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1.
1　Introduction Thestudyonthefeaturesofatmosphericenvironmentbyglaciochemistryisthemajor contentofsnow iceandglobalchangeresearch.Antarcticicesheetisfarfromtheregions pollutedbyhumanactivities,andsurroundedbyocean,andtheAntarcticCircumpolarCur rentisthewideseawaterandatmospherebarrierbetweenAntarcticaandtheoutsideworld. AlloftheuniquegeographicalfeaturesmaketheimpuritiesinsnowandiceinAntarcticice sheetissimple.Therefore,itissignificanttostudytheorigins,transmissionpathsanddep ositionalst…  相似文献   

2.
The reconstruction of air trapped in ice cores provides us the most direct information about atmospheric CH4 variations in the past history. Ice core records from the ＂Three Poles （Antarctica, Greenland and Tibetan Plateau）＂ reveal the detailed fluctuations of atmospheric CH4 concentration with time and are allowed to quantify the CH4 differences among latitudes. These data are indispensably in the farther study of the relationship between greenhouse gases and climatic change, and of the past changes in terrestrial CH4 emissions. Ice cores reconstruction indicates that atmospheric CH4 concentration has increased quickly since industrialization, and the present day＇s level of atmospheric CH4 （1800 ppby） is unprecedented during the past Glacial-Interglacial climate cycles.  相似文献   

3.
Taking South Lake and Jingyue Pool in Changchun as examples,we determined particulate Hg in ambient air and Hg concentration in precipitation.Results indicated that particulate Hg in air and Hg concentration in precipita-tion in both sites in nonheating period were lower than that in heating period,which is influenced by coal combustion.The annual particulate Hg concentrations in precipitation were 0.268μg/L(South Lake)and 0.108μg/L(Jingyue Pool).The high-er particulate Hg concentrations in precipitation were 0.268μg/L(South Lake) and 0.108μg/L(Jingyue Pool).The high-er particulate Hg concentration in air and Hg concentration in precipitation in South Lake than that of Jingyue Pool indicat-ed that mercury deposition was influenced by anthropogenic sources(especially from coas combustion).Hg concentration in precipitation is related with particulate Hg in the atmosphere.Dry deposition fluxes were estimated by using dry deposi-tion model on the base of particulate Hg concentrations in the atmosphere,they were estimated by using dry deposi-tion model on the base of particulate Hg concentrations in the atmosphere,they were 35.5μg/(m^2.a) for South lake and 15.3μg/(m^2.a)for Jingyue Pool.Combined with precipitation amount,wet deposition fluxes were estimated in these two sites,152.2μg(m^2.a)for South Lake and 61.2μg/(m^2.a)for Jingyue Pool.Atmospheric Hg deposition fluxes were 160.2g/a for South Lake and 328.62g/a for Jingyue Pool.e  相似文献   

4.
1　IntroductionAntarcticicesheetisaburialgroundforatmosphericdeposition .Sincethereiscon tinuousinteractionbetweentheicesheetandtheatmosphere,variousatmosphericsub stancesareinjectedtotheicesheetsequentiallyintimeandspace.Therefore,verticalanalysesoftheicesheetprovideuswithinformationaboutpastclimaticchange (Delmas1 992 ;LegrandandMayewski 1 997)andhorizontalanalysesoftheicesheetprovideuswithknowledgeregardinglong rangetransportofairbornematerials (Kamiyamaetal.1 989;KreutzandMayewski 1 999)…  相似文献   

5.
Mt. Yulong is the southernmost currently glacier-covered area in Eurasia, including China. There are 19 sub-tropical temperate glaciers on the mountain, controlled by the south-western monsoon climate. In the summer of 1999, a firn core, 10. 10 m long, extending down to glacier ice, was recovered in the accumulation area of the largest glacier, Baishui No. 1. Periodic variations of climatic signals above 7. 8 m depth were apparent, and net accumulation of four years was identified by the annual oscillations of isotopic and ionic composition. The boundaries of annual accumulation were confirmed by higher values of electrical conductivity and pH, and by dirty refreezing ice layers at the levels of summer surfaces. Calculated mean annual net accumulation from 1994/1995 to 1997/1998 was about 900 mm water equivalent. The amplitude of isotopic variations in the profile decreased with increasing depth, and isotopic homogenization occurred below 7. 8 m as a result of meltwater percolation. Variations of δ18O above 7. 8 m showed an approximate correlation with the winter climatic trend at Li Jiang Station, 25 km away. Concentrations of Ca2+ and Mg2+ were much higher than those of Na+ and K+ , indicating that the air masses for precipitation were mainly from a continental source, and that the core material accumulated during the winter period. The close correspondence of C1- and Na+ indicated their common origin. Very low concentrations of SO2-4 and NO3- suggest that pollution caused by human activities is quite low in the area. The mean annual net accumulation in the core and the estimated ablation indicate that the average annual precipitation above the glacier's equilibrium line is 2400 - 3150 mm, but this needs to be confirmed by long term observation of mass balance.  相似文献   

6.
The work presents microparticle concentrations in snowpits from the East Rongbuk Glacier on Mt. Qomolangma (Everest) (ER) (28.02°N, 86.96°E, 6536 m a.s.l.), the Zhadang Glacier on Mt. Nyainqentanglha (NQ) (30.47°N, 90.65°E, 5800m a.s.l.), and the Guoqu Glacier on Mt. Geladaindong (GL) (33.95°N, 91.28°E, 5823m a.s.l.) over the Tibetan Plateau (TP). Variations of microparticle and major ions (e.g. Mg2+, Ca2+) concentrations in snowpits show that the values of the microparticles and ions in the non-monsoon seasons are much higher than those in the monsoon seasons. Annual flux of microparticle deposition at ER is lower than those at NQ and GL, which could be attributed to the long distance away from the possible dust source regions as well as the elevation for ER higher than the others. Compared with other remote areas, microparticle concentrations in the southern TP are much lower than those in the northern TP, but still much higher than those in Greenland and Antarctica. The seasonal and spatial microparticle variations are clearly related to the variations of atmospheric circulation according to the air mass 5-day backward trajectory analyses of HYSPLIT Model. Resultingly, the high microparticle values in snow are mainly attributed to the westerlies and the strong dust storm outbreaks on the TP, while the monsoon circulation brings great amount of precipitation from the Indian Ocean, thus reducing in the aerosol concentrations.  相似文献   

7.
Dome A is the highest ice feature in the Antarctica,up to now,little is known about surface topography at Dome A.The first Chinese ITASE expedition was carried out from Zhongshan station to Dome A during the 1996/1997 austral summer. During the 2004/2005 austral summer,the traverse was extended to the summit of Dome A which is 1228 km from Zhongshan Station by 21st Chinese National Antarctic Research Expedition (CHINARE).The real-time kinematic (RTK) GPS survey was carried out in the summit of Dome A dur...  相似文献   

8.
The heights of automatic weather station (AWS) sensors over the Antarctic ice sheet are nominal and change with snow accumulation or ablation. Therefore, the measured data may not be used directly. In this study, we analyzed the impact of snow accumulation on AWS observations using continuous measurements from three AWS that were deployed on the traverse route from the Zhongshan Station to Dome A over East Antarctica. We then corrected the measured air temperature to account for changes in the sensor height relative to the snow surface to improve the authenticity and representativeness of the observation data from the AWS. The results show that (i) the annual mean snow accumulations at Dome A, Eagle and LGB69 were approximately 0.11 m, 0.30 m and 0.49 m, respectively, and the corresponding annual mean air temperature differences between the corrected and measured values at 1 m in height were 0.34℃, 0.29℃ and 0.35℃; (ii) the impact on air temperature from accumulation decreases with height from the surface; (iii) the air temperature difference between the corrected and measured values was not directly proportional to the snow accumulation but was related to the seasonal air temperature variations and the intensity of the local surface inversion; and (iv) the averaged corrected air temperature was higher than the measured values except during the summer when there were days without temperature inversion. The magnitude of the temperature difference between the corrected and measured was mainly determined by snow accumulation and the intensity of the local surface inversion.  相似文献   

9.
The variations of sea ice are different in different regions in Antarctica, thus have different impacts on local atmospheric circulation and global climatic system. The relationships between the sea ice in Ross Sea and Weddell Sea regions and the synoptic climate in summer of China are investigated in this paper via diagnostic analysis methods by using global sea ice concentration gridded data covering Jan. 1968 through Dec. 2002 obtained from Hadley Center, combined with Geopotential Height on 500hPa and 100hPa over North Hemisphere and monthly precipitation and air temperatures data covering the corresponding period over 160 meteorological stations in China obtained from CMA （ China Meteorological Administration）. Results disclose that both these two regions are of indicative meanings to the climate in summer of China. The Ross Sea Region is the key sea ice region to the precipitation in Northeast China in summer. More sea ice in this region in September will result in less precipitation in Northeast China in the following June. Weddell Sea Region is the key sea ice region to the air temperature in Northeast China in summer. More sea ice in this region in September will contribute to lower air temperature in Northeast China in the following June.  相似文献   

10.
Snow samples collected from a 50 m firn core and two snow pits along the route of the 1996/1997 Chinese First Antarctic Inland Traverse Expedition in Princess Elizabeth Land, East Antarctica, have been analyzed for chemical composition and oxygen isotope ratio. Analyzing the relationship between the concentration and flux of major ions and accumulation rate can draw the following conclusions. 1 ) The concentrations of major ions in the atmosphere in the study region is big enough so that the concentrations of the ions do not vary with snow accumulation rate, that is to say, the concentrations of major chemical species are independent of snow accumulation rate. 2) The results of analyzing the depositional styles of major chemical species suggest that wet deposition dominates the major ions flux. In addition, there is no apparent correlation between nssSO2-4 fluctuations and isotope profile. This would indicate the short-term climatic effect of volcanism is not evident in the region.  相似文献   

11.
利用2003-01～2013-12期间GRACE数据反演得到地球表面质量变化,使用全球正向建模恢复法改正泄露影响,获得南极冰盖质量变化。比较GRACE直接估计和泄露影响改正后的结果发现,南极冰盖在2003～2013年质量变化信号衰减20.3%,西南极有26.4%的质量消融信号泄露到了周边,东南极的泄露影响更高达70%。改正后的结果表明,南极冰盖绝大部分质量消融发生在西南极和南极半岛,质量积累发生在东南极的Ronne冰架和Amery冰架;西南极冰盖质量变化速度达到-152.47±2.00 Gt/a,基本上等同于南极全岛的质量消融速度,而南极半岛的冰盖融化速度为-27.44±0.75 Gt/a,基本与东南极的冰盖质量积累速度27.27±5.12Gt/a抵消;南极全岛冰川整体质量以-152.64±7.00 Gt/a速度消失,并以-18.85±4.87 Gt/a2的加速度加速融化,导致海平面以0.41 mm/a的速度上升。  相似文献   

12.
The lowest addition of mercury (0.1 ug Hg 1−1) was used in CEEs for research on mercury flux, speciation and budget. The removal behavior of mercury by phytoplankton in water columns of CEEs can be described by first order kinetic equations for total and particulate mercury in the CEE spiked by mercury. The removal rate of mercury in water columns depends on the size and productivity of phytoplanton in a water column to which mercuric ions were added. A 4.4 day half-life time and a 2.8 day half-life time for total and particulate mercury respectively was obtained in diatom bloom. During microflagellate bloom a 30 day total mercury half-life time was estimated with increase of particulate mercury in the water column. The 0.010 ug Hg cm−2y−1 mercury flux rate that was attained in the control bag agreed with the values from field measurements in Saanich Inlet where the bags were launched. The proportion of total mercury to dissolved and particulate mercury depended also on the size, productivity, and concentration of mercury in a water column. A more or less constant distribution of mercury species in the control bag was observed as follows: dissolved Hg 0.73, particulate Hg 0.27, inorganic Hg 0.42, dissolved organic Hg 0.31. After spiking with mercury, the particulate mercury rose rapidly and reached to over 70% of the total mercury. The concentration factor of mercury by phytoplankton in the CEEs in the order of 105 was consistent with the results from field measurements in Saanich Inlet. The mercury recovery from the water column, sediment, water with sediment, and the CEE bag walls was only 52.3% of total mercury spiked in the CEE. The losses of mercury by vaporization into the ambient air and diffusion through the wall of the enclosure should be considered. This paper was published in Chinese inOcean. Limn. Sinica,17(4):307–317, 1986.  相似文献   

13.
Acidic species, such as Nitrate, in polar snow and firn layers are “reversibly” deposited, and are sufficiently volatile to undergo significant postdepositional exchange between snow/firn and the atmosphere. Through comparison of the snowpit and snowpack nitrate concentrations from central East Antarctica and the headwater of ürumqi River, we conclude that the nitrate peaks in the uppermost surface snow layers in central Antarctica are not related to an atmospheric signal and must account for post-depositional effects. Such effects, however, are not found in the surface snowpack nitrate profiles from the headwater of ürumqi River. Two reasons may account for the post-depositional difference. At first, nitrate in the polar snow and firn layers appears to be hydrated ion, which can be taken up by the atmosphere, while at the headwater of ürumqi River it seems mainly as mineral ion, which assembles the behavior of aerosol-derived species that are “irreversibly” deposited and do not undergo significant post-depositional exchange with the atmosphere. Secondly, the chemical features of the snow and ice on the Antarctica are mainly determined by wet deposition, to the contrary, dry deposition is more significant at the headwater of lUrumqi River than that on the East Antarctic Plateau.  相似文献   

14.
The hole RM, the deepest one fully obtained core in the Qinghai-Xizang Plateau, situated in the depositional center of the Zoige Basin (33°57′N; 102° 21′E) in the northeastern Qinghai-Xizang Plateau with a depth of 310.46 m. From 14C dating and paleomagnetic stratigraphic study, the core RM can date back to 900 ka B.P.. In this paper we analyzed the compositions of δ18O and δ13C in various carbonates can date (snail, obstrode, chemical carbonate) in core RM and discussed preferably the paleoclimatic record by the proxies of δ18O and δ13C of chemical carbonate (authicarbonate) from core RM in the past 140 ka. The results showed that the values of δ18O in various carbonates are generally identical, and the values of δ13C in it are inconsistent, while there exist better relativity. The studies also demonstrated that there was a negative correlation between δ18O and δ13C of authicarbonate in core RM in the past 140 ka, showing that the changes of δ18O values were mainly relative to the water temperature. According to above, the climatic evolutionary sequence were rebuilt in the past 140 ka in the region.  相似文献   

15.
The first study of erratic boulder exposure ages in the Grove Mountains,interior Antarctica,indicates the two erratic boulders(060131-1 and 060131-2,collected from a typical nunataks,Zakharoff Ridge in the Grove Mountains) have 10Be minimum exposure ages of 1.24±0.11 Ma,1.37±0.12 Ma,and 26Al ages of 0.90±0.12 Ma,0.44±0.04 Ma,respectively.Meanwhile,another erratic boulder sample 060131-4,coming from vicinal ice surface,has 10Be and 26Al minimum exposure ages of 0.47±0.3 Ma and 0.44±0.04 Ma,respectively.The e...  相似文献   

16.
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17.
Long-term monitoring programs for measurement of atmospheric mercury concentrations are presently recognized as powerful tools for local,regional and global studies of atmospheric long-range transport processes,and they could also provide valuable information about the impact of emission controls on the global budget of atmospheric mercury,their observance and an insight into the global mercury cycle. China is believed to be an increasing atmospheric mercury emission source. However,only a few measurements of mercury,to our knowledge,have been done in ambient air over China. The highly-time resolved atmospheric mercury concen-trations have been measured at Moxi Base Station （102°72′E 29°92′N,1640 m asl） of the Gongga Alpine Ecosystem Observation and Experiment Station of Chinese Academy of Sciences （CAS） from May 2005 to June 2006 by using a set of Automatic Atmospheric Mercury Speciation Analyzers （Tekran 2537A）. Measurements were carried out with a time resolution of every 15 minutes. The overall average total gaseous mercury （TGM） covering the measurement periods was 4±1.38 ng·m^-3 （N=57310）,which is higher than the global background level of approximately 1.5～2.0 ng·m^-3. The measurements in all seasons showed a similar diurnal change pattern with a high concentration during daytime relative to nighttime and maximum concentration near solar noon and minimum concentration immediately before sunrise. The presence of diurnal TGM peaks during spring and summer was found earlier than that during autumn and winter. When divided seasonally,it was found that the concentrations of TGM were highest in winter with 6.13 ± 1.78 ng·m^-3 and lowest in summer with 3.17 ± 0.67 ng·m^-3. There were no significant differences in TGM among wind sectors during each season. Whereas Hg generally exhibited significant correlations with the parameters,such as temperature,saturated vapor pressure,precipitation,ultraviolet radiation （UV） and atmospheric pressure at the whole measurement stage,and t  相似文献   

18.
During CHINARE-22 in austral summer of 2005-2006, a lake sediment core named DG4, which is impacted by penguin droppings, was retrieved from a lake catchment in Gardner Island of Vestfold Hills, East Antarctica. In this study, the concentrations of characteristic elements in the core, local bedrocks and fresh penguin guanos were determined. P, Se, F, S, As, Sr and Cu in DG4 were identified as the bio-element assemblage by R-clustering analysis and compared with those in the local bedrocks and fresh guanos, the results are similar to Y2 in Ardley Island, Antarctic Peninsula. On this basis, P and Se were identified as the optimum bio-elements in DG4 and F, P and S were identified in Y2, respectively. This work will provides the foundation for reconstructing the past penguin populations in Gardner Island of Vest- fold Hills, East Antarctica and comparing the penguin population dynamics between East Antarctica and Antarctic Peninsula.  相似文献   

19.
The southern sea area of the Huludao City, Liaoning Province might be polluted by heavy metals because it is close to the Jinzhou Bay, one of the heaviest sea area polluted by heavy metals in China. The undisturbed modern sediment core can be used to analyze the accumulation and source of the pollutants using 137 Cs and 210 Pb ex . Thirty-five samples of surface sediment and two core sediments were collected from the southern sea area of Huludao City. The concentrations of copper (Cu), lead (Pb), chrome (Cr), zinc (Zn), arsenic (As) and mercury (Hg) in the surface sediments as well as Cu, Pb, Zn, Cr, 137 Cs and 210 Pb ex in the core sediments were determined to research the spatial distribution and accumulation characteristics, and to analyze the sources and the potential risks of heavy metals. The results show that the pollution levels of Zn and Hg are serious, and 26 stations are at moderate or heavy ecological risks. The concentrations of the heavy metals increase from east to west, as well as from open sea to offshore marine area. The concentrations of heavy metals are not high in the sediments adjacent to the Jinzhou Bay, and the influence caused by the seawater exchange with the Jinzhou Bay is little. The concentrations of the heavy metals in the core sediments show low-high-low characteristic, and it coincides with the pollution history of Huludao City. The atmospheric deposition of heavy metals from the Huludao Zinc Plant is likely to be the main source of pollution without direct discharge of wastewater. The high concentrations of heavy metals appear on the upper sediment of 20 cm. The shallow sediment with high heavy metal contents might be exposed to surface when it was disturbed by the ocean engineering and big storm surge, then cause risk to the safety of aquaculture and human healthy.  相似文献   

20.
Hydrogen and oxygen isotopes in precipitation have been widely used as effective traces to investigate hydrological processes such as evaporation and atmospheric moisture source. This study analyzed δD and δ~(18)O of precipitation in continuous event-based samples at three stations of Pailugou Catchment from November 2012 to December 2013. The δ~(18)O and δD values ranged from-32.32‰ to +3.23‰ and from-254.46‰ to +12.11‰, respectively. Results show that the δ~(18)O displayed a distinct seasonal variation, with enriched values occurring in summer and relatively depleted values in winter, respectively. There was a statistically significant positive correlation between the δ~(18)O and δD values and local surface air temperature at all the three stations. The nearest Global Network of Isotopes in Precipitation(GNIP) station(Zhangye), compared to the Meteoric Water Lines for this study, showed the obvious local evaporation effects with lower intercept and slope. Additionally, d-excess(δD- 8δ~(18)O) parameter in precipitation exhibited an anti-phase seasonal variability with the δ~(18)O. The 96-h back trajectories for each precipitation event using Hybrid Single Particle Lagrangian Integrated Trajectory(HYSPLIT) model indicated a dominant effect of westerly air masses in summer and the integrated influence of westerly and polar air masses in winter.  相似文献   

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