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51.
Ronny Schoenberg Michael A.W. Marks Jan A. Schuessler Friedhelm von Blanckenburg Gregor Markl 《Chemical Geology》2009,258(1-2):65-77
The Ilímaussaq intrusion, South Greenland, provides an exceptional test case for investigating the changes of stable Fe isotope fractionation of solidus phases with changes in the Fe3+/∑Fe ratio of an evolving melt. The intrusion comprises a sequence of four melt batches that were fed from the same parental alkali basaltic magma. Differentiation produced cumulate rocks that range from augite syenite (phase I) over peralkaline granite (phase II) to agpaitic syenites (phases IIIa and IIIb). Fe3+/∑Fe ratios in amphiboles increase substantially from phase I to phase II and III rocks and mark a major change in the parental magma composition from augite syenites to peralkaline granites and agpaitic syenites. Before this transition, olivine, clinopyroxene, and amphibole in augite syenite, the most primitive rock type in the Ilímaussaq Complex, have a uniform Fe isotope composition that is identical to that of the bulk of igneous crustal rocks and approximated by the average isotopic composition of basalts (δ56/54FeIRMM-014 = 0.072 ± 0.046‰). After the transition, amphiboles in the peralkaline granites and agpaitic syenites yield significantly heavier Fe isotope compositions with δ56/54FeIRMM-014 values ranging from 0.123 to 0.237‰. Contamination of the Ilímaussaq magma by ongoing crustal assimilation as cause for this increase can be excluded on the grounds of Nd isotope data. Large-scale metasomatic overprint with an external fluid can also be dismissed based on amphibole O and Li isotope systematics. Rather, the increase towards heavy Fe isotope compositions most likely reflects the change in chemical compositions of amphiboles (calcic in augite syenite to sodic in the agpaitic syenites) and their Fe3+/ΣFe ratios that mirror changes in the chemical composition of the melt and its oxygen fugacity. A sensitive adjustment of equilibrium Fe isotope fractionation factors to amphibole ferric/ferrous ratios is also supported by beta-factors calculated from Mössbauer spetroscopy data. Comparison of the measured isotope fractionation between clinopyroxene and amphibole with that predicted from Mössbauer data reveal Fe isotope systematics close to equilibrium in augite syenites but Fe isotopic disequilibrium between these two phases in phase IIIa agpaitic syenites. These results are in agreement with O and Li isotope systematics. While amphiboles in all Ilímaussaq lithologies crystallized at temperatures between 650 and 850 °C, textural evidence reveals later clinopyroxene crystallization at temperatures as low as 300–400 °C. Therefore, isotopic equilibrium at crystallization conditions between these two phases can not be expected, but importantly, subsolidus reequilibration can also be dismissed. 相似文献
52.
Christian Betzler John J. G. Reijmer Karin Bernet Gregor P. Eberli & Flavio S. Anselmetti 《Sedimentology》1999,46(6):1127-1143
Core, logging and high-resolution seismic data from ODP Leg 166 were used to analyse deposits of the Neogene (Miocene–Lower Pliocene) Bahamian outer carbonate ramp. Ramp sediments are cyclic alternations of light- and dark-grey wackestones/packstones with interbedded calciturbidite packages and minor slumps. Cyclicity was driven by high-frequency sea-level changes. Light-grey layers containing shallow-water bioclasts were formed when the ramp exported material, whereas the dark-grey layers are dominantly pelagic. Calciturbidites are arranged into mounded lobes with feeder channels. Internal bedding of the lobes shows a north-directed shingling as a result of the asymmetrical growth of these bodies. Calciturbidite packages occur below and above sequence boundaries, indicating that turbidite shedding occurred during third-order sea-level highstands and lowstands. Highstand turbidites contain shallow-water components, such as green algal debris and epiphytic foraminifera, whereas lowstand turbidites are dominated by abraded bioclastic detritus. Gravity flow depocentres shifted from an outer ramp position during the early Miocene to a basin floor setting during the late Miocene to early Pliocene. This change was triggered by an intensification of the strength of bottom currents during the Tortonian, which was also responsible for shaping the convex morphology of the outer ramp. The Miocene and Lower Pliocene of the leeward flank of Great Bahama Bank provides an example of the poorly known depositional setting of the outer part of distally steepened carbonate ramps. The contrast between its sedimentary patterns and the well-known Upper Pliocene–Quaternary slope facies associations of the flat-topped Great Bahama Bank shows the strong control that the morphology of a carbonate platform exerts on the depositional architecture of the adjacent slope and base-of-slope successions. 相似文献
53.
An infrared heterodyne spectrometer with a resolving power of 6 × 106 has been used to obtain detailed profiles of the 10-μm absorption lines of CO2 in the atmosphere of Mars. An analysis of the results with an empirical model atmosphere calculation indicates a nearly pure CO2 atmosphere with an average surface pressure of 5.2 ± 0.5 mbar in the observed regions, a subsolar surface temperature near 275°K, an atmospheric temperature of 235 to 240°K above the subsolar point, and a lapse rate of 2°K/km. 相似文献
54.
Susan Mau Gregor Rehder Heiko Sahling Tina Schleicher Peter Linke 《International Journal of Earth Sciences》2014,103(7):1801-1815
Methane (CH4) concentrations and CH4 stable carbon isotopic composition ( \( \delta^{13} {\text{C}}_{{{\text{CH}}_{4} }} \) ) were investigated in the water column within Jaco Scar. It is one of several scars formed by massive slides resulting from the subduction of seamounts offshore Costa Rica, a process that can open up structural and stratigraphical pathways for migrating CH4. The release of large amounts of CH4 into the adjacent water column was discovered at the outcropping lowermost sedimentary sequence of the hanging wall in the northwest corner of Jaco Scar, where concentrations reached up to 1,500 nmol L?1. There CH4-rich fluids seeping from the sedimentary sequence stimulate both growth and activity of a dense chemosynthetic community. Additional point sources supplying CH4 at lower concentrations were identified in density layers above and below the main plume from light carbon isotope ratios. The injected CH4 is most likely a mixture of microbial and thermogenic CH4 as suggested by \( \delta^{13} {\text{C}}_{{{\text{CH}}_{4} }} \) values between ?50 and ?62 ‰ Vienna Pee Dee Belemnite. This CH4 spreads along isopycnal surfaces throughout the whole area of the scar, and the concentrations decrease due to mixing with ocean water and microbial oxidation. The supply of CH4 appears to be persistent as repeatedly high CH4 concentrations were found within the scar over 6 years. The maximum CH4 concentration and average excess CH4 concentration at Jaco Scar indicate that CH4 seepage from scars might be as significant as seepage from other tectonic structures in the marine realm. Hence, taking into account the global abundance of scars, such structures might constitute a substantial, hitherto unconsidered contribution to natural CH4 sources at the seafloor. 相似文献
55.
Sources of organic matter (OM) and lipids were assessed and factors affecting OM degradation were studied for two sediment cores representing distinct depositional regimes (i.e., the oscillating oxic to suboxic/anoxic western basin and oxic Zaka Bay) for eutrophic Lake Bled, NW Slovenia. Lower surface organic carbon (OC) concentration was determined in the western basin than for Zaka Bay sediments (5.1 vs. 5.4 wt% dry sediment, respectively), but one order of magnitude greater total lipid concentration was observed in the former. Also, there was a higher proportion of autochthonous OM in the western basin (77% vs. 66%) on the basis of atomic C/N ratios. Lipid-based origin assessment suggested a similar contribution of autochthonous OM in the western basin (64–77%), but a lower one in Zaka Bay (<50%). It seems that redox potential is the main factor governing OM degradation in the western basin. In contrast, a contribution from more refractory terrestrial OM, via the surface inflow in Zaka Bay, and higher sedimentation rates may surpass redox effects in Zaka Bay. Overall, oxygen may play a more important role in degradation of the more labile pool (i.e., lipids) than bulk OM. Higher apparent degradation rate constants (k′) for lipids also suggested a greater lability than for OC, while respective k′ values were higher in the oxic than anoxic environment. 相似文献
56.
Sabine Kraushaar Gregor Ollesch Christian Siebert Hans‐Joerg Vogel Markus Fuchs 《Geoarchaeology》2015,30(4):369-378
Roman cisterns served as rainwater storage devices for centuries and are densely distributed in parts of northern Jordan. A major earthquake hit the region ca. A.D. 750 and in a short time many settlements were abandoned. As a consequence, most cisterns were not maintained, and they filled with sediments that today provide a postabandonment depositional record. In two field surveys, we mapped the locations of more than 100 cisterns in the Wadi Al‐Arab basin and selected two for detailed stratigraphic analysis that included 14C and optically stimulated luminescence dating. Catchment basin area for each cistern was determined by differential GPS. Both cisterns filled with sediments after the great earthquake and consequent abandonment of the region. Calculated sediment volumes are translated to long‐term average sediment export rates of 2.6–6.6 t ha−1a−1, which are comparable to erosion and sediment yield rates from other studies within the Mediterranean region. Our pilot study suggests that this approach can be applied elsewhere to calculate long‐term sediment export rates on hill slopes containing relict cisterns. 相似文献
57.
David T. A. Symons Kazuo Kawasaki Sabine Walther Gregor Borg 《Mineralium Deposita》2011,46(2):137-152
Syngenetic, diagenetic and epigenetic models have been proposed for the Cu?CZn?CPb Kupferschiefer mineralization at Sangerhausen, Germany. Paleomagnetic and rock magnetic measurements have been made on 205 specimens from mine workings on the margin of the Sangerhausen Syncline. The mineralization is richest in the ??0.5-m-thick Upper Permian (258?±?2?Ma) Kupferschiefer black marly shale (nine sites) and dies out over ??0.2?m in the underlying Weisliegend sandstones (three sites) and overlying Zechstein carbonates (two sites). Except for one site of fault zone gypsum, characteristic remanent magnetization directions were isolated for all 14 sites using alternating field and thermal step demagnetization. These directions provide a negative fold test, indicating that the remanence postdates Jurassic fault block tilting. Rock magnetic measurements show that the Kupferschiefer shale marks a redox front between the oxidized Weissliegend sandstones and non-oxidized Zechstein carbonates. The 14 site directions give a Late Jurassic paleopole at 149?±?3?Ma. It is significantly different from the paleopole reported by E.C. Jowett and others for primary or early diagenetic Rote F?ule alteration that gives an age of 254?±?6?Ma on the current apparent polar wander path and is associated with Kupferschiefer mineralization. We suggest that the Late Jurassic extensional tectonic event that formed the nearby North German Basin also reactivated Variscan basement faults and extended them up through the overlying strata, thereby allowing hydrothermal basement fluids to ascend and epigenetically mineralize the Kupferschiefer shale. The possibility of a 53?±?3?Ma mineralization age is also considered. 相似文献
58.
Microstructural evolution during experimental albitization of K-rich alkali feldspar 总被引:1,自引:1,他引:0
Nicholas Norberg Gregor Neusser Richard Wirth Daniel Harlov 《Contributions to Mineralogy and Petrology》2011,162(3):531-546
Crystals of K-feldspar (C2/m), in contact with highly concentrated aqueous NaCl solutions at 500°C and 200 MPa, are pseudomorphically replaced by high
albite (C[`1]) (C\bar{1}) as a result of an interface-coupled dissolution/reprecipitation process. The reaction occurs at an extremely sharp reaction
front (<10 nm) and involves the complete breakdown of the initial framework structure. This results in the release of tetrahedrally
incorporated elements such as Fe3+ and Ti4+ and a significant increase in Si/Al disorder across the reaction interface. The evolving microstructure is controlled by
crystallographic relations between the phases. This leads to highly anisotropic, sawtooth-shaped intergrowths of albite and
initial K-feldspar, resulting in the least structural misfit between the two framework structures. As a result, the newly
formed interfaces appear to be semicoherent, and cracks across the reaction fronts even indicate elastic strain. The reaction
produces 2 distinctive albite types (albite-1 and albite-2). Both are polycrystalline, with albite-2 showing significantly larger subgrain sizes. This indicates a secondary coarsening step driven by the reduction in interfacial
energy within the polycrystalline replacement product. The reaction also produces a highly porous rim. However, the porosity
is not evenly distributed resulting in a porous albite-1 and a non-porous albite-2 that mostly surrounds large, euhedral pores. Despite the substantial volume fraction of porosity in albite-1, no significant 3D interconnectivity could be detected, making the presence of a pervasive porosity unlikely. However, the
result of coarsening is the continuous modification of the 3D porosity distribution. This could potentially provide a mechanism
for fluid transport through the replacement rim until textural and chemical equilibration is achieved. 相似文献
59.
Gregor Muri Branko Čermelj Radojko Jaćimović Dragomir Skaberne Andrej Šmuc Martina Burnik Šturm Janja Turšič Polona Vreča 《Journal of Paleolimnology》2013,50(4):457-470
Several geological and geochemical parameters were determined in the sediments of the 5th (5 J) and 6th (6 J) Triglav Lakes, Julian Alps (NW Slovenia), in order to study the impact of natural catchment characteristics and anthropogenic activity. Fish were introduced into both lakes in 1991 and a mountain hut lies on the shore of 5 J. Sedimentary grain size (GS) was distinctly coarser in 5 J than 6 J, with arithmetic means ranging between 46 and 60 and 23–36 μm, respectively. In contrast, the mineralogical composition of the two sediments was similar. Calcite predominated strongly, comprising more than 77 % of total minerals, while dolomite and quartz were rare. Organic carbon (OC) and total nitrogen (TN) concentrations were highest in surficial sediments, with levels of 14.4 and 1.8 %, and 19.3 and 2.4 % observed in 5 J and 6 J, respectively. C/N ratios (atomic) were lowest in the same surface sediments, with the two lakes characterized by similar values (9.6 vs. 9.4, respectively), suggesting a predominance of autochthonous organic matter (OM) in both lakes. Contemporary δ13C values were lower in 5 J (?21.0 ‰) than 6 J (?18.5 ‰) sediments. Considerable changes in these four parameters were observed in recently deposited material, reflecting a shift in the trophic status of both lakes that was likely induced by the introduction of fish. In addition, the smaller and shallower 6 J seemed to respond to changes faster than the larger and deeper 5 J, indicating the higher sensitivity of the former. δ15N values in surface sediments of 5 J and 6 J were ?2.9 and ?4.4 ‰, respectively, with levels increasing gradually with depth to approximately +1.0 ‰ in deeper sediments. The observed changes could most likely be attributed to the atmospheric deposition of reactive nitrogen. The mountain hut has seemingly not had a significant enough impact on the lakes to be recorded in their sediments. 相似文献
60.