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81.
82.
Polyfluorinated compounds in waste water treatment plant effluents and surface waters along the River Elbe, Germany 总被引:4,自引:0,他引:4
Lutz Ahrens Sebastian Felizeter Renate Sturm Zhiyong Xie Ralf Ebinghaus 《Marine pollution bulletin》2009,58(9):1326-1333
Polyfluorinated compounds (PFCs) were investigated in waste water treatment plant (WWTP) effluents and surface waters of the River Elbe from samples collected in 2007. Concentrations of various PFCs, including C4–C8 perfluorinated sulfonates (PFSAs), C6 and C8 perfluorinated sulfinates, 6:2 fluorotelomer sulfonate, C5–C13 perfluorinated carboxylic acids (PFCAs), C4 and C8 perfluoroalkyl sulfonamides and 6:2, 8:2 and 10:2 unsaturated fluorotelomercarboxylic acids were quantified. ∑PFC concentrations of the river water ranged from 7.6 to 26.4 ng L−1, whereas ∑PFC concentrations of WWTP effluents were approximately 5–10 times higher (30.5–266.3 ng L−1), indicating that WWTPs are potential sources of PFCs in the marine environment. PFC patterns of different WWTP effluents varied depending on the origin of the waste water, whereas the profile of PFC composition in the river water was relatively constant. In both kinds of water samples, perfluorooctanoic acid (PFOA) was the major PFC, whereas perfluorobutane sulfonate (PFBS) was the predominant PFSA. 相似文献
83.
The interannual variability of East Asian Winter Monsoon and its relation to the summer monsoon 总被引:76,自引:1,他引:75
1.IntroductionOvertheEastAsiaregion,themostprominentsurfacefeatureofthewintermonsoonisstrongnortheasterliesalongtheeastflankoftheSiberianhighandthecoastofEastAsia.At500hPathereisabroadtroughcenteredaboutatthelongitudesofJapan.Thedominantfea-tureat2O0hPaistheEastAsianjetwithitsmaximumlocatedatjustsoutheastofJapan.Thisktisassociatedwithintensebaroclinicity,largeverticalwindshearandstrongadvectionofcoldair(StaffmembersofAcademiaSinica,l957,LauandChang,1987;BoyleandChen,1987;Chenetal.,1991… 相似文献
84.
Secular Variability of the Coupled Tropospheric and Stratospheric Circulation in the GCM ECHAM 3/LSG
Summary Secular or multi-decadal variability is a widely observed phenomenon, apparent in instrumental and paleo climatic records.
These long time oscillations are found in many variables of the climate system. The ocean especially experiences low frequency
variations. But also atmospheric variables such as temperature, wind velocity and sea level pressure can show secular variability.
The low frequency variability here is examined in the coupled atmosphere-ocean model ECHAM3/LSG T21. A coupled stratospheric
and tropospheric mode is detected oscillating with a period of approximately 100 years. The atmospheric pressure system mainly
involved in this oscillation is the northern hemispheric winter stratospheric polar vortex. The near surface temperature experiences
variations of the same magnitude as the observed temperature trends of the last decades. Multi decadal variability is also
shown in the North Atlantic Oscillation Index.
A shift of the length of the oscillation period between longer and shorter time scales indicates that chaotic processes might
be responsible for the variability.
Received February 22, 1999/Revised August 5, 1999 相似文献
85.
利用遥感技术对大气环境污染进行监测时,云是影响痕量气体反演精度的重要因素,因此在痕量气体反演中需要对云的影响进行校正,通常使用的云参数主要是有效云量和云压。本文基于O2-O2 477 nm吸收波段构建了O2-O2云反演算法:首先,根据有效云量和云高与连续反射率和O2-O2斜柱浓度之间的对应关系,结合假定的云模型利用VLIDORT辐射传输模型建立关于有效云量和云压的查找表;然后,通过差分吸收光谱技术拟合卫星载荷观测的大气层顶辐射,获得O2-O2斜柱浓度并计算连续反射率;最后,结合辅助数据,根据查找表进行插值反演获得有效云量和云压。通过将算法应用到OMI观测数据,将反演结果与OMCLDO2产品进行对比验证,有效云量和云压空间分布一致,相关系数R均超过0.97;并还将该算法应用于下一代大气成分监测仪器TROPOMI,与FRESCO+产品对比,有效云量和云压空间分布基本一致,当地表类型为海洋时,有效云量相关系数R大于0.97,云压相关系数R大于0.94,云压反演结果存在一定的区别;通过将O2-O2云反演算法和FRESCO+云压反演结果与CALIOP Cloud Layer产品进行对比,结果表明,在低云情况下,O2-O2云反演算法线性回归方程斜率为0.782,截距为198.0 hPa,相关系数R为0.850,算法表现优于FRESCO+。而在高云情况下,FRESCO+反演结果更接近CALIOP云压结果。在OMI和TROPOMI上的应用表明O2-O2云反演算法在大气云反演中具有较高的准确性和可行性,可以为大气痕量气体反演的校正提供云参数,并为中国同类型卫星载荷的云反演算法提供算法参考。 相似文献
86.
Emanuele Perinati Marco Barbera Sebastian Diebold Alejandro Guzman Andrea Santangelo Chris Tenzer 《Experimental Astronomy》2017,44(3):387-399
We present a preliminary assessment of the non-X-ray background for the WFI on board ATHENA conducted at IAAT in the context of the collaborative background and radiation damage working group activities. Our main result is that in the baseline configuration originally assumed for the camera the requirement on the level of non-X-ray background could not be met. In light of the results of Geant4 simulations we propose and discuss a possible optimization of the camera design and pinpoint some open issues to be addressed in the next phase of investigation. One of these concerns the possible contribution to the non-X-ray background from soft protons and ions funneled to the focal plane through the optics. This is not quantified at this stage, here we just briefly report on our ongoing activities aimed at validating the mechanisms of proton scattering at grazing incidence. 相似文献
87.
88.
Chan-Hee Park Christof Beyer Sebastian Bauer Olaf Kolditz 《Environmental Geology》2008,55(8):1755-1766
Precise and efficient numerical simulation of transport processes in subsurface systems is a prerequisite for many site investigation
or remediation studies. Random walk particle tracking (RWPT) methods have been introduced in the past to overcome numerical
difficulties when simulating propagation processes in porous media such as advection-dominated mass transport. Crucial for
the precision of RWPT methods is the accuracy of the numerically calculated ground water velocity field. In this paper, a
global node-based method for velocity calculation is used, which was originally proposed by Yeh (Water Resour Res 7:1216–1225,
1981). This method is improved in three ways: (1) extension to unstructured grids, (2) significant enhancement of computational
efficiency, and (3) extension to saturated (groundwater) as well as unsaturated systems (soil water). The novel RWPT method
is tested with numerical benchmark examples from the literature and used in two field scale applications of contaminant transport
in saturated and unsaturated ground water. To evaluate advective transport of the model, the accuracy of the velocity field
is demonstrated by comparing several published results of particle pathlines or streamlines. Given the chosen test problem,
the global node-based velocity estimation is found to be as accurate as the CK method (Cordes and Kinzelbach in Water Resour
Res 28(11):2903–2911, 1992) but less accurate than the mixed or mixed-hybrid finite element methods for flow in highly heterogeneous media. To evaluate
advective–diffusive transport, a transport problem studied by Hassan and Mohamed (J Hydrol 275(3–4):242–260, 2003) is investigated here and evaluated using different numbers of particles. The results indicate that the number of particles
required for the given problem is decreased using the proposed method by about two orders of magnitude without losing accuracy
of the concentration contours as compared to the published numbers. 相似文献
89.
Bartosz Czernecki Marek Półrolniczak Leszek Kolendowicz Michał Marosz Sebastian Kendzierski Natalia Pilguj 《Journal of Atmospheric Chemistry》2017,74(1):115-139
This study investigates atmospheric conditions’ influence on the mean and extreme characteristics of PM10 concentrations in Poznań during the period 2006–2013. A correlation analysis was carried out to identify the most important meteorological variables influencing the seasonal dynamics of PM10 concentrations. The highest absolute correlation values were obtained for planetary boundary layer height (r = ?0.57), thermal (daily minimum air temperature: r = ?0.51), anemological (average daily wind speed: r = ?0.37), and pluvial (precipitation occurrence: r = ?0.36) conditions, however the highest correlations were observed for temporal autocorrelations (1 day lag: r = 0.70). As regulated by law, extreme events were identified on the basis of daily threshold value i.e. 50 μg m?3. On average, annually there are approximately 71.3 days anywhere in the city when the threshold value is exceeded, 46.6 % of those occur in winter. Additionally, 83.7 % of these cases have been found to be continuous episodes of a few days, with the longest one persisting for 22 days. The analysis of the macro-scale circulation patterns led to the identification of an easy-to-perceive seasonal relations between atmospheric fields that favour the occurrence of high PM10 concentration, as well as synoptic situations contributing to the rapid air quality improvement. The highest PM10 concentrations are a clear reaction to a decrease in air temperature by over 3 °C, with simultaneous lowering of PBL height, mean wind speed (by around 1 m s?1) and changing dominant wind directions from western to eastern sectors. In most cases, such a situation is related to the expansion of a high pressure system over eastern Europe and weakening of the Icelandic Low. Usually, air quality conditions improve along with an intensification of westerlies associated with the occurrence of low pressure systems over western and central Europe. Opposite relations are distinguishable in summer, when air quality deterioration is related to the inflow of tropical air masses originating over the Sahara desert. 相似文献
90.
Hans-F Graf 《Climate Dynamics》1992,7(1):19-28
One of the generally accepted climatic effects of stratospheric aerosol injection is the reduction of the global radiation in high latitudes by an order of 5% during El Chichon type eruptions. To test the effect of a high-latitude radiation deficit on global climate, a GCM experiment was performed with the ECMWF T21 atmosphere general circulation model (AGCM). The results provide physically-consistent evidence that this radiation deficit is a possible external forcing factor for severe climatic anomalies not only in the area directly affected by the reduced radiation, but also in the tropics. The most important factor is the creation of enhanced snow cover in regions of Asia that are distant from the location of the introduced radiation anomaly. The simulated results show certain features that are well known from observations in weak monsoon years, i.e. the weakened easterly jet in the upper troposphere over northern India, prolonged winter monsoon conditions, and prevailing anticyclonic vorticity anomalies over the entire Indian summer monsoon region. Over the western Pacific at the end of boreal winter (May), increased convective activity leads to a negative Walker circulation anomaly with westerly wind anomalies near the surface and easterly anomalies in the upper troposphere. This is known as one of the most important anomalies at the beginning of an El Niño/Southern Oscillation (ENSO) event.This paper was presented at the International Conference on Modelling of Global Climate Change and Variability, held in Hamburg 11–15 September 1989 under the auspices of the Meteorological Institute of the University of Hamburg and the Max Planck Institute for Meteorology. Guest Editor for these papers is Dr. L. Dümenil 相似文献