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1.
Coastal wetlands play an important role in the global carbon cycle.Large quantities of sediment deposited in the Changjiang(Yangtze) estuary by the Changjiang River promote the propagation of coastal wetlands,the expansion of saltmarsh vegetation,and carbon sequestration.In this study,using the Chongming Dongtan Wetland in the Changjiang estuary as the study area,the spatial and temporal distribution of soil organic carbon(SOC) stocks and the influences of sedimentation and vegetation on the SOC stocks of the coastal wetland were examined in 2013.There was sediment accretion in the northern and middle areas of the wetland and in the Phragmites australis marsh in the southern area,and sediment erosion in the Scirpus mariqueter marsh and the bare mudflat in the southern area.More SOC accumulated in sediments of the vegetated marsh than in the bare mudflat.The total organic carbon(TOC) stocks increased in the above-ground biomass from spring to autumn and decreased in winter;in the below-ground biomass,they gradually increased from spring to winter.The TOC stocks were higher in the below-ground biomass than in the above-ground biomass in the P.australis and Spartina altemiflora marshes,but were lower in the below-ground biomass in S.mariqueter marsh.Stocks of SOC showed temporal variation and increased gradually in all transects from spring to winter.The SOC stocks tended to decrease from the high marsh down to the bare mudflat along the three transects in the order:P.australis marsh S.alterniflora marsh S.mariqueter marsh bare mudflat.The SOC stocks of the same vegetation type were higher in the northern and middle transects than in the southern transect.These results suggest that interactions between sedimentation and vegetation regulate the SOC stocks in the coastal wetland in the Changjiang estuary.  相似文献   

2.
沉积物中氮的赋存形态直接影响其参与生物地球化学循环的进程、途径和贡献大小,探究沉积物中不同氮形态的环境地球化学行为对研究氮的地球化学循环具有重要意义。以海南东寨港红树林湿地沉积物为研究对象,分别采集表层沉积物和柱状沉积物,采用分级浸提法提取不同形态的可转化态氮进行空间分布特征及影响因素分析。结果表明:研究区沉积物中总氮(TN)质量分数在1 149.0~1 690.6 mg/kg之间,总可转化态氮(TTN)的质量分数在464.6~647.5 mg/kg之间,二者均呈现出从上游至入海口逐渐降低的空间分布特征;4种可转化态氮中强氧化剂浸取态氮(SOEF-N)与TTN呈显著正相关,也是最主要的氮形态存在形式。通过沉积物C/N比值分析可知,研究区有机质主要来自污染物的大量排入,东寨港红树林柱状沉积物中TN与含水率、TOC呈极显著的正相关关系,表明氮与有机质具有相似的来源。   相似文献   

3.
Sediment samples were cored from 3 locations representing the inner bay, the outer bay and the bay mouth of Jiaozhou Bay in September 2003 to study the source and biogeochemical characteristics of nitrogen and phosphorus in the bay. The content and vertical distributions of total nitrogen (TN), total phosphorus (TP), organic nitrogen (ON), organic phosphorus (OP), inorganic nitrogen (IN), inorganic phosphorus (IP), the ratio of organic carbon and total nitrogen (OC/TN), and the ratio of total nitrogen and total phosphorus (TN/TP) in the sediments were analyzed. The results show that both TN and TP in surface sediments decrease from the inner bay to the outer bay. In general, ON occupies 50%-70% of TN and IP accounts for more than 60% of TP. In ratio of OC:TN, the nitrogen accumulated in the sediments from the inner bay and the bay mouth came mainly from terrestrial sources, and the portion of autogenetic nitrogen was 28.9% and 13.1%, respectively. However, in the outer bay, nitrogen was mainly autogenetic, accounting for 62.1% of TN, whereas phosphorus was mainly land-derived. The sedimentation fluxes of nitrogen and phosphorus varied spatially. The overall diagenesis rate of nitrogen was higher than that of phosphorus. Specifically, the diagenesis rate of OP was higher than that of IP. However, the diagenesis rate of ON was not always higher than that of IN. In species, the diagenesis rate of IN is sometimes much higher than that of the OC. In various environments, the diagenesis rate is, to some degree, affected by OC, pH, Eh, and Es.  相似文献   

4.
Sediments have a significant influence on the cycling of nutrient elements in lake environments. In order to assess the distribution characteristics and estimate the bioavailability of phosphorus and nitrogen in Dianchi Lake, organic and inorganic phosphorus and nitrogen forms were analysed. The 210 Pb radiometric dating method was employed to study temporal changes in the phosphorus and nitrogen pools in Dianchi Lake. The result show that the total phosphorus(TP) and total nitrogen(TN) were both at high concentrations, ranging from 697.5–3210.0 mg/kg and 1263.7–7155.2 mg/kg, respectively. Inorganic phosphorus(IP) and total organic nitrogen(TON) were the main constituents, at percentages of 59%–78% and 74%–95%, respectively, in the sediments. Spatially, there was a decreasing trend in phosphorus and nitrogen contents from the south and north to the lake centre, which is related to the distribution pattern of local economic production. The burial rates of the various phosphorus and nitrogen forms increased in same spatially and over time. Particularly in the past two decades, the burial rates doubled, with that TN reached to 1.287 mg/(cm~2·yr) in 2014. As the most reactive forms, nitrate nitrogen(NO_3-N) and ammonia nitrogen(NH_4-N) were buried more rapidly in the south region, implying that the potential for releasing sedimentary nitrogen increased from north to south. Based on their concentrations and burial rates, the internal loads of phosphorus and nitrogen were analysed for the last century. A TP pool of 71597.6 t and a TN pool of 81191.7 t were estimated for Dianchi Lake. Bioavailable phosphorus and nitrogen pools were also estimated at 44468.0 t and 5429.7 t, respectively, for the last century.  相似文献   

5.
For some hundred surface sediment samples from five cores taken in two cruises near the Huanghe River Estuary, total phosphorus (TP (.inorganic phosphorus (IP (and organic phosphorus (OP)were determined.On the average, 527×10-6, 455×10~6 and 72×10-6 were found for TP,IP and OP for the surface sediments taken in the two cruises. The distribution of OP and IP was controlled by the sample particle size: OP content increased with the decreasing of the sample particle size, while the maximal value of IP was found in the silt fraction due to the existence of apatite in our samples. Vertical distributions reflected well the channel change of the Huanghe River. Results from the multiple regressions between the three forms of phosphorus and the percentages of different particle size agreed well with the analytical data.  相似文献   

6.
Four short cores were obtained from the coastal wetland of the Quanzhou Bay, Fujian Province, China, and sediment samples were analyzed with a Mastersizer 2000 for grain size analysis and an Inductively Coupled Plasma Atomic Emission Spectrometer (ICP-AES) for trace metal analysis. The results of grain size analysis show that the wetland sediments are mainly composed of silt and clay, and the distribution of median grain size is affected by human activities obviously. The results of trace metal analysis show that the wetland sediments mainly originate from terrestrial materials in the Luoyangjiang River estuary and from contaminants discharged from adjacent rivers in Shuitou area. The heavy metal contamination in Luoyangjiang estuary decreased from 1984 to 2004 due to industry transformation, but has increased since 2004 because of the discharge of contaminants to the Jinjiang River and much living sewerage to the bay, and a large number of trace metals are trapped within Spartina alterniflora marsh.  相似文献   

7.
Iron-rich groundwater flowing into wetlands is a worldwide environmental pollution phenomenon that is closely associated with the stability of wetland ecosystems. Combined with high phosphorus(P) loading from agricultural runoff, the prediction of the evolution of wetland vegetation affected by compound contamination is particularly urgent. We tested the effects of anaerobic iron-rich groundwater discharge in a freshwater marsh by simulating the effect of three levels of eutrophic water on native plants(Glyceria spiculosa(Fr. Schmidt.) Rosh.). The management of wetland vegetation with 1–20 mg/L Fe input is an efficient method to promote the growth of plants, which showed an optimum response under a 0.10 mg/L P surface water environment. Iron-rich groundwater strongly affects the changes in ecological niches of some wetland plant species and the dominant species. In addition, when the P concentration in a natural body of water is too high, the governance effect of eutrophication might not be as expected. Under iron-rich groundwater conditions, the δ~(13)C values of organs were more depleted, which can partially explain the differences in δ~(13)C in the soil profile. Conversely, the carbon isotope composition of soil organic carbon is indicative of past changes in vegetation. The results of our experiments confirm that iron-rich groundwater discharge has the potential to affect vegetation composition through toxicity modification in eutrophic environments.  相似文献   

8.
To evaluate the influence of wetland reclamation on vertical distribution of carbon and nitrogen in coastal wetland soils, we measured the soil organic carbon(SOC), soil total nitrogen(STN) and selected soil properties at five sampling plots(reed marsh, paddy field, corn field, forest land and oil-polluted wetland) in the Liaohe River estuary in September 2013. The results showed that reclamation significantly changed the contents of SOC and STN in the Liaohe River estuary(P 0.001). The SOC concentrations were in the order: oil-polluted wetland corn field paddy field forest land reed marsh, with mean values of 52.17, 13.14, 11.46, 6.44 and 6.16 g/kg, respectively. STN followed a similar order as SOC, with mean values of 1351.14, 741.04, 632.32, 496.17 and 390.90 mg/kg, respectively. Interaction of reclamation types and soil depth had significant effects on SOC and STN, while soil depth had significant effects on SOC, but not on STN. The contents of SOC and STN were negatively correlated with pH and redox potential(Eh) in reed marsh and corn field, while the SOC and STN in paddy field had positive correlations with electrical conductivity(EC). Dissolved organic carbon(DOC), ammonium nitrogen(NH_4~+-N) and nitrate nitrogen(NO_3~–-N) were also significantly changed by human activities. NH_4~+-N and NO_3~–-N increased to different degrees, and forest land had the highest NO_3~–-N concentration and lowest DOC concentration, which could have been caused by differences in soil aeration and fertilization. Overall, the results indicate that reed harvest increased soil carbon and nitrogen release in the Liaohe River Estuary, while oil pollution significantly increased the SOC and STN; however, these cannot be used as indicators of soil fertility and quality because of the serious oil pollution.  相似文献   

9.
Sediment cores with length of 25 - 45cm at 12 stations in Zhujiang(Pearl) River Estuary were sampled in summer of 1999. Chemical components (Al2O3 , Fe2O3, CaO, TiO2, Cu, Pb, Cr, Zn, Co, Ni, V, Ba, Sr and Y) and grain sizes were analyzed. Sediments in Zhujiang River Estuary are characterized by relatively coarse grain size. The grain sizes of the sediments in the area outside the estuary are relatively finer than those in the north part of the estuary but coarser than those in the middle of Lingdingyang and have a trend similar to the spatial distribution trend of some chemical components such as Fe2O3, Al2O3, TiO2, V, Cu, Ni, Zn and Y. This showed that grain size is an important factor that controls the spatial distribution and depth profile of chemical elements in the Zhujiang River Estuary. Frequent re-suspension, re-transportation and redistribution of settled sediment on estuary floor could be deduced from the spatial distributions and depth profiles of chemical components. Except for CaO and Sr, the chemical components always enrich at the west side of, in the middle of, and at the north side of, the estuary. Fe2O3, Al2O3, Ti, V, Cr, Ni, Zn, Cu and Y in Zhujiang River Estuary sediments mainly result from rock and soil weathering except that parts of Cr, Ni, Zn Cu and Y are anthropogenic. CaO and Sr in sediments originate from marine source. Although Co as well as Pb derives from anthropogenic sources, human activities related to Co might differ from the activities related to Pb.  相似文献   

10.
The multi-level ditch system developed in the Sanjiang Plain, Northeast China has sped up water drainage process hence transferred more pollutants from farmlands into the rivers of this region. Understanding the seasonal dynamics of nitrogen (N) and phosphorus (P) transportation in the ditch system and the role of different ditch size is thus crucial for water pollution control of the rivers in the Sanjiang Plain. In this study, an investigation was conducted in the Nongjiang watershed of the Sanjiang Plain to study the nutrient variation and the correlation between water and sediments in the ditch system in terms of ditch level. Water and sediments samples were collected in each ditch level in growing season at regular intervals (once per month), and TN, NO3 N, NH4 +-N, TP, and PO4 3−-P were analyzed. The results show that nutrient contents in water were higher in June and July, especially in July, the contents of TN and TP were 3.21 mg/L and 0.84 mg/L in field ditch, 4.04 mg/L and 1.06 mg/L in lateral ditch, 2.46 mg/L and 0.70 mg/L in branch ditch, 1.92 mg/L and 0.63 mg/L in main ditch, respectively. In August and September, the nutrient contents in the water were relatively lower. The peak value of nutrient in ditch water had been moving from the field ditch to the main ditch over time, showing a remarkable impact of ditch system on river water environment. The nutrient transfer in ditch sediments could only be found in rainfall season. Nutrient contents in ditch sediment had effect on that in ditch water, but nutrients in ditch water and sediments had different origination. Ditch management in terms of the key factors is hence very important for protecting river water environment.  相似文献   

11.
Accumulation of metals in both sediments and Phragmites australis organs was studied. Samples were collected from seven stations located in Anzali wetland, Iran. The samples were analyzed by inductively coupled plasma mass spectrometry(ICP-MS). The results showed that concentration of the studied metals(except As and Cd) were higher in sediments than in P.australis organs. Metal accumulation was found to be signifi cantly(P 0.05) higher in roots than in above-ground organs of P.australis. The bioaccumulation factor(BAF) and the transfer factor(TF) also verifi ed the highest rate of metal accumulation in roots and their reduced mobility from roots to the above-ground organs. Pearson correlation coeffi cient showed signifi cant relationships between metal concentrations in sediments and those in plant organs. It should be pointed out that sediment and plant samples exhibited higher metal concentrations in eastern and central parts than in western and southern parts of the wetland. The mean concentrations of all studied elements(except for Fe, V and Al) were higher in these sediment samples than in the Earth's crust and shale. High accumulation of metals in P. australis organs(roots and shoots) is indicative of their high bioavailability in sediments of the wetland. The correlation between metal concentrations in sediments and in P. australis indicates that plant organs are good bioindicators of metal pollution in sediments of Anzali wetland.  相似文献   

12.
Ruxi River is a tributary of the Three Gorges Reservoir. This study examined the temporal and spatial dynamics in particle size characteristics and the associated nutrients and contaminants of the fluvial suspended and deposited sediments along the Ruxi River. Temporal variations in the particle size distribution of the suspended sediment are controlled mainly by differences in sediment source during different seasons. Total organic carbon(TOC), total nitrogen(TN) and total phosphorous(TP) in the 62μm fraction of the suspended sediment exhibit considerably higher concentrations in spring,indicating high probability of algal blooms in the backwater areas. Downstream trends in the nutrient contents of 62 μm deposited sediments imply the greatest potential for eutrophication in the backwater ends, where highest nutrient concentrations were detected. Assessment of metal contamination shows that the sediments deposited in the water-level fluctuation zone were moderately to strongly contaminated by Cadmium(Cd), with a considerably high potential ecological risk. The findings reported have emphasized the impacts of reservoir impoundment on aquatic and/or terrestrial environment in this region. More information on physical, chemical and biological processes of sediment and sediment-associated materials are needed for developing environmentally and ecologically sound policies of water and sediment management.  相似文献   

13.
GEOCHEMICAL CHARACTERISTICS OF PHOSPHORUS NEAR THE HUANGHE RIVER ESTUARY   总被引:5,自引:0,他引:5  
INTRODUCTIONPhosphorus (P)isanimportantlimitingelementinglobaloceanicproductivity (Holland ,1 978) ,soknowledgeofPisakeytobetterunderstandingofthecyclingofcarbon ,nitrogen,sulfur,andothernu trientelements.Inasimplemassbalancemodel,thelevelofdissolvedPintheoceanisafunctionoftherateofinputviarivers,andtherateofoutputviadepositioninsediments.Inthepresentstudy,thefocusisontheriverinePinputbytheHuangheRiver (YellowRiver)totheBohaiSea,andespeciallyontheamountofPsolubilizedfromsolidphasesupo…  相似文献   

14.
Investigation of phosphorus (P) sorption-desorption characteristics of drainage ditch sediments is important for better understanding on sediment P transport behaviors in ditches. Surface ditch sediment samples were collected from headwater sub-catchment of forestland, sloping cropland, paddy field, and residential area in a representative catchment in the central Sichuan Basin. These sediment samples were used for determination of P sorption-desorption characteristics by a batch equilibrium technique. Results showed that the maximum P sorption capacities (Qm) in the sediments ranged from 159.7 to 263.7 mg/kg, while higher Qm were observed in the ditch sediments from the paddy fields. The Qm was significantly and positively correlated with oxalate-extractable Fe and Al oxides (r=0.97 and 0.98, p < 0.01), clay fraction (r = 0.78, p < 0.05) and organic matter (r = 0.95, p < 0.01). Sediment pH, clay and organic matter influenced the P sorption through amorphous Fe and Al oxides. CaCO3 content was negatively correlated with the Qm (r = -0.83, p < 0.05), implying that saturated CaCO3 (> 50 g/kg) would not increase P sorption capacity in the ditch sediments. The ditch sediments featured a linear desorption curve, suggesting that P release risk would be enhanced with the increase of the P adsorption. The P desorption rate was positively correlated with Olsen P (r = 0.94, p < 0.01), but negatively related to the fine particle-size fractions (r = -0.92, p < 0.01), the sum of the amorphous Fe and Al oxides (r = -0.67, p < 0.05) and the P sorption capacity (r = -0.59, p < 0.05). The ditch sediments from residential area had a higher P release risk than that from the other ditches of forestland, sloping cropland and paddy field. The P sorption index (PSI) derived from single-point measurement was significantly correlated with the P sorption capacity (r = 0.99, p < 0.01), and could be used for estimating Qm as 1.64 times PSI plus 24.0 (Qm = 1.64 PSI + 24.0) for similar sediments with highly calcareous soils and sediments. Ditch cleaning and sediment removal for the ditch in residential area were recommended in this area to reduce the P release risk.  相似文献   

15.
Based on a new idea for research on cycling of marine biogenic elements, this study showed that only the leachable form phosphorus in natural grain sizes manne sediments constitutes the transferable phosphorous in the sediments. The transferable phosphorus content in the natural grain sizes surface sediments in the Huanghe River estuary adjacent waters ranges from 58.5-69.8 μg/g, accounting for only 9.1%-11.0% of the total phosphorus content, whereas the leachable form (“transferable” )phosphorus content in the sediment after it was totally ground into powder was found to be 454.8-529.2μg/g, accounting for 73.4%-89.1% of the total phosphorus. Analysis of the correlation between thebill,ass of benthos and the leachable form (“transferable” ) phosphorus showed that most of the leachableform (“transferable”) phosphorus in the totally ground sediment did not participate in the marine biogeo chemical cycling. Furthermore, a synchronous survey on benthos showed that the biornass of meio-and maero-benthos exhibited good positive correlation with the leachable form of phosphorus in the naturalgrain sizes sediment, but peorer correlation with the leachable form (“transferable”) phosphorus in the totally ground sediment, indicating that transferable phosphorus in marine sediment is the leachable form of phosphorus in the natural grain sizes sediments, and is not the previously known leachable form(“transferable”) phosphorus obtained from the totally ground sediment.  相似文献   

16.
Accumulation of metals in both sediments and Phragmites australis organs was studied. Samples were collected from seven stations located in Anzali wetland, Iran. The samples were analyzed by inductively coupled plasma mass spectrometry (ICP-MS). The results showed that concentration of the studied metals (except As and Cd) were higher in sediments than in P. australis organs. Metal accumulation was found to be significantly (P <0.05) higher in roots than in above-ground organs of P. australis. The bioaccumulation factor (BAF) and the transfer factor (TF) also verified the highest rate of metal accumulation in roots and their reduced mobility from roots to the above-ground organs. Pearson correlation coefficient showed significant relationships between metal concentrations in sediments and those in plant organs. It should be pointed out that sediment and plant samples exhibited higher metal concentrations in eastern and central parts than in western and southern parts of the wetland. The mean concentrations of all studied elements (except for Fe, V and Al) were higher in these sediment samples than in the Earth’s crust and shale. High accumulation of metals in P. australis organs (roots and shoots) is indicative of their high bioavailability in sediments of the wetland. The correlation between metal concentrations in sediments and in P. australis indicates that plant organs are good bioindicators of metal pollution in sediments of Anzali wetland.  相似文献   

17.
Four soil types(peat, marsh, meadow, and sandy) in the Zoige Plateau of China are associated with the severity of wetland degradation. The effects of wetland degradation on the structure and abundance of fungal communities and cellulase activity were assessed in these 4 soil types at 3 depths using DGGE(Denatured Gradient Gel Electrophoresis), q PCR(Quantitative Real-time PCR),and 3,5-dinitrosalicylic acid assays. Cellulase activity and abundance of the fungal community declined in parallel to the level of wetland degradation(from least to most disturbed). DGGE analysis indicated a major shift in composition of fungal communities among the4 soil types consistent with the level of degradation.Water content(WC), organic carbon(OC), total nitrogen(TN), total phosphorus(TP), available nitrogen(AN), and available phosphorus(AP) were strongly correlated with cellulase activity and the structure and abundance of the fungal community.The results indicate that soil physicochemical properties(WC, OC, TN, TP, AN, and AP), cellulase activity, and diversity and abundance of fungal communities are sensitive indicators of the relative level of wetland degradation. WC was the major factorinvolved in Zoige wetland degradation and lower WC levels contributed to declines in the abundance and diversity of the fungal community and reduction in cellulase activity.  相似文献   

18.
Radioactive markers are useful in dating lead(Pb) deposition patterns from industrialization in sedimentary archives. As a well-known natural reserve in the world, Yancheng coastal wetland in Jiangsu Province is one of areas most sensitive to global sea level change and is located in the most developed and polluted region of China. Two cores were collected in Yancheng wetland in October 2013 and dated using ~(210)Pb and ~(137)Cs radiometric techniques. Sediments in both cores were sectioned into depth bands and examined systematically for dry bulk density, water content, magnetic susceptibility and grain-size. Multiple elements including Pb were also measured using inductively coupled plasma systems. Unsupported ~(210)Pb activities decreased with depth in both of the two cores, and ~(210)Pb chronologies were established(covering 150 years) using the constant rate of supply(CRS) model. The measured Pb contents ranged from 14.97 mg/kg to 29.40 mg/kg with average values of 17.17–22.79 mg/kg, and the Pb fluxes ranged from 41.70 mg/(m~2·yr) to 172.70 mg/(m~2·yr) with averages of 95.59–123.41 mg/(m~2·yr). Temporal variations of Pb flux, enrichment factors and Pb isotopes show a gradual and continuous increase over time and clearly reflect increased emissions from anthropogenic activities in the region. The Pb isotopic compositions show that most of Pb deposition in Yancheng wetland is input from natural sources by water flows and has the same levels of Pb as in the surface sediment of the Yangtze River and the Pacific mineral aerosol. We also stress the anthropogenic Pb contribution in Yangcheng wetland sediment and the reason of our Pb isotopes not showing anthropogenic signature is likely the instability of anthropogenic Pb in high Fe/Mn oxide conditions. Therefore, more attention should be paid to current local pollution problems, and society should take action to seek a balance between economic development and environmental protection.  相似文献   

19.
Sediment-associated processes, such as sediment erosion, deposition, and pore water diffusion/advection affect sorptive contaminant transport. By considering these processes, we developed an equation to simulate contaminant transport. Erosion and deposition processes are considered as erosion and deposition fluxes of sediment, and adsorption-desorption processes of contaminants by sediment are simulated using the Langmuir Equation. Pore water diffusion is calculated based on the contaminant concentration gradient across the sediment-water interface. Pore water advection is estimated using pore water contained in the sediments of erosion flux. The equation is validated to simulate total phosphorus concentrations in Guanhe estuary in the northern Jiangsu, China. The simulated total phosphorus concentrations show better agreement with field observations compared to estimations that do consider sediment-associated processes.  相似文献   

20.
根据南海区半封闭型海湾规模化养殖技术研究的需要,对红海湾底质硫化物进行了研究。用碘量法分析的结果表明:红海湾底质中硫化物含量的区域分布极不均匀,呈北部河口区>虾池>鱼湾>中部>南部自然水域>礁滩区的特点。虾池、鱼的硫化物含量清淤前分别为清淤后的8.4、3.6倍;湾南部硫化物含量春季明显高于夏季,其余区域的两季差异不明显。46份样品中约13%、28%分别超过国内外评价标准,超标测站位于河口和清淤前的虾池、鱼。礁滩护养增殖区、南部自然水域、湾中部牡蛎养殖区和清淤后的虾池、鱼尚未见硫化物的污染。  相似文献   

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