Spectral surface albedo over Morocco and its impact on radiative forcing of Saharan dust     

By EIKE BIERWIRTH  MANFRED WENDISCH  RÉ EHRLICH  BIRGIT HEESE  MATTHIAS TESCHE  DIETRICH ALTHAUSEN  ALEXANDER SCHLADITZ  DETLEF MÜLLER  SEBASTIAN OTTO  THOMAS TRAUTMANN  TILMAN DINTER  WOLFGANG von HOYNINGEN-HUENE  RALPH KAHN ‡ 《Tellus. Series B, Chemical and physical meteorology》2009,61(1):252-269

In May–June 2006, airborne and ground-based solar (0.3–2.2 μm) and thermal infrared (4–42 μm) radiation measurements have been performed in Morocco within the Saharan Mineral Dust Experiment (SAMUM). Upwelling and downwelling solar irradiances have been measured using the Spectral Modular Airborne Radiation Measurement System (SMART)-Albedometer. With these data, the areal spectral surface albedo for typical surface types in southeastern Morocco was derived from airborne measurements for the first time. The results are compared to the surface albedo retrieved from collocated satellite measurements, and partly considerable deviations are observed. Using measured surface and atmospheric properties, the spectral and broad-band dust radiative forcing at top-of-atmosphere (TOA) and at the surface has been estimated. The impact of the surface albedo on the solar radiative forcing of Saharan dust is quantified. In the SAMUM case of 19 May 2006, TOA solar radiative forcing varies by 12 W m⁻² per 0.1 surface-albedo change. For the thermal infrared component, values of up to +22 W m⁻² were derived. The net (solar plus thermal infrared) TOA radiative forcing varies between −19 and +24 W m⁻² for a broad-band solar surface albedo of 0.0 and 0.32, respectively. Over the bright surface of southeastern Morocco, the Saharan dust always has a net warming effect.  相似文献   

Evaluation of long-range transport and deposition of desert dust with the CTM MOCAGE     

By M. MARTET  V.-H. PEUCH  B. LAURENT  B. MARTICORENA  G. BERGAMETTI 《Tellus. Series B, Chemical and physical meteorology》2009,61(2):449-463

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A model for large glacial–interglacial climate-induced changes in dust and sea salt concentrations in deep ice cores (central Antarctica): palaeoclimatic implications and prospects for refining ice core chronologies     

By J. R. PETIT  B. DELMONTE 《Tellus. Series B, Chemical and physical meteorology》2009,61(5):768-790

A semi-empirical model has been developed to reproduce glacial–interglacial changes of continental dust and marine sodium concentrations (factor of ∼50 and ∼5, respectively) observed in inland Antarctic ice cores. The model uses conceptual pathways of aerosols within the high troposphere; assumes the dry deposition of impurities on the Antarctic surface; uses estimates of aerosol transit times taken independent of climate; assumes a temperature-dependent removal process during aerosol pathways from the mid-latitudes. The model is fitted to the data over the last four climate cycles from Vostok and EPICA Dome C Antarctic sites. As temperature is cooling, the aerosol response suggests different modes of climate couplings between latitudes, which can be continuous or below temperature thresholds for sodium and dust, respectively. The model estimates a southern South America dust source activity two to three times higher for glacial periods than for the Holocene and a glacial temperature over the Southern Ocean 3–5 °C cooler. Both estimates appear consistent with independent observations. After removal of temperature effects, dust and sodium residuals for both sites show orbital frequencies in opposite phase at the precession timescale. Such long-term insolation-related modulation of terrestrial and marine aerosol input, could provide a chemical pacemaker useful for refining ice core chronologies.  相似文献   

An efficient retrospective optimal interpolation algorithm compared with the fixed-lag Kalman smoother by assuming a perfect model     

By HYO-JONG SONG  GYU-HO LIM 《地球，A辑:动力气象学与海洋学》2009,61(5):610-620

We developed an efficient retrospective optimal interpolation (ROI) algorithm by which we can avoid the overlap of model integration periods, which appears in the procedure of evolving a previous analysis error covariance. If the fixed-lag Kalman smoother (FLKS) is used to determine the analysis state at the beginning of the fixed analysis window as is done for ROI, the FLKS can be considered a suboptimal version of the efficient ROI when the involved model is non-linear and has no errors. We confirm that the efficient ROI analyses are more accurate than the FLKS analyses with the increase of the analysis window size. Nevertheless, the computation costs for implementing efficient ROI are almost the same as those for FLKS. Additionally, the reduced-rank version of the efficient ROI is developed based on the accuracy-saturation property.
From the experiments using Lorenz 3-variable model, it is confirmed that the non-linearity of numerical model, which becomes stronger with the increase of the analysis window size, makes the analysis of efficient ROI more accurate than that of FLKS. Our Lorenz 40-variable experiments show that the average analysis error of the efficient ROI is smaller than that of the FLKS for an analysis window size of up to 4 d. However, the efficient ROI and the FLKS requires almost the same costs for computation. From the results of Lorenz 40-variable model experiments, it is suggested that, by using the reduced-rank formulation of the efficient ROI, we can obtain the suboptimal analysis more cost-effectively rather than FLKS.  相似文献   

The H₂/CO ratio of emissions from combustion sources: comparison of top-down with bottom-up measurements in southwest Germany     

By SAMUEL HAMMER  FELIX VOGEL  MARKUS KAUL  INGEBORG LEVIN 《Tellus. Series B, Chemical and physical meteorology》2009,61(3):547-555

The hydrogen-to-carbon monoxide (H₂/CO) emission ratio of anthropogenic combustion sources was determined from more than two years of quasi-continuous atmospheric observations in Heidelberg (49°24' N, 8°42' E), located in the polluted Rhein-Neckar region. Evaluating concurrent mixing ratio changes of H₂ and CO during morning rush hours yielded mean molar H₂/CO ratios of 0.40 ± 0.06, while respective results inferred from synoptic pollution events gave a mean value of 0.31 ± 0.05 mole H₂/mole CO. After correction for the influence of the H₂ soil sink on the measured ratios, mean values of 0.46 ± 0.07 resp. 0.48 ± 0.07 mole H₂/mole CO were obtained, which are in excellent agreement with direct source studies of traffic emissions in the Heidelberg/Mannheim region (0.448 ± 0.003 mole H₂/mole CO). Including results from other European studies, our best estimate of the mean H₂/CO emission ratio from anthropogenic combustion sources (mainly traffic) ranges from 0.45 to 0.48 mole H₂/mole CO, which is about 20% smaller than the value of 0.59 mole H₂/mole CO which is frequently used as the basis to calculate global H₂ emissions from anthropogenic combustion sources.  相似文献   

The radiative effect of an aged, internally mixed Arctic aerosol originating from lower-latitude biomass burning     

By ANN-CHRISTINE ENGVALL  JOHAN STRÖM  PETER TUNVED  RADOVAN KREJCI  HANS SCHLAGER  ANDREAS MINIKIN 《Tellus. Series B, Chemical and physical meteorology》2009,61(4):677-684

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Airborne measurements of dust layer properties, particle size distribution and mixing state of Saharan dust during SAMUM 2006     

By BERNADETT WEINZIERL  REAS PETZOLD  MICHAEL ESSELBORN  MARTIN WIRTH  KATHARINA RASP  KONRAD KANDLER  LOTHAR SCHÜTZ  PETER KOEPKE  MARKUS FIEBIG 《Tellus. Series B, Chemical and physical meteorology》2009,61(1):96-117

The Saharan Mineral Dust Experiment (SAMUM) was conducted in May/June 2006 in southern Morocco. As part of SAMUM, airborne in situ measurements of the particle size distribution in the diameter range 4 nm < D _p < 100 μm were conducted. The aerosol mixing state was determined below D _p < 2.5 μm. Furthermore, the vertical structure of the dust layers was investigated with a nadir-looking high spectral resolution lidar (HSRL). The desert dust aerosol exhibited two size regimes of different mixing states: below 0.5 μm, the particles had a non-volatile core and a volatile coating; larger particles above 0.5 μm consisted of non-volatile components and contained light absorbing material. In all cases, particles larger than 10 μm were present, and in 80% of the measurements no particles larger than 40 μm were present. The abundance of large particles showed almost no height dependence. The effective diameter D _eff in the dust plumes investigated showed two main ranges: the first range of D _eff peaked around 5 μm and the second range of D _eff around 8 μm. The two ranges of D _eff suggest that it may be inadequate to use one average effective diameter or one parametrization for a typical dust size distribution.  相似文献   

Vertically resolved dust optical properties during SAMUM: Tinfou compared to Ouarzazate     

By BIRGIT HEESE  DIETRICH ALTHAUSEN  TILMAN DINTER  MICHAEL ESSELBORN  THOMAS MÜLLER  MATTHIAS TESCHE  MATTHIAS WIEGNER 《Tellus. Series B, Chemical and physical meteorology》2009,61(1):195-205

Vertical profiles of dust key optical properties are presented from measurements during the Saharan Mineral Dust Experiment (SAMUM) by Raman and depolarization lidar at two ground-based sites and by airborne high spectral resolution lidar. One of the sites, Tinfou, is located close to the border of the Sahara in Southern Morocco and was the main in situ site during SAMUM. The other site was Ouarzazate airport, the main lidar site. From the lidar measurements the spatial distribution of the dust between Tinfou and Ouarzazate was derived for 1 d. The retrieved profiles of backscatter and extinction coefficients and particle depolarization ratios show comparable dust optical properties, a similar vertical structure of the dust layer, and a height of about 4 km asl at both sites. The airborne cross-section of the extinction coefficient at the two sites confirms the low variability in dust properties. Although the general picture of the dust layer was similar, the lidar measurements reveal a higher dust load closer to the dust source. Nevertheless, the observed intensive optical properties were the same. These results indicate that the lidar measurements at two sites close to the dust source are both representative for the SAMUM dust conditions.  相似文献   

The 30–60-day oscillation in the East Asian summer monsoon and its time-dependent association with the ENSO     

By KYUNG-SOOK YUN  BAOHUA REN  KYUNG-JA HA  JOHNNY C. L. CHAN  JONG-GHAP JHUN 《地球，A辑:动力气象学与海洋学》2009,61(5):565-578

Based on 30–60-day oscillation in the East Asian summer monsoon (EASM), the relationship between its northward propagation and ENSO (El Niño and Southern Oscillation) was investigated. To explicitly describe the 30–60-day monsoonal evolution, an empirical orthogonal function (EOF) analysis was carried out on the temporal-latitude section of the longitudinal average for 115°E–120°E. The principal 30–60-day EASM mode captures a northward propagation of well-organized intraseasonal oscillation (NISO). Using the associated time series of the first mode, we found a significant lagged correlation between interannual variability of the NISO and ENSO. Its lagged correlations with NINO indices have a quasi-biennial (QB) characteristic through the preceding summer and the concurrent summer. Their relationship was found by the regression analysis relating the low-level circulation to the ocean temperature. The western North Pacific anticyclone and the anticyclone-induced easterly vertical wind shear anomalies induce the dynamical linkage between the NISO and QB-type ENSO. It is shown that the NISO is more closely tied with QB-type ENSO in its phase than in its amplitude, and may be connected to the anomalous easterly wind and the eastward evolution of an oceanic Kelvin wave, which is associated with abrupt ENSO transition. The predictability on ENSO and NISO is examined through the canonical correlation analysis.  相似文献   

A comment on 'Vulnerability of permafrost carbon to global warming. Part I: model description and role of heat generated by organic matter decomposition' by D. V. Khvorostyanov et al. (2008)     

By L. KUTZBACH 《Tellus. Series B, Chemical and physical meteorology》2009,61(3):577-578

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