ice cap to about 100 cm–3 at 6 km. The aerosol size spectrum is virtually free of giant or coarse aerosol particles, and does not vary significantly with altitude. Most of the aerosol volume is concentrated in the 0.17–0.50 m size range, and the aerosol number concentration is found to be a good surrogate for the SO4 = concentration of the Arctic haze aerosol. Comparison of the aircraft and lidar data show that, when iced crystal scattering is excluded, the aerosol light scattering coefficient and the lidar backscattering coefficient are proportional to the Arctic haze aerosol concentration. Ratios of scattering to backscattering, scattering to aerosol number concentration, and backscattering to aerosol number concentration are 15.3 steradians, 1.1×10–13 m2, and 4.8×10–15 m2 sr–1, respectively. Aerosol scattering coefficients calculated from the measured size distributions using Mie scattering agree well with measured values. The calculations indicate the aerosol absorption optical depth over 6 km to range between 0.011 and 0.018. The presence of small numbers of ice crystals (10–20 crystals 1–1 measured) increased light scattering by over a factor of ten.  相似文献   

15.
In November 1993 an airborne field study was performed in order to investigate the microphysical and radiative properties of cooling tower water clouds initiated by water vapour emissions and polluted by the exhaust from coal-fired power plants. The number-median diameter of the droplet size distributions of these artificial clouds was in the range of 13 μm. The concentration of smaller droplets (diameters dD < 10 μm) increased with height and horizontal distance from the cooling towers. Close to the cooling towers, bimodal spectra were found with a second mode at 19 μm. The liquid water content (LWC) ranged between 2 and 5 g/m3 and effective droplet radii (Re) between 6 and 9 μm were measured. LWC and Re decreased with altitude, whereas the droplet concentration (ND) remained approximately constant (about 2000 cm−3 ). An enrichment of interstitial aerosol particles with particle diameters (dp) smaller 0.2 μm compared to the power plant plume in the vicinity of the clouds was observed. Particle activation for dm > 0.3 μm. was evident, especially in cooling tower clouds further apart and separated from their sources. Furthermore, radiation measurements were performed, which revealed differences in the vertical profiles of downwelling solar and UV radiation flux densities inside the clouds.The effective droplet radius Re was parameterized in terms of LWC and ND using equations known from literature. The close agreement between measured and parameterized Re indicates a similar coupling of Re, LWC and ND as in natural clouds.By means of Mie calculations, volume scattering coefficients and asymmetry factors are derived for both the cloud droplets and the aerosol particles. For the cloud droplets, the optical parameters were described by parameterizations from the literature. The results show, that the link between radiative and microphysical properties of natural clouds is not changed by the extreme pollution of the artificial clouds.  相似文献   

16.
A high-volume cascade impactor, equipped with a PM10 inlet, was used to collect size-segregated aerosol samples during the summer of 2004 at two Portuguese locations: a coastal-rural area (Moitinhos) and an urban area (Oporto). Concentrations of airborne particulate matter (PM), total carbon (TC), organic carbon (OC), elemental carbon (EC), and water-soluble organic carbon (WSOC) were determined for the following particle size ranges: < 0.49, 0.49–0.95, 0.95–3.0, and 3.0–10 µm. The total PM mass concentrations at the urban and coastal-rural sites ranged from 22.8 to 79.6 μg m− 3 and 19.9 to 28.2 μg m− 3, respectively, and more than 56% of the total aerosol mass was found in the fractions below 3.0 μm. At both locations the highest concentrations of OC and EC were found in the submicrometer size range. The regional variability for the OC and EC concentrations, with the highest concentrations being found in the urban area, was related to the contribution of local primary sources (mostly traffic emissions). It was also verified an enrichment of the small size particles in WSOC, representing on average 37.3(± 12.4)% and 59.7(± 18.0)% of OC in the very fine aerosol at the coastal-rural and urban areas, respectively. The amount of secondary OC calculated by the minimum OC/EC ratio method indicates that secondary organic aerosol formation was important throughout the study at both sites. The obtained results suggest that long-range transport and favourable summer conditions for photochemical oxidation are key factors determining secondary OC formation in the coastal-rural and urban areas. The ultraviolet absorption properties of the chromophoric constituents of the WSOC fractions were also different among the different particle size ranges and also between the two sampling locations, thus suggesting the strong impact of the diverse emission sources into the composition of the size-segregated organic aerosol.  相似文献   

17.
Aerosol optical properties over Solar Village, Saudi Arabia have been studied using ground-based remote sensing observations through the Aerosol Robotic Network (AERONET). Our analysis covered 8 recorded years of aerosol measurements, starting from February 1999 through January 2007. The seasonal mean values of aerosol optical thickness (AOT), the Ångström wavelength exponent α and the surface wind speed (V), exhibit a one year cyclical pattern. Seasonal variations are clearly found in the shape and magnitude of the volume size distribution (VSD) of the coarse size mode due to dust emission. The Spring is characterized by dusty aerosols as the modal value of the exponent α was low ~ 0.25 while that of AOT was high ~ 0.3. The modal value of wind speed was the highest ~ 3.6 m/s in spring. The increase in wind speed is responsible for increasing the concentration of dust particles during Spring. Spring of 2003 has the highest mean values of AOT, V and VSD and the lowest mean value for the exponent α. The seasonal mean values of the exponent α are anticorrelated with those of the wind speed (r = − 0.63). The annual mean values of the exponent α are well correlated (r = 0.77) with those of the difference between the maximum and minimum values of temperature ΔT. They are anticorrelated (r = − 0.74) with the annual mean values of the relative humidity. Large aerosol particles and high relative humidity increase the radiative forcing. This results in reduction of the values of the temperature difference ΔT.  相似文献   

18.
根据位于华北平原的重污染站点——香河5年的分钟级别地表太阳辐射和人工订正的全天空成像仪数据,对21种晴空识别(CSD)方法进行了评估:晴空识别准确率较高的方法云天识别准确率较低,反之亦然;由于CSD方法采用的参数阈值不适用于污染情况,当气溶胶含量增加时,识别准确率呈下降趋势.研究结果显示,利用太阳辐射数据识别晴空的方法在高污染地区使用时需进行改进.  相似文献   

19.
Surface erythemal UV radiation is mainly affected by total column ozone, aerosols, clouds, and solar zenith angle. The effect of ozone on the surface UV radiation has been explored many times in the previous studies due to the decrease of ozone layer. In this study, we calculated the effect of aerosols on the surface UV radiation as well as that of ozone using data acquired from Ozone Monitoring Instrument (OMI). First, ozone, aerosol optical depth (AOD), and surface erythemal UVB radiation measured from satellite are compared with those from ground measurements. The results showed that the comparison for ozone was good with r 2 of 0.92. For aerosol, there was difference between satellite measurements and surface measurements due to the insufficient information on aerosol in the retrieval algorithm. The r 2 for surface erythemal UV radiation was high (～0.94) but satellite measurements showed about 30% larger values than surface measurements on average by not considering the effect of absorbing aerosols in the retrieval process from satellite measurements. Radiative amplification factor (RAF) is used to access the effect of ozone and aerosol quantitatively. RAF for ozone was 0.97～1.49 with solar zenith angle. To evaluate the effect of aerosol on the surface UV radiation, only clear-sky pixel data were used and solar zenith angle and total column amount of ozone were fixed. Also, RAF for aerosol was assessed according to the single scattering albedo (SSA) of aerosols. The results showed that RAF for aerosol with smaller SSA (< 0.90) was larger than that for with larger SSA (> 0.90). The RAF for aerosol was 0.09～0.22 for the given conditions which was relatively small compared to that for ozone. However, considering the fact that aerosol optical depth can change largely in time and space while the total column amount of ozone does not change very much, it needs to include the effect of aerosol to predict the variations of surface UV radiation more correctly.  相似文献   

20.
Measurements from July 4 to July 8, 2005 by a high resolution visible radiometer, a Raman lidar, a ground particulate matter sampler, and ground meteorological sensors have been combined in synergy to infer the intrusion over south-east Italy, of air masses from north-west Sahara, the Atlantic Ocean, and the continental Europe. It is shown that backscatter coefficient, depolarization-ratio, and lidar ratio vertical profiles represent the best tools to detect the intrusion of long range transported air masses and to monitor their effects on the vertical distribution of aerosol optical and microphysical properties. High resolution radiometers are instead important tools to monitor changes on columnar aerosol properties and size distributions.Backscatter coefficient, depolarization-ratio, and lidar ratio vertical profiles have revealed that aerosol optical and microphysical properties significantly changed with time and space during African dust outbreaks: the intrusion of dust particles that at first occurred above 2 km of altitude extending up to 6 km, affected the all aerosol load down to ground within few hours. Aerosol size distributions showed during dust events a clear bimodality with an accumulation mode maximum at 0.24 µm and a coarse mode maximum at 0.94 μm. Conversely, we have found that during the advection of air masses from the Atlantic and continental Europe, aerosol particles were mainly located below 2 km, their optical and microphysical properties were affected by smaller changes in time and space, and were characterized by depolarization ratios rather close to those due to a pure molecular atmosphere. In this case bimodal size distributions with an accumulation mode showing two sub-modes at 0.16 μm and 0.24 μm, respectively and a coarse mode centred at 0.94 μm have also been observed.  相似文献   

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