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41.
42.
Remediation of subsurface contamination requires an understanding of the contaminant (history, source location, plume extent and concentration, etc.), and, knowledge of the spatial distribution of hydraulic conductivity (K) that governs groundwater flow and solute transport. Many methods exist for characterizing K heterogeneity, but most if not all methods require the collection of a large number of small‐scale data and its interpolation. In this study, we conduct a hydraulic tomography survey at a highly heterogeneous glaciofluvial deposit at the North Campus Research Site (NCRS) located at the University of Waterloo, Waterloo, Ontario, Canada to sequentially interpret four pumping tests using the steady‐state form of the Sequential Successive Linear Estimator (SSLE) ( Yeh and Liu 2000 ). The resulting three‐dimensional (3D) K distribution (or K‐tomogram) is compared against: ( 1 ) K distributions obtained through the inverse modeling of individual pumping tests using SSLE, and ( 2 ) effective hydraulic conductivity (Keff) estimates obtained by automatically calibrating a groundwater flow model while treating the medium to be homogeneous. Such a Keff is often used for designing remediation operations, and thus is used as the basis for comparison with the K‐tomogram. Our results clearly show that hydraulic tomography is superior to the inversions of single pumping tests or Keff estimates. This is particularly significant for contaminated sites where an accurate representation of the flow field is critical for simulating contaminant transport and injection of chemical and biological agents used for active remediation of contaminant source zones and plumes. 相似文献
43.
Wafa M. Al Lawati Athanasios Rizoulis Elisabeth Eiche Christopher Boothman David A. Polya Jonathan R. Lloyd Michael Berg Patricio Vasquez-Aguilar Bart E. van Dongen 《Applied Geochemistry》2012
High concentrations of geogenic As in the groundwaters of south and SE Asia, which are used as drinking waters, are causing severe health impacts to the exposed human populations. It is widely accepted that As mobilisation from sediments into these shallow reducing groundwaters requires active metal-reducing microbes and electron donors such as organic matter (OM). Although OM in such Holocene aquifers has been characterised, there is a dearth of data on Pleistocene aquifers from the same areas. Reported here are preliminary studies of OM and microbial communities present in two aquifers, one of Pleistocene and one of Holocene age, with contrasting concentrations of As (viz. Pleistocene: low As <10 μg/L; Holocene: high As up to 600 μg/L) from Van Phuc village in the Red River Delta, Vietnam. Results revealed OM inputs from multiple sources, including potential contributions from naturally occurring petroleum seeping into the shallow aquifer sediments from deeper thermally mature source rocks. Although concentrations vary, no noticeable systematic differences in biomarker distribution patterns within the OM were observed between the two sites. Microbial analyses did not show a presence of microbial communities previously associated with As mobilisation. All clone libraries were dominated by α-, β-, and γ-Proteobacteria not known to be able to reduce Fe(III) or sorbed As(V). Furthermore, representatives of the Fe(III)-reducing genus Geobacter could only be detected at very low abundance by PCR, using highly selective 16S rRNA gene primers, supporting the hypothesis that metal reduction is not a dominant in situ process in these sediments. No correlation between As concentration in groundwater and OM composition nor microbial community in the host sediments was found. This suggests that either (i) As is not being significantly mobilised in situ in these sediments, instead As appears to be mobilised elsewhere and transported by groundwater flow to the sites or (ii) sorption/desorption processes, as implicated by geochemical data from the cores, play a critical role in controlling As concentrations at these sites. 相似文献
44.
Transient release of Ni,Mn and Fe from mixed metal sulphides under oxidising and reducing conditions
C. Naylor W. Davison M. Motelica-Heino L. M. van der Heijdt G. A. van den Berg 《Environmental Earth Sciences》2012,65(7):2139-2146
The potential release of metals from anoxic sediments exposed to oxygen was investigated by using a synthetic preparation
of metal sulphides dominated by solid phase FeS. The technique of DGT (diffusive gradients in thin-films) was used to measure
sulphide and Fe, Mn and Ni in the anoxic metal-sulphide slurry, which had a pH of 6.4. Speciation calculations based on these
data showed there was moderate supersaturation with respect to amorphous FeS in the solution phase. Measurements made using
DGT with a range of diffusion layer thicknesses showed that when Fe, Mn and Ni are removed from solution there is fairly rapid
(minutes) release from the solid phase, that is reasonably well sustained. This presumed desorptive release will be responsible
for elevated concentrations of some metals in solution when sediments are resuspended. Oxidation of the slurry by bubbling
with air rapidly (hours) removed Fe, Mn and Ni from the pore water solution. While Fe concentrations in solution remained
low after the removal, Mn and Ni were transiently released. These results were consistent with initial rapid oxidation of
Fe(II) to oxyhydroxides, which remove Mn(II) and Ni by adsorption. The slower oxidation of FeS then releases Mn and Ni, but
these too are eventually removed by adsorption to iron oxyhydroxides. These data suggest that oxidation of metal sulphides
will contribute to the release of metals from sediment disturbed by dredging or remedial aeration, but it is likely to be
short lived, with complete removal within a day. 相似文献
45.
Earthquake motion is one of the extreme loads acting on large dams. Dam owners and regulators must therefore ensure that dams
are safely operated and present minimal risk to the public in case of extreme loads such as floods and earthquakes. Owners
of many dams or officials in charge of dam safety programs may consider comparative assessment of the seismic risk associated
with their dams and establish priorities for detailed evaluation. South Africa has in excess of 100 large state-owned dams
and the characteristics of these dams have been used to perform a basic seismic hazard assessment and rank the vulnerability
of these dams from the lowest to highest. One of the most decisive factors that contributes to the risk of a dam is the wall
type; with gravity and earthfill dams being the most vulnerable to earthquake motion. Another aspect that needs further investigation
is the downstream hazard potential which, if known to a better degree of accuracy, can provide more reasonable estimates of
the risk factors. 相似文献
46.
Our objective is to understand general causes of different river channel patterns. In this paper we compare an empirical stream power‐based classification and a physics‐based bar pattern predictor. We present a careful selection of data from the literature that contains rivers with discharge and median bed particle size ranging over several orders of magnitude with various channel patterns and bar types, but no obvious eroding or aggrading tendency. Empirically a continuum is found for increasing specific stream power, here calculated with pattern‐independent variables: mean annual flood, valley gradient and channel width predicted with a hydraulic geometry relation. ‘Thresholds’, above which certain patterns emerge, were identified as a function of bed sediment size. Bar theory predicts nature and presence of bars and bar mode, here converted to active braiding index (Bi). The most important variables are actual width–depth ratio and nonlinearity of bed sediment transport. Results agree reasonably well with data. Empirical predictions are somewhat better than bar theory predictions, because the bank strength is indirectly included in the empirical prediction. In combination, empirical and theoretical prediction provide partial explanations for bar and channel patterns. Increasing potential‐specific stream power implies more energy to erode banks and indeed correlates to channels with high width–depth ratio. Bar theory predicts that such rivers develop more bars across the width (higher Bi). At the transition from meandering to braiding, weakly braided rivers and meandering rivers with chutes are found. Rivers with extremely low stream power and width–depth ratios hardly develop bars or dynamic meandering and may be straight or sinuous or, in case of disequilibrium sediment feed, anastomosing. Copyright © 2010 John Wiley & Sons, Ltd. 相似文献
47.
48.
T. K. Croat T. Berg T. Bernatowicz E. Groopman M. Jadhav 《Meteoritics & planetary science》2013,48(4):686-699
Transmission electron microscope (TEM) investigations have revealed Os, Ru, Mo‐rich refractory metal nuggets within four different presolar graphites, from both the high‐density (HD) Murchison (MUR) and low‐density (LD) Orgueil (ORG) fractions. Microstructural and chemical data suggest that these are direct condensates from the gas, rather than forming later by exsolution. The presolar refractory metal nugget (pRMN) compositions are variable (e.g., from 8 < Os atom% < 77), but follow the same chemical fractionation trends as isolated refractory metal nuggets (mRMNs) previously found in meteorites (Berg et al. 2009). From these compositions one can infer a temperature of last equilibration with the gas of 1405–1810 K (e.g., Berg et al. 2009 at approximately 100 dyne cm?2 pressure), which implies that the host graphites form over roughly the same range (in agreement with predictions) and that the pRMNs are chemically isolated from the gas when captured by graphite. Further, the pRMN compositions give evidence that HD graphites form at a higher T than LD ones. Chemical and phase similarities with the isolated mRMNs suggest that the mRMNs also condense directly from a gas, although from the early solar nebula rather than a presolar environment. Although the pRMNs themselves are too small for detection of isotopic anomalies, NanoSIMS isotopic measurements of their host graphites confirm a presolar origin for the assemblages. The two pRMN‐containing LD graphites show evidence of a supernova (SN) origin, whereas the stellar origins of the pRMNs in HD graphite are unclear, because only less‐diagnostic 12C enrichments are detectable (as is commonly true for HD graphites). 相似文献
49.
J. de Vries M. H. G. Jacobs A. P. van den Berg M. Wehber C. Lathe C. A. McCammon W. van Westrenen 《Physics and Chemistry of Minerals》2013,40(9):691-703
Iron-rich orthopyroxene plays an important role in models of the thermal and magmatic evolution of the Moon, but its density at high pressure and high temperature is not well-constrained. We present in situ measurements of the unit-cell volume of a synthetic polycrystalline end-member orthoferrosilite (FeSiO3, fs) at simultaneous high pressures (3.4–4.8 GPa) and high temperatures (1,148–1,448 K), to improve constraints on the density of orthopyroxene in the lunar interior. Unit-cell volumes were determined through in situ energy-dispersive synchrotron X-ray diffraction in a multi-anvil press, using MgO as a pressure marker. Our volume data were fitted to a high-temperature Birch–Murnaghan equation of state (EoS). Experimental data are reproduced accurately, with a $\varDelta P$ Δ P standard deviation of 0.20 GPa. The resulting thermoelastic parameters of fs are: V 0 = 875.8 ± 1.4 Å3, K 0 = 74.4 ± 5.3 GPa, and $\frac{{\text d}K}{{\text d}T} = -0.032 \pm 0.005\,\hbox{GPa K}^{-1}$ d K d T = - 0.032 ± 0.005 GPa K - 1 , assuming ${K}^{\prime}_{0} = 10 $ K 0 ′ = 10 . We also determined the thermal equation of state of a natural Fe-rich orthopyroxene from Hidra (Norway) to assess the effect of magnesium on the EoS of iron-rich orthopyroxene. Comparison between our two data sets and literature studies shows good agreement for room-temperature, room-pressure unit-cell volumes. Preliminary thermodynamic analyses of orthoferrosilite, FeSiO3, and orthopyroxene solid solutions, (Mg1?x Fe x ) SiO3, using vibrational models show that our volume measurements in pressure–temperature space are consistent with previous heat capacity and one-bar volume–temperature measurements. The isothermal bulk modulus at ambient conditions derived from our measurements is smaller than values presented in the literature. This new simultaneous high-pressure, high-temperature data are specifically useful for calculations of the orthopyroxene density in the Moon. 相似文献
50.
Iron-hydroxide clogging of public supply wells receiving artificial recharge: near-well and in-well hydrological and hydrochemical observations 总被引:2,自引:2,他引:0
Diego A. Bustos Medina Gerard A. van den Berg Boris M. van Breukelen Maria Juhasz-Holterman Pieter J. Stuyfzand 《Hydrogeology Journal》2013,21(7):1393-1412
Clogging of water wells by iron-hydroxide incrustations due to mixing of anoxic and oxic groundwater is a common well-ageing problem. The relation between well operation (on and off), the spatial and temporal variations in hydrochemistry outside and inside a supply well, and the distribution of clogging iron-hydroxides were studied in an artificial recharge well field in the Netherlands. Camera inspection, high-resolution multi-level water sampling outside the well and detailed in-well pH/EC/O2 profiles revealed remarkable patterns. During pumping, the top of the upper well screen abstracted oxic filtrate, although the larger part of the in-well water column was anoxic. The column rapidly turned oxic after shutdown due to a downward short-circuiting of oxic water via the well. Within 15 d it became anoxic due to the slow advance of anoxic lake filtrate created by local changes in flow direction as the neighboring wells continued to pump. Severe clogging occurred where the oxic filtrate entered the well, while half-clogging of the upper well screen occurred due to less inflow of oxic filtrate on the lake side. Transport of iron flocs and bacterial slimes after shutdown seemed to clog the lower part of the well screen. Frequent on/off switching should be avoided in iron-clogged wells. 相似文献