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51.
52.
The partitioning of stable carbon isotopes between calcite, graphite and CO2 was experimentally determined at temperatures from 500 to 1200 °C and 1 to 15 kbar pressure. Attainment of carbon isotope equilibrium in CO2-calcite runs was proven by achieving the same fractionation from isotopically opposite directions. The resultant CO2-calcite fractionation curve for carbon differs from Bottinga's calculation by 1.2 and confirms recent experiments of Chacko et al. and Mattey et al. In CO2-graphite experiments equilibrium fractions were extrapolated by applying the partial-exchange technique of Northrop and Clayton and by optimizing the contribution of surface reaction in graphite. CO2-graphite fractionations at temperatures up to 800 °C are in fair agreement with Bottinga's calculation, but yield a surprisingly high fractionation of 5 at upper mantle temperatures. The combination of CO2-calcite (carbon) and CO2-graphite fractionation results in a new experimentally determined calcite-grapite fractionation curve, expressed by the equation:
相似文献
53.
Alexander Scholz Jochen Eislöffel 《Monthly notices of the Royal Astronomical Society》2007,381(4):1638-1646
The cluster Praesepe (age ∼650 Myr) is an ideal laboratory to study stellar evolution. Specifically, it allows us to trace the long-term decline of rotation and activity on the main sequence. Here, we present rotation periods measured for five stars in Praesepe with masses of 0.1–0.5 M
54.
Facies architecture and sedimentology of a meandering fluvial system: a Palaeogene example from the Weisselster Basin, Germany 总被引:1,自引:0,他引:1
The Schleenhain open pit coal mine, located 30 km south of Leipzig, Germany, exposes Upper Eocene and Oligocene non-marine strata representing fluvial deposition in the centre of the Weisselster Basin. Active mining and successive cuts provided the rare opportunity to obtain a three-dimensional perspective of laterally extensive surface outcrops. These were used to construct a detailed fence diagram, which provided the basis for recognition of key architectural elements in the weakly consolidated meandering stream deposits. In addition to the eight basic architectural elements of Miall (1985 ), the element SL (shallow lake deposits) was newly defined and the element CH (channel) was subdivided into CHg (palaeo-river system) and CHk (small channel). The profiles contain parts of two fining-upward cycles, which are separated by an unconformity spanning the Early Oligocene. Deposits of the first cycle begin with transverse sand bars (downstream accretion deposits-DA) and point bars (lateral accretion deposits-LA). The upper part of the cycle is represented by overbank fines (OF) and the element SL, which consists of laterally discontinuous lenses of dark, plant-bearing, kaolinite-rich clays, that were deposited in shallow lakes adjacent to the active channel. Coal seams interlayered with palaeosols are the main constituents of element OF. Sheetlike bodies of medium to fine gravels (gravel bars and bedforms-GB) on an erosive coal surface mark the beginning of the second cycle. Dissolution of underlying Permian salts and sulphates prior to, during, and after the deposition of the Palaeogene strata caused the development of two synclines within the outcrop. Coal seams and clay horizons which thicken and dip towards the centre of the synclines, provide evidence for their chronological development. 相似文献
55.
Elizabeth Mcleod Benjamin Poulter Jochen Hinkel Enrique Reyes Rodney Salm 《Ocean & Coastal Management》2010,53(9):507-517
Conservation managers and policy makers need tools to identify coastal habitats and human communities that are vulnerable to sea-level rise. Coastal impact models can help determine the vulnerability of areas and populations to changes in sea level. Model outputs may be used to guide decisions about the location and design of future protected areas and development, and to prioritize adaptation of existing protected area investments. This paper reviews state-of-the-art coastal impact models that determine sea-level rise vulnerability and provides guidance to help managers and policy makers determine the appropriateness of various models at local, regional, and global scales. There are a variety of models, each with strengths and weaknesses, that are suited for different management objectives. We find important trade-offs exist regarding the cost and capacity needed to run and interpret the models, the range of impacts they cover, and regarding the spatial scale that each operates which may overstate impacts at one end and underestimate impacts at the other. Understanding these differences is critical for managers and policy makers to make informed decisions about which model to use and how to interpret and apply the results. 相似文献
56.
57.
Integrating knowledge to assess coastal vulnerability to sea-level rise: The development of the DIVA tool 总被引:3,自引:0,他引:3
This paper describes the development of the DIVA tool, a user-friendly tool for assessing coastal vulnerability from subnational to global levels. The development involved the two major challenges of integrating knowledge in the form of data, scenarios and models from various natural, social and engineering science disciplines and making this integrated knowledge accessible to a broad community of end-users. These challenges were addressed by (i) creating and applying the DIVA method, an iterative, modular method for developing integrating models amongst distributed partners and (ii) making the data, scenarios and integrated model, equipped with a powerful graphical user interface, directly and freely available to end-users. 相似文献
58.
Sandeep Kar Jyoti Prakash Maity Jiin-Shuh Jean Chia-Chuan Liu Bibhash Nath Huai-Jen Yang Jochen Bundschuh 《Applied Geochemistry》2010,25(12):1805-1814
Hydrogeochemical characteristics and elemental features of groundwater and core sediments have been studied to better understand the sources and mobilization process responsible for As-enrichment in part of the Gangetic plain (Barasat, West Bengal, India). Analysis of water samples from shallow tubewells (depth 24.3–48.5 m) and piezometer wells (depth 12.2–79.2 m) demonstrate that the groundwater is mostly the Ca-HCO3 type and anoxic in nature (mean EhSHE = 34 mV). Arsenic concentrations ranged from <10–538 μg/L, with high concentrations only present in the shallow to medium depth (30–50 m) of the aquifer along with high Fe (0.07–9.8 mg/L) and relatively low Mn (0.15–3.38 mg/L) as also evidenced in core sediments. Most groundwater samples contained both As(III) and As(V) species in which the concentration of As(III) was generally higher than that of As(V), exhibiting the reducing condition. Results show lower concentrations of NO3, SO4 and NO2 along with higher values of DOC and HCO3, indicating the reducing nature of the aquifer with abundant organic matter that can promote the release of As from sediments into groundwater. Positive correlations of As with Fe and DOC were also observed. The presence of DOC may actively drive the redox processes. This study revealed that reduction processes of FeOOH was the dominant mechanism for the release of As into the groundwater in this part of the Ganges Delta plain. 相似文献
59.
Dominic Papineau Bradley T. De Gregorio Marc D. Fries Stephen J. Mojzsis Rhonda M. Stroud 《Geochimica et cosmochimica acta》2010,74(20):5862-5883
Because all known Eoarchean (>3.65 Ga) volcano-sedimentary terranes are locked in granitoid gneiss complexes that have experienced high degrees of metamorphism and deformation, the origin and mode of preservation of carbonaceous material in the oldest metasedimentary rocks remain a subject of vigorous debate. To determine the biogenicity of carbon in graphite in such rocks, carbonaceous material must be demonstrably indigenous and its composition should be consistent with thermally altered biogenic carbon as well as inconsistent with abiogenic carbon. Here we report the petrological and spectroscopic characteristics of carbonaceous material, typically associated with individual apatite grains, but also with various other minerals including calcite, in a >3.83 Ga granulite-facies ferruginous quartz-pyroxene unit (Qp rock) from the island of Akilia in southern West Greenland. In thin sections of the fine-grained parts of Akilia Qp rock sample G91-26, mapped apatites were found to be associated with graphite in about 20% of the occurrences. Raman spectra of this carbonaceous material had strong G-band and small D-band absorptions indicative of crystalline graphite. Three apatite-associated graphites were found to contain curled graphite structures, identified by an anomalously intense second-order D-band (or 2D-band) Raman mode. These structures are similar to graphite whiskers or cones documented to form at high temperatures. Raman spectra of apatite-associated graphite were consistent with formation at temperatures calculated to be between 635 and 830 °C, which are consistent with granulite-facies metamorphic conditions. Three graphite targets extracted by focused ion beam (FIB) methods contained thin graphite coatings on apatite grains rather than inclusions sensu stricto as inferred from transmitted light microscopy and Raman spectroscopy. TEM analyses of graphite in these FIB sections showed a (0 0 0 2) interplanar spacing between 3.41 and 3.64 Å for apatite-associated graphite, which is larger than the spacing of pure graphite (3.35 Å) and may be caused by the presence of non-carbon heteroatoms in interlayer sites. Samples analyzed by synchrotron-based scanning transmission X-ray microscopy (STXM) also confirmed the presence of crystalline graphite, but abundances of N and O heteroatoms were below detection limit for this method. Graphite in the Akilia Qp rock was also found to occur in complex polyphase mineral assemblages of hornblende ± calcite ± sulfides ± magnetite that point to high-temperature precipitation from carbon-bearing fluids. These complex mineral assemblages may represent another generation of graphitization that could have occurred during the amphibolite-facies metamorphic event at 2.7 Ga. Several observations point to graphitization from high-temperature fluid-deposition for some of the Akilia graphite and our results do not exclude a biogenic source of carbon in graphite associated with apatite, but ambiguities remain for the origin of this carbon. 相似文献
60.
A. Steele M. D. Fries H. E. F. Amundsen B. O. Mysen M. L. Fogel M. Schweizer N. Z. Boctor 《Meteoritics & planetary science》2007,42(9):1549-1566
Abstract— We report a comprehensive imaging study including confocal microRaman spectroscopy, scanning electron microscopy (SEM), and 3‐D extended focal imaging light microscopy of carbonate globules throughout a depth profile of the Martian meteorite Allan Hills (ALH) 84001 and similar objects in mantle peridotite xenoliths from the Bockfjorden volcanic complex (BVC), Svalbard. Carbonate and iron oxide zoning in ALH 84001 is similar to that seen in BVC globules. Hematite appears to be present in all ALH 84001 carbonate‐bearing assemblages except within a magnesite outer rim found in some globules. Macromolecular carbon (MMC) was found in intimate association with magnetite in both ALH 84001 and BVC carbonates. The MMC synthesis mechanism appears similar to established reactions within the Fe‐C‐O system. By inference to a terrestrial analogue of mantle origin (BVC), these results appear to represent the first measurements of the products of an abiotic MMC synthesis mechanism in Martian samples. Furthermore, the ubiquitous but heterogeneous distribution of hematite throughout carbonate globules in ALH 84001 may be partly responsible for some of the wide range in measured oxygen isotopes reported in previous studies. Using BVC carbonates as a suitable analogue, we postulate that a low temperature hydrothermal model of ALH 84001 globule formation is most likely, although alteration (decarbonation) of a subset of globules possibly occurred during a later impact event. 相似文献
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