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41.
Angela Marinoni Paolo Laj Pierre Alexandre Deveau Federica Marino Grazia Ghermandi Fabien Aulagnier Hlne Cachier 《Atmospheric Research》2005,74(1-4):565-580
The physical and chemical properties of aerosol particles were investigated at Plan d'Aups, one of the ESCOMPTE sites located in the St. Baume mountain area (700 m a.s.l.), 50 km east of Marseilles (France). The site is ideally located for assessing the vertical and horizontal extent of the pollution plume from the Marseilles–Berre area.Our study showed that polluted air masses from the Marseilles–Berre area are advected to Plan d'Aups in the early afternoon. Average daily concentration of particles reaches up to 40 μg m−3 while 1-h average particle number concentration is greater than 30,000 cm−3. Most of the particle mass is composed of SO42− and organic carbon (OC). The chemical properties of the particles revealed that an additional source, possibly from the industrial area of Gardanne, contributes to the aerosol mass. This last source is characterised by significant emissions of elements, such as Zn, V, Al and Si.In addition to transport, we found that gas-to-particle conversion takes place at the interface between the free troposphere and the boundary layer. We estimated that on average, 30% of the particle number is accounted for by direct nucleation. This is potentially a major aerosol source to the free troposphere. 相似文献
42.
The Otranto–Leuca coastal tract is marked by the presence of numerous sea caves placed close to present sea level. They are located generally at the back of a shore platform covered by a sequence of breccia deposits, marine sediments and speleothems. At Grotta di Masseria dell'Orte, marine cemented sands rest on a narrow shore platform at about 6.2 m above mean sea level and are covered by speleothems older than 185 ka. At Grotta del Diavolo, which is mostly filled by breccia deposits, three beach levels have been detected at about 3.0, 3.5 and 5.9 m above msl. They are either covered by or overlie speleothems that yield an U/Th age of 340, 78 ka and between 170.3 and 146.5, respectively. Geomorphological evidence and radiometric ages indicate that the area after a period of uplift has been tectonically stable since the last part of the Middle Pleistocene so that marine landforms close to the present shoreline underwent a polycyclic evolution. The sedimentary fills of sea caves formed during Middle-Late Pleistocene glacial stages, when arid or semiarid conditions promoted the removal of regolith and the development of thick breccia deposits. During Marine Isotope Stages (MIS) 9.3, 5.5 and 5.1, cave sediments were partially eroded whereas beach layers and related speleothems developed. These are, in fact, the only marine isotope stages marked by a sea level position which in this Mediterranean region was either close to, or slightly higher than, the present one. 相似文献
43.
44.
Wolfram Wobrock Andrea I. Flossmann Marie Monier Jean-Marc Pichon Laurent Cortez Jean-Franois Fournol Alfons Schwarzenbck Stephan Mertes Jost Heintzenberg Paolo Laj Giordano Orsi Loretta Ricci Sandro Fuzzi Harry Ten Brink Piet Jongejan Ren Otjes 《Atmospheric Research》2001,58(4):7907
The second field campaign of the Cloud Ice Mountain Experiment (CIME) project took place in February 1998 on the mountain Puy de Dôme in the centre of France. The content of residual aerosol particles, of H2O2 and NH3 in cloud droplets was evaluated by evaporating the drops larger than 5 μm in a Counterflow Virtual Impactor (CVI) and by measuring the residual particle concentration and the released gas content. The same trace species were studied behind a round jet impactor for the complementary interstitial aerosol particles smaller than 5 μm diameter. In a second step of experiments, the ambient supercooled cloud was converted to a mixed phase cloud by seeding the cloud with ice particles by the gas release from pressurised gas bottles. A comparison between the physical and chemical characteristics of liquid drops and ice particles allows a study of the fate of the trace constituents during the presence of ice crystals in the cloud.In the present paper, an overview is given of the CIME 98 experiment and the instrumentation deployed. The meteorological situation during the experiment was analysed with the help of a cloud scale model. The microphysics processes and the behaviour of the scavenged aerosol particles before and during seeding are analysed with the detailed microphysical model ExMix. The simulation results agreed well with the observations and confirmed the assumption that the Bergeron–Findeisen process was dominating during seeding and was influencing the partitioning of aerosol particles between drops and ice crystals. The results of the CIME 98 experiment give an insight on microphysical changes, redistribution of aerosol particles and cloud chemistry during the Bergeron–Findeisen process when acting also in natural clouds. 相似文献
45.
Paolo Laj Andrea I. Flossmann Wolfram Wobrock Sandro Fuzzi Giordano Orsi Loretta Ricci Stephan Mertes Alfons Schwarzenbck Jost Heintzenberg Harry Ten Brink 《Atmospheric Research》2001,58(4):256
We investigated the partitioning of trace substances during the phase transition from supercooled to mixed-phase cloud induced by artificial seeding. Simultaneous determination of the concentrations of H2O2, NH3 and black carbon (BC) in both condensed and interstitial phases with high time resolution showed that the three species undergo different behaviour in the presence of a mixture of ice crystals and supercooled droplets. Both H2O2 and NH3 are efficiently scavenged by growing ice crystals, whereas BC stayed predominantly in the interstitial phase. In addition, the scavenging of H2O2 is driven by co-condensation with water vapour onto ice crystals while NH3 uptake into the ice phase is more efficient than co-condensation alone. The high solubility of NH4+ in the ice could explain this result. Finally, it appears that the H2O2–SO2 reaction is very slow in the ice phase with respect to the liquid phase. Our results are directly applicable for clouds undergoing limited riming. 相似文献
46.
A clinopyroxene geobarometer for basaltic systems based on crystal-structure modeling 总被引:9,自引:0,他引:9
Paolo Nimis 《Contributions to Mineralogy and Petrology》1995,121(2):115-125
The crystal chemical response of basalt clinopyroxene to increasing pressure was investigated by means of crystal-structure
simulation (a procedure that enables modeling of the structural parameters of a clinopyroxene of known chemistry without requiring
direct X-ray diffraction analysis) using available experimental chemical data. Pressure proved the main physical variable
governing clinopyroxene behavior in a magmatic environment. The general internal consistency of the simulation data permitted
construction of an empirical geobarometer based on the relationship of cell volume (Vc) vs M1-site volume (VM1). The straightforward
geobarometric formulation in the absence of direct X-ray analysis is:
P(kbar)=698.443+4.985⋅AlT−26.826⋅Fe2+
M1−3.764⋅Fe3+
+53.989⋅AlM1+3.948⋅Ti+14.651⋅Cr
−700.431⋅Ca−666.629⋅Na−682.848⋅MgM2−691.138⋅Fe2+
M2−688.384⋅Mn−6.267⋅(MgM2)2−4.144⋅(Fe2+
M2
where:
(Fe2+
M1⋅MgM2)/(Fe2+
M2⋅MgM1)=e**(0.238⋅R3++0.289⋅CNM−2.315), CNM=Ca+Na+Mn, and R3+=AlM1+Fe3++Ti+Cr,
with cations in atoms per formula unit. The geobarometer reproduces experimental pressures within ±2 kbar (=1σ; max. dev.
≤5 kbar; N=29) in the range 0–24 kbar and is applicable to near-liquidus C2/c clinopyroxenes crystallized from basaltic melts in the absence of garnet (excepting high-Al2O3 basalts). It is therefore suitable for many natural clinopyroxenes occurring as mega- or phenocrysts or forming well-preserved
cumulate pyroxenites. If the above restrictions are not wholly satisfied, the Vc vs VM1 plot can also be used qualitatively
to deduce the relative pressure conditions of clinopyroxenes forming from similar batches of magma. The structural simulation of experimental data
also provided insight into the influence of minor chemical changes of the parental magma on the crystal chemistry of clinopyroxene
at high pressure. Within the considered compositional space at given P-T, a
CaO and a
SiO2 in the melt have opposite effects on M2- and T-site cation populations. As a result, under similar physical conditions, clinopyroxenes
from higher-CaO or more undersaturated basalts have higher VM2, VT and Vc and lower VM1. For basalts with normal contents of Al2O3 (<18 wt %), variations of major elements in the melt do not reduce the accuracy of the geobarometer.
Received: 3 April 1994 / Accepted: 23 December 1995 相似文献
47.
The caldera of Pululagua is an eruptive centre of the Northern Volcanic Zone of the South American volcanic arc, located about 15 km north of Quito, Ecuador. Activity leading to formation of the caldera occurred about 2450 b.p. as a series of volcanic episodes during which an estimated 5–6 km3 (DRE) of hornblende-bearing dacitic magma was erupted. A basal pumice-fall deposit covers more than 2.2x104 km2 with a volume of about 1.1 km3 and represents the principal and best-preserved plinian layer. Circular patterns of isopachs and pumice, lithic and Md isopleths of the Basal Fallout (BF) around the caldera indicate emplacement in wind-free conditions. Absence of wind is confirmed by an ubiquitous, normally graded, thin ash bed at the top of the lapilli layer which originated from slow settling of fines after cessation of the plinian column (co-plinian ash). The unusual atmospheric conditions during deposition make the BF deposit particularly suitable for the application and evaluation of pyroclast dispersal models. Application of the Carey and Sparks' (1986) model shows that whereas the 3.2-, 1.6-, and 0.8-cm lithic isopleths predict a model column height of about 36 km, the 6.4-cm isopleth yields and estimate of only 21 km. The 4.9- and 6.4-cm isopleths yield a column height of 28 km using the model of Wilson and Walker (1987). The two models give the same mass discharge rate of 2x108 kg s-1. A simple exponential decrease of thickness with distance, as proposed by Pyle (1989) for plinian falls, fits well with the BF. Exponential decrease of size with distance is followed by clasts less than about 3 cm, suggesting, in agreement with Wilson and Walker (1987), that only a small proportion of large clasts reach the top of the column. Variations with distance in clast distribution patterns imply that, in order to obtain column heights by clast dispersal models, the distribution should be known from both proximal and distal zones. Knowledge of only a few isopleths, irrespective of their distance from the vent, is not sufficient as seemed justified by the method of Pyle (1989). 相似文献
48.
49.
Paolo Lanzano 《Astrophysics and Space Science》1973,20(1):71-83
A study has been conducted to ascertain conditions on the density distribution within a fluid, rotating planet in order that the deformation of its outer shell be expressible in terms of the Bessel functions of the first kind and the Gaussian hypergeometric series.It has been established that (1) the density must be a solution to an ordinary differential equation of the Riccati type, and (2) two already considered density distributions are the only closed-form solutions of physical relevance. 相似文献
50.
Paolo Gallitelli 《Mineralogy and Petrology》1954,4(1-4):283-287
Riassunto Viene descritta una penninite di Boccassuolo nell'Appennino modenese, e attraverso lo studio ottico, chimico, roentgenografico e termico differenziale ne vengono definite le proprietà caratteristiche. L'esame della curva termico differenziale e degli spettrogrammi Debye ottenuti da polvere di penninite scaldata fra 900° e 950° permette di stabilire che la trasformazione penninite-enstatite inizia già nell'ambito di temperatura compreso fra 910° e 940°.Con 1 figura. 相似文献