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1.
Daiki Yamamoto Shogo Tachibana Noriyuki Kawasaki Hisayoshi Yurimoto 《Meteoritics & planetary science》2020,55(6):1281-1292
Oxygen isotope exchange experiments between tens of nanometer‐sized amorphous enstatite grains and water vapor were carried out under a condition of protoplanetary disk‐like low water vapor pressure in order to investigate the survivability of distinct oxygen isotope signatures of presolar silicate grains in the protosolar disk. Oxygen isotope exchange between amorphous enstatite and water vapor proceeded at 923–1003 K and 0.3 Pa of water vapor through diffusive isotope exchange in the amorphous structure. The rate of diffusive isotope exchange is given by D (m2 s–1) = (5.0 ± 0.2) × 10–21 exp[–161.3 ± 1.7 (kJ mol–1) R–1 (1/T–1/1200)]. The activation energy for the diffusive isotope exchange for amorphous enstatite is the same as that for amorphous forsterite within the analytical uncertainties, but the isotope exchange rate is ~30 times slower in amorphous enstatite because of the difference in frequency factor of the reaction. The reaction kinetics indicates that 0.1–1 μm‐sized presolar amorphous silicate dust with enstatite and forsterite compositions would avoid oxygen isotope exchange with protosolar disk water vapor only if they were kept at temperatures below ~500–650 K within the lifetime of the disk gas. 相似文献
2.
Abstract— Fayalitic olivine (Fa32) is the major component of the matrices and dark inclusions of CV3 and other unequilibrated chondrites. It occurs most commonly as rims, veins and halos in and around chondrule silicates in the Allende-type (CV3OXA) chondrites and, to a much lesser extent, in the reduced (CV3R) and Bali-type (CV3OXB) chondrites. The olivines have distinctive platy, tabular and lath- or irregular-shaped crystals, with the ratio of the two types varying widely. In CV3OXB chondrites, matrix fayalitic olivines range up to Fag99.9; whereas, in the other CV3 chondrites, the range is much smaller. The platy and tabular anisotropic forms of the fayalitic olivines strongly suggest growth from a vapor, and the nature of the occurrences suggests that CV3 matrices are unequilibrated mixtures of nebular materials. We argue that the parent body hydration/dehydration model has numerous inconsistencies that make this hypothesis highly unlikely. These include: (1) There is no direct evidence linking fayalitic olivine to precursor phyllosilicates. (2) Dehydration of phyllosilicates cannot explain the wide range of morphologies of the fayalitic olivines. (3) Fayalitic olivine clearly predates the formation of the hydrous phases in CV3 chondrites and is one of the phases that breaks down to form phyllosilicates (Keller et al., 1994). (4) The unequilibrated nature of the matrix, including fine-scale zoning in 10 μm sized fayalitic olivine crystals, would not survive the parent body metamorphism required in the dehydration model. (5) A dark inclusion in the Ningqiang chondrite contains fayalitic olivine rimmed by glassy and microcrystalline material (Zolensky et al., 1997), which probably formed by radiation damage. This indicates that the fayalitic olivine was exposed to solar radiation in a nebular setting. (6) Some Allende chondrules contain unaltered primary, anhydrous glassy mesostasis in contact with the host matrix (e.g., Ikeda and Kimura, 1995). Chondrule mesostases would not have survived parent body hydration without becoming hydrated and would probably not survive the metamorphic heating required in the dehydration scenario. (7) Single platy and barrel-shaped crystals of fayalitic olivine are present in accretionary rims in calcium-aluminum-rich inclusions (CAIs) (MacPherson and Davis, 1997), which developed in the nebula. (8) Matrix lumps completely encased in chondrules in ordinary chondrites contain mainly fayalitic olivine (Scott et al., 1984), which indicates a nebular origin. (9) Oxygen isotopic compositions of Allende matrix and dark inclusions strongly indicate little or no hydration for Allende and its components (Clayton, 1997). We favor a nebular vaporization/recondensation model in which vaporization of chondritic dust produced a fayalite-rich vapor, followed by formation of the fayalitic olivine by direct recondensation from the vapor, epitactic growth on surfaces of existing forsterite and enstatite in chondrules, and replacement of existing forsterite and enstatite by gas-solid exchange. 相似文献
3.
The zodiacal light is the dominant source of the mid-infrared sky brightness seen from Earth, and exozodiacal light is the dominant emission from planetary and debris systems around other stars. We observed the zodiacal light spectrum with the mid-infrared camera ISOCAM over the wavelength range 5-16 μm and a wide range of orientations relative to the Sun (solar elongations 68°-113°) and the ecliptic (plane to pole). The temperature in the ecliptic ranged from 269 K at solar elongation 68° to 244 K at 113°, and the polar temperature, characteristic of dust 1 AU from the Sun, is 274 K. The observed temperature is exactly as expected for large (>10 μm radius), low-albedo (<0.08), rapidly-rotating, gray particles 1 AU from the Sun. Smaller particles (<10 μm radius) radiate inefficiently in the infrared and are warmer than observed. We present theoretical models for a wide range of particle size distributions and compositions; it is evident that the zodiacal light is produced by particles in the 10-100 μm radius range. In addition to the continuum, we detect a weak excess in the 9-11 μm range, with an amplitude of 6% of the continuum. The shape of the feature can be matched by a mixture of silicates: amorphous forsterite/olivine provides most of the continuum and some of the 9-11 μm silicate feature, dirty crystalline olivine provides the red wing of the silicate feature (and a bump at 11.35 μm), and a hydrous silicate (montmorillonite) provides the blue wing of the silicate feature. The presence of hydrous silicate suggests the parent bodies of those particles were formed in the inner solar nebula. Large particles dominate the size distribution, but at least some small particles (radii ∼1 μm) are required to produce the silicate emission feature. The strength of the feature may vary spatially, with the strongest features being at the lowest solar elongations as well as at high ecliptic latitudes; if confirmed, this would imply that the dust properties change such that dust further from the Sun has a weaker silicate feature. To compare the properties of zodiacal dust to dust around other main sequence stars, we reanalyzed the exozodiacal light spectrum for β Pic to derive the shape of its silicate feature. The zodiacal and exozodiacal spectra are very different. The exozodiacal spectra are dominated by cold dust, with emission peaking in the far-infrared, while the zodiacal spectrum peaks around 20 μm. We removed the debris disk continuum from the spectra by fitting a blackbody with a different temperature for each aperture (ranging from 3.7″ to 27″); the resulting silicate spectra for β Pic are identical for all apertures, indicating that the silicate feature arises close to the star. The shape of the silicate feature from β Pic is nearly identical to that derived from the ISO spectrum of 51 Oph; both exozodiacal features are very different from that of the zodiacal light. The exozodiacal features are roughly triangular, peaking at 10.3 μm, while the zodiacal feature is more boxy, indicating a different mineralogy. 相似文献
4.
Michael D Smith 《Icarus》2004,167(1):148-165
We use infrared spectra returned by the Mars Global Surveyor Thermal Emission Spectrometer (TES) to retrieve atmospheric and surface temperature, dust and water ice aerosol optical depth, and water vapor column abundance. The data presented here span more than two martian years (Mars Year 24, Ls=104°, 1 March 1999 to Mars Year 26, Ls=180°, 4 May 2003). We present an overview of the seasonal (Ls), latitudinal, and longitudinal dependence of atmospheric quantities during this period, as well as an initial assessment of the interannual variability in the current martian climate. We find that the perihelion season (Ls=180°-360°) is relatively warm, dusty, free of water ice clouds, and shows a relatively high degree of interannual variability in dust optical depth and atmospheric temperature. On the other hand, the aphelion season (Ls=0°-180°) is relatively cool, cloudy, free of dust, and shows a low degree of interannual variability. Water vapor abundance shows a moderate amount of interannual variability at all seasons, but the most in the perihelion season. Much of the small amount of interannual variability that is observed in the aphelion season appears to be caused by perihelion-season planet-encircling dust storms. These dust storms increase albedo through deposition of bright dust on the surface causing cooler daytime surface and atmospheric temperatures well after dust optical depth returns to prestorm values. 相似文献
5.
The infrared AOTF spectrometer is a part of the SPICAM experiment onboard the Mars-Express ESA mission. The instrument has a capability of solar occultations and operates in the spectral range of 1-1.7 μm with a spectral resolution of ∼3.5 cm−1. We report results from 24 orbits obtained during MY28 at Ls 130°-160°, and the latitude range of 40°-55° N. For these orbits the atmospheric density from 1.43 μm CO2 band, water vapor mixing ratio based on 1.38 μm absorption, and aerosol opacities were retrieved simultaneously. The vertical resolution of measurements is better than 3.5 km. Aerosol vertical extinction profiles were obtained at 10 wavelengths in the altitude range from 10 to 60 km. The interpretation using Mie scattering theory with adopted refraction indices of dust and H2O ice allows to retrieve particle size (reff∼0.5-1 μm) and number density (∼1 cm−3 at 15-30 km) profiles. The haze top is generally below 40 km, except the longitude range of 320°-50° E, where high-altitude clouds at 50-60 km were detected. Optical properties of these clouds are compatible with ice particles (effective radius reff=0.1-0.3 μm, number density N∼10 cm−3) distributed with variance νeff=0.1-0.2 μm. The vertical optical depth of the clouds is below 0.001 at 1 μm. The atmospheric density profiles are retrieved from CO2 band in the altitude range of 10-90 km, and H2O mixing ratio is determined at 15-50 km. Unless a supersaturation of the water vapor occurs in the martian atmosphere, the H2O mixing ratio indicates ∼5 K warmer atmosphere at 25-45 km than predicted by models. 相似文献
6.
From recent close encounters with Comets Wild-2 and Tempel 1 we learned that their surfaces are very rugged and no simple uniform layers model can be applied to them. Rather, a glaciological approach should be applied for describing their surface features and behavior. Such intrinsically rugged surface is formed in our large scale experiments, where an agglomerate of ∼200 μm gas-laden amorphous ice particles is accumulated to form a 20 cm diameter and few cm high ice sample. The density, tensile strength and thermal inertia of our ice sample were found to be very close to those found by Deep Impact for Comet Tempel 1: density 250-300 kg m−3 vs DI 350-400 kg m−3; tensile strength 2-4 kPa vs DI 1-10 kPa; thermal inertia 80 W K−1 m−2 s1/2 vs <100 W K−1 m−2 s1/2 and <50 W K−1 m−2 s1/2. From the close agreement between the thermal inertias measured in our ice sample, which had no dust coverage and that of Comet Tempel 1, we deduce that the low thermal inertia is an intrinsic property of the fluffy structure of the ice as a result of its low density, with an addition by the broken terrain and not due to the formation of a dust layer. Upon warming up of the ice, water vapor migrates both outward into the coma and inward. Reaching cooler layers, the water vapor condenses, forming a denser ice crust, as we show experimentally. We also demonstrate the inward and outward flow of water vapor in the outer ice layers through the exchange between layers of D2O ice and H2O ice, to form HDO. 相似文献
7.
The CIRS infrared spectrometer onboard the Cassini spacecraft has scanned Saturn's A ring azimuthally from several viewing angles since its orbit insertion in 2004. A quadrupolar asymmetry has been detected in this ring at spacecraft elevations ranging between 16° to 37°. Its fractional amplitude decreases from 22% to 8% from 20° to 37° elevations. The patterns observed in two almost complete azimuthal scans at elevations 20° and 36° strongly favor the self-gravity wakes as the origin of the asymmetry. The elliptical, infinite cylinder model of Hedman et al. [Hedman, M.M., Nicholson, P.D., Salo, H., Wallis, B.D., Buratti, B.J., Baines, K.H., Brown, R.H., Clark, R.N., 2007. Astron. J. 133, 2624-2629] can reproduce the CIRS observations well. Such wakes are found to have an average height-to-spacing ratio H/λ=0.1607±0.0002, a width-over-spacing W/λ=0.3833±0.0008. Gaps between wakes, which are filled with particles, have an optical depth τG=0.1231±0.0005. The wakes mean pitch angle ΦW is 70.70°±0.07°, relative to the radial direction. The comparison of ground-based visible data with CIRS observations constrains the A ring to be a monolayer. For a surface mass density of 40 g cm−2 [Tiscarino, M.S., Burns, J.A., Nicholson, P.D., Hedman, M.M., Porco, C.C., 2007. Icarus 189, 14-34], the expected spacing of wakes is λ≈60 m. Their height and width would then be H≈10 m and W≈24 m, values that match the maximum size of particles in this ring as determined from ground-based stellar occultations [French, R.G., Nicholson, P.D., 2000. Icarus 145, 502-523]. 相似文献
8.
A sensitive search for SO2 in the martian atmosphere: Implications for seepage and origin of methane
Vladimir A. Krasnopolsky 《Icarus》2005,178(2):487-492
Mars was observed near the peak of the strongest SO2 band at 1364-1373 cm−1 with resolving power of 77,000 using the Texas Echelon Cross Echelle Spectrograph on the NASA Infrared Telescope Facility. The observation covered the Tharsis volcano region which may be preferable to search for SO2. The spectrum shows absorption lines of three CO2 isotopomers and three H2O isotopomers. The water vapor abundance derived from the HDO lines assuming D/H = 5.5 times the terrestrial value is 12±1.0 pr. μm, in agreement with the simultaneous MGS/TES observations of 14 pr. μm at the latitudes (50° S to 10° N) of our observation. Summing of spectral intervals at the expected positions of sixteen SO2 lines puts a 2σ upper limit on SO2 of 1 ppb. SO2 may be emitted into the martian atmosphere by seepage and is removed by three-body reactions with OH and O. The SO2 lifetime, 2 years, is longer than the global mixing time 0.5 year, so SO2 should be rather uniformly distributed across Mars. Seepage of SO2 is less than 15,000 tons per year on Mars which is smaller than the volcanic production of SO2 on the Earth by a factor of 700. Because CH4/SO2 is typically 10−4-10−3 in volcanic gases on the Earth, our results show seepage is unlikely to be the source of the recently discovered methane on Mars and therefore strengthen its biogenic origin. 相似文献
9.
We measured the velocity distributions of impact ejecta with velocities higher than ∼100 m s−1 (high-velocity ejecta) for impacts at variable impact angle α into unconsolidated targets of small soda-lime glass spheres. Polycarbonate projectiles with mass of 0.49 g were accelerated to ∼250 m s−1 by a single-stage light-gas gun. The impact ejecta are detected by thin aluminum foils placed around the targets. We analyzed the holes on the aluminum foils to derive the total number and volume of ejecta that penetrated the aluminum foils. Using the minimum velocity of the ejecta for penetration, determined experimentally, the velocity distributions of the high-velocity ejecta were obtained at α=15°, 30°, 45°, 60°, and 90°. The velocity distribution of the high-velocity ejecta is shown to depend on impact angle. The quantity of the high-velocity ejecta for vertical impact (α=90°) is considerably lower than derived from a power-law relation for the velocity distribution on the low-velocity ejecta (less than 10 m s−1). On the other hand, in oblique impacts, the quantity of the high-velocity ejecta increases with decreasing impact angle, and becomes comparable to those derived from the power-law relation. We attempt to scale the high-velocity ejecta for oblique impacts to a new scaling law, in which the velocity distribution is scaled by the cube of projectile radius (scaled volume) and a horizontal component of impactor velocity (scaled ejection velocity), respectively. The high-velocity ejecta data shows a good correlation between the scaled volume and the scaled ejection velocity. 相似文献
10.
Olivine dissolution in molten silicates: An experimental study with application to chondrule formation 
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下载免费PDF全文 Mg‐rich olivine is a ubiquitous phase in type I porphyritic chondrules in various classes of chondritic meteorites. The anhedral shape of olivine grains, their size distribution, as well as their poikilitic textures within low‐Ca pyroxene suggest that olivines suffer dissolution during chondrule formation. Owing to a set of high‐temperature experiments (1450–1540 °C) we determined the kinetics of resorption of forsterite in molten silicates, using for the first time X‐ray microtomography. Results indicate that forsterite dissolution in chondrule‐like melts is a very fast process with rates that range from ~5 μm min?1 to ~22 μm min?1. Forsterite dissolution strongly depends on the melt composition, with rates decreasing with increasing the magnesium and/or the silica content of the melt. An empirical model based on forsterite saturation and viscosity of the starting melt composition successfully reproduces the forsteritic olivine dissolution rates as a function of temperature and composition for both our experiments and those of the literature. Application of our results to chondrules could explain the textures of zoned type I chondrules during their formation by gas‐melt interaction. We show that the olivine/liquid ratio on one hand and the silica entrance from the gas phase (SiOg) into the chondrule melt on the other hand, have counteracting effects on the Mg‐rich olivine dissolution behavior. Silica entrance would favor dissolution by maintaining disequilibrium between olivine and melt. Hence, this would explain the preferential dissolution of olivine as well as the preferential abundances of pyroxene at the margins of chondrules. Incipient dissolution would also occur in the silica‐poorer melt of chondrule core but should be followed by crystallization of new olivine (overgrowth and/or newly grown crystals). While explaining textures and grain size distributions of olivines, as well as the centripetal distribution of low‐Ca pyroxene in porphyritic chondrules, this scenario could also be consistent with the diverse chemical, isotopic, and thermal conditions recorded by olivines in a given chondrule. 相似文献
11.
We present an analysis of the observations of the Deep Impact event performed by the OSIRIS narrow angle camera aboard the Rosetta spacecraft over two weeks, in an effort to characterize the cometary dust grains ejected from the nucleus of Comet 9P/Tempel 1. We adopt a Monte Carlo approach to generate calibrated synthetic images, and a linear combination of them is fitted to the calibrated images so as to determine the physical parameters of the dust cloud. Our model considers spherical olivine particles with a density of 3780 kg m−3. It incorporates constraints on the direction of the cone of emission coming from additional images obtained at Pic du Midi observatory, and constraints on the dust terminal velocities coming from the physics of the impact. We find that the slope of the differential dust size distribution of grains with radii <20 μm (β>0.008) is 3.1±0.3, a value typical of cometary dust tails. This shows that there is no evidence in our data for an enhancement in sub-micron particles in the ejecta compared to the typical dust distribution of active comets. We estimate the mass of particles with radii <1.4 μm (β>0.14) to be 1.5±0.2×105 kg. These particles represent more than 80% of the cross-section of the observed dust cloud. The mass carried by larger particles depends whether the gas significantly increases the kinetic energy of the grains in the inner coma; it lies in the range 1-14×106 kg for particles with radii <100 μm (β>0.002). We obtain the distribution of terminal velocities reached by the dust after the dust-gas interaction which is very well constrained between 10 and 600 m s−1. It is characterized by Gaussian with a maximum at about 190 m s−1 and a width at half maximum of 150 m s−1. 相似文献
12.
Bruce A. Cantor 《Icarus》2007,186(1):60-96
From 15 September 1997 through 21 January 2006, only a single planet-encircling martian dust storm was observed by MGS-MOC. The onset of the storm occurred on 26 June 2001 (Ls=184.7°), earliest recorded to date. It was initiated in the southern mid-to-low latitudes by a series of local dust storm pulses that developed along the seasonal cap edge in Malea and in Hellas basin (Ls=176.2°-184.4°). The initial expansion of the storm, though asymmetric, was very rapid in all directions (3-32 m s−1). The main direction of propagation, however, was to the east, with the storm becoming planet encircling in the southern hemisphere on Ls=192.3°. Several distinct centers of active dust lifting were associated with the storm, with the longest persisting for 86 sols (Syria-Claritas). These regional storms helped generate and sustain a dust cloud (“haze”), which reached an altitude of about 60 km and a peak opacity of τdust∼5.0. By Ls=197.0°, the cloud had encircled the entire planet between 59.0° S and 60.0° N, obscuring all but the largest volcanoes. The decay phase began around Ls∼200.4° with atmospheric dust concentrations returning to nominal seasonal low-levels at Ls∼304.0°. Exponential decay time constants ranged from 30-117 sols. The storm caused substantial regional albedo changes (darkening and brightening) as a result of the redistribution (removal and deposition) of a thin veneer of surface dust at least 0.1-11.1 μm thick. It also caused changes in meteorological phenomena (i.e., dust storms, dust devils, clouds, recession of the polar caps, and possibly surface temperatures) that persisted for just a few weeks to more than a single Mars year. The redistribution of dust by large annual regional storms might help explain the long period (∼30 years) between the largest planet-encircling dust storms events. 相似文献
13.
Disruptive collisions in the main belt can liberate fragments from parent bodies ranging in size from several micrometers to tens of kilometers in diameter. These debris bodies group at initially similar orbital locations. Most asteroid-sized fragments remain at these locations and are presently observed as asteroid families. Small debris particles are quickly removed by Poynting-Robertson drag or comminution but their populations are replenished in the source locations by collisional cascade. Observations from the Infrared Astronomical Satellite (IRAS) showed that particles from particular families have thermal radiation signatures that appear as band pairs of infrared emission at roughly constant latitudes both above and below the Solar System plane. Here we apply a new physical model capable of linking the IRAS dust bands to families with characteristic inclinations. We use our results to constrain the physical properties of IRAS dust bands and their source families. Our results indicate that two prominent IRAS bands at inclinations ≈2.1° and ≈9.3° are byproducts of recent asteroid disruption events. The former is associated with a disruption of a ≈30-km asteroid occurring 5.8 Myr ago; this event gave birth to the Karin family. The latter came from the breakup of a large >100-km-diameter asteroid 8.3 Myr ago that produced the Veritas family. Using an N-body code, we tracked the dynamical evolution of ≈106 particles, 1 μm to 1 cm in diameter, from both families. We then used these results in a Monte Carlo code to determine how small particles from each population undergo collisional evolution. By computing the thermal emission of particles, we were able to compare our results with IRAS observations. Our best-fit model results suggest the Karin and Veritas family particles contribute by 5-9% in 10-60-μm wavelengths to the zodiacal cloud's brightness within 50° latitudes around the ecliptic, and by 9-15% within 10° latitudes. The high brightness of the zodiacal cloud at large latitudes suggests that it is mainly produced by particles with higher inclinations than what would be expected for asteroidal particles produced by sources in the main belt. From these results, we infer that asteroidal dust represents a smaller fraction of the zodiacal cloud than previously thought. We estimate that the total mass accreted by the Earth in Karin and Veritas particles with diameters 20-400 μm is ≈15,000-20,000 tons per year (assuming 2 g cm−3 particles density). This is ≈30-50% of the terrestrial accretion rate of cosmic material measured by the Long Duration Exposure Facility. We hypothesize that up to ≈50% of our collected interplanetary dust particles and micrometeorites may be made up of particle species from the Veritas and Karin families. The Karin family IDPs should be about as abundant as Veritas family IDPs though this ratio may change if the contribution of third, near-ecliptic source is significant. Other sources of dust and/or large impact speeds must be invoked to explain the remaining ≈50-70%. The disproportional contribution of Karin/Veritas particles to the zodiacal cloud (only 5-9%) and to the terrestrial accretion rate (30-50%) suggests that the effects of gravitational focusing by the Earth enhance the accretion rate of Karin/Veritas particles relative to those in the background zodiacal cloud. From this result and from the latitudinal brightness of the zodiacal cloud, we infer that the zodiacal cloud emission may be dominated by high-speed cometary particles, while the terrestrial impactor flux contains a major contribution from asteroidal sources. Collisions and Poynting-Robertson drift produce the size-frequency distribution (SFD) of Karin and Veritas particles that becomes increasingly steeper closer to the Sun. At 1 AU, the SFD is relatively shallow for small particle diameters D (differential slope exponent of particles with D?100 μm is ≈2.2-2.5) and steep for D?100 μm. Most of the mass at 1 AU, as well as most of the cross-sectional area, is contributed by particles with D≈100-200 μm. Similar result has been found previously for the SFD of the zodiacal cloud particles at 1 AU. The fact that the SFD of Karin/Veritas particles is similar to that of the zodiacal cloud suggests that similar processes shaped these particle populations. We estimate that there are ≈5×1024 Karin and ≈1025 Veritas family particles with D>30 μm in the Solar System today. The IRAS observation of the dust bands may be satisfactorily modeled using ‘averaged’ SFDs that are constant with semimajor axis. These SFDs are best described by a broken power-law function with differential power index α≈2.1-2.4 for D?100 μm and by α?3.5 for 100 μm?D?1 cm. The total cross-sectional surface area of Veritas particles is a factor of ≈2 larger than the surface area of the particles producing the inner dust bands. The total volumes in Karin and Veritas family particles with 1 μm<D<1 cm correspond to D=11 km and D=14 km asteroids with equivalent masses ≈1.5×1018 g and ≈3.0×1018 g, respectively (assuming 2 g cm−3 bulk density). If the size-frequency and radial distribution of particles in the zodiacal cloud were similar to those in the asteroid dust bands, we estimate that the zodiacal cloud represents ∼3×1019 g of material (in particles with 1 μm<D<1 cm) at ±10° around the ecliptic and perhaps as much as ∼1020 g in total. The later number corresponds to about a 23-km-radius sphere with 2 g cm−3 density. 相似文献
14.
Daniel B. Curtis Courtney D. Hatch Christa A. Hasenkopf Owen B. Toon Margaret A. Tolbert Christopher P. McKay 《Icarus》2008,195(2):792-801
Titan, Saturn's largest moon, has a thick nitrogen/methane atmosphere. The temperature and pressure conditions in Titan's atmosphere are such that the methane vapor should condense near the tropopause to form clouds. Several ground-based measurements have observed sparse cloud-like features in Titan's atmosphere, while the Cassini mission to Saturn has provided large scale images of the clouds. However, Titan's cloud formation conditions remain poorly constrained. Heterogeneous nucleation (from the vapor phase onto a solid or liquid aerosol surface) greatly enhances cloud formation relative to homogeneous nucleation. In order to elucidate the cloud formation mechanism near the tropopause, we have performed laboratory measurements of the adsorption of methane and ethane onto solid organic particles (tholins) representative of Titan's photochemical haze. We find that monolayers of methane adsorb onto tholin particles at saturation ratios less than unity. We also find that solid methane nucleates onto the adsorbed methane at a saturation ratio of S=1.07±0.008. This implies that Titan's methane clouds should form easily. This is consistent with recent measurements of the column of methane ruling out excessive methane supersaturation. In addition, we find ethane adsorbs onto tholin particles in a metastable phase prior to nucleation. However, ethane nucleation onto the adsorbed ethane occurs at a relatively high saturation ratio of S=1.36±0.08. These findings are consistent with the recent report of polar ethane clouds in Titan's lower stratosphere. 相似文献
15.
Ian M. Steele 《Meteoritics & planetary science》1990,25(4):301-307
Abstract— The rare Mg-rich silicate fraction of the C1 meteorites, Orgueil and Alais, is dominated by minute (< 30 μm) forsterite. Twenty three forsterite grains of these meteorites as well as large forsterites in two chondritic porous interplanetary dust particles (IDPs) are characterized by levels of MnO generally, but not always, higher than found in forsterites of C2, C3 and unequilibrated ordinary chondrites (UOC). Forsterite in Orgueil contains 900 to 6200 ppmw MnO while Alais forsterite has less than 2000 ppmw MnO suggesting that the forsterites in the two meteorites are chemically distinct. Alais forsterite shows lower Cr and Al relative to Orgueil forsterite. The C1 forsterites do not show Fe-poor (FeO < 0.3), refractory-rich (Al, Ca, Ti, V) compositions which are relatively common in the C2-C3-UOC meteorites suggesting that the most primitive forsterite compositions are not present in these C1 meteorites. While minor elements in forsterite can not distinguish unambiguously between C1 and C2-C3-UOC sources, the high Mn levels in some IDP forsterites are similar to some C1 forsterites suggesting a possible relation between the forsterites of these two extraterrestrial samples. 相似文献
16.
The potentially hazardous Asteroid (33342) 1998 WT24 approached the Earth within 0.0125 AU on 2001 December 16 and was the target of a number of optical, infrared, and radar observing campaigns. Interest in 1998 WT24 stems from its having an orbit with an unusually low perihelion distance, which causes it to cross the orbits of the Earth, Venus, and Mercury, and its possibly being a member of the E spectral class, which is rare amongst near-Earth asteroids (NEAs). We present the results of extensive thermal-infrared observations of 1998 WT24 obtained in December 2001 with the 3-m NASA Infrared Telescope Facility (IRTF) on Mauna Kea, Hawaii and the ESO 3.6-m telescope in Chile. A number of thermal models have been applied to the data, including thermophysical models that give best-fit values of 0.35±0.04 km for the effective diameter, 0.56±0.2 for the geometric albedo, pv, and 100-300 J m−2 s−0.5 K−1 for the thermal inertia. Our values for the diameter and albedo are consistent with results derived from radar and polarimetric observations. The albedo is one of the highest values obtained for any asteroid and, since no other taxonomic type is associated with albedos above 0.5, supports the suggested rare E-type classification for 1998 WT24. The thermal inertia is an order of magnitude higher than values derived for large main-belt asteroids but consistent with the relatively high values found for other near-Earth asteroids. A crude pole solution inferred from a combination of our observations and published radar results is β=−52°, λ=355° (J2000), but we caution that this is uncertain by several tens of degrees. 相似文献
17.
We obtained spatially-resolved ultraviolet spectra of Saturn in 1994 with the Faint Object Spectrometer and Goddard High Resolution Spectrograph of the Hubble Space Telescope. We observed four areas on the planet at 15° N, 33° S, 41° S, and 52° S, with a field-of-view of less than 2 × 2 arcsec2, compared to the 16-arcsec planet diameter. The wavelength range, 1550-2300 Å, encompasses absorption from major hydrocarbons (C2H6, C2H4, C2H2, CH3C2H, C4H2) and water. We find global hydrocarbon abundances and a C2H2 vertical distribution compatible with infrared observations, in contrast with previous analyses of ultraviolet spectra. The stratospheric haze opacity decreases from polar region to the equator. Saturn mid-latitudes are photochemically distinct from the rest of the planet. At 33° S, the spectrum requires either (1) a distinctly different C2H2 vertical distribution or (2) a locally enhanced water abundance. At 41° S, the hydrocarbon abundance exhibits a local minimum, within a global trend of increasing abundance from equator to pole. This global trend may result from an increased abundance of short-lived hydrocarbons such as C4H2. Photochemical models predict a depletion of hydrocarbon molecules in the presence of stratospheric water [Moses et al., 2000. Icarus 143, 166-202]. These results are consistent with a localized influx of water, in the form of high charge to mass ratio particles, flowing into Saturn's atmosphere at latitudes magnetically linked to the rings. 相似文献
18.
Atmospheric water vapor abundances in Mars’ north polar region (NPR, from 60° to 90°N) are mapped as function of latitude and longitude for spring and summer seasons, and their spatial, seasonal, and interannual variability is discussed. Water vapor data are from Mars Global Surveyor (MGS) Thermal Emission Spectrometer (TES) and the Viking Orbiter (VO) Mars Atmospheric Water Detector (MAWD). The data cover three complete northern spring-summer seasons in 1977-1978, 2000-2001 and 2002-2003, and shorter periods of spring-summer seasons during 1975, 1999 and 2004. Long term interannual variability in the averaged NPR abundances may exist, with Viking MAWD observations showing twice as much water vapor during summer as the MGS TES observations more than 10 martian years (MY) later. While the averaged abundances are very similar in TES observations for the same season in different years, the spatial distributions in the early summer season do vary significantly year over year. Spatial and temporal variabilities increase between Ls ∼ 80-140°, which may be related to vapor sublimation from the North Polar Residual Cap (NPRC), or to changes in circulation. Spatial variability is observed on scales of ∼100 km and temporal variability is observed on scales of <10 sols during summer. During late spring the TES water vapor spatial distribution is seen to correlate with the low topography/low albedo region of northern Acidalia Planitia (270-360°E), and with the dust spatial distribution across the NPR during late spring-early summer. Non-uniform vertical distribution of water vapor, a regolith source or atmospheric circulation ‘pooling’ of water vapor from the NPRC into the topographic depression may be behind the correlation with low topography/low albedo. Sublimation winds carrying water vapor off the NPRC and lifting surface dust in the areas surrounding the NPRC may explain the correlation between the water vapor and dust spatial distributions. Correlation between water vapor and dust in MAWD data are only observed over low topography/low albedo area. Maximum water vapor abundances are observed at Ls = 105-115° and outside of the NPRC at 75-80°N; the TES data, however, do not extend over the NPRC and thus, this conclusion may be biased. Some water vapor appears to be released in plumes or ‘outbursts’ in the MAWD and TES datasets during late spring and early summer. We propose that the sublimation rate of ice varies across the NPRC with varying surface winds, giving rise to the observed ‘outbursts’ at some seasons. 相似文献
19.
Maho Yamada Shogo Tachibana Hiroko Nagahara Kazuhito Ozawa 《Planetary and Space Science》2006,54(11):1096-1106
Evaporation of solid materials under low-pressure conditions could play important roles in chemical and isotopic fractionations in the early solar system. We have studied anisotropy of isotopic fractionation of 26Mg and 25Mg during kinetic evaporation of forsterite (Mg2SiO4), which is potentially a powerful tool to understand thermal histories of crystals in the early solar system. Ion-microprobe depth profiling revealed that the Mg isotopic zoning profiles of forsterite evaporated at 1500-1700 °C are notably differing along the a-, b-, and c-axes, which can be attributed to anisotropy in self-diffusion coefficient of Mg (D) and an isotopic fractionation factor for evaporation of Mg (α). The D and α were obtained from zoning profiles by applying the diffusion-controlled isotopic fractionation model of Wang et al. [1999. Evaporation of single crystal forsterite: Evaporation kinetics, magnesium isotope fractionation, and implications of mass-dependent isotopic fractionation of a diffusion-controlled reservoir. Geochim. Cosmochim. Acta 63(6), 953-966.].The D is largest and smallest along the a- and c-axes, respectively. The activation energy of 560-670 kJ/mol indicates that Mg diffusion at 1500-1700 °C occurred in the intrinsic diffusion regime.The α seems to be larger along the a- or c-axes than along the b-axis. The α along the a- or c-axes show weak temperature dependence. The α along all the crystallographic orientations is closer to unity than that expected from the kinetic theory of gases. These lines of evidence suggest that surface processes such as breaking of bonds and surface diffusion are responsible for the isotopic fractionation. 相似文献
20.
Vladimir A Krasnopolsky 《Icarus》2003,165(2):315-325
The O2 dayglow at 1.27 μm is formed by high-altitude ozone on Mars and is a sensitive tracer of Mars photochemistry. Mapping of this dayglow using the IRTF/CSHELL long-slit spectrograph requires the extraction of weak emission lines against a strong continuum of the reflected solar light. Some new tools are suggested to improve the data processing. The observed O2 dayglow intensities at LS=67°, 112°, 148°, and 173° show a decrease from late spring (aphelion) to fall equinox by a factor of ≈5 at low latitudes (±30°). This decrease agrees with that predicted by a model of Clancy and Nair (1996, J. Geophys. Res. 101 (12) 12785-12790), although the dayglow intensities are weaker than those based on that model. The measured dayglow variations with latitude are rather low at LS=67°, 112°, and 148° and unexpectedly high at 173°. The dayglow intensity peaks near noon and is smaller at 9:00 and 16:30 LT by a factor of 2. Some data on the ozone profile near aphelion are obtained from a combination of the dayglow and ozone observations. It is hardly possible to detect the O2 night airglow at 1.27 μm on Mars using the existing ground-based and on-orbit instruments. The O2 dayglow intensity as a function of latitude and season from aphelion to fall equinox has been obtained. Our goal is to extend this distribution to the full martian year and get a database for Mars photochemistry to complement the MGS/TES observations of water vapor, atmospheric temperature, and dust and ice aerosol. 相似文献