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61.
Dominique Bonnin Georges Calas Hélène Suquet Henri Pezerat 《Physics and Chemistry of Minerals》1985,12(1):55-64
New data on the structure of Garfield nontronite have been produced by the use of different spectroscopic techniques: Mössbauer spectroscopy, optical spectroscopy, X-ray absorption edges and EXAFS and NMR. The tetrahedral iron content is found to be no higher than 1 percent. All iron atoms belong to the octahedral sheet excluding the possibility of the presence of non crystallized phases. Some ambiguities remain about the coherence of the octahedral sheet because of the presence of two doublets in the Mössbauer spectrum and at least two lineshapes in NMR spectra of OH which correspond to different environments. 相似文献
62.
63.
A statistical examination of isotopic distributions for MORB from various ocean ridges leads to the “blob cluster model”, in which the oceanic crust accreting at ridges results from the mixing of two components within the ascending mantle. These are (1) upper mantle material and (2) discrete rising blobs of more radiogenic material. The blobs are fractionated to a variable degree and are distributed in the upper mantle circulation in a manner that is related to the spreading rate.(1) Themean values of the isotopic distributions allow us to calculate the probabilities of the two types of material within the mantle. The results show that theproportion of asthenospheric material in the mixtureincreases with the spreading rate, in agreement with the hypothesis of blob dilution within the upper mantle convection.Mass fluxes can be estimated for the rising blobs from these probabilities, which depend on the respective concentrations in the sources of the two types of material. If the blobs originate in the lower mantle, this flux estimation would suggest that a significant part of the lower mantle has been injected into the upper mantle during earth history.(2) Thestandard deviations of the distributions depend on the “efficiency” of the mixing process:the more imbricated are the asthenospheric and blob materials in the mixture,the smaller is theisotopic spread. This efficiency parameter is shown to increase with the spreading rate, as already suggested by previous comparisons between the East Pacific Rise and the Mid-Atlantic Ridge. Moreover, this feature may also be correlated with other data such as ridge bathymetric variations. 相似文献
64.
J Jouzel R Vaikmae J R Petit M Martin Y Duclos M Stievenard C Lorius M Toots M A Mélières L H Burckle N I Barkov V M Kotlyakov 《Climate Dynamics》1995,11(3):151-161
The two-step character of the last deglaciation is well recognized in Western Europe, in Greenland and in the North Atlantic. For example, in Greenland, a gradual temperature decrease started at the Bölling (B) around 14.5 ky BP, spanned through the Alleröd (A) and was followed by the cold Younger Dryas (YD) event which terminated abruptly around 11.5 ky BP. Recent results suggest that this BA/YD sequence may have extended throughout all the Northern Hemisphere but the evidence of a late transition cooling is still poor for the Southern Hemisphere. Here we present a detailed isotopic record analyzed in a new ice core drilled at Dome B in East Antarctica that fully demonstrates the existence of an Antarctic cold reversal (ACR). These results suggest that the two-step shape of the last deglaciation has a worldwide character but they also point to noticeable interhemispheric differences. Thus, the coldest part of the ACR, which shows a temperature drop about three times weaker than that recorded during the YD in Greenland, may have preceded the YD. Antarctica did not experienced abrupt changes and the two warming periods started there before they started in Greenland. The links between Southern and Northern Hemisphere climates throughout this period are discussed in the light of additional information derived from the Antarctic dust record. 相似文献
65.
Hélène Dupuis Alain Weill Kristina Katsaros Peter K. Taylor 《Annales Geophysicae》1995,13(10):1065-1074
Heat flux estimates obtained using the inertial dissipation method, and the profile method applied to radiosonde soundings, are assessed with emphasis on the parameterization of the roughness lengths for temperature and specific humidity. Results from the inertial dissipation method show a decrease of the temperature and humidity roughness lengths for increasing neutral wind speed, in agreement with previous studies. The sensible heat flux estimates were obtained using the temperature estimated from the speed of sound determined by a sonic anemometer. This method seems very attractive for estimating heat fluxes over the ocean. However allowance must be made in the inertial dissipation method for non-neutral stratification. The SOFIA/ASTEX and SEMAPHORE results show that, in unstable stratification, a term due to the transport terms in the turbulent kinetic energy budget, has to be included in order to determine the friction velocity with better accuracy. Using the profile method with radiosonde data, the roughness length values showed large scatter. A reliable estimate of the temperature roughness length could not be obtained. The humidity roughness length values were compatible with those found using the inertial dissipation method. 相似文献
66.
67.
Since Nb and Zr are only little fractionated during magmatic processes, the 92Nb-92Zr relative chronometer has the potential of dating the formation of the planetary bodies through their differentiation. Thus, we have analyzed the isotopic composition of zirconium in lunar, meteoritic and old and recent terrestrial samples.No isotopic variation has been found. However, the ratio of 3.8 Ga. old zircons from the Isua acid conglomerate is on the lower limit of the range of the standard measurements. If considered an anomaly, it would correspond to a +1.5 × 10?492Zr relative deficiency or to a 3.0 × 10?494Zr relative excess.Our data constrain the isotopic ratio at the time of formation of the solar system to be less than 0.007, so that the maximum sensitivity of the 92Nb-92Zr relative chronometer for the formation of planetary bodies is around 107 a. A discussion of some possible nuclear reactions indicates that zirconium isotopic variations in zircons are not easily produced, and that the 92Nb and 94Nb natural activities (Apt et al., 1974) cannot be explained by any single one of the processes proposed so far. 相似文献
68.
While the chemical structure of the earth's mantle is probably rather complex, multi-box models have been used as a first approximation to evaluate this structure. Most commonly, a three-box model is used, involving the continental crust, the upper mantle and the lower mantle. The depleted upper mantle and the continental crust are assumed to represe1nt complementary reservoirs, related by crust formation processes occurring during geologic history.Here we investigate the Rb/Sr and Sm/Nd isotopic systematics of several three-box models, using mass balance equations and the definition of the mean age of the reservoirs. The geochemical uniqueness of the models, chosen from a large family of possible models, is evaluated from elementary graph theory, and these models are then solved using a total inversion approach. This paper (Part I) describes the methodology of the procedure; the companion paper (Part II) discusses the application of this approach to multi-box mantle models. 相似文献
69.
Angela Marinoni Paolo Laj Pierre Alexandre Deveau Federica Marino Grazia Ghermandi Fabien Aulagnier Hlne Cachier 《Atmospheric Research》2005,74(1-4):565-580
The physical and chemical properties of aerosol particles were investigated at Plan d'Aups, one of the ESCOMPTE sites located in the St. Baume mountain area (700 m a.s.l.), 50 km east of Marseilles (France). The site is ideally located for assessing the vertical and horizontal extent of the pollution plume from the Marseilles–Berre area.Our study showed that polluted air masses from the Marseilles–Berre area are advected to Plan d'Aups in the early afternoon. Average daily concentration of particles reaches up to 40 μg m−3 while 1-h average particle number concentration is greater than 30,000 cm−3. Most of the particle mass is composed of SO42− and organic carbon (OC). The chemical properties of the particles revealed that an additional source, possibly from the industrial area of Gardanne, contributes to the aerosol mass. This last source is characterised by significant emissions of elements, such as Zn, V, Al and Si.In addition to transport, we found that gas-to-particle conversion takes place at the interface between the free troposphere and the boundary layer. We estimated that on average, 30% of the particle number is accounted for by direct nucleation. This is potentially a major aerosol source to the free troposphere. 相似文献
70.
Laurent Millet Boris Vannière Valérie Verneaux Michel Magny Jean Robert Disnar Fatima Laggoun-Défarge Anne Véronique Walter-Simonnet Gilles Bossuet Elena Ortu Jacques-Louis de Beaulieu 《Journal of Paleolimnology》2007,38(4):525-539
This study focuses on the response of lacustrine littoral chironomid communities to late glacial changes in limnological,
environmental and climate conditions in the Mediterranean context. Late glacial chironomid (Diptera: Chironomidae) assemblages,
organic petrography and geochemistry were analysed in a sediment core from the littoral zone of Lago dell’Accesa (Tuscany,
Italy), where the lake-level fluctuations and the vegetation history have been previously reconstructed. Comparison of the
chironomid stratigraphy to other proxies (pollen assemblages, organic petrography and geochemistry, lake-level) and regional
climate reconstruction suggested the predominant influence of lake-level changes on the littoral chironomid fauna. The main
lowering events that occurred during the Oldest and the Younger Dryas were followed by higher proportions of taxa typical
of littoral habitats. A complementary study of organic matter suggested the indirect impact of lake-level on the chironomids
through changes in humic status and habitat characteristics, such as the type of substrate and aquatic macrophyte development.
Several chironomid taxa, such as Glyptotendipes, Microtendipes and Cricotopus type patens, were identified as possible indicators of low lake-level in the late glacial records. Nevertheless, this study suggested
that parallel analyses of organic matter and chironomid assemblages may be needed to circumvent misinterpretation of littoral
chironomid assemblage stratigraphy. There was a weak response of the chironomid assemblages to small lake-level lowerings
that corresponded to the Older Dryas and Preboreal oscillations. A higher level of determination, e.g. to the species group
level, may be necessary to increase the sensibility of the indicators to lake-level changes. 相似文献