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1.
Records from lake sediment cores are critical for assessing the relative stability of climate and ecosystems over the Holocene. Duck Lake in south-central Lower Michigan, USA, was the focus of a study that identified how changes in the geochemical variables in lake sediments relate to variations in regional climate and local land use during the Holocene. More than 8.5 m of lacustrine sediment were recovered using Livingston and freeze corers and analyzed for organic carbon, inorganic (carbonate) carbon, total nitrogen, and trace metals. Repeating packages of sediment (1–10 cm thick) that grade from light (inorganic carbon-rich) to dark (organic carbon-rich) were found from the surface to a depth of about 8 m. Variations in the high-resolution gray scale data from core X-radiographs are highly correlated to the relative amount of inorganic carbon. Geochemical analyses of the upper 8.5 m of sediment revealed a wide range of values: 0.05–10.6% for inorganic carbon (i.e. 0.5–89% calcium carbonate) and 1.1–28% for organic carbon (i.e. 2.7–70% organic matter). Organic carbon to nitrogen ratios indicate that most of the sediment organic matter is produced within the lake. A core chronology based on eight AMS radiocarbon dates shows low sediment accumulation rates (0.05 cm/year) from 10,000 to 3,800 cal year BP and higher sediment accumulation rates (0.1–0.3 cm/year) from 3,800 cal year BP to present. We suggest that carbonate accumulates during relatively dry times, whereas organic matter accumulation dominates when nutrient input to the lake is enhanced by wetter climate. The Duck Lake core records a distinct low point in inorganic carbon deposition that may be related to the 8.2 ka cooling event now documented from several sites in North America. Spectral analysis of gray scale values shows significant ~200-year periodicities over the past 8,000 years, hypothesized to result from climate changes induced by solar forcing. Concentrations of trace metals (e.g. lead, iron, copper, zinc) indicate the onset of regional anthropogenic influence about 150 cal year BP.  相似文献   

2.
High-resolution quantitative analysis of ostracod assemblages from 4.3-m-thick freshwater tufa-rich sediments, deposited during the last 12.8 ka in Lake Sinijärv, northern Estonia, yielded information on water level, trophic state conditions, and temperature changes since the late glacial. AMS 14C dates from aquatic mosses provided time constraints on the palaeoenvironmental development of the region. In the ostracod assemblage structure, four faunal zones (OFZ) were determined. The most significant change in the ostracod fauna occurred at 10,590 cal. y BP, when a typical littoral, polythermophilic fauna was replaced by a mostly sublittoral, species-rich meso- to stenothermophilic fauna. The ostracod data indicate two major low-water-level periods in the lake at 12,800–10,590 and 7,600–3,700 cal. y BP. Sediment analysis indicates the most intensive tufa precipitation occurred during these low stand periods, rather than during the warmest climate in Estonia between 8,000 and 4,500 cal. y BP. The late glacial low water level in the groundwater-fed Lake Sinijärv at 12,800–10,590 cal. y BP coincides partly with the regression in the Lake Peipsi basin (14,000–12,100 cal. y BP) and with the last drainage event of the Baltic Ice Lake at 11,600 cal. y BP. The low-water-level period in Lake Sinijärv occurred earlier than in lakes in the SE sector of Scandinavian glaciation. The change from low to high water level in Lake Sinijärv at 10,590 cal. y BP preceded the first post-glacial transgression events in the small lowland lakes of Estonia, southern Sweden, Poles`ye in Belarus, and Valday in NW Russia. In general, the mid-Holocene low-water-level period in Lake Sinijärv between 7,600 and 3,700 cal. y BP is concurrent with the regressions in the lakes of the SE sector of Scandinavian glaciation.  相似文献   

3.
Stable isotope measures in organic matter are frequently used as indicators of past climate change. Although such analyses can provide valuable information, there is considerable uncertainty associated with studies of organic-rich sediments, especially those from Arctic lakes and bogs. We studied stable isotopes of carbon and nitrogen, and magnetic properties in a sediment core from a small alkaline lake with a high sedimentation rate, Lake Nattmålsvatn, Norway. There is good correspondence among the different sediment variables during the late glacial, and they seemingly reflect major climate variations such as the Allerød Interstade and the Younger Dryas, as well as the transition into the current interglacial. During the early Holocene, however, these relationships are more complex and δ13C and δ15N values do not stabilize until ~7,500 cal year BP. A significant excursion in all variables occurs between 6,850 and 6,500 cal year BP and is interpreted to represent climate deterioration. Holocene δ13C values vary little and indicate that isotopically-depleted dissolved inorganic carbon (DIC) in the lake, possibly influenced by methanotrophy and high pCO2, dominated the lake’s carbon cycle. Holocene δ15N is similarly muted, likely due to the availability of abundant dissolved nitrogen. Bulk organic matter is probably dominated by phytoplankton remains produced beneath the ice cover in late spring and during ice breakup when isotopically-depleted DIC, pCO2 and ammonium availability were maximal. Thus, use of δ13C and δ15N as indicators of Holocene paleoclimate and paleoproductivity variation can be challenging in a lake such as Nattmålsvatn, where ice cover isolates the basin for large parts of the year, allowing dissolved respiratory gases to accumulate in the water column. In contrast, magnetic variables appear to better track climate variations. In particular, runoff-driven influx of minerogenic sediments shows high variability that can be attributed to regional changes in Holocene winter precipitation. The most striking shifts occur between 4,000 and 2,300 cal year BP.  相似文献   

4.
Human activity and climatic forcing have influenced sedimentation in three of Finland's deepest lakes during the last centuries. High-resolution sediment sequences of Lake Päijänne, Lake Pääjärvi and Lake Pyhäjärvi represent records of the last 440 years, 839 years and 633 years, respectively. The accumulation rates of dry matter, organic carbon and biogenic silica refer to changes in human activity in the catchments. However, they also reveal the importance of climatic forcing on lake sediment deposition. A significant correlation was found between instrumentally measured records of temperature (163 years) and precipitation (148 years), and varve thickness. Warm winter months indicating a short ice-cover period have the strongest control on varve thickness. This shows that wind-driven resuspension of littoral material is the forcing mechanism of climate on lake sediments. The long-term human-induced erosion pulses observed may even have magnified the climatic signals in some cases. Nevertheless, increased anthropogenic field erosion in the catchment, and the associated leaching of bioavailable nutrients, hampers the observation of climate signals, especially during the last 50 years, in the lakes studied.This is the second paper a series of papers published in this issue on high-resolution paleolimnology. These papers were presented at the Sixth International Palaeolimnology Symposium held 19-April, 1993 at the Australian National University, Canberra, Australia. Dr A. F. Lotter and Dr. M. Sturm served as guest editors for these papers.  相似文献   

5.
Three sediment cores from two lakes, Fish Lake and Phalarope Lake, in Truelove Lowland, Devon Island, N.W.T. were analyzed for diatoms and chemical composition. Multivariate statistical techniques using a range of chemical variables successfully isolated three sediment groupings in the cores. Allochthonous and autochthonous chemical components in the sediments have been used to reconstruct paleoenvironmental conditions. The two lakes began approximately 10600 years ago as shallow marine lagoons that were isolated from the sea as a result of glacio-isostatic rebound. Based on the presence of distinctive diatom assemblages, the three stratigraphic zones are identified as a basal marine zone, an intermediate and transitional brackish/marine zone and an upper freshwater zone. Following isolation from the sea, the lakes were flushed with freshwater produced by snow and ice melt. In Fish Lake, the period of transition from marine to freshwater, which began approximately 7000 years ago, lasted approximately 800 years. In Phalarope Lake, which was isolated from the sea approximately 5000 years ago, flushing by fresh water was completed only within the last 300 years. Fe, Cr, and Mo in the sediments are associated with the isolation phase when lake sedimentation is sensitive to the presence of brackish water and erosion within the lake catchments. In particular, the precipitation of Mo as MoS2 reflects the presence of hypolimnetic anoxia associated with lake isolation. During the early post-isolation phase the response of lake biota to an influx of nutrients is reflected in an increase in biological silica and organic carbon in the lake sediments. On the other hand, the generally low organic content of the sediments indicates that sedimentation in these lakes has been largely determined by variations in non-biogenic factors through time. During the mid Holocene the progressive stabilization of surface materials within the lake catchments is marked by decreasing Cr, As and Na in the sediments. At the same time, an increase in allochthonous Mn and Fe is attributed to progressive soil development. During the last 2500 years the catchments have experienced decreased erosion resulting in a decrease in both allochthonous clastic input and lake productivity.  相似文献   

6.
Lake Annecy sediments have been studied to provide an insight into the evolution of the lake trophic state in response to climate changes during the Holocene. Determination of the concentration of carbonate, Fe, Mn, and different forms of P in conjunction with total sediment fluxes derived from 14C ages allows an estimation of yearly fluxes of these sediment components. High fluxes of endogenic carbonate occur during the early to middle Holocene. Non apatitic inorganic phosphorus flux is variable but shows some higher-than-present values during this period. These observations are interpreted as being a result of enhanced productivity by favourable conditions for phytoplankton development. In addition, the low Mn/Fe ratio of the redox-sensitive forms of these elements recorded during this period suggests low oxygen concentrations in the bottom waters. Therefore it appears that the lake may have undergone oxygen depletion in the bottom water during the warmer-than-present periods, due to increased productivity and subsequent oxygen consumption from the decay of organic matter. With future climate changes, this suggests that lake water quality may likely degrade under global warming.  相似文献   

7.
Sediment cores from the shallow and deep basins of Pyramid Lake, Nevada, revealed variations in composition with depth reflecting changes in lake level, river inflow, and lake productivity. Recent sediments from the period of historical record indicate: (1) CaCO3 and organic content of sediment in the shallow basin decrease at lower lake level, (2) CaCO3 content of deep basin sediments increases when lake level decreases rapidly, and (3) the inorganic P content of sediments increases with decreasing lake volume. Variations in sediment composition also indicate several periods for which productivity in Pyramid Lake may have been elevated over the past 1000 years. Our data provide strong evidence for increased productivity during the first half of the 20th Century, although the typical pattern for cultural eutrophication was not observed. The organic content of sediments also suggests periods of increased productivity in the lake prior to the discovery and development of the region by white settlers. Indeed, a broad peak in organic fractions during the 1800's originates as an increase starting around 1600. However, periods of changing organic content of sediments also correspond to periods when inflow to the lake was probably at extremes (e.g. drought or flood) indicating that fluctuations in river inflow may be an important factor affecting sediment composition in Pyramid Lake.  相似文献   

8.
Geochemical analysis of 210Pb-dated sediment cores from Otisco Lake (New York) combined with analysis of recent land cover change in the watershed revealed the history of land use change, lake management, and industrial pollution since European settlement in the northeastern US. Clearance of forestland for agriculture characterized the early settlement era that was marked in the Otisco Lake sediments by a decline in organic carbon (OC) and OC:N ratios, which indicate a change in the sources of organic matter to the lake. Agricultural land use reached its greatest areal extent in the Otisco watershed around 1900, followed by field abandonment and reforestation over the last century. In the 1920s sediment accumulation rates began to increase coincident with residential development along the lake shore. Nitrogen and organic carbon, which are transported from the watershed, show increased fluxes to the lake in response to this change. Deposition of inorganic carbon increased markedly over a short period from the 1940s to the 1980s, which is consistent with enhanced mobilization of watershed calcium by increased acidic deposition, followed by alkalinization of the lake waters and calcite precipitation. An increase in copper content in the sediments reflects application, since 1942, of the algicide copper sulfate to the lake waters to control algal blooms. This CuSO4 marker confirmed the accuracy of the 210Pb chronology. Atmospheric mercury (Hg) fluxes to the lake were affected by increased sediment transport from the watershed. The maximum Hg peak in the sediment record, however, was dated to the early 1970s and coincides with maximum Hg emissions to the atmosphere in the Great Lakes region.  相似文献   

9.
Major components of lacustrine sediments, such as carbonates, organic matter, and biogenic silica, provide significant paleoenvironmental information about lake systems. Fourier transform infrared spectroscopy (FTIR) and scanning X-ray fluorescence (XRF) techniques are fast, cost effective, efficient methods to determine the relative abundances of these components. We investigate the potential of these techniques using sediments from two large lakes, Lake Malawi in Africa and Lake Qinghai in China. Our results show statistically significant correlations of conventionally measured concentrations of carbonate (%CaCO3), total organic carbon (%TOC), and biogenic silica (%BSi), with absorbance in the corresponding FTIR spectral regions and with XRF elemental ratios including calcium:titanium (Ca/Ti), incoherent:coherent X-ray scatter intensities (Inc/Coh), and silicon:titanium (Si/Ti), respectively. The correlation coefficients (R) range from 0.66 to 0.96 for comparisons of FTIR results and conventional measurements, and from 0.70 to 0.90 for XRF results and conventional measurements. Both FTIR and XRF techniques exhibit great potential for rapid assessment of inorganic and organic contents of lacustrine sediments. However, the relationship between XRF-ratios or FTIR-absorbances and abundances of corresponding sedimentary components can vary with sediment source and lithology.  相似文献   

10.
Paleohydrological changes in an Amazonian floodplain lake: Santa Ninha Lake   总被引：1，自引：0，他引：1  
Holocene environments have been reconstructed by sedimentological, mineralogical and organic geochemical analysis of a 270-cm core from Santa Ninha Lake, a floodplain lake in lower Amazonia. Dated by fourteen AMS-radiocarbon dates, the sediment core has a basal age of 5,600?cal?years BP and different sedimentary units were identified. These units document various hydrologic phases in the evolution of this lake. Reduced Amazon River influence, with reduced high-water levels of the river, characterized the period between 5,600 and 5,100?cal?years BP. Comparison with other Amazonian and Andean paleoclimate studies point to a dryer climate during this phase. After 5,100?cal?years BP coarse sediments and quartz increase which suggest a higher inflow of the Amazon River. Between 5,000 and 2,300?cal?years BP the coarse sediments and quartz remain high but the organic carbon showed the lowest values. The riverine inflow caused dilution of the organic material produced in the lake and consequently low rates of carbon flux in these phases were recorded. These results show that the hydrodynamics of the Amazon River strongly influence the behavior, productivity and consequently the sedimentation process in the floodplain lakes.  相似文献   

11.
This paper reports a first estimate of the Holocene lake sediment carbon pool in Alberta, Canada. The organic matter content of lake sediment does not appear to depend strongly on lake size or other limnological parameters, allowing a simple first estimate in which we assume all Alberta lake sediment to have the same organic matter content. Alberta lake sediments sequester about 15 g C m-2 yr-1, for a provincial total of 0.23 Tg C yr-1, or 2.3 Pg C over the Holocene. Alberta lakes may represent as much as 1/1700 of total global, annual permanent carbon sequestration.  相似文献   

12.
Human-induced perturbations in the Lake Norrviken catchment, Sweden, over the last 100+ years have left distinctive geochemical imprints in the sediments. Disposal of sewage, industrial, and agricultural run-off into the lake since the end of the nineteenth century changed the trophic status from eutrophic to hyper-eutrophic. The primary organic matter (OM) source in the lake is in situ algal material. Total organic carbon (TOC) concentrations increased near the mid-section of a short sediment core collected from the deepest part of the lake, reflecting elevated epilimnetic productivity and consequent hypolimnetic anoxia. Accompanying shifts to lighter stable organic C and total N isotopic compositions suggest that cyanobacterial productivity increased during this period. The distribution of pigments in the core indicates a shift in the phytoplankton community to a cyanobacteria-dominated system. Moreover, pigments confirm that N2-fixing versus non-N2-fixing phytoplankton varied depending upon the external inputs of N and P. Conditions in the lake improved after sewage input was diverted and the lake is currently mesotrophic.  相似文献   

13.
The primary producer community of Lake Apopka, a large (125 km2), shallow (mean depth, 1.7 m), polymictic Florida lake, shifted from macrophyte dominance to phytoplankton dominance in the 1940s. Today, frequent wind resuspension of highly organic, unconsolidated sediments supports a meroplanktonic community that is predominantly diatoms, but during calm periods the algal community is dominated by planktonic cyanobacteria. Sedimentary algal pigments (chlorophyll derivatives and carotenoids) and chemical proxies for nutrient enrichment (polyphosphate, total phosphorus and biogenic silica) in three sediment cores were used to investigate historic changes in primary producers. Sediments were separated into three stratigraphic zones using multivariate statistical techniques. Stratigraphic zonation was established in each core although sediment deposition at one site was insufficient to adequately resolve temporal changes. These results show the importance of selecting suitable sites for paleolimnological studies. The oldest zone represents macrophyte-derived sediments, and the two overlying zones represent phytoplankton-derived sediments deposited since the 1940s. Algal pigments in the most recent sediment zone show little degradation, which might be due to the presence of viable meroplankton in the sediment. After the initial primary producer shift from macrophytes to phytoplankton, the lake experienced a short period of cyanobacterial dominance followed by a period of benthic diatom abundance before being replaced by the present algal community consisting of cyanobacteria and meroplanktonic diatoms. Chlorophyll derivatives and carotenoids were highly correlated with total phosphorus. Historic trends inferred from the data include algal and cyanobacterial productivity that increased with increased phosphorus loading. The study demonstrates that valid paleolimnological proxies for historic eutrophication are available in loosely consolidated sediments of shallow, subtropical lakes.  相似文献   

14.
A 911-m-long sediment core from Lake Biwa, Japan, provides a record of organic matter delivery and accumulation in this large lake during a succession of tectonic and climatic changes dating back to the latest Pliocene. Sediments deposited since 430 ky are profundal; older sediments vary in setting between shallow-water and fluviodeltaic conditions, with occasional deep-water intervals. C/N ratios identify algal production as the dominant source of organic matter throughout the core, although the proportion of land-derived contributions episodically increases in the fluviodeltaic and shallow-water sediments. Rates of organic matter delivery and burial in lake sediments change in response to glacial-interglacial climate changes over the past 430 ky. Sediments deposited during interglacial intervals have organic carbon mass accumulation rates up to 9 times greater than those from glacial intervals, reflecting interglacial climates that were wetter than glacial climates. Algal production of organic matter increased during interglacial times because of greater wash-in of soil nutrients, and organic matter preservation was enhanced because of faster sedimentation rates.  相似文献   

15.
A combination of water and sediment chemistry was used to investigate carbonate production and preservation in Lake Pumayum Co (altitude 5,030 m a.s.l.), south Tibet, China. We compared the chemical composition of lake water in various parts of the lake with that of input rivers and found that the loss of Ca2+ results from calcite sedimentation induced by evaporation and biogenic precipitation. This is supported by evaporation data from the catchment and δ18O measurements on water. Results suggest that CaCO3 is the predominant carbonate in this lake. There is a positive correlation in the sediments among concentrations of total inorganic carbon (TIC), Ca, total organic carbon (TOC), and total nitrogen, confirming that most carbonates in sediment are endogenic. The Jiaqu River is the largest inflow to Lake Pumayum Co and has a strong influence on both lake water chemistry and sediment composition. The river and lake bathymetry influence carbonate sedimentation by affecting water flow velocity and growing conditions for macrophytes. Different carbon contents and relationships between TIC and TOC in the two long cores from different depths in the lake reveal that hypolimnetic conditions also influence carbonate precipitation and preservation.  相似文献   

16.
Sediment cores from two neighbouring lakes (Viitna Linajärv and Viitna Pikkjärv) in northern Estonia were studied to determine lake-level fluctuations during the Holocene and their impact on biogeochemical cycling. Organic matter and pollen records dated by radiocarbon and radiolead indicated a water level rise in both lakes during the early Holocene (c. 10 000–8000 BP). A regression followed around 7500 BP and several transgressions occurred during the latter half of the Holocene, c. 6500 and 3000 BP. Human impact during the last centuries has caused short-term lake-level fluctuations and accelerated sediment accumulation in the lakes. The differences in water depth led to variations in sediment formation. During 10 000–8000 BP (Preboreal and Boreal chronozones) mineral-rich sediments with coloured interlayers deposited in L. Linajärv. These sediments indicate intensive erosion from the catchment and oxygen-rich lake, which favoured precipitation of iron oxides and carbonates. Fluctuations in water depth, leaching of nutrients from catchment soils and climatic changes increased the trophy of L. Linajärv around 6000 BP. The subsequent accumulation of gyttja, the absence of CaCO3 and the decrease in both the C/N ratio and phosphorus content in the sediments also indicate anoxic conditions in the hypolimnion. The similarity in the development of L. Linajärv and L. Pikkjärv and their proximity made it possible to discern the impact of water depths changes on biogeochemical cycling in lakes.  相似文献   

17.
Here we present datasets from a hydroacoustic survey in July 2011 at Lake Torneträsk, northern Sweden. Our hydroacoustic data exhibit lake floor morphologies formed by glacial erosion and accumulation processes, insights into lacustrine sediment accumulation since the beginning of deglaciation, and information on seismic activity along the Pärvie Fault. Features of glacial scouring with a high‐energy relief, steep slopes, and relative reliefs of more than 50 m are observed in the large W‐basin. The remainder of the lacustrine subsurface appears to host a broad variety of well preserved formations from glacial accumulation related to the last retreat of the Fennoscandian ice sheet. Deposition of glaciolacustrine and lacustrine sediments is focused in areas situated in proximity to major inlets. Sediment accumulation in distal areas of the lake seldom exceeds 2 m or is not observable. We assume that lack of sediment deposition in the lake is a result of different factors, including low rates of erosion in the catchment, a previously high lake level leading to deposition of sediments in higher elevated paleodeltas, tributaries carrying low suspension loads as a result of sedimentation in upstream lakes, and an overall low productivity in the lake. A clear off‐shore trace of the Pärvie Fault could not be detected from our hydroacoustic data. However, an absence of sediment disturbance in close proximity to the presumed fault trace implies minimal seismic activity since deposition of the glaciolacustrine and lacustrine sediments.  相似文献   

18.
This study used organic matter in oligotrophic Lake Constance (southern Germany) to reconstruct lake environment and to disentangle the multiple factors, such as climate change and human impacts, which influence sedimentation in large lakes. A sediment core from Upper Lake Constance, which represents 16,000 years of Late Glacial and Holocene lake history, was analysed for organic biomarkers, hydrogen index and elements calcium, strontium, and magnesium. Magnetic susceptibility was measured to establish a high-resolution stratigraphic framework for the core and to obtain further information about changes with respect to relative allochthonous versus autochthonous sedimentation. Dinosterol—a biomarker for dinoflagellates—and calcium have low concentrations in Younger Dryas sediments and consistently high concentrations between 10,500 and 7,000 cal. years BP. These variations are attributed to changes in lake productivity, but are not reflected in the proportion of total organic carbon within the sediment. During the Younger Dryas and between 6,000 and 2,800 cal. years BP, concentrations and accumulation rates of land-plant-derived C29-steroids (β-sitosterol, stigmastanol and stigmasterol), in combination with a relatively low HI, indicate periods of enhanced terrigenous input to the lake. For the Younger Dryas, higher runoff can be attributed to a cold climate, leading to decreased vegetation cover and increased erosion. After 6,000 cal. years BP, high terrestrial input may be explained by enhanced precipitation. Biomarker and HI results, in combination with archaeological studies, raise the question as to whether lakeshore settlements affected sedimentation in Upper Lake Constance between 6,000 and 2,800 cal. years BP.  相似文献   

19.
Lake sediment records are underrepresented in comprehensive, quantitative, high-resolution (sub-decadal), multi-proxy climate reconstructions for the past millennium. This is largely a consequence of the difficulty of calibrating biogeochemical lake sediment proxies to meteorological time series (calibration-in-time). Thanks to recent methodological advances, it is now possible. This paper outlines a step-by-step, specifically tailored methodology, with practical suggestions for calibrating and validating biogeochemical proxies from lake sediments to meteorological data. This approach includes: (1) regional climate data; (2) site selection; (3) coring and core selection; (4) core chronology; (5) data acquisition; and (6) data analysis and statistical methods. We present three case studies that used non-varved lake sediments from remote areas in the Central Chilean Andes, where little a priori information was available on the local climate and lakes, or their responses to climate variability. These case studies illustrate the potential value and application of a calibration-in-time approach to non-varved lake sediments for developing quantitative, high-resolution climate reconstructions.  相似文献   

20.
We present a paleolimnological record from shallow Lake Wuliangsu in the Yellow River Basin, north China, using a short (56 cm) sediment core. Our objective was to investigate environmental changes in this semi-arid region over the past ~150 years. The sediment core was dated using 137Cs and 210Pb. We examined stratigraphic trends in core lithology, nutrients, stable isotopes (δ13C and δ15N) and trace element concentrations in the Lake Wuliangsu core to discern between natural sediments and those affected by human agency. A lithologic transition from yellow, coarse-grained sediment to grey, fined-grained sediment marked the lake’s formation about 1860. Until ~1950, sediments displayed relatively low and constant heavy metal concentrations, indicating little human influence. In the 1950s, enrichment factors (EFs) increased, reflecting greater impact of human activities. Carbon and nitrogen stable isotopes in organic matter (OM), along with heavy metal concentrations, were used to infer past shifts in trophic state and identify pollutants that came from agriculture, industry and urbanization. In the late 1950s, the first evidence for environmental change is recorded by increases in total organic carbon (TOC), total organic nitrogen (TN), TOC/TN, EFs, δ13C and a decrease in δ15N. After about year 2000, a more rapid increase in trophic status occurred, as indicated by greater total phosphorus (TP), EFs, δ15N and lower δ13C values. Changes in isotope and TOC/TN values in the lake sediments may reflect a shift in lake ecology during this period. The first increase in trophic status during the late 1950s was mainly a result of agricultural development in the catchment. In contrast, the change after ca. AD 2000 was driven largely by urban and industrial development. Agreement between paleolimnologic data from Lake Wuliangsu, and both instrumental and written records, indicates that the lake sediments provide a reliable archive for investigating the formation and environmental history of the lake.  相似文献   

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