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81.
Matteo Vacchi Giovanni De Falco Simone Simeone Monica Montefalcone Carla Morri Marco Ferrari Carlo Nike Bianchi 《地球表面变化过程与地形》2017,42(1):42-54
Here we review the multiple interactions between the endemic Mediterranean seagrass, Posidonia oceanica, and coastal geomorphologic processes as an outstanding example of biogeomorphology, taking into account recent advances in the field. Seagrass meadows are among the most important elements for the functioning of marine coastal ecosystems, and represent a major focus for research and conservation. Being considered a priority habitat, P. oceanica meadows are protected by several European Union directives and national laws. In this paper we examine: the role of sedimentary features in controlling the development of the meadows; the interplay between P. oceanica leaf litter (i.e. beached necromass) cast ashore and erosional‐depositional processes on the beaches; the interactions between meadows and nearshore hydrodynamics, and; possible linkages between geomorphological features of the seafloor and the architecture of meadows. Finally, we provide perspectives for future research on P. oceanica and other Mediterranean seagrass meadows in a biogeomorphological context with specific reference to climate change. Copyright © 2016 John Wiley & Sons, Ltd. 相似文献
82.
Lucas O. Bianchi Juan Antonio Rivera Facundo Rojas Mauro Britos Navarro Ricardo Villalba 《水文科学杂志》2017,62(4):533-545
In the Central Andes of Argentina (30–37°S), snowmelt is the main source of freshwater, an essential natural resource for ~2.2 million people in the adjacent arid lowlands. In this region, Laguna Llancanelo collects the water inputs from the Malargüe endorheic basin. Previous studies concerning the annual and intra-annual variations of this lagoon and its relationship with regional climate are rare. We obtained a monthly record for the Laguna Llancanelo area (LLA, 1984–2013) using the modified normalized difference water index derived from Landsat images. Monthly LLA ranges between 35 km2 and 411 km2 and is significantly related to variations of the Río Malargüe, the main snow-fed tributary to the lagoon. There is no long-term relationship between LLA and local rainfall, but rapid increases in LLA result from heavy rainfall around the lagoon. Conversely, rapid reductions in LLA encompass periods with both reduced discharge from the Río Malargüe and low local rainfall. The LLA integrates moisture of both Pacific (snowfall in the upper Andes) and Atlantic (lowland rainfall) origins; therefore, we propose using LLA as an indicator of regional water balance. 相似文献
83.
R. Bianchi A. Forni F. Cámara R. Oberti H. Ohashi 《Physics and Chemistry of Minerals》2007,34(8):519-527
The synthetic LiGaSi2O6 clinopyroxene is monoclinic C2/c at room-T. Its experimental electron density, ρ(r), has been derived starting from accurate room-T single-crystal diffraction data. Topological analysis confirms an intermediate ionic-covalent character for Si–O bonding,
as found by previous electron-density studies on other silicates such as diopside, coesite and stishovite. The non-bridging
Si–O bonds have more covalent character than the bridging ones. The Ga–O bonds have different bonding characters, the Ga–O2
bond being more covalent than the two Ga–O1 bonds. Li–O bonds are classified as pure closed-shell ionic interactions. Similar
to spodumene (LiAlSi2O6), Li has sixfold coordination, but the bond critical points associated to the two longest bonds are characterized by very
low electron density values. Similar to what previously found in spodumene and diopside, O···O interactions were detected
from the topological analysis of ρ(r), and indicate a cooperative interaction among the lone pairs of neighbouring oxygen atoms. In particular, this kind of interaction
has been obtained for the O1···O1 edge shared between two Ga octahedra. Integration over the atomic basins gives net charges
of −1.39(10), 2.82(10), 1.91(10) and 0.82(8) e for O (averaged), Si, Ga and Li atoms, respectively. Periodic Hartree–Fock
and DFT calculations confirm the results obtained by multipole refinement of the experimental data. Moreover, the theoretical
topological properties of the electron density distribution on the Si2O6 group are very similar to those calculated for spodumene.
Electronic supplementary material The online version of this article (doi:) contains supplementary material, which is available to authorized users. 相似文献
84.
Giancarlo Della Ventura Günther J. Redhammer Gianluca Iezzi Frank C. Hawthorne Arnaud Papin Jean-Louis Robert 《Physics and Chemistry of Minerals》2005,32(2):103-113
A series of amphiboles along the magnesioriebeckite—Na2Mg3Fe3+ 2Si8O22(OH)2– ferri-clinoholmquistite—Li2Mg3Fe3+ 2Si8O22(OH)2 - join, defined by the BLiB Na–1 exchange vector, were hydrothermally synthesized at 700°C, 0.4 GPa, NNO + 1 redox conditions. Powder XRD and SEM-EDAX showed a very high (> 90%) amphibole yield for all samples. X-ray patterns were indexed in the C2/m space group; refined cell-parameters show a linear decrease of a and as a function of chemistry. IR spectra in the OH-stretching region show four main and rather sharp bands; these are assigned to Mg and Fe2+ at M(1,3), and indicate that the obtained amphiboles depart from the nominal octahedral composition (M1,3Mg3). The IR spectra also show that there is an increasing filling-up of the A-site for increasing Na in the system (increasing solid-solution toward, arfvedsonite). Mössbauer spectra show four well-defined quadrupole doublets which are assigned to Fe3+ at M2 and to Fe2+ at M1, M3 and M4, respectively. The Fe3+/Fe2+ content derived from fitted peak areas show variable Fe3+ concentration along the series. Mössbauer spectra also show a distinct alteration of 57Fe hyperfine parameters with changing Na–Li at M4. The most evident variation is observed for the quadrupole splitting of Fe3+ at M2, which increases by 50% from ferri-clinoholmquistite to magnesio-riebeckite; this suggest that the M2 octahedron in ferri-clinoholmquistite is much closer to the ideal geometry than the M2 octahedron in magnesio-riebeckite. Mössbauer spectra show also a well-defined increase in the Fe2+ quadrupole splitting of the M1 and M3 octahedra, which is attributed to the Na–Li distribution at the B-sites. 相似文献
85.
Weiwei Wang Matthew A. Tarr Thomas S. Bianchi Erika Engelhaupt 《Aquatic Geochemistry》2000,6(3):275-292
It has recently been shown thatnitrogen contained in humic substances can be releasedas low molecular weight species through photochemicalprocesses or reactions. Nitrogen released in thismanner may then become available for biological useand chemical reactivity. This report providesadditional kinetic data for nitrogen photochemistry oforganic matter in natural waters from Louisiana andfor Suwannee River humic and fulvic acids. Naturalwater samples were fractionated into colloidal(>0.2 m, <1000 Dalton) and dissolved (>1000Dalton) fractions and the kinetics of these fractionsas well as 0.2 m filtered water samples weremeasured. For irradiations of less than 10 hours ofsimulated noon-time sun, samples showed linearproduction of ammonium and first-order fading at350 nm. Ammonium photoproduction was enhanced asmuch as three-fold by lowering pH, but linear kineticswere maintained. Light-dark cycling showed continuedrelease of ammonium immediately after irradiation,followed by uptake at longer post irradiation times.A two step mechanism was proposed to explain theobserved kinetics. Calculated net daytime release ofammonium from natural surface waters ranged from 0.33to 1.9 M h-1 in the samples studied,corresponding to a photic zone conversion rate of9–20% of the total organic nitrogen per day intoammonium. 相似文献
86.
Paolo Benettin Scott W. Bailey Andrea Rinaldo Gene E. Likens Kevin J. McGuire Gianluca Botter 《水文研究》2017,31(16):2982-2986
We introduce a new representation of coupled solute and water age dynamics at the catchment scale, which shows how the contributions of young runoff waters can be directly referenced to observed water quality patterns. The methodology stems from recent trends in hydrologic transport that acknowledge the dynamic nature of streamflow age and explores the use of water age fractions as an alternative to the mean age. The approach uses a travel time‐based transport model to compute the fractions of streamflow that are younger than some thresholds (e.g., younger than a few weeks) and compares them to observed solute concentration patterns. The method is here validated with data from the Hubbard Brook Experimental Forest during spring 2008, where we show that the presence of water younger than roughly 2 weeks, tracked using a hydrologic transport model and deuterium measurements, mimics the variation in dissolved silicon concentrations. Our approach suggests that an age–discharge relationship can be coupled to classic concentration–discharge relationship, to identify the links between transport timescales and solute concentration. Our results highlight that the younger streamflow components can be crucial for determining water quality variations and for characterizing the dominant hydrologic transport dynamics. 相似文献
87.
88.
Carmela Freda Mario Gaeta Biagio Giaccio Fabrizio Marra Danilo M. Palladino Piergiorgio Scarlato Gianluca Sottili 《Bulletin of Volcanology》2011,73(3):241-256
Generally, the intensity and magnitude of explosive volcanic activity increase in parallel with SiO2 content. Pyroclastic-flow-forming eruptions in the Colli Albani ultrapotassic volcanic district (Italy) represent the most
striking exception on a global scale, with volumes on the order of tens of cubic kilometres and K-foiditic compositions (SiO2 even <42 wt.%). Here, we reconstruct the pre-eruptive scenario and event dynamics of the ~456 ka Pozzolane Rosse (PR) eruption,
the largest mafic explosive event of the Colli Albani district. In particular, we focus on the driving mechanisms for the
unusually explosive eruption of a low-viscosity, mafic magma. Geologic, petrographic and geochemical data with mass balance
calculations, supported by experimental data for Colli Albani magma compositions, provide evidence for significant ingestion
of carbonate wall rocks by the Pozzolane Rosse K-foiditic magma. Moreover, the scattered occurrence of cored bombs in Pozzolane
Rosse pyroclastic-flow deposits records carbonate entrainment even at the eruptive time scale, as also tested quantitatively
by thermal modelling of magma–carbonate interaction and carbonate assimilation experiments. We suggest that the addition of
free CO2 from decarbonation of country rocks was the major factor controlling magma explosivity. High CO2 activity in the volatile component, coupled with magma depressurisation, produced extensive leucite crystallisation at short
time scales, resulting in a dramatic increase in magma viscosity and volatile pressurisation, which was manifested a change
of eruptive dynamics from early effusion to the Pozzolane Rosse's highly explosive eruption climax. 相似文献
89.
Thomas S. Bianchi Laura A. Wysocki Kathryn M. Schreiner Timothy R. Filley D. Reide Corbett Alexander S. Kolker 《Aquatic Geochemistry》2011,17(4-5):431-456
High sedimentation rates along river-dominated margins make these systems important repositories for organic carbon derived from both allochthonous and autochthonous sources. Using elemental carbon/nitrogen ratios, molecular biomarker (lignin phenol), and stable carbon isotopic (bulk and compound-specific) analyses, this study examined the sources of organic carbon to the Louisiana shelf within one of the primary dispersive pathways of the Mississippi River. Surface sediment samples were collected from stations across the inner, mid, and outer Louisiana shelf, within the Mississippi River plume region, during two cruises in the spring and fall of 2000. Lignin biomarker data showed spatial patterns in terrestrial source plant materials within the river plume, such that sediments near the mouth of the Mississippi River were comparatively less degraded and richer in C4 plant carbon than those found at mid-depth regions of the shelf. A molecular and stable isotope-based mixing model defining riverine, marsh, and marine organic carbon suggested that the highest organic carbon inputs to the shelf in spring were from marine sources (55?C61% marine organic carbon), while riverine organic carbon was the highest (63%) in fall, likely due to lower inputs of marine organic carbon at this time compared with the spring season. This model also indicated that marsh inputs, ranging from 19 to 34% and 3?C15% of the organic carbon in spring and fall, respectively, were significantly more important sources of organic carbon on the inner Louisiana shelf than previously suggested. Finally, we propose that the decomposition of terrestrial-derived organic carbon (from the river and local wetlands sources) in mobile muds may serve as a largely unexplored additional source of oxygen-consuming organic carbon in hypoxic bottom waters of the Louisiana shelf. 相似文献
90.
Shuiwang Duan Rainer Amon Thomas S. Bianchi Peter H. Santschi 《Estuaries and Coasts》2011,34(1):78-89
Soluble reactive phosphorus (SRP) has recently been shown to be one of the limiting nutrients for the growth of phytoplankton
in the northern Gulf of Mexico. We show here that during the past decade, SRP concentrations in the lower reaches of North
America's largest river, the Mississippi River, were highest in summer and lowest in winter and positively correlated with
water temperature. Upstream data showed this coupling to increase in a downstream trend in the Mississippi main stem. Water
quality data analysis and phosphorus mass balances were conducted to examine the controls of this relationship. The results
showed that the positive SRP–temperature correlation in the Mississippi River system was largely a result of gradual dilution
of SRP-enriched upper Mississippi River waters, which contributed most to the Mississippi River during summer, by SRP-depleted
waters from the Ohio and other tributaries. Particle buffering and organic matter mineralization might play a role in the
observed SRP–temperature relationship, but their importance relative to tributary effects is not quantified. Future work on
the seasonal dynamics of SRP in large river systems needs to consider the effects of both tributary dilution and in situ processes. 相似文献