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1.
李勇 《现代地质》2016,30(3):606-613
为了研究树叶的磁学性质对大气环境污染的指示作用,对安徽省凤阳县城、水泥厂和石英砂厂生长的杨树叶及在凤阳县城生长的银杏树、梧桐树等树叶的磁学参数进行测量。结果显示树叶样品中主要磁性矿物都是磁铁矿,粒径较大;但不同环境生长的杨树叶中磁性矿物含量存在差异,由高到低依次排列为水泥厂、凤阳县城、石英砂厂,指示水泥厂大气环境污染较凤阳县城和石英砂厂严重。进一步分析还发现在凤阳县城采集的杨树、银杏树、梧桐树等树叶样品中磁性矿物含量各不相同,其中银杏树叶中磁性矿物含量高于杨树和梧桐树树叶。利用树叶磁学参数能监测大气环境污染,但不同树种树叶的磁学参数对大气环境污染的指示作用存在差异。  相似文献   

2.
磁学参数作为有效的气候环境变化替代指标,能为古环境演变和沉积物物源研究提供有价值的信息。对取自西菲律宾海西部的GX72柱状样沉积物进行系统的环境磁学研究,测量了磁化率(χ)、非磁滞剩磁(ARM)、等温剩磁(IRM)、磁化率变温曲线(κ-T曲线)、磁滞回线等磁学参数或曲线。结果表明,GX72柱状样沉积物中携磁矿物以低矫顽力磁铁矿为主,粒径以较粗粒准单畴(PSD)为主,这些磁性颗粒主要来源于河流输入的陆源碎屑物质,风成粉尘较少。剖面上多个磁学参数呈现出相同或相反的变化趋势,反映古气候对沉积物磁学性质的制约。χ高值样品通常对应于高饱和等温剩磁(SIRM)值、低ARM/SIRM值、低χARM/χ值以及低χfd值;这类沉积物样品中磁性矿物的含量相对更高,粒度相对较大,可能形成于冷期(相对)。相反,χ低值样品通常对应于低SIRM值、高ARM/SIRM值、高χARM/χ值以及低χfd值,这类样品中磁性矿物的含量相对较低,粒径相对较小,代表相对暖期沉积。  相似文献   

3.
沈明洁  胡守云  U.Blaha  闫海涛  W.R 《第四纪研究》2007,27(6):1113-1120
对北京首都机场高速公路旁采集的土壤柱状T01剖面的磁学参数和金属元素分析,探讨了研究区内现代交通导致的土壤磁学性质的变化及其对环境污染的响应.结果表明,磁参数(χ,ARM和SIRM)与重金属含量呈同步垂向变化趋势.来源于交通运输排放的污染物是土壤剖面上部(0～8 cm)磁性和金属含量增强的主要原因,8cm以下,土壤基本未受到污染,磁性矿物和重金属含量较低,磁性颗粒变化稳定,基本代表了该地区土壤的自然背景.尽管土壤岩石磁学分析表明剖面上下部受污染和未受污染样品的磁载体均是粒度较粗的多畴磁铁矿,但是结合磁参数比值曲线,说明底部样品的磁颗粒的粒度较顶部偏细.磁性矿物的含量变化没有影响磁颗粒的粒度特征.指标聚类等相关分析表明,土壤磁参数(χ,ARM和SIRM)与重金属元素(Pb,Zn和Cu)含量显著相关;结合模糊聚类分析,磁参数可用于追踪、识别交通污染物质在土壤剖面中的富集、迁移状态,揭示不同深度土壤的污染程度.  相似文献   

4.
岩石磁学是古地磁学和环境磁学研究的基础,是鉴定岩石和沉积物中磁性矿物种类、粒度和含量的有效途径。对黄土高原东南部三门峡盆地的水沟—会兴沟旧石器遗址会兴沟剖面黄土—古土壤序列(S_0~S_8)进行系统的岩石磁学研究表明:本剖面沉积物的主要载磁矿物为磁铁矿、磁赤铁矿和赤铁矿,显示准单畴(PSD)磁性颗粒特征。所有磁学参数曲线均表现出基本一致的变化特征,与深海氧同位素曲线能够很好的对应,反映了第四纪以来的冰期—间冰期旋回中,东亚季风影响下的风尘黄土堆积中磁性矿物种类、粒度和含量的周期性变化特征。黄土中高矫顽力磁性矿物的相对含量要高于古土壤中的,而随着成土作用的加强,在古土壤中细粒的低矫顽力磁性矿物显著增加的同时,其中高矫顽力磁性矿物的绝对含量也相应增加。质量磁化率(χ)与非磁滞剩磁磁化率(χ_(ARM))和饱和等温剩磁(SIRM)及磁粒度参数χ_(ARM)/SIRM和χ_(ARM)/χ均呈明显的正相关关系,表明由成土作用产生的单畴(SD)颗粒和较小PSD颗粒对磁化率增强有显著的贡献。  相似文献   

5.
阿勒泰地区表土磁学特性及变化机制研究   总被引：1，自引：0，他引：1  
现代表土的磁学性质反映了物源、成土过程与气候环境之间的重要信息,对认识磁学参数在气候环境研究中的应用有重要意义.干旱区表土的磁学特性表现出极大的复杂性和差异性,为了理解不同气候和环境条件下表土磁学参数的特性、变化机制及控制因素,选择位于新疆北部阿勒泰地区不同景观带的表土样品作为研究对象.通过详细系统的环境磁学分析,并结合X衍射和粒度等方法,结果表明磁性矿物来源相对稳定,磁学性质主要由来自源区的粗颗粒软磁性矿物所主导,xif(低频磁化率)和SIRM(饱和等温剩磁)与磁性颗粒表现出正相关的关系,磁性矿物浓度越大,磁畴颗粒越粗;反之,浓度越低,颗粒越细.磁性矿物的浓度和颗粒大小在不同景观带表现出一.定的差异,荒漠带表土中磁性矿物的浓度较高,磁畴主要为粗颗粒的PSD(准单畴)+MD(多畴),而其他景观带(森林、灌丛、草原和湿地)矿物浓度明显较低,磁畴也相对较细.相比较,其他景观带表土受后期改造作用比荒漠区强,主要是由于在海拔升高到1300m之后,区域气候环境因素(如气温、降水以及蒸发)发生明显变化,导致强磁性矿物的破坏,土壤矿物浓度和粒径发生变化,磁性降低.成壤作用形成的SP(超顺磁畴)颗粒相对较少.  相似文献   

6.
新疆黄土岩石磁学特征与地层性质的对应关系具有鲜明的区域特征.本文选取沙湾黄土剖面进行较为系统的岩石磁学分析.研究结果表明,沙湾剖面的磁性矿物组成与黄土高原及新疆北部其他黄土剖面相似,以亚铁磁性矿物(如磁铁矿、磁赤铁矿)为主要的载磁矿物,同时含有一定量的不完全反铁磁性矿物(如赤铁矿、针铁矿)和顺磁性矿物.假单畴(PSD)和多畴(MD)为样品的主要磁畴特征,部分土壤样品中磁性矿物磁畴状态表现为单畴(SD).进一步分析发现,磁化率与地层对应关系较为复杂,剖面3m以上地层中的磁化率及其他相关磁学参数与成壤强度呈现正相关关系,全新世以来发育的古土壤中磁化率值较高,细颗粒磁性矿物含量也较高;而3m之下地层中磁学参数显著表现为风力强度驱动变化模式.古风场强度的变化可能对剖面整体磁学性质具有一定的影响,成壤作用受到风动力条件的制约,主要决定了较细颗粒磁性矿物的含量变化.xARM/SIRM参数与磁化率相比对地层成壤强度的指示作用更为明显.  相似文献   

7.
为监测水泥粉尘对工业区土壤的影响,在水泥工业区内采集了水泥粉尘、降尘、水泥、粉煤灰、厂内绿地表土及厂周围旱地表土等样品,采用环境磁学方法进行磁学参数测量与矿物成分分析。结果显示所有样品中主要磁性矿物都是磁铁矿,水泥粉尘、水泥厂降尘、水泥、粉煤灰等样品中磁性矿物粒径较粗,主要是准单畴和多畴。被水泥粉尘和降尘污染的厂内绿地表土和厂周围旱地表土的磁学性质发生了明显改变,磁性矿物含量升高,磁性矿物粒径变粗。X射线衍射结果显示,被污染后的厂内绿地表土和厂周围旱地表土中主要矿物成分与水泥粉尘相同,都是石英和方解石。研究发现,土壤的磁学参数(χ_(fd),χ_(ARM)/χ,χ_(ARM)/SIRM)值能反映土壤被污染的程度,其值越低,表示土壤被污染越严重。因此,利用水泥工业区旱地表土磁学参数组合特征,可以监测水泥工业区土壤环境变化。  相似文献   

8.
武昌地区街道尘埃磁学特征及其对环境污染的指示意义   总被引：1，自引：0，他引：1  
对在武昌地区4个功能区域(青山、洪山、东湖风景区、东湖开发区)主要交通街道收集的尘埃样品进行详细的环境磁学测量,包括质量磁化率、频率磁化率、等温剩磁退磁系数以及典型样品的磁滞回线参数等。研究结果表明:尘埃样品中剩磁载体均以亚铁磁性矿物为主,样品中的磁性颗粒呈现低矫顽力的磁铁矿特征,软磁性的磁性矿物是样品剩余磁性的主要载体。尘埃样品χ、SIRM的区域分布特征受区域周围工业、车流量及道路状况等多种环境因素的影响,在4个功能区域中存在明显的磁性差异:青山工业区污染较重,东湖开发区、洪山、东湖风景区次之;硬剩磁(HIRM)的分布可能指示了道路交通来源的磁颗粒特征,东湖开发区和青山工业区由于行驶的货车和重型车辆较多,表现出硬剩磁量值较高。与其他城市(兰州、西安、南京、徐州等)相比,整个武昌地区街道尘埃样品的磁性含量仍较高,说明在城市环境方面还有待于进一步改善和保护。  相似文献   

9.
沉积物中磁性矿物的颗粒大小具有重要环境指示意义,是环境磁学研究的重要内容。磁性参数非磁滞剩磁磁化率/饱和等温剩磁（χARM/SIRM）常被用于指示磁性颗粒大小,当沉积物磁性特征为较粗的多畴（MD）颗粒主导时表现为低值,而为较细的单畴（SD）颗粒主导时表现为高值。本研究对罗布泊盐湖LB剖面的沉积物进行了系统环境磁学测试,结果发现剖面中含有5个χARM/SIRM值低于上覆层和下伏层的层位,指示其磁性颗粒较粗。但磁滞参数和扫描电镜结果显示这5个层位磁性颗粒明显细于上覆层和下伏层沉积物,显示χARM/SIRM在这5个层位的指示意义失真。矿物鉴定结果显示这5个层位的主导磁性矿物为早期成岩成因的SD胶黄铁矿,赋存形态主要为颗粒团聚体、单颗粒或颗粒团聚体附着于硅酸盐矿物表面以及分布于薄片状硅酸盐内,这种赋存形态导致其具有较强的磁相互作用,并限制了χARM的增加,最终造成χARM/SIRM下降,指示意义失真。本研究显示当沉积物中存在胶黄铁矿等自生矿物时,利用比值参数χARM/SIRM判断磁性矿物颗粒特征需谨慎。  相似文献   

10.
亚洲内陆晚新生代干旱化历史及其驱动机制是非常重要的科学问题。选择天山北麓柴窝堡盆地南缘乌鲁木齐河剖面为研究对象,基于磁性地层年代学研究建立的时间标尺,分析了该剖面碎屑沉积物岩石磁学特征及其控制因素,进一步探讨了柴窝堡盆地晚新生代古气候特征。磁性地层年代学研究约束乌鲁木齐河剖面底界年龄为~6.8 Ma,顶界年龄为~3.3 Ma。详细的岩石磁学测量及漫反射光谱分析结果表明,乌鲁木齐河剖面沉积物中磁性矿物主要包括磁铁矿、赤铁矿等,磁学参数χlf、χARM、SIRM、S-100mT、S-300mT、 χARM/SIRM等在~6.3 Ma、~5.2 Ma存在明显变化,揭示磁性矿物粒度、含量等存在相应变化,如在~6.3 Ma前后,磁性矿物颗粒逐渐变粗、含量降低;在~5.2 Ma前后,磁性矿物颗粒逐渐变细后趋于稳定、含量逐渐增多。基于稀土元素分析、沉积粒度与磁学参数相关性分析,认为沉积物源与沉积物粒度不是导致乌鲁木齐河剖面磁学性质变化的主要因素,自~6.8 Ma以来逐步干旱化的气候条件可能是导致该剖面磁学特征变化的重要原因。基于漫反射光谱分析得到的红度与亮度数据结果也揭示了同样的古气候特征。  相似文献   

11.
To monitor environmental implications of cement dust on soil in industrial area, magnetic parameters and mineral compositions were measured by the samples of the cement dust, cement factory dustfall, cement, coal ash, topsoil of green space in the factory and topsoil outside the factory. Results showed that the major magnetic minerals in the samples were magnetite, the magnetic mineral particle size of cement dust, dustfall, cement and coal ash was coarse Multi-Domian (MD) and Pseudo-Single-Domain (PSD). As topsoil of green space in the factory and topsoil outside the factory were polluted by cement dust, their magnetic properties had been obviously changed; the concentration of magnetic minerals elevated and particle size became coarser. The magnetic parameters (χfd,χARM/χ,χARM/SIRM) value can reflect the pollution level of the soil, the lower its value was, the more serious soil was polluted. X-ray diffraction results showed that the mineral compositions of the topsoil of green space in the factory and topsoil outside the factory were quartz and calcite, which were the same as cement dust. Magnetic parameters combination characteristics of topsoil can monitor the soil environmental changes in cement industry area.  相似文献   

12.
Detailed magnetic and geochemical measurements were performed on urban roadside soils collected from Lishui city, China, to establish a possible link between the enhanced concentration of traffic-related magnetic particles and heavy metals. Relatively higher magnetic susceptibility (mean: 124.1 × 10−8 m3 kg−1) and concentrations of metals (Cd, Cu, Pb and Zn) were observed for roadside soils. Concentration-dependent magnetic parameters (χ and SIRM) are highly significantly positively correlated to the concentration of metals (Ca, Cr, Ni, Cu, Zn, Cd, Pb, Fe, and V), but not significantly correlated with As, Mn, Co, Mg, and K. The principal component analysis showed that χ and SIRM significantly correspond to elements Ca, Cd, Cu, Pb, and Zn. The χ and SIRM also have significant linear correlation with integrated pollution index, indicating that χ and SIRM can be used as effective proxy indicators for the pollution of heavy metals. Magnetite in the pseudo-single-domain/multidomain (PSD/MD) grain size was identified as the dominant magnetic carrier by temperature-dependent measurements of saturation magnetization (Ms–T curve), XRD and hysteresis loops. Field emission scanning electron microscopy and energy dispersive X-ray spectroscopy (EDS) analysis of the magnetic particles revealed the presence of large traffic-related angular-subangular, blocky, and spherical iron oxide particles. These iron oxide particles are typical for particles produced by traffic-related anthropogenic activities. It is concluded that vehicle emissions may be the major source of elevated heavy metals and magnetic particles in roadside soils. The results proved the applicability of magnetic method in detecting roadside pollution derived from vehicle emissions.  相似文献   

13.
《Applied Geochemistry》2000,15(7):891-900
Pb isotope composition of tree rings (Celtis Australis) and urban aerosols have been determined to assess whether arboreal species can be used as bio-geochemical tracers of the evolution of heavy metal pollution to the environment. Particular care was paid to setting up a high quality analytical technique to work with arboreal species with low Pb content. The Pb isotope composition of tree rings from 1950 to 1995 is within the range of European aerosols and is correlated with the temporal evolution of Pb isotopes measured in air particulates from Firenze. The entire data set (tree rings and air particulates) demonstrate that Pb isotope composition of tree rings can be used successfully as a proxy of the atmospheric Pb isotope composition of urban areas. This, in turn, suggests that tree rings are potentially a powerful bio-geochemical tracer for monitoring air pollution history due to human activities.  相似文献   

14.
A magnetic signature of tree rings was tested as a potential paleo-climatic indicator. We examined wood from sequoia tree, located in Mountain Home State Forest, California, whose tree ring record spans over the period 600 – 1700 A.D. We measured low and high-field magnetic susceptibility, the natural remanent magnetization (NRM), saturation isothermal remanent magnetization (SIRM), and stability against thermal and alternating field (AF) demagnetization. Magnetic investigation of the 200 mm long sequoia material suggests that magnetic efficiency of natural remanence may be a sensitive paleoclimate indicator because it is substantially higher (in average >1%) during the Medieval Warm Epoch (700–1300 A.D.) than during the Little Ice Age (1300–1850 A.D.) where it is <1%. Diamagnetic behavior has been noted to be prevalent in regions with higher tree ring density. The mineralogical nature of the remanence carrier was not directly detected but maghemite is suggested due to low coercivity and absence of Verwey transition. Tree ring density, along with the wood's magnetic remanence efficiency, records the Little Ice Age (LIA) well documented in Europe. Such a record suggests that the European LIA was a global phenomenon. Magnetic analysis of the thermal stability reveals the blocking temperatures near 200 degree C. This phenomenon suggests that the remanent component in this tree may be thermal in origin and was controlled by local thermal condition.  相似文献   

15.
Magnetic parameters have been widely used as a rapid, cost-effective, and non-destructive method. To assess whether their magnetic properties reflect the development history in the Pearl River Delta, three sediment cores collected from South China coastal waters were selected for magnetic research. The results indicate that the predominant ferrimagnetic mineral is magnetite, with an additional smaller amount of surprisingly high-coercive greigite. Fine-grained superparamagnetic and single-domain particles of magnetite and the relative contribution of greigite are increased when the total concentration of ferrimagnetic minerals is higher. Three well-known stages of the Chinese history, i.e., iron smelting, cultural revolution, and the latest phase of opening and reforming were identified in the vertical variation of magnetic concentration parameters. Although the record of the three cores is not completely consistent, the results point out that magnetic concentration parameters can reflect the development and pollution history in surrounding coastal areas.  相似文献   

16.
Dendrogeomorphic research has long relied on scarred trees to reconstruct the frequency of mass‐movement processes. Injuries have mostly been dated macroscopically by counting the tree rings formed after wounding. Tree‐ring anatomical anomalies induced by cambial injury, in contrast, have only recently been recognized as proxy records of past events. We investigated 12 sub‐arctic downy birch (Betula pubescens Ehrh.) trees scarred by snow avalanches in Norway and Iceland. Earlywood vessel lumina were measured for each tree in the xylem tissue bordering the scars. Seven successive rings were examined, namely two control rings laid down prior to wounding and five rings in the wound xylem. We provide evidence that snow‐avalanche‐induced wounding resulted in atypically narrow earlywood vessels over at least two years. Our data demonstrate that wound‐associated vessel anomalies represent tangible markers of mass‐movement processes, and as such make a viable tool for reconstructing past events. Similar dendrogeomorphic studies based on tree‐ring anatomy can be readily conducted with other mass‐movement processes, as well as with other broad‐leaved tree species. Ultimately, this new approach will foster increment coring over more invasive sampling techniques.  相似文献   

17.
In this study, environmental magnetic, heavy metal and statistical analyses were conducted on 21 surface sediments collected from Chennai coast, India, to examine the feasibility of heavy metal pollution using magnetic susceptibility. The Chennai coastal sediment samples are dominated by ferrimagnetic minerals corresponding to magnetite-like minerals. The percentage of frequency dependent magnetic susceptibility reflects the presence of super-paramagnetic/single domain magnetic minerals in Chennai harbour, Cooum and Adayar rivers sediments. High pollution load index in sample E1, E2, CH7, C11, C12 and A16 is mainly due to anthropogenic activities such as, harbour activities, Cooum and Adayar rivers input and industrial effluent. Factor analysis shows that the magnetic concentration dependent parameters (χ, χ ARM and SIRM) covary with the heavy metal concentrations, suggesting that the input of magnetic minerals and heavy metals in Chennai coastal sediments are derived from the same anthropogenic sources. Strong correlation obtained between pollution load index (PLI) and concentration dependent parameters (χ, χ ARM and SIRM) for the polluted samples with magnetic susceptibility excess of 50×10 − 8 m3kg − 1. Significant correlations between heavy metals and magnetic susceptibility point out the potential of magnetic screening/monitoring for simple and rapid proxy indicator of heavy metal pollution in marine sediments.  相似文献   

18.
Annual growth rings of a common hardwood species, Picea abies L., were investigated as a potential archive of past atmospheric Pb pollution. Wide distribution of trees in terrestrial settings and straightforward chronology are two advantages of this potential geochemical archive, but several processes described in the literature may obscure the trends in past Pb deposition. These confounding factors include, e.g., radial post-depositional mobility of Pb in xylem, and ecosystem acidification leading to higher bioavailability of Pb. One- to five-year annual wood increments were analyzed for Pb concentrations and 206Pb/207Pb ratios at Jezeri (JEZ), Uhlirska (UHL) and Na Lizu (LIZ), three sites in the Czech Republic, differing in atmospheric Pb loads. Three to four trees per site were included in the study. Distinct Pb concentration maxima between 1960 and 1990 at the two heavily polluted sites (JEZ and UHL) coincided with historical Pb emissions known from inventories of industrial production. No Pb concentration maxima were found at one site, LIZ, situated in a national park 150 km from major pollution sources. Spruce tree rings from JEZ, located just 5 km from coal-burning power stations, contained a large proportion of coal-derived Pb (a high-206Pb/207Pb ratio of 1.19). A coal-related maximum in 206Pb/207Pb in JEZ tree rings was found using two different analytical techniques, laser-ablation multi-collector ICP MS, and single-collector sector-field ICP MS. In a three-isotope graph (206Pb/207Pb vs. 208Pb/207Pb), tree-ring data plotted into the field of ombrotrophic (i.e., rain-fed) peat bogs, suggesting negligible contribution of bedrock-derived Pb in the xylem. We concluded that none of the potential confounding factors played a major role at our sites. Annual growth rings of P. abies in Central Europe faithfully recorded historical changes in atmospheric Pb depositions.  相似文献   

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