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161.
162.
通过浸渍法(IM)和沉积-沉淀(DP)法制备了一系列Pt/TiO2P25)催化剂,并分别用甲醛溶液和氢气还原处理催化剂.利用原位红外监测催化剂表面吸附物种在反应过程中的变化,探究了催化剂制备和还原条件及Pt负载量对催化剂结构和催化氧化甲醛活性的影响.结果显示,用DP法制备并用甲醛还原的Pt/P25催化剂中Pt颗粒分散均匀,并具有合适的粒径和高浓度的表面活性氧,显示出良好的甲醛氧化活性.在空速30 000 ml/(g·h)、反应温度30°C和甲醛初始浓度50 mg/m的条件下,0.4%Pt/P25(DP-HCHO)上的甲醛转化率达到98%,并能稳定运行100 h以上.相比之下,Pt/P25(DP-H2)由于表面活性氧较少,不利于甲酸盐氧化,活性较低.Pt/P25(IM-H2)虽然具有高浓度的表面活性氧,却同时具有最大的Pt颗粒粒径,在甲醛转化为甲酸盐和甲酸盐氧化两步反应中的活性均较差,因而甲醛氧化活性最差. 相似文献
163.
人工神经网络与分析测试技术的研究与发展 总被引:8,自引:0,他引:8
回顾了人工神经网络研究的发展历程,简要介绍了神经网络模型与算法,对分析测试技术和相关学科中的人工神经网络研究及在流程控制、错误诊断、参数估计、传感器模型、模式识别与分类、环境监测与治理及光谱与化学分析中的应用等作了评述。引用参考文献113篇。 相似文献
164.
陕西洛川黄土-古土壤剖面中伊利石结晶度——黄土物质来源和古气候环境的指示 总被引:6,自引:0,他引:6
伊利石是我国黄土和古土壤中最主要的粘土矿物。本文选择陕西洛川黄土-古土壤国际典型剖面为研究对象,通过测定伊利石的结晶度(Kubler指数)、Srodon峰强比值(Ir)和2M_1多型含量,发现黄土物质的起源与中高温(>280℃)地质环境有关;黄土样品中伊利石结晶度值为0.25°2θ(Cu Ka),古土壤样品中伊利石结晶度值大于0.27°2θ(Cu Ka);黄土和古土壤中伊利石结晶度值的差别,是由于古土壤中伊利石含少量的膨胀层,而黄土样品中的伊利石不含有膨胀层而引起的。古土壤中伊利石的膨胀层的成因,与伊利石 相似文献
165.
166.
This paper examines historical and spatial trends in hazardous materials transportation spills from 1971 to 1991. While the number of spills Inc.reased steadily during the 1970s, peaking in 1978–1979, there has been a decline in frequency sInc.e then largely due to modifications in reporting. Monetary damages have the opposite temporal pattern, with major Inc.reases recorded from 1982 onward. Death and injury statistics are more variable. Spatially, accidents are more prevalent in the Rust Belt extending from the Northeast corridor westward to the Great Lakes states, as well as in the Southeast. The greatest potential risk to the public is found in smaller, more densely populated industrial states such as New Jersey, Delaware, and Maryland. The spatial distribution, however, has not changed. Potential risk sources (e.g., chemical industry, number of hazardous waste facilities, number of railroad miles) are the best predictors of hazmat Inc.ident frequency. Mitigation efforts (statewide regulatory and/or management policies) also help explain the variability in hazmat Inc.idents. 相似文献
167.
M. Cocco J. Pacheco S. K. Singh F. Courboulex 《Geophysical Journal International》1997,131(1):135-145
An analysis of the Zihuatanejo, Mexico, earthquake of 1994 December 10 ( M = 6.6), based on teleseismic and near-source data, shows that it was a normal-faulting, intermediate-depth ( H = 50 ± 5 km) event. It was located about 30 km inland, within the subducted Cocos plate. The preferred fault plane has an azimuth of 130°, a dip of 79° and a rake of −86°. The rupture consisted of two subevents which were separated in time by about 2 s, with the second subevent occurring downdip of the first. The measured stress drop was relatively high, requiring a Δσ of about a kilobar to explain the high-frequency level of the near-source spectra. A rough estimate of the thickness of the seismogenic part of the oceanic lithosphere below Zihuatanejo, based on the depth and the rupture extent of this event, is 40 km.
This event and the Oaxaca earthquake of 1931 January 15 ( M = 7.8) are the two significant normal-faulting, intermediate-depth shocks whose epicentres are closest to the coast. Both of these earthquakes were preceded by several large to great shallow, low-angle thrust earthquakes, occurring updip. The observations in other subduction zones show just the opposite: normal-faulting events precede, not succeed, updip, thrust shocks. Indeed, the thrust events, soon after their occurrence, are expected to cause compression in the slab, thus inhibiting the occurrence of normal-faulting events. To explain the occurrence of the Zihuatanejo earthquake, we note that the Cocos plate, after an initial shallow-angle subduction, unbends and becomes subhorizontal. In the region of the unbending, the bottom of the slab is in horizontal extension. We speculate that the large updip seismic slip during shallow, low-angle thrust events increases the buckling of the slab, resulting in an incremental tensional stress at the bottom of the slab and causing normal-faulting earthquakes. This explanation may also hold for the 1931 Oaxaca event. 相似文献
This event and the Oaxaca earthquake of 1931 January 15 ( M = 7.8) are the two significant normal-faulting, intermediate-depth shocks whose epicentres are closest to the coast. Both of these earthquakes were preceded by several large to great shallow, low-angle thrust earthquakes, occurring updip. The observations in other subduction zones show just the opposite: normal-faulting events precede, not succeed, updip, thrust shocks. Indeed, the thrust events, soon after their occurrence, are expected to cause compression in the slab, thus inhibiting the occurrence of normal-faulting events. To explain the occurrence of the Zihuatanejo earthquake, we note that the Cocos plate, after an initial shallow-angle subduction, unbends and becomes subhorizontal. In the region of the unbending, the bottom of the slab is in horizontal extension. We speculate that the large updip seismic slip during shallow, low-angle thrust events increases the buckling of the slab, resulting in an incremental tensional stress at the bottom of the slab and causing normal-faulting earthquakes. This explanation may also hold for the 1931 Oaxaca event. 相似文献
168.
169.
塔克拉玛干沙漠土壤沙化发生条件及对土壤性状影响 总被引:1,自引:0,他引:1
土壤沙化是土壤发育逆向演替恢复母质特性的过程,土壤沙化发生条件可以概括为4个方面:土壤干旱是沙化的根本条件、植被衰败为风沙活动创造了条件、土壤质地轻是沙化物质基础、大风和频繁起沙风是沙化的动力条件。土壤沙化结果使土壤粗粒化、贫瘠化,同时也使土壤含盐量降低。 相似文献
170.
粒度分析在塔克拉玛干沙漠研究中的应用 总被引:18,自引:6,他引:18
本文重点探讨了塔克拉玛干沙漠的风成沙粒度组成特征及其与物源的关系,同时对沙丘的下伏地层沙、现代河流沙及丘间地沙的粒度组成也进行了对比。通过对该沙漠第四纪沉积物的粒度分析,证实了风成沙的粒度分布以极细沙为主,不含粗沙,粉沙含量极小;粒度组合、分选主要受营力和源区物质制约,结果使粒度空间分布形成格局。总之,通过粒度分析得到一系列量化指征,可为研究风沙流运动,探讨沉积环境和改造沙漠、发展沙产业提供理论依据。 相似文献