The retention of ammonia and sulfur dioxide during riming of ice particles and dendritic snow flakes: laboratory experiments in the Mainz vertical wind tunnel     

Nadine v. Blohn  Karoline Diehl  Anke Nölscher  Alexander Jost  Subir K. Mitra  Stephan Borrmann 《Journal of Atmospheric Chemistry》2013,70(2):131-150

Laboratory experiments were carried out in the Mainz vertical wind tunnel to determine the retention of the trace gases ammonia and sulfur dioxide dissolved in supercooled cloud droplets during riming. The conditions during riming were similar to the ones in atmospheric mixed phase clouds: temperatures from ?18 °C to ?5 °C, liquid water contents between 1 and 1.5 g m^?3, liquid drop radii between 10 and 20 μm, liquid phase concentrations from 1 to 22 mg/l. As collectors, floating ice particles and snow flakes with diameters between 6 mm and 1.5 cm were used. After riming the retention coefficients, i.e. the fractions of the species which remained in the ice phase after freezing were determined. Retention coefficients lying between 0.1 and 1.0 were measured depending on the solubility and dissociation of the trace gas, liquid phase concentration, ambient air temperature, and shape of rimed collector. This can be explained from the chemists’ point of view by the effective Henry’s law constant of the species and physically with the rate of latent heat removal from the rimed collector during freezing. Parameterizations derived from the different experimental cases describe the retention coefficients as a function of temperature. In general, an average retention of ammonia of 92?±?21 % was determined independently of liquid phase concentration while mean values for sulfur dioxide were 53?±?10 % at low liquid phase concentrations and 29?±?7 % at high liquid phase concentrations.  相似文献   

Cambrian sedimentary dykes in the Proterozoic basement of the Västervik area (southeast Sweden): episodic formation inferred from macro- and microfabrics     

Nadine Friese  Axel Vollbrecht  Bernd Leiss  Olaf Jacke 《International Journal of Earth Sciences》2011,100(4):741-752

Fabrics of Cambrian sedimentary dykes formed in Proterozoic granites of the Västervik area (Southeast Sweden) evidence repeated opening/filling and mineralisation/cementation events under varying conditions. Diagnostic features include (1) wall-parallel boundaries between epiclastic fillings and (2) early formed dyke sediments that appear as lithoclasts in subsequently formed sedimentary fillings. The psammitic components mostly consist of well-rounded quartz grains related to a coastal environment and fragments from the granitic host rock. Platy calcitic fragments embedded in the epiclastic matrix originally formed as microveins within already-lithified dyke sediments and the adjacent host rock. Convex downward-pointing, internal sagging structures, together with the preferred orientation of compositional boundaries and long axes of grains/rock fragments parallel to the dyke walls, are interpreted as the result of suction-controlled flow of unconsolidated fillings during episodes of downward dyke growth. Pressure solution of quartz grains are evidence of extensional phases with dyke propagation that were interrupted by phases of horizontal compression normal to the dyke walls. The N–S and NE–SW striking sedimentary dykes formed by opening of a pre-existing joint set during NW–SE oriented rifting during the Cambrian.  相似文献   

Stakeholders’ expectations towards a proposed marine protected area: A multi-criteria analysis of MPA performance criteria     

Nadine Heck  Philip Dearden  Adrian McDonald 《Ocean & Coastal Management》2011,54(9):687-695

In order to enable effective management of marine protected areas (MPAs), desired MPA achievements need to be identified as early as possible for the development of relevant and clear management goals, objectives and conservation targets. As the definition of MPA success is a social construct, the involvement of multiple groups in this process including government agencies, stakeholders, and other interested parties is increasingly advocated. This study investigates diverse groups’ opinions on the performance of a proposed National Marine Conservation Area (NMCA) on the West coast of Canada prior to its establishment. In order to analyse and quantify the importance of MPA performance criteria among multiple stakeholder groups, the Analytical Hierarchy Process (AHP) is applied. Findings reveal that marine stakeholder groups have distinct preferences for future MPA performance. Most differences are obvious between user and non-user groups. The study also finds that respondents’ characteristics other than stakeholder groups affiliations influence expectations towards the proposed MPA including livelihood dependency on the marine environment, amount of time spent in the area, and engagement in fishing activities.  相似文献   

预料之外的安第斯地震     

韩立波 《国际地震动态》2011,(10):12-14

沿南美安第斯山脉西缘的俯冲带边界预期会发生大地震。而沿东边界的地表运动测量表明,曾预期不会发生大地震的安第斯山脉东缘也具有发生同等规模大地震的潜在可能。  相似文献   

Style for the Zeitgeist: The Stealthy Revival of Historicist Housing Since the Late 1960s     

Nadine Dostrovsky  Richard Harris 《The Professional geographer》2013,65(3):314-332

A revival has occurred in the use of historical architectural styles for modern suburban houses but this has attracted little attention from journalists and academics. Those who have noted it disagree about when it began and gathered momentum. Newspaper and trade journal evidence for Canadian cities indicates that the revival began in the late 1960s; that it has reached market saturation; and that Victorian and neo-classical styles became dominant after 1980. Coinciding with the beginnings of inner-city gentrification, the historicist revival in suburban dwellings preceded the recent interest in neotraditional urban design. Not a fringe taste, it says something about the zeitgeist.  相似文献   

Tweet Me Your Talk: Geographical Learning and Knowledge Production 2.0   总被引：1，自引：0，他引：1  

Nadine Schuurman 《The Professional geographer》2013,65(3):369-377

We are in a Gutenberg moment in which we are migrating from book reading to Internet browsing. We are subtly shifting to more ephemeral, summary methods of learning and producing knowledge, shaped by how we consume information on the Web. Thus, a strong determinant of learning might be the very technology that hosts the information, such that technology is both the arbiter of our understanding of the world and how we come to gain that understanding. Based on recent evidence that the Internet is reshaping our learning processes, I argue that geographical knowledge production and translation are not so much products of individualism but rather shaped by rapidly changing work styles that favor concise and highly accessible methods of academic production. I offer examples of changes in journal formats, academic social networking, and academic reviewing to reveal that we are catering to shorter attention spans that prefer to browse.  相似文献   

Storage,mixing, and fluxes of water in the critical zone across northern environments inferred by stable isotopes of soil water          下载免费PDF全文

Matthias Sprenger  Doerthe Tetzlaff  Jim Buttle  Sean K. Carey  James P. McNamara  Hjalmar Laudon  Nadine J. Shatilla  Chris Soulsby 《水文研究》2018,32(12):1720-1737

Quantifying soil water storage, mixing, and release via recharge, transpiration, and evaporation is essential for a better understanding of critical zone processes. Here, we integrate stable isotope (²H and ¹⁸O of soil water, precipitation, and groundwater) and hydrometric (soil moisture) data from 5 long‐term experimental catchments along a hydroclimatic gradient across northern latitudes: Dry Creek (USA), Bruntland Burn (Scotland), Dorset (Canada), Krycklan (Sweden), and Wolf Creek (Canada). Within each catchment, 6 to 11 isotope sampling campaigns occurred at 2 to 4 sampling locations over at least 1 year. Analysis for ²H and ¹⁸O in the bulk pore water was done for >2,500 soil samples either by cryogenic extraction (Dry Creek) or by direct equilibration (other sites). The results showed a similar general pattern that soil water isotope variability reflected the seasonality of the precipitation input signal. However, pronounced differences among sampling locations occurred regarding the isotopic fractionation due to evaporation. We found that antecedent precipitation volumes mainly governed the fractionation signal, temperature and evaporation rates were of secondary importance, and soil moisture played only a minor role in the variability of soil water evaporation fractionation across the hydroclimatic gradient. We further observed that soil waters beneath conifer trees were more fractionated than beneath heather shrubs or red oak trees, indicating higher soil evaporation rates in coniferous forests. Sampling locations closer to streams were more damped and depleted in their stable isotopic composition than hillslope sites, revealing increased subsurface mixing towards the saturated zone and a preferential recharge of winter precipitation. Bulk soil waters generally comprised a high share of waters older than 14 days, which indicates that the water in soil pores are usually not fully replaced by recent infiltration events. The presented stable isotope data of soil water were, thus, a useful tool to track the spatial variability of water fluxes within and from the critical zone. Such data provide invaluable information to improve the representation of critical zone processes in spatially distributed hydrological models.  相似文献   

A two-moment parameterization of aerosol nucleation and impaction scavenging for a warm cloud microphysics: description and results from a two-dimensional simulation     

D. Caro  W. Wobrock  A. I. Flossmann  N. Chaumerliac 《Atmospheric Research》2004,70(3-4):171-208

A new two-moment warm bulk scheme has been developed including explicitly nucleation and impaction scavenging of aerosol particles as well as all other microphysical processes. The scheme is built upon a quasispectral representation of the aerosol particle, cloud droplet and raindrop distributions. It predicts mixing ratios and number concentrations for each category. Each process is treated explicitly and independently to establish an analytic expression for each contribution for the time-dependant microphysical equations. The scheme has been tested in the dynamical framework of a two-dimensional kinematic model, developed for the Hawaiian Rainband Project (HaRP, 1990). In this frame, the scheme has performed reasonably well compared to the observations as well as to other similar parameterization schemes, and to the spectral model DESCAM.Sensitivity tests demonstrate the great sensitivity of the scheme to the initial aerosol spectrum characteristics. Moreover, they have also shown its capability to calculate nucleation and impaction scavenging and to follow the taken up particle mass in the cloud and raindrop spectra until the deposition on the ground by the rain.Therefore, the parameterization offers a possibility of treating the evolution of the liquid phase of the cloud together with the aerosol particle scavenging. However, due to the severe limitations of a two-dimensional kinematic model, the scheme needs to be further validated in a three-dimensional dynamical model.  相似文献   

Impact of cloud dynamics on tropospheric chemistry: Advances in modeling the interactions between microphysical and chemical processes     

P. J. Grégoire  N. Chaumerliac  E. C. Nickerson 《Journal of Atmospheric Chemistry》1994,18(3):247-266

A chemical module describing the tropospheric photochemistry of ozone precursors in both gaseous and aqueous phases for a remote continental atmosphere has been developed within the framework of a two-dimensional cloud model. Dynamical, microphysical and chemical processes are fully interacting in order to study the influence of clouds on ozone chemistry and to quantify the relative importance of the different processes on the budget and evolution of 12 chemical species. Whereas the concentrations of highly soluble species are strongly affected by evaporation and sedimentation, less soluble species are affected primarily by accretion. The model reproduces previously observed chemical phenomena such as the enrichment of formic acid at the top of the cloud.  相似文献   

A numerical study of the seasonal variations for tracer redistribution by clouds over West Africa     

M. Renard  N. Chaumerliac  S. Cautenet  N. Audiffren  E. C. Nickerson 《Journal of Atmospheric Chemistry》1995,20(3):237-258

The sensitivity of the horizontal and vertical transport of an inert tracer to seasonal variability of the complex West Africa circulations is explored by means of a 2D mesoscale meteorological model including explicit microphysics and describing the cloud dynamics of these circulations. The seasonal variations of the location and spatial extent of the cloudy masses associated with the Inter Tropical Convergence Zone (ITCZ) are reproduced in a meridional cross section over West Africa. The redistribution of the inert tracer is shown to be due to the northward migration of the ITCZ from January to July and also to the enhancement of the convective activity of the ITCZ in July. The redistribution of carbon monoxide during the dry and wet seasons is discussed, highlighting the importance of the biomass burning during the dry season as a source of trace gas enrichment in the upper levels of the tropical troposphere over West Africa.  相似文献