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11.
Neil Cory Ishi Buffam Hjalmar Laudon Louise Bjrkvald Carl-Magnus Mrth Stephan Khler Kevin Bishop 《Applied Geochemistry》2009,24(9):1677-1685
The adverse impacts of the inorganic labile monomeric Al (Ali) fraction on aquatic organisms have meant that Al (Altot) determination and even speciation has become a routine part of environmental monitoring and assessment. However, if samples are not filtered prior to analysis then particulate Al (Altot(p)) could influence the determination of Altot, and therefore the determination of the more toxicologically important (Ali), both when it is measured analytically or modelled from Altot. This paper shows that the Al/DOC ratio in unfiltered samples can identify the Altot(p) fraction, and thus improve the speciation of Ali. These findings are based on data from a study in a 67 km2 catchment in northern Sweden during the snowmelt-driven spring flood of two consecutive years. Filtered and unfiltered samples were studied to determine the spatial and temporal patterns in Altot(p). The concentrations of Altot(p) were greatest in larger downstream sites where significant silt deposits are located. The sites with no silt in their drainage area showed a mean difference between filtered (Altot(f)) and unfiltered (Altot(uf)) samples of 6%, while sites with silt deposits had a mean difference of 65%. The difference between filtered and unfiltered samples was greatest at peak flow. Spikes in Altot(p) did not behave consistently during fractionation with a cation exchange column, resulting in increases in either measured Ali(f) or non-labile monomeric Al (Alo(f)). Altot(p) spikes were associated with sharp increases in the Al:DOC ratio. The baseflow Al:DOC ratio could be used to model filtered Altot from DOC with a Spearman rho of 0.75. 相似文献
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Aqua Incognita: the unknown headwaters 总被引：1，自引：1，他引：0
K. Bishop I. Buffam M. Erlandsson J. Fölster H. Laudon J. Seibert J. Temnerud 《水文研究》2008,22(8):1239-1242
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Bluhm Hartmut Borowski Christian Ahnert Ahmed Vopel Kay Schriever Gerd Thiel Hjalmar 《Ocean Dynamics》1999,51(10):149-152
Ocean Dynamics - Das Ökosystem der Tiefsee wird zunehmend durch industrielle Eingriffe beeinflusst. Über die Auswirkungen dieser Aktivitäten auf das Benthos wurden bisher nur... 相似文献
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Abstract. Sediment parameters (grain size, organic content, chloroplastic pigments, Adenylates, Potential hydrolytic activity and electron transport system activity) and benthic biota were studied in methane seep area south-west of the Crimean Peninsula in the Black Sea over a depth range from 60 to 260m. A control transect with similar depths was performed in an adjacent nonseep area. Methane seepage in this region occurs from 35 to ˜ 85m depth, passing the oxic anoxic interface zone at 130 to 180m. The methane seep areas were characterized by abundant carbonate precipitates which occurred in various shapes from small, flat structures to tall chimneys with increasing anoxia. The carbonates were associated with distinct bacterial mats. Most of the measured biochemical parameters in the sediment were quite similar in the seep and nonseep areas. The content of organic matter was higher and grain size was more uniform in the nonseep areas. However, the seep areas were charaterized by highter proportions of the larger fauna (size classes 0.5–1 mm and ≥ 1mm) as well as increased total numbers of benthic fauna in the suboxic and upper anoxic zone. The animals did not show any seep-specific adaptations. In addition to methane seepage, highly variable hydrochemical and sedimentary conditions on the lower shelf and upper slope may also play an important role in structuring the composition and distribution of the benthic fauna. 相似文献
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Nearby catchments in the same landscape are often assumed to have similar specific discharge (runoff per unit catchment area). Five years of streamflow from 14 nested catchments in a 68 km2 landscape was used to test this assumption, with the hypothesis that the spatial variability in specific discharge is smaller than the uncertainties in the measurement. The median spatial variability of specific discharge, defined as subcatchment deviation from the catchment outlet, was 33% at the daily scale. This declined to 24% at a monthly scale and 19% at an annual scale. These specific discharge differences are on the same order of magnitude as predicted for major land‐use conversions or a century of climate change. Spatial variability remained when considering uncertainties in specific discharge, and systematic seasonal patterns in specific discharge variation further provide confidence that these differences are more than just errors in the analysis of catchment area, rainfall variability or gauging. Assuming similar specific discharge in nearby catchments can thus lead to spurious conclusions about the effects of disturbance on hydrological and biogeochemical processes. Copyright © 2016 John Wiley & Sons, Ltd. 相似文献
16.
Sean K. Carey Doerthe Tetzlaff Jan Seibert Chris Soulsby Jim Buttle Hjalmar Laudon Jeff McDonnell Kevin McGuire Daniel Caissie Jamie Shanley Mike Kennedy Kevin Devito John W. Pomeroy 《水文研究》2010,24(24):3591-3602
The higher mid‐latitudes of the Northern Hemisphere are particularly sensitive to climate change as small differences in temperature determine frozen ground status, precipitation phase, and the magnitude and timing of snow accumulation and melt. An international inter‐catchment comparison program, North‐Watch, seeks to improve our understanding of the sensitivity of northern catchments to climate change by examining their hydrological and biogeochemical responses. The catchments are located in Sweden (Krycklan), Scotland (Mharcaidh, Girnock and Strontian), the United States (Sleepers River, Hubbard Brook and HJ Andrews) and Canada (Catamaran, Dorset and Wolf Creek). This briefing presents the initial stage of the North‐Watch program, which focuses on how these catchments collect, store and release water and identify ‘types’ of hydro‐climatic catchment response. At most sites, a 10‐year data of daily precipitation, discharge and temperature were compiled and evaporation and storage were calculated. Inter‐annual and seasonal patterns of hydrological processes were assessed via normalized fluxes and standard flow metrics. At the annual‐scale, relations between temperature, precipitation and discharge were compared, highlighting the role of seasonality, wetness and snow/frozen ground. The seasonal pattern and synchronicity of fluxes at the monthly scale provided insight into system memory and the role of storage. We identified types of catchments that rapidly translate precipitation into runoff and others that more readily store water for delayed release. Synchronicity and variance of rainfall–runoff patterns were characterized by the coefficient of variation (cv) of monthly fluxes and correlation coefficients. Principal component analysis (PCA) revealed clustering among like catchments in terms of functioning, largely controlled by two components that (i) reflect temperature and precipitation gradients and the correlation of monthly precipitation and discharge and (ii) the seasonality of precipitation and storage. By advancing the ecological concepts of resistance and resilience for catchment functioning, results provided a conceptual framework for understanding susceptibility to hydrological change across northern catchments. Copyright © 2010 John Wiley & Sons, Ltd. 相似文献
17.
Marcus Nathanson Jason W. Kean Thomas J. Grabs Jan Seibert Hjalmar Laudon Steve W. Lyon 《水文研究》2012,26(9):1427-1434
Accurate stream discharge measurements are important for many hydrological studies. In remote locations, however, it is often difficult to obtain stream flow information because of the difficulty in making the discharge measurements necessary to define stage‐discharge relationships (rating curves). This study investigates the feasibility of defining rating curves by using a fluid mechanics‐based model constrained with topographic data from an airborne LiDAR scanning. The study was carried out for an 8m‐wide channel in the boreal landscape of northern Sweden. LiDAR data were used to define channel geometry above a low flow water surface along the 90‐m surveyed reach. The channel topography below the water surface was estimated using the simple assumption of a flat streambed. The roughness for the modelled reach was back calculated from a single measurment of discharge. The topographic and roughness information was then used to model a rating curve. To isolate the potential influence of the flat bed assumption, a ‘hybrid model’ rating curve was developed on the basis of data combined from the LiDAR scan and a detailed ground survey. Whereas this hybrid model rating curve was in agreement with the direct measurements of discharge, the LiDAR model rating curve was equally in agreement with the medium and high flow measurements based on confidence intervals calculated from the direct measurements. The discrepancy between the LiDAR model rating curve and the low flow measurements was likely due to reduced roughness associated with unresolved submerged bed topography. Scanning during periods of low flow can help minimize this deficiency. These results suggest that combined ground surveys and LiDAR scans or multifrequency LiDAR scans that see ‘below’ the water surface (bathymetric LiDAR) could be useful in generating data needed to run such a fluid mechanics‐based model. This opens a realm of possibility to remotely sense and monitor stream flows in channels in remote locations. Copyright © 2012 John Wiley & Sons, Ltd. 相似文献
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Storage,mixing, and fluxes of water in the critical zone across northern environments inferred by stable isotopes of soil water 
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下载免费PDF全文 Matthias Sprenger Doerthe Tetzlaff Jim Buttle Sean K. Carey James P. McNamara Hjalmar Laudon Nadine J. Shatilla Chris Soulsby 《水文研究》2018,32(12):1720-1737
Quantifying soil water storage, mixing, and release via recharge, transpiration, and evaporation is essential for a better understanding of critical zone processes. Here, we integrate stable isotope (2H and 18O of soil water, precipitation, and groundwater) and hydrometric (soil moisture) data from 5 long‐term experimental catchments along a hydroclimatic gradient across northern latitudes: Dry Creek (USA), Bruntland Burn (Scotland), Dorset (Canada), Krycklan (Sweden), and Wolf Creek (Canada). Within each catchment, 6 to 11 isotope sampling campaigns occurred at 2 to 4 sampling locations over at least 1 year. Analysis for 2H and 18O in the bulk pore water was done for >2,500 soil samples either by cryogenic extraction (Dry Creek) or by direct equilibration (other sites). The results showed a similar general pattern that soil water isotope variability reflected the seasonality of the precipitation input signal. However, pronounced differences among sampling locations occurred regarding the isotopic fractionation due to evaporation. We found that antecedent precipitation volumes mainly governed the fractionation signal, temperature and evaporation rates were of secondary importance, and soil moisture played only a minor role in the variability of soil water evaporation fractionation across the hydroclimatic gradient. We further observed that soil waters beneath conifer trees were more fractionated than beneath heather shrubs or red oak trees, indicating higher soil evaporation rates in coniferous forests. Sampling locations closer to streams were more damped and depleted in their stable isotopic composition than hillslope sites, revealing increased subsurface mixing towards the saturated zone and a preferential recharge of winter precipitation. Bulk soil waters generally comprised a high share of waters older than 14 days, which indicates that the water in soil pores are usually not fully replaced by recent infiltration events. The presented stable isotope data of soil water were, thus, a useful tool to track the spatial variability of water fluxes within and from the critical zone. Such data provide invaluable information to improve the representation of critical zone processes in spatially distributed hydrological models. 相似文献
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Stability of the time‐domain analysis method including a frequency‐dependent soil–foundation system 下载免费PDF全文
下载免费PDF全文 A number of methods have been proposed that utilize the time‐domain transformations of frequency‐dependent dynamic impedance functions to perform a time‐history analysis. Though these methods have been available in literature for a number of years, the methods exhibit stability issues depending on how the model parameters are calibrated. In this study, a novel method is proposed with which the stability of a numerical integration scheme combined with time‐domain representation of a frequency‐dependent dynamic impedance function can be evaluated. The method is verified with three independent recursive parameter models. The proposed method is expected to be a useful tool in evaluating the potential stability issue of a time‐domain analysis before running a full‐fledged nonlinear time‐domain analysis of a soil–structure system in which the dynamic impedance of a soil–foundation system is represented with a recursive parameter model. Copyright © 2015 John Wiley & Sons, Ltd. 相似文献