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581.
Gerhard?LammelEmail author Thomas?Engelhardt Adrian?Leip Christian?Neusü? Andreas?R?hrl Birgit?Wehner Alfred?Wiedensohler Paul?Wieser 《Journal of Atmospheric Chemistry》2005,51(1):95-117
The change of the chemical composition of the near-ground level atmospheric aerosol was studied during two summer episodes by a Lagrangian type of experimental approach. Bulk and single-particle chemical analyses of ions and elements in the particulate phase were deployed. N(-III) and N(V) components were also measured in the gas-phase. The measurements were completed by particle size distributions.Secondary inorganic aerosols (SIA) and fine particles of ≈0.2–0.4 μm size were still elevated 50 km downwind of the city. The direct comparison of transport over the city in contrast to transport over the surrounding areas showed that SIA was formed from emission from the city within less than 3 h. Relative increases, i.e., enrichment during transport were observed for primary and secondary aerosol components. The degree of mixing on the individual particle level increased significantly during transport in the area. In particular, newly emitted carbonaceous particles became internally mixed within hours with pre-existing sulphate particles. Mostly due to secondary aerosol formation the average particle size (mass median diameter) of major constituents of the aerosol was significantly decreased while being transported over 13 h. Given recent insights which link fine particles number and mass concentrations with health risks, the results suggest that rural populations in areas which frequently are located within an urban plume might run an elevated health risk relative to populations in areas not affected by urban plumes. 相似文献
582.
Fred A. Blaine Robert L. Linnen Gerhard E. Brügmann 《Geochimica et cosmochimica acta》2005,69(5):1265-1273
Haplobasaltic melts with a 101 kPa dry eutectic composition (An42Di58) and varying water contents were equilibrated with their platinum capsule at 1523 K and 200 MPa in an internally heated pressure vessel (IHPV) equipped with a rapid quench device. Experimental products were inclusion-free glasses representative of the Pt-saturated silicate melts at the experimental conditions. Platinum concentrations were determined using an isotope dilution multicollector inductively coupled plasma mass spectrometer and water contents and distribution by Karl Fischer titration and Fourier transform infrared spectroscopy, respectively.The water content of the melt has no intrinsic effect on platinum solubility, for concentrations between 0.9 wt.% and 4.4 wt.% H2O (saturation). Platinum solubility increases with increasing water content, but this effect is an indirect effect because increasing water content at fixed fH2 (imposed by the IHPV) increases the oxygen fugacity of the experiment.The positive oxygen fugacity dependence of Pt solubility in a hydrous silicate melt at 200 MPa is identical to that in anhydrous melts of the same composition determined in previous studies at 101 kPa. This study extends the range of platinum solubilities to oxygen fugacities lower than was previously possible. Combining the data of this and previous studies, Pt solubility is related to oxygen fugacity (in bar) at 1523 K by the equation:
[Pt]total(ppb)=1389×fO2+7531×(fO2)1/2 相似文献
583.
Wal-Mart entered the German market at the end of 1997 but is still running at a loss in its 92 stores. This article tests the hypothesis that there are two main reasons for Wal-Mart’s problems in Germany. First of all, Wal-Mart is competing against very strong and well established deep discounters, especially Aldi. Secondly, there is the difference between the so-called Wal-Mart culture and German customer values. So far, Wal-Mart has not managed to close this gap or create a positive image in Germany. The first part of the article describes the differences between the two retail companies Wal-Mart and Aldi, whereas the second part focuses on the consumer perspective. Four hundred people were interviewed on the phone about their shopping behaviour in the city of Würzburg (northern Bavaria, 140,000 inhabitants). This survey is part of an international study also undertaken in Canada, Great Britain and China. 相似文献
584.
Gerhard?JentzschEmail author Adelheid?Weise Carlos?Rey Carl?Gerstenecker 《Pure and Applied Geophysics》2004,161(7):1415-1431
Temporal gravity changes provide information about mass and/or density variations within and below the volcano edifice. Three active volcanoes have been under investigation; each of them related to a plate boundary: Mayon/Luzon/Philippines, Merapi/Java/Indonesia, and Galeras/Colombia. The observed gravity changes are smaller than previously expected but significant. For the three volcanoes under investigation, and within the observation period, mainly the increase of gravity is observed, ranging from 1,000 nm–2 to 1,600 nms–2. Unexpectedly, the gravity increase is confined to a rather small area with radii of 5 to 8 km around the summit. At Mayon and Merapi the parallel GPS measurements yield no significant elevation changes. This is crucial for the interpretation, as the internal pressure variations do not lead to significant deformation at the surface. Thus the classical Mogi-model for a shallow extending magma reservoir cannot apply. To confine the possible models, the attraction due to changes of groundwater level or soil moisture is estimated along the slope of Merapi exemplarily by 2-D modelling. Mass redistribution or density changes were evaluated within the vent as well as deeper fluid processes to explain the gravity variations; the results are compared to the model incorporating the additional effect of elastic deformation. 相似文献
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588.
A study of lunar impact crater size-distributions 总被引：3，自引：0，他引：3
Discrepancies in published crater frequency data prompted this study of lunar crater distributions. Effects modifying production size distributions of impact craters such as surface lava flows, blanketing by ejecta, superposition, infilling, and abrasion of craters, mass wasting, and the contribution of secondary and volcanic craters are discussed. The resulting criteria have been applied in the determination of the size distributions of unmodified impact crater populations in selected lunar regions of different ages. The measured cumulative crater frequencies are used to obtain a general calibration size distribution curve by a normalization procedure. It is found that the lunar impact crater size distribution is largely constant in the size range 0.3 km ?D ? 20 km for regions with formation ages between ≈ 3 × 109 yr and ? 4 × 109 yr. A polynomial of 4th degree, valid in the size range 0.8 km ?D ? 20 km, and a polynomial of 7th degree, valid in the size range 0.3 km ?D ? ? 20 km, have been approximated to the logarithm of the cumulative crater frequencyN as a function of the logarithm of crater diameterD. The resulting relationship can be expressed asN ～D α(D) where α is a function depending onD. This relationship allows the comparison of crater frequencies in different size ranges. Exponential relationships with constant α, commonly used in the literature, are shown to inadequately approximate the lunar impact crater size distribution. Deviations of measured size distributions from the calibration distribution are strongly suggestive of the existence of processes having modified the primary impact crater population. 相似文献
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590.
A new technique has been developed for the determination of the oxygen isotope composition from biogenic silica. The iHTR method (inductive high temperature carbon reduction) is based on the reduction of silica by carbon with temperatures of up to 1830°C (maximum T 2200°C) to produce carbon monoxide for isotope analysis. Basically, samples of silica are mixed with graphite and filled into a sample holder made of a glassy carbon rod. The rod is introduced into a glassy carbon cylinder liner closed at the top which itself is enclosed by a double-walled glass vessel. The glassy carbon rod is inductively heated under vacuum to the temperature needed for quantitative conversion of the particular silica material to CO. The most critical process of dehydration (in the case of opal) and reduction to CO is routinely achieved in the iHTR device. Weakly bound oxygen and oxygen-containing contaminants, like hydroxyl groups, as well as remaining minor organic constituents are volatilized stepwise under high vacuum at temperatures of 850°C and 1050°C without isotopic exchange before the reduction of the silica. After completion of dehydration, the temperature is raised to the value needed for silica reduction. For both biogenic silica and quartz a temperature of 1550°C was found to be adequate. The technical design with a standard preparation routine and various test experiments is presented proving the reliability and capability of the new iHTR method, especially with respect to fresh diatom materials and diatom opal. The amount of sample material necessary at present is ∼1.5 mg of silica and the reproducibility achieved for natural samples is better than ±0.15‰. Replicate analysis of the quartz standard NBS28 resulted in a δ18O value of 9.62‰ ± 0.11‰ (n = 17). 相似文献