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91.
The morphology of materials on the floor of Gusev Crater (14° S, 175° W), Mars, imply a history of volcanism and subsequent removal of an ice-rich deposit. Fluid lava flows observed in the western portion of Gusev Crater paradoxically terminate in a steep, thick (<60 m) flow front adjacent to hummocky terrain. The hummocky terrain is morphologically similar to deglaciated terrain on Earth, generated when glacial debris are left behind after the glacier has retreated. We propose the following scenario for the floor of Gusev Crater. First, ice-rich material was deposited adjacent to Thira Crater. Second, fluid lavas were emplaced and ponded against the ice-rich deposits. At some later time, the ice within the deposit sublimated, leaving hummocky terrain. Current age estimates for the Gusev flows are Hesperian, suggesting that the ice removal occurred in the upper Hesperian or more recently. If this hypothesis is correct, quench features (glassy rinds, columnar jointing) should be observed at the lava flow margin; the hummocky deposit should be poorly sorted, angular debris.  相似文献   
92.
Abstract— Organic compounds in the Murchison (C2M) and Allende (CV3) carbonaceous chondrites were analyzed by photoionization time-of-flight mass spectrometry; thermal (25–850 °C) and stimulated (7 keV Ar+) desorption were combined with either nonresonant single-photon ionization using 118 nm light or resonantly enhanced multiphoton ionization (selective for aromatic compounds) using 266 nm light. Samples weighing only 1–10 mg were sufficient for sensitive quantitative analysis of aromatic compounds using thermal desorption. The detection limits for phenanthrene and pyrene using 118 nm light were determined to be 0.8 and 1.4 picomoles, respectively, and the concentrations of these compounds (including their isomers anthracene and fluoranthene) in the Murchison meteorite were determined to be 9 and 12 μg/g, respectively, in good agreement with previously published values. Thermal-desorption (–75–500 °C) field-ionization mass spectra (activated foil-type ionizing source and magnetic sector mass analyzer) of 20–40 mg of the same meteorite material were obtained to verify that the 118 nm photoionization mass spectra were not affected by photofragmentation or photodecomposition and were representative of the organic material extracted by thermal desorption. Photoionization mass spectrometry is a useful technique for studying small quantities (< 1 nanomole) of organic matter in terrestrial and extraterrestrial samples. The present study aims to provide the background and analytical methods necessary for application to new and unsolved cosmochemical problems. Some potential applications are discussed.  相似文献   
93.
Summary ?Orangeite occurring as a complex series of dikes at Swartruggens (South Africa), is host to a diversity of accessory minerals, the most common of which are apatite, barite and calcite. Less common, but important phases are perovskite, wadeite, an unidentified Ca–Ti–Fe-silicate, strontianite, unidentified Ca-REE phosphate, zircon, rutile, titaniferous magnetite, quartz and diverse sulphides. The accessory minerals show wide variations in their mode in different segments of the dike suite as a consequence of crystal sorting during flow differentiation. Compositional data are given for apatite, barite, calcite, perovskite, wadeite and the unidentified Ca–Ti–Fe-silicate. The accessory mineral suite is similar to that found in lamproites but is sufficiently distinct in composition and paragenesis to preclude inclusion with that clan. Differences include the common presence of groundmass calcite, barite and serpentine in the orangeite and the absence of typomorphic minerals (leucite, sanidine, richterite) of the lamproite clan. Received January 15, 2001; revised version accepted October 15, 2001  相似文献   
94.
Marsh soil properties vary drastically across estuarine salinity gradients, which can affect soil strength and, consequently, marsh edge erodibility. Here, we quantify how marsh erosion differs between saline and brackish marshes of the Mississippi Delta. We analyzed long-term (1932–2015) maps of marsh loss and developed an algorithm to distinguish edge erosion from interior loss. We found that the edge erosion rate remains nearly constant at decadal timescales, whereas interior loss varies by more than 100%. On average, roughly half of marsh loss can be attributed to edge erosion, the other half to interior loss. Based on data from 42 cores, brackish marsh soils had a lower bulk density (0.17 vs. 0.27 g/cm3), a higher organic content (43% vs. 26%), a lower shear strength (2.0 vs. 2.5 kPa), and a lower shear strength in the root layer (13.8 vs. 20.7 kPa) than saline marsh soils. We then modified an existing marsh edge erosion model by including a salinity-dependent erodibility. By calibrating the erodibility with the observed retreat rates, we found that the brackish marsh is two to three times more erodible than the saline marshes. Overall, this model advances the ability to simulate estuarine systems as a whole, thus transcending the salinity boundaries often used in compartmentalized marsh models.  相似文献   
95.
We investigated exterior and interior subsamples from the Martian shergottite meteorites Allan Hills (ALH) A77005 and Roberts Massif (RBT) 04261 for secondary minerals, oxygen isotopes, Ar‐Ar, and noble gas signatures. Electron microprobe investigations revealed that RBT 04261 does not contain any visible alteration even in its most exterior fractures, whereas fracture fillings in ALHA77005 penetrate into the meteorite up to 300 μm, beyond which the fractures are devoid of secondary minerals. Light noble gases seem to be almost unaffected by terrestrially induced alteration in both meteorites. Thus, a shock metamorphic overprint of 30–35 GPa can be deduced from the helium measurements in RBT 04261. Oxygen isotopes also seem unaffected by terrestrially weathering and variations can easily be reconciled with the differences in modal mineralogy of the exterior and interior subsamples. The measurements on irradiated samples (Ar‐Ar) showed a clear Martian atmospheric contribution in ALHA77005, but this is less apparent in our sample of RBT 04261. Exterior and interior subsamples show slight differences in apparent ages, but the overall results are very similar between the two. In contrast, krypton and xenon are severely affected by terrestrial contamination, demonstrating the ubiquitous presence of elementally fractionated air in RBT 04261. Although seemingly contradictory, our results indicate that RBT 04261 was more affected by contamination than ALHA77005. We conclude that irrespective of on which planet the alteration occurred, exposure of Martian rocks to atmosphere (or brine) introduces noble gases with signatures elementally fractionated relative to the respective atmospheric composition into the rock, and relationships of that process with oxygen isotopes or mineralogical observations are not straightforward.  相似文献   
96.
Because of the importance of snow for river discharge in mountain regions, hydrological research often focuses on seasonally snow-covered zones. However, in many basins the majority of the land surface area is intermittently snow-covered. Discharge monitoring in these areas is less common, so their contributions to downstream rivers remain largely unknown. We evaluated hydrological differences between three intermittently snow-covered (mean annual Jan 1–Jul 3 snow persistence <60%) and two seasonally snow-covered headwater catchments in the Colorado Front Range. We compared water balance variables to evaluate how and why discharge differs between the snow zones and estimated the relative contributions from each snow zone to regional river discharge. We focused on water years 2016–2019 and used a combination of in situ sensors and regional climate datasets. Annual discharge from the intermittent snow zone was low for all three catchments (10–77 mm), despite covering a wide range in annual snow persistence (25%–64%), whereas annual discharge from the seasonal snow zone was up to 73 times higher. Soil moisture in the seasonal snow zone was above field capacity for longer periods of time than in the intermittent snow zone, and the intermittent snow zone was uniquely subject to soil freezing (up to 102 days per year). For most of the year, potential evapotranspiration exceeded rainfall and snowmelt inputs in the intermittent snow zone, but was lower than rainfall and snowmelt inputs in the seasonal snow zone. This is likely a primary driver of the differences in soil moisture and discharge for catchments with a seasonal versus intermittent snow cover. Despite the large difference in discharge between these two snow zones, the intermittent snow zone contributed about a quarter of the discharge in the regional river, highlighting the importance of studying discharge generation across all elevations.  相似文献   
97.
98.
Uranium series dating has been carried out on secondary uranyl silicate minerals formed during sub-glacial and post-glacial weathering of Proterozoic uraninite ores in south west Finland. The samples were obtained from two sites adjacent to the Salpauselkä III ice marginal formation and cover a range of depths, from the surface to more than 60 m. Measured ages fall into three distinct groups, 70–100 ka, 28–36 ka and < 2500 yr. The youngest set is associated with surface exposures and the crystals display clear evidence of re-working. The most likely trigger for uranium release at depths below the surface weathering zone is intrusion of oxidising glacial melt water. The latter is often characterised by very high discharge rates along channels, which close once the overpressure generated at the ice margin is released. There is excellent correspondence between the two Finnish sites and published data for similar deposits over a large area of southern and central Sweden. None of the seventy samples analysed gave a U–Th age between 40 and 70 ka; a second hiatus is apparent at 20 ka, coinciding with the Last Glacial Maximum. Thus, the process responsible for uranyl silicate formation was halted for significant periods, owing to a change in geochemical conditions or the hydrogeological regime. These data support the presence of interstadial conditions during the Early and Middle Weichselian since in the absence of major climatic perturbations the uranium phases at depth are stable. When viewed in conjunction with proxy data from mammoth remains it would appear that the region was ice-free prior to the Last Glacial Maximum.  相似文献   
99.
We compare the daily, interannual, and decadal variability and trends in the thermal structure of the Arctic troposphere using eight observation-based, vertically resolved data sets, four of which have data prior to 1948. Comparisons on the daily scale between historical reanalysis data and historical upper-air observations were performed for Svalbard for the cold winters 1911/1912 and 1988/1989, the warm winters 1944/1945 and 2005/2006, and the International Geophysical Year 1957/1958. Excellent agreement is found at mid-tropospheric levels. Near the ground and at the tropopause level, however, systematic differences are identified. On the interannual time scale, the correlations between all data sets are high, but there are systematic biases in terms of absolute values as well as discrepancies in the magnitude of the variability. The causes of these differences are discussed. While none of the data sets individually may be suitable for trend analysis, consistent features can be identified from analyzing all data sets together. To illustrate this, we examine trends and 20-year averages for those regions and seasons that exhibit large sea-ice changes and have enough data for comparison. In the summertime Pacific Arctic and the autumn eastern Canadian Arctic, the lower tropospheric temperature anomalies for the recent two decades are higher than in any previous 20-year period. In contrast, mid-tropospheric temperatures of the European Arctic in the wintertime of the 1920s and 1930s may have reached values as high as those of the late 20th and early 21st centuries.  相似文献   
100.
Co sorption was measured as a function of pH, ionic strength (0.001-0.1 M NaNO3) and sorbate/sorbent ratio on pure quartz, HFO and kaolinite and on binary and ternary mixtures of the three solids. Sorption data measured for the pure solids were used to derive internally-consistent diffuse layer surface complexation model (DLM) stability constants for Co sorption. Co sorption on HFO could be adequately modeled over a broad range of ionic strengths and sorbate/sorbent ratios with a two variable-charge site model. Fits based on a single variable-charge site model were reasonable, but were improved by using ionic-strength dependent stability constants. A single variable-charge site model with an additional permanent ion exchange site produced the best fit to Co edges measured on kaolinite over a range of ionic strength and sorbate/sorbent ratios. These DLM fits were also improved by using ionic-strength dependent stability constants. The DLM approach could not adequately describe the slope of Co sorption edges on quartz. This study demonstrates that for accurate prediction of Co sorption over wide ranges of ionic strength and sorbate/sorbent ratio, the DLM may require ionic-strength dependent stability constants. DLM stability constants for Co sorption derived for the pure solids were used to predict sorption as a function of pH and solid concentration on binary and ternary mixtures of the three solids. Discrepancies between predictions and measurements were quantitatively similar to those observed for the pure mineral systems. Thus, a simple component additivity approach provides useful predictions of metal sorption in the mixed solid systems.  相似文献   
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