Quantification of sediment source contributions in two paired catchments of the Brazilian Pampa using conventional and alternative fingerprinting approaches     

Mirian Lago Valente  José Miguel Reichert  Cédric Legout  Tales Tiecher  Rosane Barbosa Lopes Cavalcante  Olivier Evrard 《水文研究》2020,34(13):2965-2986

The knowledge of the contribution of sediment sources to river networks is a prerequisite to understand the impact of land use change on sediment yield. We calculated the relative contributions of sediment sources in two paired catchments, one with commercial eucalyptus plantations (0.83 km²) and the other with grassland used for livestock farming (1.10 km²), located in the Brazilian Pampa biome, using different combinations of conventional [geochemical (G), radionuclide (R) and stable isotopes and organic matter properties (S)] and alternative tracer properties [spectrocolorimetric visible-based-colour parameters (V)]. Potential sediment sources evaluated were stream channel, natural grassland and oat pasture fields in the grassland catchment, and stream channel, unpaved roads and eucalyptus plantation in the eucalyptus catchment. The results show that the best combination of tracers to discriminate the potential sources was using GSRV tracers in the grassland catchment, and using GSRV, GSV and GS tracers in the eucalyptus catchment. In all these cases, samples were 100% correctly classified in their respective groups. Considering the best tracers results (GSRV) in both catchments, the sediment source contributions estimated in the catchment with eucalyptus plantations was 63, 30 and 7% for stream channel, eucalyptus stands and unpaved roads, respectively. In the grassland catchment, the source contributions to sediment were 84, 14 and 2% for natural grassland, stream channel and oats pasture fields, respectively. The combination of these source apportionment results with the annual sediment loads monitored during a 3-year period demonstrates that commercial eucalyptus plantations supplied approximately 10 times less sediment (0.1 ton ha⁻¹ year⁻¹) than the traditional land uses in this region, that is, 1.0 ton ha⁻¹ year⁻¹ from grassland and 0.3 ton ha⁻¹ year⁻¹ from oats pasture fields. These results demonstrate the potential of combining conventional and alternative approaches to trace sediment sources originating from different land uses in this region. Furthermore, they show that well-managed forest plantations may be less sensitive to erosion than grassland used for intensive livestock farming, which should be taken into account to promote the sustainable use of land in this region of South America.  相似文献   

Impact of the LMDZ atmospheric grid configuration on the climate and sensitivity of the IPSL-CM5A coupled model   总被引：3，自引：3，他引：0  

Frédéric Hourdin  Marie-Alice Foujols  Francis Codron  Virginie Guemas  Jean-Louis Dufresne  Sandrine Bony  Sébastien Denvil  Lionel Guez  François Lott  Josefine Ghattas  Pascale Braconnot  Olivier Marti  Yann Meurdesoif  Laurent Bopp 《Climate Dynamics》2013,40(9-10):2167-2192

The IPSL-CM5A climate model was used to perform a large number of control, historical and climate change simulations in the frame of CMIP5. The refined horizontal and vertical grid of the atmospheric component, LMDZ, constitutes a major difference compared to the previous IPSL-CM4 version used for CMIP3. From imposed-SST (Sea Surface Temperature) and coupled numerical experiments, we systematically analyze the impact of the horizontal and vertical grid resolution on the simulated climate. The refinement of the horizontal grid results in a systematic reduction of major biases in the mean tropospheric structures and SST. The mid-latitude jets, located too close to the equator with the coarsest grids, move poleward. This robust feature, is accompanied by a drying at mid-latitudes and a reduction of cold biases in mid-latitudes relative to the equator. The model was also extended to the stratosphere by increasing the number of layers on the vertical from 19 to 39 (15 in the stratosphere) and adding relevant parameterizations. The 39-layer version captures the dominant modes of the stratospheric variability and exhibits stratospheric sudden warmings. Changing either the vertical or horizontal resolution modifies the global energy balance in imposed-SST simulations by typically several W/m² which translates in the coupled atmosphere-ocean simulations into a different global-mean SST. The sensitivity is of about 1.2 K per 1 W/m² when varying the horizontal grid. A re-tuning of model parameters was thus required to restore this energy balance in the imposed-SST simulations and reduce the biases in the simulated mean surface temperature and, to some extent, latitudinal SST variations in the coupled experiments for the modern climate. The tuning hardly compensates, however, for robust biases of the coupled model. Despite the wide range of grid configurations explored and their significant impact on the present-day climate, the climate sensitivity remains essentially unchanged.  相似文献   

Skill assessment of three earth system models with common marine biogeochemistry   总被引：1，自引：0，他引：1  

Roland Séférian  Laurent Bopp  Marion Gehlen  James C. Orr  Christian Ethé  Patricia Cadule  Olivier Aumont  David Salas y Mélia  Aurore Voldoire  Gurvan Madec 《Climate Dynamics》2013,40(9-10):2549-2573

We have assessed the ability of a common ocean biogeochemical model, PISCES, to match relevant modern data fields across a range of ocean circulation fields from three distinct Earth system models: IPSL-CM4-LOOP, IPSL-CM5A-LR and CNRM-CM5.1. The first of these Earth system models has contributed to the IPCC 4th assessment report, while the latter two are contributing to the ongoing IPCC 5th assessment report. These models differ with respect to their atmospheric component, ocean subgrid-scale physics and resolution. The simulated vertical distribution of biogeochemical tracers suffer from biases in ocean circulation and a poor representation of the sinking fluxes of matter. Nevertheless, differences between upper and deep ocean model skills significantly point to changes in the underlying model representations of ocean circulation. IPSL-CM5A-LR and CNRM-CM5.1 poorly represent deep-ocean circulation compared to IPSL-CM4-LOOP degrading the vertical distribution of biogeochemical tracers. However, their representations of surface wind, wind stress, mixed-layer depth and geostrophic circulations (e.g., Antarctic Circumpolar Current) have been improved compared to IPSL-CM4-LOOP. These improvements result in a better representation of large-scale structure of biogeochemical fields in the upper ocean. In particular, a deepening of 20–40 m of the summer mixed-layer depth allows to capture the 0–0.5 μgChl L^?1 concentrations class of surface chlorophyll in the Southern Ocean. Further improvements in the representation of the ocean mixed-layer and deep-ocean ventilation are needed for the next generations of models development to better simulate marine biogeochemistry. In order to better constrain ocean dynamics, we suggest that biogeochemical or passive tracer modules should be used routinely for both model development and model intercomparisons.  相似文献   

The use of a Multilayer Perceptron for detecting new human settlements from a time series of MODIS images     

B.P. Salmon  J.C. Olivier  W. Kleynhans  K.J. Wessels  F. van den Bergh  K.C. Steenkamp 《International Journal of Applied Earth Observation and Geoinformation》2011

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Volcanic and solar activity, and atmospheric circulation influences on cosmogenic Be fallout at Vostok and Concordia (Antarctica) over the last 60 years     

Mélanie Baroni  Edouard Bard  Olivier Magand 《Geochimica et cosmochimica acta》2011,75(22):7132-7145

The cosmogenic nuclide beryllium-10 (¹⁰Be), recovered from ice cores, is often used to study solar activity on long timescales. However, the ¹⁰Be signal is also influenced by factors other than the Sun. To identify and quantify various contributions to the ¹⁰Be signal, two Antarctic snow records from the Vostok and Concordia sites spanning the last 60 years were studied at a sub-annual resolution. Three factors that contribute to the ¹⁰Be signal were identified. First, a significant period of approximately 11 yr that can be associated with the modulation of ¹⁰Be production by solar activity was detected in both records. The solar imprint constitutes 20-35% of the variance within the total signal. The 11-yr ¹⁰Be snow component was attenuated by a factor of ∼0.5 and was delayed by ∼1.4 yr compared to the ¹⁰Be production expected within the polar atmosphere. The result could be interpreted as the composite response of a stratospheric ¹⁰Be reservoir with an 11-yr modulation that was attenuated and delayed (with respect to ¹⁰Be polar production) and to a tropospheric ¹⁰Be reservoir with an 11-yr modulation that was not attenuated or delayed. Then, peaks in ¹⁰Be concentrations that were ∼66% and ∼35% higher than the average concentration were observed during the stratospheric volcanic eruptions of Agung (in 1963) and Pinatubo (in 1991), respectively. In light of these new results, published ¹⁰Be ice core records could be reinterpreted because spikes in ¹⁰Be concentration appear at the time of several stratospheric events. The data indicate that stratospheric volcanic eruptions can impact ¹⁰Be transport and deposition as a result of the roles played by the sedimentation of sulfate aerosols and the formation and rapid settling of polar stratospheric clouds (PSC). Also, an interannual variability of ∼4 yr was determined in both ¹⁰Be records, corresponding to ∼26% of the variance within the signal at Vostok. As with species of marine origin (sodium), this 4-yr variability is interpreted as a tropospheric modulation. The 4-yr variability could be associated with atmospheric circulation associated with the coupled Southern Ocean ocean-atmosphere system. The results presented here, from sites within the high Antarctic plateau, open new possibilities for ice core dating over the last few centuries and for the reconstruction of past solar activity in relation to climate.  相似文献   

Age of river basins in Guadeloupe impacting chemical weathering rates and land use     

Sétareh Rad  Olivier Cerdan  Karine Rivé  Gilles Grandjean 《Applied Geochemistry》2011

The Lesser Antilles have very high chemical weathering rates, with values that can reach 1290 t/km²/a. The tropical environment induces high precipitation rates, high temperature, dense vegetation, with sharp relief and thick soils. Because of volcanic activity, frequent pyroclastic flows produce very erodible and porous materials. In addition, agriculture induces important land use changes which replace existing native forest cover with banana and sugar cane plantations. Their surface can cover as much as 40% of the total area of a river basin. The aim of this study is to identify key parameters, either natural or anthropogenic, that control chemical weathering rates. Among the combined impact of all parameters (climate, runoff, slopes, vegetation etc.), basin age seems to be the control parameter: the younger the basin, the higher the weathering rate. A correlation between the chemical weathering rate and the basin age suggests that young volcanic rocks are more easily weathered than old ones: young fresh material is easily mobilized by erosion, while for older rocks with thick soil covers, chemical rates are much lower. A combined effect between the higher erodibility and a higher climate erosivity of the younger relief could be observed. Moreover, a correlation between banana plantations and the chemical weathering rates that can be explained by an increase of infiltration, due to stem flow processes is shown here. Banana plantations also have a correlation with the basin age, older basins being more favorable terrains for cultivation.  相似文献   

Pyrite tracks assimilation of crustal sulfur in Pyrenean peridotites     

Jean-Pierre Lorand  Olivier Alard 《Mineralogy and Petrology》2011,101(1-2):115-128

Cobalt-bearing pyrite (0.5?C2.0?wt.% Co) is abnormally abundant (up to 35?vol.% of the total volume of the sulfide phase) in some eastern Pyrenean peridotite massifs, compared to pieces of subcontinental mantle studied so far for sulfides. Pyrite occurs as vermicular intergrowths inside pentlandite and/or chalcopyrite or as coarser, blocky grains in the intergranular pores of host peridotites. Those different pyrites are characterized by different platinum-group element systematics (measured by laser ablation microprobe and ICP-MS). Vermicular pyrite intergrown with pentlandite displays Os-, Ir-, Ru- and Rh-enriched chondrite normalized PGE patterns of Monosulfide solid solution (Mss). In contrast, coarse-grained intergranular (??blocky??) pyrites, are PGE-poor. Chalcophile trace elements (i.e. Zn, Pb, Ag, Au) that are not usually concentrated in mantle-derived sulfides were commonly detected. By contrast, selenium contents are generally low, yielding thus pyrite with high S/Se ratio (>10⁵), consistent with a sedimentary sulfur source. Pyrite microtextures and chalcophile trace element contents support a process of assimilation of crustal sulfur from the metamorphosed sedimentary country rocks. These latter generated highly reactive CO₂-S fluids, which were injected into structural discontinuities of the lherzolitic bodies. Sulfur has reacted at T?=?300?C550°C with pre-existing, mantle-derived, metal-rich sulfide assemblages (pentlandite-chalcopyrite). Addition of crustal sulfur did produce Mss which, on cooling, exsolved the Os-rich pyrite in addition to pentlandite. The coarse-grained pyrite types have crystallized directly from S-rich fluids.  相似文献   

CO2 geological storage: The environmental mineralogy perspective     

François Guyot  Damien Daval  Sébastien Dupraz  Isabelle Martinez  Bénédicte Ménez  Olivier Sissmann 《Comptes Rendus Geoscience》2011,343(2-3):246-259

Geological storage of carbon dioxide (CO₂) is one of the options envisaged for mitigating the environmental consequences of anthropogenic CO₂ increases in the atmosphere. The general principle is to capture carbon dioxide at the exhaust of power plants and then to inject the compressed fluid into deep geological formations. Before implementation over large scales, it is necessary to assess the efficiency of the process and its environmental consequences. The goal of this paper is to discuss some environmental mineralogy research perspectives raised by CO₂ geological storage.  相似文献   

Origin of high Zn contents in Jurassic limestone of the Jura mountain range and the Burgundy: evidence from Zn speciation and distribution     

Olivier Jacquat  Claire Rambeau  Andreas Voegelin  Natalia Efimenko  André Villard  Karl B. Föllmi  Ruben Kretzschmar 《Swiss Journal of Geoscience》2011,104(3):409-424

In order to better understand the origin and enrichment mechanisms leading to elevated Zn concentrations in Jurassic limestone of the Jura mountain range (JMR) and the Burgundy (B), we investigated four locations of Bajocian age (JMR: Lausen–Schleifenberg, Gurnigel; B: Vergisson–Davayé, Lucy-le-Bois) and two locations of Oxfordian age (JMR: Dornach, Pichoux) for their Zn distribution and speciation. Measurements of the acid-extractable and bulk Zn contents showed that Zn is stratigraphically and spatially heterogeneously distributed, in association with permeable carbonate levels. Up to 3,580 and 207 mg/kg Zn was detected in Bajocian and Oxfordian limestone, respectively, with numerous limestone samples having Zn contents above 50 mg/kg. Using X-ray absorption near edge structure spectroscopy and micro-X-ray fluorescence spectrometry, the speciation and micro-scale distribution of Zn was investigated for selected limestone samples. In Bajocian limestone sphalerite and/or Zn-substituted goethite and a minor fraction of Zn-bearing carbonates were identified. In contrast, Zn-bearing carbonates (Zn-substituted calcite and hydrozincite) were accounting for most of the total Zn in Oxfordian limestone. The micro-scale distribution of Zn for Bajocian and Oxfordian limestone was however similar with localized Zn-rich zones in the limestone cement and at the rim of oolites. The stratigraphic sporadicity and microscale heterogeneity of the Zn distribution together with the Zn speciation results point to a hydrothermal origin of Zn. Occurence of Zn-goethite is probably linked to the oxidative transformation of framboidal pyrite and hydrothermal sphalerite in contact with meteoritic waters. Difference in speciation between Bajocian limestone and Oxfordian limestone may be related to differences in rock permeability and/or to various hydrothermal events. Isotopic dating of the different mineralizations will be needed to decipher differences in Zn speciation and the precise chronology of hydrothermal episodes.  相似文献   

Oscarella balibaloi,a new sponge species (Homoscleromorpha: Plakinidae) from the Western Mediterranean Sea: cytological description,reproductive cycle and ecology     

Thierry Pérez  Julijana Ivanisevic  Maude Dubois  Laura Pedel  Olivier P. Thomas  Daria Tokina  Alexander V. Ereskovsky 《Marine Ecology》2011,32(2):174-187

A new homoscleromorph sponge species was observed for the first time in 2002 along the coast of Provence (France) and since then, several investigations have been implemented. The new homoscleromorph species is devoid of skeleton and it is thus related to the Oscarella genus. Oscarella balibaloi sp. nov. has been found in several littoral submarine caves of the Western Mediterranean Sea (France and Spain). After several years of monitoring, we show that this sponge is becoming abundant in several locations. The species has a peculiar habit, often overgrowing massive sponges, gorgonians or some erected bryozoans. Oscarella balibaloi sp. nov. is thinly encrusting, with an irregular morphology, lobate surface, and soft and very slimy consistency. Its color is white to orange. At the cytological level, this new species is characterized by three distinct types of cells with inclusions in its mesohyl: one with vacuoles and the others with paracrystalline inclusions. The reproduction pattern is very similar to other Oscarella species. We also present a specific metabolic fingerprint and compare it to that of other Mediterranean Oscarella species.  相似文献